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Am. Chem. Soc.<\/b><\/strong>\u4e0a\u3002<\/p>\n \u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/p>\n \u56fe1.<\/p>\n (a-e) Bi-MOF\u8f6c\u5316\u6210Bi\u5355\u539f\u5b50\u7684\u8fc7\u7a0b\u7684\u793a\u610f\u56fe\u4ee5\u53ca\u4e0d\u540c\u6e29\u5ea6\u4e0b\u53cc\u6c30\u80fa\u8f85\u52a9\u70ed\u89e3\u7684Bi-MOF\u7684TEM\u56fe<\/p>\n \u56fe2.<\/p>\n Bi SAs\/NC\u7684(a) TEM\u56fe\u3001(b) STEM\u56fe\u3001(c) SAED\u56fe\u3001(d, e)\u653e\u5927\u7684HAADF-STEM\u56fe\u548c(f) EDS\u5143\u7d20\u5206\u6790\u7684\u7ed3\u679c\u3002<\/p>\n \u56fe3.<\/p>\n \uff08b\uff09Bi SAs\/NC\u3001Bi Cs\/NC\u548cBi NPs\/NC\u7684C K-edge XANES\u56fe<\/p>\n \uff08c\uff09EXAFS\u56fe\u7684k3<\/sup>\u52a0\u6743\u7684\u03c7(k)\u51fd\u6570<\/p>\n \uff08d\uff09Bi SAs\/NC\u7684EXAFS\u62df\u5408<\/p>\n \u56fe4.<\/p>\n (a-c) Bi SAs\/NC\u3001Bi Cs\/NC\u548cBi NPs\/NC\u7684(a) LSV\u66f2\u7ebf\u3001(b) CO\u6cd5\u62c9\u7b2c\u6548\u7387\u548c(c) CO\u7535\u6d41\u5bc6\u5ea6\uff1b<\/p>\n (d) Bi SAs\/NC\u548c\u5927\u90e8\u5206\u6700\u65b0\u7684CO2<\/sub>\u8fd8\u539f\u6210CO\u7684\u53cd\u5e94\u7684\u50ac\u5316\u5242\u7684TOF\u7684\u5bf9\u6bd4<\/p>\n \u56fe5.<\/p>\n \uff08b\uff09\u63d0\u51faBiN4<\/sub>\/C\u8868\u9762\u4e0a\u8fdb\u884c\u7684\u6574\u4e2aCO2<\/sub>\u7535\u8fd8\u539f\u53cd\u5e94\u7684\u53cd\u5e94\u8def\u5f84<\/p>\n \uff08c\uff09BiN4<\/sub>\/C\u3001BiC4<\/sub>\u548cBi(110)\u7684CO2<\/sub>\u7535\u8fd8\u539f\u53cd\u5e94\u548c\u6790\u6c22\u53cd\u5e94\u7684\u6781\u9650\u7535\u4f4d\u7684\u5dee\u503c<\/p>\n \u6587\u732e\u94fe\u63a5\uff1aBismuth Single Atoms Resulting from Transformation of Metal\u2013Organic Frameworks and Their Use as Electrocatalysts for CO<\/u>2<\/sub><\/u>\u00a0Reduction<\/u><\/a>\uff08<\/b><\/strong>J. Am. Chem. Soc.\uff0c2019\uff0cDOI\uff1a10.1021\/jacs.9b08259<\/a>\uff09<\/b><\/strong><\/p>\n <\/b>\uff081\uff09 \u56e2\u961f\u4ecb\u7ecd \uff1b<\/b><\/strong><\/p>\n \u5f20\u52a0\u6d9b<\/b><\/strong>\u7814\u7a76\u56e2\u961f<\/b><\/strong>\u805a\u7126\u5316\u5b66\u5408\u6210\u6cd5\u7cbe\u51c6\u6784\u5efa\u539f\u5b50\u7ea7\u7cbe\u5ea6\u5f02\u8d28\u754c\u9762\u7684\u5355\u539f\u5b50\u6d3b\u6027\u4f4d\u70b9\u3001\u96f6\u7ef4\u3001\u4e8c\u7ef4\u7b49\u4f4e\u7ef4\u7eb3\u7c73\u7ed3\u6784\u57fa\u5143\uff0c\u5229\u7528\u4e8c\u7ef4\u3001\u4e09\u7ef4\u8d85\u6676\u683c\u7ec4\u88c5\u4ee5\u53ca\u8de8\u5c3a\u5ea6\u7684\u8868\/\u754c\u9762\u6539\u6027\uff0c\u5b9e\u73b0\u5149\u7535\u7b49\u6027\u80fd\u7684\u4f20\u9012\u3001\u96c6\u6210\u3001\u8026\u5408\u3002\u5f53\u524d\uff0c\u672c\u8bfe\u9898\u7ec4\u9762\u5411\u5149\u7535\u8f6c\u6362\u7684\u65b0\u80fd\u6e90\u53ca\u751f\u7269\u7528\u7eb3\u7c73\u6750\u6599\uff0c\u7cbe\u51c6\u8bbe\u8ba1\u3001\u5408\u6210\u5e76\u7814\u7a76\u5176\u5728\u5149\u50ac\u5316\u3001\u5149\u7535\u50ac\u5316\u3001\u5149\u7535\u63a2\u6d4b\u3001\u7535\u50ac\u5316\u7b49\u65b0\u80fd\u6e90\u53ca\u5149\u70ed\u3001\u5149\u52a8\u529b\u751f\u7269\u764c\u75c7\u6cbb\u7597\u7b49\u65b9\u9762\u7684\u5e94\u7528\u7814\u7a76\uff0c\u53d6\u5f97\u4e86\u4e00\u7cfb\u5217\u6709\u7279\u8272\u7684\u79d1\u7814\u6210\u679c\u3002\u8bfe\u9898\u7ec4\u5305\u62ec1\u540d\u526f\u6559\u6388\uff0c1\u540d\u7814\u7a76\u5458\uff0c2\u540d\u526f\u7814\u7a76\u5458\u548c1\u540d\u8bb2\u5e08\u3002\u8fd15\u5e74\uff0c\u4ee5\u901a\u8baf\u4f5c\u8005\u5355\u4f4d\u53d1\u8868\u8bba\u658770\u4f59\u7bc7\uff0c\u5305\u62ecNature\u00a0Nanotech\uff081\u7bc7\uff09\u3001JACS\uff081\u7bc7\uff09\u3001Adv. Mater. (3\u7bc7)\u3001Angew. Chem. Int. Ed.\u00a0(2\u7bc7)\u3001Nano\u00a0Energy\uff082\u7bc7\uff09\u3001Adv.\u00a0Engergy\u00a0Mater.\uff081\u7bc7\uff09\u3001Adv. Funct. Mater.\uff081\u7bc7\uff09\u3001Adv. Sci. (1\u7bc7\uff0cESI\u9ad8\u88ab\u5f15)\u4ee5\u53caJ. Phys. Chem. Lett.\uff083\u7bc7\uff09\u3001Chem. Mater.\uff082\u7bc7\uff09\u3001Small\u3001J. Mater. Chem. A\u00a0\uff084\u7bc7\uff09\u3001Nano\u00a0Res.\u3001NPG Asia Mater.\u3001ACS Appl. Mater. Interfaces\u3001Chem. Eur. J.\u7b49\u3002\u7814\u7a76\u5de5\u4f5c\u88abNature\u7f51\u7ad9\u3001ACS\u7f51\u7ad9\u3001Wiley\u7f51\u7ad9\u7b49\u4e13\u9898\u3001\u89c6\u9891\u62a5\u9053\u548cHighlight\u3002\u88abNature\u3001Science\u3001Chem. Rev.\u3001J. Am. Chem. Soc.\u7b49\u520a\u7269\u51e0\u5341\u6b21\u6b63\u9762\u5f15\u7528\u548c\u5927\u7bc7\u5e45\u62a5\u9053\u3002<\/p>\n \u5f20\u52a0\u6d9b\uff0c\u6559\u6388\uff0c\u535a\u58eb\u751f\u5bfc\u5e08\uff0c\u56fd\u5bb6\u4f18\u79c0\u9752\u5e74\u57fa\u91d1\u83b7\u5f97\u8005\uff0c\u82f1\u56fd\u7687\u5bb6\u5316\u5b66\u4f1a\u4f1a\u58eb\uff08FRSC\uff09\u3002\u7ed3\u6784\u53ef\u63a7\u5148\u8fdb\u529f\u80fd\u6750\u6599\u4e0e\u7eff\u8272\u5e94\u7528\u5317\u4eac\u5e02\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u4e3b\u4efb\u30022006\u5e74\u6e05\u534e\u5927\u5b66\u535a\u58eb\u5b66\u4f4d\u30022006.9-2007.11\uff0c\u5fb7\u56fd\u5361\u5c14\u65af\u9c81\u5384\u5927\u5b66\u535a\u58eb\u540e\u30022008.1-2011.1\uff0c\u7f8e\u56fd\u9a6c\u91cc\u5170\u5927\u5b66\u52a9\u7406\u7814\u7a76\u5458\u3002\u5148\u540e\u83b7\u5f97\u6559\u80b2\u90e8\u201c\u65b0\u4e16\u7eaa\u4f18\u79c0\u4eba\u624d\u201d\u3001\u201c\u5317\u4eac\u5e02\u4f18\u79c0\u4eba\u624d\u201d\u3001\u56fd\u5bb6\u4f18\u79c0\u9752\u5e74\u57fa\u91d1\u7b49\u3002\u4e00\u4f5c\u6216\u901a\u8baf\u4f5c\u8005\u5728Nature\u3001Science\u3001Nature Nanotech.\u3001JACS\u3001Angew. 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Mater.\u7b49\u671f\u520a\u53d1\u8868SCI\u8bba\u658770\u4f59\u7bc7\uff0c\u53d7\u9080\u4e13\u8457\/\u7ae0\u82827\u90e8\uff0c\u4ed6\u5f154000\u4f59\u6b21\u3002\u4e3b\u6301\/\u53c2\u4e0e\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u91cd\u5927\/\u91cd\u70b9\u9879\u76ee\u3001\u4f18\u9752\/\u9762\u4e0a\u9879\u76ee\u7b497\u9879\u3002\u62c5\u4efb\u7eb3\u7c73\u6750\u6599\u4e0e\u5668\u4ef6\u5206\u4f1a\u526f\u79d8\u4e66\u957f\uff0cPNS: MI\u3001Rare Metals SCI\u671f\u520a\u7f16\u59d4\u3002\u8363\u83b7IUPAC\u6770\u51fa\u6210\u5c31\u5956\u3001\u4e2d\u56fd\u6750\u6599\u5b66\u672f\u8054\u76dfIFAM2018\u9752\u5e74\u79d1\u5b66\u5bb6\u5956\u7b49\u3002<\/p>\n \uff082\uff09\u56e2\u961f\u5728\u8be5\u9886\u57df\u7684<\/b><\/strong>\u5178\u578b<\/b><\/strong>\u5de5\u4f5c\u6c47\u603b \uff1b<\/b><\/strong><\/p>\n \u672c\u6587\u7531kv1004\u4f9b\u7a3f\u3002<\/p>\n","protected":false},"excerpt":{"rendered":" \u3010\u5f15\u8a00\u3011 \u4e3a\u4e86\u51cf\u8f7bCO2\u6392\u653e\u548c\u79ef\u805a\uff0c\u6700\u5177\u5438\u5f15\u529b\u7684\u65b9\u6cd5\u4e4b\u4e00\u662f\u5229\u7528\u7535\u80fd\u5c06CO2\u7535\u8fd8\u539f\u6210\u6e05\u6d01\u80fd\u6e90\u3002\u7136\u800c\uff0cCO2\u7535\u8fd8\u539f\u53cd\u5e94\u7684\u50ac\u5316\u5242\u9700\u8981\u9ad8\u7684\u8fc7\u7535\u4f4d\uff0c\u5728\u52a8\u529b\u5b66\u4e0a\u80dc\u4e8eCO2\u8fd8…<\/p>\n","protected":false},"author":1592,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[],"class_list":["post-187323","post","type-post","status-publish","format-standard","hentry","category-jiedu"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/187323"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/1592"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=187323"}],"version-history":[{"count":7,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/187323\/revisions"}],"predecessor-version":[{"id":188654,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/187323\/revisions\/188654"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=187323"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=187323"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=187323"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}
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\uff08a\uff09Bi SAs\/NC\u3001Bi Cs\/NC\u548cBi NPs\/NC\u7684N K-edge XANES\u56fe<\/p>\n
<\/p>\n
\uff08a\uff09\u4e0d\u540c\u50ac\u5316\u5242\u50ac\u5316\u7684CO2<\/sub>\u7535\u8fd8\u539f\u6210CO\u7684\u53cd\u5e94\u7684\u5409\u5e03\u65af\u81ea\u7531\u80fd<\/p>\n
\n