{"id":188463,"date":"2019-10-29T06:30:23","date_gmt":"2019-10-28T22:30:23","guid":{"rendered":"\/\/m.iemloyee.com\/?p=188463"},"modified":"2019-10-28T14:37:10","modified_gmt":"2019-10-28T06:37:10","slug":"%e3%80%90%e5%ae%a1%e7%a8%bf%e5%b7%b2%e5%9b%9e%e5%a4%8d%e3%80%91%e4%b8%8a%e4%ba%a4%e8%83%a1%e6%99%93%e6%96%8cacs-nano%e9%94%82%e7%a1%ab%e7%94%b5%e6%b1%a0%e9%98%b3%e6%9e%81%e5%92%8c%e9%98%b4%e6%9e%81","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=188463","title":{"rendered":"\u4e0a\u4ea4\u80e1\u6653\u658cACS Nano:\u9502\u786b\u7535\u6c60\u9633\u6781\u548c\u9634\u6781\u76843D\u6709\u5e8f\u591a\u5b54\u7eb3\u7c73\u7ed3\u6784\u8d4b\u4e88\u4f18\u5f02\u7684\u50a8\u80fd\u6027\u80fd"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u4e0e\u9502\u79bb\u5b50\u548c\u9502\u91d1\u5c5e\u7535\u6c60\u7684\u5feb\u901f\u53d1\u5c55\u6709\u5173\uff0c\u7535\u52a8\u6c7d\u8f66\uff08EV\uff09\u548c\u6df7\u5408\u7535\u52a8\u6c7d\u8f66\uff08HEV\uff09\u7684\u5e02\u573a\u8d8a\u6765\u8d8a\u5e7f\u6cdb\u3002\u8fd9\u4e9b\u7535\u52a8\u6c7d\u8f66\u53ef\u4ee5\u901a\u8fc7\u589e\u5f3a\u7684\u8d85\u9ad8\u5bb9\u91cf\u7535\u6c60\u8fdb\u4e00\u6b65\u53d1\u5c55\uff0c\u4f46\u662f\u7531\u4e8e\u7535\u6c60\u7cfb\u7edf\u8fc7\u70ed\uff0c\u9502\u7535\u6c60\u81ea\u71c3\u662f\u4e00\u4e2a\u4e25\u91cd\u7684\u95ee\u9898\u3002\u5b89\u5168\u95ee\u9898\u4e25\u91cd\u5f71\u54cd\u4e86\u6d88\u8d39\u8005\u5bf9\u7535\u52a8\u6c7d\u8f66\u7684\u4fe1\u5fc3\uff0c\u963b\u788d\u5e76\u9650\u5236\u7535\u52a8\u6c7d\u8f66\u7684\u8fdb\u4e00\u6b65\u53d1\u5c55\u3002\u70ed\u5931\u63a7\u662f\u5f15\u8d77\u7535\u6c60\u7cfb\u7edf\u5b89\u5168\u95ee\u9898\u7684\u4e3b\u8981\u56e0\u7d20\uff0c\u5176\u4e3b\u8981\u539f\u56e0\u7531\u4e8e\u7535\u6c60\u7684\u5fae\u89c2\u975e\u5747\u5300\u7535\u5316\u5b66\u53cd\u5e94\u5f15\u8d77\u7684\u3002\u5c40\u90e8\u5fae\u89c2\u53cd\u5e94\u5dee\u5f02\uff0c\u6d3b\u6027\u6750\u6599\u4e0e\u7535\u89e3\u8d28\u6d53\u5ea6\u5fae\u89c2\u5206\u5e03\u4e0d\u5747\u5300\uff0c\u7535\u5b50\u4f20\u8f93\u548c\u79bb\u5b50\u6269\u6563\u4e0d\u5747\u5300\u7b49\u5bfc\u81f4\u7535\u5316\u5b66\u53cd\u5e94\u4e0d\u5747\u5300\uff0c\u4ece\u800c\u5f15\u53d1\u7535\u6c60\u5c40\u90e8\u53cd\u5e94\u8fc7\u70ed\u800c\u5bfc\u81f4\u5b8f\u89c2\u70ed\u5931\u63a7\u3002\u540c\u65f6\uff0c\u6d3b\u6027\u6750\u6599\u7684\u5747\u5300\u5206\u5e03\u548c\u826f\u597d\u7684\u7535\u5b50\u4f20\u8f93\u53ca\u79bb\u5b50\u6269\u6563\u4f1a\u4ea7\u751f\u534f\u540c\u6548\u5e94\uff0c\u6709\u5229\u4e8e\u63d0\u9ad8\u7535\u6c60\u7684\u80fd\u91cf\u5bc6\u5ea6\u548c\u5faa\u73af\u5bff\u547d\u3002<\/p>\n

\u901a\u8fc7\u6784\u5efa\u5177\u6709\u4e09\u7ef4\u6709\u5e8f\u591a\u5b54\u7684\u5149\u5b50\u6676\u4f53\u7ed3\u6784\u4f5c\u4e3a\u7535\u6c60\u7684\u4e3b\u4f53\u7ed3\u6784\uff0c\u6709\u6548\u7684\u5728\u5fae\u89c2\u4e0a\u786e\u4fdd\u6d3b\u6027\u6750\u6599\u3001\u7535\u89e3\u8d28\u7684\u5747\u5300\u5206\u5e03\uff0c\u540c\u65f6\u63d0\u4f9b\u9ad8\u901f\u7684\u7535\u5b50\u4f20\u8f93\u548c\u79bb\u5b50\u6269\u6563\u901a\u9053\uff0c\u4e3a\u9502\u786b\u7535\u6c60\u7684\u56fa\u786b\u548c\u6291\u5236\u9502\u679d\u6676\u63d0\u4f9b\u4e86\u4e00\u4e2a\u79ef\u6781\u6709\u6548\u7684\u89e3\u51b3\u65b9\u6cd5\u3002\u6709\u7814\u7a76\u4eba\u5458\u66fe\u62a5\u9053\u4f7f\u7528\u954d\u5149\u5b50\u6676\u4f53\u548c\u6c22\u5316\u4e8c\u6c27\u5316\u949b\u5149\u5b50\u6676\u4f53\u4f5c\u4e3aLi-S\u7535\u6c60\u7684\u7535\u6781\u7ed3\u6784\u3002\u4f46\u662f\uff0c\u7531\u4e8e\u954d\u8f83\u9ad8\u7684\u8d28\u91cf\u5bc6\u5ea6\u548c\u4e8c\u6c27\u5316\u949b\u8f83\u4f4e\u7684\u5bfc\u7535\u6027\uff0c\u56e0\u6b64\u6211\u4eec\u63a2\u7d22\u5bfb\u6c42\u65e2\u5177\u6709\u9002\u5f53\u7684\u8d28\u91cf\u5bc6\u5ea6\u53c8\u5177\u6709\u9ad8\u7535\u5bfc\u7387\u7684\u5149\u5b50\u6676\u4f53\u3002\u6765\u540c\u65f6\u89e3\u51b3Li-S\u7535\u6c60\u7684\u6b63\u6781\u56fa\u786b\u548c\u8d1f\u6781\u6291\u5236\u9502\u679d\u6676\u95ee\u9898\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb<\/strong>\u3011<\/p>\n

\u8fd1\u65e5\uff0c\u4e0a\u6d77\u4ea4\u901a\u5927\u5b66\u80e1\u6653\u658c\u526f\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7b49\u4eba\u62a5\u9053\u4e86\u4e00\u7c7b\u57fa\u4e8e\u53cc\u5c42\u5149\u5b50\u6676\u4f53\uff08DLPC\uff09\u76843D DLPC@S\/DLPC@Li\u7535\u6c60\uff0c\u8be5\u53cc\u5c42\u5149\u5b50\u6676\u4f53\u5177\u6709\u901a\u8fc7\u80f6\u4f53\u6676\u4f53\u6a21\u677f\u6cd5\u5236\u9020\u76843D\u6709\u5e8f\u4e92\u8fde\u7ed3\u6784\u3002\u6d3b\u6027\u6750\u6599\uff0c\u7535\u5b50\u548c\u79bb\u5b50\u7684\u5747\u5300\u5206\u5e03\u53ef\u786e\u4fdd\u7535\u5316\u5b66\u53cd\u5e94\u7684\u5747\u5300\u6027\u3002\u5b83\u4e5f\u514b\u670d\u4e86\u901a\u8fc7\u5176\u4ed6\u65b9\u6cd5\u5408\u6210\u7684\u591a\u5b54\u6750\u6599\u4e2d\u5e38\u89c1\u7684\u7eb3\u7c73\u9897\u7c92\u805a\u96c6\u548c\u584c\u9677\u7684\u68d8\u624b\u95ee\u9898\u3002\u4e0e\u5176\u4ed6\u53cd\u86cb\u767d\u77f3\u5149\u5b50\u6676\u4f53\u76f8\u6bd4\uff0cDLPC\u5177\u6709\u53cc\u5c42\u7ed3\u6784\uff0c\u56e0\u6b64\u5177\u6709\u66f4\u9ad8\u7684\u7535\u5bfc\u7387\u548c\u66f4\u4f4e\u7684\u7535\u6781\u8d28\u91cf\u6bd4\u3002\u53e6\u5916\uff0c\u5728\u8fd9\u79cdDLPC@S\/DLPC@Li\u5168\u7535\u6c60\u4e2d\uff0c\u786b\u7684\u4f4e\u7535\u5bfc\u7387\uff0c\u663e\u8457\u7684\u7a7f\u68ad\u6548\u5e94\uff0c\u6d3b\u6027\u6750\u6599\u7684\u4f53\u79ef\u81a8\u80c0\u4ee5\u53ca\u5e38\u89c4\u9502\u91d1\u5c5e\u8d1f\u6781\u4e0a\u7684\u9502\u679d\u6676\u7b49\u5e38\u89c1\u95ee\u9898\u4e5f\u5f97\u5230\u4e86\u6709\u6548\u89e3\u51b3\u3002DLPC\u53ef\u4ee5\u901a\u8fc7\u53cc\u5c42\u58c1\u7ed3\u6784\u4e3a\u7535\u5b50\u548c\u901a\u8fc7\u7eb3\u7c73\u901a\u9053\u4e3a\u79bb\u5b50\u63d0\u4f9b\u4e92\u8fde\u7684\u5feb\u901f\u4f20\u8f93\u8def\u5f84\uff0c\u4ece\u800c\u786e\u4fdd\u7535\u6781\u7684\u9ad8\u7535\u5bfc\u7387\u3001\u9ad8\u79bb\u5b50\u4f20\u5bfc\u7387\u548c\u826f\u597d\u7684\u500d\u7387\u6027\u80fd\u3002\u7403\u5f62\u7eb3\u7c73\u5b54\u7684\u8d1f\u66f2\u7387\u4ea7\u751f\u7684\u5f3a\u5927\u6bdb\u7ec6\u4f5c\u7528\u4ee5\u53ca\u91d1\u5c5e\u4e0e\u591a\u786b\u5316\u7269\u4e4b\u95f4\u5316\u5b66\u952e\u7684\u76f8\u4e92\u4f5c\u7528\u963b\u6b62\u4e86\u7a7f\u68ad\u6548\u5e94\u5e76\u63d0\u4f9b\u4e86\u826f\u597d\u7684\u5faa\u73af\u5bff\u547d\u3002DLPC\u7684\u9ad8\u8868\u9762\u79ef\u5728\u7535\u6781\u4e0a\u4ea7\u751f\u4f4e\u7535\u6d41\u5bc6\u5ea6\uff0c\u4e0d\u4ec5\u6709\u52a9\u4e8e\u500d\u7387\u7279\u6027\uff0c\u8fd8\u53ef\u4ee5\u51cf\u5c11\u9633\u6781\u4e0a\u9502\u679d\u6676\u7684\u751f\u957f\u3002\u6709\u5e8f\u7684\u4e92\u8fde\u7eb3\u7c73\u5b54\u8fd8\u963b\u6b62\u4e86\u786b\u548c\u9502\u91d1\u5c5e\u7684\u4f53\u79ef\u81a8\u80c0\uff0c\u4ece\u800c\u8fdb\u4e00\u6b65\u63d0\u9ad8\u4e86\u7535\u6c60\u7684\u5b89\u5168\u6027\u548c\u5faa\u73af\u5bff\u547d\u3002\u4ee4\u4eba\u5370\u8c61\u6df1\u523b\u7684\u662f\uff0c\u5373\u4f7f\u572810 C\u7684\u6781\u9ad8\u500d\u7387\u4e0b\uff0c\u5236\u5907\u7684\u5168\u7535\u6c60\u4ecd\u663e\u793a\u51fa703.3 mAhg-1<\/sup>\u7684\u4f18\u5f02\u6bd4\u5bb9\u91cf\uff0c\u4ee5\u53ca\u51fa\u8272\u7684\u5faa\u73af\u6027\u80fd\uff0c\u57280.5 C\u500d\u7387\u4e0b\u5faa\u73af1200\u6b21\uff0c\u6bcf\u4e2a\u5faa\u73af\u7684\u8d85\u4f4e\u8870\u51cf\u7387\u4e3a0.0317\uff05\u3002\u8fd9\u9879\u5de5\u4f5c\u53ef\u4ee5\u4e3a\u9502\u7535\u6c60\u5728\u5feb\u901f\u5145\u653e\u7535\u4e2d\u7684\u672a\u6765\u5b9e\u9645\u5e94\u7528\u63d0\u4f9b\u4e00\u79cd\u53ef\u884c\u800c\u6709\u6548\u7684\u65b9\u6cd5\u3002\u8be5\u6210\u679c\u4ee5\u9898\u4e3a\u201c<\/strong>3D Ordered Porous Nanostructures for Lithium-Sulfur Battery Anodes and Cathodes Confer Superior Energy Storage Performance<\/strong>\u201d\u53d1\u8868\u5728<\/strong>ACS Nano<\/strong>\u4e0a<\/strong>\u3002\u540c\u65f6\uff0c\u8be5\u7814\u7a76\u5c0f\u7ec4\u6700\u8fd1\u8fd8\u5728Small(DOI: 10.1002\/smll.201800616, DOI: 10.1002\/smll.201804930)<\/strong>\u4e0a\u53d1\u8868\u4e86<\/strong>2<\/strong>\u7bc7\u7cfb\u5217\u6587\u7ae0\uff0c\u5176\u4e2d\u4e00\u7bc7\u8fd8\u88ab\u9009\u4e3a\u5c01\u9762\u8bba\u6587\u3002<\/strong><\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

Scheme 1.DLPC@S\/DLPC@Li<\/strong>\u5168\u7535\u6c60\u7684\u6574\u4e2a\u8fc7\u7a0b\u7684\u793a\u610f\u56fe<\/strong>\u00a0<\/strong>\"\"<\/strong><\/p>\n

Figure 1.<\/strong>\u6837\u54c1\u7684\u5f62\u8c8c<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u4e8c\u6c27\u5316\u7845\u6a21\u677f\u7684SEM\u56fe\u50cf<\/p>\n

\uff08b\uff09\u4e8c\u6c27\u5316\u7845PC@MOF\u7684SEM\u56fe\u50cf<\/p>\n

\uff08c\uff09\u5177\u6709\u4e0d\u540c\u653e\u5927\u500d\u6570\u7684\u78b3PC\u7684SEM\u56fe\u50cf<\/p>\n

\uff08d\uff09\u78b3PC\u7684TEM\u56fe\u50cf<\/p>\n

\uff08e\uff09\u78b3PC\u7684STEM\u56fe\u50cf\u548c\u76f8\u5e94\u7684\u5143\u7d20\u80fd\u8c31\u56fe\u50cf<\/p>\n

\uff08fg\uff09DLPC\u7684SEM\u56fe\u50cf\u548c\u76f8\u5e94\u7684\u5143\u7d20\u80fd\u8c31\u56fe\u50cf<\/p>\n

\uff08h\uff09DLPC@S\u9634\u6781\u7684SEM\u56fe\u50cf\u548c\u76f8\u5e94\u7684\u786b\u8c31\u56fe<\/p>\n

Figure 2.<\/strong>\u6837\u54c1\u7684\u7535\u5316\u5b66\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u6837\u54c1\u7684CV\u6027\u8d28<\/p>\n

\uff08b\uff09DLPC-10@S\u9634\u6781\u5728\u4e0d\u540c\u901f\u7387\u4e0b\u7684\u5145\u7535\/\u653e\u7535\u66f2\u7ebf<\/p>\n

\uff08cd\uff09\u6837\u54c1\u57280.5 C\u548c10 C\u4e0b\u7684\u5faa\u73af\u6027\u80fd<\/p>\n

\uff08e\uff090.5 C\u81f310 C\u7684\u6837\u54c1\u7684\u500d\u7387\u7279\u6027<\/p>\n

\uff08f\uff09\u6837\u54c1\u7684EIS\u66f2\u7ebf<\/p>\n

Figure 3.<\/strong>\u57fa\u4e8e\u7535\u6781\u7684\u603b\u8d28\u91cf\uff0c<\/strong>CC@S, NPC @ S, SLPC@S<\/strong>\u548c<\/strong>DLPC@S<\/strong>\u9634\u6781\u7684\u500d\u7387\u7279\u6027<\/strong><\/p>\n

\"\"<\/p>\n

Figure 4.<\/strong>\u9502\u91d1\u5c5e\u9633\u6781\u7684\u5f62\u8c8c<\/strong><\/p>\n

\"\"<\/p>\n

\uff08ab\uff09\u5faa\u73af\u524d\u540e\u7684\u5e38\u89c4\u9502\u7b94<\/p>\n

\uff08cd\uff09\u5faa\u73af\u524d\u540e\u7684DLPC@Li\u9633\u6781<\/p>\n

Figure 5.<\/strong>\u5bf9\u79f0\u7535\u6c60\u7684\u7535\u5316\u5b66\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08abc\uff09\u5206\u522b\u57281 mA\/cm2<\/sup>\u30013 mA\/cm2<\/sup>\u548c5 mA\/cm2<\/sup>\u4e0b\u7684\u5faa\u73af\u6027\u80fd<\/p>\n

\uff08d\uff091 mA\/cm2<\/sup>\u81f35 mA\/cm2<\/sup>\u7684\u500d\u7387\u7279\u6027<\/p>\n

\uff08e\uff0910\u4e2a\u5faa\u73af\u540e\u7684EIS\u66f2\u7ebf<\/p>\n

Figure 6.Li<\/strong>\u5265\u79bb<\/strong>\/<\/strong>\u9540\u8986\u884c\u4e3a<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u5e38\u89c4\u9502\u7b94\u7684Li\u5265\u79bb\u884c\u4e3a<\/p>\n

\uff08b\uff09DLPC@Li\u9633\u6781\u7684Li\u5265\u79bb\u884c\u4e3a<\/p>\n

\uff08c\uff09\u5e38\u89c4\u9502\u7b94\u7684\u9502\u7535\u9540\u884c\u4e3a<\/p>\n

\uff08d\uff09DLPC@Li\u9633\u6781\u7684Li\u7535\u9540\u884c\u4e3a<\/p>\n

Figure 7.DLPC@S\/DLPC@Li<\/strong>\u5168\u7535\u6c60\u7684\u7535\u5316\u5b66\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff091.6 V\u81f32.8 V\u7684CV\u6027\u80fd<\/p>\n

\uff08b\uff09\u5145\u653e\u7535\u66f2\u7ebf\u4ece0.5 C\u523010 C<\/p>\n

\uff08c\uff09\u5206\u522b\u57280.5 C\u548c10 C\u500d\u7387\u4e0b\u7684\u5faa\u73af\u6027\u80fd<\/p>\n

\uff08d\uff090.5 C\u81f310 C\u7684\u500d\u7387\u7279\u6027<\/p>\n

\uff08e\uff09EIS\u66f2\u7ebf<\/p>\n

\u3010\u603b\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5<\/strong>\uff1a3D Ordered Porous Nanostructures for Lithium-Sulfur Battery Anodes and Cathodes Confer Superior Energy Storage Performance<\/a>. ACS Nano<\/em>, 2019<\/strong>, DOI: 10.1021\/acsnano.9b05718<\/p>\n

\u901a\u8baf\u4f5c\u8005<\/strong>\/<\/strong>\u56e2\u961f\u7b80\u4ecb<\/strong><\/p>\n

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