{"id":177859,"date":"2019-06-18T06:30:45","date_gmt":"2019-06-17T22:30:45","guid":{"rendered":"\/\/m.iemloyee.com\/?p=177859"},"modified":"2019-06-17T20:08:55","modified_gmt":"2019-06-17T12:08:55","slug":"%e3%80%90%e5%b7%b2%e5%9b%9e%e5%a4%8d%e3%80%91%e5%9b%bd%e5%ae%b6%e7%ba%b3%e7%b1%b3%e7%a7%91%e5%ad%a6%e4%b8%ad%e5%bf%83nano-today%ef%bc%9a%e9%87%91%e5%b1%9e%e6%9c%89%e6%9c%ba%e6%a1%86%e6%9e%b6%e6%9d%90","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=177859","title":{"rendered":"\u56fd\u5bb6\u7eb3\u7c73\u79d1\u5b66\u4e2d\u5fc3Nano Today\uff1a\u91d1\u5c5e\u6709\u673a\u6846\u67b6\u6750\u6599\u2014\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u7684\u7406\u60f3\u8f7d\u4f53"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u7531\u4e8e\u5176\u5747\u4e00\u7684\u7ed3\u6784\u4e0e\u72ec\u7279\u7684\u50ac\u5316\u6027\u80fd\u800c\u5f15\u8d77\u4e86\u50ac\u5316\u9886\u57df\u7684\u6781\u5927\u5174\u8da3\u3002\u5728\u5404\u79cd\u591a\u5b54\u8f7d\u4f53\u4e2d\uff0c\u91d1\u5c5e\u6709\u673a\u6846\u67b6\u6750\u6599\uff08MOF\uff09\u7531\u4e8e\u5177\u6709\u6bd4\u8868\u9762\u79ef\u5927\uff0c\u7a33\u5b9a\u6027\u597d\uff0c\u7ed3\u6784\u660e\u786e\u6613\u8c03\u8282\u7b49\u7279\u70b9\uff0c\u6709\u671b\u6210\u4e3a\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u7684\u4e00\u79cd\u7406\u60f3\u8f7d\u4f53\u3002MOF\u7684\u8282\u70b9\u3001\u914d\u4f53\u4e0e\u7eb3\u7c73\u5b54\u9053\u63d0\u4f9b\u591a\u79cd\u7ed3\u5408\u4f4d\u70b9\uff0c\u53ef\u4ee5\u7cbe\u786e\u951a\u5b9a\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u5e76\u7cbe\u51c6\u8c03\u63a7\u5176\u6d3b\u6027\uff0c\u4fbf\u4e8e\u8fdb\u4e00\u6b65\u7814\u7a76\u50ac\u5316\u5242\u7684\u6784\u6548\u5173\u7cfb\u3002\u7ed3\u5408MOF\u7684\u7eb3\u7c73\u5b54\u9053\u9650\u57df\u6548\u5e94\uff0c\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u5728\u50ac\u5316\u6d3b\u6027\u3001\u9009\u62e9\u6027\u548c\u7a33\u5b9a\u6027\u65b9\u9762\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u6027\u80fd\u3002\u672c\u6587\u5bf9\u91d1\u5c5e\u6709\u673a\u6846\u67b6\u6750\u6599\u4f5c\u4e3a\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u7684\u8f7d\u4f53\u7684\u7814\u7a76\u8fdb\u884c\u4e86\u603b\u7ed3\u3001\u5206\u6790\u548c\u5c55\u671b\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u56fd\u5bb6\u7eb3\u7c73\u79d1\u5b66\u4e2d\u5fc3\u7684\u5510\u667a\u52c7\u7814\u7a76\u5458\u548c\u674e\u56fd\u680b\u7814\u7a76\u5458\uff08\u5171\u540c\u901a\u8baf\uff09<\/strong>\u7b49\u4eba\uff0c\u603b\u7ed3\u4e86MOF\u8d1f\u8f7d\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u7684\u8bbe\u8ba1\u3001\u7cbe\u51c6\u5408\u6210\u3001\u8868\u5f81\u548c\u50ac\u5316\u5e94\u7528\u7684\u6700\u65b0\u8fdb\u5c55\uff0c\u5e76\u9610\u660e\u4e86\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u7684\u7ed3\u6784\u4e0e\u6027\u80fd\u4e4b\u95f4\u7684\u5173\u7cfb\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201c<\/strong>Metal-organic frameworks as emerging platform for supporting isolated single-site catalysts<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728NanoToday<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u00a0<\/strong>1 MOF<\/strong>\u7684\u914d\u4f53\u3001\u8282\u70b9\u548c\u5b54\u9053\u8d1f\u8f7d\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u7684\u4e0d\u540c\u65b9\u6cd5\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe\u00a0<\/strong>2 MOF<\/strong>\u8282\u70b9\u4e0a\u4e0d\u540c\u6d3b\u6027\u7684\u6c22\u4f4d\u70b9<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09UiO-66\uff1b<\/p>\n

\uff08b\uff09NU-1000\uff1b<\/p>\n

\uff08c\uff09MOF-125\u3002<\/p>\n

\u56fe\u00a0<\/strong>3 MOF<\/strong>\u8282\u70b9\u7f9f\u57fa\u56fa\u5b9a\u5355\u4f4d\u70b9\u50ac\u5316\u5242<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09TPHN-MOF\u4e0eMe2<\/sub>Mg\u7684SBU\u7684\u5408\u6210\u540e\u91d1\u5c5e\u5316\u7684\u65b9\u6848\uff1b<\/p>\n

\uff08B\uff09UiO-68\u4e0eCoCl\uff1b<\/p>\n

\uff08C\uff09\u542bCoCl2<\/sub>\u7684MIL-125(Ti)\u3002<\/p>\n

\u56fe\u00a0<\/strong>4\u00a0<\/strong>\u79bb\u5b50\u4ea4\u6362\u6cd5\u5728<\/strong>MOF<\/strong>\u8282\u70b9\u8d1f\u8f7d\u5355\u4f4d\u70b9\u50ac\u5316\u5242<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe\u00a0<\/strong>5\u00a0<\/strong>\u5229\u7528<\/strong>ALD<\/strong>\u5728<\/strong>MOF<\/strong>\u8282\u70b9\u8d1f\u8f7d\u5355\u4f4d\u70b9\u50ac\u5316\u5242<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09Zr6<\/sub>\u57fa\u91d1\u5c5e\u9aa8\u67b6NU-1000\uff1b<\/p>\n

\uff08B\uff09\u5728MOF\u8868\u9762\u4e0aALD\u6c89\u79ef\u7684\u91d1\u5c5e\u5316\u8584\u819c\uff1b<\/p>\n

\uff08C\uff09Facac-\u914d\u4f53\u548cNi\u79bb\u5b50\u8d1f\u8f7d\u5230NU-1000\u7684Zr6<\/sub>\u8282\u70b9\u7684\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe\u00a0<\/strong>6 MOF<\/strong>\u914d\u4f53\u4e0a\u7684\u4e0d\u540c\u79cd\u7c7b\u7684\u7ed3\u5408\u4f4d\u70b9\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe\u00a0<\/strong>7\u00a0<\/strong>\u5229\u7528<\/strong>PSD<\/strong>\u548c<\/strong>PSE<\/strong>\u5408\u6210<\/strong>UiO-66-CAT<\/strong>\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe\u00a0<\/strong>8 MOF<\/strong>\u7eb3\u7c73\u5b54\u5185\uff0c\u5f00\u5b54\u5c01\u88c5\u6cd5\u8d1f\u8f7d\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe\u00a0<\/strong>9 <\/strong>\u914d\u4f53\u4ea4\u6362\u6cd5\u5728<\/strong>PCN-160<\/strong>\u4e2d\u8d1f\u8f7d\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u7684\u65b9\u6cd5\u53ca\u5176\u5408\u6210\u4ea7\u7269\u7167\u7247<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09PCN-160\u548cPCN-160-R\uff05M\u7684\u7ed3\u6784\u4ee5\u53ca\u8d1f\u8f7d\u4e0d\u540c\u91d1\u5c5e\u79bb\u5b50\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08B\uff09PCN-160\uff0cPCN-160-65\uff05\u548cPCN-160-65\uff05M\uff08M = Mn\uff0cFe\uff0cCo\uff0cNi\uff0cCu\u548cPd\uff09\u7684\u7167\u7247\u548c\u5149\u5b66\u663e\u5fae\u955c\u56fe\u50cf\u3002<\/p>\n

\u56fe<\/strong> 10 MOF<\/strong>\u8d1f\u8f7d\u4e0d\u540c\u6d3b\u6027\u4f4d\u70b9\u5b9e\u73b0\u7684\u534f\u540c\u50ac\u5316\u4f5c\u7528<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09Zr12<\/sub>-Ir\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

\uff08B\uff09Zr12<\/sub>-Ir\u7684HRTEM\u56fe\u50cf\u53caFFT\u56fe\uff1b<\/p>\n

\uff08C\uff09\u8d1f\u8f7d\u76840.02mol\uff05Zr12<\/sub>-Ir-Ni\u50ac\u5316\u5242\u4e0e\u5747\u76f8\u50ac\u5316\u5242\u7684\u8f6c\u5316\u7387\u4e0e\u65f6\u95f4\u7684\u5173\u7cfb\u66f2\u7ebf\u5bf9\u6bd4\u56fe\uff1b<\/p>\n

\uff08D\uff09\u8fde\u7eed\u516d\u6b21\u56de\u6536\u7684Zr12<\/sub>-Ir-Ni\u50ac\u5316\u7684\u4ea7\u7269\u7684\u4ea7\u7387\u56fe\uff1b<\/p>\n

\uff08E\uff09Zr12<\/sub>-Ir-Ni\u50ac\u5316\u7684C-S\u4ea4\u53c9\u5076\u8054\u53cd\u5e94\u7684\u673a\u7406\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe\u00a0<\/strong>11\u00a0<\/strong>\u5b54\u9053\u9650\u57df\u5b9e\u73b0\u975e\u70ed\u529b\u5b66\u4ea7\u7269\u7684\u9ad8\u9009\u62e9\u6027<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09\u50ac\u5316\u5242UiO-67-Mix-Ir\u7684\u5408\u6210\u65b9\u6848\uff1b<\/p>\n

\uff08B\uff09\u7532\u70f7\u4e0eB2<\/sub>pin2<\/sub>\u7684\u53cd\u5e94\u65b9\u6848\u3002<\/p>\n

\u56fe<\/strong> 12 MOF<\/strong>\u5b54\u4e2d\u5c40\u90e8\u7a7a\u95f4\u4f4d\u963b\u5bf9\u53cd\u5e94\u7684\u5f71\u54cd<\/strong><\/p>\n

\"\"<\/p>\n

\u3010\u7ed3\u8bba\u4e0e\u5c55\u671b\u3011<\/strong><\/p>\n

\u672c\u6587\u603b\u7ed3\u4e86MOF\u8d1f\u8f7d\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u7684\u53ef\u63a7\u5408\u6210\u7684\u6700\u65b0\u8fdb\u5c55\u4ee5\u53ca\u5176\u5728\u4e0d\u540c\u7684\u50ac\u5316\u53cd\u5e94\u4e2d\u7684\u5e94\u7528\u3002\u968f\u7740\u5408\u6210\u5316\u5b66\u7684\u5feb\u901f\u53d1\u5c55\uff0c\u53ef\u901a\u8fc7\u4e0d\u540c\u7684\u7b56\u7565\u6210\u529f\u6784\u5efaMOFs\u8d1f\u8f7d\u5355\u4f4d\u70b9\u50ac\u5316\u5242\uff0c\u5e76\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u50ac\u5316\u6027\u80fd\uff1a\uff081\uff09\u6709\u673a\u914d\u4f53\u548c\u91d1\u5c5e\u8282\u70b9\u7684\u9ad8\u5ea6\u6709\u5e8f\u6392\u5217\u4ee5\u53ca\u591a\u7ea7\u6b21\u7684\u7eb3\u7c73\u5b54\u7ed3\u6784\u4f7fMOF\u6210\u4e3a\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u7684\u7406\u60f3\u8f7d\u4f53\uff0c\u8f7d\u4f53\u4e0e\u50ac\u5316\u5242\u7ed3\u6784\u660e\u786e\uff1b\uff082\uff09\u9ad8\u6bd4\u8868\u9762\u79ef\u53ef\u4ee5\u63d0\u9ad8\u50ac\u5316\u5242\u7684\u8d1f\u8f7d\u91cf\uff1b\uff083\uff09\u7eb3\u7c73\u5b54\u9053\u53ef\u4e3a\u5e95\u7269\u63d0\u4f9b\u7279\u6b8a\u7684\u5316\u5b66\u73af\u5883\uff0c\u4f7f\u5176\u4e0e\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\u76f8\u4e92\u4f5c\u7528\uff0c\u7c7b\u4f3c\u4e8e\u9176\u6d3b\u6027\u4f4d\u70b9\u7684\u4e8c\u7ea7\u7ed3\u6784\uff0c\u53ef\u8fdb\u4e00\u6b65\u63d0\u9ad8\u6d3b\u6027\u548c\u9009\u62e9\u6027\u3002MOF\u7ed3\u6784\u660e\u786e\u4e14\u9ad8\u5ea6\u53ef\u8c03\uff0c\u5176\u4e0e\u5355\u4f4d\u70b9\u50ac\u5316\u5242\u4e4b\u95f4\u7684\u529f\u80fd\u534f\u540c\u4f5c\u7528\u4e3a\u7cbe\u51c6\u6784\u5efa\u5177\u6709\u539f\u5b50\u7ea7\u7cbe\u786e\u7ed3\u6784\u50ac\u5316\u5242\u63d0\u4f9b\u4e86\u65e0\u9650\u53ef\u80fd\u3002<\/p>\n

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\u672c\u6587\u7684\u7b2c\u4e00\u4f5c\u8005\u4e3a\u56fd\u5bb6\u7eb3\u7c73\u79d1\u5b66\u4e2d\u5fc3\u76f4\u535a\u751f\u8d75\u6587\u4e16<\/strong>\u3002\u8be5\u5de5\u4f5c\u5f97\u5230\u4e86\u79d1\u6280\u90e8\u91cd\u70b9\u7814\u53d1\u8ba1\u5212\u3001\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u548c\u4e2d\u79d1\u9662\u7b49\u9879\u76ee\u7684\u652f\u6301\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Metal-organic frameworks as emerging platform for supporting isolated single-site catalysts<\/strong><\/a>\uff08Nano Today, 2019, DOI: 10.1016\/j.nantod.2019.05.007\uff09\u3002<\/p>\n

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