{"id":199581,"date":"2020-04-28T06:28:27","date_gmt":"2020-04-27T22:28:27","guid":{"rendered":"\/\/m.iemloyee.com\/?p=199581"},"modified":"2020-04-27T21:28:40","modified_gmt":"2020-04-27T13:28:40","slug":"%e9%a2%84%e8%a8%80%e4%b8%8e%e9%87%91%e5%88%9a%e7%9f%b3%e7%9b%b8%e5%aa%b2%e7%be%8e-%e6%b0%ae%e5%8c%96%e7%a2%b3%e6%9c%80%e6%96%b0%e6%88%90%e6%9e%9c%e9%80%9f%e9%80%92","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=199581","title":{"rendered":"\u9884\u8a00\u4e0e\u91d1\u521a\u77f3\u76f8\u5ab2\u7f8e \/ \u6c2e\u5316\u78b3\u6700\u65b0\u6210\u679c\u901f\u9012"},"content":{"rendered":"

\u6c2e\u5316\u78b3(C3<\/sub>N4<\/sub>)\u662f\u8fd1\u5e74\u6765\u65b0\u5174\u7684\u4e00\u79cd\u78b3\u6750\u6599\uff0c\u5176\u7531\u78b3\u548c\u6c2e\u7684\u5355\u539f\u5b50\u8fdb\u884csp2<\/sup>\u6742\u5316\u5f62\u6210\uff0c\u5177\u6709\u72ec\u7279\u7684\u5e73\u9762\u7ed3\u6784\u3001\u826f\u597d\u7684\u7535\u5b66\u3001\u5149\u5b66\u548c\u7269\u7406\u5316\u5b66\u6027\u8d28\uff0c\u4e14\u5236\u5907\u5de5\u827a\u7b80\u5355\u3001\u6210\u672c\u8f83\u4f4e\uff0c\u5f15\u8d77\u4e86\u7535\u5316\u5b66\u50a8\u80fd\u9886\u57df\u7814\u7a76\u4eba\u5458\u7684\u5f3a\u70c8\u5174\u8da3\u3002\u5176\u4e2d\uff0c\u77f3\u58a8\u76f8\u6c2e\u5316\u78b3(g-C3<\/sub>N4<\/sub>)\u662f\u4e00\u79cd\u65b0\u578b\u7684\u975e\u91d1\u5c5e\u5149\u50ac\u5316\u6750\u6599\uff0c\u5728\u53ef\u89c1\u5149\u8303\u56f4\u5185\u5177\u6709\u4e00\u5b9a\u7684\u5149\u5438\u6536\uff0c\u540c\u65f6\u8fd8\u5177\u6709\u5f88\u597d\u7684\u70ed\u7a33\u5b9a\u6027\u3001\u5316\u5b66\u7a33\u5b9a\u6027\u548c\u5149\u7a33\u5b9a\u6027\uff0c\u88ab\u5e7f\u6cdb\u5e94\u7528\u4e8e\u5149\u50ac\u5316\u4ea7\u6c22\u3001\u6c34\u6c27\u5316\u3001\u6709\u673a\u7269\u964d\u89e3\u3001\u5149\u5408\u6210\u4ee5\u53ca\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\u7b49\u3002\u672c\u6587\u603b\u7ed3\u4e86\u79d1\u7814\u754c\u5b66\u672f\u5927\u725b\u5728\u6c2e\u5316\u78b3\u9886\u57df\u7684\u6700\u65b0\u6210\u679c\uff0c\u5e0c\u671b\u5bf9\u4ece\u4e8b\u6c2e\u5316\u78b3\u6750\u6599\u76f8\u5173\u9886\u57df\u7684\u4f60\u6709\u6240\u542f\u53d1\u3002<\/p>\n

\u738b\u5fc3\u6668\uff08\u798f\u5dde\u5927\u5b66\uff09<\/b><\/strong><\/p>\n

1. Angew. Chem. Int. Ed. \u6c2e\u5316\u78b3\u6676\u754c\u5316\u5b66\u7528\u4ee5\u589e\u5f3a\u592a\u9633\u80fd\u4ea7\u6c22\u548c\u8fd8\u539f\u4e8c\u6c27\u5316\u78b3<\/b><\/strong><\/p>\n

\u5149\u50ac\u5316\u6c34\u5206\u89e3\u662f\u4ee5\u53ef\u6301\u7eed\u65b9\u5f0f\u6a21\u62df\u690d\u7269\u5149\u5408\u4f5c\u7528\u7684\u6709\u524d\u9014\u6e05\u6d01\u65b9\u6cd5\u4e4b\u4e00\u3002\u5728\u53ef\u884c\u8303\u56f4\u5185\u63d0\u9ad8\u91cf\u5b50\u6548\u7387\u548c\u5149\u5438\u6536\u662f\u63a5\u8fd1\u5b9e\u7528\u6027\u7684\u5fc5\u8981\u6b65\u9aa4\u3002\u798f\u5dde\u5927\u5b66\u738b\u5fc3\u6668\u8bfe\u9898\u7ec4\u62a5\u9053\u4e86\u4f7f\u7528\u9ad8\u6c2e\u542b\u91cf\u7684\u5355\u4f535-\u6c28\u57fa\u56db\u5511\u5408\u6210\u6c2e\u5316\u78b3\u53ef\u4ee5\u63d0\u9ad8\u91cf\u5b50\u6548\u7387\u548c\u5149\u5438\u6536\u7528\u4e8e\u589e\u5f3a\u592a\u9633\u80fd\u4ea7\u6c22\u548c\u8fd8\u539f\u4e8c\u6c27\u5316\u78b3\u3002\u7194\u878d\u76d0\u6df7\u5408\u7269NaCl \/ KCl\u7528\u4f5c\u9ad8\u6e29\u6eb6\u5242\u4ee5\u8c03\u6574\u6676\u754c\u7ed3\u6784\u548c\u5316\u5b66\u6027\u8d28\u3002\u5728\u53cc\u5c42\u6539\u6027\u5242\uff08K2<\/sub>HPO4<\/sub>\uff09\u7684\u5b58\u5728\u4e0b\uff0c\u4ea7\u6c22\u7684\u53ef\u89c1\u5149\u91cf\u5b50\u6548\u7387\u4e3a0.65\u3002\u8be5\u7b56\u7565\u53ef\u4ee5\u5408\u6210\u4e00\u79cd\u9ad8\u6548\u7684\u5149\u50ac\u5316\u5242\uff0c\u4ee5\u8c03\u8282\u7ed3\u6676\u5ea6\u3001\u6676\u754c\u7ed3\u6784\u548c\u5316\u5b66\u6027\u8d28\uff0c\u8fd9\u662f\u663e\u7740\u589e\u5f3a\u5149\u5438\u6536\u548c\u7535\u5b50\u6027\u80fd\u662f\u5149\u50ac\u5316\u6027\u80fd\u7684\u4e3b\u8981\u539f\u56e0\u3002\u8fd9\u9879\u7814\u7a76\u4e3a\u83b7\u5f97\u5177\u6709\u4f18\u5316\u6027\u80fd\u548c\u589e\u5f3a\u6d3b\u6027\u7684\u7ec4\u7ec7\u826f\u597d\u7684\u6c2e\u5316\u78b3\u63d0\u4f9b\u4e86\u65b0\u601d\u8def\u3002[1]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cTailoring the Grain Boundary Chemistry of Polymeric Carbon Nitride\u00a0for Enhanced Solar Hydrogen Production and CO2<\/sub>\u00a0Reduction\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Angew. Chem. Int. Ed.\u3002<\/p>\n

\u56fe\u4e00\uff1a\u4e00\u9505\u6cd5\u5408\u6210\u6c2e\u5316\u78b3\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

2. ChemSusChem<\/b><\/strong>\u8d85\u5206\u5b50\u9884\u7ec4\u88c5\u8c03\u8282\u6c2e\u5316\u78b3\u5149\u50ac\u5316\u4ea7\u6c22<\/b><\/strong><\/p>\n

\u901a\u8fc7\u8bbe\u8ba1\u8fdb\u884c\u8d85\u5206\u5b50\u9884\u7ec4\u88c5\u4ee5\u9002\u5e94\u6c2e\u5316\u78b3\u7684\u7269\u7406\u5316\u5b66\u6027\u8d28\u662f\u63d0\u9ad8\u592a\u9633\u80fd\u8f6c\u5316\u6027\u80fd\u7684\u4e00\u79cd\u6709\u6548\u7b56\u7565\u3002\u798f\u5dde\u5927\u5b66\u738b\u5fc3\u6668\u8bfe\u9898\u7ec4\u62a5\u9053\u4e86\u4f7f\u7528\u6c34\u4f5c\u4e3a\u81ea\u7ec4\u88c5\u4ecb\u8d28\u3001\u8fc7\u786b\u9178\u94a0\u4f5c\u4e3a\u6539\u6027\u5242\u7684\u4e00\u79cd\u65b0\u7684\u8d85\u5206\u5b50\u9884\u7ec4\u88c5\u8fc7\u7a0b\uff0c\u4ee5\u8c03\u8282\u6c2e\u5316\u78b3\u7684\u6784\u6210\u548c\u5149\u7535\u7279\u6027\uff0c\u5b9e\u73b0\u6709\u6548\u7684\u53ef\u89c1\u5149\u4ea7\u6c22\u3002\u8fc7\u786b\u9178\u94a0\u53ef\u4ee5\u7cbe\u786e\u5730\u63a7\u5236\u6c2e\u5316\u78b3\u5177\u6709\u8f83\u591a\u7684\u591a\u5b54\u5c42\u72b6\u7ed3\u6784\uff0c\u5e76\u4fc3\u8fdb\u7535\u8377\u5206\u79bb\u548c\u8fc1\u79fb\u52a8\u529b\u5b66\u3002\u4e0e\u884d\u751f\u81ea\u65e0\u6539\u6027\u5242\u7684\u4e09\u805a\u6c30\u80fa\u7684\u7c7b\u4f3c\u7269\u76f8\u6bd4\uff0c\u5177\u6709\u4f18\u5316\u7ed3\u6784\u548c\u5904\u7406\u5f97\u5230\u7684\u6c2e\u5316\u78b3\u5177\u6709\u663e\u7740\u4e30\u5bcc\u7684\u5149\u50ac\u5316\u4ea7\u6c22\u6d3b\u6027\u3002\u8fd9\u9879\u5de5\u4f5c\u53ef\u80fd\u4e3a\u63a8\u8fdb\u6c2e\u5316\u78b3\u5149\u50ac\u5316\u5242\u5728\u592a\u9633\u80fd\u5230\u5316\u5b66\u80fd\u8f6c\u5316\u5e94\u7528\u4e2d\u7684\u5408\u6210\u3001\u7ed3\u6784\u548c\u6027\u80fd\u63d0\u4f9b\u65b0\u7684\u89c1\u89e3\u3002[2]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cModulation of Polymeric Carbon Nitrides through Supramolecular Preorganization for Efficient\u00a0Photocatalytic Hydrogen Generation\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728ChemSusChem\u3002<\/p>\n

\u56fe\u4e8c\uff1a\u8d85\u5206\u5b50\u7ec4\u88c5\u7b56\u7565\u8c03\u8282\u6c2e\u5316\u78b3\u5408\u6210\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

3. Appl. Catal. B Environ.<\/b><\/strong>\u5149\u523b\u8680\u7684\u6c2e\u7a7a\u4f4d\u6c2e\u5316\u78b3\u7528\u4e8e\u65e0\u91d1\u5c5e\u6c27\u6790\u51fa\u53cd\u5e94<\/b><\/strong><\/p>\n

\u5149\u50ac\u5316\u6c34\u5206\u89e3\u9700\u8981\u52a9\u50ac\u5316\u5242\u6765\u52a0\u901f\u6c27\u6790\u51fa\u53cd\u5e94\uff08OER\uff09\uff0c\u4f46\u5927\u591a\u6570OER\u52a9\u50ac\u5316\u5242\u5747\u57fa\u4e8e\u8d35\u91d1\u5c5e\u6c27\u5316\u7269\uff0c\u5e76\u4e14\u534a\u5bfc\u4f53\u548c\u52a9\u50ac\u5316\u5242\u4e4b\u95f4\u7684\u677e\u6563\u754c\u9762\u5bfc\u81f4\u7535\u8377\u8f6c\u79fb\u6548\u7387\u4f4e\u4e0b\uff0c\u5f00\u53d1\u96c6\u6210\u7684\u5149\u5438\u6536\u548c\u50ac\u5316\u4e2d\u5fc3\u7684\u5149\u50ac\u5316\u5242\u7528\u4e8eOER\u5177\u6709\u91cd\u8981\u610f\u4e49\u3002\u798f\u5dde\u5927\u5b66\u738b\u5fc3\u6668\u8bfe\u9898\u7ec4\u63d0\u51fa\u4e86\u4e00\u79cd\u5149\u523b\u8680\u7b56\u7565\u7528\u4e8e\u5728\u6c2e\u5316\u78b3\u4e0a\u4ea7\u751f\u6c2e\u7a7a\u4f4d\u3002\u5d4c\u5165\u7684\u6c2e\u7a7a\u4f4d\u53ef\u4ee5\u5145\u5f53\u50ac\u5316OER\u7684\u6d3b\u6027\u4f4d\u70b9\uff0c\u540c\u65f6\u4fc3\u8fdbOER\u7684\u5149\u751f\u7535\u8377\u7684\u8f6c\u79fb\u3002\u4e0e\u666e\u901a\u6c2e\u5316\u78b3\u76f8\u6bd4\uff0c\u6ca1\u6709\u4efb\u4f55\u8d35\u91d1\u5c5e\u52a9\u50ac\u5316\u5242\u8f85\u52a9\u7684\u6c2e\u7a7a\u4f4d\u6c2e\u5316\u78b3\u8868\u73b0\u51fa\u66f4\u9ad8\u7684\u6c27\u6c14\u6790\u51fa\u901f\u7387\u3002\u4ece\u5176\u4ed6\u524d\u4f53\u83b7\u5f97\u7684\u6c2e\u5316\u78b3\u4e5f\u53ef\u4ee5\u901a\u8fc7\u8fd9\u79cd\u5149\u523b\u8680\u65b9\u6cd5\u8fdb\u884c\u5de5\u7a0b\u5316\uff0c\u540c\u65f6\u4fc3\u8fdb\u5149\u50ac\u5316\u6c27\u6790\u51fa\u53cd\u5e94\u3002\u8be5\u5de5\u4f5c\u4e3a\u8bbe\u8ba1\u5177\u6709\u5149\u6536\u96c6\u548c\u50ac\u5316\u7ed3\u6784\u7ec4\u5408\u7684\u5149\u6362\u80fd\u5668\u7528\u4e8e\u6c27\u6790\u51fa\u53cd\u5e94\u63d0\u4f9b\u4e86\u9014\u5f84\u3002[3]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cPhotocarving nitrogen vacancies in a polymeric carbon nitride for metal-free\u00a0oxygen synthesis\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Appl. Catal. B Environ.\u3002<\/p>\n

\u56fe\u4e09\uff1a\u5149\u523b\u8680\u6c2e\u5316\u78b3\u5f62\u6210\u6c2e\u7a7a\u4f4d\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

4. ChemSusChem<\/b><\/strong>\u7f3a\u9677\u5de5\u7a0b\u63d0\u5347\u7ed3\u6676\u6c2e\u5316\u78b3\u7684\u53ef\u89c1\u5149\u6790\u6c22\u6027\u80fd<\/b><\/strong><\/p>\n

\u7ed3\u6676\u6c2e\u5316\u78b3\u534a\u5bfc\u4f53\u5728\u592a\u9633\u80fd\u8f6c\u6362\u4e2d\u5f15\u8d77\u4e86\u5e7f\u6cdb\u7684\u5173\u6ce8\uff0c\u4f46\u8fdb\u4e00\u6b65\u6539\u53d8\u7ed3\u6676\u6c2e\u5316\u78b3\u7684\u5149\u50ac\u5316\u80fd\u529b\u603b\u662f\u5bfc\u81f4\u9ad8\u7ed3\u6676\u5ea6\u548c\u826f\u597d\u7684\u5149\u50ac\u5316\u6027\u80fd\u4e4b\u95f4\u7684\u6b64\u6d88\u5f7c\u957f\u3002\u798f\u5dde\u5927\u5b66\u738b\u5fc3\u6668\u8bfe\u9898\u7ec4\u62a5\u9053\u4e86\u4e00\u79cd\u53ef\u884c\u7684\u7f3a\u9677\u5de5\u7a0b\u7b56\u7565\u6765\u4fee\u9970\u7ed3\u6676\u6c2e\u5316\u78b3\u5149\u50ac\u5316\u5242\u3002\u7f3a\u9677\u578b\u7684\u7ed3\u6676\u6c2e\u5316\u78b3\u4fdd\u6301\u9ad8\u7ed3\u6676\u5ea6\uff0c\u4ea7\u6c22\u901f\u7387\u6bd4\u7ed3\u6676\u6c2e\u5316\u78b3\u7684\u9ad8\u7ea68\u500d\u3002\u5165\u5c04\u5149\u6ce2\u957f\u6269\u5c55\u5230610 nm\uff0c\u4e5f\u53ef\u4ea7\u6c22\u3002\u7f3a\u9677\u578b\u7684\u7ed3\u6676\u6c2e\u5316\u78b3\u663e\u7740\u6539\u5584\u4e86\u6c2e\u5316\u78b3\u7684\u5149\u50ac\u5316\u6d3b\u6027\u662f\u7531\u4e8e\u5c06\u7f3a\u9677\u5f15\u5165\u7ed3\u6676\u6c2e\u5316\u78b3\u805a\u5408\u7269\u7f51\u7edc\u4ee5\u5f62\u6210\u4e2d\u95f4\u80fd\u9699\u72b6\u6001\uff0c\u4ece\u800c\u663e\u7740\u62d3\u5bbd\u4e86\u53ef\u89c1\u5149\u5438\u6536\u8303\u56f4\u5e76\u52a0\u901f\u4e86\u5149\u6c27\u5316\u8fd8\u539f\u50ac\u5316\u7684\u7535\u8377\u5206\u79bb\u3002\u8fd9\u4e3a\u6539\u5584\u5149\u50ac\u5316\u5242\u7684\u5149\u50ac\u5316\u6027\u80fd\u63d0\u4f9b\u4e00\u79cd\u65b0\u7684\u7b56\u7565\u3002[4]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cEnhancing Visible-Light Hydrogen Evolution Performance\u00a0of Crystalline Carbon Nitride by Defect Engineering\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728ChemSusChem\u3002<\/p>\n

\u56fe\u56db\uff1a\u7ed3\u6676\u6c2e\u5316\u78b3\u7684\u7f3a\u9677\u5de5\u7a0b\u7b56\u7565\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

5. Journal of Catalysis<\/b><\/strong>\u7852\u4fee\u9970\u7684\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u6539\u5584\u5149\u50ac\u5316\u6d3b\u6027<\/b><\/strong><\/p>\n

\u5982\u4f55\u63d0\u5347\u6c2e\u5316\u78b3\u7684\u5149\u50ac\u5316\u6027\u80fd\u662f\u76ee\u524d\u7814\u7a76\u7684\u91cd\u70b9\u4e4b\u4e00\u3002\u798f\u5dde\u5927\u5b66\u738b\u5fc3\u6668\u8bfe\u9898\u7ec4\u901a\u8fc7\u6709\u6548\u7684\u4e24\u6b65\u8fde\u7eed\u70ed\u5904\u7406\u65b9\u6cd5\u5236\u5907\u4e86\u5177\u6709\u7852\u5316\u7269\uff08Se\uff09\u6539\u6027\u7684\u591a\u5b54\u8584\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u7ed3\u6784\u3002\u5728\u53ef\u89c1\u5149\u4e0b\uff0c\u6240\u5236\u5907\u7684\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u663e\u793a\u51fa\u5149\u50ac\u5316\u4ea7\u6c22\u548c\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\u6027\u80fd\uff0c\u5176\u4e2d\u6c22\u6c14\u751f\u6210\u7684\u8868\u89c2\u91cf\u5b50\u4ea7\u7387\u8fbe\u52308.1\uff05\u3002\u51fa\u73b0\u589e\u5f3a\u7684\u5149\u50ac\u5316\u6027\u80fd\u7531\u4e8e\u8f83\u5927\u7684\u8868\u9762\u79ef\u548c\u591a\u5b54\u7684\u7eb3\u7c73\u7ed3\u6784\uff0c\u8fd9\u53ef\u52a0\u901f\u5149\u6fc0\u53d1\u7535\u8377\u8f7d\u4f53\u7684\u5206\u79bb\u5e76\u4fc3\u8fdb\u8d28\u91cf\u8f6c\u79fb\u8fc7\u7a0b\u3002\u5728\u6c2e\u5316\u78b3\u8584\u7247\u4e2dSe\u7684\u5f62\u6210\u8fdb\u4e00\u6b65\u4f7f\u5176\u51cf\u5c0f\u5e26\u9699\uff0c\u66f4\u591a\u7684\u66b4\u9732\u6d3b\u6027\u8fb9\u7f18\u548c\u6269\u5c55\u7684\u53ef\u89c1\u5149\u5438\u6536\u8303\u56f4\u3002\u8be5\u5de5\u4f5c\u4e0d\u4ec5\u63d0\u51fa\u4e86\u4e00\u79cd\u7b80\u5355\u7684\u7b56\u7565\u6765\u589e\u5f3a\u6c2e\u5316\u78b3\u7684\u5149\u50ac\u5316\u6027\u80fd\uff0c\u800c\u4e14\u8fd8\u5229\u7528\u534f\u540c\u6548\u5e94\u4f18\u5316\u4e86\u6c2e\u5316\u78b3\u805a\u5408\u7269\u5149\u50ac\u5316\u5242\u7684\u7535\u5b50\u548c\u9aa8\u67b6\u7ed3\u6784\uff0c\u4e3a\u5408\u7406\u5236\u5907\u6709\u6548\u7684\u6c2e\u5316\u78b3\u805a\u5408\u7269\u5149\u50ac\u5316\u5242\u5f00\u8f9f\u4e86\u4e00\u6761\u65b0\u9014\u5f84\u3002[5]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cSe-modified polymeric carbon nitride nanosheets with improved\u00a0photocatalytic activities\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Journal of Catalysis\u3002<\/p>\n

\u56fe\u4e94\uff1aSe\u6539\u6027\u7684\u6c2e\u5316\u78b3\u7528\u4e8e\u5149\u50ac\u5316\u4ea7\u6c22\u548c\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

6. Angew. Chem. Int. Ed.<\/b><\/strong>\u6c2e\u5316\u78b3\/\u8fd8\u539f\u6c27\u5316\u77f3\u58a8\u70ef\/ Fe<\/b><\/strong>2<\/b><\/sub><\/strong>O<\/b><\/strong>3<\/b><\/sub><\/strong>\u5168\u56fa\u6001Z\u578b\u5f02\u8d28\u7ed3\u7528\u4e8e\u5149\u50ac\u5316\u6c34\u5206\u89e3<\/b><\/strong><\/p>\n

\u8c03\u63a7Z\u578b\u5f02\u8d28\u7ed3\u5149\u50ac\u5316\u6c34\u5206\u89e3\u7cfb\u7edf\u603b\u4f53\u6027\u80fd\u7684\u91cd\u8981\u56e0\u7d20\u662f\u6790\u6c22\u5149\u50ac\u5316\u5242\u548c\u6790\u6c27\u5149\u50ac\u5316\u5242\u4e4b\u95f4\u7684\u7535\u8377\u8f6c\u79fb\u3002\u798f\u5dde\u5927\u5b66\u738b\u5fc3\u6668\u8bfe\u9898\u7ec4\u8bbe\u8ba1\u4e86\u8fd8\u539f\u6c27\u5316\u77f3\u58a8\u70ef\u7eb3\u7c73\u7247\uff08RGO\uff09\u4f5c\u56fa\u6001\u4ecb\u4f53\uff0c\u4ee5\u52a0\u901f\u6790\u6c22\u5149\u50ac\u5316\u5242\uff08\u6c2e\u5316\u78b3\uff09\u548c\u6790\u6c27\u5149\u50ac\u5316\u5242\uff08Fe2<\/sub>O3<\/sub>\uff09\u4e4b\u95f4\u7684\u7535\u8377\u8f7d\u6d41\u5b50\u8f6c\u79fb\uff0c\u4ece\u800c\u53bb\u7684\u6709\u6548\u7684\u6c34\u5206\u89e3\u6027\u80fd\u3002\u901a\u8fc7\u5316\u5b66\u952e\u5408\u548cp\u2013p\u5806\u57fa\u5c06Fe2<\/sub>O3<\/sub>\u7eb3\u7c73\u9897\u7c92\u4e0e\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u8fde\u63a5\uff0c\u5f62\u6210Fe2<\/sub>O3<\/sub>\u00a0\/ RGO \/ \u6c2e\u5316\u78b3\u4e09\u5143\u5f02\u8d28\u7ed3\u63d0\u9ad8\u4e86\u6c34\u7684\u5149\u50ac\u5316\u5206\u89e3\u6548\u7387\u3002\u8fd8\u539f\u6c27\u5316\u77f3\u58a8\u70ef\u7eb3\u7c73\u7247\u7684\u91cd\u8981\u4f5c\u7528\u8fd8\u53ef\u4ee5\u5728\u5176\u4ed6\u57fa\u4e8e\u6c2e\u5316\u78b3\u7684Z\u578b\u5f02\u8d28\u7ed3\u4e2d\u5f97\u5230\u8fdb\u4e00\u6b65\u8bc1\u660e\uff0c\u8fd9\u8bf4\u660e\u4e86\u8be5\u7b56\u7565\u7684\u666e\u904d\u6027\u3002\u8fd9\u9879\u7814\u7a76\u901a\u8fc7\u4f7f\u7528RGO\u4f5c\u4e3a\u7535\u5b50\u4ecb\u4f53\uff0c\u4e3a\u5168\u56fa\u6001Z\u578b\u5f02\u8d28\u7ed3\u7cfb\u7edf\u7684\u6784\u5efa\u63d0\u4f9b\u4e86\u65b0\u7684\u89c1\u89e3\uff0c\u8fd9\u4e5f\u4e3a\u5f00\u53d1\u5176\u4ed6\u7528\u4e8e\u76f8\u5173\u5316\u5b66\u53cd\u5e94\u7684\u56fa\u6001\u7cfb\u7edf\u63d0\u4f9b\u4e86\u673a\u4f1a\u3002[6]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cPolymeric Carbon Nitride\/Reduced Graphene Oxide\/Fe2<\/sub>O3<\/sub>: All-Solid-State Z-Scheme System for Photocatalytic Overall Water Splitting\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Angew. Chem. Int. Ed.\u3002<\/p>\n

\u56fe\u516d\uff1aFe<\/b><\/strong>2<\/b><\/sub><\/strong>O<\/b><\/strong>3<\/b><\/sub><\/strong>\u00a0\/ RGO \/ \u6c2e\u5316\u78b3\u4e09\u5143\u5f02\u8d28\u7ed3\u6784\u5efa\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u5f20\u8881\u5065\uff08\u4e1c\u5357\u5927\u5b66\uff09<\/b><\/strong><\/p>\n

7. Angew. Chem. Int. Ed.<\/b><\/strong>\u7535\u6781\u4e0a\u6c2e\u5316\u78b3\u8d85\u5feb\u901f\u7f29\u5408\u589e\u5f3a\u5149\u7535\u6d41\u548c\u7535\u5316\u5b66\u53d1\u5149\u54cd\u5e94<\/b><\/strong><\/p>\n

\u7531\u4e8e\u65e0\u91d1\u5c5e\u3001\u5ec9\u4ef7\u3001\u9ad8\u5ea6\u7a33\u5b9a\u4e14\u5177\u6709\u72ec\u7279\u7684\u5149\u7535\u7279\u6027\uff0c\u534a\u5bfc\u4f53\u6c2e\u5316\u78b3\u53d7\u5230\u4e86\u4ece\u5149\u50ac\u5316\u5230\u751f\u7269\u4f20\u611f\u7684\u5e7f\u6cdb\u5173\u6ce8\u3002\u4e1c\u5357\u5927\u5b66\u5f20\u8881\u5065\u8bfe\u9898\u7ec4\u62a5\u9053\u4e86\u53ea\u9700\u51e0\u79d2\u949f\u5373\u53ef\u901a\u8fc7\u5fae\u6ce2\u8f85\u52a9\u51b7\u51dd\u7b80\u5355\u5730\u5b9e\u73b0\u6c2e\u5316\u78b3\u5728\u7535\u6781\u4e0a\u7684\u751f\u957f\u3002\u8d85\u5feb\u52a0\u70ed\u7a0b\u5e8f\u4e0d\u4ec5\u89e3\u51b3\u4e86\u805a\u5408\u8fc7\u7a0b\u4e2d\u524d\u9a71\u7269\u6325\u53d1\u7684\u70ed\u529b\u5b66\u77db\u76fe\uff0c\u800c\u4e14\u8fd8\u5728\u7535\u6781\u4e0a\u4ea7\u751f\u4e86\u5177\u6709\u5bcc\u78b3\u68af\u5ea6\u7ed3\u6784\u7684\u5f3a\u56fa\u6027\u6c2e\u5316\u78b3\u5c42\uff0c\u6781\u5927\u5730\u52a0\u5feb\u4e86\u7535\u5b50-\u7a7a\u7a74\u7684\u5206\u79bb\u548c\u8fc1\u79fb\u7387\u3002\u6c2e\u5316\u78b3\u5149\u7535\u7535\u6781\u663e\u793a\u51fa\u589e\u5f3a\u7684\u5149\u7535\u6d41\uff0c\u5e76\u4e14\u7535\u5316\u5b66\u53d1\u5149\u7684\u9634\u6781\u6548\u7387\u662f\u6c34\u6eb6\u6db2\u4e2d\u57fa\u51c6\u7269\u8d28Ru(bpy)3<\/sub>Cl2<\/sub>\u76847\u500d\u3002\u8be5\u7b56\u7565\u63d0\u51fa\u7684\u5fae\u6ce2\u8f85\u52a9\u6c89\u79ef\u65b9\u6cd5\u4e3a\u4f7f\u7528\u5176\u4ed6\u524d\u9a71\u7269\u548c\u57fa\u677f\u6765\u5b9e\u73b0\u5176\u4ed6\u7269\u8d28\u7684\u5236\u5907\u63d0\u4f9b\u4e86\u4e00\u79cd\u65b0\u7684\u65b9\u6cd5\u3002[7]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cUltrafast Condensation of Carbon Nitride on Electrodes with\u00a0Exceptional Boosted Photocurrent and Electrochemiluminescence\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Angew. Chem. Int. Ed.\u3002<\/p>\n

\u56fe\u4e03\uff1a\u5fae\u6ce2\u8f85\u52a9\u6c89\u79ef\u6cd5\u5236\u5907\u6c2e\u5316\u78b3\u793a\u610f\u56fe\u53ca\u76f8\u5173\u8868\u5f81\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

8. Adv. Funct. Mater.<\/b><\/strong>\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u7684\u5149\u81f4\u53d1\u5149\u7279\u6027\u5728\u5206\u5c42\u77e9\u9635\u4e2d\u7684\u5e94\u7528<\/b><\/strong><\/p>\n

\u5feb\u901f\u7b5b\u9009\u6709\u6bd2\u548c\u81f4\u764c\u5316\u5408\u7269–\u591a\u73af\u82b3\u70c3\uff0c\u73af\u5883\u548c\u98df\u54c1\u5b89\u5168\u9886\u57df\u5177\u6709\u91cd\u8981\u610f\u4e49\u30022D\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u662f\u9ad8\u6548\u3001\u7a33\u5b9a\u3001\u4f4e\u6210\u672c\u548c\u73af\u4fdd\u7684\u5149\u654f\u6750\u6599\uff0c\u4f46\u5e38\u89c4\u5e94\u7528\u9650\u4e8e\u6c34\u6eb6\u6db2\u4e2d\uff0c\u96be\u4ee5\u89e3\u51b3\u5176\u957f\u671f\u5206\u6563\u6027\uff0c\u9650\u5236\u4e86\u5149\u81f4\u53d1\u5149\u5206\u6790\u7684\u5e7f\u6cdb\u5e94\u7528\u3002\u4e1c\u5357\u5927\u5b66\u5f20\u8881\u5065\u8bfe\u9898\u7ec4\u901a\u8fc7\u5728\u9759\u7535\u76f8\u4e92\u4f5c\u7528\u7684\u9a71\u52a8\u4e0b\u5c06\u6c2e\u5316\u78b3\u5206\u6563\u5728\u5206\u5c42\u7684\u805a\u5408\u7269\u57fa\u4f53\u4e2d\uff0c\u4ece\u800c\u5229\u7528\u4e86\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u7684\u72ec\u7279\u5149\u81f4\u53d1\u5149\u7279\u6027\u3002\u8be5\u7b56\u7565\u4e0d\u4ec5\u4f7f\u56fa\u6001\u4e3b\u4f53\u80fd\u591f\u6c38\u4e45\u4fdd\u6301\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u7684\u5747\u5300\u5206\u6563\u6027\uff0c\u800c\u4e14\u8fd8\u53ef\u4ee5\u5904\u7406\u81ea\u7531\u901a\u9053\u4ee5\u8fdb\u884c\u8db3\u591f\u7684\u8d28\u91cf\u8f6c\u79fb\u3002\u4f7f\u7528b-CD\u4f5c\u4e3a\u5206\u5b50\u8bc6\u522b\u5355\u5143\uff0c\u901a\u8fc7\u5185\u6ee4\u6548\u5e94\u6784\u5efa\u4e86\u4e00\u79cd\u7ecf\u6d4e\u3001\u9ad8\u5ea6\u9009\u62e9\u6027\u548c\u7075\u654f\u7684\u591a\u73af\u82b3\u70c3\u7eb8\u57fa\u5149\u81f4\u53d1\u5149\u4f20\u611f\u5668\u3002\u8fd9\u9879\u5de5\u4f5c\u4e3a\u5229\u7528\u56fa\u6001\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u72ec\u7279\u7684\u5149\u81f4\u53d1\u5149\u7279\u6027\u548c\u7a33\u5b9a\u6027\u5f00\u8f9f\u4e86\u4e00\u6761\u65b0\u9014\u5f84\uff0c\u9002\u7528\u4e8e\u5404\u79cd\u6f5c\u5728\u7684\u4f20\u611f\u5e94\u7528\u3002[8]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cHarnessing Photoluminescent Properties of Carbon Nitride\u00a0Nanosheets in a Hierarchical Matrix\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Adv. Funct. Mater.\u3002<\/p>\n

\u56fe\u516b\uff1a\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u6784\u5efa\u7eb8\u57fa\u4f20\u611f\u5668\u793a\u610f\u56fe\u53ca\u626b\u63cf\u7535\u955c\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/p>\n

9. Chem. Eur.J.<\/b><\/strong>\u5265\u79bb\u548c\u654f\u5316\u7684\u4e8c\u7ef4\u6c2e\u5316\u78b3\u5728\u7ea2\u5149\u4e0b\u8fdb\u884c\u5149\u7535\u5316\u5b66\u751f\u7269\u4f20\u611f<\/b><\/strong><\/p>\n

\u4e8c\u7ef4\u6c2e\u5316\u78b3\u4f5c\u4e3a\u4e00\u79cd\u5171\u8f6d\u65e0\u91d1\u5c5e\u805a\u5408\u7269\u7528\u4e8e\u5149\u7535\u5316\u5b66\uff08PEC\uff09\u751f\u7269\u4f20\u611f\u5f15\u8d77\u5e7f\u6cdb\u7684\u5173\u6ce8\uff0c\u4f46\u6c2e\u5316\u78b3\u4ec5\u5438\u6536\u7d2b\u5916\u7ebf\u548c\u975e\u5e38\u6709\u9650\u7684\u53ef\u89c1\u5149\uff08l\u00a0<460 nm\uff09\uff0c\u8fd9\u5bf9\u4f53\u5916\u5206\u6790\u548c\u4f53\u5185\u68c0\u6d4b\u90fd\u5177\u6709\u6f5c\u5728\u98ce\u9669\u3002\u4e1c\u5357\u5927\u5b66\u5f20\u8881\u5065\u8bfe\u9898\u7ec4\u62a5\u9053\u4e86\u57fa\u4e8ep-p\u76f8\u4e92\u4f5c\u7528\uff0c\u901a\u8fc7\u673a\u68b0\u7814\u78e8\u6cd5\u5c06\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u4e0e\u94dc\u915e\u83c1\u540c\u65f6\u5265\u79bb\u548c\u529f\u80fd\u5316\u3002\u7531\u4e8e\u80fd\u7ea7\u5339\u914d\u3001\u6709\u6548\u7684\u4f9b\u4f53-\u53d7\u4f53\u76f8\u4e92\u4f5c\u7528\u7b49\u56e0\u7d20\uff0c\u5728\u7ea2\u5149\uff08l> 630 nm\uff09\u7167\u5c04\u4e0b\u5236\u5907\u7684\u590d\u5408\u7269\u663e\u793a\u51fa\u589e\u5f3a\u7684\u5149\u7535\u6d41\u3002\u4f7f\u7528\u8be5\u590d\u5408\u7269\u5149\u7535\u6781\u7ecf\u7ea2\u5149\u9009\u62e9\u6027\u68c0\u6d4b\u8840\u6db2\u4e2d\u7684\u591a\u5df4\u80fa\uff0c\u5176\u7ebf\u6027\u8303\u56f4\u548c\u68c0\u6d4b\u9650\u5747\u4e0d\u53d7\u5f71\u54cd\u3002\u8be5\u7b56\u7565\u4e3a\u7814\u7a76\u5149\u7535\u6781\u7684\u5c0f\u578b\u5316\u3001\u690d\u5165\u7ec4\u7ec7\u4ee5\u53ca\u4f53\u5185\u5e94\u7528\u7684\u751f\u7269\u76f8\u5bb9\u6027\u548c\u751f\u7269\u964d\u89e3\u6027\u8bc4\u4f30\u63d0\u4f9b\u4e00\u79cd\u65b0\u7684\u89c1\u89e3\u3002[9]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cExfoliation and Sensitization of 2D Carbon Nitride for\u00a0Photoelectrochemical Biosensing under Red Light\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Chem. Eur. J.\u3002<\/p>\n

\u56fe\u4e5d\uff1a\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u590d\u5408\u7269\u7684\u5236\u5907\u793a\u610f\u56fe\u53ca\u8868\u5f81\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

10. Chinese Chem. Lett.<\/b><\/strong>\u7eb3\u7c73\u6c89\u6dc0\u6cd5\u5236\u5907\u9ad8\u4ea7\u7387\u9ad8\u5149\u50ac\u5316\u6d3b\u6027\u7684\u6c2e\u5316\u78b3\u7eb3\u7c73\u7c92\u5b50<\/b><\/strong><\/p>\n

\u6c2e\u5316\u78b3\u4f5c\u4e3a\u8f6c\u5316\u592a\u9633\u80fd\u7684\u91cd\u8981\u50ac\u5316\u4ecb\u8d28\uff0c\u7eb3\u7c73\u7ed3\u6784\u8c03\u8282\u662f\u63d0\u9ad8\u50ac\u5316\u6d3b\u6027\u7684\u6709\u6548\u65b9\u6cd5\u3002\u4e1c\u5357\u5927\u5b66\u5f20\u8881\u5065\u8bfe\u9898\u7ec4\u63d0\u51fa\u4e86\u4e00\u79cd\u4f7f\u7528\u4e0d\u826f\u6eb6\u5242\u7684\u7eb3\u7c73\u6c89\u6dc0\u65b9\u6cd5\u6765\u5236\u5907\u6c2e\u5316\u78b3\u7eb3\u7c73\u9897\u7c92\u3002\u901a\u8fc7\u7b80\u5355\u7684\u6c2e\u5316\u78b3\u6eb6\u89e3\u548c\u6c89\u6dc0\u8fc7\u7a0b\u5feb\u901f\u5408\u6210\u6c2e\u5316\u78b3\u7eb3\u7c73\u7c92\u5b50\uff0840 nm\uff09\uff0c\u4ea7\u7387\u9ad8\u8fbe50\uff05\u3002\u5c06\u6240\u5236\u5907\u7684\u6c2e\u5316\u78b3\u7eb3\u7c73\u7c92\u5b50\u7528\u4e8e\u67d3\u6599\u7684\u5149\u50ac\u5316\u964d\u89e3\uff0c\u5177\u6709\u9ad8\u8fbe2.5\u500d\u7684\u6027\u80fd\u3002\u8be5\u5de5\u4f5c\u5c06\u4e3a\u6279\u91cf\u5236\u5907\u7eb3\u7c73\u7ed3\u6784\u7684\u6c2e\u5316\u78b3\u5f00\u8f9f\u65b0\u9014\u5f84\uff0c\u5e76\u4e3a\u5176\u5927\u89c4\u6a21\u7684\u5de5\u4e1a\u5e94\u7528\u94fa\u5e73\u9053\u8def\u3002[10]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cPreparation of carbon nitride nanoparticles by nanoprecipitation\u00a0method with high yield and enhanced photocatalytic activity\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Chinese Chem. Lett.\u3002<\/p>\n

\u56fe\u5341\uff1a\u6c2e\u5316\u78b3\u7eb3\u7c73\u7c92\u5b50\u7684\u5236\u5907\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u6731\u6c38\u6cd5\uff08\u6e05\u534e\u5927\u5b66\uff09<\/b><\/strong><\/p>\n

11. Nano Energy<\/b><\/strong>\u4e09\u7ef4\u591a\u5b54g-C<\/b><\/strong>3<\/b><\/sub><\/strong>N<\/b><\/strong>4<\/b><\/sub><\/strong>\u7528\u4e8e\u9ad8\u6548\u5149\u50ac\u5316\u6c34\u5206\u89e3<\/b><\/strong><\/p>\n

\u5728\u4e0d\u4f7f\u7528\u727a\u7272\u5242\u7684\u6761\u4ef6\u4e0b\uff0c\u5c06\u6c34\u5149\u50ac\u5316\u5206\u89e3\u4e3aH2<\/sub>\u548cO2<\/sub>\u88ab\u8ba4\u4e3a\u662f\u5c06\u592a\u9633\u80fd\u8f6c\u5316\u4e3a\u53ef\u518d\u751fH2<\/sub>\u80fd\u6e90\u7684\u6700\u7406\u60f3\u65b9\u6cd5\u4e4b\u4e00\u3002\u6e05\u534e\u5927\u5b66\u6731\u6c38\u6cd5\u8bfe\u9898\u7ec4\u5408\u4f5c\u6784\u5efa\u4e86\u7531\u9ad8\u7ed3\u6676\u5ea6\u548c\u8d85\u8584\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u7ec4\u88c5\u800c\u6210\u7684\u4e09\u7ef4\u591a\u5b54\u77f3\u58a8\u6c2e\u5316\u78b3\u3002\u5728\u53ef\u89c1\u5149\u4e0b\uff0c\u4e09\u7ef4\u591a\u5b54\u77f3\u58a8\u6c2e\u5316\u78b3\u53ef\u4ee5\u5c06\u7eaf\u6c34\u76f4\u63a5\u5206\u89e3\u4e3aH2<\/sub>\u548cO2<\/sub>\uff0c\u9ad8\u5206\u89e3\u7387\u5206\u522b\u8fbe\u5230101.4\u548c49.1 mmol g-1<\/sup>\u00a0h-1<\/sup>\uff0c\u6bd4\u5927\u5757\u6c2e\u5316\u78b3\u548c\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u9ad8\u51fa\u7ea611.8\u548c5.1\u500d\u3002\u6b64\u5916\uff0c\u5b83\u5728420 nm\u5904\u9ad8\u8fbe1.4\uff05\u7684\u8868\u89c2\u91cf\u5b50\u4ea7\u7387\uff0c\u660e\u663e\u9ad8\u4e8e\u7684Pt \/ \u6c2e\u5316\u78b3\u590d\u5408\u7269\u3002\u4e09\u7ef4\u591a\u5b54\u77f3\u58a8\u6c2e\u5316\u78b3\u7684\u6709\u6548\u6d3b\u6027\u4e3b\u8981\u5f52\u56e0\u4e8e\u9ad8\u5ea6\u7ed3\u6676\u7684\u8d85\u8584\u7eb3\u7c73\u7247\u5355\u5143\u7ec4\u88c5\u800c\u6210\u76843D\u4e92\u8fde\u5f00\u653e\u6846\u67b6\uff0c\u4e3a\u66f4\u5feb\u7684\u8f7d\u6d41\u5b50\u4f20\u8f93\u63d0\u4f9b\u4e86\u9014\u5f84\uff1b\u53e6\u4e00\u65b9\u9762\u5f97\u76ca\u4e8e\u51763D\u7ed3\u6784\u53ef\u9632\u6b62\u6c2e\u5316\u78b3\u7eb3\u7c73\u7247\u7684\u56e2\u805a\uff0c\u4f7f\u5176\u5728\u8d85\u8fc7100\u5c0f\u65f6\u6c34\u5206\u89e3\u53cd\u5e94\u4e2d\u4fdd\u6301\u7a33\u5b9a\u3002\u8fd9\u9879\u5de5\u4f5c\u4e3a\u8bbe\u8ba1\u5177\u6709\u4f4e\u7ef4\u7eb3\u7c73\u6750\u6599\u76843D\u591a\u5b54\u7ed3\u6784\u7684\u805a\u5408\u7269\u5149\u50ac\u5316\u5242\u7528\u4e8e\u6539\u5584\u592a\u9633\u80fd\u5438\u6536\u548c\u8f6c\u5316\u63d0\u4f9b\u4e86\u65b0\u7684\u89c1\u89e3\u3002[11]<\/sup>\u201cThree-dimensional porous g-C3<\/sub>N4<\/sub>\u00a0for highly efficient photocatalytic overall\u00a0water splitting\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Nano Energy\u3002<\/p>\n

\u56fe\u5341\u4e00\uff1a\u4e09\u7ef4\u591a\u5b54\u77f3\u58a8\u6c2e\u5316\u78b3\u5408\u6210\u793a\u610f\u56fe\u53ca\u8868\u5f81\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

12. Appl. Catal. B Environ.<\/b><\/strong>g-C<\/b><\/strong>3<\/b><\/sub><\/strong>N<\/b><\/strong>4<\/b><\/sub><\/strong>\u7eb3\u7c73\u68d2\u7ec4\u88c5\u7684\u4e09\u7ef4\u7f51\u7edc\u7ed3\u6784\u6539\u5584\u53ef\u89c1\u5149\u7684\u5149\u50ac\u5316\u6027\u80fd<\/b><\/strong><\/p>\n

\u5927\u5757\u6c2e\u5316\u78b3\u5177\u6709\u6bd4\u8868\u9762\u79ef\u4f4e\u548c\u5149\u751f\u7535\u5b50-\u7a7a\u7a74\u5bf9\u7684\u9ad8\u91cd\u7ec4\u7b49\u7f3a\u70b9\u3002\u6e05\u534e\u5927\u5b66\u6731\u6c38\u6cd5\u8bfe\u9898\u7ec4\u901a\u8fc7\u5316\u5b66\u5b9a\u5236\u9014\u5f84\u6210\u529f\u5730\u5236\u5907\u4e86\u7531\u7eb3\u7c73\u68d2\u7ec4\u88c5\u7684\u4e09\u7ef4\u7f51\u7edc\u7ed3\u6784\u6c2e\u5316\u78b3\u3002 \u4e09\u7ef4\u6c2e\u5316\u78b3\u7eb3\u7c73\u68d2\u7f51\u7edc\u7ed3\u6784\u8868\u73b0\u51fa\u66f4\u5927\u7684\u6bd4\u8868\u9762\u79ef\uff08\u662f\u5927\u5757\u6c2e\u5316\u78b3\u76846.7\u500d\uff09\u548c\u66f4\u5feb\u7684\u7535\u8377\u8f7d\u6d41\u5b50\u4f20\u8f93\u52a8\u529b\u5b66\u3002\u5c06\u4e09\u7ef4\u6c2e\u5316\u78b3\u7eb3\u7c73\u68d2\u7f51\u7edc\u7ed3\u6784\u7528\u4e8e\u5149\u50ac\u5316\u964d\u89e3\u82ef\u915a\u548c\u6790\u6c22\uff0c\u5176\u53ef\u89c1\u5149\u5149\u50ac\u5316\u6d3b\u6027\u660e\u663e\u589e\u5f3a\uff0c\u5206\u522b\u662f\u5927\u5757\u6c2e\u5316\u78b3\u76844.3\u548c5.9\u500d\u3002\u8fd9\u9879\u5de5\u4f5c\u4e3a\u6539\u5584\u6c2e\u5316\u78b3\u805a\u5408\u7269\u5149\u50ac\u5316\u5242\u5bf9\u592a\u9633\u80fd\u7684\u6355\u83b7\u548c\u8f6c\u5316\u63d0\u4f9b\u4e86\u65b0\u7684\u7b56\u7565\u3002[12]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cThree-dimensional network structure assembled by g-C3<\/sub>N4<\/sub>\u00a0nanorods for\u00a0improving visible-light photocatalytic performance”\u4e3a\u9898\uff0c\u53d1\u8868\u5728ACB\u3002<\/p>\n

\u56fe\u5341\u4e8c\uff1a\u4e09\u7ef4\u6c2e\u5316\u78b3\u7eb3\u7c73\u68d2\u7f51\u7edc\u7ed3\u6784\u5236\u5907\u793a\u610f\u56fe\u53ca\u5176\u8868\u5f81\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

13. Appl. Catal. B Environ.<\/b><\/strong>\u5ef6\u4f38\u7a7a\u95f4\u7535\u8377\u5206\u79bb\u80fd\u529b\u7684CN \/ rGO @ BPQDs\u9ad8-\u4f4e\u5f02\u8d28\u7ed3\u7528\u4e8e\u5149\u50ac\u5316\u964d\u89e3\u548c\u4ea7H<\/b><\/strong>2<\/b><\/sub><\/strong>O<\/b><\/strong>2<\/b><\/sub><\/strong><\/p>\n

\u77f3\u58a8\u8d28\u6c2e\u5316\u78b3\u56e0\u5176\u6613\u4e8e\u5236\u5907\u3001\u7a33\u5b9a\u6027\u9ad8\u3001\u6210\u672c\u4f4e\u548c\u53ef\u89c1\u5149\u54cd\u5e94\u800c\u5907\u53d7\u5173\u6ce8\u3002\u6e05\u534e\u5927\u5b66\u6731\u6c38\u6cd5\u8bfe\u9898\u7ec4\u901a\u8fc7\u8d85\u58f0\u8f85\u52a9\u6db2\u76f8\u6cd5\u7528\u5728\u8fd8\u539f\u6c27\u5316\u77f3\u58a8\u70ef\uff08rGO\uff09\u4e0a\u4fee\u9970\u9ed1\u78f7\u91cf\u5b50\u70b9\uff08BPQDs\uff09\u5f97\u5230\u8fd8\u539f\u7684\u6c27\u5316\u77f3\u58a8\u70ef\u4fee\u9970\u7684\u9ed1\u78f7\u91cf\u5b50\u70b9\uff08rGO @ BPQDs\uff09\uff0crGO @ BPQDs\u53ef\u4ee5\u6709\u6548\u5730\u589e\u5f3aBPQDs\u7684\u5316\u5b66\u548c\u7ed3\u6784\u7a33\u5b9a\u6027\u3002\u96f6\u7ef4rGO @ BPQDs\u901a\u8fc7\u81ea\u9677\u5b54\u9650\u5236\u4f5c\u7528\u548cp-p\u76f8\u4e92\u4f5c\u7528\u7262\u56fa\u5730\u56fa\u5b9a\u5728\u4ecb\u5b54\u6c2e\u5316\u78b3\u4e2d\uff0c\u5f62\u6210\u6c2e\u5316\u78b3 \/ rGO @ BPQDs\uff0c\u4ece\u800c\u663e\u7740\u6539\u5584\u4e86\u6c2e\u5316\u78b3\u7684\u5149\u7535\u6027\u80fd\u3002\u6c2e\u5316\u78b3 \/ rGO @ BPQDs\u7684\u54cd\u5e94\u6ce2\u957f\u53ef\u4ee5\u6269\u5c55\u5230800 nm\u3002\u7f57\u4e39\u660eB\u548c\u56db\u73af\u7d20\u964d\u89e3\u7684\u52a8\u529b\u5b66\u5e38\u6570\u5206\u522b\u8fbe\u52300.183\u548c0.0194 min-1<\/sup>\u3002\u6c2e\u5316\u78b3 \/ rGO @ BPQDs\u7684H2<\/sub>O2<\/sub>\u751f\u4ea7\u7387\u662f\u591a\u5b54\u6c2e\u5316\u78b3\u76842.6\u500d\u3002\u5149\u50ac\u5316\u6027\u80fd\u7684\u63d0\u9ad8\u548c\u81ea\u7531\u57fa\u7684\u663e\u7740\u589e\u52a0\u5f52\u56e0\u4e8en-n\u578b\u9ad8-\u4f4e\u5f02\u8d28\u7ed3\u7684\u5f62\u6210\u4ee5\u53ca\u57fa\u4e8e\u6c2e\u5316\u78b3\u548cBPQDs\u4e4b\u95f4\u4e0d\u540c\u8d39\u7c73\u80fd\u7ea7\u7684\u5185\u90e8\u7535\u573a\u3002\u8fd9\u9879\u5de5\u4f5c\u5171\u540c\u4fc3\u8fdb\u4e86\u5149\u751f\u8f7d\u6d41\u5b50\u7684\u7a7a\u95f4\u5206\u79bb\u3002[13]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cCN\/rGO@BPQDs high-low junctions with stretching spatial charge\u00a0separation ability for photocatalytic degradation and H2<\/sub>O2<\/sub>\u00a0production\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Appl. Catal. B Environ.\u3002<\/p>\n

\u56fe\u5341\u4e09\uff1a<\/b><\/strong>n-n<\/b><\/strong>\u578b\u9ad8<\/b><\/strong>–<\/b><\/strong>\u4f4e\u5f02\u8d28\u7ed3\u5149\u50ac\u5316\u673a\u5236\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

14. Chemical Engineering Journal<\/b><\/strong>3D g-C<\/b><\/strong>3<\/b><\/sub><\/strong>N<\/b><\/strong>4<\/b><\/sub><\/strong>\/ TiO<\/b><\/strong>2<\/b><\/sub><\/strong>\u65e0\u5206\u79bb\u5149\u50ac\u5316\u5242\u901a\u8fc7\u5438\u9644\/\u5149\u50ac\u5316\u534f\u540c\u4f5c\u7528\u589e\u5f3a\u6709\u673a\u6c61\u67d3\u7269\u7684\u5149\u964d\u89e3<\/b><\/strong><\/p>\n

\u6c34\u6c61\u67d3\u5df2\u7ecf\u6210\u4e3a\u4e00\u4e2a\u4e25\u91cd\u7684\u95ee\u9898\uff0c\u5a01\u80c1\u7740\u4eba\u7c7b\u7684\u5065\u5eb7\u3002\u6e05\u534e\u5927\u5b66\u6731\u6c38\u6cd5\u8bfe\u9898\u7ec4\u5408\u6210\u4e863D\u6c2e\u5316\u78b3 \/ TiO2<\/sub>\u5f02\u8d28\u7ed3\u5149\u50ac\u5316\u5242\u5e76\u663e\u793a\u51fa\u9ad8\u6548\u7684\u6c61\u67d3\u7269\u964d\u89e3\u6027\u80fd\u3002\u5728\u9759\u6001\u7cfb\u7edf\u4e2d\uff0c\u4e9a\u7532\u57fa\u84dd\uff08MB\uff09\u548c\u82ef\u915a\u7684\u964d\u89e3\u6548\u7387\u662f\u5927\u5757\u6c2e\u5316\u78b3\u76844.0\u548c4.5\u500d\u3002\u5728\u52a8\u6001\u7cfb\u7edf\u4e2d\uff0c\u6c61\u67d3\u7269\u53ef\u4ee5\u8fde\u7eed\u4e0d\u65ad\u5730\u964d\u89e3\u800c\u4e0d\u5206\u79bb\uff0c\u5e76\u4e14\u572890\u5c0f\u65f6\u5185\u975e\u5e38\u7a33\u5b9a\uff0c\u53bb\u9664\u7387\u4e3a16.0\uff05\u30023D\u6c2e\u5316\u78b3 \/ TiO2<\/sub>\u5f02\u8d28\u7ed3\u5149\u50ac\u5316\u5242\u589e\u5f3a\u7684\u6d3b\u6027\u4e3b\u8981\u5f52\u56e0\u4e8e\u6c2e\u5316\u78b3 \/ TiO2<\/sub>\u76843D\u7ed3\u6784\u548c\u5f02\u8d28\u7ed3\u30023D\u7ed3\u6784\u4e0d\u4ec5\u53ef\u4ee5\u6709\u6548\u5730\u63d0\u9ad8\u5438\u9644\u5bcc\u96c6\u80fd\u529b\uff0c\u800c\u4e14\u8fd8\u53ef\u4ee5\u63d0\u4f9b\u591a\u7ef4\u8d28\u91cf\u548c\u7535\u5b50\u4f20\u9012\u901a\u9053\u3002\u540c\u65f6\uff0c\u5f02\u8d28\u7ed3\u53ef\u4ee5\u4fc3\u8fdb\u5149\u751f\u8f7d\u6d41\u5b50\u7684\u5206\u79bb\u548c\u8fc1\u79fb\u30023D \u6c2e\u5316\u78b3 \/ TiO2<\/sub>\u5f02\u8d28\u7ed3\u5149\u50ac\u5316\u5242\u53ef\u4ee5\u4fc3\u8fdb\u5176\u5728\u6c34\u6c61\u67d3\u6cbb\u7406\u4e2d\u7684\u6f5c\u5728\u5e94\u7528\uff0c\u8fd9\u4e3a\u6c61\u6c34\u6cbb\u7406\u63d0\u4f9b\u4e86\u4e00\u79cd\u65b0\u7684\u8bbe\u60f3\u3002[14]<\/sup>\u76f8\u5173\u7814\u7a76\u4ee5\u201cEnhanced organic pollutant photodegradation via adsorption\/photocatalysis\u00a0synergy using a 3D g-C3<\/sub>N4<\/sub>\u00a0<\/sub>\/\u00a0TiO2<\/sub>\u00a0free-separation photocatalyst\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Chemical Engineering Journal\u3002<\/p>\n

\u56fe\u5341\u56db\uff1a<\/b><\/strong>3D g-C<\/b><\/strong>3<\/b><\/sub><\/strong>N<\/b><\/strong>4<\/b><\/sub><\/strong>\u00a0<\/b><\/sub><\/strong>\/<\/b><\/strong>\u00a0<\/b><\/strong>TiO<\/b><\/strong>2<\/b><\/sub><\/strong>\u00a0\u5f02\u8d28\u7ed3\u5149\u964d\u89e3\u6c61\u67d3\u7269\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u53c2\u8003\u6587\u732e\uff1a<\/b><\/strong><\/p>\n

1. Zhang G., Li G., Heil T.,et al. Tailoring the Grain Boundary Chemistry of Polymeric Carbon Nitridefor Enhanced Solar Hydrogen Production and CO2<\/sub>\u00a0Reduction. [J] Angew. Chem. Int. Ed. 2019, 58, 3433 -3437.<\/p>\n

2. Yin L., Wang S., Yang C. et al.Modulation of Polymeric Carbon Nitrides throughSupramolecular Preorganization for Efficient Photocatalytic Hydrogen Generation. [J] ChemSusChem 2019, 12, 3320-3325.<\/p>\n

3. Yang P., WangL., Zhuzhang H., et al. Photocarving nitrogen vacancies in a polymeric carbon nitride for metal-freeoxygen synthesis. [J] Appl. Catal. B Environ.\u00a02019, 256,\u00a0117794.<\/p>\n

4. Ren W., Cheng J., Ou H.,et al.Enhancing Visible-Light Hydrogen Evolution Performance\u00a0of Crystalline Carbon Nitride by Defect Engineering. [J] ChemSusChem 2019, 12, 3257-3262.<\/p>\n

5. Ou H., Tang C., Zhang Y., et al.Se-modified polymeric carbon nitride nanosheets with improvedphotocatalytic activities. [J] Journal of Catalysis\u00a02019, 375,\u00a0104-112.<\/p>\n

6. Pan Z., Zhang G., WangX.Polymeric Carbon Nitride\/Reduced Graphene Oxide\/Fe2<\/sub>O3<\/sub>: All-Solid-State Z-Scheme System for Photocatalytic Overall Water Splitting. [J] Angew. Chem. Int. Ed.\u00a02019, 58, 7102 -7106.<\/p>\n

7. Zhao T., Zhou Q., LvY., et al.Ultrafast Condensation of Carbon Nitride on Electrodes with\u00a0Exceptional Boosted Photocurrent and Electrochemiluminescence. [J] Angew. Chem. Int. Ed.\u00a02020, 59, 1139-1143.<\/p>\n

8. Han D., Ni D., Zhou Q., et al.Harnessing Photoluminescent Properties of Carbon NitrideNanosheets in a Hierarchical Matrix. [J] Adv. Funct. Mater. 2019, 29, 1905576.<\/p>\n

9. Zhao L., Ji J., ShenY., et al.Exfoliation and Sensitization of 2D Carbon Nitride for\u00a0Photoelectrochemical Biosensing under Red Light. [J] Chem. Eur. J. 2019, 25, 15680-15686.<\/p>\n

10. Gan Z., Huang C., ShenY., et al.Preparation of carbon nitride nanoparticles by nanoprecipitation\u00a0method with high yield and enhanced photocatalytic activity. [J] Chinese Chem. Lett.\u00a02020, 31,\u00a0513-516.<\/p>\n

11. ChenX., Shi\u00a0R., Chen\u00a0Q., et al.\u00a0Three-dimensional porous g-C3<\/sub>N4<\/sub>\u00a0for highly efficient photocatalytic overall\u00a0water splitting. [J] Nano Energy 2019, 59,\u00a0644-650.<\/p>\n

12. LuoW., ChenX., Wei Z., et al.\u00a0Three-dimensional network structure assembled by g-C3<\/sub>N4<\/sub>\u00a0nanorods for\u00a0improving visible-light photocatalytic performance. [J] Appl. Catal. B Environ.\u00a02019, 255,\u00a0117761.<\/p>\n

13. XiongJ., LiX., Huang J., et al. CN\/rGO@BPQDs high-low junctions with stretching spatial charge\u00a0separation ability for photocatalytic degradation and H2<\/sub>O2<\/sub>\u00a0production. [J] Appl. Catal. B Environ.\u00a02020, 266,\u00a0118602.<\/p>\n

14. ShengY., WeiZ., Miao\u00a0H., et al.\u00a0Enhanced organic pollutant photodegradation via adsorption\/photocatalysis\u00a0synergy using a 3D g-C3<\/sub>N4<\/sub>\u00a0<\/sub>\/\u00a0TiO2<\/sub>\u00a0free-separation photocatalyst. [J] Chemical Engineering Journal\u00a02019, 370,\u00a0287-294.<\/p>\n

\u672c\u6587\u7531\u559c\u6b22\u957f\u9888\u9e7f\u7684\u9ad8\u4f9b\u7a3f\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1: tougao@cailiaoren.com.<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1acailiaorenVIP\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"

\u6c2e\u5316\u78b3(C3N4)\u662f\u8fd1\u5e74\u6765\u65b0\u5174\u7684\u4e00\u79cd\u78b3\u6750\u6599\uff0c\u5176\u7531\u78b3\u548c\u6c2e\u7684\u5355\u539f\u5b50\u8fdb\u884csp2\u6742\u5316\u5f62\u6210\uff0c\u5177\u6709\u72ec\u7279\u7684\u5e73\u9762\u7ed3\u6784\u3001\u826f\u597d\u7684\u7535\u5b66\u3001\u5149\u5b66\u548c\u7269\u7406\u5316\u5b66\u6027\u8d28\uff0c\u4e14\u5236\u5907\u5de5\u827a\u7b80\u5355\u3001\u6210\u672c\u8f83\u4f4e\uff0c…<\/p>\n","protected":false},"author":10213,"featured_media":199595,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[1187],"tags":[],"class_list":["post-199581","post","type-post","status-publish","format-standard","has-post-thumbnail","hentry","category-zhuanlan"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/199581"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/10213"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=199581"}],"version-history":[{"count":3,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/199581\/revisions"}],"predecessor-version":[{"id":199852,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/199581\/revisions\/199852"}],"wp:featuredmedia":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/media\/199595"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=199581"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=199581"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=199581"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}