{"id":188207,"date":"2019-10-28T06:30:38","date_gmt":"2019-10-27T22:30:38","guid":{"rendered":"\/\/m.iemloyee.com\/?p=188207"},"modified":"2019-10-27T19:56:38","modified_gmt":"2019-10-27T11:56:38","slug":"%e3%80%90%e5%ae%a1%e7%a8%bf%e5%b7%b2%e5%9b%9e%e5%a4%8d%e3%80%91%e5%a4%a7%e8%bf%9e%e7%90%86%e5%b7%a5%e5%a4%a7%e5%ad%a6%e7%b2%be%e7%bb%86%e5%8c%96%e5%b7%a5%e5%9b%bd%e5%ae%b6%e9%87%8d%e7%82%b9%e5%ae%9e","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=188207","title":{"rendered":"\u5927\u8fde\u7406\u5de5\u5927\u5b66\u7cbe\u7ec6\u5316\u5de5\u56fd\u5bb6\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u5f6d\u5b5d\u519b\u9662\u58eb\u8bfe\u9898\u7ec4Acc. Chem. Res.: \u57fa\u4e8e\u5149\u611f\u5e94\u7535\u5b50\u8f6c\u79fb\u7684\u4f20\u611f\u548c\u8bca\u7597\u63a2\u9488"},"content":{"rendered":"

\u3010\u5f15\u8a00<\/strong>\u3011<\/p>\n

\u7531\u4e8e\u8367\u5149\u63a2\u9488\u7684\u9ad8\u7075\u654f\u5ea6\uff0c\u7279\u5f02\u6027\uff0c\u5feb\u901f\u54cd\u5e94\u548c\u6280\u672f\u7b80\u4fbf\u6027\uff0c\u5b83\u4eec\u5df2\u6210\u4e3a\u68c0\u6d4b\uff0c\u6210\u50cf\u548c\u75be\u75c5\u8bca\u65ad\u7684\u5f3a\u5927\u5de5\u5177\u3002\u5728\u8fc7\u53bb\u7684\u51e0\u5341\u5e74\u4e2d\uff0c\u7814\u7a76\u4eba\u5458\u5728\u5f00\u53d1\u7528\u4e8e\u8bbe\u8ba1\u8367\u5149\u63a2\u9488\u7684\u4fe1\u53f7\u4f20\u5bfc\u673a\u5236\u65b9\u9762\u53d6\u5f97\u4e86\u663e\u7740\u8fdb\u5c55\uff0c\u4f8b\u5982\u5149\u81f4\u7535\u5b50\u8f6c\u79fb\uff08PET\uff09\uff0c\u5206\u5b50\u5185\u7535\u8377\u8f6c\u79fb\uff08ICT\uff09\u548c\u8367\u5149\u5171\u632f\u80fd\u91cf\u8f6c\u79fb\uff08FRET\uff09\u3002\u5178\u578b\u7684PET\u7531\u591a\u7ec4\u5206\u7cfb\u7edf\u7ec4\u6210\uff0c\u5176\u4e2d\u8367\u5149\u56e2\uff08\u7535\u5b50\u53d7\u4f53\uff09\u901a\u8fc7\u4e00\u4e2a\u77ed\u7684\u95f4\u9694\u5b50\u4e0e\u4e00\u4e2a\u8bc6\u522b\u57fa\u56e2\uff08\u7535\u5b50\u4f9b\u4f53\uff09\u5206\u5f00\u8fde\u63a5\u3002PET\u63a2\u9488\u901a\u5e38\u5177\u6709\u4f4e\u8367\u5149\u80cc\u666f\u548c\u663e\u7740\u7684\u8367\u5149\u589e\u5f3a\u54cd\u5e94\u76ee\u6807\u3002\u6700\u8fd1\u7684\u7814\u7a76\u8868\u660e\uff0cPET\u63a2\u9488\u4e5f\u5df2\u88ab\u7528\u4f5c\u6cbb\u7597\u8bca\u65ad\u5242\uff0c\u5176\u8367\u5149\u548c\u6bd2\u6027\u53ef\u901a\u8fc7\u764c\u75c7\u7279\u5b9a\u53c2\u6570\u540c\u65f6\u6fc0\u6d3b\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb<\/strong>\u3011<\/p>\n

\u8fd1\u65e5\uff0c\u5927\u8fde\u7406\u5de5\u5927\u5b66\u7cbe\u7ec6\u5316\u5de5\u5f6d\u5b5d\u519b\u9662\u58eb\u56e2\u961f<\/strong>\u5728\u8fd9\u7bc7\u7efc\u8ff0\u4e2d\u91cd\u70b9\u4ecb\u7ecd\u4e86PET\u63a2\u9488\u5408\u7406\u8bbe\u8ba1\u548c\u5e94\u7528\u7684\u6700\u65b0\u8fdb\u5c55\uff0c\u4e3b\u8981\u4fa7\u91cd\u4e8e\u4f5c\u8005\u56e2\u961f\u7684\u7814\u7a76\u3002\u4f8b\u5982\uff0c\u4e0e\u5178\u578bPET\u4e2d\u4f20\u7edf\u7684\u5355\u539f\u5b50\u7535\u5b50\u4f9b\u4f53\uff08O\uff0cS\uff0cN\uff0cSe\uff0cTe\u7b49\uff09\u4e0d\u540c\uff0c\u4f5c\u8005\u4f7f\u7528\u4e86\u66f4\u591a\u7684\u5bcc\u7535\u5b50\u5421\u54af\u73af\u6765\u201c\u731d\u706d\u201d\u8367\u5149\u7684\u8367\u5149\u3002\u8367\u5149\u56e2\u901a\u8fc7\u201c\u589e\u5f3a\u7684PET\u201d\u6548\u5e94\u66f4\u6709\u6548\u5730\u4ea7\u751f\uff0c\u8be5\u6548\u5e94\u63d0\u4f9b\u4e86\u8f83\u4f4e\u7684\u80cc\u666f\u8367\u5149\u548c\u8f83\u9ad8\u7684\u4fe1\u566a\u6bd4\u3002\u6b64\u5916\uff0c\u666e\u901aPET\u4ee3\u8868\u4e86\u5c0f\u5206\u5b50\u201coff-on\u201d\u8367\u5149\u4f20\u611f\u5668\u8bbe\u8ba1\u80cc\u540e\u7684\u4e3b\u8981\u539f\u7406\u3002\u4f5c\u8005\u901a\u8fc7\u5206\u5b50\u5185\u7a7a\u95f4\u6298\u53e0\u5f00\u53d1\u4e86\u65b0\u7684PET\u5e73\u53f0\uff0c\u4ece\u800c\u514b\u670d\u4e86\u8bbe\u8ba1PET\u9176\u9776\u5411\u63a2\u9488\u7684\u96be\u9898\u3002\u56e0\u6b64\uff0c\u4f8b\u5982\uff0c\u57fa\u4e8e\u5178\u578b\u7684PET\u548c\u8fd9\u4e9b\u65b0\u7684PET\u6982\u5ff5\uff0c\u4f5c\u8005\u62a5\u544a\u4e86\u7528\u4e8e\u68c0\u6d4bZn2+\u800c\u65e0\u8d28\u5b50\u5e72\u6270\u7684PET\u63a2\u9488\uff0c\u7528\u4e8e\u62a5\u544a\u6eb6\u9176\u4f53\u4e2d\u5c40\u90e8\u4eb2\u6c34\u6027\u7684\u57fa\u4e8eBODIPY\u7684d-PET\u63a2\u9488\uff0c\u4ee5\u53ca\u201c\u589e\u5f3a\u578bPET\u201d\u8367\u5149\u63a2\u9488\uff0c\u7528\u4e8e\u5bf9\u764c\u7ec6\u80de\u4e2d\u7684HClO\u8fdb\u884c\u6210\u50cf\u3002\u6b64\u5916\u56e2\u961f\u8fd8\u5f00\u53d1\u4e86\u7528\u4e8e\u8bc6\u522b\u764c\u7ec6\u80de\u548c\u5b9a\u91cf\u764c\u75c7\u7684COX-2\u7279\u5f02\u6027\u63a2\u9488\uff0c\u4ee5\u53ca\u7528\u4e8e\u8ddf\u8e2a\u6d3b\u5c0f\u9f20\u5b9e\u4f53\u7624\u7684KIAA1363\u654f\u611f\u63a2\u9488\u3002\u4f5c\u8005\u9996\u5148\u5c06\u57fa\u4e8ePET\u7684\u6c28\u57fa\u80bd\u9176N\uff08APN\uff09\u654f\u611f\u63a2\u9488\u7528\u4e8e\u764c\u75c7\u8bca\u65ad\u548c\u6cbb\u7597\u3002\u9884\u8ba1\u8fdb\u4e00\u6b65\u5f00\u53d1\u63d0\u4f9b\u5bf9\u76ee\u6807\u5206\u6790\u7269\u66f4\u9ad8\u7684\u7075\u654f\u5ea6\u548c\u9009\u62e9\u6027\u7684PET\u8367\u5149\u63a2\u9488\u5c06\u5177\u6709\u66f4\u591a\u529f\u80fd\uff0c\u5e76\u5728\u75c5\u7406\u5b66\uff0c\u8bca\u65ad\u5b66\u548c\u764c\u75c7\u6cbb\u7597\u7684\u7814\u7a76\u4e2d\u8d77\u4e0d\u53ef\u6216\u7f3a\u7684\u4f5c\u7528\u3002\u8be5\u6210\u679c\u4ee5\u9898\u4e3a\u201c<\/strong>Activity-Based Sensing and Theranostic Probes Based on Photoinduced Electron Transfer<\/strong>\u201d\u53d1\u8868\u5728<\/strong>Acc. Chem. Res.<\/strong>\u4e0a<\/strong>\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

Figure 1.PET<\/strong>\u673a\u7406\u7684\u524d\u6cbf\u8f68\u9053\u80fd\u91cf\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

Figure 2.Zn2+<\/sup><\/strong>\u63a2\u9488\u7684\u7ed3\u6784\u548c\u673a\u7406\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

Figure 3.<\/strong>\u63a2\u9488\u5206\u5b50\u7684\u7ed3\u6784\u548c\u673a\u7406\u793a\u610f\u56fe<\/strong>\"\"<\/strong><\/p>\n

\uff08A\uff09N5\uff0cN4\u548cNMO\u7684\u5316\u5b66\u7ed3\u6784<\/p>\n

\uff08B\uff09N5\uff0cN4\u548cNMO\u7684\u524d\u6cbf\u5206\u5b50\u8f68\u9053\u80fd\u91cf\u63d2\u56fe<\/p>\n

Figure 4.Hg2+<\/sup><\/strong>\u63a2\u9488\u7684\u7ed3\u6784\u548c\u673a\u7406\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

Figure 5.<\/strong>\u63a2\u9488\u5206\u5b50<\/strong>B3<\/strong>\u7684\u7ed3\u6784\u4e0e\u68c0\u6d4b\u6027\u80fd\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09B3\u7684\u5316\u5b66\u7ed3\u6784<\/p>\n

\uff08B\uff09\u6dfb\u52a0Hg2+<\/sup>\u540eB3\u7684\u8367\u5149\u54cd\u5e94<\/p>\n

\uff08C\uff09\u5728Hg2+<\/sup>\u548cS2-<\/sup>\u6216EDTA\u5b58\u5728\u4e0bB3\u7684\u8367\u5149\u54cd\u5e94<\/p>\n

Figure 6.BTCu<\/strong>\u7684\u5316\u5b66\u7ed3\u6784\u548c\u4f20\u611f\u673a\u7406<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09BTCu\u5bf9Cu2+<\/sup>\u7684\u5316\u5b66\u7ed3\u6784\u548c\u4f20\u611f\u673a\u7406<\/p>\n

\uff08B\uff09\u5728\u6709\u6216\u6ca1\u6709Cu2+<\/sup>\u7684\u60c5\u51b5\u4e0bBTCu\u5b75\u80b2\u540eHeLa\u7ec6\u80de\u7684\u8367\u5149\u56fe\u50cf<\/p>\n

Figure 7.<\/strong>\u63a2\u9488\u5206\u5b50<\/strong>RC1<\/strong>\u5bf9<\/strong>Ag+<\/sup><\/strong>\u7684\u54cd\u5e94<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09RC1\u5bf9Ag+<\/sup>\u7684\u5316\u5b66\u7ed3\u6784\u548c\u4f20\u611f\u673a\u7406<\/p>\n

\uff08B\uff09\u5728\u6d3bMCF-7\u7ec6\u80de\u4e2d\u4f7f\u7528RC-1\u7684Ag+<\/sup>\u6c34\u5e73\u7684\u8367\u5149\u56fe\u50cf<\/p>\n

Figure 8.<\/strong>\u5def\u57fa\u68c0\u6d4b\u8367\u5149\u63a2\u9488<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A-C\uff09\u63a2\u9488\u5206\u5b50\u7684\u7ed3\u6784\u548c\u68c0\u6d4b\u673a\u7406<\/p>\n

\uff08D\uff09\u63a2\u9488\u5206\u5b50\u7684\u53cc\u5149\u5b50\u6210\u50cf<\/p>\n

Figure 9.<\/strong>\u8367\u5149\u63a2\u9488\u5bf9<\/strong>ClO–<\/sup><\/strong>\u7684\u68c0\u6d4b<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09\u4eceBClO\u5230HClO\u7684\u5316\u5b66\u7ed3\u6784\u548c\u4f20\u611f\u673a\u7406<\/p>\n

\uff08B\uff09\u6dfb\u52a0NaClO\u540e\uff0cBClO\u7684\u8367\u5149\u54cd\u5e94<\/p>\n

\uff08C\uff09\u901a\u8fc7\u4f7f\u7528BClO\u76d1\u6d4b\u7531\u4f0a\u53f8\u83ab\u5c14\u5728\u6d3b\u7684MCF-7\u7ec6\u80de\u4e2d\u8bf1\u5bfc\u7684\u65f6\u95f4\u4f9d\u8d56\u6027HClO\u751f\u6210\u7684\u8367\u5149<\/p>\n

Figure 10.NI-OPD<\/strong>\u7684\u7ed3\u6784\u3001\u673a\u7406\u4e0e\u68c0\u6d4b<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09NI-OPD\u7684\u5316\u5b66\u7ed3\u6784\u548c\u4f20\u611f\u673a\u7406<\/p>\n

\uff08B\uff09\u6dfb\u52a0\u7532\u57fa\u4e59\u4e8c\u919b\u540eNI-OPD\u7684\u8367\u5149\u54cd\u5e94<\/p>\n

\uff08C\uff09\u6b63\u5e38\u548c\u7cd6\u5c3f\u75c5\u5c0f\u9f20\u7ec4\u7ec7\u4e2dMGO\u7684\u8367\u5149\u6210\u50cf\u3002<\/p>\n

Figure 11.B1<\/strong>\u548c<\/strong>B2<\/strong>\u5bf9\u6c22\u79bb\u5b50\u7684\u68c0\u6d4b<\/strong><\/p>\n

\"\"<\/p>\n

Figure 12.CI3<\/strong>\u7684\u68c0\u6d4b\u673a\u7406\u548c\u6210\u50cf<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09CI3\u5bf9H+<\/sup>\u7684\u5316\u5b66\u7ed3\u6784\u548c\u4f20\u611f\u673a\u7406<\/p>\n

\uff08B\uff09MCF-7\u7ec6\u80de\u4e2d1<\/sup>O2<\/sub>\u751f\u6210\u7684\u8367\u5149\u56fe\u50cf<\/p>\n

Figure 13.<\/strong>\u8367\u5149\u63a2\u9488\u7684\u5206\u5b50\u7ed3\u6784\u548c\u68c0\u6d4b<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09BP1-4\u7684\u5316\u5b66\u7ed3\u6784<\/p>\n

\uff08B\uff09BP-2\u5bf9\u6781\u6027\u7684\u8367\u5149\u54cd\u5e94<\/p>\n

\uff08C\uff09BP-2\u4e2dd-PET\u8fc7\u7a0b\u7684\u524d\u6cbf\u8f68\u9053\u80fd\u91cf\u8868\u793a<\/p>\n

\uff08D\uff09\u8367\u5149\u56fe\u50cf<\/p>\n

Figure 14.<\/strong>\u63a2\u9488\u5206\u5b50\u7684\u7ed3\u6784\u4e0e\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09ANQ-IMC-6\u5bf9COX-2\u7684\u5316\u5b66\u7ed3\u6784\u548c\u4f20\u611f\u673a\u7406<\/p>\n

\uff08B\uff09\u6dfb\u52a0\u51cb\u4ea1\u8bf1\u5bfc\u5242\uff08\u8336\u591a\u915a\uff09\u540e0\u5c0f\u65f6\uff08a\uff09\uff0c6\u5c0f\u65f6\uff08b\uff09\u548c24\u5c0f\u65f6\uff08c\uff09\uff0c\u7528ANQ-IMC-6\u67d3\u8272\u7684MCF-7\u7ec6\u80de\u7684\u9ad8\u5c14\u57fa\u4f53\u5f62\u6001\u53d8\u5316<\/p>\n

\uff08C\uff09\uff08B\uff09\u7684\u653e\u5927\u56fe\u50cf<\/p>\n

\uff08D\uff09BTDAN-COX-2\u7684\u5316\u5b66\u7ed3\u6784<\/p>\n

Figure 15.<\/strong>\u63a2\u9488\u5206\u5b50\u7684\u7ed3\u6784\u4e0e\u6210\u50cf<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09Niblue-C6-IMC\u7684\u5316\u5b66\u7ed3\u6784<\/p>\n

\uff08B\uff09\u4f53\u5185\u80bf\u7624\u5149\u5b66\u6210\u50cf\u548c\u7ade\u4e89\u6027\u963b\u65ad\u7814\u7a76<\/p>\n

Figure 16.NANQ-IMC6<\/strong>\u7684\u7ed3\u6784\u4e0e\u6210\u50cf<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09NANQ-IMC6\u7684\u5316\u5b66\u7ed3\u6784<\/p>\n

\uff08B\uff09\u901a\u8fc7\u9759\u8109\u5185\u6ce8\u5c04NANQ-IMC6\u5bf9\u4f53\u5185\u80bf\u7624\u8fdb\u884c\u8367\u5149\u6210\u50cf<\/p>\n

\uff08C\uff09\u5728\u65e5\u5149\u6216\u7d2b\u5916\u7ebf\u7167\u5c04\u4e0b\uff0c\u88abNANQ-IMC6\u67d3\u8272\u7684\u4e0d\u540c\u7ec4\u7ec7\u7684\u8367\u5149\u5f3a\u5ea6<\/p>\n

\uff08D\uff09\uff08C\uff09\u4e2d\u7ec4\u7ec7\u7684ELISA\u5206\u6790<\/p>\n

Figure 17.<\/strong>\u63a2\u9488\u5206\u5b50<\/strong>NB-AX<\/strong>\u7684\u7ed3\u6784\u4e0e\u6210\u50cf<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09NB-AX\u7684\u5316\u5b66\u7ed3\u6784\u548c\u68c0\u6d4b\u673a\u7406<\/p>\n

\uff08B\uff09\u901a\u8fc7\u6d41\u5f0f\u7ec6\u80de\u672f\u5206\u6790NB-AX\u6807\u8bb0\u7684\u764c\u7ec6\u80de\u7cfb\u548c\u975e\u764c\u7ec6\u80de\u7cfb<\/p>\n

\uff08C\uff09\u90e8\u5206\u764c\u7ec4\u7ec7\u548c\u90e8\u5206\u90bb\u8fd1\u7ec4\u7ec7\u7684\u8367\u5149\u6210\u50cf<\/p>\n

Figure 18.NB-BF<\/strong>\u7684\u7ed3\u6784\u4e0e\u6210\u50cf<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09NB-BF\u5bf9Pim-1\u6fc0\u9176\u7684\u5316\u5b66\u7ed3\u6784\u548c\u4f20\u611f\u673a\u7406<\/p>\n

\uff08B\uff09\u6b63\u5e38\u7ec4\u7ec7\u548c\u764c\u7ec4\u7ec7\u7684\u8367\u5149\u56fe\u50cf<\/p>\n

\uff08C\uff09\u901a\u8fc7\u76ae\u4e0b\u6ce8\u5c04NB-BF\u5bf9\u80bf\u7624\u8fdb\u884c\u4f53\u5185\u8367\u5149\u6210\u50cf<\/p>\n

Figure 19.NBFMeI<\/strong>\u7684\u7ed3\u6784\u4e0e\u6210\u50cf<\/strong><\/p>\n

\"\"<\/p>\n

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\u3010\u603b\u7ed3\u3011<\/strong><\/p>\n

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\u8be5\u7efc\u8ff0\u7b2c\u4e00\u4f5c\u8005\u4e3a\u5927\u8fde\u7406\u5de5\u5927\u5b66\u5b59\u6587\u526f\u6559\u6388\uff0c\u5171\u540c\u901a\u8baf\u4f5c\u8005\u4e3a\u6a0a\u6c5f\u8389\u6559\u6388\uff0c\u5f6d\u5b5d\u519b\u9662\u58eb\u3002<\/p>\n

\u8bfe\u9898\u7ec4\u4e3b\u9875\uff1ahttp:\/\/peng-group.dlut.edu.cn\/<\/p>\n

 <\/p>\n

\u6587\u732e\u94fe\u63a5<\/strong>\uff1aActivity-Based Sensing and Theranostic Probes Based on Photoinduced Electron Transfer<\/a>. Acc. Chem. Res.<\/em>, 2019<\/strong>, DOI: 10.1021\/acs.accounts.9b00340.<\/p>\n

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