{"id":175677,"date":"2019-05-22T12:00:50","date_gmt":"2019-05-22T04:00:50","guid":{"rendered":"\/\/m.iemloyee.com\/?p=175677"},"modified":"2019-05-21T23:16:21","modified_gmt":"2019-05-21T15:16:21","slug":"%e9%99%95%e8%a5%bf%e5%b8%88%e5%a4%a7%e5%88%98%e7%94%9f%e5%bf%a0%e5%9b%a2%e9%98%9fnat-commun-%ef%bc%9a%e5%8d%95%e5%8e%9f%e5%ad%90%e9%92%a8%e6%8e%ba%e6%9d%82%e8%b6%85%e8%96%84%ce%b1-nioh2%e5%a2%9e","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=175677","title":{"rendered":"\u9655\u897f\u5e08\u5927\u5218\u751f\u5fe0\u56e2\u961fNat. Commun.\uff1a\u5355\u539f\u5b50\u94a8\u63ba\u6742\u8d85\u8584\u03b1-Ni(OH)2\u589e\u5f3a\u7535\u50ac\u5316\u6c34\u6c27\u5316"},"content":{"rendered":"

<\/b>\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u7535\u50ac\u5316\u5206\u89e3\u6c34\u751f\u6210H2<\/sub>\u548cO2<\/sub>\uff0c\u7136\u800c\uff0c\u6c27\u7684\u534a\u53cd\u5e94\u4ecd\u7136\u662f\u5236\u7ea6\u8fd9\u79cd\u8fdb\u5c55\u7684\u74f6\u9888\u3002\u6c27\u6790\u51fa\u53cd\u5e94\uff08OER\uff09\u5728\u52a8\u529b\u5b66\u4e0a\u662f\u7f13\u6162\u7684\uff0c\u9700\u8981O-H\u952e\u65ad\u88c2\u548c\u4f34\u968fO-O\u952e\u5f62\u6210\u7684\u4e24\u4e2a\u5fc5\u8981\u6b65\u9aa4\uff0c\u5176\u4e2d\u5305\u62ec\u56db\u4e2a\u7535\u5b50\u7684\u8f6c\u79fb\u3002\u56e0\u6b64\uff0c\u9700\u8981\u8bbe\u8ba1OER\u7535\u50ac\u5316\u5242\u3002\u4ee5\u8d35\u91d1\u5c5e\u57fa\u50ac\u5316\u5242\uff0c\u5982IrO2<\/sub>\u548cRuO2<\/sub>\uff0c\u8868\u73b0\u51fa\u5438\u5f15\u529b\u7684OER\u6d3b\u6027\uff0c\u4f46\u5b83\u4eec\u7684\u7a00\u6709\u6027\u963b\u788d\u4e86\u5b83\u4eec\u7684\u5927\u89c4\u6a21\u5e94\u7528\u3002\u8fd1\u5e74\u6765\uff0c\u5229\u7528\u4e30\u5bcc\u7684\u4e09\u7ef4\u91d1\u5c5e\uff08Fe\uff0cCo\uff0cMn\u548cNi\uff09\uff0c\u7814\u7a76\u4e86\u8bb8\u591a\u975e\u8d35\u91d1\u5c5e\u7684OER\u50ac\u5316\u5242\uff0c\u5176\u6d3b\u6027\u548c\u7a33\u5b9a\u6027\u5747\u6709\u63d0\u9ad8\u3002\u7279\u522b\u662f\uff0cNi(OH)2<\/sub>\u57fa\u6837\u54c1\u5f15\u8d77\u4e86\u6781\u5927\u7684\u5174\u8da3\uff0c\u7814\u7a76\u8868\u660e\u5b83\u4eec\u5177\u6709\u5f88\u597d\u7684\u6c34\u6c27\u5316\u6f5c\u529b\u3002\u6b64\u5916\uff0c\u4f4e\u542b\u91cfFe\u63ba\u6742Ni(OH)2<\/sub>\u5df2\u88ab\u8bc1\u660e\u5927\u5927\u63d0\u9ad8\u4e86\u6027\u80fd\u3002\u7136\u800c\uff0c\u63d0\u9ad8\u6d3b\u6027\u7684Ni(OH)2<\/sub>\u57faOER\u50ac\u5316\u5242\u7684\u5f00\u53d1\u8fd8\u9700\u8981\u53d6\u5f97\u5b9e\u8d28\u6027\u8fdb\u5c55\u3002\u5728Fe\u63ba\u6742\u7684Ni(OH)2<\/sub>\u6837\u54c1\uff0c\u867d\u7136Fe3+<\/sup>\u66ff\u4ee3\u90e8\u5206Ni2+<\/sup>\u5df2\u88ab\u8bc1\u660e\u53ef\u4ee5\u589e\u5f3a\u6c27\u6790\u51fa\uff0c\u8fd9\u662f\u57fa\u4e8eNi(OH)2<\/sub>\u7684\u6837\u54c1\u8868\u9762\u6c34\u6c27\u5316\u7684\u6838\u5fc3\u90e8\u5206\uff0c\u5373\u66b4\u9732\/\u63a5\u89e6\u7684Ni(OH)2<\/sub>\u8868\u9762\u4e0a\u7684\u53cd\u5e94\u884c\u4e3a\u5f88\u5c11\u88ab\u7814\u7a76\u548c\u62a5\u9053\u3002\u6b64\u5916\uff0cNi(OH)2<\/sub>\u57fa\u7535\u50ac\u5316\u5242\u7684OER\u6027\u80fd\u4ecd\u7136\u9700\u8981\u901a\u8fc7\u63ba\u6742\u6765\u6539\u5584\uff0c\u5e76\u4e14\u4ecd\u7136\u9700\u8981\u5f00\u53d1\u5408\u9002\u5143\u7d20\u7684\u53d1\u73b0\u3002\u5728\u7535\u50ac\u5316\u8fc7\u7a0b\u4e2d\uff0c\u5728\u50ac\u5316\u5242|\u6eb6\u6db2\u754c\u9762\u5b58\u5728\u53cc\u7535\u5c42\uff08Helmholtz layer, HL\uff09\u3002\u7535\u8def\u662f\u901a\u8fc7\u4e09\u79cd\u7535\u963b\u63aa\u65bd\u5b8c\u6210\u7684\uff0c\u5373\u50ac\u5316\u5242\u3001\u50ac\u5316\u5242|\u6eb6\u6db2\u754c\u9762\u3001\u6eb6\u6db2\u3002\u7531\u4e8e\u56fa\u4f53\u5411\u6eb6\u6db2\u8f6c\u53d8\u6240\u4ea7\u751f\u7684\u7535\u5bb9\u6027\u548c\u963b\u6027\u7279\u6027\uff0cHL\u5bf9\u6700\u7ec8\u7684\u7535\u50ac\u5316\u6548\u7387\u5177\u6709\u91cd\u8981\u7684\u51b3\u5b9a\u4f5c\u7528\u3002\u5728\u6c34\u5206\u89e3\u7684\u60c5\u51b5\u4e0b\uff0cH2<\/sub>O\u5206\u5b50\u548cOH–<\/sup>\u57fa\u56e2\u5728HL\u4e2d\u7684\u5438\u9644\u548c\u89e3\u5438\u884c\u4e3a\u5c06\u76f4\u63a5\u5f71\u54cdH2<\/sub>\u6216O2<\/sub>\u7684\u751f\u6210\u3002\u56e0\u6b64\uff0c\u5e94\u8be5\u8fdb\u4e00\u6b65\u7814\u7a76\u66b4\u9732\u5143\u7d20\uff08\u5982Ni\u6216Fe\uff09\u7684\u914d\u4f4d\u7279\u6027\uff0c\u4ee5\u6f5c\u5728\u5730\u63d0\u9ad8\u6027\u80fd\u3002\u9002\u5f53\u7684\u5316\u5b66\u73af\u5883\u3001\u7535\u6781\u4e0e\u4e2d\u95f4\u4f53\u4e4b\u95f4\u7684\u952e\u5408\u5f3a\u5ea6\u548c\u7535\u5b50\u8fc1\u79fb\u963b\u529b\u662f\u5bfc\u81f4\u660e\u663e\u7684OER\u589e\u5f3a\u7684\u5173\u952e\u56e0\u7d20\u3002\u56e0\u6b64\uff0c\u9700\u8981\u627e\u5230\u4e00\u4e2a\u5408\u9002\u7684\u53cd\u5e94\u4f4d\u70b9\u6765\u5b9e\u73b0\u4e2d\u95f4\u4f53\u7684\u5f62\u6210\u548c\u8fc1\u79fb\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5728\u9655\u897f\u5e08\u8303<\/b><\/strong>\u5927\u5b66\u5218\u751f\u5fe0\u6559\u6388\u3001<\/b><\/strong>\u82cf\u5dde<\/b><\/strong>\u5927\u5b66\u674e\u6709\u52c7<\/b><\/strong>\u6559\u6388<\/b><\/strong>\u56e2\u961f\uff08<\/b><\/strong>\u5171\u540c<\/b><\/strong>\u901a\u8baf\u4f5c\u8005\uff09<\/b><\/strong>\u5e26\u9886\u4e0b\uff0c\u4e0e\u6fb3\u5927\u5229\u4e9a<\/b><\/strong>\u7ebd\u5361\u65af\u5c14\u5927\u5b66<\/b><\/strong>\u3001\u4e2d\u79d1\u9662\u9ad8\u80fd\u7269\u7406\u7814\u7a76\u6240<\/b><\/strong>\u548c\u4e2d\u79d1\u9662\u5927\u8fde\u5316\u7269\u6240<\/b><\/strong>\u5408\u4f5c\uff0c\u62a5\u544a\u4e86\u4e00\u4e2a\u5355\u539f\u5b50W6+<\/sup>\u63ba\u6742Ni(OH)2<\/sub>\u7eb3\u7c73\u7247\u6837\u54c1\uff08w-Ni(OH)2<\/sub>\uff09\uff0cw-Ni(OH)2<\/sub>\u7531w-Ni(OH)2<\/sub>-e\u7684\u957f\u65f6\u95f4\u8d85\u58f0\u5265\u79bb\u5408\u6210\uff0c\u91c7\u7528\u9187\u70ed\u6cd5\u5408\u6210\u3002w-Ni(OH)2<\/sub>\u5177\u6709\u4f18\u5f02\u7684\u6790\u6c27\u53cd\u5e94\u6027\u80fd\uff0c\u5373\u57281 M KOH\u4ecb\u8d28\u4e2d\uff0c\u572810 mA\/cm2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u65f6\u83b7\u5f97\u4e86237 mV\u7684\u8fc7\u7535\u4f4d\u3002\u6b64\u5916\uff0c\u5728\u9ad8\u7535\u6d41\u5bc6\u5ea6\u4e3a80 mA\/cm2<\/sup>\u65f6\uff0c\u8fc7\u7535\u4f4d\u503c\u4ec5\u4e3a267 mV\u3002\u6d4b\u5f97\u76f8\u5e94\u7684\u5854\u83f2\u5c14\u659c\u7387\u4e3a33 mV\/dec\u3002\u4f4e\u81ea\u65cb\u6001\u7684d0<\/sup>\u00a0W6+<\/sup>\u539f\u5b50\u6709\u66f4\u591a\u7684\u6700\u5916\u5c42\u7a7a\u8f68\u9053\uff0c\u5bfc\u81f4\u66f4\u591a\u7684\u6c34\u548cOH–<\/sup>\u57fa\u56e2\u88ab\u5438\u9644\u5728Ni(OH)2<\/sub>\u7eb3\u7c73\u8584\u7247\u7684W\u4f4d\u70b9\u4e0a\u3002\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\uff08DFT\uff09\u8ba1\u7b97\u8bc1\u5b9e\uff0cO\u57fa\u548cO-O\u8026\u5408\u90fd\u662f\u5728W6+<\/sup>\u7684\u540c\u4e00\u4f4d\u70b9\u4ea7\u751f\u7684\u3002\u7814\u7a76\u8868\u660e\uff0cW6+<\/sup>\u63ba\u6742\u5bf9Ni(OH)2<\/sub>\u7535\u50ac\u5316\u6c34\u6c27\u5316\u6d3b\u6027\u7684\u4fc3\u8fdb\u4f5c\u7528\u6700\u5f3a\u3002\u76f8\u5173\u6210\u679c\u4ee5\u9898\u4e3a\u201c<\/b><\/strong>Single atom tungsten doped ultrathin \u03b1-Ni(OH)<\/b><\/strong>2<\/b><\/sub><\/strong>\u00a0for enhanced electrocatalytic water oxidation<\/b><\/strong>\u201d<\/b><\/strong>\u53d1\u8868\u5728\u4e86Nat. Commun.<\/b><\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe1<\/b><\/strong>\u00a0<\/b><\/strong>Ni(OH)<\/b><\/strong>2<\/b><\/sub><\/strong>\u5728OER\u8fc7\u7a0b\u4e2d\u7684\u7535\u5316\u5b66\u5206\u6790<\/b><\/strong>\"\" <\/b><\/strong>a.Ni(OH)2<\/sub>\u7684\u5faa\u73af\u4f0f\u5b89\u6cd5\uff08CV\uff09\uff0c\u7535\u4f4d\u8303\u56f4\u4e3a0.6-1.8\u00a0V\u3002<\/p>\n

b.\u57281.2\uff0c1.45\u548c1.6\u00a0V\u7684\u4e09\u4e2a\u7535\u4f4d\u4e0b\u7684Ni(OH)2<\/sub>\u7684EIS\u56fe\u3002<\/p>\n

c.EIS\u56fe\u62df\u5408\u7684\u7b49\u6548\u7535\u8def\u3002<\/p>\n

d.\u88681\u4e2d\u62df\u5408\u7535\u963b\u503c\u7684\u53d8\u5316\u7387\u3002\u76f8\u5e94\u7684\u589e\u52a0\u548c\u51cf\u5c11\u901f\u7387\u5206\u522b\u4e3aR\u03a9<\/sub>\u548cRct<\/sub>\u3002\u57281\u00a0M KOH\u6eb6\u6db2\u4e2d\u6d4b\u91cfCV\u548cEIS\u3002<\/p>\n

\u00a0<\/b><\/strong>\u56fe2<\/b><\/strong>\u00a0<\/b><\/strong>\u7269\u7406\u5316\u5b66\u6027\u8d28\u8868\u5f81<\/b><\/strong>\"\"<\/p>\n

a.Ni(OH)2<\/sub>-r\uff0cw-Ni(OH)2<\/sub>-e\u548cw-Ni(OH)2<\/sub>\u6837\u54c1\u7684XRD\u56fe\u8c31\u3002<\/p>\n

b.Ni(OH)2<\/sub>-r\uff0cw-Ni(OH)2<\/sub>-e\u548cw-Ni(OH)2<\/sub>\u6837\u54c1\u7684\u7d2b\u5916-\u53ef\u89c1\u5438\u6536\u5149\u8c31\u3002<\/p>\n

c,d.\u5206\u522b\u4e3aw-Ni(OH)2<\/sub>\uff0cWO3<\/sub>\u548cW\u7c89\u672b\u7684W K\u8fb9\u7f18XANES\u5149\u8c31\u548c\u76f8\u5e94\u7684K2<\/sup>\u52a0\u6743\u5085\u91cc\u53f6\u53d8\u6362\u5149\u8c31\u3002<\/p>\n

\u56fe3<\/b><\/strong>\u00a0<\/b><\/strong>w-Ni(OH)<\/b><\/strong>2<\/b><\/sub><\/strong>\u6837\u54c1<\/b><\/strong>\u7684\u7535\u955c\u8868\u5f81<\/b><\/strong>\"\"<\/p>\n

a.w-Ni(OH)2<\/sub>\u6837\u54c1\u7684\u626b\u63cf\u7535\u955c\u56fe\uff0c\u6bd4\u4f8b\u5c3a\uff1a100\u00a0nm\u3002<\/p>\n

b.w-Ni(OH)2<\/sub>\u6837\u54c1\u7684\u900f\u5c04\u7535\u955c\u56fe\uff0c\u63d2\u56fe\u663e\u793a\u4e86\u76f8\u5e94\u7684\u7535\u5b50\u884d\u5c04\u8c31\uff0c\u6bd4\u4f8b\u5c3a\uff1a100\u00a0nm\u3002<\/p>\n

c.w-Ni(OH)2<\/sub>\u6837\u54c1\u7684HADDF\u56fe\u4e0e\u76f8\u5e94\u7684\u5143\u7d20\u5206\u5e03\u56fe\uff0c\u6bd4\u4f8b\u5c3a\u4e3a100 nm\u3002<\/p>\n

d,e.w-Ni(OH)2<\/sub>\u6837\u54c1\u7684HAADF-STEM\u56fe\u50cf\uff0cd\u548ce\u7684\u6bd4\u4f8b\u5c3a\u5206\u522b\u4e3a0.5\u548c1 nm\u3002<\/p>\n

\u56fe<\/b><\/strong>4<\/b><\/strong>\u00a0<\/b><\/strong>\u7535\u50ac\u5316\u6c34\u6c27\u5316\u6027\u80fd<\/b><\/strong>\"\"<\/p>\n

a.Ni(OH)2<\/sub>-r\uff0cw-Ni(OH)2<\/sub>-e\u548cw-Ni(OH)2<\/sub>\u6837\u54c195\uff05iR\u6821\u6b63\u7684\u6781\u5316\u66f2\u7ebf\u3002<\/p>\n

b.\u4e0d\u540c\u7535\u6781\u4e0bj = 10,50,80\u00a0mA cm-2<\/sup>\u7684\u8fc7\u7535\u4f4d\u3002<\/p>\n

c.Ni(OH)2<\/sub>-r\uff0cw-Ni(OH)2<\/sub>-e\u548cw-Ni(OH)2<\/sub>\u7535\u6781\u7684Tafel\u66f2\u7ebf\u3002<\/p>\n

d.\u57281.48V\u7684\u504f\u7f6e\u7535\u4f4d\u4e0b\uff0cNi(OH)2<\/sub>-r\uff0cw-Ni(OH)2<\/sub>-e\u548cw-Ni(OH)2<\/sub>\u7535\u6781\u7684EIS\u56fe\u3002<\/p>\n

e.\u4ee5w-Ni(OH)2<\/sub>\u4e3a\u50ac\u5316\u5242\uff0c\u5728\u5404\u79cd\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5bf9OER\u8fdb\u884c\u8ba1\u65f6\u7535\u4f4d\u6d4b\u91cf\u3002\u6240\u6709\u6d4b\u8bd5\u5747\u57281\u00a0M KOH\u6eb6\u6db2\uff08O2<\/sub>\u9971\u548c\uff09\u4e2d\u8fdb\u884c\u3002<\/p>\n

\u56fe5<\/b><\/strong>\u00a0<\/b><\/strong>DFT\u8ba1\u7b97<\/b><\/strong>\"\"<\/p>\n

a,b.\u57fa\u4e8eDFT\u8ba1\u7b97\u7684\uff08a\uff09W\u63ba\u6742Ni(OH)2<\/sub>\u548c\uff08b\uff09\u88f8Ni(OH)2<\/sub>\u50ac\u5316\u5242\u4e0aOER\u673a\u7406\uff0c\u5176\u4e2d\u7ea2\u3001\u767d\u3001\u7eff\u3001\u84dd\u539f\u5b50\u5206\u522b\u4ee3\u8868\u6c27\u3001\u6c22\u3001\u954d\u548c\u94a8\u539f\u5b50\u3002\u201c+\u201d\u548c\u201c-\u201d\u7684\u7b26\u53f7\u4ee3\u8868\u5438\u70ed\u548c\u653e\u70ed\u81ea\u7531\u80fd\u3002\u5bf9\u4e8e\u4ece\u72b6\u60016\u5230\u72b6\u60011\u7684\u6b65\u9aa4\uff0c\u5bf9\u4e8e\u63ba\u6742\u6837\u54c1\u548c\u88f8\u6837\u54c1\u5206\u522b\u9700\u89811.0 eV\u548c0.4 eV\u5438\u70ed\u81ea\u7531\u80fd\u503c\uff0c\u800c\u8fd9\u4e9b\u81ea\u7531\u80fd\u53d8\u5316\u672a\u5728\u4e0a\u9762\u663e\u793a\u3002<\/p>\n

\u3010\u5c0f\u7ed3<\/b><\/strong>\u3011<\/p>\n

\u603b\u4e4b\uff0c\u56e2\u961f\u62a5\u9053\u4e86\u5355\u539f\u5b50W\u63ba\u6742Ni(OH)2<\/sub>\u7eb3\u7c73\u7247\u7528\u4e8e\u7535\u50ac\u5316\u6c34\u6c27\u5316\u53cd\u5e94\u3002\u4e0e\u7eaf\u5c42\u72b6Ni(OH)2<\/sub>\u7684\u53c2\u8003\u6837\u54c1\u76f8\u6bd4\uff0cw-Ni(OH)2<\/sub>\u7684OER\u6027\u80fd\u6709\u660e\u663e\u7684\u63d0\u9ad8\uff1a\u8fbe\u523010 mA\/cm2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u53ea\u9700\u8981237 mV\u7684\u8fc7\u7535\u4f4d\u3002\u6b64\u5916\uff0c\u5728\u9ad8\u7535\u6d41\u5bc6\u5ea6\u4e3a80 mA\/cm2<\/sup>\u65f6\uff0cw-Ni(OH)2<\/sub>\u6837\u54c1\u7684\u8fc7\u7535\u4f4d\u503c\u4ec5\u4e3a267 mV\uff0c\u6d4b\u91cf\u7684Tafel\u659c\u7387\u4e3a33 mV\/dec\u3002\u6240\u6709\u503c\u5747\u4e3a\u6587\u732e\u4e2d\u76ee\u524d\u62a5\u9053\u7684\u6837\u672c\u7684\u6700\u4f73\/\u6700\u9ad8\u6c34\u5e73\u3002\u6839\u636eDFT\u8ba1\u7b97\uff0cw-Ni(OH)2<\/sub>\u5728\u6c34\u6c27\u5316\u53cd\u5e94\u7684\u524d\u4e09\u4e2a\u9636\u6bb5\u8868\u73b0\u4e3a\u653e\u70ed\u53cd\u5e94\uff1a\u6c34\u5438\u9644\u3001\u5438\u9644OH–<\/sup>\u57fa\u56e2\u548cO\u57fa\u56e2\u7684\u5f62\u6210\u3002\u7531\u4e8e0.05\u7684\u4f4e\u81ea\u65cb\u96c6\u5c45\u6570\uff0cd0<\/sup>\u00a0W6+<\/sup>\u4f4d\u70b9\u7a33\u5b9a\u4e86O\u57fa\u56e2\u3002\u6700\u91cd\u8981\u7684\u662f\uff0c\u63a5\u4e0b\u6765\u7684O-O\u8026\u5408\u6b65\u9aa4\u4e5f\u5728W6+<\/sup>\u4f4d\u70b9\u4ea7\u751f\uff0c\u4ec5\u9700\u8981\u51e0\u4e4e\u4e3a\u96f6\u7684\u5409\u5e03\u65af\u81ea\u7531\u80fd\u3002\u8fd9\u79cd\u6548\u5e94\u6709\u52a9\u4e8eW6+<\/sup>\u79bb\u5b50\u4fc3\u8fdbNi(OH)2<\/sub>\u7684\u6700\u7ec8\u6c34\u6c27\u5316\u53cd\u5e94\u3002\u8fd9\u9879\u5de5\u4f5c\u6709\u52a9\u4e8e\u6211\u4eec\u4e86\u89e3HL\u5bf9\u6c34\u6c27\u5316\u7684\u5f71\u54cd\uff0c\u4e3a\u8bbe\u8ba1\u63ba\u6742OER\u50ac\u5316\u5242\u63d0\u4f9b\u4e86\u65b0\u7684\u65b9\u5411\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>Single atom tungsten doped ultrathin \u03b1-Ni(OH)<\/u>2<\/sub><\/u>\u00a0for enhanced electrocatalytic water oxidation<\/u><\/a>\uff08Nat. Commun.\uff0c2019\uff0c\u00a0DOI:10.1038\/s41467-019-09845-z\uff09<\/p>\n

\u672c\u6587\u7531\u6728\u6587\u97ec<\/b><\/strong>\u7ffb\u8bd1\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n

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