{"id":175148,"date":"2019-05-14T06:30:30","date_gmt":"2019-05-13T22:30:30","guid":{"rendered":"\/\/m.iemloyee.com\/?p=175148"},"modified":"2019-05-13T21:01:46","modified_gmt":"2019-05-13T13:01:46","slug":"%e9%82%a3%e4%ba%9b%e5%b9%b4%ef%bc%8c%e9%a1%b6%e5%88%8ascience%e4%b8%8a%e7%94%b5%e5%82%ac%e5%8c%96%e9%a2%86%e5%9f%9f%e7%9a%84%e7%b2%be%e5%8d%8e%ef%bc%8c%e4%bd%a0%e6%9c%89%e6%b2%a1%e6%9c%89%e9%94%99","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=175148","title":{"rendered":"\u90a3\u4e9b\u5e74\uff0c\u9876\u520aScience\u4e0a\u7535\u50ac\u5316\u9886\u57df\u7684\u7cbe\u534e\uff0c\u4f60\u6709\u6ca1\u6709\u9519\u8fc7\uff1f"},"content":{"rendered":"
\u7ecf\u8fc7100\u5e74\u7684\u53d1\u5c55\uff0c\u7535\u50ac\u5316\u4ece\u6700\u521d\u7535\u5316\u5b66\u7684\u4e00\u4e2a\u5206\u652f\u5230\u76ee\u524d\u5df2\u7ecf\u6210\u4e3a\u4e00\u95e8\u4ea4\u53c9\u6027\u6781\u5f3a\u7684\u5b66\u79d1\uff0c\u57fa\u7840\u77e5\u8bc6\u6d89\u53ca\u7535\u5316\u5b66\u3001\u50ac\u5316\u79d1\u5b66\u3001\u8868\u754c\u9762\u79d1\u5b66\u53ca\u6750\u6599\u5b66\u7b49\uff0c\u5176\u5e94\u7528\u5e7f\u6cdb\u5b58\u5728\u4e8e\u80fd\u6e90\u8f6c\u6362\u53ca\u5b58\u50a8\u9886\u57df\uff08\u71c3\u6599\u7535\u6c60\u3001\u8d85\u7ea7\u7535\u5bb9\u5668\u3001\u7535\u89e3\u6c34\u5236\u6c22\u3001\u592a\u9633\u80fd\u7535\u6c60\u7b49\uff09\u3002\u672c\u6587\u5206\u4eab\u4e86\u5341\u7bc72016-2019\u5e74Science\u4e0a\u53d1\u8868\u7684\u7535\u50ac\u5316\u7ecf\u5178\u5de5\u4f5c\uff0c\u5185\u5bb9\u6db5\u76d6\u7535\u89e3\u6c34\u4e2d\u7684\u6790\u6c22 (HER)\u3001\u6790\u6c27\u53cd\u5e94 (OER)\uff0c\u71c3\u6599\u7535\u6c60\u4e2d\u91cd\u8981\u7684\u534a\u53cd\u5e94\u6c27\u8fd8\u539f\u53cd\u5e94 (ORR)\uff0c\u4ee5\u53ca\u7535\u50ac\u5316\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\u53cd\u5e94\u3002\u65e0\u8bba\u5e94\u7528\u7684\u9886\u57df\u662f\u54ea\u79cd\u7535\u50ac\u5316\u53cd\u5e94\uff0c\u50ac\u5316\u5242\u5747\u662f\u6838\u5fc3\uff0c\u7535\u50ac\u5316\u7814\u7a76\u7684\u9996\u8981\u4efb\u52a1\u5c31\u662f\u8bbe\u8ba1\u5e76\u5236\u5907\u51fa\u5bf9\u7279\u5b9a\u53cd\u5e94\u5177\u6709\u9ad8\u6d3b\u6027\u3001\u9ad8\u9009\u62e9\u6027\u548c\u957f\u5bff\u547d\u7684\u7535\u50ac\u5316\u5242\uff0c\u9876\u7ea7\u671f\u520a\u4e2d\u57fa\u672c\u90fd\u4f1a\u540c\u65f6\u6d89\u53ca\u6750\u6599\u7ed3\u6784\u8bbe\u8ba1\u7b56\u7565\u548c\u6784\u6548\u5173\u7cfb\u5206\u6790\uff0c\u4ee5\u53ca\u5982\u4f55\u5b9e\u73b0\u529f\u80fd\u6027\u50ac\u5316\u5242\u7684\u8bbe\u8ba1\u548c\u5e94\u7528\uff0c\u5e0c\u671b\u5206\u4eab\u7684\u76f8\u5173\u5de5\u4f5c\u80fd\u591f\u5bf9\u76f8\u5173\u9886\u57df\u7684\u7814\u7a76\u4eba\u5458\u6709\u6240\u542f\u53d1\u3002<\/p>\n
\u4e00\u3001Direct atomic-level insight into the active sites of a high-performance PGM-free ORR catalyst1<\/sup><\/strong><\/p>\n \u50ac\u5316\u53cd\u5e94\u4e2d\u660e\u786e\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\u4e00\u76f4\u662f\u76f8\u5173\u7814\u7a76\u9886\u57df\u7684\u91cd\u70b9\uff0c\u7f8e\u56fd\u6d1b\u65af\u963f\u62c9\u83ab\u65af\u56fd\u5bb6\u5b9e\u9a8c\u5ba4Piotr Zelenay\u6559\u6388\u7b49\u4eba\u5236\u5907\u51fa\u4e00\u79cd\u6709\u9ad8\u5b54\u9699\u7387\u7ed3\u6784\u7684Fe-N-C\u50ac\u5316\u5242\uff0c\u63d0\u51fa\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\u662f\u78b3\u5d4c\u5165\u7684\u6c2e\u914d\u4f4d\u94c1\uff08FeN4<\/sub>\uff09\uff0c\u5e76\u901a\u8fc7\u50cf\u5dee\u6821\u6b63\u7684\u626b\u63cf\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c\u5f97\u5230\u4e86FeN4<\/sub>\u6d3b\u6027\u4f4d\u70b9\u7684\u539f\u5b50\u7ea7\u56fe\u50cf\uff0c\u6750\u6599\u8868\u9762\u80fd\u591f\u89c2\u5bdf\u5230\u76f8\u5f53\u9ad8\u6d53\u5ea6\u7684\u5206\u6563\u7684Fe\u5355\u539f\u5b50\u3002\u901a\u8fc7\u8ba1\u7b97\u63a2\u7d22\u4e86\u4e0e\u7279\u5b9a\u6676\u683c\u7ea7\u78b3\u7ed3\u6784\u76f8\u5173\u7684\u8fd9\u4e9b\u6d3b\u6027\u4f4d\u70b9\u5bf9\u50ac\u5316ORR\u7684\u8d21\u732e\u3002\u4e0e\u5927\u591a\u6570M-N-C\u6750\u6599\u4f5c\u805a\u5408\u7269\u7535\u89e3\u8d28\u71c3\u6599\u7535\u6c60\uff08PEFC\uff09\u9634\u6781\u7684\u7814\u7a76\u4e0d\u540c\uff0c\u8be5\u50ac\u5316\u5242\u76f4\u63a5\u7528\u4e8e\u6c7d\u8f66\u5e94\u7528\u7684H2<\/sub>-\u7a7a\u6c14\u7535\u6c60\uff0c\u800c\u4e0d\u662f\u5728H2<\/sub>-O2<\/sub>\u6761\u4ef6\u4e0b\u8fdb\u884c\u7535\u6c60\u6027\u80fd\u6d4b\u8bd5\uff0c\u907f\u514d\u4e86\u6c27\u6c14\u53ef\u80fd\u5f15\u8d77\u7684\u6d53\u5dee\u6781\u5316\uff0c\u5728\u5b9e\u9645\u5e94\u7528\u4e2d\u6709\u91cd\u8981\u610f\u4e49\u3002<\/p>\n \u8fd1\u5e74\u6765\u5355\u539f\u5b50\u50ac\u5316\u5242\u4e5f\u662f\u4e00\u4e2a\u7814\u7a76\u70ed\u70b9\uff0c\u672c\u6587\u53ef\u89c6\u5316\u5730\u8bc1\u660e\u4e86\u5355\u539f\u5b50\u7684\u5b58\u5728\u53ca\u5176\u4e0e\u5468\u56f4\u539f\u5b50\u7684\u8fde\u63a5\u65b9\u5f0f\uff0c\u4ece\u539f\u5b50\u7ea7\u5256\u6790\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\uff0c\u6784\u6548\u5173\u7cfb\u6e05\u6670\u660e\u4e86\uff0c\u5728\u5355\u539f\u5b50\u50ac\u5316\u9886\u57df\u6709\u5f88\u91cd\u8981\u7684\u53c2\u8003\u610f\u4e49\u3002<\/p>\n \u4e8c\u3001A highly active and stable IrOx\/SrIrO3<\/sub>\u00a0catalyst for the oxygen evolution reaction2<\/sup><\/strong><\/p>\n \u5927\u91cf\u8d35\u91d1\u5c5e\u548c\u975e\u8d35\u91d1\u5c5e\u50ac\u5316\u5242\u5728\u78b1\u6027\u7535\u89e3\u6db2\u4e2d\u5bf9\u6790\u6c27\u53cd\u5e94\u6709\u9ad8\u50ac\u5316\u6d3b\u6027\u548c\u7a33\u5b9a\u6027\uff0c\u4f46\u662f\u53ea\u6709IrOx\u548cRuOx\u662f\u76ee\u524d\u552f\u4e00\u80fd\u591f\u5728\u9178\u6027\u7535\u89e3\u6db2\u4e2d\u8fbe\u5230~5 mA \/ cm2<\/sup>\u65f6\u8fc7\u7535\u4f4d\u5c0f\u4e8e750 mV\u7684\u6750\u6599\uff0c\u672c\u6587\u901a\u8fc7\u8109\u51b2\u6fc0\u5149\u6c89\u79ef\u6cd5\u5236\u5907\u4e86\u80fd\u591f\u5728\u9178\u6027\u7535\u89e3\u6db2\u4e2d\u540c\u65f6\u5177\u6709\u9ad8\u50ac\u5316\u6d3b\u6027\u53ca\u7a33\u5b9a\u6027\u7684IrOx\/SrIrO3<\/sub>\uff0c\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0c\u5728IrO3<\/sub>\u6216\u9510\u949b\u77ffIrO2<\/sub>\u57fa\u5e8f\u7684\u9536\u6d78\u51fa\u8fc7\u7a0b\u4e2d\u5f62\u6210\u4e86\u9ad8\u6d3b\u6027\u7684\u8868\u9762\u5c42\uff0c\u4f7f\u5176\u5728\u9178\u6027\u7535\u89e3\u8d28\u4e2d\u5177\u6709\u53ef\u89c2\u6d3b\u6027\u5e76\u4f18\u4e8eIrOx\u548cRuOx\u4f53\u7cfb\u3002<\/p>\n \u4e09\u3001Nanostructured transition metal dichalcogenide electrocatalysts for CO2<\/sub>\u00a0reduction in ionic liquid3<\/sup><\/strong><\/p>\n \u5c06\u4e8c\u6c27\u5316\u78b3\u8f6c\u5316\u4e3a\u71c3\u6599\u662f\u89e3\u51b3\u8bb8\u591a\u80fd\u6e90\u548c\u73af\u5883\u95ee\u9898\u7684\u4e00\u79cd\u7406\u60f3\u65b9\u6848\uff0c\u7136\u800c\uff0cCO2<\/sub>\u7684\u5316\u5b66\u60f0\u6027\u4f7f\u8bb8\u591a\u7535\u5316\u5b66\u548c\u5149\u5316\u5b66\u8f6c\u5316\u8fc7\u7a0b\u6548\u7387\u4f4e\u4e0b\u3002\u672c\u6587\u4ecb\u7ecd\u4e86\u8fc7\u6e21\u91d1\u5c5e\u4e8c\u786b\u5316\u7269\uff08TMDC\uff09\u7684\u4e8c\u7ef4\u7eb3\u7c73\u8584\u7247\u50ac\u5316\u5242\uff0c\u540c\u65f6\u5e94\u7528\u79bb\u5b50\u6db2\u4f53\u4f5c\u4e3a\u53cd\u5e94\u4ecb\u8d28\u63d0\u9ad8CO2<\/sub>\u8f6c\u5316\u6548\u7387\uff1aEMIM+<\/sup>\u79bb\u5b50\u6709\u52a9\u4e8e\u5728\u9178\u6027\u6761\u4ef6\u4e0b\u901a\u8fc7\u7edc\u5408\u5c06CO2<\/sub>\u8f93\u9001\u5230\u50ac\u5316\u5242\u8868\u9762\uff0c\u589e\u5f3a\u4e86\u5c40\u90e8CO2<\/sub>\u6d53\u5ea6\u3002<\/p>\n \u4e8c\u7ef4\u8d85\u8584\u7eb3\u7c73\u7247\u7ed3\u6784\u6750\u6599\u5728\u50ac\u5316\u9886\u57df\u7684\u5e94\u7528\u53ca\u5176\u5e7f\u6cdb\uff0c\u9ad8\u6bd4\u8868\u9762\u79ef\u3001\u5927\u91cf\u66b4\u9732\u7684\u6d3b\u6027\u4f4d\u70b9\u3001\u65e0\u5806\u53e0\u7684\u7ed3\u6784\u7279\u70b9\u4f7f\u5176\u5177\u6709\u5929\u7136\u7684\u50ac\u5316\u4f18\u52bf\uff0c\u79bb\u5b50\u6db2\u4f53\u80fd\u591f\u63d0\u9ad8\u53cd\u5e94\u7269\u7684\u5c40\u90e8\u6d53\u5ea6\u4e5f\u5f15\u8d77\u4e86\u7535\u50ac\u5316\u9886\u57df\u7814\u7a76\u4eba\u5458\u7684\u5e7f\u6cdb\u5173\u6ce8\uff0c\u4e2a\u4eba\u89c9\u5f97\u5728\u7535\u50ac\u5316\u9886\u57df\u878d\u5408\u8fd9\u4e24\u70b9\u80fd\u591f\u63d0\u9ad8\u5de5\u4f5c\u7684\u521b\u65b0\u6027\u3002<\/p>\n \u56db\u3001Selective increase in CO2<\/sub>\u00a0electroreduction activity at grain-boundary surface terminations4<\/sup><\/strong><\/p>\n \u91d1\u5c5e\u4e2d\u7684\u672c\u5f81\u7f3a\u9677\uff08\u4f8b\u5982\u6676\u754c\uff09\u80fd\u591f\u5728\u5176\u8868\u9762\u4ea7\u751f\u589e\u52a0\u5e94\u53d8\u7684\u533a\u57df\uff0c\u8fd9\u53ef\u80fd\u5f71\u54cd\u5176\u50ac\u5316\u6d3b\u6027\u3002\u63d0\u9ad8\u6750\u6599\u7684\u50ac\u5316\u6027\u80fd\u9700\u8981\u8bc6\u522b\u4ea7\u751f\u6d3b\u6027\u8868\u9762\u7684\u7ed3\u6784\u7279\u5f81\uff0c\u5728\u591a\u6676\u6750\u6599\u4e2d\u6676\u754c\u901a\u8fc7\u7a33\u5b9a\u4f4d\u9519\u4ea7\u751f\u5e94\u53d8\u533a\u57df\uff0c\u5e76\u4e14\u53ef\u4ee5\u4ea7\u751f\u7528\u4e8e\u52a8\u529b\u5b66\u6355\u83b7\u7684\u50ac\u5316\u7684\u9ad8\u80fd\u8868\u9762\u3002\u5c3d\u7ba1\u5148\u524d\u7814\u7a76\u63d0\u51fa\u6676\u754c\u5bc6\u5ea6\u4e0e\u67d0\u4e9b\u53cd\u5e94\u7684\u50ac\u5316\u6d3b\u6027\u76f8\u5173\uff0c\u4f46\u7f3a\u4e4f\u6676\u754c\u4ea7\u751f\u5177\u6709\u589e\u5f3a\u6d3b\u6027\u7684\u8868\u9762\u7684\u76f4\u63a5\u8bc1\u636e\u3002<\/p>\n \u65af\u5766\u798f\u5927\u5b66\u7684Matthew W. Kanan\u6559\u6388\u901a\u8fc7\u5bf9\u591a\u6676\u91d1\u8584\u819c\u8fdb\u884c\u9000\u706b\u4ee5\u4ea7\u751f\u66f4\u5927\u7684\u6676\u7c92\uff0c\u6539\u53d8\u8868\u9762\u5904\u6676\u754c\u7684\u7c7b\u578b\u548c\u5206\u5e03\u3002\u5927\u91cf\u7535\u5316\u5b66\u6d4b\u91cf\u548c\u4e9a\u5fae\u7c73\u5206\u8fa8\u7387\u7684\u626b\u63cf\u7535\u5316\u5b66\u7535\u6c60\u663e\u5fae\u955c\u6570\u636e\u8bc1\u660e\u4e86\u91d1\u7535\u6781\u4e2d\u7684\u6676\u754c\u8868\u9762\u6bd4\u6676\u7c92\u8868\u9762\u5bf9\u7535\u8fd8\u539f\u4e8c\u6c27\u5316\u78b3\u6210\u4e00\u6c27\u5316\u78b3\u50ac\u5316\u6d3b\u6027\u66f4\u5f3a\u3002\u4f4d\u9519\u5bc6\u5ea6\u4e0eCO2<\/sub>\u7535\u8fd8\u539f\u6d3b\u6027\u76f8\u5173\uff0c\u4f46\u8fd9\u79cd\u7f3a\u9677\u5bf9\u5176\u7ade\u4e89\u53cd\u5e94HER\u6ca1\u6709\u5f71\u54cd\u3002<\/p>\n \u6676\u754c\u7684\u50ac\u5316\u6548\u679c\u4e0e\u5176\u4f4d\u9519\u8bf1\u5bfc\u7684\u5e94\u53d8\u573a\u76f8\u5173\uff0c\u672c\u6587\u4e3a\u591a\u76f8\u50ac\u5316\u4e2d\u5229\u7528\u6676\u754c\u6548\u5e94\u63d0\u4f9b\u4e86\u91cd\u8981\u7684\u4f9d\u636e\u548c\u601d\u8def\u3002<\/p>\n \u4e94\u3001CO2<\/sub>\u00a0electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface5<\/sup><\/strong><\/p>\n \u4e59\u70ef\u662f\u5851\u6599\u7684\u91cd\u8981\u539f\u6599\uff0c\u662f\u4e8c\u6c27\u5316\u78b3\u7535\u8fd8\u539f\u53ef\u4ee5\u5176\u539f\u6599\u6765\u6e90\u4e4b\u4e00\u3002\u4f46\u662f\u76ee\u524d\u5728\u6240\u9700\u7684\u78b1\u6027\u53cd\u5e94\u6761\u4ef6\u4e0b\u7528\u4e8e\u8be5\u8f6c\u5316\u7684\u94dc\u7535\u50ac\u5316\u5242\u7684\u6027\u80fd\u53d7\u5230CO2<\/sub>\u4e0e\u78b1\u751f\u6210\u78b3\u9178\u6c22\u76d0\u7684\u7ade\u4e89\u53cd\u5e94\u7684\u963b\u788d\u3002\u591a\u4f26\u591a\u5927\u5b66\u7684Edward H. Sargent\u6559\u6388\u8bbe\u8ba1\u4e86\u4e00\u79cd\u80fd\u591f\u901a\u8fc7\u4f18\u5316CO2<\/sub>\u6269\u6563\u5230\u50ac\u5316\u4f4d\u70b9\u6765\u8010\u53d7\u78b1\u7684\u7535\u6781\u3002\u4ed6\u4eec\u8ba4\u4e3a\u6c89\u79ef\u5728\u6c14\u4f53\u6269\u6563\u5c42\u4e0a\u7684\u50ac\u5316\u5242\u5728\u7535\u6c60\u4e2d\u80fd\u663e\u8457\u589e\u52a0CO2<\/sub>\u7684\u5c40\u90e8\u6d53\u5ea6\uff0c\u94dc\u8868\u9762\u6216\u9644\u8fd1\u7684\u6c22\u6c27\u5316\u7269\u79bb\u5b50\u964d\u4f4e\u4e86CO2<\/sub>\u8fd8\u539f\u548c\u4e00\u6c27\u5316\u78b3-CO\u5076\u8054\u6d3b\u5316\u80fd\u5792\uff0c\u5f15\u5165\u57fa\u4e8e\u805a\u5408\u7269\u7684\u6c14\u4f53\u6269\u6563\u5c42\u589e\u5f3a\u4e86\u64cd\u4f5c\u7a33\u5b9a\u6027\uff0c\u6240\u8ff0\u6c14\u4f53\u6269\u6563\u5c42\u5c06\u53cd\u5e94\u754c\u9762\u5939\u5728\u5355\u72ec\u7684\u758f\u6c34\u6027\u548c\u5bfc\u7535\u6027\u8f7d\u4f53\u4e4b\u95f4\uff0c\u5728\u957f\u65f6\u95f4\u7684\u7535\u89e3\u4e2d\u4fdd\u8bc1\u6052\u5b9a\u9ad8\u6548\u7684\u4e59\u70ef\u9009\u62e9\u6027\u3002<\/p>\n \u867d\u7136\u7535\u50ac\u5316\u4e2d\u50ac\u5316\u5242\u662f\u6838\u5fc3\uff0c\u4f46\u662f\u6539\u5584\u6c14\u4f53\u6269\u6563\u5c42\u3001\u589e\u52a0\u50ac\u5316\u5242\u5468\u56f4\u53cd\u5e94\u7269\u7684\u6d53\u5ea6\u80fd\u591f\u8d77\u5230\u5982\u864e\u6dfb\u7ffc\u7684\u4f5c\u7528\uff0c\u4e0a\u9762\u4e24\u7bc7\u5173\u4e8e\u7535\u8fd8\u539fCO2<\/sub>\u7684\u5de5\u4f5c\u90fd\u7ed9\u4e88\u4e86\u6211\u4eec\u8fd9\u4e2a\u65b9\u9762\u6781\u5927\u7684\u542f\u53d1\u3002<\/p>\n \u516d\u3001Self-assembly of noble metal monolayers on transition metal carbide nanoparticle catalysts6<\/sup><\/strong><\/p>\n \u5c06\u8d35\u91d1\u5c5e\u4fee\u9970\u5728\u50a8\u91cf\u4e30\u5bcc\u7684\u8fc7\u6e21\u91d1\u5c5e\u6838\u8868\u9762\u662f\u63d0\u9ad8\u8d35\u91d1\u5c5e\u50ac\u5316\u5242\u6d3b\u6027\u3001\u964d\u4f4e\u6210\u672c\u7684\u4e00\u79cd\u65b9\u6cd5\uff0c\u4f46\u8fd9\u4e9b\u7ed3\u6784\u5728\u53cd\u5e94\u8fc7\u7a0b\u4e2d\u901a\u5e38\u4f1a\u53d1\u751f\u5408\u91d1\u5316\u6216\u5931\u6d3b\u3002\u672c\u6587\u901a\u8fc7\u5c06\u6e17\u78b3\u8d35\u91d1\u5c5e\u76d0\u548c\u8fc7\u6e21\u91d1\u5c5e\u6c27\u5316\u7269\u7684\u6df7\u5408\u7269\u6e17\u900f\u5728\u4e8c\u6c27\u5316\u7845\u6a21\u677f\u4e2d\uff0c\u5b9e\u73b0\u4e86\u8868\u9762\u6d82\u6709\u539f\u5b50\u7ea7\u7684\u5355\u5c42\u8d35\u91d1\u5c5e\u58f3\u7684\u8fc7\u6e21\u91d1\u5c5e\u78b3\u5316\u7269\u7eb3\u7c73\u7c92\u5b50\u7684\u81ea\u7ec4\u88c5\u3002\u6750\u6599\u5bf9\u7532\u9187\u7535\u6c27\u5316\u5177\u6709\u9ad8\u6d3b\u6027\uff0c\u8868\u73b0\u51fa\u5f3a\u7684\u6297\u70e7\u7ed3\u548cCO\u4e2d\u6bd2\u6027\uff0c\u7a33\u5b9a\u8d85\u5f3a\u3002<\/p>\n \u6587\u4e2d\u4e3a\u964d\u4f4e\u8d35\u91d1\u5c5e\u8d1f\u8f7d\u91cf\uff0c\u589e\u5f3a\u6d3b\u6027\u548c\u63d0\u9ad8\u7a33\u5b9a\u6027\u63d0\u4f9b\u4e86\u65b0\u7684\u65b9\u5411\uff0c\u4e3a\u540e\u6765\u4e00\u7cfb\u5217\u6838-\u58f3\u7ed3\u6784\u50ac\u5316\u5242\u7684\u53d1\u5c55\u6709\u5f15\u9886\u4f5c\u7528\u3002<\/p>\n \u4e03\u3001Combining theory and experiment in electrocatalysis: Insights into materials design7<\/sup><\/strong><\/p>\n \u8be5\u7efc\u8ff0\u8ba8\u8bba\u4e86\u6700\u65b0\u7684\u975e\u5747\u76f8\u7535\u50ac\u5316\u5242\u548c\u76f8\u5173\u6750\u6599\u7684\u8bbe\u8ba1\u7b56\u7565\uff0c\u5f3a\u8c03\u4e86\u4f9d\u9760\u7406\u8bba\u8ba1\u7b97\u7ed3\u679c\u5408\u7406\u8bbe\u8ba1\u50ac\u5316\u5242\u6027\u80fd\u7684\u91cd\u8981\u6027\uff0c\u901a\u8fc7\u7814\u7a76\u4e0d\u540c\u7684\u50ac\u5316\u4f53\u7cfb\uff0c\u4f8b\u5982\u6c27\u8fd8\u539f\u3001\u6c2e\u8fd8\u539f\u3001\u6790\u6c22\u3001\u6790\u6c27\u7b49\u53cd\u5e94\uff0c\u63a2\u7a76\u5176\u50ac\u5316\u4f5c\u7528\u7684\u5171\u540c\u539f\u7406\uff0c\u6307\u51fa\u4e86\u5384\u5f85\u89e3\u51b3\u7684\u5173\u952e\u95ee\u9898\uff0c\u7cfb\u7edf\u5730\u603b\u7ed3\u4e86\u8fd9\u4e9b\u50ac\u5316\u53cd\u5e94\u7684\u53d1\u5c55\u8d8b\u52bf\uff0c\u4e3a\u65b0\u50ac\u5316\u5242\u7684\u5f00\u53d1\u6307\u660e\u65b9\u5411\u3002\u4e2a\u4eba\u89c9\u5f97\u8fd9\u7bc7\u6587\u7ae0\u662f\u6750\u6599\u8bbe\u8ba1\u4e0e\u5236\u5907\u9636\u6bb5\u5fc5\u8bfb\u7684\u7ecf\u5178\u6587\u732e\uff0c\u6bcf\u8bfb\u4e00\u904d\u5fc5\u6709\u65b0\u7684\u6536\u83b7\u3002<\/p>\n \u516b\u3001Direct and continuous strain control of catalysts with tunable battery electrode materials8<\/sup><\/strong><\/p>\n \u6539\u53d8\u7535\u5b50\u7ed3\u6784\u53ef\u4ee5\u6539\u53d8\u975e\u5747\u76f8\u50ac\u5316\u5242\u4e2d\u91d1\u5c5e\u7684\u50ac\u5316\u6d3b\u6027\uff0c\u6676\u683c\u5e94\u53d8\uff08\u538b\u7f29\u6216\u62c9\u4f38\uff09\u53ef\u4ee5\u901a\u8fc7\u6539\u53d8\u8868\u9762\u539f\u5b50\u4e4b\u95f4\u7684\u8ddd\u79bb\u6765\u6539\u53d8\u8868\u9762\u7535\u5b50\u7ed3\u6784\u4ee5\u53ca\u50ac\u5316\u6d3b\u6027\u3002\u6539\u53d8\u9499\u949b\u77ff\u6c27\u5316\u7269\u4e2d\u7684d\u5e26\u586b\u5145\u3001\u8fc7\u6e21\u91d1\u5c5e\u5408\u91d1\u5316\u3001\u5728\u5c42\u72b6\u6750\u6599\u4e2d\u4f7f\u7528\u9502\u5d4c\u5165\u7b49\u90fd\u5c5e\u4e8e\u6b64\u8303\u56f4\u3002\u672c\u6587\u901a\u8fc7\u7535\u6c60\u7535\u6781\u7684\u5145\u7535\u548c\u653e\u7535\u72b6\u6001\u4e4b\u95f4\u7684\u7535\u5316\u5b66\u8f6c\u6362\uff0c\u7cbe\u786e\u5730\u63a7\u5236\u4f53\u79ef\u7684\u53d8\u5316\u4ee5\u5728\u8d1f\u8f7d\u7684\u50ac\u5316\u5242\u4e0a\u5f15\u8d77\u538b\u7f29\u6216\u62c9\u4f38\u5e94\u53d8\u3002\u50cf\u5dee\u6821\u6b63\u7684\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c\u53ef\u89c6\u5316\u5730\u663e\u793a\u4e86\u9502\u7535\u6c60\u6b63\u6781\u7684\u6c27\u5316\u94b4\u9897\u7c92\u5982\u4f55\u968f\u7740\u5145\u7535\u800c\u81a8\u80c0\u6216\u6536\u7f29\uff0c\u5e76\u5c06\u5e94\u53d8\u8f6c\u79fb\u5230\u5438\u9644\u7684\u94c2\u7eb3\u7c73\u9897\u7c92\u4e0a\uff0c\u8bf1\u5bfc\u6676\u683c\u538b\u7f29\u6216\u8005\u4ea7\u751f\u5f20\u529b\u3002\u5bf9\u4e8eORR\uff0c\u538b\u7f29\u5e94\u53d8\u63d0\u9ad8\u4e8690\uff05\u7684\u6d3b\u6027\uff0c\u62c9\u4f38\u5e94\u53d8\u4f7f\u5176\u964d\u4f4e\u4e8640\uff05\uff0c\u4e0e\u7406\u8bba\u9884\u6d4b\u4e00\u81f4\u3002<\/p>\n \u4e5d\u3001Tunable intrinsic strain in two-dimensional transition metal electrocatalysts9<\/sup><\/strong><\/p>\n \u4ece\u4e0a\u7bc7\u5de5\u4f5c\u4e2d\u6211\u4eec\u5df2\u7ecf\u4e86\u89e3\u5230\u5e94\u53d8\u53ef\u4ee5\u6539\u53d8\u91d1\u5c5e\u7684\u7535\u5b50\u7279\u6027\uff0c\u5e76\u4e14\u80fd\u589e\u5f3a\u7535\u50ac\u5316\u6d3b\u6027\u3002\u5b9e\u9645\u50ac\u5316\u5242\u9700\u8981\u5177\u6709\u9ad8\u8868\u9762\u79ef\u7684\u7eb3\u7c73\u6750\u6599\uff0c\u7136\u800c\u5bf9\u4e8e\u7eb3\u7c73\u9897\u7c92\uff0c\u901a\u5e38\u7528\u8986\u76d6\u5c42\uff08\u5438\u9644\u7269\u6216\u6742\u539f\u5b50\uff09\u8bf1\u5bfc\u5e94\u53d8\uff0c\u6240\u8ff0\u8986\u76d6\u7269\u53ef\u5728\u64cd\u4f5c\u671f\u95f4\u7ecf\u5386\u91cd\u5efa\u4ee5\u91ca\u653e\u8bf1\u5bfc\u7684\u5e94\u53d8\u3002\u4f20\u7edf\u4e0a\uff0c\u8868\u9762\u5e94\u53d8\u662f\u7531\u6765\u81ea\u5f02\u8d28\u57fa\u5e95\u7684\u5916\u90e8\u5e94\u529b\u65bd\u52a0\u7684\uff0c\u4f46\u662f\u8fd9\u79cd\u6548\u5e94\u901a\u5e38\u56e0\u4e3a\u754c\u9762\u91cd\u5efa\u548c\u7eb3\u7c73\u50ac\u5316\u5242\u51e0\u4f55\u5f62\u72b6\u800c\u53d8\u5f97\u6a21\u7cca\u3002Chao Wang\u6559\u6388\u7b49\u4eba\u53d1\u73b0\u5229\u7528\u4e8c\u7ef4\u8fc7\u6e21\u91d1\u5c5e\u7eb3\u7c73\u7247\u4e2d\u7684\u56fa\u6709\u8868\u9762\u5e94\u529b\u53ef\u4ee5\u89e3\u51b3\u8fd9\u4e9b\u95ee\u9898\uff0c\u4e0e\u7eb3\u7c73\u9897\u7c92\u76f8\u6bd4\uff0c\u8fd9\u4e9b\u4e8c\u7ef4\u7eb3\u7c73\u7ed3\u6784\u4e0d\u5305\u542b\u50ac\u5316\u5242-\u57fa\u5e95\u754c\u9762\uff0c\u5176\u5c06\u5355\u6676\u50ac\u5316\u5242\u7684\u9ad8\u6bd4\u6d3b\u6027\u4e0e\u4f20\u7edf\u7eb3\u7c73\u9897\u7c92\u7684\u9ad8\u8868\u9762\u79ef\u7ed3\u5408\u5728\u4e00\u8d77\u3002\u4ed6\u4eec\u5229\u7528\u8868\u9762\u5e94\u529b\u9a71\u52a8\u72ec\u7acb\u91d1\u5c5e\u7eb3\u7c73\u7247\u4e2d\u7684\u5185\u5728\u5e94\u53d8\u3002\u5408\u6210\u5177\u6709\u539f\u5b50\u7ea7\u63a7\u5236\u539a\u5ea6\u7684\u8d85\u8584Pd\u7eb3\u7c73\u7247\u72ec\u7acb\u7684\u94af\u7eb3\u7c73\u7247\u5fae\u8c03\u5185\u5728\u5e94\u53d8\u4ee5\u4f18\u5316\u50ac\u5316\u53cd\u5e94\u6027\u3002<\/p>\n \u5341\u3001Ultralow-loading platinum-cobalt fuel cell catalysts derived from imidazolate frameworks10<\/sup><\/strong><\/p>\n \u5c3d\u53ef\u80fd\u964d\u4f4e\u94c2\u5728\u50ac\u5316\u5242\u4e2d\u7684\u8f7d\u91cf\u5e76\u5b9e\u73b0\u9ad8\u50ac\u5316\u6027\u80fd\u5bf9\u4e8e\u964d\u4f4e\u71c3\u6599\u7535\u6c60\u6210\u672c\u81f3\u5173\u91cd\u8981\u3002\u672c\u6587\u4f7f\u7528\u94b4\u6216\u53cc\u91d1\u5c5e\u94b4\u3001\u950c\u6cb8\u77f3\u54aa\u5511\u916f\u9aa8\u67b6\u4f5c\u4e3a\u524d\u9a71\u4f53\u5236\u5907\u542b\u6709\u8d85\u4f4e\u94c2\u8d1f\u8f7d\u91cf\u7684\u9ad8\u6d3b\u6027\u7a33\u5b9a\u7535\u50ac\u5316\u5242\u3002\u5728\u4e0d\u542b\u94c2\u65cf\u91d1\u5c5e\uff08PGM\uff09\u7684\u50ac\u5316\u57fa\u6750\u4e0a\uff0c\u5b58\u5728\u5e94\u53d8\u7684\u94c2-\u94b4\u6838-\u58f3\u7eb3\u7c73\u7c92\u5b50\u4e4b\u95f4\u5b58\u5728\u534f\u540c\u50ac\u5316\u4f5c\u7528\u3002Pt-Co\u5408\u91d1\u4e0d\u4ec5\u76f4\u63a5\u63d0\u9ad8ORR\u50ac\u5316\u6d3b\u6027\uff0c\u8fd8\u51cf\u5c11\u4e86\u9644\u8fd1\u65e0PGM\u4f4d\u70b9\u4ea7\u751f\u7684H2<\/sub>O2<\/sub>\uff0c\u4f7fORR\u53d1\u751f\u8fd1\u56db\u7535\u5b50\u8f6c\u79fb\u63d0\u9ad8\u71c3\u6599\u7535\u6c60\u6027\u80fd\u3002\u56e0\u4e3aH2<\/sub>O2<\/sub>\u4f1a\u8150\u8680\u57fa\u4e8eTM\u7684\u65e0PGM\u4f4d\u70b9\u548c\u591a\u5b54\u78b3\u57fa\u8d28\uff0c\u56e0\u6b64\u5176\u5206\u89e3\u4e5f\u6709\u52a9\u4e8e\u4fdd\u6301\u50ac\u5316\u5242\u7684\u5b8c\u6574\u6027\u548c\u8010\u4e45\u6027\u3002<\/p>\n \u53c2\u8003\u6587\u732e\uff1a<\/strong><\/p>\n 1.Chung, H. T.; Cullen, D. A.; Higgins, D.; Sneed, B. T.; Holby, E. F.; More, K. L.; Zelenay, P., Direct atomic-level insight into the active sites of a high-performance PGM-free ORR catalyst. Science <\/i><\/em>2017,<\/b><\/strong>357<\/i><\/em>(6350), 479-484.<\/p>\n 2.Seitz, L. C.; Dickens, C. F.; Nishio, K.; Hikita, Y.; Montoya, J.; Doyle, A.; Kirk, C.; Vojvodic, A.; Hwang, H. Y.; Norskov, J. K.; Jaramillo, T. F., A highly active and stable IrOSrIrO3<\/sub>catalyst for the oxygen evolution reaction. Science <\/i><\/em>2016,<\/b><\/strong>353<\/i><\/em>\u00a0(6303), 1011-1014.<\/p>\n 3.Asadi, M.; Kim, K.; Liu, C.; Addepalli, A. V.; Abbasi, P.; Yasaei, P.; Phillips, P.; Behranginia, A.; Cerrato, J. M.; Haasch, R.; Zapol, P.; Kumar, B.; Klie, R. F.; Abiade, J.; Curtiss, L. A.; Salehi-Khojin, A., Nanostructured transition metal dichalcogenide electrocatalysts for CO2<\/sub>reduction in ionic liquid. Science <\/i><\/em>2016,<\/b><\/strong>353<\/i><\/em>\u00a0(6298), 467-470.<\/p>\n 4.Mariano, R. G.; McKelvey, K.; White, H. S.; Kanan, M. W., Selective increase in CO2<\/sub>electroreduction activity at grain-boundary surface terminations. Science <\/i><\/em>2017,<\/b><\/strong>358<\/i><\/em>\u00a0(6367), 1187-1192.<\/p>\n 5.Dinh, C.-T.; Burdyny, T.; Kibria, M. G.; Seifitokaldani, A.; Gabardo, C. M.; Garc\u00eda de Arquer, F. P.; Kiani, A.; Edwards, J. P.; De Luna, P.; Bushuyev, O. S.; Zou, C.; Quintero-Bermudez, R.; Pang, Y.; Sinton, D.; Sargent, E. H., CO2 <\/sub>electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface. Science <\/i><\/em>2018,<\/b><\/strong>360<\/i><\/em>(6390), 783-787.<\/p>\n 6.Hunt, S. T.; Milina, M.; Alba-Rubio, A. C.; Hendon, C. H.; Dumesic, J. A.; Rom\u00e1n-Leshkov, Y., Self-assembly of noble metal monolayers on transition metal carbide nanoparticle catalysts. Science <\/i><\/em>2016,<\/b><\/strong>352<\/i><\/em>(6288), 974-978.<\/p>\n 7.Zhi Wei Seh, J. K., Colin F. Dickens, Ib Chorkendorff,; Jens K. N\u00f8rskov, T. F. J., Combining theory and experiment in electrocatalysis \u00a0Insights into materials design. science <\/i><\/em>2017,<\/b><\/strong>355<\/i><\/em>(146).<\/p>\n 8.Wang, H.; Xu, S.; Tsai, C.; Li, Y.; Liu, C.; Zhao, J.; Liu, Y.; Yuan, H.; Abild-Pedersen, F.; Prinz, F. B.; N\u00f8rskov, J. K.; Cui, Y., Direct and continuous strain control of catalysts with tunable battery electrode materials. Science <\/i><\/em>2016,<\/b><\/strong>354<\/i><\/em>(6315), 1031-1036.<\/p>\n 9.Wang, L.; Zeng, Z.; Gao, W.; Maxson, T.; Raciti, D.; Giroux, M.; Pan, X.; Wang, C.; Greeley, J., Tunable intrinsic strain in two-dimensional transition metal electrocatalysts. Science <\/i><\/em>2019,<\/b><\/strong>363<\/i><\/em>(6429), 870-874.<\/p>\n 10.Chong, L.; Wen, J.; Kubal, J.; Sen, F. G.; Zou, J.; Greeley, J.; Chan, M.; Barkholtz, H.; Ding, W.; Liu, D.-J., Ultralow-loading platinum-cobalt fuel cell catalysts derived from imidazolate frameworks. Science <\/i><\/em>2018,<\/b><\/strong>362<\/i><\/em>(6420), 1276-1281.<\/p>\n \u5f80\u671f\u56de\u987e\uff1a<\/strong><\/p>\n \u7535\u50ac\u5316\u65b0\u5ba0\u4e4b\u5e38\u6e29\u5e38\u538b\u6c2e\u8fd8\u539f\uff08NRR\uff09\uff0c\u6700\u5168NRR\u4ecb\u7ecd\uff0c\u4f60\u60f3\u8981\u7684\u90fd\u5728\u8fd9\uff01<\/a><\/p>\n \u8ba4\u8bc6\u8fd9\u4e9b\u5e26\u4f60\u8f7b\u677e\u4e0a\u738b\u8005\u2014\u2014\u7535\u50ac\u5316\u4ea7\u6c27\uff08OER\uff09\u6d4b\u8bd5\u624b\u6bb5\u89e3\u6790<\/a><\/p>\n \u4f60\u771f\u7684\u4e86\u89e3\u7535\u50ac\u5316\u4ea7\u6c22\u8fd9\u4e9b\u77e5\u8bc6\u5417\uff1f\u5df2\u4e3a\u4f60\u603b\u7ed3\u597d\uff0c\u5feb\u6233\uff01<\/a><\/p>\n
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