{"id":171207,"date":"2019-03-29T06:30:00","date_gmt":"2019-03-28T22:30:00","guid":{"rendered":"\/\/m.iemloyee.com\/?p=171207"},"modified":"2019-03-28T18:22:42","modified_gmt":"2019-03-28T10:22:42","slug":"%e6%b8%85%e5%8d%8e%e5%a4%a7%e5%ad%a6%e5%90%95%e7%91%9e%e6%b6%9bmater-today%e7%bb%bc%e8%bf%b0%ef%bc%9a%e6%b0%ae%e8%bf%98%e5%8e%9f%e5%8f%8d%e5%ba%94%ef%bc%88nrr%ef%bc%89%e5%82%ac%e5%8c%96%e6%9d%90","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=171207","title":{"rendered":"\u6e05\u534e\u5927\u5b66\u5415\u745e\u6d9bMater. Today\u7efc\u8ff0\uff1a\u6c2e\u8fd8\u539f\u53cd\u5e94\uff08NRR\uff09\u50ac\u5316\u6750\u6599\u7814\u7a76\u8fdb\u5c55"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/b><\/strong><\/p>\n

\u6c28\u662f\u4e00\u79cd\u91cd\u8981\u7684\u5316\u5de5\u539f\u6599\uff0c\u5728\u5de5\u3001\u519c\u4e1a\u751f\u4ea7\u548c\u80fd\u6e90\u50a8\u5b58\u8f6c\u6362\u7b49\u9886\u57df\u53d1\u6325\u7740\u91cd\u8981\u4f5c\u7528\u3002\u76ee\u524d\uff0c\u5de5\u4e1a\u4e0a\u5408\u6210\u6c28\u4e3b\u8981\u4f9d\u8d56\u4e8e\u4f20\u7edf\u7684Haber-Bosch\u5de5\u827a\uff0c\u7531\u4e8e\u8be5\u6280\u672f\u9700\u8981\u5728\u9ad8\u6e29\u9ad8\u538b\u4e0b\u8fdb\u884c\uff08300~500\u00a0\u2103\u3001150~200\u00a0atm\uff09\uff0c\u4e0d\u4ec5\u80fd\u8017\u5de8\u5927\u800c\u4e14\u6392\u653e\u5927\u91cf\u7684\u6e29\u5ba4\u6c14\u4f53\u3002\u56e0\u6b64\uff0c\u5728\u80fd\u6e90\u5371\u673a\u548c\u73af\u5883\u95ee\u9898\u65e5\u76ca\u51f8\u663e\u7684\u60c5\u5f62\u4e0b\uff0c\u4e9f\u5f85\u5f00\u53d1\u5728\u6e29\u548c\u6761\u4ef6\u4e0b\u9ad8\u6548\u5408\u6210\u6c28\u7684\u65b0\u5de5\u827a\u3002<\/p>\n

\u76f8\u6bd4Haber-Bosch\u6cd5\uff0c\u7535\u50ac\u5316\u6c2e\u8fd8\u539f\u4ea7\u6c28\u7406\u8bba\u4e0a\u53ef\u5728\u5e38\u6e29\u5e38\u538b\u4e0b\u8fdb\u884c\uff0c\u5e76\u4e14\u539f\u6599\u6c34\u548c\u6c2e\u6c14\u6765\u6e90\u5e7f\u6cdb\uff0c\u8fd9\u4e3a\u5728\u6e29\u548c\u6761\u4ef6\u4e0b\u5b9e\u73b0\u6c28\u7684\u7eff\u8272\u5408\u6210\u5e26\u6765\u4e86\u5951\u673a\u3002\u8fd1\u5e74\u6765\uff0c\u7535\u50ac\u5316\u6c2e\u8fd8\u539f\u4ea7\u6c28\u5f15\u8d77\u4e86\u4eba\u4eec\u7684\u9ad8\u5ea6\u5173\u6ce8\uff0c\u76f8\u5173\u7684\u7814\u7a76\u62a5\u9053\u5448\u73b0\u8fc5\u901f\u589e\u957f\u4e4b\u52bf\u3002\u7136\u800c\u76ee\u524d\u7684\u7814\u7a76\u8868\u660e\uff0c\u7535\u50ac\u5316\u6280\u672f\u867d\u7136\u53ef\u4ee5\u5b9e\u73b0\u6c28\u7684\u7eff\u8272\u5408\u6210\uff0c\u4f46\u5728\u5e38\u6e29\u5e38\u538b\u4e0b\uff0c\u7531\u4e8eN\u2261N\u4e09\u952e\u7a33\u5b9a\u6027\u6781\u9ad8\u4e14\u6c2e\u6c14\u7684\u5438\u9644\u7f13\u6162\uff0c\u7535\u50ac\u5316\u6c2e\u8fd8\u539f\u4ea7\u6c28\u5728\u70ed\u529b\u5b66\u548c\u52a8\u529b\u5b66\u4e0a\u90fd\u5b58\u5728\u5de8\u5927\u7684\u963b\u788d\uff0c\u5e76\u4e14\u7531\u4e8e\u6790\u6c22\u7ade\u4e89\u53cd\u5e94\u7684\u5b58\u5728\uff0c\u81f4\u4f7f\u6c2e\u6c14\u8fd8\u539f\u53cd\u5e94\u7684\u9009\u62e9\u6027\u548c\u4ea7\u6c28\u901f\u7387\u90fd\u5927\u5927\u964d\u4f4e\u3002\u56e0\u6b64\uff0c\u5982\u4f55\u63d0\u9ad8\u4ea7\u6c28\u901f\u7387\u7684\u540c\u65f6\u63d0\u5347\u50ac\u5316\u5242\u7684\u9009\u62e9\u6027\u662f\u5e38\u6e29\u5e38\u538b\u4e0b\u7535\u50ac\u5316\u6c2e\u8fd8\u539f\u7814\u7a76\u9762\u4e34\u7684\u6700\u5927\u6311\u6218\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u6e05\u534e\u5927\u5b66\u6750\u6599\u5b66\u9662\u5415\u745e\u6d9b\u7814\u7a76\u7ec4<\/b><\/strong>\u5728Materials Today<\/b><\/strong>\u4e0a\u5728\u7ebf\u53d1\u8868\u957f\u7bc7\u7efc\u8ff0\u6587\u7ae0\u201cHeterogeneous electrocatalysts design for nitrogen reduction reaction under ambient conditions<\/b><\/strong>\u201d<\/b><\/strong>\u3002\u8be5\u8bba\u6587\u7cfb\u7edf\u603b\u7ed3\u4e86\u8fd1\u51e0\u5e74\u5e38\u6e29\u5e38\u538b\u6c2e\u6c14\u8fd8\u539f\u5408\u6210\u6c28\u7684\u7814\u7a76\u8fdb\u5c55\u5e76\u6307\u51fa\u4e86\u8be5\u9886\u57df\u76ee\u524d\u9762\u4e34\u7684\u4e3b\u8981\u6311\u6218\uff0c\u63d0\u51fa\u901a\u8fc7\u5f02\u76f8\u50ac\u5316\u5242\u7684\u8bbe\u8ba1\u5bf9\u5176\u6027\u80fd\u8fdb\u884c\u8c03\u63a7\uff0c\u5b9e\u73b0\u6c2e\u6c14-\u6c28\u7684\u9ad8\u6548\u8f6c\u5316\u3002<\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/b><\/strong><\/p>\n

1.NRR\u53cd\u5e94\u673a\u5236<\/strong><\/p>\n

\u56fe1<\/p>\n

\"\"<\/p>\n

\u7535\u50ac\u5316\u6c2e\u8fd8\u539f\u4ea7\u6c28\u53cd\u5e94\u7684\uff08a\uff09\u53cd\u5e94\u8fc7\u7a0b\u793a\u610f\u56fe\uff08b-d\uff09\u4e3b\u8981\u53cd\u5e94\u673a\u5236<\/p>\n

2.NRR\u7535\u50ac\u5316\u5242\u7684\u8bbe\u8ba1\u7b56\u7565<\/strong><\/p>\n

2.1 \u6676\u9762\u8c03\u63a7<\/p>\n

\u5408\u7406\u8c03\u63a7\u50ac\u5316\u5242\u7684\u8868\u9762\u6676\u9762\uff0c\u53ef\u4ee5\u589e\u52a0\u50ac\u5316\u5242\u8868\u9762\u7684\u6d3b\u6027\u4f4d\u70b9\uff0c\u5f71\u54cd\u53cd\u5e94\u7269\u4e0e\u4e2d\u95f4\u4ea7\u7269\u5728\u50ac\u5316\u5242\u8868\u9762\u7684\u5438\u9644\u7279\u6027\uff0c\u4ece\u800c\u63d0\u5347\u5176\u50ac\u5316\u6027\u80fd\u3002<\/p>\n

\u56fe2.<\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u8d35\u91d1\u5c5eNRR\u50ac\u5316\u5242Au\u7eb3\u7c73\u68d2\u7684\u7ed3\u6784\u793a\u610f\u56fe\u548c{730}\u6676\u9762\u793a\u610f\u56fe\uff08b\uff09Au\u7eb3\u7c73\u68d2\u7684\u900f\u5c04\u7535\u955c\u56fe\uff08c\uff09Au\u7eb3\u7c73\u68d2\u7684\u7d2b\u5916\u53ef\u89c1\u5149\u8c31\u56fe\uff08d\uff09Au\u7eb3\u7c73\u68d2\u7684\u7403\u5dee\u900f\u5c04\u7535\u955c\u56fe<\/p>\n

2.2 \u5f62\u8c8c\u5c3a\u5bf8\u8c03\u63a7<\/p>\n

\u901a\u8fc7\u8c03\u63a7NRR\u7535\u50ac\u5316\u5242\u7684\u5c3a\u5bf8\uff0c\u53ef\u4ee5\u5728\u539f\u6709\u7684\u5bc6\u6392\u4f4d\u70b9\u4e0a\u521b\u9020\u51fa\u4f4e\u914d\u4f4d\u4f4d\u70b9\uff0c\u4ece\u800c\u5f71\u54cd\u53cd\u5e94\u4e2d\u95f4\u4ea7\u7269\u7684\u6210\u952e\u5f3a\u5ea6\uff0c\u56e0\u6b64\u5f71\u54cd\u50ac\u5316\u5242\u7684\u9009\u62e9\u6027\u548c\u6d3b\u6027\u3002\u901a\u8fc7\u5f62\u8c8c\u8c03\u63a7\u53ef\u4ee5\u8d4b\u4e88\u50ac\u5316\u5242\u5927\u7684\u6bd4\u8868\u9762\u79ef\uff0c\u589e\u52a0\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\u7684\u5bc6\u5ea6\uff0c\u4ece\u800c\u4fc3\u8fdb\u50ac\u5316\u53cd\u5e94\u7684\u53d1\u751f\u3002<\/p>\n

\u56fe3.\u4e0d\u540c\u5f62\u8c8cAu\u7eb3\u7c73\u9897\u7c92\u7684\u900f\u5c04\u7535\u955c\u56fe<\/p>\n

\"\"<\/p>\n

\uff08a\uff09Au\u7a7a\u5fc3\u7eb3\u7c73\u7b3c\uff08b\uff09Au\u7eb3\u7c73\u7403\uff08c\uff09Au\u7eb3\u7c73\u68d2\uff08d\uff09Au\u7eb3\u7c73\u7acb\u65b9\uff1b\uff08e\uff09Au\u7a7a\u5fc3\u7eb3\u7c73\u7b3c\u50ac\u5316\u5242\u5728\u4e0d\u540c\u7535\u538b\u4e0b\u7684\u4ea7\u6c28\u901f\u7387\u548c\u6cd5\u62c9\u7b2c\u6548\u7387\uff08f\uff09-0.4V\u4e0b\u4e0d\u540c\u5f62\u8c8cAu\u7eb3\u7c73\u9897\u7c92\u7684\u4ea7\u6c28\u901f\u7387\u548c\u6cd5\u62c9\u7b2c\u6548\u7387<\/p>\n

2.3 \u7a7a\u4f4d\u8c03\u63a7<\/p>\n

\u5f15\u5165\u7a7a\u4f4d\u53ef\u4ee5\u663e\u8457\u8c03\u63a7\u50ac\u5316\u5242\u7684\u7535\u5b50\u7ed3\u6784\uff0c\u6539\u5584\u53cd\u5e94\u4e2d\u95f4\u4ea7\u7269\u7684\u5438\u9644\u7279\u6027\uff0c\u4ece\u800c\u63d0\u5347\u50ac\u5316\u5242\u7684\u53cd\u5e94\u6d3b\u6027\u3002\u6b64\u5916\uff0c\u7a7a\u4f4d\u53ef\u4ee5\u4f5c\u4e3a\u53cd\u5e94\u6d3b\u6027\u4f4d\u70b9\u5438\u9644\u53cd\u5e94\u7269\u5206\u5b50\uff0c\u4ece\u800c\u964d\u4f4e\u53cd\u5e94\u80fd\u5792\uff0c\u6709\u5229\u4e8e\u50ac\u5316\u53cd\u5e94\u7684\u5feb\u901f\u8fdb\u884c\u3002<\/p>\n

\u56fe4.<\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u975e\u6676\u76f8Bi4<\/sub>V2<\/sub>O11<\/sub>\/CeO2<\/sub>\uff08BVC-A\uff09\u7684\u80fd\u5e26\u6392\u5217\uff08b\uff09BVC-A\u754c\u9762\u7684\u7535\u8377\u8f6c\u79fb\uff08c\uff09BVC-A\u50ac\u5316\u5242\u5728\u4e0d\u540c\u7535\u538b\u4e0b\u7684\u4ea7\u6c28\u901f\u7387\u548c\u6cd5\u62c9\u7b2c\u6548\u7387\uff08d\uff09\u805a\u5408\u6c2e\u5316\u78b3\uff08PCN\uff09\u7684\u6c2e\u7a7a\u4f4d\u793a\u610f\u56fe\uff08e\uff09PCN\u7684\u6c2e\u6c14\u5438\u9644\u793a\u610f\u56fe\uff08f\uff09\u6c2e\u5438\u9644PCN\u7684\u7535\u8377\u5dee\u5f02<\/p>\n

2.4 \u63ba\u6742<\/p>\n

\u5f02\u8d28\u539f\u5b50\u63ba\u6742\u4e0d\u4ec5\u80fd\u8c03\u63a7\u50ac\u5316\u5242\u7684\u80fd\u5e26\u7ed3\u6784\uff0c\u8d4b\u4e88\u50ac\u5316\u5242\u9ad8\u7535\u8377\u5bc6\u5ea6\u4e0e\u9ad8\u672c\u5f81\u5bfc\u7535\u6027\uff0c\u540c\u65f6\u80fd\u591f\u964d\u4f4e\u53cd\u5e94\u7269\u5728\u50ac\u5316\u5242\u8868\u9762\u7684\u5438\u9644\u80fd\u5792\uff0c\u4ece\u800c\u964d\u4f4e\u7535\u50ac\u5316\u53cd\u5e94\u7684\u8fc7\u7535\u52bf\u3002<\/p>\n

\u56fe5.<\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u6c2e\u63ba\u6742\u591a\u5b54\u78b3\uff08NPC\uff09\u7684NRR\u53cd\u5e94\u8fc7\u7a0b\u793a\u610f\u56fe\uff08b\uff09\u4e0d\u540c\u6e29\u5ea6\u4e0b\u5408\u6210\u7684NPC\u7684\u5421\u54af\u3001\u5421\u5576\u548c\u77f3\u58a8\u6c2e\u7684\u542b\u91cf\uff08c\uff09NPC\u7684\u6c2e\u6c14\u6e29\u63a7\u5438\u9644\u56fe\uff08d\uff09NPC\u5728-0.7V\u548c-0.9V\u4e0b\u7684\u4ea7\u6c28\u901f\u7387\uff08e\uff09N3<\/sub>\u4f4d\u70b9\u7684NRR\u53cd\u5e94\u8def\u5f84\u793a\u610f\u56fe<\/p>\n

3.\u9ad8\u6548NRR\u7535\u50ac\u5316\u5242<\/strong><\/p>\n

3.1 \u8d35\u91d1\u5c5e\u57fa\u7535\u50ac\u5316\u5242<\/p>\n

\u56fe6.<\/p>\n

\"\"<\/p>\n

\uff08a\uff09Ru\u7eb3\u7c73\u9897\u7c92\u7684DFT\u8ba1\u7b97\u6a21\u578b\uff08b\uff09Pd\/C\u50ac\u5316\u5242\u5728\u4e0d\u540c\u7535\u89e3\u8d28\u4e0b\u7684\u7ebf\u6027\u626b\u63cf\u4f0f\u5b89\u66f2\u7ebf\uff08c\uff09Pd\/C\u3001Au\/C\u548cPt\/C \u4e0d\u540c\u50ac\u5316\u5242\u4e4b\u95f4\u7684\u6027\u80fd\u5bf9\u6bd4\uff08d\uff09Au\u3001Pt\u548c\u03b1-PdH\u00a0(211)\u8868\u9762\u7684NRR\u8def\u5f84<\/p>\n

3.2 \u975e\u8d35\u91d1\u5c5e\u57fa\u50ac\u5316\u5242<\/p>\n

\u56fe7.<\/p>\n

\"\"<\/p>\n

\uff08a\uff09VN\u50ac\u5316\u5242\u5728-0.1V\u548c-0.2V\u4e0b\u6d4b\u8bd58\u5c0f\u65f6\u5bf9\u5e94\u7684\u4ea7\u6c28\u901f\u7387\u548c\u6cd5\u62c9\u7b2c\u6548\u7387\uff08b\uff09VN0.7<\/sub>O0.45<\/sub>\u8868\u9762\u7684NRR\u53cd\u5e94\u8def\u5f84\uff08c\uff09Mo2<\/sub>C\/C\u5728\u8d28\u5b50\u532e\u4e4f\u548c\u8d28\u5b50\u5bcc\u96c6\u7684\u6761\u4ef6\u4e0b\u7684NRR\u53cd\u5e94\u673a\u5236\uff08d\uff09Mo2<\/sub>C\/C\u5728\u8d28\u5b50\u532e\u4e4f\u548c\u8d28\u5b50\u5bcc\u96c6\u7684\u6761\u4ef6\u4e0d\u540c\u7535\u538b\u4e0b\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff08e\uff09Mo2<\/sub>C\/C\u5728\u8d28\u5b50\u532e\u4e4f\u548c\u8d28\u5b50\u5bcc\u96c6\u7684\u6761\u4ef6\u4e0d\u540c\u7535\u538b\u4e0b\u7684\u4ea7\u6c28\u901f\u7387\uff08f\uff09MXene\u7684\u4f18\u5316\u7ed3\u6784\uff08g\uff09\u6c2e\u5206\u5b50\u5728MXene\u4e0d\u540c\u539f\u5b50\u4f4d\u70b9\u4e0a\u7684\u5438\u9644\u80fd\uff08h\uff09MXene\/FeOOH\u5728\u4e0d\u540c\u7535\u538b\u4e0b\u7684\u6cd5\u62c9\u7b2c\u6548\u7387<\/p>\n

3.3 \u5355\u539f\u5b50\u50ac\u5316\u5242<\/p>\n

\u56fe8.<\/p>\n

\"\"<\/p>\n

\uff08a\uff09Au\/C3<\/sub>N4<\/sub>\u7684EDX\u5143\u7d20\u5206\u5e03\uff08b,c\uff09Au\/C3<\/sub>N4<\/sub>\u7684HAADF-STEM\u56fe\uff08d\uff09\u6c2e\u63ba\u6742\u78b3\u57faRu\u5355\u539f\u5b50\u50ac\u5316\u5242\u7684\u5408\u6210\u8fc7\u7a0b\u793a\u610f\u56fe\uff1b\u4e0d\u540c\u7535\u538b\u6761\u4ef6\u4e0b\u7684Ru@NC\u3001Ru@C\u3001Ru@ZrO2<\/sub>\/NC\u548cRu@ZrO2<\/sub>\/C\u7684\uff08e\uff09\u4ea7\u6c28\u901f\u7387\uff08f\uff09\u6cd5\u62c9\u7b2c\u6548\u7387\uff1b\uff08g\uff09Ru@Zr32<\/sub>O63<\/sub>\u548cRu@NC2<\/sub>\u7684\u8ba1\u7b97\u6a21\u578b<\/p>\n

3.4 \u975e\u91d1\u5c5e\u50ac\u5316\u5242<\/p>\n

\u56fe9.<\/p>\n

\"\"<\/p>\n

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\u300aMaterials Today\u300b\u662f\u56fd\u9645\u6750\u6599\u79d1\u5b66\u7814\u7a76\u9886\u57df\u7684\u77e5\u540d\u7efc\u8ff0\u6027\u5b66\u672f\u671f\u520a\uff08\u5f71\u54cd\u56e0\u5b50\uff1a24.537\uff09\uff0c\u4e3b\u8981\u520a\u767b\u5728\u6750\u6599\u79d1\u5b66\u4e0e\u5de5\u7a0b\u9886\u57df\u6700\u65b0\u7814\u7a76\u8fdb\u5c55\u7684\u8bc4\u8ff0\u8bba\u6587\u53ca\u91cd\u8981\u7684\u539f\u521b\u6027\u7814\u7a76\u8bba\u6587\uff0c\u6bcf\u5e74\u51fa\u724810\u671f\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/p>\n

Yuchi Wan, Jichu Xu, Ruitao Lv*, Heterogeneous electrocatalysts design for nitrogen reduction reaction under ambient conditions. Mater. Today, 2019: doi.org\/10.1016\/j.mattod.2019.03.002.<\/p>\n

https:\/\/doi.org\/10.1016\/j.mattod.2019.03.002<\/u><\/a><\/p>\n

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