{"id":204404,"date":"2020-07-10T12:00:33","date_gmt":"2020-07-10T04:00:33","guid":{"rendered":"\/\/m.iemloyee.com\/?p=204404"},"modified":"2020-07-10T09:41:18","modified_gmt":"2020-07-10T01:41:18","slug":"%e3%80%90%e5%b7%b2%e6%a0%a1%e7%a8%bf%e3%80%91%e5%b1%b1%e4%b8%9c%e5%a4%a7%e5%ad%a6nat-commun-%ef%bc%9a%e7%94%a8%e4%ba%8e%e5%85%89%e7%94%b5%e5%8c%96%e5%ad%a6%e6%b0%b4%e5%88%86%e8%a7%a3%e7%9a%84","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=204404","title":{"rendered":"\u5c71\u4e1c\u5927\u5b66Nat. Commun.\uff1a\u7528\u4e8e\u5149\u7535\u5316\u5b66\u6c34\u5206\u89e3\u7684\u9ad8\u6d3b\u6027\u7f3a\u9677\u578b\u4e09\u5143\u786b\u5316\u7269\u5149\u9633\u6781"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u6709\u6548\u5229\u7528\u592a\u9633\u80fd\u53ef\u4ee5\u63d0\u4f9b\u4e00\u6761\u53ef\u518d\u751f\u7684\u9014\u5f84\uff0c\u4ee5\u7f13\u89e3\u56e0\u5316\u77f3\u71c3\u6599\u6d88\u8017\u91cf\u589e\u52a0\u800c\u9020\u6210\u7684\u80fd\u6e90\u548c\u73af\u5883\u95ee\u9898\u3002\u9664\u4e86\u5c06\u592a\u9633\u80fd\u8f6c\u5316\u4e3a\u7535\u80fd\u7684\u5149\u4f0f\uff08PV\uff09\u4e4b\u5916\uff0c\u5149\u7535\u5b50\u5316\u5b66\uff08PEC\uff09\u7684\u6c34\u5206\u89e3\u88ab\u8ba4\u4e3a\u662f\u53e6\u4e00\u79cd\u6709\u524d\u9014\u7684\u7b56\u7565\u3002\u4e3a\u4e86\u5728\u5b9e\u7528\u7684PEC\u7535\u6c60\u4e2d\u5b9e\u73b0\u8f83\u9ad8\u7684\u592a\u9633\u80fd\u5230\u6c22\u6c14\uff08STH\uff09\u7684\u8f6c\u5316\u6548\u7387\uff0c\u8003\u8651\u5230\u5149\u9633\u6781\u8868\u9762\u6c34\u6c27\u5316\u7684\u7f13\u6162\u3001\u591a\u6b65\u3001\u8d28\u5b50\u8026\u5408\u7535\u5b50\u8f6c\u79fb\u52a8\u529b\u5b66\uff0c\u7535\u6781\u6750\u6599\u7684\u9009\u62e9\uff0c\u5c24\u5176\u662f\u5149\u9633\u6781\u7684\u9009\u62e9\u975e\u5e38\u91cd\u8981\u3002\u5230\u76ee\u524d\u4e3a\u6b62\uff0c\u4e00\u4e9b\u6700\u6709\u524d\u666f\u7684\u534a\u5bfc\u4f53\u88ab\u7528\u4f5c\u5149\u9633\u6781\uff0c\u5305\u62ec\u03b1-Fe2<\/sub>O3<\/sub>\u3001BiVO4<\/sub>\u3001Ta3<\/sub>N5<\/sub>\uff08TaON\uff09\u548cTiO2<\/sub>\u3002\u7136\u800c\uff0c\u8fc4\u4eca\u4e3a\u6b62\u8fd8\u6ca1\u6709\u4e00\u79cd\u534a\u5bfc\u4f53\u80fd\u5b8c\u5168\u6ee1\u8db3\u5b9e\u9645\u5e94\u7528\u7684\u6240\u6709\u4e25\u683c\u8981\u6c42\uff0c\u5305\u62ec\u9ad8\u7684STH\u6548\u7387\u3001\u5728\u6c34\u7cfb\u7535\u89e3\u8d28\u4e2d\u7684\u7a33\u5b9a\u6027\u4ee5\u53ca\u53ef\u89c4\u6a21\u5316\u5236\u9020\u7684\u4f4e\u6210\u672c\uff0c\u8fd9\u4f7f\u5f97\u8bbe\u8ba1\u51fa\u4ee4\u4eba\u6ee1\u610f\u7684\u5149\u9633\u6781\u6750\u6599\u4ecd\u7136\u662f\u4e00\u4e2a\u6311\u6218\u3002\u9664\u4e86\u5728\u76ee\u524d\u7684\u5149\u9633\u6781\u6750\u6599\u4e0a\u4e0b\u529f\u592b\u5916\uff0c\u63a2\u7d22\u65b0\u578b\u534a\u5bfc\u4f53\u5e76\u7528\u4f5c\u5149\u9633\u6781\u6216\u8bb8\u80fd\u63d0\u4f9b\u4e00\u6761\u65b0\u7684\u8def\u7ebf\u3002\u6700\u7406\u60f3\u7684\u4e32\u8054PEC\u7535\u6c60\u662f\u7531\u5e26\u9699\u7ea62.0eV\u7684\u5149\u9633\u6781\u548c\u5e26\u9699\u7ea61.2eV\u7684\u5149\u9634\u6781\u7ec4\u6210\uff0c\u4ee5\u5b9e\u73b0\u6700\u9ad8\u7684STH\u6548\u7387\u548c\u65e0\u8f85\u52a9\u6c34\u5206\u89e3\u3002\u56e0\u6b64\uff0c\u4ece\u7406\u8bba\u4e0a\u8bb2\uff0c\u62e5\u6709\u9002\u5f53\u5e26\u9699\u548c\u80fd\u5e26\u4f4d\u7f6e\u7684\u534a\u5bfc\u4f53\u5728\u7406\u8bba\u4e0a\u5177\u6709\u4f5c\u4e3a\u5149\u7535\u9633\u6781\u7684\u6f5c\u529b\u3002\u5176\u4e2d\uff0c\u91d1\u5c5e\u786b\u5316\u7269\u7531\u4e8e\u5176\u5408\u9002\u7684\u5e26\u9699\u3001\u66b4\u9732\u7684\u6d3b\u6027\u4f4d\u70b9\u3001\u591a\u6837\u4e14\u53ef\u8c03\u7684\u5316\u5b66\u7ed3\u6784\u7b49\u7279\u70b9\uff0c\u4e00\u76f4\u662f\u4eba\u4eec\u7814\u7a76\u7684\u70ed\u70b9\uff0c\u5c24\u5176\u662f\u5728\u5149\u50ac\u5316\u65b9\u9762\u3002\u4f46\u662f\uff0c\u9664\u4e86\u5149\u5316\u5b66\u5149\u8150\u8680\u7684\u56e0\u7d20\uff08\u901a\u8fc7\u4f7f\u7528\u727a\u7272\u5242\u6216\u949d\u5316\u5c42\u7684\u8868\u9762\u4fee\u9970\u53ef\u4ee5\u5927\u5927\u6291\u5236\uff09\u5916\uff0c\u76f4\u63a5\u7528\u4f5c\u5149\u9633\u6781\u7684\u91d1\u5c5e\u786b\u5316\u7269\u901a\u5e38\u663e\u793a\u51fa\u8f83\u4f4e\u7684\u5149\u81f4\u7535\u5b50-\u7a7a\u7a74\u5206\u79bb\u6548\u7387\u548c\u7f13\u6162\u7684\u8868\u9762\u6c34\u6c27\u5316\u52a8\u529b\u5b66\uff0c\u8fd9\u9650\u5236\u4e86\u91d1\u5c5e\u786b\u5316\u7269\u57fa\u5149\u9633\u6781\u7684\u5e94\u7528\u3002\u91d1\u5c5e\u786b\u5316\u7269\u4e2d\u7684\u7f3a\u9677\uff0c\u7279\u522b\u662f\u5f15\u5165\u786b\u7a7a\u4f4d\uff0c\u88ab\u8bc1\u660e\u662f\u63d0\u9ad8\u5149\u50ac\u5316\u548cPEC\u6027\u80fd\u7684\u6709\u6548\u7b56\u7565\u3002\u786b\u7a7a\u4f4d\u5f15\u5165\u7684\u9677\u9631\u6001\u53ef\u4ee5\u4f5c\u4e3a\u6355\u83b7\u4e2d\u5fc3\uff0c\u4f7f\u8f7d\u6d41\u5b50\u5206\u79bb\u3002\u6b64\u5916\uff0c\u5f15\u5165\u786b\u7a7a\u4f4d\u540e\uff0c\u91d1\u5c5e\u786b\u5316\u7269\u7684\u7535\u8377\u5bc6\u5ea6\u4e5f\u53ef\u4ee5\u663e\u8457\u63d0\u9ad8\uff0c\u4ece\u800c\u7f29\u77ed\u8017\u5c3d\u5bbd\u5ea6\uff0c\u589e\u5f3a\u5149\u7535\u9633\u6781\/\u7535\u89e3\u8d28\u754c\u9762\u80fd\u5e26\u5f2f\u66f2\u3002\u6b64\u5916\uff0c\u6700\u8fd1\u7684\u7814\u7a76\u8868\u660e\uff0c\u5f15\u5165\u786b\u7a7a\u4f4d\u540e\uff0c\u76f8\u90bb\u7684\u539f\u5b50\u53d8\u6210\u4e86\u6790\u6c27\u53cd\u5e94\uff08OER\uff09\u7684\u6d3b\u6027\u4f4d\u70b9\uff0c\u4fc3\u8fdb\u8868\u9762\u6c34\u7684\u6c27\u5316\u52a8\u529b\u5b66\u3002\u57fa\u4e8e\u4ee5\u4e0a\u539f\u56e0\uff0c\u56e2\u961f\u8ba4\u4e3a\u5728\u91d1\u5c5e\u786b\u5316\u7269\u57fa\u5149\u9633\u6781\u4e2d\u5f15\u5165\u786b\u7a7a\u4f4d\u4e5f\u662f\u63d0\u9ad8\u5176PEC\u6027\u80fd\u7684\u6709\u6548\u7b56\u7565\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5c71\u4e1c\u5927\u5b66\u590f\u7389\u56fd\u8001\u5e08<\/b><\/strong>\u3001\u9648\u4ee3\u8363\u6559\u6388<\/b><\/strong>\uff08<\/b><\/strong>\u5171\u540c<\/b><\/strong>\u901a\u8baf\u4f5c\u8005\uff09<\/b><\/strong>\u7b49\u4eba\u5f00\u53d1\u4e86\u4e00\u79cd\u7f3a\u9677\u578b\u7684\u4e09\u5143\u91d1\u5c5e\u786b\u5316\u7269\uff08CdIn2<\/sub>S4<\/sub>\uff09\u5149\u7535\u9633\u6781\uff0c\u901a\u8fc7\u5f15\u5165\u8868\u9762\u786b\u7a7a\u4f4d\u6765\u663e\u7740\u63d0\u9ad8\u4e86\u5176PEC\u6027\u80fd\uff0c\u5728\u6a21\u62df\u592a\u9633\u5149\uff0c1.23 V vs. RHE\u504f\u538b\u4e0b\u7684\u5149\u7535\u6d41\u5bc6\u5ea6\u4e3a5.73 mA cm-2<\/sup>\uff0c\u57280.477 V vs. RHE\u7684\u5149\u7535\u8f6c\u6362\u6548\u7387\u4e3a2.49%\u3002\u5b9e\u9a8c\u8868\u5f81\u548c\u7406\u8bba\u8ba1\u7b97\u7a81\u51fa\u4e86\u8868\u9762\u786b\u7a7a\u4f4d\u5bf9\u754c\u9762\u7535\u8377\u5206\u79bb\u548c\u8f6c\u79fb\u52a8\u529b\u5b66\u7684\u589e\u5f3a\u4f5c\u7528\uff0c\u4e5f\u8bc1\u660e\u4e86\u5f15\u5165\u8868\u9762\u786b\u7a7a\u4f4d\u540e\uff0c\u8868\u9762\u6001\u5206\u5e03\u53d7\u5230\u6291\u5236\uff0c\u4e3a\u8c03\u8282\u534a\u5bfc\u4f53\/\u7535\u89e3\u8d28\u754c\u9762\u7535\u4f4d\u63d0\u4f9b\u4e86\u4e00\u79cd\u9014\u5f84\u3002\u8fd9\u9879\u5de5\u4f5c\u53ef\u80fd\u5bf9\u5f00\u53d1\u786b\u5316\u7269\u57fa\u5149\u7535\u9633\u6781\u6709\u91cd\u8981\u7684\u542f\u53d1\u4f5c\u7528\u3002\u8be5\u6210\u679c\u4ee5\u9898\u4e3a\u201c<\/b><\/strong>Highly active deficient ternary sulfide photoanode for photoelectrochemical water splitting<\/b><\/strong>\u201d<\/b><\/strong>\u53d1\u8868\u5728\u4e86Nat. Commun.<\/b><\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe1\u00a0<\/b><\/strong>S\u7f3a\u9677CdIn<\/b><\/strong>2<\/b><\/sub><\/strong>S<\/b><\/strong>4<\/b><\/sub><\/strong>\u5149\u7535\u9633\u6781<\/b><\/strong>\u7684\u5408\u6210\u4e0e\u8868\u5f81<\/b><\/strong><\/b>\"\"<\/p>\n

a\uff09\u542b\u786b\u7a7a\u4f4d\u7684CdIn2<\/sub>S4<\/sub>\u5149\u7535\u9633\u6781\u7684\u5408\u6210\u8fc7\u7a0b\u793a\u610f\u56fe\u3002<\/p>\n

b\uff09PXRD\u884d\u5c04\u8c31\u56fe\u3002<\/p>\n

c\uff09ESR\u5149\u8c31\u3002<\/p>\n

d\uff09CdIn2<\/sub>S4<\/sub>\u548cVs-CIS-500\u7684S 2p\u00a0XPS\u5149\u8c31\u3002<\/p>\n

e\uff09Vs<\/sub>-CIS-500\u7684SEM\u56fe\u50cf\u3002\u63d2\u56fe\u662f\u57fa\u4e8eBFDH\u7406\u8bba\u7684\u6a21\u578b\u3002<\/p>\n

f\uff09Vs<\/sub>-CIS-500\u7684HADDF-STEM\u56fe\u50cf\u3002\u63d2\u56fe\u662fCdIn2<\/sub>S4<\/sub>\uff0801\u00af1\uff09\u7684\u539f\u5b50\u7ed3\u6784\uff0c\u5176\u4e2dIn\u548cS\u4e3a\u622a\u65ad\u539f\u5b50\u3002<\/p>\n

g\uff09CdIn2<\/sub>S4<\/sub>\u5757\u4f53\u548c\u5177\u6709\u8868\u9762\u786b\u7a7a\u4f4d\u7684CdIn2<\/sub>S4<\/sub>\uff0801\u00af1\uff09\u7684\u6001\u5bc6\u5ea6\u3002<\/p>\n

h\uff09\u5177\u6709\u8868\u9762\u786b\u7a7a\u4f4d\uff08\u7b49\u503c\u9762\u4e3a0.04e Bohr-3<\/sup>\uff09\u7684CdIn2<\/sub>S4<\/sub>\uff0801\u00af1\uff09\u7684\u4e0d\u540c\u7535\u8377\u5bc6\u5ea6\u56fe\u50cf\uff1b\u9ec4\u8272\u548c\u9752\u8272\u533a\u57df\u5206\u522b\u8868\u793a\u7535\u5b50\u7d2f\u79ef\u548c\u8017\u5c3d\u3002<\/p>\n

\u56fe2 <\/b><\/strong>\u5149\u7535\u9633\u6781\u7684PEC\u6027\u80fd<\/b><\/strong>\"\"<\/p>\n

a\uff09\u5728\u9ed1\u6697\u548cAM 1.5 G\uff0c100 mW cm-2<\/sup>\u7167\u660e\u548c\u626b\u63cf\u901f\u7387\u4e3a10 mV s-1<\/sup>\u7684\u6761\u4ef6\u4e0b\uff0c\u57280.35 M Na2<\/sub>SO3<\/sub>\u548c0.25 M Na2<\/sub>S\u6df7\u5408\u6eb6\u6db2\uff08pH = 12.5\uff09\u4e2d\u6d4b\u5f97\u7684\u7535\u6d41-\u7535\u538b\u66f2\u7ebf\uff08J-V\uff09\u3002<\/p>\n

b\uff09\u57280.5 M Na2<\/sub>SO4<\/sub>\u6eb6\u6db2\uff08pH = 7\uff09\u4e2d\uff0c\u5728\u9ed1\u6697\u548c\u5149\u7167\u6761\u4ef6\u4e0b\uff0cCdIn2<\/sub>S4<\/sub>\u548cVs<\/sub>-CIS-500\u5149\u7535\u9633\u6781\u7684\u5f00\u8def\u7535\u538b\u3002<\/p>\n

c\uff09\u5728\u9ed1\u6697\u548cAM 1.5 G\uff0c100 mW cm-2<\/sup>\u7167\u660e\u4e0b\uff0c\u57280.35 M Na2<\/sub>SO3<\/sub>\u548c0.25 M Na2<\/sub>S\u6df7\u5408\u6eb6\u6db2\uff08pH = 12.5\uff09\u4e2d\u7684ABPE\u3002<\/p>\n

d\uff09\u5355\u8272\u5149\u7167\u5c04\u4e0b\u57280.6 V vs. RHE\u7684\u6761\u4ef6\u4e0b\u6d4b\u5f97\u7684IPCE\u3002<\/p>\n

e\uff09CdIn2<\/sub>S4<\/sub>\u548cVs-CIS-500\u6750\u6599\u7684SPV\u5149\u8c31\u3002<\/p>\n

f\uff09\u5728AM 1.5 G\uff0c100 mW cm-2<\/sup>\u7167\u660e\u4e0b\uff0c\u57280.35 M Na2<\/sub>SO3<\/sub>\u548c0.25 M Na2<\/sub>S\u6df7\u5408\u6eb6\u6db2\uff08pH = 12.5\uff09\u4e2d\u8fdb\u884c\u7a33\u5b9a\u6027\u6d4b\u8bd5\uff0c\u4ee5\u53ca\u5b9e\u9a8c\u548c\u7406\u8bba\u4e0a\u7684\u6790\u6c22\u4ea7\u7387\u3002<\/p>\n

\u56fe3 <\/b><\/strong>\u5149\u5b66\u548c<\/b><\/strong>\u5149\u7535\u5316\u5b66\u7684\u673a\u7406<\/b><\/strong>\"\"<\/p>\n

a\uff09UV-vis\u6f2b\u53cd\u5c04\u5149\u8c31\u3002<\/p>\n

b\uff09\u7535\u8377\u5206\u79bb\u6548\u7387\u3002<\/p>\n

c\uff09\u7535\u8377\u6ce8\u5165\u6548\u7387-\u7535\u4f4d\u66f2\u7ebf\u3002<\/p>\n

d\uff09\u6fc0\u53d1\u6ce2\u957f\u4e3a\u03bbex<\/sub>\u00a0<\/sub>= 370 nm\u7684\u7a33\u6001PL\u5149\u8c31\u3002<\/p>\n

e\uff09\u6fc0\u53d1\u6ce2\u957f\u4e3a\u03bbex<\/sub>\u00a0= 370 nm\u7684\u65f6\u95f4\u5206\u8fa8\u77ac\u6001PL\u8870\u51cf\u8c31\u3002<\/p>\n

f\uff09CdIn2<\/sub>S4<\/sub>\u548cVs<\/sub>-CIS-500\u7684PALS\u8c31\u56fe\u3002<\/p>\n

\u56fe4 <\/b><\/strong>\u7535\u8377\u8f6c\u79fb\u548c\u91cd\u7ec4\u52a8\u529b\u5b66<\/b><\/strong>\"\"<\/p>\n

a\uff09\u7531EIS\u5149\u8c31\u8ba1\u7b97\u7684\u4e0d\u540c\u65bd\u52a0\u7535\u52bf\u7684\u8868\u9762\u6001\u4e0e\u7535\u8377\u4fd8\u83b7\u76f8\u5173\u7684\u7535\u5bb9\u548c\u7535\u963b\u53c2\u6570\u3002<\/p>\n

b\uff09\u8868\u9762\u6001\uff08SS\uff09\u7684DOS\u968fCdIn2<\/sub>S4<\/sub>\u548cVs<\/sub>-CIS-500\u5149\u7535\u9633\u6781\u7684\u65bd\u52a0\u504f\u538b\u7684\u53d8\u5316\u3002<\/p>\n

c\uff09Mott-Schottky\u56fe\u3002<\/p>\n

d\uff09CdIn2<\/sub>S4<\/sub>\u548cVs<\/sub>-CIS-500\u5149\u9633\u6781\u57281.13 V\u504f\u538b\u4e0b\u7684IMPS\u5149\u8c31\u3002<\/p>\n

e\uff09\u7535\u8377\u8f6c\u79fb\u901f\u7387\u5e38\u6570\u56fe\u3002<\/p>\n

f\uff09\u7535\u8377\u590d\u5408\u901f\u7387\u5e38\u6570\u56fe\u3002<\/p>\n

\u56fe<\/b><\/strong>5<\/b><\/strong>\u00a0<\/b><\/strong>CdIn<\/b><\/strong>2<\/b><\/sub><\/strong>S<\/b><\/strong>4<\/b><\/sub><\/strong>\u5149\u7535\u9633\u6781\u7684OER\u673a\u5236<\/b><\/strong>\"\"<\/p>\n

a\uff09CdIn2<\/sub>S4<\/sub>\uff0801\u00af1\uff09\u7684OER\u9636\u8dc3\u7684\u81ea\u7531\u80fd\u3002<\/p>\n

b\uff09Vs<\/sub>-CdIn2<\/sub>S4<\/sub>\uff0801\u00af1\uff09\u7684OER\u9636\u8dc3\u7684\u81ea\u7531\u80fd\u3002<\/p>\n

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d\uff09Vs<\/sub>-CdIn2<\/sub>S4<\/sub>\uff0801\u00af1\uff09\u4eceHOMO\u6001\uff08\u5728\u8d39\u7c73\u80fd\u7ea7\u4ee5\u4e0b0-0.5 eV\u7684\u8303\u56f4\u5185\uff09\u5230LUMO\u6001\uff08\u5728\u8d39\u7c73\u80fd\u7ea7\u4ee5\u4e0a0-1 eV\u7684\u8303\u56f4\u5185\uff09\u7684\u5149\u6fc0\u53d1\u7535\u8377\u8dc3\u8fc1\u8def\u5f84\u53d8\u5316\uff0c\u65bd\u52a0\u7684\u504f\u538b\u4e3a1.23 V\uff08\u7b49\u503c\u9762\u4e3a0.004e Bohr-3<\/sup>\uff09\u3002\u7535\u8377\u5dee\u5bc6\u5ea6\u7531\u0394\u03c1\uff1d\u03c11.23V<\/sub>-\u03c10V<\/sub>\u8ba1\u7b97\uff0c\u9ec4\u8272\u533a\u57df\u8868\u793a\u7535\u5b50\u7d2f\u79ef\u3002<\/p>\n

\u3010\u5c0f\u7ed3<\/b><\/strong>\u3011<\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u56e2\u961f\u5f00\u53d1\u4e86\u4e00\u79cd\u7528\u4e8ePEC\u6c34\u5206\u89e3\u7684\u9ad8\u6d3b\u6027\u3001\u7f3a\u9677\u578b\u4e09\u5143\u786b\u5316\u7269\uff08CdIn2<\/sub>S4<\/sub>\uff09\u5149\u9633\u6781\u3002CdIn2<\/sub>S4<\/sub>\u8868\u9762\u7684\u786b\u7a7a\u4f4d\u662f\u5bfc\u81f4\u5149\u7535\u6d41\u6539\u5584\u7684\u4e3b\u8981\u539f\u56e0\u3002\u901a\u8fc7\u7406\u8bba\u8ba1\u7b97\u548c\u5b9e\u9a8c\u8868\u5f81\uff0c\u7814\u7a76\u4e86\u8868\u9762\u786b\u7a7a\u4f4d\u7684\u5f71\u54cd\u3002\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0c\u5f15\u5165\u7684\u8868\u9762\u786b\u7a7a\u4f4d\u5bfc\u81f4\u90bb\u8fd1\u7684In\u548cCd\u539f\u5b50\u4e0a\u7684\u7535\u8377\u79ef\u7d2f\uff0c\u8fd9\u4e9b\u539f\u5b50\u6210\u4e3aOER\u4e2d\u95f4\u4f53\u7684\u6d3b\u6027\u4f4d\u70b9\uff0c\u5bfc\u81f4\u8fc7\u7535\u4f4d\u4e0b\u964d\u3002\u5149\u5b66\u8868\u5f81\u8868\u660e\u8868\u9762\u786b\u7a7a\u4f4d\u5bf9\u7535\u8377\u5206\u79bb\u548c\u6ce8\u5165\u6548\u7387\u7684\u4e3b\u8981\u5f71\u54cd\uff0c\u8868\u660e\u786b\u7a7a\u4f4d\u5f15\u5165\u7684\u6d45\u9631\u6001\u4fc3\u8fdb\u7535\u8377\u5206\u79bb\u548c\u8f6c\u79fb\u3002\u7535\u8377\u8f6c\u79fb\u548c\u590d\u5408\u52a8\u529b\u5b66\u7684\u8868\u5f81\u8fdb\u4e00\u6b65\u8bc1\u5b9e\u4e86\u5149\u7535\u6d41\u589e\u5f3a\u7684\u6839\u672c\u539f\u56e0\u662f\u7a7a\u7a74\u8f6c\u79fb\u901f\u7387\u7684\u63d0\u9ad8\u548c\u8868\u9762\u7535\u8377\u91cd\u7ec4\u7684\u6291\u5236\u3002\u5f97\u76ca\u4e8e\u8868\u9762\u786b\u7a7a\u4f4d\uff0cCdIn2<\/sub>S4<\/sub>\u5149\u9633\u6781\u57281.23 V vs. RHE\u65f6\u7684\u5149\u7535\u6d41\u5bc6\u5ea6\u4e3a5.73 mA cm-2<\/sup>\uff0c\u57280.477 V vs. RHE\u65f6\u7684ABPE\u503c\u4e3a2.49%\uff0c\u8fd9\u4f7f\u5176\u6210\u4e3aPEC\u6c34\u5206\u89e3\u6709\u524d\u666f\u7684\u6750\u6599\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>Highly active deficient ternary sulfide photoanode for photoelectrochemical water splitting<\/u><\/a>\uff08Nat. Commun.\uff0c 2020\uff0cDOI:10.1038\/s41467-020-16800-w\uff09<\/p>\n

\u3010\u56e2\u961f\u4ecb\u7ecd<\/b>\u3011<\/p>\n

\u9648\u4ee3\u8363\u6559\u6388\u7b80\u4ecb\uff1a<\/strong><\/p>\n

\u535a\u58eb\u751f\u5bfc\u5e08\uff0c\u517c\u4efb\u4e2d\u56fd\u7ed5\u6708\u63a2\u6d4b\u5de5\u7a0b\u79d1\u5b66\u5e94\u7528\u4e13\u5bb6\u59d4\u5458\u4f1a\u4e13\u5bb6\u3001\u4e2d\u56fd\u6750\u6599\u7814\u7a76\u7406\u4e8b\u4f1a\u9752\u59d4\u4f1a\u5e38\u52a1\u7406\u4e8b\u3001The Open Crystallography J. \u56fd\u9645\u671f\u520a\u7f16\u59d4\uff0c\u5c71\u4e1c\u7701\u6709\u7a81\u51fa\u8d21\u732e\u7684\u4e2d\u9752\u5e74\u4e13\u5bb6\uff0c\u5165\u9009\u6cf0\u5c71\u5b66\u8005\u6500\u767b\u8ba1\u5212\uff0c\u4eab\u53d7\u56fd\u52a1\u9662\u653f\u5e9c\u6d25\u8d34\u3002\u8fd1\u5e74\u6765\u4e3b\u8981\u4ece\u4e8b\u529f\u80fd\u7eb3\u7c73\u6750\u6599\u7684\u7406\u8bba\u548c\u5e94\u7528\u7814\u7a76\u5de5\u4f5c\uff0c\u5305\u62ec\u7eb3\u7c73\u6750\u6599\u5f62\u6210\u8fc7\u7a0b\u548c\u673a\u7406\u7684\u7814\u7a76\u3001Sol-Gel\u5236\u5907\u65e0\u673a\u7ea4\u7ef4\u6750\u6599\u7684\u7814\u7a76\u4ee5\u53ca\u7eb3\u7c73\u6750\u6599\u5fae\u89c2\u7ed3\u6784\u4e0e\u5176\u7269\u7406\u548c\u5316\u5b66\u6027\u8d28\u76f8\u4e92\u5173\u7cfb\u7684\u7814\u7a76\uff0c\u5728Nature Commun. Adv. Mater\u3001Chem. Mater\u3001J. Phys. Chem.\u7b49\u56fd\u9645\u671f\u520a\u4e0a\u4f5c\u4e3a\u7b2c\u4e00\u4f5c\u8005\u6216\u901a\u8baf\u4f5c\u8005\u53d1\u8868SCI\u8bba\u6587180\u4f59\u7bc7\uff0c\u7814\u7a76\u5de5\u4f5c\u5f15\u8d77\u4e86\u56fd\u9645\u4e0a\u76f8\u5173\u9886\u57df\u79d1\u5b66\u5bb6\u7684\u5e7f\u6cdb\u5173\u6ce8\uff0c\u8bba\u6587\u88abSCI \u4ed6\u5f153000\u4f59\u6b212017-2019\u5e74\u79d1\u777f\u552f\u5b89\u9ad8\u5f15\u4f5c\u8005\u3002\u5e94\u7528\u6210\u679c\u5e94\u7528\u540e\u4ea7\u751f\u4e86\u663e\u8457\u7684\u7ecf\u6d4e\u4e0e\u793e\u4f1a\u6548\u76ca\uff0c\u4f5c\u4e3a\u7b2c\u4e00\u5b8c\u6210\u4eba\uff0c\u83b7\u5f97\u56fd\u5bb6\u79d1\u6280\u8fdb\u6b65\u4e8c\u7b49\u5956\u3001\u5c71\u4e1c\u7701\u79d1\u6280\u8fdb\u6b65\u4e00\u7b49\u5956\u3001\u5c71\u4e1c\u7701\u79d1\u6280\u8fdb\u6b65\u4e8c\u7b49\u5956\u3001\u6559\u80b2\u90e8\u79d1\u6280\u8fdb\u6b65\u4e8c\u7b49\u5956\u5404\u4e00\u9879\u3002<\/p>\n

\u672c\u6587\u7531\u6728\u6587\u97ec<\/b><\/strong>\u7ffb\u8bd1\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n

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