{"id":167978,"date":"2019-02-27T06:30:39","date_gmt":"2019-02-26T22:30:39","guid":{"rendered":"\/\/m.iemloyee.com\/?p=167978"},"modified":"2019-02-26T15:17:56","modified_gmt":"2019-02-26T07:17:56","slug":"%e3%80%90%e5%b7%b2%e6%a0%a1%e7%a8%bf%e3%80%91%e6%b5%99%e6%b1%9f%e5%a4%a7%e5%ad%a6%e9%99%86%e7%9b%88%e7%9b%88%e5%9b%a2%e9%98%9fadv-funct-mater-%ef%bc%9a%e5%85%b7%e6%9c%89%e4%bc%98%e5%bc%82%e7%9a%84","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=167978","title":{"rendered":"\u6d59\u6c5f\u5927\u5b66\u9646\u76c8\u76c8\u56e2\u961fAdv. Funct. Mater.\uff1a\u5177\u6709\u4f18\u5f02\u7684\u4eb2Na\/Li\u7279\u6027\u7684\u591a\u7ea7Co3O4\u7eb3\u7c73\u7ea4\u7ef4-\u78b3\u7247\u9aa8\u67b6\u7528\u4e8e\u9ad8\u5ea6\u7a33\u5b9a\u7684\u78b1\u91d1\u5c5e\u7535\u6c60"},"content":{"rendered":"

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\u968f\u7740\u4eba\u4eec\u5bf9\u9ad8\u5bc6\u5ea6\u548c\u5b89\u5168\u50a8\u80fd\u7684\u9700\u6c42\u4e0d\u65ad\u589e\u957f\uff0c\u7535\u6c60\u6280\u672f\u7684\u53d1\u5c55\u9700\u8981\u5177\u5907\u9ad8\u5bb9\u91cf\u3001\u7a33\u5b9a\u7684\u5faa\u73af\u6027\u80fd\u548c\u957f\u5bff\u547d\u3002Li\u548cNa\u7b49\u78b1\u91d1\u5c5e\u7531\u4e8e\u7406\u8bba\u6bd4\u5bb9\u91cf\u9ad8\u548c\u6c27\u5316\u8fd8\u539f\u7535\u4f4d\u4f4e\u800c\u53d7\u5230\u5e7f\u6cdb\u7814\u7a76\u3002\u4f46\u78b1\u91d1\u5c5e\u8d1f\u6781\u7531\u4e8e\u5e93\u4ed1\u6548\u7387\u4f4e\u3001\u679d\u6676\u751f\u957f\u4e25\u91cd\uff0c\u5728\u5b9e\u9645\u5e94\u7528\u4e2d\u9762\u4e34\u7740\u5de8\u5927\u7684\u6311\u6218\u3002\u5176\u4e2d\uff0c\u91d1\u5c5e\u7535\u6781\u8868\u9762\u7684\u7ec6\u5fae\u6ce2\u52a8\u548c\u4e0d\u5747\u5300\u7684\u56fa\u4f53\u7535\u89e3\u8d28\u754c\u9762\uff08SEI\uff09\u5bfc\u81f4\u4e86\u7535\u6781\u754c\u9762\u7535\u8377\u5206\u5e03\u7684\u4e0d\u5747\u5300\uff0c\u4ece\u800c\u5bfc\u81f4\u4e86\u4e0d\u5747\u5300\u7684\u91d1\u5c5e\u6c89\u79ef\uff1b\u53e6\u4e00\u4e2a\u9650\u5236\u662f\u78b1\u91d1\u5c5e\u8d1f\u6781\u5728\u5faa\u73af\u671f\u95f4\u4e0d\u53ef\u907f\u514d\u7684\u4f53\u79ef\u53d8\u5316\uff0c\u5176\u4e0d\u65ad\u7684\u754c\u9762\u91cd\u6784\u8bf1\u5bfcSEI\u819c\u5728\u8868\u9762\u4e0a\u7684\u7834\u88c2\u548c\u5f62\u6210\uff0c\u5e76\u6d88\u8017\u7535\u6c60\u7cfb\u7edf\u4e2d\u7684\u91d1\u5c5e\u6e90\uff0c\u5bfc\u81f4\u7535\u6c60\u7684\u4e25\u91cd\u5b89\u5168\u9690\u60a3\u548c\u5bff\u547d\u7f29\u77ed\u3002\u56e0\u6b64\uff0c\u8bbe\u8ba1\u4e00\u79cd\u5177\u6709\u4eb2\u78b1\u91d1\u5c5e\u6027\u7684\u8f7d\u4f53\u9aa8\u67b6\u6765\u6291\u5236\u679d\u6676\u7684\u751f\u957f\u662f\u5341\u5206\u5fc5\u8981\u7684\u3002<\/p>\n

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\u8fd1\u65e5\uff0c\u6d59\u6c5f\u5927\u5b66\u9646<\/b><\/strong>\u76c8\u76c8<\/b><\/strong>\u6559\u6388\u56e2\u961f\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/b><\/strong>\u62a5\u9053\u4e86\u5177\u6709\u4f18\u5f02\u4eb2Na\/Li\u7684\u591a\u7ea7Co3<\/sub>O4<\/sub>\u7eb3\u7c73\u7ea4\u7ef4-\u78b3\u7247\uff08CS\uff09\u9aa8\u67b6\uff0c\u4f5c\u4e3a\u78b1\u91d1\u5c5e\u7535\u6781\u7684\u7a33\u5b9a\u57fa\u4f53\u3002\u91c7\u7528\u5546\u7528\u5bfc\u7535\u78b3\u5e03\u4f5c\u4e3a\u4e00\u7ea7\u7ed3\u6784\uff0c\u91c7\u7528\u7b80\u5355\u7684\u6c34\u70ed\u6cd5\u5236\u5907\u5782\u76f4\u751f\u957f\u7684\u4e8c\u7ea7Co3<\/sub>O4<\/sub>\u7eb3\u7c73\u7ea4\u7ef4\uff0c\u4e4b\u540e\u518d\u5c06\u7194\u878d\u78b1\u91d1\u5c5e\u6ce8\u5165\u9aa8\u67b6\u4e2d\u5f62\u6210\u91d1\u5c5e\/Co-CS\u590d\u5408\u8d1f\u6781\u3002\u4e0e\u4f20\u7edf\u7684\u94dc\u7f51\u548c\u954d\u6ce1\u6cab\u7b493D\u91d1\u5c5e\u96c6\u6d41\u4f53\u76f8\u6bd4\uff0c\u6240\u5236\u5907\u7684Li\/Na-Co\u78b3\u7247\u590d\u5408\u8d1f\u6781\u5177\u6709\u56db\u4e2a\u4e3b\u8981\u4f18\u70b9\uff1a1\uff09\u78b1\u91d1\u5c5e\u4e0eCo3<\/sub>O4<\/sub>\u53cd\u5e94\u7684\u81ea\u7531\u80fd\u53d8\u5316\u0394G\u4e3a\u8d1f\uff0c\u5bfc\u81f4\u7194\u878d\u78b1\u91d1\u5c5e\u4e0eCo3<\/sub>O4<\/sub>\u53cd\u5e94\u5f62\u6210Li2<\/sub>O\u548cCo\uff0c\u4ece\u800c\u964d\u4f4e\u4e86\u57fa\u4f53\u7684\u8868\u9762\u80fd\u30022\uff09\u5728\u5267\u70c8\u53cd\u5e94\u4e4b\u540e\uff0c\u7eb3\u7c73\u7ea4\u7ef4\u4ecd\u7136\u53ef\u4ee5\u7262\u56fa\u5730\u7c98\u9644\u5230\u78b3\u7ea4\u7ef4\u57fa\u8d28\u4e0a\uff0c\u4e3a\u6c89\u79efLi\u63d0\u4f9b\u7269\u7406\u9650\u5236\uff0c\u5e76\u4e0e\u8db3\u591f\u7684\u7535\u89e3\u8d28\/\u7535\u6781\u63a5\u89e6\uff0c\u4e3aLi\/Li+<\/sup>\u6216Na\/Na+<\/sup>\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\u7684\u63d0\u4f9b\u4e86\u5145\u8db3\u7684\u7535\u8377\u8f6c\u79fb\u4f4d\u70b9\uff0c\u4ece\u800c\u5f15\u5bfc\u5747\u5300\u7684\u6210\u6838\u30023\uff09COMSOL\u6a21\u62df\u8868\u660e\uff0c\u8fd9\u4e9b\u5782\u76f4\u751f\u957f\u7684\u7eb3\u7c73\u7ea4\u7ef4\u6709\u6548\u5730\u5206\u6563\u4e86\u9502\u79bb\u5b50\u6d41\uff0c\u4ece\u800c\u964d\u4f4e\u4e86\u6bcf\u6839\u78b3\u7ea4\u7ef4\u4e0a\u7684\u5c40\u90e8\u7535\u6d41\u5bc6\u5ea6\uff0c\u8fdb\u4e00\u6b65\u6291\u5236\u4e86\u91d1\u5c5e\u79bb\u5b50\u7684\u4e0d\u5747\u5300\u6c89\u79ef\u30024\uff09\u5206\u5c423D\u7ed3\u6784\u53ef\u4ee5\u9650\u5236\u4f53\u76f8\u91d1\u5c5e\u5728\u5faa\u73af\u4e2d\u7684\u4f53\u79ef\u53d8\u5316\uff0c\u6709\u5229\u4e8e\u5f62\u6210\u7a33\u5b9a\u7684SEI\u819c\u3002\u57fa\u4e8e\u4e0a\u8ff0\u65b0\u9896\u7684\u8bbe\u8ba1\u548c\u4f18\u70b9\uff0cLi\/Co-CS\u5bf9\u79f0\u7535\u6c60\u53ef\u4ee5\u572820mA cm-2<\/sup>\u7684\u8d85\u9ad8\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5faa\u73af\u8d85\u8fc7120\u5708\u3002\u4e0eLiFePO4<\/sub>\u6b63\u6781\u914d\u5bf9\u65f6\uff0cLi\/Co-CS\u7535\u6c60\u57282C\u4e0b200\u6b21\u5faa\u73af\u540e\u663e\u793a\u51fa88.4%\u7684\u5bb9\u91cf\u4fdd\u6301\u7387\u3002\u4f7f\u7528NaClO4<\/sub>\u57fa\u7535\u89e3\u8d28\u7684Na\/Co-CS\u5bf9\u79f0\u7535\u6c60\u4e2d\u4e5f\u89c2\u5bdf\u5230\u660e\u663e\u7684\u6539\u5584\u3002\u76f8\u5173\u6210\u679c\u4ee5\u9898\u4e3a\u201c<\/b><\/strong>Hierarchical Co<\/b><\/strong>3<\/b><\/sub><\/strong>O<\/b><\/strong>4<\/b><\/sub><\/strong>\u00a0Nanofiber\u2013Carbon Sheet Skeleton with Superior Na\/Li-Philic Property Enabling Highly Stable Alkali Metal Batteries<\/b><\/strong>\u201d<\/b><\/strong>\u53d1\u8868\u5728Adv. Funct. Mater.<\/b><\/strong>\u4e0a\uff0c\u7b2c\u4e00\u4f5c\u8005\u4e3a\u535a\u58eb\u751f\u674e\u601d\u8fdc\u3002<\/p>\n

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\u56fe1<\/b><\/strong>\u00a0<\/b><\/strong>\u78b1\u91d1\u5c5e\/Co-CS\u590d\u5408\u8d1f\u6781\u7684\u5236\u5907\u4e0e\u8868\u5f81<\/b><\/strong>\"\"<\/b><\/strong><\/p>\n

a\uff09CS\u548cCo3<\/sub>O4<\/sub>-CS\u9aa8\u67b6\u7684\u7167\u7247\u3002<\/p>\n

b\uff09\u591a\u7ea7\u7ed3\u6784Co3<\/sub>O4<\/sub>-CS\u9aa8\u67b6\u53ca\u5176\u4e0e\u7194\u878d\u78b1\u91d1\u5c5e\u63a5\u89e6\u65f6\u7684\u884c\u4e3a\u793a\u610f\u56fe\u3002<\/p>\n

c\uff09CS\u548cCo3<\/sub>O4<\/sub>-CS\u9aa8\u67b6\u7684SEM\u56fe\u50cf\uff08\u63d2\u56fe\uff1a\u666e\u901a\u7684\u78b3\u7eb3\u7c73\u7ea4\u7ef4\u8868\u9762\uff09\u3002<\/p>\n

d\uff09\u7194\u878dLi\u6ce8\u5165\u540eLi\/Co-CS\u590d\u5408\u8d1f\u6781\u7684SEM\u56fe\u50cf\uff08\u63d2\u56fe\uff1a\u5177\u6709\u5149\u6cfd\u8868\u9762\u7684Li\/Co-CS\u8d1f\u6781\u7684\u7167\u7247\uff09\u3002<\/p>\n

e\uff09Co3<\/sub>O4<\/sub>\u7c89\u672b\uff0cCS\uff0cCo3<\/sub>O4<\/sub>-CS\u548cLi\/Co-CS\u7684XRD\u56fe\u3002<\/p>\n

f\uff09\u5355\u6839Li\/Co\u78b3\u7ea4\u7ef4\u6a2a\u622a\u9762\u4e0a\u7684\u5143\u7d20\u5206\u5e03\u3002<\/p>\n

\u56fe2<\/b><\/strong>\u00a0<\/b><\/strong>\u5409\u5e03\u65af\u81ea\u7531\u80fd\u53d8\u5316\u548c\u79bb\u5b50\u8fc1\u79fb\u7684\u8ba1\u7b97<\/b><\/strong>\"\"<\/p>\n

a\uff09Co3<\/sub>O4<\/sub>\u548cLi\u53cd\u5e94\u7684\u5409\u5e03\u65af\u81ea\u7531\u80fd\u53d8\u5316\u3002<\/p>\n

b\uff09COMSOL\u6a21\u62df\u7eb3\u7c73\u7ea4\u7ef4\/\u7535\u89e3\u8d28\u754c\u9762\u5904\u7684\u7a33\u6001\u7535\u6d41\u5bc6\u5ea6\u3002\u6b63\u5e38\u7535\u6d41\u5bc6\u5ea6\u8bbe\u5b9a\u4e3a10 mA cm-2<\/sup>\u3002\u56fe\u7247\u4e2d\u7684\u989c\u8272\u53cd\u6620\u4e86\u5782\u76f4\u4e8e\u8d1f\u6781\u8868\u9762\u7684\u7535\u6d41\u5bc6\u5ea6\u7684\u5927\u5c0f\u3002<\/p>\n

c\uff09\u7ebf-\u7535\u6d41\u5bc6\u5ea6\u5728y\u8f74\u65b9\u5411\u4e0a\u7684\u5206\u5e03\uff08\u4ecey=0\u5230y=24\uff09\u3002<\/p>\n

d\uff09\u7531\u4e8e\u5c40\u90e8\u7535\u6d41\u5bc6\u5ea6\u51cf\u5c0f\u548c\u7269\u7406\u9650\u57df\u6548\u5e94\uff0c\u4f7f\u5f97Li\/Na\u7535\u6c89\u79ef\u66f4\u52a0\u5747\u5300\u3002<\/p>\n

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a,c,e\uff09Li\u91d1\u5c5e\u7535\u6c60\u5206\u522b\u5728a\uff092 mA cm\u22122<\/sup>\uff0c1 mAh cm\u22122<\/sup>\uff1bc\uff0920 mA cm\u22122<\/sup>\uff0c1 mAh cm\u22122<\/sup>\uff1be\uff091 mA cm\u22122<\/sup>\uff0c3 mAh cm\u22122<\/sup>\u7684\u7535\u538b\u66f2\u7ebf\u3002<\/p>\n

g\uff09Li\u91d1\u5c5e\u7535\u6c60\u5728\u7535\u6d41\u5bc6\u5ea6\u4e3a1\u81f310mA cm\u22122<\/sup>\u65f6\u7684\u500d\u7387\u6027\u80fd\u3002<\/p>\n

b,d,f\uff09Na\u91d1\u5c5e\u7535\u6c60\u5206\u522b\u5728b\uff091mA cm\u22122<\/sup>\uff0c1mA h cm\u22122<\/sup>\uff1bd\uff092 mA cm\u22122<\/sup>\uff0c1 mA h cm\u22122<\/sup>\uff1b<\/p>\n

f\uff091mA cm\u22122<\/sup>\uff0c3mA h cm\u22122<\/sup>\u7684\u7535\u538b\u66f2\u7ebf\u3002<\/p>\n

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i\uff09\u5728\u7b2c0\uff0c1\uff0c10\u6b21\u5faa\u73af\u524d\u540e\u7684\u672a\u6539\u6027Li\u548cLi\/Co-CS\u5bf9\u79f0\u7535\u6c60\u7684\u963b\u6297\u8c31\u3002<\/p>\n

j\uff09\u57280\uff0c90\u6b21\u5faa\u73af\u524d\u540e\u672a\u6539\u6027Na\u548cNa\/Co-CS\u5bf9\u79f0\u7535\u6c60\u7684\u963b\u6297\u8c31\u3002<\/p>\n

\u56fe<\/b><\/strong>4\u00a0<\/b><\/strong>\u5265\u79bb\u548c\u7535\u9540\u540e\u78b1\u91d1\u5c5e\/Co-CS\u8d1f\u6781\u7684\u5f62\u6001\u6f14\u53d8\u7684SEM\u56fe\u50cf<\/b><\/strong><\/b>\"\"<\/p>\n

a\uff09Na\/Co-CS\u8d1f\u6781\u7684\u4f4e\u500dSEM\u56fe\u50cf\u3002<\/p>\n

b\uff09\u5728\u4e0d\u540cNa\u6c89\u79ef\u91cf\u7684\u9aa8\u67b6\u9ad8\u500dSEM\u56fe\u50cf\uff08\u63d2\u56fe\uff1a\u5728\u591a\u7ea7Co-CS\u9aa8\u67b6\u4e0a\u7684\u6c89\u79ef\u884c\u4e3a\u7684\u793a\u610f\u56fe\uff09\u3002<\/p>\n

c\uff09\u5728\u4e0d\u540cLi\u6c89\u79ef\u91cf\u7684\u9aa8\u67b6\u9ad8\u500dSEM\u56fe\u50cf\u3002<\/p>\n

\u56fe<\/b><\/strong>5\u00a0<\/b><\/strong><\/b>\u4e0d\u540c\u7535\u6d41\u5bc6\u5ea6\u4e0b50\u6b21\u5faa\u73af\u540e<\/b><\/strong>\u672a\u6539\u6027\u7684<\/b><\/strong>\u78b1\u91d1\u5c5e\u7535\u6781\u6216\u78b1\u91d1\u5c5e\/Co-CS\u590d\u5408\u7535\u6781\u4e0aLi\/Na\u7535\u6c89\u79ef\u7684\u5f62\u8c8c<\/b><\/strong><\/b>\"\"<\/p>\n

a\uff09\u672a\u6539\u6027\u7684Na\u7535\u6781\u548cc\uff09Na\/Co-CS\u590d\u5408\u7535\u6781\u5728\u5faa\u73af\u4e4b\u524d\u548c\u5728\u7535\u6d41\u5bc6\u5ea6\u4e3a1mA cm-2<\/sup>\u768450\u4e2a\u5faa\u73af\u4e4b\u540e\u7684\u6a2a\u622a\u9762SEM\u56fe\u50cf\u3002<\/p>\n

b\uff09\u672a\u6539\u6027\u7684Na\u7535\u6781\u548cd\uff09Na\/Co-CS\u590d\u5408\u7535\u6781\u5728\u5faa\u73af\u4e4b\u524d\u548c\u5728\u7535\u6d41\u5bc6\u5ea6\u4e3a1mA cm-2<\/sup>\u768450\u4e2a\u5faa\u73af\u4e4b\u540e\u7684SEM\u56fe\u50cf\u3002<\/p>\n

\u56fe<\/b><\/strong>6\u00a0<\/b><\/strong><\/b>\u4f7f\u7528<\/b><\/strong>\u6539\u6027<\/b><\/strong>\u78b1\u91d1\u5c5e\/Co-CS\u7535\u6781\u7684\u534a\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd<\/b><\/strong><\/b>\"\"<\/p>\n

a\uff09Li-Co-CS\/LFP\u548cLi\/LFP\u7535\u6c60\u57282C\u4e0b\u7684\u957f\u5faa\u73af\u6027\u80fd\uff0c\u8d28\u91cf\u8d1f\u8f7d\u4e3a4mg cm-2<\/sup>\u3002<\/p>\n

b\uff09Li-Co-CS\/LFP\u548cLi\/LFP\u7535\u6c60\u57281.0\u523010.0 C\u7684\u4e0d\u540c\u500d\u7387\u4e0b\u7684\u500d\u7387\u80fd\u529b\u3002<\/p>\n

c\uff09Li-Co-CS\/LFP\u548cLi\/LFP\u7535\u6c60\u5728\u500d\u7387\u4e3a3.0\uff0c5.0\u548c10.0 C\u7684\u7535\u538b\u66f2\u7ebf\u3002<\/p>\n

d\uff09\u57281C\u4e0bNa-CS\/NVPF\u548cNa\/NVPF\u7535\u6c60\u7684\u957f\u5faa\u73af\u6027\u80fd\uff0c\u8d28\u91cf\u8d1f\u8f7d\u4e3a1.5mg cm-2<\/sup>\u3002<\/p>\n

\u3010\u5c0f\u7ed3<\/b><\/strong>\u3011<\/p>\n

\u8be5\u56e2\u961f\u8bbe\u8ba1\u4e86\u4e00\u79cd\u591a\u7ea73D Co3<\/sub>O4<\/sub>-CS\u9aa8\u67b6\uff0c\u901a\u8fc7\u5728\u78b3\u7247\u57fa\u4f53\u4e0a\u5f15\u5165\u4eb2\u78b1\u91d1\u5c5e\u7684Co3<\/sub>O4<\/sub>\u7eb3\u7c73\u7ea4\u7ef4\uff0c\u6539\u5584\u4e86\u78b1\u91d1\u5c5e\u8d1f\u6781\u5bf9\u78b3\u57fa\u5e95\u7684\u6da6\u6e7f\u6027\u3002\u8fd9\u9879\u5de5\u4f5c\u4e3a\u591a\u7ed3\u6784\u7684\u9502\u91d1\u5c5e\u6846\u67b6\u521b\u9020\u4e86\u65b0\u7684\u8bbe\u8ba1\u539f\u5219\uff0c\u4e3a\u5b9e\u73b0\u4e0b\u4e00\u4ee3\u80fd\u6e90\u5bc6\u96c6\u578b\u78b1\u91d1\u5c5e\u7535\u6c60\u7684\u5b89\u5168\u8fd0\u884c\u521b\u9020\u4e86\u673a\u4f1a\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>Hierarchical Co<\/u>3<\/sub><\/u>O<\/u>4<\/sub><\/u>\u00a0Nanofiber\u2013Carbon Sheet Skeleton with Superior Na\/Li<\/u>–<\/u>Philic Property Enabling Highly Stable Alkali Metal Batteries<\/u><\/a>\uff08Adv. Funct. Mater., 2019, DOI:10.1002\/adfm.201808847\uff09<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u5b66\u672f\u7ec4\u6728\u6587\u97ec<\/b><\/strong>\u7ffb\u8bd1\uff0c\u6d59\u6c5f\u5927\u5b66\u9646\u76c8\u76c8\u6559\u6388<\/strong>\u4fee\u6b63\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"

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