{"id":184682,"date":"2019-09-01T06:30:47","date_gmt":"2019-08-31T22:30:47","guid":{"rendered":"\/\/m.iemloyee.com\/?p=184682"},"modified":"2019-09-01T16:53:23","modified_gmt":"2019-09-01T08:53:23","slug":"%e3%80%90%e5%b7%b2%e6%a0%a1%e7%a8%bf%e3%80%91%e5%be%b7%e5%85%8b%e8%90%a8%e6%96%af%e5%a4%a7%e5%ad%a6%e5%a5%a5%e6%96%af%e6%b1%80%e5%88%86%e6%a0%a1%e4%bd%99%e6%a1%82%e5%8d%8e%e5%9b%a2%e9%98%9fnano-lett","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=184682","title":{"rendered":"\u5fb7\u514b\u8428\u65af\u5927\u5b66\u5965\u65af\u6c40\u5206\u6821\u4f59\u6842\u534e\u56e2\u961fNano Lett.: \u65e0\u673a\u51dd\u80f6\u884d\u751f\u91d1\u5c5e\u6846\u67b6\u52a9\u529b\u9ad8\u6027\u80fd\u7845\u8d1f\u6781"},"content":{"rendered":"<p><strong><b>\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n<p>\u5728\u4e0b\u4e00\u4ee3\u9502\u79bb\u5b50\u7535\u6c60\u8d1f\u6781\u6750\u6599\u4e2d\uff0cSi\u56e0\u5176\u7406\u8bba\u6bd4\u5bb9\u91cf\u9ad8\u548c\u542b\u91cf\u4e30\u5bcc\u7b49\u4f18\u52bf\u800c\u6781\u5177\u5e94\u7528\u524d\u666f\u3002\u4f46\u662f\uff0cSi\u8d1f\u6781\u4ecd\u5b58\u5728\u4f53\u79ef\u5f62\u53d8\u5927\u3001SEI\u819c\u4e0d\u7a33\u5b9a\u548c\u53cd\u5e94\u52a8\u529b\u5b66\u7f13\u6162\u7b49\u95ee\u9898\u3002\u5728Si\u4e2d\u5f15\u5165\u5f02\u8d28\u7ec4\u5206\u53ef\u8c03\u63a7\u5176\u7535\u5316\u5b66\u884c\u4e3a\u3002\u4e0e\u5e38\u7528\u7684\u78b3\u4ecb\u8d28\u7c7b\u4f3c\uff0c\u91d1\u5c5e\u4ecb\u8d28\u4e5f\u53ef\u4ee5\u4fc3\u8fdb\u7535\u8377\u4f20\u8f93\u5e76\u4fdd\u6301\u7535\u6781\u5b8c\u6574\u6027\u3002\u6b64\u5916\uff0c\u7845-\u91d1\u5c5e\uff08Si-M\uff09\u8d1f\u6781\u80fd\u8868\u73b0\u51fa\u6bd4Si\u548cSi-C\u8d1f\u6781\u66f4\u9ad8\u7684\u632f\u5b9e\u5bc6\u5ea6\u548c\u4f53\u79ef\u80fd\u91cf\u5bc6\u5ea6\uff1b\u50a8\u9502\u6d3b\u6027\u91d1\uff08M&#8217;=Ge\uff0cSn\uff0cSb\u7b49\uff09\u4e0e\u7845\u7684\u5171\u8131\u5d4c\u8fc7\u7a0b\u53ef\u63d0\u5347\u53cd\u5e94\u52a8\u529b\u5b66\uff1b\u800c\u50a8\u9502\u60f0\u6027\u91d1\u5c5e\uff08M&#8221;=Ti\uff0cNi\uff0cFe\u7b49\uff09\u80fd\u6291\u5236\u7ed3\u6676Li<sub>15<\/sub>Si<sub>4<\/sub>\u7684\u751f\u6210\u8fdb\u800c\u907f\u514d\u4e0d\u5747\u5300\u4f53\u79ef\u53d8\u5316\u3002\u56e0\u6b64\uff0c\u7845\u57fa\u5168\u91d1\u5c5e\u6750\u6599\u7279\u522b\u662fSi-M&#8217;-M&#8221;\u6750\u6599\u6709\u671b\u6210\u4e3a\u7efc\u5408\u6027\u80fd\u4f18\u5f02\u7684\u5b9e\u7528\u7845\u57fa\u8d1f\u6781\u6750\u6599\u3002\u7136\u800c\uff0c\u5f53\u524d\u91d1\u5c5e\u4ecb\u8d28\u591a\u4ee5\u76f8\u4e92\u6e38\u79bb\u7684\u7eb3\u7c73\u9897\u7c92\u5f62\u5f0f\u5b58\u5728\uff0c\u96be\u4ee5\u63d0\u4f9b\u8db3\u591f\u7684\u81ea\u7531\u7f13\u51b2\u7a7a\u95f4\u4ee5\u53ca\u6301\u7eed\u7684\u7535\u5b50\/\u79bb\u5b50\u4f20\u8f93\u901a\u9053\uff0c\u672a\u80fd\u6709\u6548\u53d1\u6325\u91d1\u5c5e\u4ecb\u8d28\u7684\u7279\u6027\u6765\u63d0\u5347Si\u8d1f\u6781\u50a8\u9502\u6027\u80fd\u3002<strong><b>\u00a0<\/b><\/strong><\/p>\n<p><strong><b>\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n<p>\u8fd1\u65e5\uff0c<strong><b>\u7f8e\u56fd<\/b><\/strong><strong><b>\u5fb7\u514b\u8428\u65af\u5927\u5b66<\/b><\/strong><strong><b>\u5965\u65af\u6c40\u5206\u6821\u4f59\u6842\u534e\u6559\u6388<\/b><\/strong>\u8054\u5408<strong><b>\u5357\u4eac\u5e08\u8303\u5927\u5b66\u5434\u5e73\u526f\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/b><\/strong>\u63d0\u51fa\u4e86\u4e00\u79cd\u7b80\u4fbf\u53ef\u91cf\u4ea7\u7684\u51dd\u80f6\u8fd8\u539f\u6cd5\u5c06Si\u9897\u7c92\u5747\u5300\u5730\u56fa\u5b9a\u4e8e3D\u91d1\u5c5e\u6846\u67b6\u5185\u8fdb\u800c\u663e\u8457\u63d0\u5347\u50a8\u9502\u6027\u80fd\u3002\u5177\u4f53\u6765\u8bf4\uff0c\u5c06\u5546\u4e1a\u5316Si\u9897\u7c92\u5305\u8986\u4e8e\u6c30\u57fa\u6865\u8054(Sn\u2013N\u2261C\u2013Ni)\u914d\u4f4d\u805a\u5408\u7269\u51dd\u80f6(Sn-Ni\u6c30\u80f6)\u4e2d\uff0c\u8fdb\u4e00\u6b65\u8fd8\u539f\u8be5\u590d\u5408\u6c30\u80f6\u53ef\u5c06Si\u9897\u7c92\u5747\u5300\u56fa\u5b9a\u4e8e3D\u9521\u954d\u5408\u91d1\u6846\u67b6\uff0c\u5f62\u6210Si@Sn-Ni\u5168\u91d1\u5c5e\u6846\u67b6\u6750\u6599\u3002\u5faa\u73af\u4e2d\uff0cSi\u9897\u7c92\u7684\u81ea\u91cd\u6392\u8fdb\u4e00\u6b65\u589e\u5927\u4e86Si\u5728\u5408\u91d1\u6846\u67b6\u4e2d\u7684\u5206\u6563\u5ea6\u4ee5\u53caSi\u4e0eSn-Ni\u5408\u91d1\u7684\u534f\u540c\u6548\u5e94\u3002\u8fd9\u79cd\u9ad8\u7684\u7ed3\u6784\u5b8c\u6574\u6027\u30013D\u79bb\u5b50\/\u7535\u5b50\u6df7\u5408\u4f20\u8f93\u901a\u9053\u4ee5\u53caSi\/Sn-Ni\u534f\u540c\u6548\u5e94\u4f7f\u5f97Si@Sn-Ni\u5168\u91d1\u5c5e\u6846\u67b6\u6750\u6599\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u957f\u5faa\u73af\u5bff\u547d\u548c\u500d\u7387\u6027\u80fd\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201c<strong><b>Inorganic Gel-Derived Metallic Frameworks Enabling High-Performance Silicon Anodes<\/b><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728<strong><b>Nano Letters<\/b><\/strong>\u4e0a\u3002<\/p>\n<p><strong><b>\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n<p><strong><b>\u56fe\u4e00<\/b><\/strong><strong><b>Si@Sn-Ni\u5168\u91d1\u5c5e<\/b><\/strong><strong><b>\u6846\u67b6\u6750\u6599<\/b><\/strong><strong><b>\u7684<\/b><\/strong><strong><b>\u5408\u6210<\/b><\/strong><strong><b>\u793a\u610f\u56fe\u4ee5\u53ca\u5de5\u4f5c\u539f\u7406\u56fe<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-184683\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/1-46.jpg\" alt=\"\" width=\"600\" height=\"336\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/1-46.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/1-46-300x168.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\uff08a\uff09Si@Sn-Ni\u5168\u91d1\u5c5e\u6846\u67b6\u6750\u6599\u7684\u5408\u6210\u793a\u610f\u56fe\u3002<\/p>\n<p>\uff08b\uff09Si@Sn-Ni\u5168\u91d1\u5c5e\u6846\u67b6\u6750\u6599\u7684\u5faa\u73af\u81ea\u91cd\u6392\u548c\u8131\u5d4c\u9502\u8fc7\u7a0b\u793a\u610f\u56fe\u3002<strong><b>\u00a0<\/b><\/strong><\/p>\n<p><strong><b>\u56fe\u4e8c<\/b><\/strong><strong><b>Si@Sn-Ni\u5168\u91d1\u5c5e<\/b><\/strong><strong><b>\u6846\u67b6\u6750\u6599<\/b><\/strong><strong><b>\u7684<\/b><\/strong><strong><b>\u5f62\u8c8c\u3001\u7ec4\u6210\u548c\u7ed3\u6784<\/b><\/strong><strong><b>\u8868\u5f81<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-184684\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/2-43.jpg\" alt=\"\" width=\"600\" height=\"330\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/2-43.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/2-43-300x165.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\uff08a\uff09\u590d\u5408\u6c30\u80f6\u7684\u5149\u5b66\u7167\u7247\u3002<\/p>\n<p>\uff08b\uff09TEM\u56fe\u50cf\u548cSAED\u56fe\u6848\u3002<\/p>\n<p>\uff08c\uff09XRD\u8c31\u56fe\u3002<\/p>\n<p>\uff08d\uff09\u9ad8\u500dTEM\u56fe\u50cf\u548cSEM\u56fe\u50cf\u3002<\/p>\n<p>\uff08e\uff09TEM-EDS\u5143\u7d20\u5206\u5e03\u56fe\u50cf\u3002<\/p>\n<p>\uff08f\uff09XPS\u8c31\u56fe\u3002<\/p>\n<p><strong><b>\u56fe\u4e09\u7535\u5316\u5b66\u6027\u80fd\u8868\u5f81<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-184685\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/3-42.jpg\" alt=\"\" width=\"600\" height=\"294\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/3-42.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/3-42-300x147.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\uff08a\uff09CV\u66f2\u7ebf\u3002<\/p>\n<p>\uff08b\uff09\u5faa\u73af\u7a33\u5b9a\u6027\u3002<\/p>\n<p>\uff08c\uff0cd\uff09\u500d\u7387\u6027\u80fd\u4ee5\u53ca\u4e0e\u76f8\u5173\u6587\u732e\u7684\u6bd4\u8f83<\/p>\n<p>\uff08e\uff0cf\uff09EIS\u963b\u6297\u8c31\u4ee5\u53caZ&#8217;\u548c\u03c9<sup>-1\/2<\/sup>\u7684\u5173\u7cfb\u56fe\u3002<\/p>\n<p><strong><b>\u56fe\u56db<\/b><\/strong><strong><b>Si@Sn-Ni\u5168\u91d1\u5c5e<\/b><\/strong><strong><b>\u6846\u67b6\u6750\u6599\u5faa\u73af\u540e\u7684\u5f62\u8c8c\u3001\u7ec4\u6210\u548c\u7ed3\u6784\u8868\u5f81<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-184686\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/4-39.jpg\" alt=\"\" width=\"600\" height=\"596\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/4-39.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/4-39-150x150.jpg 150w, \/\/m.iemloyee.com\/wp-content\/uploads\/2019\/08\/4-39-300x298.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\uff08a\uff09Si\u9897\u7c92\u5728Sn-Ni\u6846\u67b6\u4e2d\u7684\u5faa\u73af\u81ea\u91cd\u6392\u793a\u610f\u56fe\u3002<\/p>\n<p>\uff08b\uff0cc\uff09TEM\u56fe\u50cf\u548c\u5143\u7d20\u5206\u5e03\u56fe\u50cf\u3002<\/p>\n<p>\uff08d\uff09HRTEM\u56fe\u50cf\u3002<\/p>\n<p>\uff08e\uff09\u62c9\u66fc\u5149\u8c31\u3002<\/p>\n<p><strong><b>\u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n<p>\u603b\u4e4b\uff0c\u672c\u6587\u5f00\u53d1\u4e86\u4e00\u79cd\u7b80\u4fbf\u6613\u91cf\u4ea7\u7684\u51dd\u80f6\u8fd8\u539f\u6cd5\u5c06Si\u9897\u7c92\u5747\u5300\u5730\u56fa\u5b9a\u4e8e3D\u00a0Sn-Ni\u5408\u91d1\u6846\u67b6\u5185\u3002\u8be5Si@Sn-Ni\u5168\u91d1\u5c5e\u6846\u67b6\u6750\u6599\u5177\u6709\u9ad8\u7684\u7ed3\u6784\u5b8c\u6574\u6027\u30013D\u79bb\u5b50\/\u7535\u5b50\u6df7\u5408\u4f20\u8f93\u901a\u9053\u548cSi\/Sn-Ni\u534f\u540c\u6548\u5e94\uff0c\u800c\u4e14\uff0cSi\u9897\u7c92\u7684\u5faa\u73af\u81ea\u91cd\u6392\u8fdb\u4e00\u6b65\u63d0\u9ad8\u4e86\u5176\u5728\u6846\u67b6\u4e2d\u7684\u5206\u6563\u5ea6\u53ca\u534f\u540c\u6548\u5e94\u3002\u56e0\u6b64\uff0c\u8be5Si@Sn-Ni\u6846\u67b6\u6750\u6599\u8868\u73b0\u51fa\u4e86\u4f18\u5f02\u7684\u7ed3\u6784\u7a33\u5b9a\u6027\u548c\u7535\u8377\u4f20\u8f93\u80fd\u529b\u4ee5\u53ca\u957f\u5faa\u73af\u5bff\u547d(\u57280.5\u00a0A g<sup>-1<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7ecf\u8fc7100\u6b21\u5faa\u73af\uff0c\u53ef\u9006\u6bd4\u5bb9\u91cf\u4e3a1205\u00a0mA h g<sup>-1<\/sup>)\u548c\u500d\u7387\u6027\u80fd(\u572810 A g<sup>-1<\/sup>\u7684\u5927\u7535\u6d41\u5bc6\u5ea6\u4e0b\uff0c\u5e73\u5747\u6bd4\u5bb9\u91cf\u9ad8\u8fbe653\u00a0mA h g<sup>-1<\/sup>)\u3002\u8be5\u6c30\u80f6\u8fd8\u539f\u8def\u7ebf\u53ef\u5ef6\u4f38\u81f3\u5236\u5907\u5176\u5b83\u7ed3\u6784\u548c\u7ec4\u5206\u53ef\u63a7\u7684\u91d1\u5c5e\u57fa\u590d\u5408\u6846\u67b6\u6750\u6599\u7528\u4e8e\u7535\u5316\u5b66\u80fd\u6e90\u9886\u57df\u3002<\/p>\n<p><strong><b>\u6587\u732e\u94fe\u63a5\u201c<\/b><\/strong><a href=\"https:\/\/pubs.acs.org\/doi\/10.1021\/acs.nanolett.9b02429\"><strong><u><b>Inorganic Gel-Derived Metallic Frameworks Enabling High-Performance Silicon Anodes<\/b><\/u><\/strong><\/a>\u201d\u00a0<strong><b>(Nano Lett.<\/b><\/strong><strong><b>\u00a0<\/b><\/strong><strong><b>2019.<\/b><\/strong>\u00a0<strong><b>DOI: 10.1021\/acs.nanolett.9b02429)<\/b><\/strong><\/p>\n<p><strong><b>\u3010<\/b><\/strong><strong><b>\u76f8\u5173\u6587\u732e\u63a8\u8350<\/b><\/strong><strong><b>\u3011<\/b><\/strong><\/p>\n<ul>\n<li>Fang, A. Zhang, P.Wu*,\u00a0G. Yu*,\u00a0&#8220;Inorganic Cyanogels and Their Derivatives for Electrochemical Energy Storage and Conversion&#8221;, ACS Materials Lett., 1, 158 (2019).<\/li>\n<\/ul>\n<p>https:\/\/pubs.acs.org\/doi\/abs\/10.1021\/acsmaterialslett.9b00125<\/p>\n<ul>\n<li>Shi, Z. Fang, X. Zhang, F. Li, Y. Tang, Y. Zhou, P. Wu*, G. Yu*, &#8220;Double-Network Nanostructured Hydrogel-Derived Ultrafine Sn\u2013Fe Alloy in 3D Carbon Framework for Enhanced Lithium Storage&#8221;, Nano Lett.,18, 3193 (2018).<\/li>\n<\/ul>\n<p>https:\/\/pubs.acs.org\/doi\/abs\/10.1021\/acs.nanolett.8b00898<\/p>\n<ul>\n<li>Wu, A. Zhang, L. Peng, F. Zhao, Y. Tang, Y. Zhou, G. Yu*, &#8220;Cyanogel-Enabled Homogeneous Sb\u2013Ni\u2013C Ternary Framework Electrodes for Enhanced Sodium Storage&#8221;, ACS Nano, 12, 759 (2018).<\/li>\n<\/ul>\n<p>https:\/\/pubs.acs.org\/doi\/abs\/10.1021\/acsnano.7b07985<\/p>\n<ul>\n<li>P.Wu, Z.\u00a0Fang, A.\u00a0Zhang, X.\u00a0Zhang, Y. Tang, Y. Zhou, G Yu*,\u00a0&#8220;Chemically Binding Scaffolded Anodes with 3D Graphene Architectures Realizing Fast and Stable Lithium Storage&#8221;, Research, DOI: 10.34133\/2019\/8393085\u00a0(2019).<\/li>\n<\/ul>\n<p>https:\/\/spj.sciencemag.org\/research\/2019\/8393085\/<\/p>\n<ul>\n<li>Zhang, X. Xu, C. Zhang, Z. Yu, Y. Zhou, Y. Tang, P.Wu*, S. 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