{"id":201322,"date":"2020-05-20T06:49:05","date_gmt":"2020-05-19T22:49:05","guid":{"rendered":"\/\/m.iemloyee.com\/?p=201322"},"modified":"2020-05-19T19:49:37","modified_gmt":"2020-05-19T11:49:37","slug":"%e5%9b%bd%e4%ba%a7%e6%9d%90%e6%96%99%e7%b1%bb%e6%9c%9f%e5%88%8a%ef%bc%9ascience-bulletin%e3%80%81jec%e3%80%81scms%e3%80%81scc%e5%89%8d%e6%b2%bf%e5%8a%a8%e6%80%81","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=201322","title":{"rendered":"\u56fd\u4ea7\u6750\u6599\u7c7b\u671f\u520a\uff1aScience Bulletin\u3001JEC\u3001SCMs\u3001SCC\u524d\u6cbf\u52a8\u6001"},"content":{"rendered":"

\u56fd\u5185\u5b66\u672f\u671f\u520a\u7684\u53d1\u5c55\uff0c\u6d77\u5185\u5916\u534e\u4eba\u79d1\u5b66\u5bb6\u7684\u652f\u6301\u5fc5\u4e0d\u53ef\u5c11\u3002\u8fd1\u5e74\u6765\uff0c\u968f\u7740\u56fd\u5185\u5b66\u672f\u671f\u520a\u56e2\u961f\u7684\u8f9b\u52e4\u8015\u8018\u548c\u4e0d\u65ad\u52aa\u529b\uff0c\u56fd\u5185\u591a\u4e2a\u5b66\u672f\u671f\u520a\u5df2\u7ecf\u53d6\u5f97\u5f88\u4e0d\u9519\u7684\u6210\u7ee9\uff0c\u5927\u91cf\u4f18\u79c0\u79d1\u7814\u6210\u679c\u5728\u56fd\u5185\u4f18\u79c0\u671f\u520a\u4e0a\u53d1\u8868\u3002\u4ee5\u540e\uff0c\u4f60\u6216\u8bb8\u4f1a\u5728\u4f18\u79c0\u7684\u56fd\u4ea7\u671f\u520a\u4e0a\u53d1\u8868\u8fc7\u6587\u7ae0\u800c\u611f\u5230\u81ea\u8c6a\u3002\u524d\u6bb5\u65f6\u95f4\u7ed9\u5927\u5bb6\u5206\u4eab\u4e86\u56fd\u4ea7\u671f\u520a\u4e94\u5927\u82b1\u65e6\uff1aNational\u00a0Science Review\u3001npj\u00a0Computational Materials\u3001Nano Research\u3001Nano-Micro Letters\u3001Microsystems & Nanoengineering\u524d\u6cbf\u52a8\u6001\uff0c\u4eca\u5929\u7b14\u8005\u7ee7\u7eed\u5e26\u9886\u5927\u5bb6\u9886\u7565\u53e6\u5916\u51e0\u7bc7\u671f\u520a\u7684\u79d1\u6280\u52a8\u6001\u524d\u6cbf\u3002<\/p>\n

Science Bulletin<\/b><\/strong><\/p>\n

\u7c7b\u5408\u91d1\u7684\u4e09\u5143\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\u7684\u6548\u7387\u8d85\u8fc717.2%<\/b><\/strong><\/p>\n

\u5355\u5757\u5f02\u8d28\u7ed3\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60(PSCs)\u5728\u6750\u6599\u8fdb\u5316\u3001\u5668\u4ef6\u5236\u9020\u4f18\u5316\u548c\u5de5\u4f5c\u673a\u7406\u63a2\u7d22\u7b49\u65b9\u9762\u53d6\u5f97\u4e86\u957f\u8db3\u7684\u8fdb\u5c55\uff0c\u4ee5\u7a84\u7981\u5e26\u975e\u5bcc\u52d2\u70ef\u6750\u6599Y6\u4e3a\u53d7\u4f53\uff0cPSCs\u7684\u529f\u7387\u8f6c\u6362\u6548\u7387(PCE)\u5df2\u8d85\u8fc716%\uff0c\u5728\u4f18\u5316\u7684\u4e8c\u5143PSCs\u7684\u57fa\u7840\u4e0a\uff0c \u4e09\u5143\u7b56\u7565\u88ab\u8ba4\u4e3a\u662f\u5b9e\u73b0\u9ad8\u6027\u80fd\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\u7684\u6709\u6548\u65b9\u6cd5\u3002\u5728\u6b64\uff0c\u5317\u4eac\u4ea4\u901a\u5927\u5b66\u5f20\u798f\u4fca\u6559\u6388\u3001\u6b66\u6c49\u5927\u5b66\u6768\u695a\u7f57\u6559\u6388\u7b49\u4eba\u4f18\u5316\u540e\u7684\u4e09\u5143PSCs\u7684\u529f\u7387\u8f6c\u6362\u6548\u7387(PCE)\u4e3a17.22%,\u53d7\u4f53\u4e2dMF1\u542b\u91cf\u4e3a10%\u3002\u91c7\u7528\u4e09\u5143\u7b56\u7565\u540e\uff0cPCE\u7684\u6539\u5584\u5e45\u5ea6\u8d85\u8fc78%\uff0c\u8fd9\u662f\u56e0\u4e3a\u4e0e\u57fa\u4e8eY6\u4e8c\u5143PSCs\u76f8\u6bd4\uff0cJSC<\/sub>\u540c\u65f6\u589e\u52a0\u4e8625.68 mA cm–<\/sup>2<\/sup>, VOC\u589e\u52a0\u4e860.853 V, FF\u589e\u52a0\u4e8678.61%\u3002\u4ece\u62c9\u66fc\u6620\u5c04\u3001\u63a5\u89e6\u89d2\u3001\u5faa\u73af\u4f0f\u5b89\u548c\u5f62\u8c8c\u7b49\u65b9\u9762\u53ef\u4ee5\u786e\u5b9aMF1\u548cY6\u7684\u826f\u597d\u76f8\u5bb9\u6027\uff0c\u8fd9\u662f\u5f62\u6210\u5408\u91d1\u6001\u7684\u524d\u63d0\u3002\u7531\u4e8eY6\u548cMF1\u7684\u6700\u4f4e\u672a\u5360\u636e\u5206\u5b50\u8f68\u9053(LUMO)\u6c34\u5e73\u4e0d\u540c\uff0c\u4e09\u6d3b\u6027\u5c42\u4e2d\u7684\u7535\u5b50\u8fc1\u79fb\u7387\u5f88\u5927\u7a0b\u5ea6\u4e0a\u53d6\u51b3\u4e8e\u53d7\u4f53\u4e2d\u7684MF1\u542b\u91cf\uff0c\u8fd9\u53ef\u4ee5\u5f88\u597d\u5730\u89e3\u91ca\u4e09\u5143\u7ed3\u6784\u4e2d\u6ce2\u52a8\u578bFF\u7684\u53d8\u5316\u3002\u7b2c\u4e09\u65b9\u8ba4\u8bc1\u7684PCE\u4e3a16.8%\uff0c\u5e94\u8be5\u662f\u5355\u5757\u5f02\u8d28\u7ed3PSCs\u7684\u6700\u9ad8\u503c\u4e4b\u4e00\u3002\u672c\u5de5\u4f5c\u4e3a\u5b9e\u73b0\u9ad8\u6548\u7684\u4e09\u5143PSCs\u6750\u6599\u9009\u62e9\u63d0\u4f9b\u4e86\u5145\u5206\u7684\u53c2\u8003\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cAlloy-like ternary polymer solar cells with over 17.2% efficiency\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Science Bulletin\u4e0a\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/p>\n

DOI: 10.1016\/j.scib.2020.01.012<\/p>\n

\u5206\u5b50\u7ed3\u6784\u3001\u6027\u80fd\u548c\u5668\u4ef6\u7ed3\u6784<\/p>\n

\"\"<\/p>\n

DMF<\/b><\/strong>\u5bf9\u6c2e\u5316\u9502\u7684\u7a33\u5b9a\u6027\u673a\u7406\u53ca\u5176\u5728\u9502\u79bb\u5b50\u8d85\u7ea7\u7535\u5bb9\u5668\u9884\u9502\u5316\u4e2d\u7684\u5e94\u7528<\/b><\/strong><\/p>\n

\u6c2e\u5316\u9502\u662f\u4e00\u79cd\u6781\u597d\u7684\u96f6\u6b8b\u7559\u6b63\u6781\u9884\u9502\u5316\u6dfb\u52a0\u5242\uff0c\u53ef\u7528\u4e8e\u5f25\u8865\u9502\u79bb\u5b50\u7535\u5bb9\u5668\u53ca\u9502\u79bb\u5b50\u7535\u6c60\u5728\u9996\u5708\u7684\u9502\u635f\u5931\u3002\u4f46\u662f\uff0c\u5728\u7535\u6781\u5236\u9020\u8fc7\u7a0b\u4e2d\uff0c\u6c2e\u5316\u9502\u4e0e\u975e\u8d28\u5b50\u6781\u6027\u6eb6\u5242\u7684\u76f8\u5bb9\u6027\u5dee\uff0c\u4e0eN-\u7532\u57fa-2-\u5421\u54af\u70f7\u916e(NMP)\u7b49\u5e38\u7528\u6eb6\u5242\u5177\u6709\u5f88\u9ad8\u7684\u53cd\u5e94\u6027\uff0c\u9650\u5236\u4e86\u4ee5\u6c2e\u5316\u9502\u4f5c\u4e3a\u9884\u9502\u6dfb\u52a0\u5242\u7684\u6280\u672f\u63a8\u5e7f\u5e94\u7528\u3002\u4e2d\u79d1\u9662\u5927\u8fde\u5316\u7269\u6240\u674e\u5148\u950b\u3001\u5f20\u6d2a\u7ae0\u7b49\u4eba\u901a\u8fc7\u5546\u4e1a\u4e0a\u53ef\u7528\u7684\u5300\u6d46\u6d82\u5e03\u9014\u5f84\u5236\u5907\u4e86\u542b\u6c2e\u5316\u9502\u7684\u7535\u6781\uff0c\u4f7f\u7528 DMF\u4f5c\u4e3a\u5300\u6d46\u6eb6\u5242\uff0c\u5b9e\u9a8c\u5206\u6790\u548cDFT\u6a21\u62df\u8bc1\u5b9e\u4e86DMF\u7684\u5206\u5b50\u7a33\u5b9a\u673a\u7406\uff0cDMF\u7684\u8131\u6c22\u80fd\u660e\u663e\u5927\u4e8e\u5176\u4ed6\u5e38\u7528\u6eb6\u5242\u3002\u6dfb\u52a020%\u6c2e\u5316\u9502\u7684\u8f6f\u5305\u88c5\u9502\u79bb\u5b50\u7535\u5bb9\u5668\u5177\u6709\u51fa\u8272\u7684\u500d\u7387\u6027\u80fd\u3001\u5faa\u73af\u7a33\u5b9a\u6027\u548c\u8d85\u9ad8\u7684\u80fd\u91cf\u5bc6\u5ea6\uff0c\u5176\u80fd\u91cf\u5bc6\u5ea6\u662f\u4e0d\u542bLi3<\/sub>N\u5668\u4ef6\u76842.3\u500d\uff0c1\u4e07\u6b21\u5145\u653e\u7535\u5faa\u73af\u540e\uff0c\u5176\u80fd\u91cf\u4fdd\u6301\u7387\u9ad8\u8fbe90%\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cDMF stabilized Li3N slurry for manufacturing self-prelithiatable lithium-ion capacitors\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Science Bulletin\u4e0a\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/p>\n

DOI: 10.1016\/j.scib.2019.11.014<\/p>\n

DFT\u7684\u8ba1\u7b97\u548c\u53ef\u80fd\u7684\u53cd\u5e94<\/p>\n

\"\"<\/p>\n

Journal of Energy Chemistry<\/b><\/strong><\/p>\n

\u6709\u673a\u4e09\u7ef4\u4e92\u8054\u77f3\u58a8\u70ef\u6c14\u51dd\u80f6\u4f5c\u4e3a\u9ad8\u6027\u80fd\u950c\u79bb\u5b50\u7535\u6c60\u7684\u8d1f\u6781\u6750\u6599<\/b><\/strong><\/p>\n

\u6c34\u6027\u53ef\u5145\u7535\u950c\u79bb\u5b50\u7535\u6c60\u5177\u6709\u5b89\u5168\u6027\u9ad8\u3001\u6210\u672c\u4f4e\u3001\u8010\u4e45\u6027\u597d\u7b49\u4f18\u70b9\uff0c\u5728\u5927\u89c4\u6a21\u7684\u5b58\u50a8\u5e94\u7528\u4e2d\u5177\u6709\u5f88\u5927\u7684\u5438\u5f15\u529b\u3002\u7136\u800c\uff0c\u7531\u4e8eZn2+<\/sup>\u5728\u56fa\u4f53\u65e0\u673a\u6846\u67b6\u4e2d\u7684\u7f13\u6162\u6269\u6563\uff0c\u5bfc\u81f4\u9634\u6781\u6750\u6599\u7684\u7f3a\u4e4f\uff0c\u963b\u788d\u4e86\u5b83\u4eec\u7684\u53d1\u5c55\u3002\u5728\u6b64\uff0c\u54c8\u5c14\u6ee8\u5de5\u7a0b\u5927\u5b66\u53f6\u514b\u3001\u66f9\u6bbf\u5b66\u6559\u6388\u7b49\u4eba\u62a5\u9053\u4e86\u4e00\u79cd\u65b0\u578b\u7684\u6709\u673a\u7535\u6781\u6750\u6599\uff0c\u5176\u6750\u6599\u4e3a\u805a3\u30014\u30019\u300110-perylentetracarboxylic dianhydrode (PPTCDA)\/\u77f3\u58a8\u70ef\u6c14\u51dd\u80f6(GA)\u3002\u901a\u8fc7\u7b80\u5355\u7684\u6eb6\u5242\u70ed\u53cd\u5e94\u5408\u6210\u4e86\u4e09\u7ef4\u4e92\u8054\u591a\u5b54\u7ed3\u6784\uff0c\u5176\u4e2dPPTCDA\u5747\u5300\u5730\u5d4c\u5165\u5230GA\u7eb3\u7c73\u8584\u7247\u4e2d\u3002PPTCDA\/GA\u81ea\u7ec4\u88c5\u7ed3\u6784\u4e0d\u9700\u8981\u8f85\u52a9\u7535\u6781\u548c\u5bfc\u7535\u5242\u6765\u5236\u5907\u7535\u6781\u6750\u6599\uff0c\u662f\u5236\u5907\u6295\u5e01\u5f0f\u7535\u6c60\u7684\u4e00\u79cd\u7b80\u5355\u65b9\u6cd5\uff0c\u4e3a\u4e0b\u4e00\u6b65\u7684\u5927\u89c4\u6a21\u751f\u4ea7\u5960\u5b9a\u4e86\u57fa\u7840\u3002PPTCDA\/GA\u7684\u8f93\u51fa\u7535\u538b0.0 ~ 1.5 V\uff0c\u5bb9\u91cf\u2265200 mAh g-1<\/sup>\u3002\u7ecf\u8fc7300\u6b21\u5faa\u73af\u540e\uff0c\u5bb9\u91cf\u4fdd\u6301\u7387\u4ecd\u7136\u63a5\u8fd1100%\u3002\u901a\u8fc7FT-IR\u3001XRD\u548cXPS\u8868\u5f81\uff0c\u63a2\u8ba8\u4e86Zn2+<\/sup>\u63d2\u5c42\/\u8131\u5c42\u5728PPTCDA\/GA\u7535\u6781\u4e2d\u7684\u4f5c\u7528\u673a\u7406\u3002\u7528\u626b\u63cf\u7535\u955c(SEM)\u548c\u900f\u5c04\u7535\u955c(TEM)\u89c2\u5bdf\u4e86PPTCDA\/GA\u7684\u5f62\u8c8c\u548c\u7ed3\u6784\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cOrganic 3D interconnected graphene aerogel as cathode materials for high-performance aqueous zinc ion battery\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Journal of Energy Chemistry\u4e0a\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/p>\n

DOI:\u00a010.1016\/j.jechem.2019.09.026<\/p>\n

PPTCDA\/GA\u4e3a\u9634\u6781\u7684\u7535\u5316\u5b66\u6027\u80fd<\/p>\n

\"\"<\/p>\n

\u591a\u5b54\u78b3\u4e0e\u4ea4\u9519\u7684MoP-MoS<\/b><\/strong>2<\/b><\/sub><\/strong>\u5f02\u8d28\u7ed3\u6742\u5316\u9ad8\u6548\u7684\u6790\u6c22\u53cd\u5e94<\/b><\/strong><\/p>\n

\u7531\u975e\u8d35\u91d1\u5c5e\u50ac\u5316\u5242\u7ec4\u6210\u7684\u5177\u6709\u5927\u8868\u9762\u79ef\u548c\u9ad8\u7535\u5bfc\u7387\u7684\u7535\u50ac\u5316\u5242\u7684\u8bbe\u8ba1\u4e0e\u5f00\u53d1\u662f\u6790\u6c22\u53cd\u5e94\u7684\u5173\u952e\u3002\u5728\u6b64\uff0c\u534e\u5357\u7406\u5de5\u5927\u5b66\u5f6d\u65b0\u6587\u6559\u6388\u7b49\u4eba\u4ee5\u6728\u8d28\u7d20\u4e3a\u57fa\u7840\u7684\u591a\u5b54\u78b3\u4e0eMoS2<\/sub>-MoP\u5f02\u8d28\u7ed3(MoS2<\/sub>-MoP\/FPC)\u6742\u5316\u76f8\u5076\u8054\uff0c\u5e76\u4f5c\u4e3a\u6709\u524d\u9014\u7684\u50ac\u5316\u5242\u3002\u901a\u8fc7\u5728\u591a\u5b54\u78b3(MoS2<\/sub>\/FPC)\u4e0a\u56fa\u5b9a\u82b1\u74e3\u72b6\u7684\u4e8c\u786b\u5316\u94bc\u7eb3\u7c73\u7247\uff0c\u7136\u540e\u63a7\u5236\u5176\u5728Ar\/H2<\/sub>\u4e2d\u7684\u78f7\u5316\u53cd\u5e94\u5f62\u6210MoS2<\/sub>-MoP\/FPC\u3002\u7ea2\u78f7\u63d0\u4f9b\u4e86\u80fd\u5728\u8fd8\u539f\u6027\u6c14\u6c1b\u4e0b\u8bf1\u5bfc\u5f02\u8d28\u7ed3\u6784\u5efa\u7684P\u5143\u7d20\uff0c\u540c\u65f6\u4ea7\u751f\u4e86MoP\u548cMoS2<\/sub>\u76f8\u7684\u5206\u88c2\u3002\u5236\u5907\u7684MoS2<\/sub>\u2212MoP\/FPC\u50ac\u5316\u5242\u5728\u7535\u6d41\u5bc6\u5ea6\u4e3a10 mA cm\u22122<\/sup>\u65f6\uff0c\u5176\u8fc7\u7535\u4f4d\u4e3a144 mV\uff0c\u5728\u9178\u6027\u4ecb\u8d28\u4e2d\u5bf9HER\u7684Tafel\u659c\u7387\u4e3a41 mV dec\u22121<\/sup>\uff0c\u4e14\u7a33\u5b9a\u6027\u663e\u8457\u3002\u9664\u4e86\u6742\u5316\u4ea7\u7269\u7684\u6d3b\u6027\u5916\uff0c\u5176\u4f18\u5f02\u7684\u6d3b\u6027\u8fd8\u5f52\u529f\u4e8eMoS2-MoP\u7684\u5f02\u8d28\u7ed3\uff0c\u4ee5\u53ca\u591a\u5b54\u78b3\u826f\u597d\u7684\u7535\u8377\/\u4f20\u8d28\u80fd\u529b\u3002\u8be5\u7b56\u7565\u4e3a\u9ad8\u6210\u672c\u3001\u9ad8\u6027\u80fd\u50ac\u5316\u5242\u7684\u5f00\u53d1\u548c\u8bbe\u8ba1\u63d0\u4f9b\u4e86\u4e00\u79cd\u65b0\u65b9\u6cd5\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cPorous carbon coupled with an interlaced MoP\u2013MoS2 heterojunction hybrid for efficient hydrogen evolution reaction\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Journal of Energy Chemistry\u4e0a\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/p>\n

DOI:\u00a010.1016\/j.jechem.2019.09.010<\/p>\n

MoS2<\/sub>\u2212MoP\/FPC\u7684\u5236\u9020\u5de5\u827a\u793a\u610f\u56fe<\/p>\n

\"\"<\/p>\n

\u6742\u5316MOF@COF\u4f5c\u4e3a\u9009\u62e9\u6027\u6c27\u5316\u9187\u7684\u9ad8\u6548\u53ef\u89c1\u5149\u9a71\u52a8\u5149\u50ac\u5316\u5242<\/b><\/strong><\/p>\n

\u5229\u7528\u52a0\u901f\u5149\u8bf1\u5bfc\u7535\u5b50\u548c\u534a\u5bfc\u4f53\u95f4\u7535\u8377-\u8f7d\u6d41\u5b50\u5206\u79bb\u5efa\u7acb\u5171\u4ef7\u8fde\u63a5\u7ed3\u6784\u53ef\u4ee5\u63d0\u9ad8\u5149\u50ac\u5316\u6027\u80fd\u3002\u5728\u8fd9\u9879\u5de5\u4f5c\u4e2d\uff0c\u5317\u4eac\u79d1\u6280\u5927\u5b66\u738b\u6208\u6559\u6388\u3001\u5fb7\u56fd\u6ce2\u9e3f\u5927\u5b66Guixia Zhao \u6559\u6388\u7b49\u4eba\u62a5\u9053\u4e86\u4e00\u79cd\u7b80\u5355\u800c\u65b0\u9896\u7684\u751f\u957f\u65b9\u6cd5\uff0c\u7528\u7ed3\u6676\u548c\u591a\u5b54\u7684\u5171\u4ef7\u6709\u673a\u6846\u67b6(COFs)\u6750\u6599\u8986\u76d6NH2<\/sub>-MIL-125\u00a0(MOFs\uff09\uff0c\u5f62\u6210\u4e00\u7cfb\u5217\u4e0d\u540cCOF\u539a\u5ea6\u7684NH2<\/sub>-MIL-125@TAPB-PDA\u7eb3\u7c73\u590d\u5408\u6750\u6599\u3002\u5f15\u5165\u9002\u91cf\u7684COF\u4e0d\u4ec5\u53ef\u4ee5\u6539\u53d8\u5176\u56fa\u6709\u7684\u7535\u5b50\u548c\u5149\u5b66\u6027\u8d28\uff0c\u800c\u4e14\u53ef\u4ee5\u663e\u8457\u63d0\u9ad8\u5176\u5149\u50ac\u5316\u6d3b\u6027\u3002\u7279\u522b\u662fCOF\u539a\u5ea6\u572820nm\u5de6\u53f3\u7684NH2<\/sub>-MIL-125@TAPB-PDA-3\u82ef\u7532\u919b\u7684\u6536\u7387\u6700\u9ad8(94.7%)\uff0c\u7ea6\u4e3a\u6838\u4f53NH2<\/sub>–\u00a0MIL-125-\u76842.5\u500d\u548cCOF\u768415.5\u500d\u3002\u6742\u5316\u6750\u6599\u5149\u50ac\u5316\u6027\u80fd\u7684\u63d0\u9ad8\u4e3b\u8981\u662f\u7531\u4e8e\u901a\u8fc7\u5171\u4ef7\u952e\u589e\u5f3a\u4e86\u5149\u81f4\u8f7d\u6d41\u5b50\u5728MOF\u548cCOF\u4e4b\u95f4\u7684\u8f6c\u79fb\u3002\u6b64\u5916\uff0c\u8fd8\u63a2\u8ba8\u4e86\u9610\u660e\u5149\u50ac\u5316\u8fc7\u7a0b\u7684\u53ef\u80fd\u673a\u5236\u3002\u8fd9\u79cd\u57fa\u4e8eMOF\u7684\u5149\u50ac\u5316\u5242\u5728\u672a\u6765\u7684\u7eff\u8272\u6709\u673a\u5408\u6210\u4e2d\u5177\u6709\u5de8\u5927\u7684\u6f5c\u529b\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cCovalently integrated core-shell MOF@COF hybrids as efficient visible-light-driven photocatalysts for selective oxidation of alcohols\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Journal of Energy Chemistry\u4e0a\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/p>\n

DOI: 10.1016\/j.jechem.2019.07.014<\/p>\n

NH2<\/sub>-MIL-125@TAPB-PDA\u6742\u5316\u7684\u5408\u6210\u5de5\u827a\u793a\u610f\u56fe<\/p>\n

\"\"<\/p>\n

SCIENCE CHINA Materials<\/b><\/strong><\/p>\n

\u9000\u706b\u8c03\u63a7\u76843D\u4ea4\u8054TiNb<\/b><\/strong>2<\/b><\/sub><\/strong>O<\/b><\/strong>7<\/b><\/sub><\/strong>\u7eb3\u7c73\u68d2\u7535\u6781\u7528\u4e8e\u9ad8\u6548\u67d4\u6027\u9502\u79bb\u5b50\u7535\u5bb9\u5668<\/b><\/strong><\/p>\n

TiNb2<\/sub>O7<\/sub>\u7684\u7406\u8bba\u6bd4\u5bb9\u91cf\u9ad8\u8fbe280\u2005mA\u2005h\u2005g\u2212<\/sup>1<\/sup>, \u662f\u4e00\u7c7b\u6709\u524d\u666f\u7684\u9502\u79bb\u5b50\u7535\u5bb9\u5668\u8d1f\u6781\u6750\u6599\u3002\u7136\u800c\u5176\u8f83\u5dee\u7684\u7535\u5b50\u5bfc\u7535\u6027\u4e25\u91cd\u9650\u5236\u4e86\u5176\u500d\u7387\u6027\u80fd\u7684\u63d0\u5347\u3002\u5728\u6b64\uff0c\u6b66\u6c49\u7406\u5de5\u5927\u5b66\u5218\u91d1\u5e73\u6559\u6388\u8bfe\u9898\u7ec4\u5728\u67d4\u6027\u78b3\u5e03\u8868\u9762\u76f4\u63a5\u751f\u957f3D\u4ea4\u8054\u7684TiNb2<\/sub>O7<\/sub>\u7eb3\u7c73\u68d2\u591a\u5b54\u8d1f\u6781, \u5e76\u5c06\u5176\u9996\u6b21\u5e94\u7528\u4e8e\u67d4\u6027\u9502\u79bb\u5b50\u7535\u5bb9\u5668; \u78b3\u5e03\u7684\u9ad8\u5bfc\u7535\u6027, \u5355\u6676\u7eb3\u7c73\u68d2\u7ed3\u6784\u8f83\u77ed\u7684\u79bb\u5b50\/\u7535\u5b50\u4f20\u8f93\u8def\u5f84\u4ee5\u53ca\u826f\u597d\u7684\u7ed3\u6784\u7a33\u5b9a\u6027, \u6709\u6548\u63d0\u9ad8\u4e86\u6750\u6599\u7684\u500d\u7387\u6027\u80fd\u548c\u5faa\u73af\u7a33\u5b9a\u6027\u3002\u00a0\u7814\u7a76\u8868\u660e, TiNb2<\/sub>O7<\/sub>\u8d1f\u6781\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u500d\u7387\u6027\u80fd(\u4ece1\u523040\u2005C, \u5bb9\u91cf\u4fdd\u6301\u7387\u9ad8\u8fbe66.3%), \u51fa\u8272\u7684\u5faa\u73af\u7a33\u5b9a\u6027(>2000\u5708), \u4ee5\u53ca\u826f\u597d\u7684\u67d4\u97e7\u6027(\u8fde\u7eed\u5f2f\u66f2500\u6b21\u540e\u5bb9\u91cf\u65e0\u635f\u5931)\u3002\u6b64\u5916, \u5c06\u65e0\u7c98\u7ed3\u5242\u7684TiNb2<\/sub>O7<\/sub>\u8d1f\u6781\u548c\u5546\u7528\u6d3b\u6027\u70ad\u6b63\u6781\u642d\u914d\u6210\u9502\u79bb\u5b50\u7535\u5bb9\u5668, \u5c55\u73b0\u51fa\u4e86\u8f83\u9ad8\u7684\u8d28\u91cf\u548c\u4f53\u79ef\u80fd\u91cf\/\u529f\u7387\u5bc6\u5ea6(~100.6\u2005W\u2005h\u2005kg\u22121<\/sup>\/4108.8\u2005W\u2005kg\u22121<\/sup>; 10.7\u2005mW\u2005h\u2005cm\u22123<\/sup>\/419.3\u2005mW\u2005cm\u22123<\/sup>), \u4f18\u4e8e\u5148\u524d\u62a5\u9053\u7684\u6df7\u5408\u8d85\u7ea7\u7535\u5bb9\u5668, \u540c\u65f6\u8be5\u5668\u4ef6\u53ef\u4ee5\u5728180\u00b0\u5f2f\u66f2\u72b6\u6001\u4e0b\u4e3aLED\u706f\u4f9b\u7535\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cPost-annealing tailored 3D cross-linked TiNb2<\/sub>O7<\/sub>\u00a0nanorod electrode: towards superior lithium storage for flexible lithium-ion capacitors\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728SCIENCE CHINA Materials\u4e0a\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/p>\n

DOI: 10.1007\/s40843-019-1225-1<\/p>\n

\u57fa\u4e8eTNO-750-7h\u7684LIC\u6a21\u578b\u7684\u7535\u5316\u5b66\u6027\u80fd<\/p>\n

\"\"<\/p>\n

\u4e00\u6b65\u7403\u78e8\u6cd5\u5236\u5907\u77f3\u58a8\u70ef\/\u70ad\u9ed1\u6c34\u6027\u5bfc\u7535\u6cb9\u58a8\u5e94\u7528\u4e8e\u67d4\u6027\u7535\u5b50\u5668\u4ef6<\/b><\/strong><\/p>\n

\u4e2d\u56fd\u79d1\u5b66\u9662\u7164\u70ad\u5316\u5b66\u7814\u7a76\u6240\u9648\u6210\u731b\u7814\u7a76\u5458\u7b49\u4ee5\u77f3\u58a8\u70ef\u548c\u70ad\u9ed1\u4f5c\u4e3a\u5bfc\u7535\u586b\u6599, \u901a\u8fc7\u4e00\u6b65\u7403\u78e8\u6cd5\u5236\u5907\u4e86\u9ad8\u5bfc\u7535\u7684\u6c34\u6027\u78b3\u7cfb\u6cb9\u58a8\u3002\u5f53\u77f3\u58a8\u70ef\u8d28\u91cf\u5206\u6570\u4e3a10%\u65f6, \u590d\u5408\u6cb9\u58a8\u5177\u6709\u6700\u4f18\u7684\u6d41\u53d8\u5b66\u6027\u80fd; \u5728\u4e1d\u7f51\u5370\u5237\u4e2d, \u8be5\u6cb9\u58a8\u5728\u805a\u9170\u4e9a\u80fa\u57fa\u5e95\u4e0a\u5f62\u6210\u5747\u5300\u81f4\u5bc6\u7684\u6d82\u5c42\u3002\u5728\u5fae\u89c2\u4e0a, \u6d82\u5c42\u5177\u6709\u5939\u5c42\u4e09\u7ef4\u7f51\u7edc\u7ed3\u6784, \u7535\u963b\u7387\u662f\u7eaf\u70ad\u9ed1\u6d82\u5c42\u7535\u963b\u7387\u768430%\u3002\u8f8a\u538b\u5904\u7406\u540e, \u7535\u963b\u7387\u964d\u81f30.18\u00b10.01\u2005\u03a9\u2005cm, \u4e14\u6d82\u5c42\u5177\u6709\u826f\u597d\u7684\u673a\u68b0\u67d4\u6027, \u7ecf\u8fc73000\u6b21\u5faa\u73af\u5f2f\u6298\u8bd5\u9a8c\u540e\u7535\u963b\u4ec5\u589e\u52a012%\u3002\u5c06\u77f3\u58a8\u70ef\/\u70ad\u9ed1\u590d\u5408\u6d82\u5c42\u4f5c\u4e3a\u67d4\u6027\u5bfc\u4f53, \u6210\u529f\u7ec4\u88c5\u4e86\u53d1\u5149\u4e66\u7b7e\u548c\u8584\u819c\u5f00\u5173, \u8868\u660e\u8be5\u6d82\u5c42\u5728\u67d4\u6027\u7535\u5b50\u5668\u4ef6\u5927\u89c4\u6a21\u751f\u4ea7\u4e2d\u5177\u6709\u5de8\u5927\u7684\u6f5c\u529b\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cOne-pot ball-milling preparation of graphene\/carbon black aqueous inks for highly conductive and flexible printed electronics\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728SCIENCE CHINA Materials\u4e0a\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/p>\n

DOI: 10.1007\/s40843-019-1210-3<\/p>\n

\u6cb9\u58a8\u5236\u5907\u8fc7\u7a0b\u7684\u793a\u610f\u56fe\u53ca\u7a33\u5b9a\u6027\u5149\u5b66\u7167\u7247<\/p>\n

\"\"<\/p>\n

CALPHAD\u8f85\u52a9\u8bbe\u8ba1\u9ad8\u5f3a\u5ea6\u6c89\u6dc0\u5f3a\u5316\u578b\u9ad8\u71b5\u5408\u91d1<\/b><\/strong><\/p>\n

\u8fd1\u5e74\u6765, \u8bbe\u8ba1\u5177\u6709\u9ad8\u5f3a\u5ea6\u548c\u4f18\u5f02\u5ef6\u5c55\u6027\u7684\u9ad8\u71b5\u5408\u91d1(HEAs)\u5f15\u8d77\u4e86\u4eba\u4eec\u7684\u5e7f\u6cdb\u5174\u8da3\u3002\u4e2d\u5357\u5927\u5b66\u5b8b\u65fc\u6559\u6388\u7b49\u4eba\u91c7\u7528CALPHAD\u65b9\u6cd5\u6765\u8bbe\u8ba1\u6c89\u6dc0\u5f3a\u5316\u578b(FeCoNi)92<\/sub>Al2.5<\/sub>Ti5.5<\/sub>\u9ad8\u71b5\u5408\u91d1. \u901a\u8fc7\u70ed\u673a\u68b0\u5904\u7406\u8fc7\u7a0b\u6765\u8c03\u63a7\u5408\u91d1\u6676\u7c92\u5c3a\u5bf8\u3001\u6790\u51fa\u76f8\u5927\u5c0f\u53ca\u4f53\u79ef\u5206\u6570, \u4ece\u800c\u4f18\u5316\u5408\u91d1\u529b\u5b66\u6027\u80fd\u3002\u5728\u4e00\u5b9a\u6e29\u5ea6\u65f6\u6548\u540e, \u5177\u6709L<\/i><\/em>12<\/sub>\u6709\u5e8f\u7ed3\u6784\u7684Ni3<\/sub>(Al,Ti)\u578b\u7b2c\u4e8c\u76f8\u5728\u9762\u5fc3\u7acb\u65b9(FCC)\u57fa\u4f53\u4e2d\u5747\u5300\u6790\u51fa, \u5e76\u4e0eFCC\u57fa\u4f53\u5171\u683c\u3002\u901a\u8fc7\u70ed\u673a\u68b0\u5904\u7406\u8fc7\u7a0b, \u5408\u91d1\u7684\u5c48\u670d\u5f3a\u5ea6\u4ece338.3\u2005MPa\u589e\u52a0\u52301355.9\u2005MPa, \u6297\u62c9\u5f3a\u5ea6\u4ece759.3\u2005MPa\u589e\u52a0\u52301488.1\u2005MPa, \u800c\u4f38\u957f\u7387\u4ecd\u7136\u4fdd\u6301\u57288.1%\u3002\u57fa\u4e8e\u5206\u6790\u6a21\u578b\u5b9a\u91cf\u8bc4\u4f30\u5c48\u670d\u5f3a\u5ea6\u7684\u589e\u52a0, \u7ed3\u679c\u8868\u660e\u5c48\u670d\u5f3a\u5ea6\u7684\u663e\u8457\u589e\u52a0\u4e3b\u8981\u662f\u7531\u6c89\u6dc0\u5f3a\u5316\u673a\u5236\u5f15\u8d77\u7684\u3002\u53d8\u5f62\u5f15\u8d77\u7684\u5fae\u89c2\u6761\u5e26\u548c\u4f4d\u9519\u5207\u8fc7\u6790\u51fa\u76f8\u662f\u8be5\u5408\u91d1\u7684\u53d8\u5f62\u673a\u5236\u548c\u5f3a\u5316\u673a\u5236, \u6709\u52a9\u4e8e\u8be5\u5408\u91d1\u540c\u65f6\u5177\u6709\u4f18\u5f02\u7684\u5ef6\u5c55\u6027\u548c\u9ad8\u5f3a\u5ea6\u3002\u00a0\u7814\u7a76\u8868\u660e, CALPHAD\u65b9\u6cd5\u53ef\u4ee5\u4e3a\u9ad8\u71b5\u5408\u91d1\u7684\u8bbe\u8ba1\u548c\u4f18\u5316\u63d0\u4f9b\u501f\u9274\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cCALPHAD-aided design of high entropy alloy to achieve high strength via precipitate strengthening\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728SCIENCE CHINA Materials\u4e0a\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/p>\n

DOI: 10.1007\/s40843-019-1170-7<\/p>\n

\u4e0d\u540c\u70ed\u673a\u68b0\u8fc7\u7a0b\u540e\u7684\u7c92\u5ea6\u6f14\u5316<\/p>\n

\"\"<\/p>\n

Science China Chemistry<\/b><\/strong>\u00a0<\/b><\/strong>\u00a0<\/b><\/strong><\/p>\n

\u5229\u7528AIE\u6d3b\u6027\u5355\u5143\u6784\u5efa\u7684\u5171\u4ef7\u6709\u673a\u7a7a\u5fc3\u7eb3\u7c73\u7403\u7528\u4e8e\u785d\u57fa\u915a\u7c7b\u7206\u70b8\u7269\u7684\u68c0\u6d4b<\/b><\/strong><\/p>\n

\u5177\u6709\u9ad8\u7075\u654f\u5ea6\u548c\u8d85\u653e\u5927\u731d\u706d\u6548\u5e94\u7684\u5171\u8f6d\u7eb3\u7c73\u6750\u6599\u5bf9\u785d\u57fa\u915a\u7c7b\u7206\u70b8\u7269\u7684\u68c0\u6d4b\u4ecd\u662f\u4e00\u4e2a\u5de8\u5927\u7684\u6311\u6218\u3002\u5728\u6b64\uff0c\u5409\u6797\u5927\u5b66\u7530\u6587\u6676\u3001\u5218\u4fca\u79cb\u6559\u6388\u5f00\u53d1\u4e86\u5229\u7528\u805a\u5408\u8bf1\u5bfc\u53d1\u5c04(AIE)\u6d3b\u6027TFPB\u6784\u5efa\u7684\u5171\u8f6d\u7a7a\u5fc3\u7eb3\u7c73\u7403\u3002\u7531\u4e8e\u7a7a\u82af\u7eb3\u7c73\u7403\u4e0e\u785d\u57fa\u915a\u7c7b\u70b8\u836f\u7684\u5149\u81f4\u7535\u5b50\u8f6c\u79fb(PET)\uff0c\u4f7f\u5f97\u7a7a\u82af\u7eb3\u7c73\u7403\u5728\u52a0\u5165\u785d\u57fa\u915a\u7c7b\u70b8\u836f\u540e\u5177\u6709\u5747\u5300\u7684\u5c3a\u5bf8\u548c\u826f\u597d\u7684\u5206\u6563\u6027\uff0c\u5e76\u8868\u73b0\u51fa\u660e\u663e\u7684\u8367\u5149\u731d\u706d\u53cd\u5e94\u3002 \u70b8\u836f\u7269\uff1aTNP\u30014-\u785d\u57fa\u915a(NP)\u548c2,4-\u4e8c\u785d\u57fa\u82ef\u915a(DNP)\u4e0e\u7a7a\u5fc3\u7403\u7684Stern-Volmer\u5e38\u6570\u53ef\u5206\u522b\u8fbe\u52309.67\u00d7105<\/sup>\u30013.14\u00d7105<\/sup>\u548c4.8\u00d7104<\/sup>\u00a0M\u22121<\/sup>\u3002\u5236\u5907\u4e86\u7a7a\u5fc3\u7eb3\u7c73\u7403\u5305\u8986\u7684\u7b80\u6613\u8bd5\u7eb8\uff0c\u5bf9TNP\u6eb6\u6db2\u548c\u6c34\u84b8\u6c14\u7684\u54cd\u5e94\u826f\u597d\u3002\u8be5\u7814\u7a76\u4e3a\u6784\u5efa\u9ad8\u6548\u785d\u57fa\u915a\u7c7b\u7206\u70b8\u7269\u4f20\u611f\u7684AIE \u5171\u8f6d\u7a7a\u5fc3\u7eb3\u7c73\u7403\u63d0\u4f9b\u4e86\u4e00\u79cd\u65b0\u7684\u7b56\u7565\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cCovalent organic hollow nanospheres constructed by using AIE-active units for nitrophenol explosives detection\u201d\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Science China Chemistry\u4e0a\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/p>\n

DOI: 10.1007\/s11426-019-9667-1<\/p>\n

\u7a7a\u5fc3\u7eb3\u7c73\u7403\u7684\u5f62\u6210\u53ca\u5728\u785d\u57fa\u915a\u7c7b\u7206\u70b8\u7269\u68c0\u6d4b\u4e2d\u7684\u5e94\u7528<\/p>\n

\"\"<\/p>\n

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\u975e\u5bcc\u52d2\u70ef\u53d7\u4f53(NFA)\u7684\u51fa\u73b0\u4e3a\u5f00\u53d1\u5177\u6709\u9ad8\u529f\u7387\u8f6c\u6362\u6548\u7387\u7684\u9ad8\u6027\u80fd\u65bd\u4e3b\/\u53d7\u4f53\u5bf9\u63d0\u4f9b\u4e86\u4e00\u4e2a\u6709\u5e0c\u671b\u7684\u673a\u4f1a\uff0c\u56e0\u4e3aNFAs\u63d0\u4f9b\u53ef\u8c03\u7684\u80fd\u91cf\u6c34\u5e73\u3001\u5e7f\u6cdb\u7684\u5438\u6536\u548c\u5408\u9002\u7684\u805a\u96c6\u7279\u6027\u3002\u4e3a\u4e86\u63d0\u9ad8\u6d3b\u6027\u5c42\u7684\u5438\u5149\u80fd\u529b\uff0c\u82cf\u5dde\u5927\u5b66\u5d14\u8d85\u534e\u6559\u6388\u3001\u674e\u6c38\u822b\u9662\u58eb\u7b49\u4eba\u9009\u62e9\u5bbd\u7981\u5e26\u805a\u5408\u7269PTQ10\u4f5c\u4e3a\u4f9b\u4f53\uff0c\u800c\u7a84\u7981\u5e26NFA Y6\u4f5c\u4e3a\u53d7\u4f53\u3002\u4e0ePTQ10: IDIC\u5171\u6df7\u7269\u76f8\u6bd4\uff0c\u5728PTQ10:Y6\u5171\u6df7\u7269\u4e2d\u89c2\u5bdf\u5230\u7ea6130 nm\u7684\u7ea2\u79fb\u5438\u6536\u5149\u8c31\uff0c\u8fd9\u53ef\u80fd\u4f1a\u589e\u5f3aPSCs\u7684\u77ed\u8def\u7535\u6d41\u5bc6\u5ea6(Jsc)\u3002\u6b64\u5916\uff0c\u6700\u4f73PTQ10:Y6\u5171\u6df7\u7269\u5177\u6709\u66f4\u9ad8\u7684\u5149\u81f4\u53d1\u5149\u731d\u706d\u6548\u7387\u548c\u66f4\u9ad8\u6548\u7684\u7535\u8377\u5206\u79bb\uff0c\u5177\u6709\u66f4\u9ad8\u7684\u7535\u8377\u6d41\u52a8\u6027\uff0c\u5176\u53cc\u5206\u5b50\u590d\u5408\u80fd\u529b\u8f83\u5f31\uff0c\u529f\u7387\u8f6c\u6362\u6548\u7387(PCE)\u4e3a16.53%\uff0cJsc\u4e3a26.65 mA cm\u22122<\/sup>\uff0c\u586b\u5145\u7cfb\u6570(FF)\u4e3a0.751\u3002\u76f8\u5173\u7814\u7a76\u4ee5\u201cRationally pairing photoactive materials for high-performance polymer solar cells with efficiency of 16.53%\u201c\u4e3a\u9898\u76ee\uff0c\u53d1\u8868\u5728Science China Chemistry\u4e0a\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/p>\n

DOI: 10.1007\/s11426-019-9599-1<\/p>\n

PSC\u7684\u5668\u4ef6\u7ed3\u6784\u53ca\u5728\u8584\u819c\u4e2d\u7684\u5f52\u4e00\u5316\u5438\u6536\u5149\u8c31<\/p>\n

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\u672c\u6587\u7531Junas\u4f9b\u7a3f\u3002<\/p>\n

\u672c\u5185\u5bb9\u4e3a\u4f5c\u8005\u72ec\u7acb\u89c2\u70b9\uff0c\u4e0d\u4ee3\u8868\u6750\u6599\u4eba\u7f51\u7acb\u573a\u3002<\/p>\n

\u672a\u7ecf\u5141\u8bb8\u4e0d\u5f97\u8f6c\u8f7d\uff0c\u6388\u6743\u4e8b\u5b9c\u8bf7\u8054\u7cfbkefu@cailiaoren.com\u3002<\/p>\n

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