{"id":178512,"date":"2019-06-22T06:30:27","date_gmt":"2019-06-21T22:30:27","guid":{"rendered":"\/\/m.iemloyee.com\/?p=178512"},"modified":"2019-06-22T12:18:11","modified_gmt":"2019-06-22T04:18:11","slug":"%e8%a5%bf%e5%8c%97%e5%b7%a5%e4%b8%9a%e5%a4%a7%e5%ad%a6%e7%8e%8b%e6%b4%aa%e5%bc%banature-communications%e5%9c%a8%e9%92%92%e9%85%b8%e9%93%8b%e5%85%89%e9%98%b3%e6%9e%81%e4%b8%ad%e6%bf%80%e5%85%89","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=178512","title":{"rendered":"\u897f\u5317\u5de5\u4e1a\u5927\u5b66\u738b\u6d2a\u5f3aNature Communications:\u5728\u9492\u9178\u94cb\u5149\u9633\u6781\u4e2d\u6fc0\u5149\u690d\u5165\u7eb3\u7c73\u6676\u5b9e\u73b0\u9ad8\u6548\u5149\u7535\u5316\u5b66\u6c34\u5206\u89e3"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u5149\u7535\u50ac\u5316\u5206\u89e3\u6c34\u88ab\u8ba4\u4e3a\u662f\u4e00\u79cd\u6781\u5177\u6f5c\u80fd\u7684\u4ea7\u6c22\u6280\u672f\u3002\u5176\u4e2d\u9492\u9178\u94cb(BiVO4<\/sub>)\u4f5c\u4e3a\u4e00\u79cd\u5177\u6709\u4ee3\u8868\u6027\u7684\u91d1\u5c5e\u6c27\u5316\u7269\u5149\u9633\u6781\u6750\u6599\u53d7\u5230\u4e86\u7814\u7a76\u8005\u7684\u5e7f\u6cdb\u7814\u7a76\u3002\u7136\u800c\uff0c\u9492\u9178\u94cb\u7684\u8f7d\u6d41\u5b50\u8fc1\u79fb\u7387\u4f4e\uff0c\u8fd9\u4f7f\u5f97\u5149\u751f\u8f7d\u6d41\u5b50\u5728\u9492\u9178\u94cb\u4f53\u5185\u590d\u5408\u4e25\u91cd\uff0c\u5bfc\u81f4\u4e86\u9492\u9178\u94cb\u6750\u6599\u7684\u5149\u7535\u6d41\u5bc6\u5ea6\u8fdc\u8fdc\u4f4e\u4e8e\u7406\u8bba\u503c(7.5 mA cm-2<\/sup>)\u3002\u56e0\u6b64\uff0c\u5982\u4f55\u901a\u8fc7\u63d0\u5347\u8f7d\u6d41\u5b50\u8f93\u8fd0\u6027\u80fd\u6765\u8bbe\u8ba1\u9ad8\u6548\u7387\u7684\u9492\u9178\u94cb\u5149\u9633\u6781\u4e00\u76f4\u662f\u4e00\u4e2a\u5de8\u5927\u7684\u6311\u6218\u3002\u7814\u7a76\u8005\u901a\u8fc7\u4e00\u7cfb\u5217\u7b56\u7565\u6765\u63d0\u5347\u9492\u9178\u94cb\u5149\u9633\u6781\u7684\u7535\u8377\u8f93\u8fd0\u6027\u8d28\uff0c\u6bd4\u5982\u63ba\u6742\u3001\u6784\u5efa\u5f02\u8d28\u7ed3\u6784\u3001\u7b49\u79bb\u5b50\u4f53\u548c\u7eb3\u7c73\u7ed3\u6784\u7b49\u3002\u5c3d\u7ba1\u8fd9\u4e9b\u7b56\u7565\u53ef\u4ee5\u6709\u6548\u5730\u63d0\u5347\u9492\u9178\u94cb\u5149\u9633\u6781\u7684\u6027\u80fd\uff0c\u4f46\u5176\u56fa\u6709\u8f7d\u6d41\u5b50\u8f93\u8fd0\u6027\u80fd\u5dee\u7684\u95ee\u9898\u4ecd\u7136\u963b\u788d\u7740\u9492\u9178\u94cb\u6027\u80fd\u7684\u8fdb\u4e00\u6b65\u63d0\u9ad8\u3002\u56e0\u6b64\uff0c\u63d0\u5347\u9492\u9178\u94cb\u7684\u56fa\u6709\u8f7d\u6d41\u5b50\u8f93\u8fd0\u6027\u80fd\u662f\u63d0\u5347\u9492\u9178\u94cb\u5149\u9633\u6781\u6027\u80fd\u7684\u5173\u952e\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u00a0 \u8fd1\u65e5\uff0c\u897f\u5317\u5de5\u4e1a\u5927\u5b66\u7684\u738b\u6d2a\u5f3a\u6559\u6388\u8bfe\u9898\u7ec4\u5728Nature Communications\u4e0a\u53d1\u8868\u4e86\u4e00\u7bc7\u9898\u4e3a\u201cEmbedding laser generated nanocrystals in BiVO4<\/sub> photoanode for efficient photoelectrochemical water splitting\u201d\u7684\u6587\u7ae0\u3002\u8be5\u6587\u7ae0\u62a5\u9053\u4e86\u4e00\u79cd\u901a\u8fc7\u6db2\u76f8\u8109\u51b2\u6fc0\u5149\u8f90\u7167\u65b9\u6cd5\u5728\u9492\u9178\u94cb\u5149\u9633\u6781\u4f53\u5185\u5f15\u5165\u7eb3\u7c73\u6676\uff0c\u4e3a\u89e3\u51b3\u9492\u9178\u94cb\u8f7d\u6d41\u5b50\u8f93\u8fd0\u6027\u8d28\u5dee\u7684\u95ee\u9898\u63d0\u4f9b\u4e86\u4e00\u79cd\u89e3\u51b3\u65b9\u6848\uff0c\u9492\u9178\u94cb\u53cc\u9633\u6781\u7684\u5149\u7535\u6d41\u5bc6\u5ea6\u53ef\u63d0\u5347\u81f36.22 mA cm-2<\/sup>@ 1.23 V RHE\uff0c\u535a\u58eb\u751f\u7b80\u6d01\u548c\u7855\u58eb\u751f\u5f90\u6709\u52cb\u4e3a\u8be5\u5de5\u4f5c\u7684\u5171\u540c\u7b2c\u4e00\u4f5c\u8005\u3002<\/p>\n

\u3010\u56fe\u6587\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u56fe<\/strong>1 La:BaSnO3<\/sub>(LBSO)<\/strong>\u80f6\u4f53\u7684\u6fc0\u5149\u5408\u6210\u4e0e\u52a0\u5de5<\/strong>(LSPC)<\/strong><\/p>\n

\"\"<\/p>\n

a) \u80f6\u4f53\u6fc0\u5149\u5408\u6210\u52a0\u5de5(LSPC)\u793a\u610f\u56fe\uff1b<\/p>\n

b) LSPC\u5904\u7406\u4e4b\u524d\u7684LBSO\u9897\u7c92\u5206\u6563\u6db2\u7684\u5149\u5b66\u56fe\u7247\uff1b<\/p>\n

c, d) LBSO\u9897\u7c92\u7684SEM\u56fe\u7247\u548cXRD\u8c31\uff1b<\/p>\n

e) LSPC\u5904\u7406\u4e4b\u540e\u7684LBSO\u80f6\u4f53\u7eb3\u7c73\u6676\u5149\u5b66\u56fe\u7247\uff1b<\/p>\n

f, g) LBSO\u80f6\u4f53\u7eb3\u7c73\u6676\u7684TEM\u56fe\u548cXRD\u3002<\/p>\n

\u56fe<\/strong>2 Mo:BiVO4(MBVO)<\/strong>\u548c<\/strong>LBSO-MBVO<\/strong>\u8584\u819c\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

a-d) MBVO\u8584\u819c\u7684\u4fef\u89c6\u56fe\u548c\u4fa7\u89c6\u56feSEM\u56fe\uff0cTEM\u548cHRTEM\u56fe\uff1b<\/p>\n

e-i) LBSO-MBVO\u8584\u819c\u7684\u4fef\u89c6\u56fe\u548c\u4fa7\u89c6\u56feSEM\u56fe\uff0cTEM\u3001\u884d\u5c04\u56fe\u548cHRTEM\u56fe\uff1b<\/p>\n

j) MBVO\u4e3b\u4f53\u7684\u884d\u5c04\u56fe\uff1b<\/p>\n

k) LBSO\u7eb3\u7c73\u6676\u7684\u884d\u5c04\u56fe\uff1b<\/p>\n

l) LBSO-MBVO\u8584\u819c\u7684HAADF\u56fe\uff1bm) LBSO-MBVO\u8584\u819c\u7684\u5143\u7d20TEM-mapping\u3002<\/p>\n

\u56fe<\/strong>3 M<\/strong>BVO<\/strong>\u548c<\/strong>LBSO-MBVO<\/strong>\u5149\u9633\u6781\u8584\u819c\u7684\u50ac\u5316\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

a) \u8109\u51b2\u6fc0\u5149\u4ea7\u751f\u7684\u7eb3\u7c73\u6676\u4f53\u5d4c\u5165MBVO\u8584\u819c\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

b) \u4e0d\u540c\u7684LBSO-MBVO\u5149\u9633\u6781\u7684J-V\u66f2\u7ebf\uff1b<\/p>\n

c) MBVO\u548cLBSO-MBVO\u7684\u5149\u7535\u6d41\u5bc6\u5ea6\u7edf\u8ba1\uff08\u7535\u538b\u4e3a23V\u5904\uff09\uff1b<\/p>\n

d) LBSO-MVO-2\u53cc\u5149\u9633\u6781\u7684J-V\u66f2\u7ebf\uff1b<\/p>\n

e-f) \u4e0d\u540c\u7684LBSO-MBVO\u5149\u9633\u6781\u7684IPCE\u548cEIS\u66f2\u7ebf\uff1b<\/p>\n

g-i) MBVO\u548cLBSO-MBVO-2\u8584\u819c\u7684MS\u66f2\u7ebf\uff0c\u65f6\u95f4\u5206\u8fa8\u5fae\u6ce2\u4fe1\u53f7\uff0c\u6700\u5927TRMC\u4fe1\u53f7\u5165\u5c04\u5149\u5b50\u6570\u7684\u5173\u7cfb\u66f2\u7ebf\u3002<\/p>\n

\u56fe<\/strong>4 WO3<\/sub><\/strong>\u548c<\/strong>Au<\/strong>\u7eb3\u7c73\u6676\u5bf9<\/strong>MBVO<\/strong>\u7684\u6027\u80fd\u589e\u5f3a\u4f5c\u7528<\/strong><\/p>\n

\"\"<\/p>\n

a-b) \u6fc0\u5149\u5904\u7406\u524d\u540e\u7684WO3<\/sub>\u7eb3\u7c73\u6676\u80f6\u4f53\u6eb6\u6db2\uff1b<\/p>\n

c) WO3<\/sub>\u7eb3\u7c73\u6676\u7684TEM\u56fe\uff1b<\/p>\n

d-e) WO3<\/sub>-MBVO\u548cMBVO\u7684J-V\u66f2\u7ebf\u548cIPCE\u66f2\u7ebf\uff1b<\/p>\n

f-g) \u6fc0\u5149\u5904\u7406\u524d\u540e\u7684Au\u7eb3\u7c73\u6676\u80f6\u4f53\u6eb6\u6db2\uff1b<\/p>\n

h) Au\u7eb3\u7c73\u6676\u7684TEM\u56fe\uff1b<\/p>\n

i-j)\u00a0 Au-MBVO\u548cMBVO\u7684J-V\u66f2\u7ebf\u548cIPCE\u66f2\u7ebf\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u00a0 \u7814\u7a76\u8005\u5f00\u53d1\u4e86\u4e00\u79cd\u666e\u9002\u6027\u7684\u8109\u51b2\u6fc0\u5149\u8f90\u7167\u8f85\u52a9\u7eb3\u7c73\u6676\u5f15\u5165\u65b9\u6cd5\uff0c\u8fd9\u79cd\u7eb3\u7c73\u6676\u4e0eMBVO\u7ed3\u5408\u53ef\u4ee5\u83b7\u5f97\u8f83\u9ad8\u7684\u5149\u7535\u50ac\u5316\u6027\u80fd\uff0c\u5176\u4e2d\u53ccLBSO-MBVO\u9633\u6781\u4f53\u7cfb\u7684\u7535\u6d41\u5bc6\u5ea6\u53ef\u8fbe6.22 mA cm-2<\/sup>\u3002\u8be5\u7814\u7a76\u5c06\u4e3a\u63d0\u9ad8\u91d1\u5c5e\u6c27\u5316\u7269\u57fa\u5149\u7535\u6781\u7684PEC\u6027\u80fd\u63d0\u4f9b\u4e00\u4e2a\u6709\u6548\u7684\u89e3\u51b3\u65b9\u6848\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Embedding laser generated nanocrystals in BiVO4<\/sub> photoanode for efficient photoelectrochemical water splitting<\/a>, 2019, Nature communications, 10, 2609. DOI: 10.1038\/s41467-019-10543-z.<\/p>\n

\u3010\u8bfe\u9898\u7ec4\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u738b\u6d2a\u5f3a\uff0c\u897f\u5317\u5de5\u4e1a\u5927\u5b66\u6559\u6388\uff0c\u6750\u6599\u5b66\u9662\u526f\u9662\u957f\uff0c\u9655\u897f\u7701\u77f3\u58a8\u70ef\u8054\u5408\u5b9e\u9a8c\u5ba4\u526f\u4e3b\u4efb\u3002\u4e00\u76f4\u81f4\u529b\u4e8e\u77ac\u6001\u6781\u7aef\u6761\u4ef6\u4e0b\uff0c\u7eb3\u7c73\u6750\u6599\u7684\u7ed3\u6784\u6f14\u53d8\u53ca\u76f8\u5173\u7269\u7406\/\u5316\u5b66\u6027\u80fd\u7814\u7a76\u3002\u8fc4\u4eca\u4e3a\u6b62\uff0c\u5df2\u5728Chem. Soc. Rev., Nature Commun., J. Am. Chem. Soc., Angew. Chem. Int. Ed., Adv. Mater., Energy\u00a0Enviorn. Sci., ACS Nano, Nano Energy\u7b49\u671f\u520a\u53d1\u8868SCI\u8bba\u658770\u4f59\u7bc7\uff0c\u88ab\u5f153000\u4f59\u6b21\uff0cH\u56e0\u5b50\u662f30\u3002\u8bfe\u9898\u7ec4\u96b6\u5c5e\u4e8e\u897f\u5317\u5de5\u4e1a\u5927\u5b66\u51dd\u56fa\u6280\u672f\u56fd\u5bb6\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u548c\u7eb3\u7c73\u80fd\u6e90\u6750\u6599\u7814\u7a76\u4e2d\u5fc3\uff0c\u76ee\u524d\u4e3b\u8981\u5f00\u5c55\u77ac\u6001\u6781\u7aef\u6761\u4ef6\u6750\u6599\u4e0e\u5668\u4ef6\u7814\u7a76\uff0c\u7814\u7a76\u6d89\u53ca\u6fc0\u5149\u7269\u8d28\u76f8\u4e92\u4f5c\u7528\u3001\u754c\u9762\u8d85\u58f0\u5316\u5b66\u3001\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u3001\u5149\u7535\u5316\u5b66\u6c34\u5206\u89e3\u4ee5\u53ca\u9502\u79bb\u5b50\/\u9502\u786b\u7535\u6c60\u3002\u00a0<\/p>\n

\u672c\u6587\u7531\u91d1\u4e5f\u7f16\u8bd1\u4f9b\u7a3f\u3002<\/p>\n

\u00a0<\/strong><\/p>\n","protected":false},"excerpt":{"rendered":"

\u3010\u5f15\u8a00\u3011 \u5149\u7535\u50ac\u5316\u5206\u89e3\u6c34\u88ab\u8ba4\u4e3a\u662f\u4e00\u79cd\u6781\u5177\u6f5c\u80fd\u7684\u4ea7\u6c22\u6280\u672f\u3002\u5176\u4e2d\u9492\u9178\u94cb(BiVO4)\u4f5c\u4e3a\u4e00\u79cd\u5177\u6709\u4ee3\u8868\u6027\u7684\u91d1\u5c5e\u6c27\u5316\u7269\u5149\u9633\u6781\u6750\u6599\u53d7\u5230\u4e86\u7814\u7a76\u8005\u7684\u5e7f\u6cdb\u7814\u7a76\u3002\u7136\u800c\uff0c\u9492\u9178\u94cb\u7684\u8f7d…<\/p>\n","protected":false},"author":2114,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[],"class_list":["post-178512","post","type-post","status-publish","format-standard","hentry","category-jiedu"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/178512"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/2114"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=178512"}],"version-history":[{"count":4,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/178512\/revisions"}],"predecessor-version":[{"id":178621,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/178512\/revisions\/178621"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=178512"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=178512"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=178512"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}