{"id":202910,"date":"2020-06-03T06:40:20","date_gmt":"2020-06-02T22:40:20","guid":{"rendered":"\/\/m.iemloyee.com\/?p=202910"},"modified":"2020-06-02T20:41:10","modified_gmt":"2020-06-02T12:41:10","slug":"%e8%a5%bf%e5%ae%89%e4%ba%a4%e5%a4%a7%e5%90%b4%e6%9c%9d%e6%96%b0nano-energy-%e5%9f%ba%e4%ba%8e%e8%a1%a8%e9%9d%a2%e6%99%b6%e6%a0%bc%e5%ba%94%e5%8f%98%e8%b0%83%e6%8e%a7%e7%9a%84%e9%ab%98%e6%95%88","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=202910","title":{"rendered":"\u897f\u5b89\u4ea4\u5927\u5434\u671d\u65b0Nano Energy: \u57fa\u4e8e\u8868\u9762\u6676\u683c\u5e94\u53d8\u8c03\u63a7\u7684\u9ad8\u6548\u53cd\u578b\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u5982\u4eca\uff0c\u7531\u4e8e\u5316\u77f3\u71c3\u6599\u50a8\u5b58\u9650\u5236\uff0c\u5bf9\u53ef\u518d\u751f\u80fd\u91cf\u7684\u9700\u6c42\u6025\u5267\u589e\u957f\uff0c\u6025\u9700\u53d1\u5c55\u9ad8\u6548\u7a33\u5b9a\u592a\u9633\u80fd\u7535\u6c60\u3002\u6709\u673a-\u65e0\u673a\u91d1\u5c5e\u5364\u7d20\u9499\u949b\u77ff\u6750\u6599\u4f5c\u4e3a\u8fd1\u5e74\u7684\u660e\u661f\u6750\u6599\uff0c\u7531\u4e8e\u5176\u7406\u60f3\u7684\u76f4\u63a5\u5e26\u9699\uff0c\u9ad8\u5438\u6536\u7cfb\u6570\uff0c\u9ad8\u8f7d\u6d41\u5b50\u8fc1\u79fb\u7387\u7b49\u4f18\u826f\u5149\u7535\u7279\u6027\u800c\u5f97\u5230\u5e7f\u6cdb\u7814\u7a76\u3002\u7136\u800c\uff0c\u7531\u4e8e\u5176\u6750\u6599\u4f4e\u5f62\u6210\u80fd\u548c\u5feb\u901f\u7ed3\u6676\u9650\u5236\u5668\u4ef6\u957f\u671f\u7a33\u5b9a\u6027\uff0c\u963b\u788d\u5176\u53d1\u5c55\u3002\u8fd1\u5e74\u6765\uff0c\u529f\u80fd\u5316\u6709\u673a\u5206\u5b50\u5df2\u88ab\u9009\u62e9\u7528\u4e8e\u6291\u5236\u7f3a\u9677\u5f62\u6210\u7b49\u5bfc\u81f4\u7684\u7a33\u5b9a\u6027\u95ee\u9898\u3002\u8def\u6613\u65af\u9178\u78b1\u6dfb\u52a0\u5242\u8bc1\u660e\u5728\u5ef6\u7f13\u7ed3\u6676\u3001\u6291\u5236\u7f3a\u9677\u5f62\u6210\u65b9\u9762\u7279\u522b\u6709\u6548\u3002Henry J. Snaith\u7ec4\u5df2\u7ecf\u8bc1\u660e\u8def\u6613\u65af\u78b1\u53ef\u4ee5\u949d\u5316\u6676\u683c\u4e2d\u672a\u914d\u4f4d\u7684Pb\u539f\u5b50\uff0c\u964d\u4f4e\u975e\u8f90\u5c04\u590d\u5408\uff0c\u5927\u5e45\u63d0\u9ad8\u8367\u5149\u5bff\u547d\u3002\u6b64\u5916\uff0c\u5173\u4e8e\u540c\u65f6\u5177\u6709\u7f3a\u9677\u949d\u5316\u548c\u6676\u683c\u8868\u754c\u9762\u7a33\u56fa\uff0c\u5b9e\u73b0\u76f8\u5e94\u5206\u5b50\u7684\u8bbe\u8ba1\u548c\u9009\u62e9\u4e5f\u663e\u5f97\u5c24\u4e3a\u91cd\u8981\u3002\u56e0\u6b64\uff0c\u5728\u89e3\u51b3\u8868\u754c\u9762\u6676\u683c\u7a33\u56fa\uff0c\u63d0\u9ad8\u529f\u80fd\u6750\u6599\u56fa\u6709\u7a33\u5b9a\uff0c\u8fd9\u5c06\u6709\u5229\u4e8e\u9ad8\u6548\u7387\u5668\u4ef6\u7684\u5b9e\u73b0\u548c\u957f\u671f\u7a33\u5b9a\u6027\u3002<\/p>\n

\u3010\u7814\u7a76\u5185\u5bb9\u3011<\/b><\/strong><\/p>\n

\u9488\u5bf9\u4ee5\u4e0a\u9499\u949b\u77ff\u592a\u9633\u80fd\u5668\u4ef6\u4e2d\u5b58\u5728\u7684\u95ee\u9898\uff0c\u5434\u671d\u65b0\u6559\u6388\u7ec4\u5f00\u53d1\u4e86\uff1a\u4e00\u79cd\u5177\u6709\u521a\u6027\u548c\u79bb\u57df\u7684\u5171\u8f6d\u914d\u4f534-phenylpyridine (4-pPy)\uff0c\u901a\u8fc7\u8c03\u8282\u7ed3\u6676\u52a8\u529b\u5b66\uff0c\u5236\u5907\u9ad8\u8d28\u91cf\u3001\u9ad8\u7ed3\u6676\u53d6\u5411\u8584\u819c\uff0c\u51cf\u5c11\u6676\u683c\u8868\u9762\u7a7a\u4f4d\u5f62\u6210\uff0c\u5e76\u6709\u6548\u6291\u5236\u6676\u683c\u626d\u66f2\u5bfc\u81f4\u7684\u5668\u4ef6\u4e0d\u7a33\u5b9a\u3002\u6b64\u5916\uff0c\u6709\u5e8f\u6392\u5217\u663e\u8457\u6291\u5236\u6676\u683c\u7578\u53d8\u3002DFT\u8ba1\u7b97\u8868\u660e\uff0c\u5421\u5576\u884d\u751f\u7269\u4e0e\u9499\u949b\u77ff\u6676\u754c\u8868\u9762\u4e09\u7ef4\u6392\u5217\u4f18\u5316\u7279\u6027\uff0c\u5b9e\u73b0\u4e86\u521a\u6027\u5206\u5b504-pPy\u6700\u4f18\u7684\u4e09\u7ef4\u6392\u5217\u7279\u6027\u3002\u8be5\u65b9\u5f0f\u4e0d\u4ec5\u964d\u4f4e\u4e86\u8584\u819c\u5206\u89e3\uff0c\u800c\u4e14\u8d21\u732e\u4e86\u6770\u51fa\u7684\u5149\u7535\u7279\u6027\u3002\u91c7\u75284-pPy\u521a\u6027\u5206\u5b50\uff0c\u5b9e\u73b0p-i-n\u53cd\u578b\u5e73\u9762\u5f02\u8d28\u7ed3\u9499\u949b\u77ff\u5668\u4ef621.12%\uff08\u8ba4\u8bc1\u6548\u738720.2%\uff09\u7684\u5149\u7535\u8f6c\u5316\u6548\u7387\uff0c\u5e76\u5c55\u73b0\u4e86\u6770\u51fa\u7684\u7a33\u5b9a\u6027\u3002 \u00a0\u00a0<\/p>\n

\"\"<\/p>\n

\u8be5\u9879\u7814\u7a76\u5de5\u4f5c\u4ee5\u9898\u76ee\u4e3a\u201cLocal nearly non-strained perovskite lattice approaching a broad environmental stability window of efficient solar cells\u201d\u8fd1\u671f\u53d1\u8868\u4e8e\u56fd\u9645\u671f\u520aNano Energy\u00a0(2020\uff09<\/b><\/strong>\u3002\u7b2c\u4e00\u4f5c\u8005\u4e3a\u8bfe\u9898\u7ec4\u535a\u58eb\u751f\u5f90\u6d01\uff0c\u8463\u5316\u526f\u6559\u6388\u3001\u5434\u671d\u65b0\u6559\u6388\u548c\u674e\u749f\u777f\u7279\u8058\u7814\u7a76\u5458\u4e3a\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff0c\u897f\u5b89\u4ea4\u901a\u5927\u5b66\u4e3a\u7b2c\u4e00\u4f5c\u8005\u5355\u4f4d\u548c\u552f\u4e00\u901a\u8baf\u4f5c\u8005\u5355\u4f4d\u3002\u8be5\u5de5\u4f5c\u5f97\u5230\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u59d4\u9879\u76ee\uff08\u7f16\u53f761904145\u300161505161\u548c11574248\uff09\u7b49\u7684\u652f\u6301\u3002<\/p>\n

\u897f\u5b89\u4ea4\u901a\u5927\u5b66\u5434\u671d\u65b0\u6559\u6388\u56e2\u961f\u957f\u671f\u7814\u7a76\u65b0\u578b\u529f\u80fd\u6750\u6599\u7684\u201c\u5149-\u7535\u201d\u4e0e\u201c\u7535-\u5149\u201d\u7269\u7406\u673a\u5236\u53ca\u5176\u5668\u4ef6\u5e94\u7528\u5982\u592a\u9633\u80fd\u7535\u6c60\u4e0e\u53d1\u5149\u4e8c\u6781\u7ba1\uff0c\u8fd1\u671f\u6709\u591a\u9879\u91cd\u8981\u6210\u679c\u53d1\u8868\u4e8e\u56fd\u9645\u9876\u7ea7\u671f\u520a\uff1aJoule<\/i><\/b><\/em><\/strong>\uff0cAdvanced Materials, Angewandte Chemie International Edition, \u00a0Advanced Functional Materials, ACS Energy Letters, Nano Energy<\/i><\/b><\/em><\/strong>\u7b49\uff0c\u66f4\u591a\u7814\u7a76\u5185\u5bb9\u53ef\u53c2\u89c1\u5434\u671d\u65b0\u6559\u6388\u8bfe\u9898\u7ec4\u4e3b\u9875\uff1ahttp:\/\/zhaoxinwu.gr.xjtu.edu.cn<\/u><\/a><\/p>\n

\"\"<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe\u4e00.\u9499\u949b\u77ff\u8584\u819c\u7ed3\u6676\u3001\u5f62\u8c8c\u53ca\u5176\u5149\u5b66\u7279\u6027<\/b><\/strong><\/p>\n

\"\"<\/p>\n

(a-d) \u63a7\u5236\u7ec4\u548c\u5421\u5576\u884d\u751f\u7269\u4fee\u9970\u7684\u9499\u949b\u77ff\u8584\u819c\u7684SEM\u56fe.(e) \u7ed3\u6676\u6210\u6838\u539f\u7406\u56fe.(f) XRD\u56fe\u8c31. g) \u5438\u6536\u56fe\u8c31\u3002<\/p>\n

\u56fe\u4e8c.\u9499\u949b\u77ff\u8584\u819c\u7ed3\u6676\u53d6\u5411\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/p>\n

(a-d)\u63a7\u5236\u7ec4\u548c\u5421\u5576\u884d\u751f\u7269\u4fee\u9970\u7684\u9499\u949b\u77ff\u8584\u819c\u7684GIWAXS. (e)MAPbI3<\/sub>\u00a0(110) \u6676\u9762GIWAXS\u5f3a\u5ea6\u66f2\u7ebf\u56fe.(f)\u63a7\u5236\u7ec4\u548c\u5421\u5576\u884d\u751f\u7269\u4fee\u9970\u7684\u9499\u949b\u77ff\u8584\u819c\u7684\u7ed3\u6676\u53d6\u5411\u5806\u79ef\u6a21\u5f0f. (g)\u9499\u949b\u77ff\u4e0d\u540c\u8584\u819c\u5668\u4ef6\u7684\u622a\u9762\u56fe.<\/p>\n

\u56fe\u4e09.<\/b><\/strong>\u00a0<\/b><\/strong>\u5668\u4ef6\u7535\u5b66\u6027\u80fd\u6d4b\u8bd5<\/b><\/strong><\/p>\n

\"\"<\/p>\n

(a-b)\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u5668\u4ef6\u7ed3\u6784\u548c\u80fd\u7ea7\u56fe. (c)\u4e0d\u540c\u5668\u4ef6\u7684J-V\u66f2\u7ebf. (d)\u63a7\u5236\u7ec4\u548c4-pPy\u4fee\u9970\u7684\u5668\u4ef6\u7684\u6b63\u53cd\u626bJ-V\u66f2\u7ebf\u3002(e)\u63a7\u5236\u7ec4\u548c4-pPy\u4fee\u9970\u7684\u5668\u4ef6\u7684IPCE. (f)\u63a7\u5236\u7ec4\u548c4-pPy\u4fee\u9970\u7684\u5668\u4ef6, \u5728\u6700\u5927\u529f\u7387\u70b9\u7684\u7a33\u6001\u7535\u6d41\u8f93\u51fa.<\/p>\n

\u56fe\u56db. \u7f3a\u9677\u6001\u548c\u7535\u8377\u4f20\u8f93\u6027\u80fd<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u4fee\u9970\u524d\u540e\u9499\u949b\u77ff\u8584\u819c\uff1a(a) FTIR\u66f2\u7ebf.(b)XPS\u66f2\u7ebf. (c)DFT\u4f30\u7b97\u7684I\u7a7a\u4f4d\u7684\u5f62\u6210\u80fd. (d) \u7f3a\u9677\u6001\u5bc6\u5ea6\uff08tDOS\uff09. (e-h) DFT\u4f30\u7b97\u7684\u7a7a\u95f4\u6392\u5217. (i) TPC\u6d4b\u8bd5. LUMO\u7535\u5b50\u5bc6\u5ea6\u5206\u5e03: (j) 4-mPy, (k)4-ePy \u548c(l)4-pPy\u5206\u5b50.<\/p>\n

\u56fe\u4e94. \u4e0d\u540c\u5668\u4ef6\u7a33\u5b9a\u6027\u8868\u5f81\u53ca\u76f8\u5173\u8868\u9762\u6676\u683c\u5e94\u529b\u7279\u6027<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u63a7\u5236\u7ec4\u548c\u5421\u5576\u884d\u751f\u7269\u4fee\u9970\u7684\u5668\u4ef6\u7a33\u5b9a\u6027\uff1aa )\u6e7f\u5ea660%\uff0c1000h. b)\u572885 \u00b0C \uff0c 500 h\u7684\u70ed\u7a33\u5b9a\u6027\u66f2\u7ebf. c )600 h\u7684\u5de5\u4f5c\u7a33\u5b9a\u6027. d )\u4e0d\u540c\u884d\u751f\u7269\u4fee\u9970\u7684\u9499\u949b\u77ff\u8868\u9762\u6676\u683c\u5e94\u529b\u60c5\u51b5\u3002<\/p>\n

\u8bba\u6587\u94fe\u63a5\uff1ahttps:\/\/ doi.org\/10.1016\/j.nanoen.2020.104940<\/p>\n","protected":false},"excerpt":{"rendered":"

\u3010\u5f15\u8a00\u3011 \u5982\u4eca\uff0c\u7531\u4e8e\u5316\u77f3\u71c3\u6599\u50a8\u5b58\u9650\u5236\uff0c\u5bf9\u53ef\u518d\u751f\u80fd\u91cf\u7684\u9700\u6c42\u6025\u5267\u589e\u957f\uff0c\u6025\u9700\u53d1\u5c55\u9ad8\u6548\u7a33\u5b9a\u592a\u9633\u80fd\u7535\u6c60\u3002\u6709\u673a-\u65e0\u673a\u91d1\u5c5e\u5364\u7d20\u9499\u949b\u77ff\u6750\u6599\u4f5c\u4e3a\u8fd1\u5e74\u7684\u660e\u661f\u6750\u6599\uff0c\u7531\u4e8e\u5176\u7406\u60f3\u7684\u76f4\u63a5\u5e26…<\/p>\n","protected":false},"author":14360,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[],"class_list":["post-202910","post","type-post","status-publish","format-standard","hentry","category-jiedu"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/202910"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/14360"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=202910"}],"version-history":[{"count":4,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/202910\/revisions"}],"predecessor-version":[{"id":203051,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/202910\/revisions\/203051"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=202910"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=202910"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=202910"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}