{"id":199801,"date":"2020-04-24T06:25:36","date_gmt":"2020-04-23T22:25:36","guid":{"rendered":"\/\/m.iemloyee.com\/?p=199801"},"modified":"2020-04-23T21:25:57","modified_gmt":"2020-04-23T13:25:57","slug":"%e5%8c%97%e8%88%aa%e6%b0%b4%e6%b1%9f%e6%be%9c%e5%9b%a2%e9%98%9fadv-energy-mater-%ef%bc%9a%e7%94%a8%e4%ba%8e%e6%b0%a7%e8%bf%98%e5%8e%9f%e5%8f%8d%e5%ba%94%e5%92%8cpem%e7%87%83%e6%96%99%e7%94%b5","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=199801","title":{"rendered":"\u5317\u822a\u6c34\u6c5f\u6f9c\u56e2\u961fAdv. Energy Mater.\uff1a\u7528\u4e8e\u6c27\u8fd8\u539f\u53cd\u5e94\u548cPEM\u71c3\u6599\u7535\u6c60\u7684\u8d35\u91d1\u5c5e\u5355\u539f\u5b50\u50ac\u5316\u5242\u7684\u987a\u5e8f\u5408\u6210\u548c\u6d3b\u6027\u4f4d\u70b9\u914d\u4f4d\u539f\u5219"},"content":{"rendered":"

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c\uff09H2<\/sub>-air PEMFC\u4e2dIr1<\/sub>-N\/C\u7684\u6781\u5316\u66f2\u7ebf\u548c\u529f\u7387\u5bc6\u5ea6\u56fe\u3002H2<\/sub>\/air 2 bar\uff0c80\u2103\uff0c100\uff05RH\uff0c5 cm2<\/sup>\u5355\u4f53\u7535\u6c60\u3002<\/p>\n

\u3010\u5c0f\u7ed3<\/b><\/strong>\u3011<\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u8be5\u56e2\u961f\u53d1\u660e\u4e86\u4e00\u79cd\u987a\u5e8f\u914d\u4f4d\u6cd5\uff0c\u53ef\u5c06\u5927\u91cf\u8d35\u91d1\u5c5e\u79bb\u5b50\u63ba\u6742\u5230ZIF\u4e2d\uff0c\u5408\u6210\u78b3\u8f7d\u6c2e\u914d\u4f4d\u7684Ir\u3001Rh\u3001Pt\u548cPd SACs\uff0c\u4e0e\u5176\u4ed6ZIF\u57fa\u7684SACs\u76f8\u6bd4\uff0c\u5b9e\u73b0\u4e86\u6700\u9ad8\u7684\u8d35\u91d1\u5c5e\u8d1f\u8f7d\u3002Ir1<\/sub>-N\/C\u548cRh1<\/sub>-N\/C\u7684ORR\u6d3b\u6027\u660e\u663e\u9ad8\u4e8eIr\u548cRh NPs\uff1b\u800cPd1<\/sub>-N\/C\u548cPt1<\/sub>-N\/C\u7684\u6d3b\u6027\u5219\u4f4e\u4e8ePd\u548cPt NPs\u3002DFT\u8ba1\u7b97\u8868\u660ePM SACs\u7684ORR\u6d3b\u6027\u53d6\u51b3\u4e8e\u914d\u4f4d\u9634\u79bb\u5b50\u7684\u7535\u8d1f\u6027\u4e0ePM\uff08111\uff09\u8868\u9762\u5bf9OH*\u7684\u5438\u9644\u80fd\u0394GOH*<\/sub>\u3002\u5177\u6709\u5f3aOH*\u5438\u9644\u529b\u7684\u91d1\u5c5e\u9700\u8981\u9ad8\u7535\u8d1f\u6027\u914d\u4f4d\u9634\u79bb\u5b50\uff1b\u800c\u5bf9OH*\u5438\u9644\u5f31\u7684\u91d1\u5c5e\u9700\u8981\u5339\u914d\u4f4e\u7535\u8d1f\u6027\u914d\u4f4d\u9634\u79bb\u5b50\u3002\u672c\u6587\u63ed\u793a\u7684\u5355\u539f\u5b50\u6d3b\u6027\u4f4d\u70b9\u914d\u4f4d\u539f\u7406\u4e3a\u8bbe\u8ba1\u9002\u7528\u4e8e\u9178\u6027ORR\u548cPEMFCs\u7684\u8d35\u91d1\u5c5eSACs\u63d0\u4f9b\u4e86\u6307\u5bfc\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>Sequential Synthesis and Active<\/u>–<\/u>Site Coordination Principle of Precious Metal Single<\/u>–<\/u>Atom Catalysts for Oxygen Reduction Reaction and PEM Fuel Cells<\/u><\/a>\uff08Adv. Energy Mater.\uff0c 2020\uff0cDOI:10.1002\/aenm.202000689\uff09<\/p>\n

\u3010\u56e2\u961f\u4ecb\u7ecd<\/b><\/strong>\u3011<\/p>\n

\u6c34\u6c5f\u6f9c\u6559\u6388<\/strong>\u8bfe\u9898\u7ec4\uff08\u5317\u4eac\u822a\u7a7a\u822a\u5929\u5927\u5b66\u6750\u6599\u5b66\u9662\uff09\u81ea2015\u5e74\u6210\u7acb\u4ee5\u6765\uff0c\u81f4\u529b\u4e8e\u6c22\u80fd\u76f8\u5173\u6750\u6599\u7684\u7814\u7a76\uff0c\u5305\u62ec\u7535\u5236\u6c22\u50ac\u5316\u5242\u3001\u50a8\u6c22\u6750\u6599\u3001\u8d28\u5b50\u819c\u71c3\u6599\u7535\u6c60\u50ac\u5316\u5242\u3002\u5728\u71c3\u6599\u7535\u6c60\u50ac\u5316\u5242\u65b9\u9762\uff0c\u56f4\u7ed5\u5982\u4f55\u63d0\u9ad8\u975e\u94c2\u50ac\u5316\u5242\u6d3b\u6027\u548c\u7a33\u5b9a\u6027\u5f00\u5c55\u6df1\u5165\u3001\u7cfb\u7edf\u7684\u7814\u7a76\uff0c\u63d0\u51fa\u82e5\u5e72\u79cdFe-N-C\u50ac\u5316\u5242\u6027\u80fd\u589e\u5f3a\u673a\u5236\uff0c\u9996\u6b21\u8fbe\u5230\u4e86\u7f8e\u56fd\u80fd\u6e90\u90e8\u975ePt\u50ac\u5316\u52422018\u5e74\u6d3b\u6027\u76ee\u6807\u3010Nat.\u00a0Catal.\u00a02019,\u00a02,\u00a0259-268\u3011\u3002\u4e0e\u672c\u8bfe\u9898\u76f8\u5173\u7684\u7eff\u8272\u56fa\u76f8\u5408\u6210\u5de5\u827a\u8fd8\u7528\u4e8e\u5236\u5907Fe-N-C\u5355\u539f\u5b50\u50ac\u5316\u5242\uff0c\u5728\u8d28\u5b50\u819c\u71c3\u6599\u7535\u6c60\u4e2d\u5c55\u73b0\u51fa\u9ad8\u529f\u7387\u5bc6\u5ea6\u3010Angew.\u00a0Chem.\u00a0Int.\u00a0Ed.,\u00a02018,\u00a057,\u00a01204-1208\u3011\uff1b\u56fa\u76f8\u5408\u6210\u6cd5\u8fd8\u6210\u529f\u5236\u5907\u4e86\u7a00\u571fY\u548cSc\u5355\u539f\u5b50\u50ac\u5316\u5242\uff0c\u662f\u7a00\u571f\u5355\u539f\u5b50\u50ac\u5316\u5242\u7684\u9996\u6b21\u62a5\u9053\u3010ACS\u00a0Nano\u00a02020,\u00a014,\u00a01093-1101\u3011\u3002\u5728\u975e\u91d1\u5c5e\u50ac\u5316\u5242\u4e0a\uff0c\u62a5\u9053\u4e86\u9ad8\u6548\u7a33\u5b9a\u7684\u4e4b\u5b57\u5f62\u78b3\u50ac\u5316\u5242\u3010Nat. Commun. <\/i><\/em>2018,<\/b><\/strong>\u00a09<\/i><\/em>, 3819\u3011\u3002<\/p>\n

\u6c34\u6c5f\u6f9c\u8bfe\u9898\u7ec4\u8fd1\u671f\u53d1\u8868\u7684\u90e8\u5206\u5b66\u672f\u8bba\u6587:<\/p>\n

    \n
  1. Wan, X. F. Liu, Y. C. Li, R. H. Yu, L. R. Zheng, W. S. Yan, H. Wang, M. Xu,*<\/b><\/strong>J. L. Shui.*<\/b><\/strong>\u00a0Fe\u2013N\u2013C Electrocatalyst with Dense Active Sites and Efficient Mass Transport for High-performance Proton Exchange Membrane Fuel Cells, Nat<\/i><\/b><\/em><\/strong>.<\/i><\/b><\/em><\/strong>\u00a0Catal.<\/i><\/b><\/em><\/strong>\u00a02019, 2, 259-268.\u00a0<\/b><\/strong><\/li>\n
  2. F. Xue, Y. C. Li, X. F. Liu, Q. T. Liu, J. X. Shang, H. P. Duan,*<\/b><\/strong>L.M. Dai,*<\/b><\/strong>\u00a0J. L. Shui.* \u201cZigzag carbon as efficient and stable oxygen\u00a0reduction electrocatalyst for proton exchange\u00a0membrane fuel cells\u201d Nat. Commun.<\/i><\/b><\/u><\/em><\/strong>\u00a02018, 9:3819.<\/li>\n
  3. -T. Liu, Y.-C. Li, L.-R. Zheng, J.-X. Shang, X.-F. Liu, R.-H. Yu, J.-L. Shui*. Sequential Synthesis and Active-Site Coordination Principle of Precious Metal Single-Atom Catalysts for Oxygen Reduction Reaction and PEM Fuel Cells, Adv. Energy Mater.<\/i><\/b><\/em><\/strong>2020, DOI.\u00a010.1002\/aenm.202000689.<\/li>\n
  4. J. Zeng, J.L. Shui,* X.F. Liu, Q.T. Liu, Y.C. Li, J.X. Shang, L.R. Zheng,* R.H. Yu.* Single-Atom to Single-Atom Grafting of Pt1<\/sub>onto Fe\u2212N4<\/sub>\u00a0Center: Pt1<\/sub>@Fe\u2212N\u2212C Multifunctional Electrocatalyst with Significantly Enhanced Properties\u201d\u00a0Adv<\/i><\/b><\/u><\/em><\/strong>.<\/i><\/b><\/u><\/em><\/strong>\u00a0Energy Mater<\/i><\/b><\/u><\/em><\/strong>.<\/i><\/b><\/u><\/em><\/strong>\u00a02018, 8, 1701345.<\/li>\n
  5. T. Liu,X. F. Liu,* L. R. Zheng, and J. L. Shui* “The Solid-Phase Synthesis of an Fe-N-C Electrocatalyst for High Power Proton-Exchange Membrane Fuel Cells”\u00a0Angew. Chem. Int. Ed.<\/i><\/b><\/u><\/em><\/strong>, 2018, 57, 1204 \u20131208.<\/li>\n
  6. Y. Chen, X. F. Liu, L. Zheng, Y. Li, X. Guo, X. Wan, Q.T. Liu, J. X. Shang, J. L. Shui*<\/b><\/strong>Insights into the Role of Active Site Density in the Fuel Cell Performance of Co-N-C Catalysts, App<\/i><\/b><\/em><\/strong>l.<\/i><\/b><\/em><\/strong>\u00a0Cata<\/i><\/b><\/em><\/strong>l.<\/i><\/b><\/em><\/strong>\u00a0B<\/i><\/b><\/em><\/strong>–<\/i><\/b><\/em><\/strong>Environ<\/i><\/b><\/em><\/strong>.<\/i><\/b><\/em><\/strong>\u00a02019, 256, 117849.<\/li>\n
  7. Y. Liu, X. Kong, L. R. Zheng, X. Guo, X. F. Liu, J.L. Shui*. Rare Earth Single Atom Catalysts for Nitrogen and Carbon Dioxide Reduction. ACS Nano<\/i><\/b><\/em><\/strong>2020, 14(1), 1093-1101.\u00a0<\/li>\n
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  10. Y. Zhu, Q.T. Liu, X.F. Liu, J.L. Shui*. Temperature Impacts on Oxygen Reduction Reaction Measured by the Rotating Disk Electrode Technique. J. Phys. Chem. C<\/i><\/b><\/em><\/strong>2020, 124, 3069\u22123079.<\/li>\n
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  12. X. Wang, J. Ren, X. Gao, W.J. Zhang, H.P. Duan, M. Wang, J.L. Shui,* M. Xu,* Self-Adaptive Electrode with SWCNT Bundles as Elastic Substrate for High-Rate and Long-Cycle-Life Lithium\/Sodium Ion BatteriesSmall<\/i><\/b><\/u><\/em><\/strong>\u00a02018, 1802913.<\/li>\n<\/ol>\n

    \u672c\u6587\u7531\u6728\u6587\u97ec<\/b><\/strong>\u7ffb\u8bd1\u7f16\u8f91\u3002<\/p>\n

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