{"id":183180,"date":"2019-08-13T06:30:01","date_gmt":"2019-08-12T22:30:01","guid":{"rendered":"\/\/m.iemloyee.com\/?p=183180"},"modified":"2019-08-12T16:11:43","modified_gmt":"2019-08-12T08:11:43","slug":"%e5%8c%97%e4%ba%ac%e5%a4%a7%e5%ad%a6%e4%b8%ad%e7%a7%91%e9%99%a2%e7%89%a9%e7%90%86%e7%a0%94%e7%a9%b6%e6%89%80adv-mater-%e5%8e%9f%e5%ad%90%e7%ba%a7%e5%8e%9a%e5%ba%a6%e7%9a%84%e7%a1%92%e6%b0%a7","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=183180","title":{"rendered":"\u5317\u4eac\u5927\u5b66&\u4e2d\u79d1\u9662\u7269\u7406\u7814\u7a76\u6240Adv. Mater.: \u539f\u5b50\u7ea7\u539a\u5ea6\u7684\u7852\u6c27\u5316\u7269\u8584\u819c\u7684\u5206\u5b50\u675f\u5916\u5ef6\u548c\u7535\u5b50\u7ed3\u6784"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

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\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5317\u4eac\u5927\u5b66\u5f6d\u6d77\u7433\u6559\u6388<\/strong>\u4e0e\u4e2d\u79d1\u9662\u7269\u7406\u7814\u7a76\u6240\u90ed\u5efa\u4e1c\u7814\u7a76\u5458<\/strong>\u5408\u4f5c\uff0c\u901a\u8fc7\u5728\u6c27\u6c14\u6c1b\u56f4\u4e2d\u5171\u540c\u84b8\u53d1Bi\u548cSe\u524d\u9a71\u4f53\u7387\u5148\u5b9e\u73b0\u4e86\u5728SrTiO3<\/sub>\u57fa\u5e95\u4e0a\u5355\u5c42\u539f\u5b50\u7ea7\u8584Bi2<\/sub>O2<\/sub>Se\u819c\u7684\u5206\u5b50\u675f\u5916\u5ef6\uff08MBE\uff09\uff0c\u5e76\u8fdb\u4e00\u6b65\u63ed\u793a\u4e86MBE\u751f\u957f\u7684Bi2<\/sub>O2<\/sub>Se\/SrTiO3<\/sub>\u7684\u754c\u9762\u539f\u5b50\u6392\u5217\uff0c\u7814\u7a76\u8868\u660e\u5176\u5177\u6709\u539f\u5b50\u7ea7\u5206\u8fa8\u7684\u6e05\u6670\u754c\u9762\u53ca\u539f\u5b50\u6392\u5217\u3002\u66f4\u91cd\u8981\u7684\u662f\uff0c\u901a\u8fc7\u89d2\u5206\u8fa8\u5149\u7535\u5b50\u80fd\u8c31\u89e3\u6790\u4e86\u5355\u4e2a\u6676\u80de\uff081-UC\uff09\u539aBi2<\/sub>O2<\/sub>Se\u8584\u819c\u7684\u7535\u5b50\u80fd\u5e26\u7ed3\u6784\uff08\u5177\u6709\u7ea60.15 m0<\/sub>\u7684\u4f4e\u7535\u5b50\u6709\u6548\u8d28\u91cf\u548c\u7ea60.8 eV\u7684\u5e26\u9699\uff09\uff0c\u8fd9\u8868\u660e\u5355\u4e2a\u6676\u80de\u539a\u7684Bi2<\/sub>O2<\/sub>Se\u8584\u819c\u4f9d\u7136\u662f\u8d85\u9ad8\u8fc1\u79fb\u7387\u7684\u534a\u5bfc\u4f53\u6750\u6599\u3002\u8fd9\u4e9b\u7814\u7a76\u7ed3\u679c\u5bf9\u4e8e2D\u6c27\u786b\u65cf\u5316\u5408\u7269\u7684\u5408\u6210\u53ca\u5176\u7269\u7406\u6027\u8d28\u7684\u7814\u7a76\u5177\u6709\u5efa\u8bbe\u6027\u7684\u6307\u5bfc\u610f\u4e49\u3002\u8be5\u6210\u679c\u4ee5\u9898\u4e3a” Molecular Beam Epitaxy and Electronic Structure of Atomically Thin Oxyselenide Films<\/strong>“\u53d1\u8868\u5728\u56fd\u9645\u8457\u540d\u6750\u6599\u671f\u520aAdv. Mater.<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

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\"\"<\/p>\n

(a) \u5728\uff08001\uff09\u53d6\u5411\u7684SrTiO3<\/sub>\uff08STO\uff09\u886c\u5e95\u4e0a\u5916\u5ef6\u751f\u957f\u539f\u5b50\u7ea7\u539aBi2<\/sub>O2<\/sub>Se\u8584\u819c\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

(b) Bi2<\/sub>O2<\/sub>Se\u7684\u6676\u4f53\u7ed3\u6784\uff1b<\/p>\n

(c) SrTiO3<\/sub>\u7684\u6676\u4f53\u7ed3\u6784\u3002<\/p>\n

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\"\"<\/p>\n

(a) \u4ee5TiO2<\/sub>\u4e3a\u7ec8\u6b62\u9762\u7684STO\u57fa\u5e95\u7684\u8868\u9762\u5f62\u8c8c\uff1b<\/p>\n

(b-e) MBE\u751f\u957f\u7684\u3001\u4e0d\u540c\u539a\u5ea6\u7684Bi2<\/sub>O2<\/sub>Se\u8584\u819c\u7684AFM\u5f62\u8c8c\uff1b<\/p>\n

(c) MBE\u751f\u957f\u7684Bi2<\/sub>O2<\/sub>Se\u8584\u819c\u539a\u5ea6\u4e0e\u751f\u957f\u65f6\u95f4\u7684\u5173\u7cfb\u3002<\/p>\n

\u56fe3 MBE\u751f\u957fBi2<\/sub>O2<\/sub>Se\u7684\u6a2a\u622a\u9762TEM\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

(a) Bi2<\/sub>O2<\/sub>Se\u8584\u819c\u4e0eSTO\u95f4\u754c\u9762\u7684\u6a2a\u622a\u9762HAADF-STEM\u56fe\u50cf\uff1b<\/p>\n

(b) a\u56fe\u4e2d\u767d\u6846\u533a\u57df\u754c\u9762\u7684\u539f\u5b50\u7ea7\u5206\u8fa8\u7387HAADF-STEM\u56fe\u50cf\uff1b<\/p>\n

(c) b\u56fe\u4e2dHAADF\u56fe\u50cf\u5728\u5177\u6709\u5355\u8f74\u5e94\u53d8\u5206\u91cf\u03b5xx<\/sub>\u6761\u4ef6\u4e0b\u7684\u51e0\u4f55\u76f8\u4f4d\u5206\u6790\uff1b<\/p>\n

(d) b\u56fe\u4e2dHAADF\u56fe\u50cf\u5728\u5177\u6709\u5355\u8f74\u5e94\u53d8\u5206\u91cf\u03b5zz<\/sub>\u6761\u4ef6\u4e0b\u7684\u51e0\u4f55\u76f8\u4f4d\u5206\u6790\uff1b<\/p>\n

(e) \u7531EDS\u5f97\u5230\u7684\u754c\u9762\u4e0aBi\u3001Se\u3001O\u3001Sr\u548cTi\u7684\u539f\u5b50\u7ea7\u5206\u8fa8\u7387\u5143\u7d20\u56fe\uff1b<\/p>\n

(f) \u663e\u793a\u539f\u5b50\u6a21\u578b\u7684\u754c\u9762\u7684HAADF-STEM\u56fe\u50cf\u3002<\/p>\n

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\"\"<\/p>\n

(a) \u901a\u8fc7ARPES\u68c0\u6d4b\u76841-UC\u539aBi2<\/sub>O2<\/sub>Se\u819c\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

(b) \u5728\u5bbd\u80fd\u91cf\u8303\u56f4\u5185\u6052\u5b9a\u80fd\u91cf\u8f6e\u5ed3\u7684\u5806\u53e0\u56fe\uff1b<\/p>\n

(c) \u5728i) VBM\u548cii) VBM-0.4 eV\u9891\u5e26\u5904\u7684\u6052\u5b9a\u80fd\u91cf\u8f6e\u5ed3\u7684\u5149\u7535\u53d1\u5c04\u5f3a\u5ea6\u56fe\uff1b<\/p>\n

(d) 1-UC\u539aBi2<\/sub>O2<\/sub>Se\u819c\u7684\u8272\u6563\uff1b<\/p>\n

(e) \u5728\u8868\u9762\u94be\u63ba\u6742\u524d\uff08i\uff09\u548c\u76f8\u5e94\u7684EDC\uff08ii\uff09\u7684\u80fd\u5e26\u8272\u6563\uff1b<\/p>\n

(f) \u5728\u8868\u9762\u94be\u63ba\u6742\u540e\uff08i\uff09\u548c\u76f8\u5e94\u7684EDC\uff08ii\uff09\u7684\u80fd\u5e26\u8272\u6563\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aMolecular Beam Epitaxy and Electronic Structure of Atomically Thin Oxyselenide Films<\/a>\u00a0(Adv. Mater., 2019, DOI: 10.1002\/adma.201901964)<\/strong><\/p>\n

\u00a0\u3010\u56e2\u961f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

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\u3010\u56e2\u961f\u5728\u8be5\u9886\u57df\u5de5\u4f5c\u6c47\u603b\u3011<\/strong><\/p>\n

\u5f6d\u6d77\u7433\u6559\u6388\u8bfe\u9898\u7ec4\u548c\u5408\u4f5c\u8005\u4e8e2017\u5e74\u7387\u5148\u53d1\u73b0\u5e76\u5236\u5907\u4e86\u4e00\u7c7b\u5168\u65b0\u7684\u8d85\u9ad8\u8fc1\u79fb\u7387\u534a\u5bfc\u4f53\u578b\u5c42\u72b6\u7852\u6c27\u5316\u7269\u6750\u6599Bi2<\/sub>O2<\/sub>Se\uff0c\u5b9e\u9a8c\u548c\u7406\u8bba\u4e0a\u8bc1\u660e\u4e86\u5178\u578b\u7684\u4e8c\u7ef4\u7852\u6c27\u5316\u94cbBi2<\/sub>O2<\/sub>Se\u7684\u5e26\u9699\u4e3a~0.8 eV\uff0c\u5e76\u5177\u6709\u5f88\u5c0f\u7684\u7535\u5b50\u6709\u6548\u8d28\u91cf\uff08~0.14 m0<\/sub>\uff09\u548c\u8d85\u9ad8\u7684\u8f7d\u6d41\u5b50\u8fc1\u79fb\u7387\uff08\u4f4e\u6e29\u970d\u5c14\u8fc1\u79fb\u7387\u9ad8\u8fbe280,000 cm2<\/sup>\/V\u00b7s\uff09\u3002\u6807\u51c6\u7684\u4e8c\u7ef4Bi2<\/sub>O2<\/sub>Se\u9876\u6805\u573a\u6548\u5e94\u6676\u4f53\u7ba1\u5c55\u73b0\u4e86\u5f88\u9ad8\u7684\u5ba4\u6e29\u8868\u89c2\u573a\u6548\u5e94\u8fc1\u79fb\u7387\uff08\uff5e2000 cm2<\/sup>\/V\u00b7s\uff09\u548c\u970d\u5c14\u8fc1\u79fb\u7387\uff08\uff5e450 cm2<\/sup>\/V\u00b7s\uff09\u3001\u5f88\u5927\u7684\u7535\u6d41\u5f00\u5173\u6bd4\uff08>106<\/sup>\uff09\u4ee5\u53ca\u7406\u60f3\u7684\u5668\u4ef6\u4e9a\u9608\u503c\u6446\u5e45\uff08\uff5e65 mV\/dec\uff09\uff08Nature Nanotech. <\/em>2017, 12<\/em>, 530\uff09\u3002\u5e76\u57fa\u4e8e\u4e8c\u7ef4\u7852\u6c27\u5316\u94cb\u534a\u5bfc\u4f53\u6750\u6599\u7814\u5236\u4e86\u53ef\u5728\u5ba4\u6e29\u5de5\u4f5c\u7684\u8d85\u5feb\u9ad8\u654f\u8fd1\u7ea2\u5916\u5149\u7535\u63a2\u6d4b\u5668\uff08Nature Commun. <\/em>2018, 9, <\/em>3311\uff09\uff0c\u5e76\u7ed3\u5408\u626b\u63cf\u96a7\u9053\u663e\u5fae\u955c\u53ca\u89d2\u5206\u8fa8\u5149\u7535\u5b50\u80fd\u8c31\u5bf9\u5176\u89e3\u7406\u540e\u7684\u8868\u754c\u9762\u7535\u5b50\u7ed3\u6784\u53ca\u539f\u5b50\u6392\u5e03\u8fdb\u884c\u4e86\u5168\u9762\u89e3\u6790\uff08Science Advances<\/em> 2018 4, eaat8355.<\/em><\/a>\uff09\uff1b\u8fd1\u671f\u5b9e\u73b0\u4e86\u6676\u5706\u7ea7Bi2<\/sub>O2<\/sub>Se\u7684\u5355\u6676\u8584\u819c\u7684CVD\u751f\u957f\uff08Nano Lett.<\/em> 2019, 19, 2148\uff09\u3002<\/p>\n

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