{"id":153568,"date":"2018-09-15T06:17:31","date_gmt":"2018-09-14T22:17:31","guid":{"rendered":"\/\/m.iemloyee.com\/?p=153568"},"modified":"2018-09-15T17:29:42","modified_gmt":"2018-09-15T09:29:42","slug":"%e8%8b%8f%e5%b7%9e%e5%a4%a7%e5%ad%a6%e5%88%98%e5%ba%84adv-funct-mater-%ef%bc%9a%e5%9f%ba%e4%ba%8e%e6%b0%9f%e5%8c%96%e5%8d%9f%e5%95%89%e7%9a%84%e5%85%b1%e4%bb%b7%e6%9c%89%e6%9c%ba%e8%81%9a%e5%90%88","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=153568","title":{"rendered":"\u82cf\u5dde\u5927\u5b66\u5218\u5e84Adv. Funct. Mater.\uff1a\u57fa\u4e8e\u6c1f\u5316\u535f\u5549\u7684\u5171\u4ef7\u6709\u673a\u805a\u5408\u7269\u4f5c\u4e3a\u6c27\u6c14\u7eb3\u7c73\u68ad\u7528\u4e8e\u80bf\u7624\u7f3a\u6c27\u7f13\u89e3\u548c\u589e\u5f3a\u5149\u52a8\u529b\u7597\u6cd5"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u80bf\u7624\u7f3a\u6c27\u662f\u80bf\u7624\u7684\u4e00\u4e2a\u6076\u6027\u7279\u70b9\uff0c\u5176\u80fd\u591f\u4fc3\u8fdb\u80bf\u7624\u7684\u8fdb\u4e00\u6b65\u751f\u957f\u548c\u8f6c\u79fb\uff0c\u540c\u65f6\u80bf\u7624\u7f3a\u6c27\u4f1a\u4e25\u91cd\u5f71\u54cd\u80bf\u7624\u7684\u6cbb\u7597\u6548\u679c\u3002\u5149\u52a8\u529b\u6cbb\u7597\u662f\u5229\u7528\u6d3b\u6027\u6c27\u6765\u5b9e\u73b0\u80bf\u7624\u6cbb\u7597\u7684\u4e00\u79cd\u65b9\u6cd5\uff0c\u5728\u4e34\u5e8a\u524d\u548c\u4e34\u5e8a\u7814\u7a76\u4e2d\u90fd\u88ab\u8bc1\u5b9e\u8f83\u4e3a\u6709\u6548\uff0c\u4f46\u662f\u80bf\u7624\u7f3a\u6c27\u4ecd\u7136\u4f1a\u9650\u5236\u5149\u52a8\u529b\u6cbb\u7597\u7684\u5b9e\u9645\u6548\u679c\u3002\u56e0\u6b64\uff0c\u8fd1\u4e9b\u5e74\u6765\u53d1\u5c55\u51fa\u4e86\u591a\u79cd\u65e8\u5728\u901a\u8fc7\u6291\u5236\u80bf\u7624\u7f3a\u6c27\u6765\u63d0\u9ad8\u80bf\u7624\u6cbb\u7597\u6548\u679c\u7684\u65b9\u6cd5\u3002\u4f8b\u5982\u901a\u8fc7\u589e\u52a0\u80bf\u7624\u8840\u6d41\u91cf\u6216\u8005\u5206\u89e3\u80bf\u7624\u5185H2<\/sub>O2<\/sub>\u5b9e\u73b0\u80bf\u7624\u7684\u6709\u6548\u6c27\u5408\u3002\u6b64\u5916\uff0c\u6c27\u6c14\u7eb3\u7c73\u68ad\u4e5f\u88ab\u5f00\u53d1\u51fa\u6765\uff0c\u5b9e\u73b0\u4e86\u76f4\u63a5\u5411\u80bf\u7624\u90e8\u4f4d\u8f93\u9001\u6c27\u6c14\u3002\u7eb3\u7c73\u5171\u4ef7\u6709\u673a\u805a\u5408\u7269\u5177\u6709\u660e\u786e\u7ec4\u6210\u548c\u5b54\u7ed3\u6784\uff0c\u5728\u836f\u7269\u8d1f\u8f7d\u548c\u75be\u75c5\u6cbb\u7597\u7b49\u65b9\u9762\u53d1\u6325\u4e86\u91cd\u8981\u4f5c\u7528\uff0c\u7136\u800c\u8fd9\u7c7b\u7eb3\u7c73\u5171\u4ef7\u6709\u673a\u805a\u5408\u7269\u8fd8\u6ca1\u6709\u88ab\u4f5c\u4e3a\u7eb3\u7c73\u6c27\u6c14\u7eb3\u7c73\u68ad\u7528\u4e8e\u80bf\u7624\u7684\u5149\u52a8\u529b\u6cbb\u7597\u4e2d\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u82cf\u5dde\u5927\u5b66\u5218\u5e84\u6559\u6388\u4e0e\u51af\u826f\u73e0\u52a9\u7406\u7814\u7a76\u5458<\/strong>\u5236\u5907\u4e86\u4e00\u79cd\u591a\u529f\u80fd\u6c1f\u5316\u7684\u5171\u4ef7\u6709\u673a\u805a\u5408\u7269\uff0c\u5176\u5728\u51b7\u51bb\u5e72\u71e5\u5904\u7406\u540e\u4ecd\u663e\u793a\u51fa\u4f18\u5f02\u7684\u751f\u7406\u7a33\u5b9a\u6027\uff0c\u7136\u540e\u5168\u6c1f-15-\u51a0-5-\u919a(PFCE)\u88ab\u8d1f\u8f7d\u5230\u8be5\u5171\u4ef7\u6709\u673a\u805a\u5408\u7269\u4e2d\uff0c\u8fdb\u800c\u5b9e\u73b0\u9ad8\u6548\u7684\u6c27\u6c14\u8d1f\u8f7d\u3002\u7814\u7a76\u8868\u660e\uff0c\u57fa\u4e8ePFCE\u7684\u6c27\u6c14\u4f20\u8f93\u80fd\u529b\uff0c\u80fd\u591f\u5b9e\u73b0\u6709\u6548\u7684\u80bf\u7624\u6c27\u5408\uff0c\u8fdb\u800c\u5728660\u7eb3\u7c73\u6fc0\u5149\u7167\u5c04\u4e0b\u53d6\u5f97\u826f\u597d\u7684\u5149\u52a8\u529b\u6cbb\u7597\u6548\u679c\u3002\u8be5\u6210\u679c\u4ee5\u9898\u4e3a”Covalent Organic Polymers Based on Fluorinated Porphyrin as Oxygen Nanoshuttles for Tumor Hypoxia Relief and Enhanced Photodynamic Therapy”<\/strong>\u53d1\u8868\u5728Advanced Functinal Materials<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe<\/strong>1 <\/strong>\u6c1f\u5316\u7eb3\u7c73\u5171\u4ef7\u6709\u673a\u805a\u5408\u7269\uff08<\/strong>COP<\/strong>\uff09\u7684\u5408\u6210\u4e0e\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

(a) THPPpf<\/sub>-PEG\u7684\u5408\u6210\u8def\u7ebf\u4ee5\u53ca\u968f\u540e\u7684PFCE\u8d1f\u8f7d\u793a\u610f\u56fe\uff1b<\/p>\n

(b) \u6e38\u79bb\u6001THPP\u548cTHPPpf<\/sub>-PEG\u5728\u7532\u9187\u4e2d\u7684UV\u2013vis\u2013NIR \u5438\u6536\u5149\u8c31\uff1b<\/p>\n

(c) THPPpf<\/sub>-PEG\u7684TEM\u7167\u7247\uff1b<\/p>\n

(d) \u65b0\u9c9c\u5236\u5907\u4ee5\u53ca\u51b7\u51bb\u5e72\u71e5\u540e\u518d\u6c34\u5316\u7684THPPpf<\/sub>-PEG\u7684DLS\u7684\u5c3a\u5bf8\u5206\u5e03\u66f2\u7ebf\uff1b<\/p>\n

(e) \u5229\u7528GC-MS\u6d4b\u8bd5\u7684THPPpf<\/sub>\u2013PEG and THPPsea<\/sub>\u2013PEG\u7684PFCE\u8d1f\u8f7d\u80fd\u529b\uff1b<\/p>\n

(f) THPPpf<\/sub>\u2013PEG\u3001PFCE@THPPpf<\/sub>\u2013PEG\u548cTHPPsea<\/sub>\u2013PEG\u7684\u6c27\u6c14\u8d1f\u8f7d\u80fd\u529b\uff1b<\/p>\n

(g) \u66b4\u9732\u4e8e660 nm LED\uff0810mW cm-2<\/sup>\uff09\u65f6\u901a\u8fc7SOSG\u8367\u5149\u5f3a\u5ea6\u6765\u8bc4\u4f30\u5f97\u5230\u7684THPPpf<\/sub>\u2013PEG\u3001PFCE@THPPpf<\/sub>\u2013PEG\u548cTHPPsea<\/sub>\u2013PEG\u7684\u5149\u52a8\u529b\u5b66\u6548\u5e94\u3002<\/p>\n

\u56fe2 THPPpf\u2013PEG\u548cPFCE@THPPpf\u2013PEG\u7684\u7ec6\u80de\u5185\u5185\u5316\u7279\u5f81\u3001\u5149\u52a8\u529b\u6548\u5e94\u548c\u751f\u7269\u76f8\u5bb9\u6027<\/strong><\/p>\n

\"\"<\/p>\n

(a) \u4e0eTHPPpf<\/sub>-PEG\u4e00\u8d77\u5b75\u53161\u30012\u548c4\u5c0f\u65f6\uff0c\u901a\u8fc7\u6fc0\u5149\u5171\u805a\u7126\u663e\u5fae\u955c\u89c2\u5bdf4T1\u7ec6\u80de\u7684\u7ec6\u80de\u5185\u5185\u5316\u7279\u5f81\uff1b<\/p>\n

(b) \u5728\u6709\u65e0\u5149\u7167\u5c04\u6761\u4ef6\u4e0b\uff0c\u4e0eTHPPpf<\/sub>-PEG\u548cPFCE @ THPPpf<\/sub>-PEG\u4e00\u8d77\u5b75\u5316\u65f6\u901a\u8fc7\u6fc0\u5149\u5171\u805a\u7126\u663e\u5fae\u955c\u89c2\u5bdf4T1\u7ec6\u80de\u7684\u6d3b\u6027\u6c27\u4ea7\u751f\u60c5\u51b5\uff1b<\/p>\n

(c) 660 nm LED \u5149\u7167\u4e0b\uff0c\u4f7f\u7528\u4e0d\u540c\u6d53\u5ea6\u7684THPPpf<\/sub>-PEG\u548cPFCE @ THPPpf<\/sub>-PEG\u5904\u74064T1\u7ec6\u80de\u540e\u7684\u76f8\u5bf9\u7ec6\u80de\u6d3b\u529b\uff1b<\/p>\n

(d) \u65e0660 nm LED \u5149\u7167\u4e0b\uff0c\u4f7f\u7528\u4e0d\u540c\u6d53\u5ea6\u7684THPPpf<\/sub>-PEG\u548cPFCE @ THPPpf<\/sub>-PEG\u5904\u74064T1\u7ec6\u80de\u540e\u7684\u76f8\u5bf9\u7ec6\u80de\u6d3b\u529b\u3002<\/p>\n

\u56fe3 THPPpf<\/sub>-PEG\u548cPFCE @ THPPpf<\/sub>-PEG\u7684\u4f53\u5185SPECT\u6210\u50cf\u548c\u836f\u4ee3\u52a8\u529b\u5b66<\/strong><\/p>\n

\"\"<\/p>\n

(a) \u4f53\u5185\u6ce8\u5c04THPPpf<\/sub>-PEG\u540e\u4e0d\u540c\u65f6\u95f4\u95f4\u9694\u8bb0\u5f55\u76844T1\u8377\u7624\u5c0f\u9f20\u7684SPECT\u56fe\u50cf\uff1b<\/p>\n

(b) \u4f53\u5185\u6ce8\u5c04PFCE @THPPpf<\/sub>-PEG\u540e\u4e0d\u540c\u65f6\u95f4\u95f4\u9694\u8bb0\u5f55\u76844T1\u8377\u7624\u5c0f\u9f20\u7684SPECT\u56fe\u50cf\uff1b<\/p>\n

(c) (a)\u548c(b)\u4e2dSPECT\u56fe\u50cf\u611f\u5174\u8da3\u533a\u57df\uff08ROI\uff09\u7684\u5b9a\u91cf\u5206\u6790\uff1b<\/p>\n

(d) 4T1\u8377\u7624\u5c0f\u9f20\u9759\u8109\u6ce8\u5c04THPPpf<\/sub>-PEG\u548cPFCE @THPPpf<\/sub>-PEG\u540e\u7684\u8840\u6db2\u5faa\u73af\u66f2\u7ebf\uff1b<\/p>\n

(e) 24\u5c0f\u65f64T1\u8377\u7624\u5c0f\u9f20\u5185THPPpf<\/sub>-PEG\u548cPFCE @THPPpf<\/sub>-PEG\u7684\u751f\u7269\u5206\u5e03\u60c5\u51b5\u3002<\/p>\n

\u56fe4\u4f53\u5185\u80bf\u7624\u6c27\u5408<\/strong><\/p>\n

\"\"<\/p>\n

(a) \u80bf\u7624\u6c27\u5408\u8fc7\u7a0b\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

(b) \u4ee5Oxy-hemo\u6a21\u5f0f\u8bb0\u5f55\u7684\u4f53\u5185\u6ce8\u5c04THPPpf<\/sub>-PEG\u548cPFCE @THPPpf<\/sub>-PEG 24\u5c0f\u65f6\u540e\u5c0f\u9f20\u4f53\u51854T1\u80bf\u7624\u7684PA\u56fe\u50cf\uff1b<\/p>\n

(c) \u56fe(b)\u4e2d\u7684\u7ea2\u8272\u865a\u7ebf\u5706\u5708\u6240\u793aPA\u56fe\u50cf\u6240\u5bf9\u5e94sO2\u5e73\u5747\u603b\u503c\u7684\u5b9a\u91cf\u5206\u6790\uff1b<\/p>\n

(d) \u5206\u522b\u6ce8\u5c04THPPpf<\/sub>-PEG\u548cPFCE @THPPpf<\/sub>-PEG 4\u548c24\u5c0f\u65f6\u540e\u4ece\u5c0f\u9f20\u4f53\u5185\u6536\u96c6\u7684\u80bf\u7624\u5207\u7247\u7684\u79bb\u4f53\u514d\u75ab\u8367\u5149\u67d3\u8272\uff1b<\/p>\n

(e) \u4e0d\u540c\u5904\u7406\u5207\u7247\u7684\u9633\u6027\u7f3a\u6c27\u533a\u57df\u767e\u5206\u6bd4\u7684\u534a\u5b9a\u91cf\u5206\u6790\u3002<\/p>\n

\u56fe5 \u7528PFCE @ THPPpf-PEG\u8fdb\u884c\u4f53\u5185\u589e\u5f3a\u7684PDT\u6cbb\u7597<\/strong><\/p>\n

\"\"<\/p>\n

(a) \u6cbb\u7597\u540e\u56db\u7ec4\u5c0f\u9f20\u7684\u80bf\u7624\u751f\u957f\u66f2\u7ebf\uff1b<\/p>\n

(b) 14\u5929\u65f6\u4e0d\u540c\u6cbb\u7597\u540e\u6bcf\u7ec4\u7684\u5e73\u5747\u80bf\u7624\u8d28\u91cf\uff1b<\/p>\n

(c) \u5404\u79cd\u6cbb\u7597\u540e\u572824\u5c0f\u65f6\u4ece\u5c0f\u9f20\u4f53\u5185\u6536\u96c6\u7684\u80bf\u7624\u5207\u7247H&E\u67d3\u8272\uff1b<\/p>\n

(d) \u5404\u79cd\u6cbb\u7597\u540e\u572824\u5c0f\u65f6\u4ece\u5c0f\u9f20\u4f53\u5185\u6536\u96c6\u7684\u80bf\u7624\u5207\u7247TUNTL\u67d3\u8272\u3002<\/p>\n

\u56fe6 \u9759\u8109\u6ce8\u5c04\u540ePFCE @ THPPpf-<\/sub>PEG\u7684\u4f53\u5185\u957f\u671f\u6bd2\u6027<\/strong><\/p>\n

\"\"<\/p>\n

(a) 1\uff0c3\uff0c7\u548c14\u5929\u6ce8\u5c04\u540e\u809d\u6216\u80be\u529f\u80fd\u6807\u5fd7\u7269\u4e19\u6c28\u9178\u6c28\u57fa\u8f6c\u79fb\u9176\uff1b<\/p>\n

(b) 1\uff0c3\uff0c7\u548c14\u5929\u6ce8\u5c04\u540e\u809d\u6216\u80be\u529f\u80fd\u6807\u5fd7\u7269\u5929\u51ac\u6c28\u9178\u6c28\u57fa\u8f6c\u79fb\u9176\uff1b<\/p>\n

(c) 1\uff0c3\uff0c7\u548c14\u5929\u6ce8\u5c04\u540e\u809d\u6216\u80be\u529f\u80fd\u6807\u5fd7\u7269\u5929\u51ac\u6c28\u9178\u6c28\u57fa\u8f6c\u79fb\u9176\u8840\u5c3f\u7d20\u6c2e\uff1b<\/p>\n

(d) 1\uff0c3\uff0c7\u548c14\u5929\u6ce8\u5c04\u540e\u6d89\u53ca\u767d\u8840\u7ec6\u80de\u8840\u6db2\u6c34\u5e73\u7684\u8840\u6db2\u5e38\u89c4\uff1b<\/p>\n

(e) 1\uff0c3\uff0c7\u548c14\u5929\u6ce8\u5c04\u540e\u6d89\u53ca\u7ea2\u8840\u7ec6\u80de\u8840\u6db2\u6c34\u5e73\u7684\u8840\u6db2\u5e38\u89c4\uff1b<\/p>\n

(f) 1\uff0c3\uff0c7\u548c14\u5929\u6ce8\u5c04\u540e\u6d89\u53ca\u5e73\u5747\u7ea2\u7ec6\u80de\u4f53\u79ef\u8840\u6db2\u6c34\u5e73\u7684\u8840\u6db2\u5e38\u89c4\uff1b<\/p>\n

(g) 1\uff0c3\uff0c7\u548c14\u5929\u6ce8\u5c04\u540e\u6d89\u53ca\u5206\u8840\u5668\u8840\u6db2\u6c34\u5e73\u7684\u8840\u6db2\u5e38\u89c4\uff1b<\/p>\n

(h) 1\uff0c3\uff0c7\u548c14\u5929\u6ce8\u5c04\u540e\u6d89\u53ca\u8840\u5c0f\u677f\u8840\u6db2\u6c34\u5e73\u7684\u8840\u6db2\u5e38\u89c4\uff1b<\/p>\n

(i) 1\uff0c3\uff0c7\u548c14\u5929\u6ce8\u5c04\u540e\u6d89\u53ca\u8840\u7ea2\u86cb\u767d\u8840\u6db2\u6c34\u5e73\u7684\u8840\u6db2\u5e38\u89c4\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u672c\u6587\u4e2d\u62a5\u9053\u4e86\u4e00\u79cd\u6c1f\u5316\u7684\u7eb3\u7c73\u5171\u4ef7\u6709\u673a\u805a\u5408\u7269(THPPpf<\/sub>\u2013PEG)\uff0c\u7814\u7a76\u53d1\u73b0\u5176\u5177\u6709\u4f18\u5f02\u7684\u751f\u7406\u7a33\u5b9a\u6027\uff0c\u56e0\u4e3a\u5b9e\u73b0\u4e86\u5168\u6c1f-15-\u51a0-5-\u919a(PFCE)\u7684\u9ad8\u6548\u8d1f\u8f7d\u3002\u6240\u5236\u5907\u7684PFCE@THPPpf<\/sub>\u2013PEG\u4e0d\u4ec5\u53ef\u4ee5\u4f5c\u4e3a\u7eb3\u7c73\u6c27\u6c14\u68ad\uff0c\u8fd8\u662f\u9ad8\u6548\u7684\u5149\u52a8\u529b\u5242\u3002PFCE@THPPpf<\/sub>\u2013PEG\u53ef\u4ee5\u5b9e\u73b0\u5728\u80ba\u90e8\u7684\u6c27\u6c14\u8d1f\u8f7d\uff0c\u5e76\u8fdb\u800c\u5c06\u6c27\u6c14\u91ca\u653e\u5230\u80bf\u7624\u4e2d\u3002\u5728660\u7eb3\u7c73\u6fc0\u5149\u7167\u5c04\u4e0b\uff0c\u83b7\u5f97\u4e86\u4f18\u5f02\u7684\u80bf\u7624\u5149\u52a8\u529b\u6cbb\u7597\u6548\u679c\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aCovalent Organic Polymers Based on Fluorinated Porphyrin as Oxygen Nanoshuttles for Tumor Hypoxia Relief and Enhanced Photodynamic Therapy\u00a0<\/a>\u00a0(Adv. Mater. 2018, DOI: 10.1002\/adfm.201804901)<\/strong><\/p>\n

\u3010\u56e2\u961f\u7c7b\u4f3c\u6587\u732e\u3011<\/strong><\/p>\n

Min Gao, Chao Liang, Xuejiao Song, Qian Chen, Qiutong Jin, Chao Wang, and\u00a0Zhuang Liu<\/strong>*. \u201cErythrocyte Membrane-Enveloped Perfluorocarbon as Nanoscale Artificial Red Blood Cells to Relieve Tumor Hypoxia and Enhance Cancer Radiotherapy\u201d Adv. Mater., 29(35), 1701429 (2017)\u261e<\/a><\/p>\n

Guosheng Song, Chenghong Ji, Chao Liang, Xuejiao Song, Xuan Yi, Ziliang Dong, Kai Yang, and\u00a0Zhuang Liu<\/strong>*. \u201cTaOx Decorated Perfluorocarbon Nanodroplets as Oxygen Reservoirs to Overcome Tumor Hypoxia and Enhance Cancer Radiotherapy\u201d Biomaterials, 112, 257-63 (2017)\u00a0\u261e<\/a><\/p>\n

Xuejiao Song, Liangzhu Feng, Chao Liang, Kai Yang, and\u00a0Zhuang Liu<\/strong>*. \u201cUltrasound Triggered Tumor Oxygenation with Oxygen-Shuttle Nanoperfluorocarbon to Overcome Hypoxia-Associated Resistance in Cancer Therapies\u201d Nano Lett., 16, 6145\u20136153(2016)\u00a0\u261e<\/a><\/p>\n

Guosheng Song, Chao Liang, Xuan Yi, Qi Zhao, Liang Cheng, Kai Yang, and\u00a0Zhuang Liu<\/strong>*., \u201cPerfluorocarbon Loaded Hollow Bi2Se3 Nanoparticles for Timely Supply of Oxygen under Near-Infrared Light to Enhance Radiotherapy of Cancer\u201d Adv. Mater., 28, 2716\u20132723 (2016)\u00a0\u261e<\/a><\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u751f\u7269\u5b66\u672f\u7ec4biotech\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u5ba1\u6838\u6574\u7406\u3002<\/p>\n

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