{"id":162678,"date":"2018-12-27T06:30:16","date_gmt":"2018-12-26T22:30:16","guid":{"rendered":"\/\/m.iemloyee.com\/?p=162678"},"modified":"2018-12-27T10:38:16","modified_gmt":"2018-12-27T02:38:16","slug":"%e3%80%90%e9%80%9a%e8%ae%af%e4%bd%9c%e8%80%85%e4%b8%ba%e5%9b%bd%e5%a4%96%ef%bc%8c%e6%9c%aa%e6%a0%a1%e7%a8%bf%e3%80%91adv-funct-mater-%e7%bb%bc%e8%bf%b0%ef%bc%9a%e6%b7%b7%e5%90%88%e5%b0%ba%e5%af%b82d","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=162678","title":{"rendered":"Adv. Funct. Mater.\u7efc\u8ff0\uff1a\u6df7\u5408\u5c3a\u5bf82D \/ 3D\u6df7\u5408\u9499\u949b\u77ff\u5438\u6536\u5242\uff0c\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7684\u672a\u6765\uff1f"},"content":{"rendered":"<p>\u3010\u5f15\u8a00\u3011<\/p>\n<p>\u6709\u673a-\u65e0\u673a\u91d1\u5c5e\u5364\u5316\u7269\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60(PSCs)\u51ed\u501f\u5176\u4f4e\u6210\u672c\u3001\u6613\u5236\u5907\u548c\u51fa\u8272\u7684\u5149\u7535\u6027\u80fd\uff0c\u5728\u8fd1\u51e0\u5e74\u53d6\u5f97\u4e86\u8fc5\u731b\u53d1\u5c55\uff0c\u8dfb\u8eab\u6750\u6599\u79d1\u5b66\u9886\u57df\u6700\u70ed\u95e8\u7684\u7814\u7a76\u65b9\u5411\u4e4b\u4e00\uff0c\u5728\u6e05\u6d01\u80fd\u6e90\u4ea7\u4e1a\u4e2d\u5177\u6709\u7740\u5de8\u5927\u7684\u53d1\u5c55\u6f5c\u529b\u548c\u79ef\u6781\u4f5c\u7528\u3002\u7136\u800c\uff0c\u5728\u5927\u89c4\u6a21\u5de5\u4e1a\u5316\u751f\u4ea7\u4e4b\u524d\uff0c\u8fd8\u6709\u4e00\u4e2a\u5173\u952e\u7684\u95ee\u9898\u4e9f\u5f85\u89e3\u51b3\u2014\u2014\u8fd9\u7c7b\u6750\u6599\u5bf9\u6e7f\u5ea6\u3001\u5149\u7167\u548c\u70ed\u7b49\u5916\u754c\u73af\u5883\u56e0\u7d20\u654f\u611f\uff0c\u7a33\u5b9a\u6027\u8f83\u5dee\u3002\u5f53\u524d\u63d0\u51fa\u7684\u5e94\u5bf9\u7b56\u7565\u4e4b\u4e00\u662f\u53d1\u5c55\u6e90\u4e8eRuddlesden\u2013Popper(\u7b80\u79f0RP)\u76f8\u7684\u4e8c\u7ef4\u9499\u949b\u77ff\u7ed3\u6784\uff0c\u4e8c\u7ef4RP\u76f8\u9499\u949b\u77ff\u5728\u73af\u5883\u6761\u4ef6\u4e0b\u5177\u6709\u4f18\u5f02\u7684\u7a33\u5b9a\u6027\uff0c\u662f\u83b7\u53d6\u7a33\u5b9a\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7684\u6700\u53ef\u9760\u8def\u5f84\u4e4b\u4e00\u3002<\/p>\n<p>\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/p>\n<p>\u8fd1\u65e5\uff0c<strong>\u6cd5\u56fd\u4e9a\u7720\u5927\u5b66<\/strong>\uff08\u76ae\u5361\u7b2c\u5112\u52d2-\u51e1\u5c14\u7eb3\u5927\u5b66\uff0cUniversit\u00e9 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Cells?<\/strong>\u201d\u7684\u7efc\u8ff0\u6587\u7ae0\u3002\u6b64\u7bc7\u7efc\u8ff0\u805a\u71262D\/3D\u6df7\u5408\u4f53\u7cfb\u5149\u7535\u6750\u6599\u7684\u6676\u4f53\u7ed3\u6784\u3001\u5149\u7535\u6027\u80fd\u3001\u7535\u8377\u8f7d\u6d41\u5b50\u52a8\u529b\u5b66\u53ca\u5176\u5bf9\u5149\u7535\u6027\u80fd\u7684\u5f71\u54cd\uff0c\u5c55\u5f00\u4e86\u8be6\u7ec6\u8ba8\u8bba\u548c\u9610\u91ca\u3002\u6700\u540e\uff0c\u5f3a\u8c03\u4e86\u63a5\u4e0b\u6765\u9762\u4e34\u7684\u4e00\u7cfb\u5217\u6311\u6218\uff0c\u5e76\u5bf9\u7528\u4e8e\u9ad8\u6027\u80fd\u3001\u7a33\u5b9a\u7684\u592a\u9633\u80fd\u7535\u6c60\u76842D\/3D\u9499\u949b\u77ff\u6750\u6599\u4f5c\u6982\u8ff0\u3002<\/p>\n<p>\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/p>\n<p>\u56fe1\uff1a\u6742\u5316\u9499\u949b\u77ff\u7684\u6676\u4f53\u7ed3\u6784\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-162680\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/1-8.png\" alt=\"\" width=\"600\" height=\"237\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/1-8.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/1-8-300x119.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/>(a) \u5316\u5b66\u7ec4\u6210\u6bd4\u4e3aABX<sub>3<\/sub>\u7684\u7acb\u65b9\u9499\u949b\u77ff\u7684\u6676\u4f53\u7ed3\u6784\uff1b<\/p>\n<p>(b) \u7406\u60f3\u7acb\u65b9\u9499\u949b\u77ff\u7ed3\u6784\u5408\u6210\u7684\u5bb9\u5fcd\u56e0\u5b50(tolerance factor)\u3002<\/p>\n<p>\u56fe2\uff1a\u4e8c\u7ef4\u5c42\u72b6\u6742\u5316\u6709\u673a-\u65e0\u673a\u9499\u949b\u77ff\u7684\u7ed3\u6784\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-162681\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/2-9.png\" alt=\"\" width=\"600\" height=\"201\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/2-9.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/2-9-300x101.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/>(a) \u4e8c\u7ef4\u5c42\u72b6\u6742\u5316\u6709\u673a-\u65e0\u673a\u9499\u949b\u77ffn=1\u4e14\u5e26\u6709\u5355\u4e00\u7684\u4e8c\u53d6\u4ee3\u80fa\u7684\u5178\u578b\u7ed3\u6784\uff1b<\/p>\n<p>(b) \u5177\u6709\u591a\u91cd\u91cf\u5b50\u9631\u7684\u4e8c\u7ef4\u9499\u949b\u77ff\u7684\u80fd\u5e26\u6392\u5217\u3002<\/p>\n<p>\u56fe3\uff1a\u4e8c\u7ef4\u6676\u4f53\u7ed3\u6784\u3001\u6df7\u5408\u7ef4\u65702D\/3D\u9499\u949b\u77ff\u548c\u4e09\u7ef4\u9499\u949b\u77ff\u7684\u793a\u610f\u56fe\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-162682\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/3-8.png\" alt=\"\" width=\"600\" height=\"641\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/3-8.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/3-8-281x300.png 281w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u56fe4\uff1a 2D\/3D\u9499\u949b\u77ff\u7684\u7ed3\u6784\u53ca\u5176\u5149\u7535\u6027\u80fd\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-162683\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/4-11.png\" alt=\"\" width=\"600\" height=\"891\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/4-11.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/4-11-202x300.png 202w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>(a) 2D\/3D\u9499\u949b\u77ff(PEA)<sub>2<\/sub>(MA)<sub>2<\/sub>[Pb<sub>3<\/sub>I<sub>10<\/sub>]\u548c\u4e09\u7ef4\u9499\u949b\u77ffMAPBI<sub>3<\/sub>\u7684\u6676\u4f53\u7ed3\u6784\uff1b<\/p>\n<p>(b) (PEA)<sub>2<\/sub>(MA)<sub>n\u22121<\/sub>PbnI<sub>3n+1<\/sub>\u9499\u949b\u77ff\u7684\u5355\u4f4d\u6676\u80de\u7ed3\u6784\u548c\u4e0d\u540cn\u503c\u7684\u5668\u4ef6\u6027\u80fd\u3002<\/p>\n<p>\u56fe5\uff1a\u8584\u819c\u6837\u54c1\u7684\u62e9\u4f18\u751f\u957f\u548cXRD\u7ed3\u679c\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-162684\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/5-6.png\" alt=\"\" width=\"600\" height=\"904\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/5-6.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/5-6-199x300.png 199w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/>(a) BA<sub>2<\/sub>PbI<sub>4<\/sub>\u548cMAPbI<sub>3<\/sub>\u9499\u949b\u77ff\u7684\u8584\u819c\u548c\u5757\u4f53\u6837\u54c1\u7684X\u5c04\u7ebf\u884d\u5c04\u7ed3\u679c\uff0c\u793a\u610f\u56fe\u662f\u6cbf\u62e9\u4f18\u53d6\u5411\u7684\u6676\u4f53\u7ed3\u6784\uff1b<\/p>\n<p>(b) (BA)<sub>2<\/sub>(MA)Pb<sub>2<\/sub>I<sub>7<\/sub>, (BA)<sub>2<\/sub>(MA)<sub>2<\/sub>Pb<sub>3<\/sub>I<sub>10<\/sub>, \u548c(BA)<sub>2<\/sub>(MA)<sub>3<\/sub>Pb<sub>4<\/sub>I<sub>13<\/sub>\u9499\u949b\u77ff\u7684\u8584\u819c\u548c\u5757\u4f53\u6837\u54c1\u7684X\u5c04\u7ebf\u884d\u5c04\u7ed3\u679c\uff0c\u793a\u610f\u56fe\u662f\u6cbf\u62e9\u4f18\u53d6\u5411\u7684\u6676\u4f53\u7ed3\u6784\u3002<\/p>\n<p>\u56fe6\uff1a\u70ed\u94f8\u6cd5(hot-cast)\u5236\u59072D\/3D \u7ed3\u6784\u7684\u9499\u949b\u77ff\u53ef\u6709\u6548\u63d0\u9ad8\u7a33\u5b9a\u6027\u53ca\u6548\u7387\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-162685\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/6-1.png\" alt=\"\" width=\"600\" height=\"877\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/6-1.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/6-1-205x300.png 205w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/>(a) \u5ba4\u6e29\u5236\u5907\u7684\u591a\u6676(BA)<sub>2<\/sub>(MA)<sub>3<\/sub>Pb<sub>4<\/sub>I<sub>13<\/sub>\u7684GIWAXS\u5206\u5e03\u56fe\uff0c\u6807\u6ce8\u4e86\u51e0\u4e2a\u4e3b\u5cf0\u7684Miller\u6307\u6570\uff1b<\/p>\n<p>(b) \u70ed\u94f8\u7684\u8fd1\u4e4e\u5355\u6676\u7684\u591a\u6676(BA)<sub>2<\/sub>(MA)<sub>3<\/sub>Pb<sub>4<\/sub>I<sub>13<\/sub>\u7684GIWAXS\u5206\u5e03\u56fe\uff0c\u6807\u6ce8\u4e86\u51e0\u4e2a\u4e3b\u5cf0\u7684Miller\u6307\u6570\uff1b<\/p>\n<p>(c) (101)\u53d6\u5411\uff0c\u6cbf(111)\u548c(202)\u5e73\u9762\u7684\u4e8c\u7ef4\u9499\u949b\u77ff\u6676\u4f53\u7684\u793a\u610f\u56fe\uff0c\u548cGIWAXS\u6570\u636e\u4e00\u81f4\uff1b<\/p>\n<p>(d) \u4f7f\u7528\u4e8c\u7ef4(BA)<sub>2<\/sub>(MA)<sub>3<\/sub>Pb<sub>4<\/sub>I<sub>13<\/sub>\u9499\u949b\u77ff\u4f5c\u4e3a\u5438\u6536\u5c42\uff08\u5c42\u539a\u5ea6\u4e3a230nm\uff0c\u4e3a\u6700\u4f18\u539a\u5ea6\uff09\u7684\u5e73\u9762\u5668\u4ef6\uff0c\u5728\u6807\u51c6\u5149\u7167(AM 1.5G)\u4e0b\uff0c\u5206\u522b\u7ecf\u5b9e\u9a8c\u548c\u6a21\u62df\u5f97\u5230\u7684\u7535\u6d41\u5bc6\u5ea6-\u7535\u538b\u66f2\u7ebf\uff1b<\/p>\n<p>(e~h) \u5e73\u9762\u592a\u9633\u80fd\u7535\u6c60\u7684\u7a33\u5b9a\u6027\u6d4b\u91cf\uff0c\u5176\u4e2d(e)\u548c(g)\u662f\u5728\u6052\u5b9a\u5149\u7167\u4e0b\uff08AM 1.5G\uff09\u6d4b\u91cf\uff0c(f)\u548c(h)\u662f\u572865% \u6e7f\u5ea6\u73af\u5883\u4e0b\u6d4b\u91cf\uff0c(e)\u548c(f)\u662f\u672a\u5c01\u88c5\u7684\uff0c(g)\u548c(h)\u662f\u5c01\u88c5\u540e\u7684\u3002<\/p>\n<p>\u56fe7\uff1a\u57fa\u4e8e2D\/3D\u5f02\u8d28\u7ed3\u548c\u53cc\u5c42\u7ed3\u6784\u7684\u592a\u9633\u80fd\u7535\u6c60\u5668\u4ef6\u7684\u7a33\u5b9a\u6027\u6d4b\u8bd5\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-162686\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/7-1.png\" alt=\"\" width=\"600\" height=\"779\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/7-1.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/12\/7-1-231x300.png 231w\" sizes=\"(max-width: 600px) 100vw, 600px\" 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href=\"https:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/adfm.201806482\" target=\"_blank\" rel=\"noopener\">Mixed Dimensional 2D\/3D Hybrid Perovskite Absorbers: The Future of Perovskite Solar Cells?<\/a>\uff08Adv. Funct. 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