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\u8fc7\u7535\u52bf\uff08\u03b7\uff09\uff1a<\/p>\n

\u00a0\"\"\uff08Eeq<\/sub>\u662f\u5e73\u8861\u7535\u52bf\uff09<\/p>\n

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\"\"<\/p>\n

\u95ee\u9898\uff1a\u5728\u6d4bLSV\u6781\u5316\u66f2\u7ebf\u65f6\uff0c\u6240\u52a0\u8fc7\u7535\u52bf\u4e3a0\u65f6\uff0c\u7535\u6d41\u5374\u5927\u5e45\u5ea6\u504f\u79bb0\uff0c\u600e\u4e48\u529e\uff1f<\/p>\n

\u56de\u7b54\uff1a\u7531\u6781\u5316\u66f2\u7ebf\u7684\u5b9a\u4e49\u53ef\u77e5\uff0c\u5982\u6240\u52a0\u8fc7\u7535\u52bf\u4e3a0\u800c\u7535\u6d41\u5927\u5e45\u5ea6\u504f\u79bb0\u65f6\uff0c\u6b64\u65f6\u7535\u6781\u8868\u9762\u5e76\u6ca1\u6709\u5904\u4e8e\u7a33\u6001\uff0c\u6240\u4ee5\u6b64\u65f6\u53ea\u8981\u964d\u4f4e\u626b\u63cf\u901f\u7387\u4f7f\u7535\u6781\u8868\u9762\u8fbe\u5230\u7a33\u6001\u5373\u53ef\u3002<\/p>\n

4.\u5854\u83f2\u5c14\u659c\u7387\u66f2\u7ebf<\/b><\/strong><\/p>\n

\u5728\u5b9e\u9645\u5e94\u7528\u4e2d\uff0c\u4e3a\u4e86\u4f7f\u7535\u6d41\u5bc6\u5ea6(i)\u589e\u5927\uff0c\u9700\u8981\u65bd\u52a0\u9ad8\u8fc7\u7535\u4f4d(\u03b7)\u3002\u4e00\u822c\u6765\u8bf4\uff0c\u5e0c\u671b\u8fc7\u7535\u4f4d(\u03b7)\u8d8a\u5c0f\uff0c\u5bf9\u5e94\u7684\u7535\u6d41\u5bc6\u5ea6(i)\u589e\u957f\u8d8a\u5feb\u3002\u7535\u6d41\u5bc6\u5ea6(i)\u548c\u8fc7\u7535\u4f4d\u53ef\u4ee5\u7528\u5df2\u77e5\u7684Butler-Volmer\u65b9\u7a0b\u6765\u63cf\u8ff0\uff1a<\/p>\n

\"\"<\/p>\n

\u5728\u9ad8\u9633\u6781\u8fc7\u7535\u4f4d\u6761\u4ef6\u4e0b\uff0c\u6574\u4f53\u7535\u6d41\u4e3b\u8981\u6765\u81ea\u9633\u6781\u7aef\u90e8\uff0c\u800c\u9634\u6781\u90e8\u5206\u7684\u8d21\u732e\u53ef\u4ee5\u5ffd\u7565\u4e0d\u8ba1\u3002\u56e0\u6b64\uff0cButler-Volmer\u65b9\u7a0b\u53ef\u4ee5\u7b80\u5316\u4e3a:<\/p>\n

\"\"<\/p>\n

\u00a0\u4e5f\u79f0\u4e3aTafel\u65b9\u7a0b\u3002<\/p>\n

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\"\"<\/p>\n

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Tafel\u659c\u7387(b)\u53ef\u4ee5\u8868\u793a\u4e3a\uff1a<\/p>\n

\"\"\u00a0<\/p>\n

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\"\"<\/p>\n

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5.\u7535\u5316\u5b66<\/b><\/strong>\u963b\u6297\uff08<\/b><\/strong>EIS<\/b><\/strong>\uff09<\/b><\/strong><\/p>\n

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\"\"<\/p>\n

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6<\/b><\/strong>.<\/b><\/strong>\u7535\u5316\u5b66<\/b><\/strong>\u6d3b\u6027\u6bd4\u8868\u9762\u79ef<\/b><\/strong>\uff08<\/b><\/strong>ESCA<\/b><\/strong>\uff09<\/b><\/strong><\/p>\n

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\"\"<\/p>\n

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\u00a0\u00a0\u00a0\u00a0\u00a0\u00a0\u00a0\u00a0\"\" \"\"<\/b><\/strong><\/p>\n

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\u56de\u7b54\uff1a\u8ba1\u65f6\u7535\u6d41\u6cd5\u548c\u8ba1\u65f6\u7535\u4f4d\u6cd5\u5728\u6d4b\u91cf\u7535\u50ac\u5316\u5242\u7a33\u5b9a\u6027\u65f6\uff0c\u90fd\u6709\u4e00\u4e2a\u5c40\u9650\uff0c\u5c31\u662f\u53ea\u80fd\u5728\u540c\u4e00\u7535\u6d41\u6216\u540c\u4e00\u7535\u538b\u4e0b\u8fdb\u884c\u6d4b\u91cf\u3002\u76f8\u5bf9\u800c\u8a00\uff0c\u591a\u6b65\u8ba1\u65f6\u7535\u6d41\u6cd5\uff0c\u5373\u63a7\u5236\u7535\u538b\uff0c\u4ece\u65e0\u7535\u5316\u5b66\u53cd\u5e94\u7684\u7535\u4f4d\u9636\u8dc3\u5230\u53d1\u751f\u7535\u5316\u5b66\u53cd\u5e94\u7684\u7535\u4f4d\uff0c\u540c\u65f6\u6d4b\u91cf\u6d41\u8fc7\u7535\u6781\u7684\u7535\u6d41\u968f\u65f6\u95f4\u7684\u53d8\u5316\u3002\u8fd9\u6837\u53ef\u4ee5\u540c\u65f6\u6d4b\u91cf\u4e0d\u540c\u7535\u4f4d\u4e0b\u7535\u50ac\u5316\u5242\u7684\u7a33\u5b9a\u6027\u3002<\/p>\n

\u53c2\u8003\u6587\u732e<\/b><\/strong><\/p>\n

1.M.B. Stevens, L.J. Enman, A.S. Batchellor, M.R. Cosby, A.E. Vise, C.D.M. Trang, S.W. Boettcher, Measurement Techniques for the Study of Thin Film Heterogeneous Water Oxidation Electrocatalysts, Chem. Mater., 29 (2016) 120-140.<\/p>\n

2.T.Y. Ma, S. Dai, M. Jaroniec, S.Z. Qiao, Metal-organic framework derived hybrid Co3O4-carbon porous nanowire arrays as reversible oxygen evolution electrodes, J. Am. Chem. Soc., 136 (2014) 13925-13931.<\/p>\n

3.Nai, Y. Lu, L. Yu, X. Wang, X.W.D. Lou, Formation of Ni-Fe Mixed Diselenide Nanocages as a Superior Oxygen Evolution Electrocatalyst, Adv. Mater., 29 (2017).<\/p>\n

4.Chauhan, K.P. Reddy, C.S. Gopinath, S. Deka, Copper Cobalt Sulfide Nanosheets Realizing a Promising Electrocatalytic Oxygen Evolution Reaction, ACS Catal., 7 (2017) 5871-5879.<\/p>\n

5.Zeng, Y. Li, Recent advances in heterogeneous electrocatalysts for the hydrogen evolution reaction, J. Mater. Chem. A, 3 (2015) 14942-14962.<\/p>\n

6.Barber, S. Morin , B.E. Conway,Specificity of the kinetics of H2 evolution to the structure of single-crystal Pt surfaces, and the relation between opd and upd H, J. Electroanal. Chem., 1998, 446: 125<\/p>\n

7.Subbaraman, D. Tripkovic, K.C. Chang, D. Strmcnik, A.P. Paulikas, P. Hirunsit, M. Chan, J. Greeley, V. Stamenkovic, N.M. Markovic, Trends in activity for the water electrolyser reactions on 3d M(Ni,Co,Fe,Mn) hydr(oxy)oxide catalysts, Nat. Mater., 11 (2012) 550-557.<\/p>\n

\u56db\u3001\u7535\u50ac\u5316OER\u5927\u725b<\/b><\/strong><\/p>\n

<\/b>1.\u4fc4\u52d2\u5188\u5927\u5b66Shannon W. Boettcher\u8bfe\u9898\u7ec4<\/strong><\/p>\n

\u8bfe\u9898\u7ec4\u94fe\u63a5\uff1a\u00b7 https:\/\/wiki.uoregon.edu\/\/display\/BOETTCHERLAB\/<\/p>\n

\u7814\u7a76\u6210\u679c\uff1aAngew. Chem. Int. Ed. 2018, 57\uff1bChemSusChem 2018, 11, 1\u20138\uff1bJ. Am. Chem. Soc.<\/i><\/em>,\u00a02019<\/b><\/strong>,\u00a0141<\/i><\/em>\u00a0(4), pp 1394\u20131405\uff1bPRL 112, 148304 (2014)\uff1bACS Appl. Mater. Interfaces<\/i><\/em>,\u00a02019<\/b><\/strong>,\u00a011<\/i><\/em>\u00a0(6), pp 5590\u20135594\uff1bJ. Am. Chem. Soc.<\/i><\/em>,\u00a02017<\/b><\/strong>,\u00a0139<\/i><\/em>\u00a0(33), pp 11361\u201311364\uff1bAcc. Chem. Res.<\/i><\/em>,\u00a02016<\/b><\/strong>,\u00a049<\/i><\/em>\u00a0(4), pp 733\u2013740\uff1bJ. Phys. Chem. Lett.<\/i><\/em>,\u00a02015<\/b><\/strong>,\u00a06<\/i><\/em>\u00a0(18), pp 3737\u20133742\uff1bJ. Am. Chem. Soc.<\/i><\/em>,\u00a02015<\/b><\/strong>,\u00a0137<\/i><\/em>\u00a0(10), pp 3638\u20133648\uff1bChem. Commun., 2015, 51, 5261\uff1bAngew. Chem. Int. Ed. 2018, 57, 12840 \u201312844\uff1b<\/p>\n

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\u7814\u7a76\u9886\u57df\uff1a\u592a\u9633\u80fd\u7535\u6c60\uff0c\u80fd\u6e90\u5b58\u50a8\u548c\u8f6c\u5316\uff0c\u591a\u76f8OER\u50ac\u5316\u5242\u3002<\/p>\n

2.\u52a0\u5dde\u5927\u5b66\u4f2f\u514b\u5229\u5206\u6821Alexis T.Bell \u8bfe\u9898\u7ec4<\/strong><\/p>\n

\u8bfe\u9898\u7ec4\u94fe\u63a5\uff1ahttp:\/\/www.cchem.berkeley.edu\/atbgrp\/<\/u><\/a><\/p>\n

\u7814\u7a76\u6210\u679c\uff1a\u00a0Green Chem.<\/a>, 2018,\u00a020<\/b><\/strong>, 2903-2912\uff1b\u00a0Phys. Chem. Chem. Phys.<\/u><\/a>,<\/u>\u00a02018,\u00a020<\/b><\/strong>, 16973-16984\uff1bCatalysis Today 312 (2018) 51\u201365\uff1b: Chem. Commun., 2017, 53, 10870\uff1bT. Kessler et al. \/ Fuel 206 (2017) 171\u2013179\uff1bSynlett 2017; 28(17): 2299-2302\uff1bJ. Am. Chem. Soc.<\/i><\/em>\u00a0137,<\/b><\/strong>\u00a01305\u20131313 (2015).\uff1bEnergy Fuels<\/i><\/em>\u00a029,<\/b><\/strong>\u00a01743\u20131750 (2015).\uff1bJ. Phys. Chem. C<\/i><\/em>\u00a0119,<\/b><\/strong>\u00a07243\u20137254 (2015).\uff1bJ. Catal.<\/i><\/em>\u00a0328,<\/b><\/strong>\u00a0111\u2013122 (2015).\uff1bJ. Am. Chem. Soc.<\/i><\/em>\u00a0137,<\/b><\/strong>\u00a09595\u20139603 (2015)\uff1bJ. Phys. Chem. C<\/i><\/em>\u00a0119,<\/b><\/strong>\u00a018303\u201318316 (2015).<\/p>\n

\"\"<\/p>\n

\u7814\u7a76\u9886\u57df\uff1a\u591a\u76f8\u50ac\u5316\u5242\uff0c<\/p>\n

3.\u745e\u58eb\u8054\u90a6\u7406\u5de5\u5b66\u9662Xile Hu\u8bfe\u9898\u7ec4<\/strong><\/p>\n

\u8bfe\u9898\u7ec4\u94fe\u63a5\uff1ahttp:\/\/lsci.epfl.ch\/<\/u><\/a><\/p>\n

\u7814\u7a76\u6210\u679c\uff1aNature communications<\/i><\/em>, 2014, 5<\/b><\/strong>, 4477.,\u00a0Chemical Science 2 (7), 1262-1267\uff0cAngewandte Chemie International Edition 51 (51), 12703-12706, Energy & Environmental Science 4 (10), 3878-3888, Energy & Environmental Science 8 (8), 2347-2351, Energy & Environmental Science 7 (1), 387-392, Journal of the American Chemical Society 136 (47), 16481-16484\uff0cChemical Science 3 (8), 2515-2525, Journal of the American Chemical Society 129 (29), 8988-8998\uff0cNature communications 7, 12324, Journal of the American Chemical Society 137 (31), 9927-9936\uff0cJournal of the American Chemical Society 138 (28), 8946-8957.<\/p>\n

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\u7814\u7a76\u9886\u57df\uff1a\u6709\u673a\u91d1\u5c5e\u5316\u5b66\uff0c\u592a\u9633\u80fd\u71c3\u6599\uff0c\u7535\u50ac\u5316\uff0c\u5149\u50ac\u5316\uff0c\u65e0\u673a\u6750\u6599\u3002<\/p>\n

4.\u5927\u8fde\u7406\u5de5\u5927\u5b66Licheng Sun\u8bfe\u9898\u7ec4<\/strong><\/p>\n

\u8bfe\u9898\u7ec4\u94fe\u63a5\uff1ahttp:\/\/solar.dlut.edu.cn\/<\/u><\/a><\/p>\n

\u7814\u7a76\u6210\u679c\uff1aNature Commun.\u00a0<\/i><\/em>2018<\/b><\/strong>,\u00a09<\/i><\/em>, 381.\uff1bAdv. Energy Mater.\u00a0<\/i><\/em>2018<\/b><\/strong>,\u00a08,\u00a0<\/i><\/em>1702598.\uff1bAdv. Funct. Mater.\u00a0<\/i><\/em>2018<\/b><\/strong>,\u00a028<\/i><\/em>,\u00a01803278.\uff1bAdv. Funct. Mater.\u00a0<\/i><\/em>2018<\/b><\/strong>,\u00a028<\/i><\/em>,\u00a01801397.\uff1bAdv. Funct. Mater.\u00a0<\/i><\/em>2018<\/b><\/strong>,\u00a028,\u00a0<\/i><\/em>1704447.\uff1bACS Catal.\u00a0<\/i><\/em>2018<\/b><\/strong>,\u00a08<\/i><\/em>, 4612-4621.\uff1bACS Catal.\u00a0<\/i><\/em>2018<\/b><\/strong>,\u00a08<\/i><\/em>, 4375-4382.\uff1bCHEMSUSCHEM<\/i><\/em>\u00a02018<\/b><\/strong>,\u00a011<\/i><\/em>, 1761-1767.\uff1bChem. Commun.<\/i><\/em>\u00a02018<\/b><\/strong>,\u00a054<\/i><\/em>, 4979-4982.\uff1bChemElectroChem<\/i><\/em>\u00a02018<\/b><\/strong>,\u00a05<\/i><\/em>,\u00a02064-2068.<\/p>\n

\"\"<\/p>\n

\u7814\u7a76\u9886\u57df\uff1a\u7535\u50ac\u5316\uff0c\u5149\u50ac\u5316\uff0c\u592a\u9633\u80fd\u7535\u6c60\uff0c\u65b0\u578b\u50a8\u80fd\u5668\u4ef6\u3002<\/p>\n

5.\u65af\u5766\u798f\u5927\u5b66Hongjie Dai\u8bfe\u9898\u7ec4<\/strong><\/p>\n

\u8bfe\u9898\u7ec4\u94fe\u63a5\uff1ahttp:\/\/web.stanford.edu\/group\/dailab\/<\/u><\/a><\/p>\n

\u7814\u7a76\u6210\u679c\uff1aScience 273 (5274), 483-487\uff1bscience 287 (5453), 622-625\uff1bscience 319 (5867), 1229-1232\uff1bScience 280 (5367), 1253-1256\uff1bScience 283 (5401), 512-514\uff1bNature 386 (6624), 474\uff1bNature materials 10 (10), 780\uff1bnature 424 (6949), 654\uff1bNature 384 (6605), 147\uff1bJournal of the American Chemical Society 133 (19), 7296-7299\uff1bJournal of the American Chemical Society 135 (23), 8452-8455\uff1bJournal of the American Chemical Society 134 (7), 3517-3523\uff1bNature communications 5, 4695\uff1bNano Research 8 (1), 23-39\uff1bProceedings of the National Academy of Sciences 102 (45), 16141-16145\uff1bScience 342 (6160), 836-840.<\/p>\n

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\u7814\u7a76\u65b9\u5411\uff1a\u65b0\u578b\u7eb3\u7c73\u6750\u6599\uff0c\u7269\u7406\u5316\u5b66\uff0c\u7535\u50ac\u5316\u548c\u94dd\u79bb\u5b50\u7535\u6c60<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u79d1\u6280\u987e\u95ee luna\u00a0<\/strong>\u4f9b\u7a3f\uff0c<\/b><\/strong>\u6750\u6599\u4eba\u7f16\u8f91\u90e8Alisa\u7f16\u8f91\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1: tougao@cailiaoren.com.<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1acailiaorenVIP.<\/p>\n","protected":false},"excerpt":{"rendered":"

\u3010\u5f15\u8bed\u3011 \u5e72\u8d27\u4e13\u680f \u6750\u6599\u4eba\u73b0\u5728\u5df2\u7ecf\u63a8\u51fa\u4e86\u5f88\u591a\u4f18\u8d28\u7684\u4e13\u680f\u6587\u7ae0\uff0c\u6240\u6d89\u53ca\u9886\u57df\u4e5f\u6b63\u5728\u6162\u6162\u5b8c\u5584\u3002\u6709\u5f88\u591a\u5c0f\u4f19\u4f34\u5df2\u7ecf\u52a0\u5165\u4e86\u6211\u4eec\uff0c\u4f46\u662f\u8fd8\u6ee1\u8db3\u4e0d\u4e86\u6211\u4eec\u7684\u9700\u6c42\uff0c\u671f\u5f85\u66f4\u591a\u7684\u4f18\u79c0\u4f5c\u8005\u52a0…<\/p>\n","protected":false},"author":10213,"featured_media":174203,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[1187],"tags":[],"class_list":["post-169587","post","type-post","status-publish","format-standard","has-post-thumbnail","hentry","category-zhuanlan"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/169587"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/10213"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=169587"}],"version-history":[{"count":8,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/169587\/revisions"}],"predecessor-version":[{"id":169636,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/169587\/revisions\/169636"}],"wp:featuredmedia":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/media\/174203"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=169587"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=169587"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=169587"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}