{"id":189990,"date":"2019-11-22T06:30:19","date_gmt":"2019-11-21T22:30:19","guid":{"rendered":"\/\/m.iemloyee.com\/?p=189990"},"modified":"2019-11-21T21:39:01","modified_gmt":"2019-11-21T13:39:01","slug":"%ef%bc%88%e5%b7%b2%e6%a0%a1%e7%a8%bf%ef%bc%89acs-energy-lett-%e5%85%89%e7%85%a7%e8%be%85%e5%8a%a9%e5%90%88%e6%88%90%e5%87%8f%e5%b0%91%e9%92%99%e9%92%9b%e7%9f%bf%e7%94%b5%e6%b1%a0%e7%bc%ba%e9%99%b7","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=189990","title":{"rendered":"ACS Energy Lett. : \u5149\u7167\u8f85\u52a9\u5408\u6210\u51cf\u5c11\u9499\u949b\u77ff\u7535\u6c60\u7f3a\u9677"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u6709\u673a-\u65e0\u673a\u6742\u5316\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u56e0\u5176\u9ad8\u7684\u5149\u7535\u8f6c\u6362\u6548\u7387\u53ca\u7b80\u5355\u5ec9\u4ef7\u7684\u5236\u5907\u5de5\u827a\uff0c\u5728\u5149\u4f0f\u9886\u57df\u6380\u8d77\u4e86\u65b0\u7684\u7814\u7a76\u70ed\u6f6e\uff0c\u662f\u5f53\u524d\u53d1\u5c55\u6700\u5feb\u7684\u65b0\u4e00\u4ee3\u8584\u819c\u5149\u4f0f\u5668\u4ef6\u3002\u5df2\u6709\u7814\u7a76\u8868\u660e\u5728\u9499\u949b\u77ff\u5f62\u6210\u8fc7\u7a0b\u4e2d\uff0c\u65bd\u52a0\u7167\u660e\u6709\u52a9\u4e8e\u6539\u5584\u754c\u9762\u5904\u5f62\u6838\uff0c\u5e76\u5728\u8fde\u7eed\u6c89\u79ef\u9499\u949b\u77ff\u8fc7\u7a0b\u4e2d\u52a0\u5feb\u79bb\u5b50\u6269\u6563\u3002\u53e6\u4e00\u65b9\u9762\uff0c\u5149\u7167\u4e5f\u5e26\u6765\u4e86\u4e24\u4e2a\u4e3b\u8981\u95ee\u9898\uff0c\u5206\u522b\u4e3a\u7531\u4e8e\u52a0\u901f\u7684\u79bb\u5b50\u8fc1\u79fb\u8bf1\u53d1\u7684\u76f8\u5206\u79bb\uff0c\u4ee5\u53ca\u7531\u4e8eMAI\u84b8\u53d1\u5f15\u8d77\u7684\u9499\u949b\u77ff\u7684\u5206\u89e3\u3002\u56e0\u6b64\uff0c\u4ec5\u5f53\u8584\u819c\u8868\u9762\u5bcc\u542bMAI\u65f6\uff0c\u5149\u7167\u624d\u80fd\u5728\u9499\u949b\u77ff\u5408\u6210\u4e2d\u5c55\u73b0\u79ef\u6781\u7684\u4f5c\u7528\uff0c\u7136\u800c\u5149\u7167\u5bf9MA\u9633\u79bb\u5b50\u548cI\u9634\u79bb\u5b50\u7684\u5177\u4f53\u5f71\u54cd\u673a\u5236\u76ee\u524d\u5c1a\u4e0d\u6e05\u695a\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb<\/strong>\u3011<\/p>\n

\u8fd1\u65e5\uff0c\u5929\u6d25\u7406\u5de5\u5927\u5b66\u5370\u5bff\u6839<\/b><\/strong>\u6559\u6388\u3001<\/b><\/strong>\u897f\u5b89\u7535\u5b50\u79d1\u6280\u5927\u5b66\u5e38\u6676\u6676\u6559\u6388<\/b><\/strong>\uff08<\/b><\/strong>\u5171\u540c<\/b><\/strong>\u901a\u8baf\u4f5c\u8005\uff09<\/b><\/strong>\u7b49\u4eba\u5728\u8fde\u7eed\u6c14\u76f8\u6c89\u79ef\u6cd5\u5236\u5907\u9499\u949b\u77ff\u8584\u819c\u8fc7\u7a0b\u4e2d\uff0c\u91c7\u7528\u4e0d\u540c\u6ce2\u957f\u7684\u5149\uff08\u7ea2\u3001\u7eff\u3001\u84dd\u548c\u767d\u5149\uff09\u7167\u5c04\u8f85\u52a9\u9499\u949b\u77ff\u5408\u6210\u3002\u98de\u884c\u65f6\u95f4\u2212\u4e8c\u6b21\u79bb\u5b50\u8d28\u8c31\uff08ToF-SIMS\uff09\u53ca\u6df1\u80fd\u7ea7\u77ac\u6001\u5149\u8c31\uff08DLTS\uff09\u7814\u7a76\u7ed3\u679c\u8868\u660e\u5728\u65e0\u5149\u7167\u6761\u4ef6\u4e0b\uff0c\u7898\u4f1a\u5728\u9499\u949b\u77ff\u8868\u9762\u5bcc\u96c6\uff0c\u5bfc\u81f4\u5668\u4ef6\u5185\u90e8\u51fa\u73b0\u5927\u91cf\u7f3a\u9677\uff1b\u767d\u5149\u53ef\u4ee5\u9a71\u4f7f\u7898\u8fdb\u5165\u8584\u819c\u4f53\u76f8\uff0c\u4f7f\u5176\u5728\u8584\u819c\u5185\u5747\u5300\u5206\u5e03\uff0c\u8fdb\u800c\u6709\u6548\u6d88\u9664\u7f3a\u9677\u3002\u57fa\u4e8e\u767d\u5149\u8f85\u52a9\u7b56\u7565\u5236\u5907\u7684\u9499\u949b\u77ff\u5668\u4ef6\u76f8\u6bd4\u5bf9\u7167\u6837\u5c55\u73b0\u4e86\u66f4\u9ad8\u7684\u5149\u7535\u8f6c\u6362\u6548\u7387\u53ca\u5149\u7a33\u5b9a\u6027\uff0c\u4e09\u5143\u9633\u79bb\u5b50\u4f53\u7cfb\u9499\u949b\u77ff\u7535\u6c60\u6548\u7387\u753118.3%\u63d0\u9ad8\u81f320%\u4ee5\u4e0a\u3002\u76f8\u5173\u6210\u679c\u4ee5\u9898\u4e3a\u00a0\u201c<\/b><\/strong>Reducing Defects in Perovskite Solar Cells with White Light Illumination Assisted Synthesis<\/b><\/strong>\u201d<\/b><\/strong>\u00a0<\/b><\/strong>\u53d1\u8868\u5728ACS Energy Letter<\/b><\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe\u4e00 <\/b><\/strong>\u5149\u6e90\u9009\u62e9\u53ca\u5668\u4ef6\u5236\u5907\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

(a-b) \u4e0d\u540c\u5149\u6e90\u7684\u5149\u8c31\u53ca\u524d\u9a71\u819c\u81ea\u8eab\u7684\u5149\u5438\u6536\u3002\u524d\u9a71\u819c\u5728\u53ef\u89c1\u5149\u533a\u5177\u6709\u975e\u5e38\u5fae\u5f31\u7684\u5149\u5438\u6536\uff0c\u4ece\u800c\u907f\u514d\u4e86MAI\u4e0ePbI2<\/sub>\u53cd\u5e94\u4e4b\u524d\u5165\u5c04\u5149\u7684\u5f71\u54cd\uff1b
\n (c-g) \u5b9e\u9a8c\u6d41\u7a0b\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe\u4e8c <\/b><\/strong>\u9499\u949b\u77ff\u5408\u6210\u8fc7\u7a0b\u4e2d\u7684\u539f\u4f4d\u7535\u963b\u6d4b\u8bd5<\/b><\/strong>\"\"<\/b><\/strong><\/p>\n

(a) \u4e0d\u540c\u5149\u7167\u6761\u4ef6\u4e0b\u9499\u949b\u77ff\u8584\u819c\u7684\u539f\u4f4d\u7535\u963b\u6d4b\u8bd5\u7ed3\u679c\u3002\u767d\u5149\u4e0b\u5236\u5907\u8584\u819c\u7684\u672c\u5f81\u7535\u963b\u5927\u5e45\u964d\u4f4e\uff0c\u8868\u660e\u8584\u819c\u53cd\u5e94\u5145\u5206\uff0c\u8f7d\u6d41\u5b50\u6d53\u5ea6\u589e\u52a0\uff1b
\n (b) \u5b9e\u9a8c\u8fc7\u7a0b\u4e2d\u4e0a\u57fa\u677f\uff08MAI\uff09\u548c\u4e0b\u57fa\u677f(PbI2<\/sub>)\u7684\u6e29\u5ea6\u53d8\u5316\u56fe\uff1b
\n (c) \u89e3\u91ca\u7535\u963b\u6d4b\u8bd5\u7ed3\u679c\u7684\u6a21\u578b\u793a\u610f\u56fe\u3002<\/b><\/p>\n

\u56fe\u4e09 <\/b><\/strong>ToF-SIMS\u6df1\u5ea6\u5256\u6790<\/b><\/strong><\/p>\n

\"\"<\/p>\n

(a, b) MIA\u8584\u819c\uff08R\/G\/B\uff09\u4e0e\u5bf9\u7167\u6837\u4e2d\u9634\u3001\u9633\u79bb\u5b50\u7684ToF-SIMS\u6df1\u5ea6\u5256\u6790\u3002\u53ef\u89c1\u968f\u7740\u5149\u6ce2\u957f\u7684\u589e\u52a0\uff0c\u7898\u5728\u8584\u819c\u5185\u90e8\u53d8\u5f97\u66f4\u52a0\u5747\u5300\uff0c\u800cMA\u5219\u5bcc\u96c6\u5728\u8584\u819c\u8868\u9762\uff0c\u4e0d\u5229\u4e8e\u7f3a\u9677\u7684\u6d88\u9664\uff1b
\n (c) WIA\u8584\u819c\uff08W\uff09\u4e0e\u5bf9\u7167\u6837\u4e2d\u9634\u3001\u9633\u79bb\u5b50\u7684ToF-SIMS\u6df1\u5ea6\u5256\u6790\u3002\u53ef\u89c1\u767d\u5149\u4e0d\u4f46\u4f7f\u66f4\u591a\u7684\u7898\u5411\u8584\u819c\u5185\u90e8\u6269\u6563\uff0c\u800c\u4e14\u6d88\u9664\u4e86\u8868\u9762\u5bcc\u96c6\u7684\u8fc7\u91cfMA\uff0c\u4f7f\u4e8c\u8005\u5728\u8584\u819c\u5185\u90e8\u66f4\u52a0\u5747\u5300\uff0c\u6709\u5229\u4e8e\u7f3a\u9677\u7684\u6d88\u9664\uff1b
\n (d) WIA\u8584\u819c\uff08W\uff09\u4e0e\u5bf9\u7167\u6837\u7684XPS\u6df1\u5ea6\u5256\u6790\u7ed3\u679c\uff0c\u4e0eToF-SIMS\u7ed3\u679c\u543b\u5408\u3002<\/p>\n

\u56fe\u56db <\/b><\/strong>\u4e0d\u540c\u5149\u7167\u6761\u4ef6\u4e0b\u5236\u5907\u7684<\/b><\/strong>\u9499\u949b\u77ff<\/b><\/strong>\u7535\u6c60\u6027\u80fd\u7bb1\u5f0f\u5206\u5e03\u56fe<\/b><\/strong>\"\"<\/p>\n

(a) MAPbI3<\/sub>\u5668\u4ef6\u6548\u7387\u7edf\u8ba1\uff1b
\n (b) FA(Cs, MA)PbI(Br)3<\/sub>\u5668\u4ef6\u6548\u7387\u7edf\u8ba1\u3002<\/p>\n

\u56fe\u4e94 \u9499\u949b\u77ff<\/b><\/strong>\u5668\u4ef6\u5de5\u4f5c\u7a33\u5b9a\u6027\u6d4b\u8bd5<\/b><\/strong><\/p>\n

\"\"<\/p>\n

MPP\u6761\u4ef6\u4e0b\uff0c\u5668\u4ef6\u5728\u4e0d\u540c\u5149\u6e90\uff08\u84dd\u3001\u7eff\u3001\u7ea2\u548c\u767d\u5149\uff09\u7167\u660e\u4e0b\u7684\u7a33\u6001\u6548\u7387\u8f93\u51fa\uff0c\u5176\u4e2d\u66f2\u7ebf\u989c\u8272\u4ee3\u8868\u4e0d\u540c\u5149\u7167\u4e0b\u5408\u6210\u7684\u9499\u949b\u77ff\uff08\u7c89\u8272\u4ee3\u8868\u767d\u5149\uff09\u3002\u767d\u5149\u5668\u4ef6\u5177\u6709\u6bd4\u5355\u8272\u5149\u5668\u4ef6\u66f4\u9ad8\u7684\u5149\u7a33\u5b9a\u6027<\/p>\n

\u00a0<\/b><\/strong>\u56fe<\/b><\/strong>\u516d<\/b><\/strong>\u00a0\u9499\u949b\u77ff<\/b><\/strong>\u5668\u4ef6\u7684\u7f3a\u9677\u8868\u5f81<\/b><\/strong>\"\"(a) \u4e0d\u540c\u5149\u7167\u6761\u4ef6\u4e0b\u5236\u5907\u7684\u9499\u949b\u77ff\u7535\u6c60\u7684\u6df1\u80fd\u7ea7\u77ac\u6001\u8c31\u7ed3\u679c\u3002\u7ea2\u5149\u548c\u9ed1\u6697\u4e0b\u5236\u5907\u5668\u4ef6\u7684\u7f3a\u9677\u6700\u591a\uff0c\u800c\u767d\u5149\uff08\u7c89\u7ebf\uff09\u5236\u5907\u5668\u4ef6\u7684\u7f3a\u9677\u6700\u5c11\uff08\u66f2\u7ebf\u6700\u5e73\uff09\uff1b
\n (b-c) \u4e0d\u540c\u5149\u7167\u6761\u4ef6\u4e0b\u5236\u5907\u7684\u9499\u949b\u77ff\u7535\u6c60\u7684\u963f\u5c14\u5c3c\u4e4c\u65af\u65b9\u6cd5\u62df\u5408\u7ed3\u679c\uff1b
\n (d) \u6839\u636e\u6df1\u80fd\u7ea7\u77ac\u6001\u5149\u8c31\u6d4b\u8bd5\u5f97\u5230\u7684\u6001\u5bc6\u5ea6\u7ed3\u679c\uff1b
\n (e) \u4e0d\u540c\u5149\u7167\u6761\u4ef6\u4e0b\u5236\u5907\u7684\u9499\u949b\u77ff\u8584\u819c\u7684PL\u5149\u8c31\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n

\u7814\u7a76\u4eba\u5458\u5728\u8be5\u5de5\u4f5c\u4e2d\u5bf9\u6bd4\u4e86\u4e0d\u540c\u6ce2\u957f\u7684\u5149\u5bf9\u8fde\u7eed\u6c14\u76f8\u6c89\u79ef\u6cd5\u5236\u5907\u7684\u9499\u949b\u77ff\u7684\u5f71\u54cd\uff0c\u53d1\u73b0\u5355\u8272\u5149\uff08\u7ea2\u3001\u7eff\u548c\u84dd\uff09\u53ef\u4ee5\u5f15\u8d77\u5364\u5316\u7269\u7684\u5782\u76f4\u5747\u5300\u5316\u5206\u5e03\u4ee5\u53caMA\u5728\u8868\u9762\u7684\u5bcc\u96c6\uff1b\u800c\u767d\u5149\u53ef\u4ee5\u4fc3\u4f7f\u66f4\u591a\u7684\u5364\u5316\u7269\u8fdb\u5165\u819c\u4e2d\uff0c\u5e76\u4e14\u4f7f\u8fc7\u91cf\u7684MA\u4ece\u8868\u9762\u84b8\u53d1\uff0c\u5bfc\u81f4\u6709\u673a\u94f5\u5364\u5316\u7269\u5728\u8584\u819c\u4f53\u76f8\u4e2d\u975e\u5e38\u5747\u5300\u7684\u5782\u76f4\u5206\u5e03\u3002\u9884\u5148\u5149\u7167\u5904\u7406\u5236\u5907\u5f97\u5230\u7684\u9499\u949b\u77ff\u5668\u4ef6\u5185\u90e8\u7f3a\u9677\u5f97\u5230\u6709\u6548\u6d88\u9664\uff0c\u5149\u7a33\u5b9a\u6027\u5927\u5927\u63d0\u9ad8\u3002\u8be5\u767d\u5149\u7167\u660e\u8f85\u52a9\u5408\u6210\u7b56\u7565\u6709\u6548\u6539\u5584\u4e86\u9499\u949b\u77ff\u7684\u5f62\u6210\uff0c\u4e5f\u4e3a\u66f4\u597d\u7684\u9499\u949b\u77ff\u5408\u6210\u73af\u5883\u8bbe\u8ba1\u63d0\u4f9b\u4e86\u6709\u6548\u7684\u501f\u9274\u548c\u6307\u5bfc\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>Reducing Defects in Perovskite Solar Cells with White Light Illumination Assisted Synthesis<\/u><\/a>\uff08ACS Energy Lett.\u00a02019, DOI: 10.1021\/acsenergylett.9b02145\uff09<\/p>\n

\u3010\u901a\u8baf\u4f5c\u8005\/\u56e2\u961f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

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