{"id":154213,"date":"2018-09-23T06:23:29","date_gmt":"2018-09-22T22:23:29","guid":{"rendered":"\/\/m.iemloyee.com\/?p=154213"},"modified":"2018-09-22T20:24:10","modified_gmt":"2018-09-22T12:24:10","slug":"%e3%80%90%e5%b7%b2%e6%a0%a1%e7%a8%bf%e3%80%91%e7%94%b5%e5%ad%90%e7%a7%91%e5%a4%a7%e8%8b%8f%e5%b7%9e%e5%a4%a7%e5%ad%a6adv-mater-%e9%94%82%e8%92%99%e8%84%b1%e5%9c%9f%ef%bc%88li-mmt%ef%bc%89","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=154213","title":{"rendered":"\u7535\u5b50\u79d1\u5927&\u82cf\u5dde\u5927\u5b66Adv. Mater: \u9502\u8499\u8131\u571f\uff08Li-MMT\uff09\u4f5c\u4e3a\u786b\u4e3b\u4f53\u7528\u4e8e\u9ad8\u786b\u8d1f\u8f7d\u91cf\u548c\u9ad8\u500d\u7387\u6027\u80fd\u7684\u9502\u786b\u7535\u6c60"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/b><\/strong><\/p>\n

\u9502-\u786b(Li-S)\u7535\u6c60\u5177\u6709\u6781\u9ad8\u7684\u7406\u8bba\u6bd4\u5bb9\u91cf(1675 mAhg-1<\/sup>)\uff0c\u4e14\u786b\u542b\u91cf\u4e30\u5bcc\uff0c\u4ef7\u683c\u4f4e\u5ec9\uff0c\u88ab\u5e7f\u6cdb\u5730\u8ba4\u4e3a\u662f\u672a\u6765\u5927\u89c4\u6a21\u50a8\u80fd\u9886\u57df\u5e94\u7528\u53d1\u5c55\u7684\u65b9\u5411\u3002\u7136\u800c\uff0c\u9502\u786b\u7535\u6c60\u7684\u53d1\u5c55\u901a\u5e38\u53d7\u5230\u4ee5\u4e0b3\u4e2a\u95ee\u9898\u7684\u963b\u788d\uff1a\uff081\uff09\u786b\u53ca\u5176\u653e\u7535\u4ea7\u7269\u786b\u5316\u9502(Li2<\/sub>S)\u7535\u5bfc\u7387\u4f4e\uff0c\u901a\u5e38\u9700\u8981\u4e0e\u5bfc\u7535\u5242\u590d\u5408\uff0c\u4ee5\u589e\u5f3a\u7535\u5b50\u4f20\u8f93\uff0c\u8fd9\u964d\u4f4e\u4e86\u7535\u6c60\u7684\u80fd\u91cf\u5bc6\u5ea6\u3002\uff082\uff09\u786b\u548c\u786b\u5316\u9502\u53cd\u590d\u8f6c\u6362\u7684\u4f53\u79ef\u53d8\u5316\uff0c\u5bfc\u81f4\u6d3b\u6027\u6750\u6599\u7684\u8131\u843d\u3002\uff083\uff09\u591a\u786b\u5316\u7269\u4e2d\u95f4\u4f53\u5728\u7535\u89e3\u6db2\u4e2d\u7684\u6eb6\u89e3\u4ee5\u53ca\u201c\u7a7f\u68ad\u6548\u5e94\u201d\u3002\u800c\u5bf9\u4e8e\u5b9e\u73b0\u9502\u786b\u7535\u6c60\u7684\u9ad8\u500d\u7387\u6027\u80fd\uff0cLi\u79bb\u5b50\u7684\u6269\u6563\u80fd\u529b\u8d77\u5230\u51b3\u5b9a\u6027\u4f5c\u7528\uff0c\u5176\u4f5c\u7528\u53ef\u80fd\u8fdc\u5927\u4e8e\u6750\u6599\u7684\u7535\u5b50\u5bfc\u7535\u6027\u3002\u7279\u522b\u662f\uff0c\u968f\u7740\u786b\u8d1f\u8f7d\u91cf\u7684\u589e\u52a0\uff0cLi\u79bb\u5b50\u5728\u6b63\u6781\u4e2d\u7684\u8fc1\u79fb\u95ee\u9898\u5c06\u9010\u6e10\u88ab\u653e\u5927\uff0c\u8fd9\u662f\u56e0\u4e3a\u5728\u539a\u786b\u6b63\u6781\u4e2d\uff0c\u7535\u89e3\u6db2\u6da6\u6e7f\u6027\u53d8\u5dee\u540c\u65f6Li\u79bb\u5b50\u5728\u78b3\u57fa\u6750\u6599\u8868\u9762\u7684\u6269\u6563\u52bf\u5792\u8f83\u9ad8\uff0c\u5bfc\u81f4Li\u79bb\u5b50\u5f88\u96be\u5feb\u901f\u7684\u8fdb\u5165\u539a\u786b\u6b63\u6781\u5185\u90e8\u5e76\u53c2\u4e0e\u53cd\u5e94\u3002\u5bfc\u81f4\u901a\u5e38\u6240\u5236\u5907\u7684\u786b\u7535\u6781\u819c\u7684\u539a\u5ea6\u4f4e\u4e8e100\u03bcm\u7684\u5de5\u4e1a\u6807\u51c6\uff08\u786b\u8d1f\u8f7d\u91cf<1mg cm-2<\/sup>\uff09\u5e76\u4e14\u79bb\u5b50\u4f20\u8f93\u7535\u6d41\u5bc6\u5ea6\u53d7\u9650\uff08\u901a\u5e38<2mA cm -2<\/sup>\uff09\u3002\u56e0\u6b64\uff0c\u9ad8\u786b\u8d1f\u8f7d\u91cf\u6b63\u6781\u5728\u5145\u7535\u548c\u653e\u7535\u8fc7\u7a0b\u4e2d\u5e38\u5e38\u53ea\u80fd\u627f\u53d7\u4f4e\u7535\u6d41\u5bc6\u5ea6\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u7535\u5b50\u79d1\u6280\u5927\u5b66\u718a\u6770\u3001\u4f55\u4f1f\u4e1c\u6559\u6388<\/b><\/strong>\u8054\u5408\u82cf\u5dde\u5927\u5b66\u664f\u6210\u6797\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/b><\/strong>\u9996\u6b21\u5f15\u5165\u5177\u6709\u539f\u5b50\u5c42\u95f4\u79bb\u5b50\u8def\u5f84\u7684\u9502\u8499\u8131\u571f\uff08Li-MMT\uff09\u4f5c\u4e3a\u786b\u4e3b\u4f53\uff0c\u6784\u9020\u4e86\u5177\u6709\u9ad8\u786b\u8d1f\u8f7d\u91cf\u548c\u9ad8\u500d\u7387\u6027\u80fd\u7684\u9502\u786b\u7535\u6c60\u3002\u7531\u4e8eLi-MMT\u7684\u72ec\u7279\u7ed3\u6784\uff0c\u5c42\u95f4\u8ddd\u5927\u4e8e1 nm\uff0c\u7535\u89e3\u6db2\u53ef\u6709\u6548\u6e17\u900f\u786b\u7535\u6781\u3002\u6b64\u5916\uff0c Li\u79bb\u5b50\u53ef\u4ee5\u5728\u5c42\u95f4\u5feb\u901f\u7684\u8fc1\u79fb\uff0c\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\uff08DFT\uff09\u8ba1\u7b97\u8868\u660e\u5176\u8fc1\u79fb\u52bf\u5792\u7ea6\u4e3a\u5728\u78b3\u57fa\u6750\u6599\u8868\u9762\u7684\u4e00\u534a\uff0c\u4ece\u800c\u5b9e\u73b0Li\u79bb\u5b50\u80fd\u591f\u8f83\u5feb\u901f\u7684\u8fdb\u5165\u6750\u6599\u5185\u90e8\u3002\u5f53\u4e0e80\uff05\u786b\u7c89\u7ed3\u5408\u4f7f\u7528\u65f6\uff0c\u8d85\u5bbd\u5c42\u95f4\u8def\u5f84\u7684\u72ec\u7279\u4f18\u52bf\u4f7fLi-MMT\/S\u7535\u6781\u5728\u786b\u8d1f\u8f7d\u91cf\u4e3a4 mg cm\u22122<\/sup>\u65f6\uff0c\u57281 mA cm-2<\/sup>\u4e0b\u5177\u6709865 mAh g-1<\/sup>\u7684\u9ad8\u5bb9\u91cf\uff0c\u572815 mA cm\u22122<\/sup>\u7684\u9ad8\u7535\u6d41\u5bc6\u5ea6\u4e0b\uff0c\u5bb9\u91cf\u4e3a345 mAh g\u22121<\/sup>\u3002\u7ed3\u5408\u8def\u6613\u65af\u9178\u78b1\u7ed3\u5408\u7406\u8bba\uff0cDFT\u8ba1\u7b97\u8868\u660e\uff0cLi-MMT\u4e0e\u4f20\u7edf\u7684\u7c98\u5408\u5242\uff0c\u5982\u529f\u80fd\u805a\u5408\u7269\uff0c\u6742\u539f\u5b50\u63ba\u6742\u548c\u91d1\u5c5e\u786b\u5c5e\u5143\u7d20\u5316\u7269\u76f8\u6bd4\uff0c\u5176\u5438\u9644\u80fd\u66f4\u5747\u8861\uff0c\u65e0\u8bba\u957f\u94fe\u6216\u77ed\u94fe\u5747\u5177\u6709\u8f83\u9ad8\u7684\u5438\u9644\u80fd\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u201cAtomic Interlamellar Ion Path in High Sulfur Content Lithium-Montmorillonite Host Enables High-Rate and Stable Lithium<\/b><\/strong>\u2013<\/b><\/strong>Sulfur Battery<\/b><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Advanced Materials<\/b><\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u56fe\u4e00<\/b><\/strong>\u6676\u4f53\u7ed3\u6784<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u5177\u6709\u5c42\u95f4\u5206\u5b50\u7a7a\u95f4\u7684MMT\u548c\u9633\u79bb\u5b50\u7684\u6846\u67b6\u7ed3\u6784<\/p>\n

\uff08b\uff09\u4eceMMT\u5230Li-MMT\u7684\u9633\u79bb\u5b50\u4ea4\u6362\u7684\u793a\u610f\u56fe<\/p>\n

\uff08c\uff09Li\u79bb\u5b50\u6269\u6563\u7684\u80fd\u5792\u4e0eLi-MMT\u7684\u5c42\u95f4\u8868\u9762\u7684\u793a\u610f\u56fe\uff0c\u5176\u8fdc\u4f4e\u4e8e\u78b3\u57fa\u7535\u6781\u4e2d\u7684\u6269\u6563\u52bf\u5792<\/p>\n

\u56fe\u4e8c<\/b><\/strong>\u7ed3\u6784\u8868\u5f81\u548c\u7269\u76f8\u8868\u5f81<\/b><\/strong><\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

\uff08a\uff0cb\uff09Li-MMT\u7684SEM\u56fe\u50cf<\/p>\n

\uff08c\uff09\u63a5\u89e6\u89d2\u6d4b\u8bd5<\/p>\n

\uff08d\uff0ce\uff09Li-MMT\/S\u7684HRTEM\u56fe\u50cf\uff0c\u663e\u793a\u5c42\u95f4\u95f4\u8ddd\u4e3a1.396nm<\/p>\n

\uff08f\uff09S\u7c89\u672b\uff0cLi-MMT \/ S\u548cLi-MMT\u7684XRD\u56fe\u8c31<\/p>\n

\u56fe\u4e09<\/b><\/strong>\u9502\u79bb\u5b50\u6269\u6563\u548c\u7535\u5316\u5b66\u6027\u80fd<\/b><\/strong><\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

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\uff08b\uff09\u9502\u79bb\u5b50\u6269\u6563\u80fd\u529b\u5bf9\u6bd4<\/p>\n

\uff08c\uff09AB\/S\u548cLi-MMT\/S\u7535\u6781\u4e4b\u95f4\u7684\u7a7f\u68ad\u7535\u6d41\u4e0e\u65bd\u52a0\u7684\u6052\u7535\u4f4d\u5145\u7535\u7535\u538b\u7684\u6bd4\u8f83<\/p>\n

\uff08d\uff09AB\/S\u548cLi-MMT\/S\u7535\u6781\u7684\u500d\u7387\u6027\u80fd\u5bf9\u6bd4<\/p>\n

\uff08e\uff09Li-MMT\/S\u7535\u6781\u57285mAcm-2<\/sup>\u4e0b\u7684\u957f\u671f\u5faa\u73af\u6027\u80fd<\/p>\n

\u56fe\u56db Li-MMT\/S\u7535\u6781\u7684\u9ad8\u7535\u6d41\u5bc6\u5ea6\u5faa\u73af\u5206\u6790<\/b><\/strong><\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

\uff08a\uff0cb\uff09\u5206\u522b\u5177\u67094mg cm\u22122<\/sup>\u786b\u8d1f\u8f7d\u7684AB\/S\u548cLi-MMT\/S\u7535\u6781\u7684\u6052\u7535\u6d41\u5145\u7535\/\u653e\u7535\u66f2\u7ebf<\/p>\n

\uff08c\uff09\u786b\u8d1f\u8f7d\u91cf\u548c\u7535\u6d41\u5bc6\u5ea6\u4e4b\u95f4\u7684\u76f8\u5173\u6027\u4ee5\u53ca\u6587\u732e\u4e2d\u6700\u8fd1\u7684\u76f8\u5173\u62a5\u9053<\/p>\n

\uff08d\uff09\u4e0d\u540c\u786b\u8f7d\u91cf\u7684EIS\u56fe<\/p>\n

\uff08e\uff09Li-MMT\/S\u7535\u6781\u57288mA cm\u22122<\/sup>\u4e0b\u7684\u957f\u5faa\u73af\u6027\u80fd\uff0c\u786b\u8f7d\u91cf\u4e3a5.2mg cm\u22122<\/sup><\/p>\n

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\u56fe\u4e94\u7406\u8bba\u8ba1\u7b97<\/b><\/strong><\/p>\n

\"\"<\/p>\n

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\uff08c\uff09\u5206\u522b\u66b4\u9732\u4e8eAB\uff0cMMT\u548cLi-MMT\u540e\uff0cLi2<\/sub>S8<\/sub>\u6eb6\u6db2\u7684\u7d2b\u5916-\u53ef\u89c1\u5149\u8c31\uff08350-700nm\uff09<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/b><\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1a<\/b><\/strong>\u201c<\/b><\/strong>Atomic Interlamellar Ion Path in High Sulfur Content<\/b><\/u><\/strong>\u00a0<\/b><\/u><\/strong>Lithium-Montmorillonite Host Enables High-Rate and<\/b><\/u><\/strong>\u00a0<\/b><\/u><\/strong>Stable Lithium\u2013Sulfur Battery<\/b><\/u><\/strong><\/a>\u201d(<\/b><\/strong>Adv.Mater<\/b><\/strong>.<\/b><\/strong>\u00a0DOI: 10.1002\/adma.201804084)<\/b><\/strong><\/p>\n

\u00a0<\/b><\/strong>\u3010\u4f5c\u8005\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u664f\u6210\u6797\uff1a<\/b><\/strong>\u82cf\u5dde\u5927\u5b66\u80fd\u6e90\u5b66\u9662\uff0c\u00a0\u9662\u957f\uff0c\u6559\u6388\/\u535a\u5bfc\uff0c\u4e2d\u7ec4\u90e8\u9752\u5e74\u201c\u5343\u4eba\u8ba1\u5212\u201d\u5165\u9009\u8005\uff0c\u56fd\u5bb6\u201c\u4f18\u79c0\u9752\u5e74\u57fa\u91d1\u201d\u83b7\u5f97\u8005\u3002\u664f\u6210\u6797\u6559\u6388\u662f\u79d1\u6280\u90e8\u201c\u56fd\u5bb6\u56fd\u9645\u79d1\u6280\u5408\u4f5c\u4e13\u9879\u201d\u8bc4\u5ba1\u4e13\u5bb6\u3001\u6559\u80b2\u90e8\u9752\u5e74\u201c\u957f\u6c5f\u5b66\u8005\u201d\u6db5\u8bc4\u4e13\u5bb6\u3002\u4e3b\u8981\u4ece\u4e8b\u9502\u79bb\u5b50\u7535\u6c60\u4e0e\u539f\u4f4d\u8868\u5f81\u65b9\u9762\u7684\u7814\u7a76\u5de5\u4f5c\uff0c\u8fd1\u5e74\u6765\u7684\u9879\u76ee\u5305\u62ec\u56fd\u5bb6\u91cd\u70b9\u57fa\u7840\u7814\u7a76\u53d1\u5c55\u8ba1\u5212\u9879\u76ee\u8bfe\u9898\u3001\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u9879\u76ee\u3001\u4e2d\u7ec4\u90e8\u9752\u5e74\u5343\u4eba\u8ba1\u5212\u9879\u76ee\u548c\u4e2d\u5fb7\u56fd\u9645\u5408\u4f5c\u9879\u76ee\u7b49\u3002\u53d1\u8868\u8bba\u6587100\u591a\u7bc7\uff0c\u4e3b\u8981\u53d1\u8868\u5728\u56fd\u9645\u6743\u5a01\u5b66\u672f\u671f\u520a\u5982Chem. Soc. Rev.\u3001J. Am. Chem. Soc.\u3001Angew.Chem. Int. Ed.\u3001Adv. Mater.\u7b49\u6742\u5fd7\u4e0a\uff0c\u5176\u4e2d\u53d1\u8868\u5f71\u54cd\u56e0\u5b50\u5927\u4e8e10\u7684\u8bba\u658740\u591a\u7bc7\u3002<\/p>\n

\u4f55\u4f1f\u4e1c\uff1a<\/b><\/strong>\u7535\u5b50\u79d1\u6280\u5927\u5b66\u7269\u7406\u5b66\u9662\uff0c\u6559\u6388\/\u535a\u5bfc\uff0c\u4e3b\u8981\u7814\u7a76\u65b9\u5411\u4e3a\u9502\u7535\u6c60\/\u71c3\u6599\u7535\u6c60\u79bb\u5b50\u5668\u4ef6\uff0c\u9502\u7535\u6c60\u6750\u6599\u7684\u751f\u957f\u7406\u8bba\u3001\u5236\u5907\u3001\u5668\u4ef6\u96c6\u6210\u53ca\u6027\u80fd\u5206\u6790\uff0c\u53ca\u65b0\u578b\u73af\u4fdd\u6750\u6599\u53ca\u6280\u672f\u3002\u622a\u81f3\u76ee\u524d\uff0c\u53d7\u9080\u505a\u4e3a\u7b2c\u4e00\u4f5c\u8005\u4e3a\u56fd\u9645\u51fa\u7248\u793eSpringer\u3001Scholars\u2019 Press\u51fa\u7248\u7535\u6c60\u53ca\u6750\u6599\u4e66\u7c4d3\u90e8\uff0c\u5e76\u5728Adv. Energy Mater.\u00a0ACS Nano,\u00a0ACS Energy Lett. Nano Energy, Small\u7b49\u56fd\u9645SCI\u671f\u520a\u4e0a\u53d1\u8868\u8bba\u6587100\u4f59\u7bc7\u3002<\/p>\n

\u718a\u6770\uff1a<\/b><\/strong>\u7535\u5b50\u79d1\u6280\u5927\u5b66\u7535\u5b50\u79d1\u5b66\u4e0e\u5de5\u7a0b\u5b66\u9662\uff0c\u6559\u6388\/\u535a\u5bfc\uff0c\u56fd\u5bb6\u201c\u4f18\u79c0\u9752\u5e74\u57fa\u91d1\u201d\u83b7\u5f97\u8005\u3002\u4e3b\u8981\u4ece\u4e8b\u65b0\u578b\u4e8c\u7ef4\u6750\u6599\u4e0e\u5668\u4ef6\u3001\u8d85\u5bfc\u7eb3\u7c73\u5355\u5149\u5b50\u63a2\u6d4b\u5173\u952e\u6280\u672f\u7814\u7a76\u3001\u5149\u7535\u6750\u6599\u4e0e\u5668\u4ef6\u53ca\u50a8\u80fd\u5143\u4ef6\u7814\u7a76\u7b49\u65b9\u9762\u7814\u7a76\u3002\u5df2\u5728Adv. Mater. Adv. Energy\u00a0Mater.\u7b49\u6742\u5fd7\u4e0a\u53d1\u8868\u591a\u7bc7\u9ad8\u6c34\u5e73\u6587\u7ae0\u3002<\/p>\n

\u3010\u4f18\u8d28\u6587\u732e\u63a8\u8350\u3011<\/strong><\/p>\n

\u7535\u5b50\u79d1\u6280\u5927\u5b66\u718a\u6770\u6559\u6388\u56e2\u961f\u3001\u4f55\u4f1f\u4e1c\u6559\u6388\u56e2\u961f\u4ee5\u53ca\u82cf\u5dde\u5927\u5b66\u664f\u6210\u6797\u6559\u6388\u56e2\u961f\u5728\u9502\u786b\u7535\u6c60\u7814\u7a76\u65b9\u9762\u53d6\u5f97\u4e86\u4e00\u7cfb\u5217\u7814\u7a76\u6210\u679c\uff0c\u53d1\u8868\u4e86\u591a\u7bc7\u9ad8\u6c34\u5e73\u6587\u7ae0\u3002\u5982\u5728\u7c98\u63a5\u5242\uff08Adv. Mater.\u00a02017, 29, 1605160. Adv. Energy Mater. 2018, 8, 1702889. Small 2018, 14, 1801536\uff09\u3001\u6b63\u6781\u6750\u6599\u7ed3\u6784\u8bbe\u8ba1\uff08Adv. Mater.\u00a02017, 29, 1701294. Adv. Energy Mater. 2017, 7, 1601843. Nano Lett.\u00a02017, 17, 5064. Nano Energy,\u00a02017,\u00a041, 758. Small 2017, 13, 1701013.\uff09\u3001\u9694\u819c\u4f18\u5316\u8bbe\u8ba1\uff08Joule. DOI: 10.1016\/j.joule.2018.07.022\uff09\u3001\u91d1\u5c5e\u9502\u8d1f\u6781\u4fdd\u62a4\uff08Nano Lett.\u00a02018, 30, nl-2018-01882e.R1.\uff09\u7b49\u65b9\u9762\u3002\u4e3a\u8fdb\u4e00\u6b65\u63a8\u52a8\u9502\u786b\u7535\u6c60\u5546\u4e1a\u5316\u6253\u4e0b\u4e86\u575a\u5b9e\u7684\u57fa\u7840\u3002<\/p>\n

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