{"id":163687,"date":"2019-01-08T06:38:43","date_gmt":"2019-01-07T22:38:43","guid":{"rendered":"\/\/m.iemloyee.com\/?p=163687"},"modified":"2019-01-07T21:55:11","modified_gmt":"2019-01-07T13:55:11","slug":"acs-energy-lett-%e5%b0%81%e9%9d%a2-mof%e8%a1%8d%e7%94%9f%e5%87%ba%e7%9a%84%e4%ba%8c%e7%bb%b4%e6%9d%90%e6%96%99%e5%9c%a8%e7%94%b5%e5%82%ac%e5%8c%96%e4%b8%ad%e7%9a%84%e5%ba%94%e7%94%a8","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=163687","title":{"rendered":"ACS Energy Lett. \u5c01\u9762 |\u00a0MOF\u884d\u751f\u51fa\u7684\u4e8c\u7ef4\u6750\u6599\u5728\u7535\u50ac\u5316\u4e2d\u7684\u5e94\u7528"},"content":{"rendered":"
\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n \u7531\u4e8e\u5177\u6709\u66f4\u591a\u7684\u6d3b\u6027\u4f4d\u70b9\u548c\u66f4\u77ed\u7684\u53cd\u5e94\u7269\/\u4ea7\u7269\u6269\u6563\u8def\u5f84\uff0c\u4e8c\u7ef4\u6750\u6599\u8fd1\u5e74\u6765\u5728\u70b9\u50ac\u5316\u9886\u57df\u5f97\u5230\u8d8a\u6765\u8d8a\u591a\u7684\u5e94\u7528\u3002\u4f46\u76ee\u524d\u4e8c\u7ef4\u6750\u6599\u7684\u5236\u5907\u4e3b\u8981\u5c40\u9650\u4e8e\u6c34\u70ed\u5408\u6210\u53ca\u6db2\u76f8\u5265\u79bb\u3002\u6b64\u7c7b\u65b9\u6cd5\u5f80\u5f80\u5177\u6709\u660e\u663e\u7684\u7f3a\u9677\uff1a\u4f8b\u5982\u6c34\u70ed\u4e0d\u6613\u63a7\u5236\u6750\u6599\u7684\u539a\u5ea6\uff0c\u800c\u6db2\u76f8\u5265\u79bb\u4e0d\u4ec5\u4ea7\u7387\u8f83\u4f4e\u800c\u4e14\u64cd\u4f5c\u8fc7\u7a0b\u7ecf\u5e38\u4f1a\u4f7f\u7528\u5230\u5bf9\u4eba\u4f53\u6709\u5bb3\u7684\u5316\u5b66\u8bd5\u5242\u3002\u7eb3\u7c73\u5c3a\u5ea6\u7684\u6676\u754c\u7f3a\u9677\u5de5\u7a0b\u80fd\u591f\u663e\u8457\u63d0\u9ad8\u7eb3\u7c73\u7535\u50ac\u5316\u5242\u5728OER\u3001CO2\u8fd8\u539f\u7b49\u53cd\u5e94\u4e2d\u7684\u50ac\u5316\u6d3b\u6027\u3002\u56e0\u6b64\uff0c\u7406\u8bba\u4e0a\uff0c\u5728\u4e8c\u7ef4\u6750\u6599\u5185\u5f15\u5165\u7eb3\u7c73\u5c3a\u5ea6\u7684\u6676\u754c\u7f3a\u9677\u53ef\u4ee5\u8fdb\u4e00\u6b65\u63d0\u9ad8\u4e8c\u7ef4\u6750\u6599\u7684\u7535\u50ac\u5316\u6027\u80fd\u3002\u7136\u800c\uff0c\u76ee\u524d\u4e3b\u8981\u4f7f\u7528\u9502\u79bb\u5b50\u7535\u5316\u5b66\u8c03\u63a7\u7684\u65b9\u6cd5\u6765\u7834\u574f\u6676\u7c92\u5f97\u5230\u7eb3\u7c73\u591a\u6676\u6750\u6599\u3002\u56e0\u6b64\uff0c\u5728\u5236\u5907\u65b9\u6cd5\u4e0a\u5c1a\u6709\u4e00\u4e9b\u56f0\u96be\u9700\u8981\u514b\u670d\u3002<\/p>\n \u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n \u7f8e\u56fd\u7231\u8377\u534e\u5dde\u7acb\u5927\u5b66<\/b><\/strong>\u7684\u79d1\u7814\u5de5\u4f5c\u8005\u5728ACS<\/b><\/strong>\u00a0<\/b><\/strong>Energy<\/b><\/strong>\u00a0<\/b><\/strong>Letters<\/b><\/strong>\u4e0a\uff0c\u53d1\u8868\u4e86\u9898\u4e3a\u201cDefect-Rich 2D Material Networks for Advanced Oxygen Evolution Catalysts\u201d\u7684\u7814\u7a76\u8bba\u6587\uff0c\u5e76\u88ab\u9009\u4e3a\u671f\u520a\u5c01\u9762\u3002\u8be5\u5de5\u4f5c\u4e3b\u8981\u4ee5\u5ba4\u6e29\u5408\u6210Co-MOF\u9635\u5217\u4e3a\u524d\u9a71\u4f53\uff0c\u901a\u8fc7\u5ba4\u6e29\u6761\u4ef6\u4e0b\u4e59\u9187\u6eb6\u6db2\u4f53\u7cfb\u5bf9MOF\u8fdb\u884c\u7834\u574f\/\u91cd\u7ec4\uff0c\u5f97\u5230\u7eb3\u7c73\u5c3a\u5ea6\u7684\u591a\u6676\u4e8c\u7ef4\u6750\u6599\u7684\u4e09\u7ef4\u7f51\u7edc\u7ed3\u6784\u3002\u78b1\u6027\u6761\u4ef6\u4e0b\u8be5\u6750\u6599\u8868\u73b0\u51fa\u4f18\u5f02\u7684OER\u6d3b\u6027\u548c\u7a33\u5b9a\u6027\u3002\u8be5\u5de5\u4f5c\u540c\u65f6\u4e5f\u5bf9Co-MOF\u7684\u751f\u957f\u53ca\u4e8c\u7ef4\u6750\u6599\u7684\u5f62\u6210\u673a\u7406\u8fdb\u884c\u4e86\u63a2\u8ba8\u3002<\/p>\n \u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n Schem<\/b><\/strong>e 1. <\/b><\/strong>\u5ba4\u6e29\u6761\u4ef6\u4e0bCo-MOF\u7684\u5408\u6210\u8def\u5f84\u53ca\u591a\u6676\u4e8c\u7ef4\u6750\u6599\u7684\u751f\u6210\u793a\u610f\u56fe\u3002<\/b><\/strong><\/p>\n Figure 1. Co-MOF <\/b><\/strong>\u53ca\u751f\u6210\u7684C<\/b><\/strong>o(OH)<\/b><\/strong>2<\/b><\/sub><\/strong>\u4e8c\u7ef4\u6750\u6599\u7684\u7ed3\u6784\/\u6210\u5206\u8868\u5f81\u3002<\/b><\/strong><\/p>\n Figure 2. <\/b><\/strong>\u7eb3\u7c73\u591a\u6676\u7684C<\/b><\/strong>o(OH)<\/b><\/strong>2<\/b><\/sub><\/strong>\u4e8c\u7ef4\u6750\u6599\u7684\u9ad8\u500dHAADF<\/b><\/strong>-STEM<\/b><\/strong>\u56fe\u3002<\/b><\/strong><\/p>\n Figure 3. <\/b><\/strong>\u7eb3\u7c73\u591a\u6676\u7684C<\/b><\/strong>o(OH)<\/b><\/strong>2<\/b><\/sub><\/strong>\u4e8c\u7ef4\u6750\u6599\u57281M<\/b><\/strong>\u00a0<\/b><\/strong>KOH\u4e2d\u7684\u6027\u80fd\u6d4b\u8bd5\u53ca\u5bf9\u6bd4\u56fe\u3002<\/b><\/strong><\/p>\n Figure 4. <\/b><\/strong>\u5728\u7eaf\u5316\u7684KOH<\/b><\/strong>, <\/b><\/strong>\u672a\u7eaf\u5316\u7684KOH<\/b><\/strong>, <\/b><\/strong>\u53ca\u542b2<\/b><\/strong>m<\/b><\/strong>M<\/b><\/strong>\u00a0Fe<\/b><\/strong>\u7684KOH\u4e2d\u7684OER\u6027\u80fd\u6d4b\u8bd5\u5bf9\u6bd4\u3002\u7ed3\u679c\u8868\u660eFe\u6742\u8d28\u7684\u5f15\u5165\u80fd\u591f\u663e\u8457\u589e\u5f3aCo<\/b><\/strong>\/Ni <\/b><\/strong>OER\u50ac\u5316\u5242\u7684\u6d3b\u6027\u3002<\/b><\/strong><\/p>\n Figure<\/b><\/strong>\u00a05. <\/b><\/strong>\u901a\u8fc7\u6539\u53d8\u4e59\u9187\u8150\u8680\u4f53\u7cfb\u7684\u5316\u5b66\u6210\u5206\uff0c\u6700\u7ec8\u5f97\u5230\u7684\u4e8c\u7ef4\u6750\u6599\u7684\u5316\u5b66\u6210\u5206\u5f97\u5230\u4e86\u8c03\u63a7\u3002\u6750\u6599\u53ca\u5316\u5b66\u6210\u5206\u8868\u5f81\u8868\u660e\u5f97\u5230\u7684\u4f9d\u65e7\u662f\u7eb3\u7c73\u591a\u6676\u7684\u4e8c\u7ef4\u6750\u6599\u3002<\/b><\/strong><\/p>\n \u00a0 \u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n \u8be5\u5de5\u4f5c\u63d0\u51fa\u4e86\u5ba4\u6e29\u6761\u4ef6\u4e0b\u4ee5\u5408\u6210\u7684Co-MOF\u4e3a\u524d\u9a71\u4f53\u6765\u5236\u5907\u7eb3\u7c73\u591a\u6676\u4e8c\u7ef4\u6750\u6599\u7f51\u7edc\u7684\u65b0\u65b9\u6cd5\uff0c\u5e76\u8be6\u7ec6\u8ba8\u8bba\u4e86\u5404\u4e2a\u5316\u5b66\u53cd\u5e94\u4e2d\u7684\u673a\u7406\u3002\u8be5\u65b9\u6cd5\u64cd\u4f5c\u7b80\u5355\uff0c\u6240\u6709\u8fc7\u7a0b\u5747\u5728\u5ba4\u6e29\u6761\u4ef6\u4e0b\u5b8c\u6210\uff0c\u4e3a\u5927\u89c4\u6a21\u5236\u5907\u4e8c\u7ef4\u6750\u6599\u53ca\u80fd\u6e90\u8f6c\u6362\u548c\u5b58\u50a8\u9886\u57df\u7684\u53d1\u5c55\u63d0\u4f9b\u4e86\u65b0\u7684\u601d\u8def\u3002<\/p>\n<\/p>\n
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