{"id":148292,"date":"2018-08-01T14:00:29","date_gmt":"2018-08-01T06:00:29","guid":{"rendered":"\/\/m.iemloyee.com\/?p=148292"},"modified":"2018-08-01T16:34:25","modified_gmt":"2018-08-01T08:34:25","slug":"%e5%a4%8d%e6%97%a6%e5%a4%a7%e5%ad%a6jacs%ef%bc%9a%e5%8d%95%e9%a2%97%e7%b2%92%e7%ba%a7%e5%88%ab%e7%a2%b3%e5%92%8c%e4%ba%8c%e6%b0%a7%e5%8c%96%e7%a1%85%e7%a9%ba%e9%97%b4%e5%88%86%e7%a6%bb%e7%9a%84","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=148292","title":{"rendered":"\u590d\u65e6\u5927\u5b66JACS\uff1a\u5355\u9897\u7c92\u7ea7\u522b\u78b3\u548c\u4e8c\u6c27\u5316\u7845\u7a7a\u95f4\u5206\u79bb\u7684\u975e\u5bf9\u79f0\u4e24\u4eb2\u6027\u4ecb\u5b54\u7eb3\u7c73\u9897\u7c92"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

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\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u4e2d\u56fd\u590d\u65e6\u5927\u5b66<\/strong>\u7684\u8d75\u5929\u806a\u535a\u58eb\u7814\u7a76\u751f\uff08\u7b2c\u4e00\u4f5c\u8005\uff09<\/strong>\u7b49\u4eba\uff0c\u5728\u8d75\u4e1c\u5143\u9662\u58eb\u548c\u674e\u6653\u6c11\u7814\u7a76\u5458\uff08\u5171\u540c\u901a\u8baf\uff09<\/strong>\u7684\u6307\u5bfc\u4e0b\uff0c\u901a\u8fc7\u8868\u9762\u7535\u8377\u8bf1\u5bfc\u9009\u62e9\u6027\u751f\u957f\u7684\u65b9\u6cd5\u5236\u5907\u4e86Fe3<\/sub>O4<\/sub>@mC&mSiO2<\/sub>\u53cc\u4ecb\u5b54\u4e0d\u5bf9\u79f0\u7eb3\u7c73\u9897\u7c92\u3002\u8be5\u7eb3\u7c73\u9897\u7c92\u5728\u5355\u9897\u7c92\u7ea7\u522b\u4e0a\u5b9e\u73b0\u4e86\u78b3\u548c\u4e8c\u6c27\u5316\u7845\u5b8c\u5168\u5206\u79bb\u3002\u5e76\u4e14\u78b3\uff08\u758f\u6c34\uff09\u548c\u4e8c\u6c27\u5316\u7845\uff08\u4eb2\u6c34\uff09\u7aef\u7684\u5c3a\u5bf8\u6bd4\u4f8b\u53ef\u4ee5\u7cbe\u786e\u63a7\u5236\uff0c\u4f7f\u5f97\u6b64\u7eb3\u7c73\u9897\u7c92\u4f5c\u4e3a\u201c\u56fa\u4f53\u8868\u9762\u6d3b\u6027\u5242\u201d\u5177\u5907\u4f18\u79c0\u53ef\u8c03\u7684\u5fae\u4e73\u6db2\u7a33\u5b9a\u80fd\u529b\u3002\u5728\u8be5\u975e\u5bf9\u79f0\u7ed3\u6784\u4e24\u7aef\u9009\u62e9\u6027\u8d1f\u8f7d\u4e0d\u540c\u50ac\u5316\u5242\u540e\uff0c\u8be5\u7eb3\u7c73\u9897\u7c92\u8868\u73b0\u51fa\u4f18\u79c0\u7684\u50ac\u5316\u6027\u80fd\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201c<\/strong>Spatial Isolation of Carbon and Silica in a Single Janus Mesoporous Nanoparticle with Tunable Amphiphilicity<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Journal of the American Chemical Society<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe<\/strong> 1 <\/strong>\u6240\u5236\u5907\u7684\u78b3<\/strong>\/<\/strong>\u4e8c\u6c27\u5316\u7845\u5b8c\u5168\u5206\u79bb<\/strong>Fe3<\/sub>O4<\/sub>@mC&mSiO2<\/sub><\/strong>\u975e\u5bf9\u79f0\u7eb3\u7c73\u9897\u7c92\u7684\u5408\u6210\u793a\u610f\u56fe\u53ca\u5176\u7ed3\u6784\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09Fe3<\/sub>O4<\/sub>@mC&mSiO2<\/sub>\u4e0d\u5bf9\u79f0\u7eb3\u7c73\u9897\u7c92\u7684\u5408\u6210\u8def\u5f84\uff1b<\/p>\n

\uff08B-E\uff09\u4e0d\u540c\u653e\u5927\u500d\u6570\u7684\u4e0d\u5bf9\u79f0\u7eb3\u7c73\u9897\u7c92\u7684\u626b\u63cf\u548c\u900f\u5c04\u7535\u955c\u56fe\u50cf\uff1b<\/p>\n

\uff08F\uff0cG\uff09\u6240\u5236\u5907\u7684\u4e0d\u5bf9\u79f0\u7eb3\u7c73\u9897\u7c92\u7684\u6c2e\u6c14\u7b49\u6e29\u5438\u8131\u9644\u66f2\u7ebf\u53ca\u5b54\u5f84\u5206\u5e03\u56fe\uff1b<\/p>\n

\uff08H\uff09\u6240\u5236\u5907\u7684\u4e0d\u5bf9\u79f0\u7eb3\u7c73\u9897\u7c92\u7684\u5143\u7d20Mapping\u56fe\u3002<\/p>\n

\u56fe<\/strong> 2 <\/strong>\u8868\u9762\u7535\u8377\u8bf1\u5bfc\u9009\u62e9\u6027\u751f\u957f<\/strong>PDA<\/strong>\u5f62\u6210\u53cc\u4ecb\u5b54<\/strong>Fe3<\/sub>O4<\/sub>@mC<\/strong>\uff06<\/strong>mSiO2<\/sub> <\/strong>\u975e\u5bf9\u79f0\u7ed3\u6784\u4ecb\u5b54\u7eb3\u7c73\u9897\u7c92\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong> 3 <\/strong>\u5177\u6709\u4e0d\u540c\u4eb2\u6c34\u7aef\u5c3a\u5bf8\u7684<\/strong>Fe3<\/sub>O4<\/sub>@mC<\/strong>\uff06<\/strong>mSiO2<\/sub><\/strong>\u975e\u5bf9\u79f0\u7eb3\u7c73\u9897\u7c92\u7684<\/strong>TEM<\/strong>\u56fe\u50cf\u53ca\u5176\u4e73\u6db2\u7a33\u5b9a\u80fd\u529b\u7814\u7a76<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A-H\uff09\u5177\u6709\u4e0d\u540c\u4eb2\u6c34\u7aef\uff08mSiO2<\/sub>\u68d2\uff09\u957f\u5ea6\u7684Fe3<\/sub>O4<\/sub>&mSiO2<\/sub>\u548cFe3<\/sub>O4<\/sub>@mC&mSiO2<\/sub>\u7eb3\u7c73\u9897\u7c92\u7684TEM\u56fe\u50cf\uff1a(A, E) 400 nm, (B, F) 200 nm, (C, G) 100 nm, (D, H), 50 nm\uff1b<\/p>\n

\uff08I\uff09\u4e0d\u540c\u7eb3\u7c73\u9897\u7c92\u7a33\u5b9a\u7684\u6c34\/\u7532\u82ef\u5fae\u4e73\u6db2\u7684\u7167\u7247\uff1b<\/p>\n

\uff08J\uff0cK\uff09Fe3<\/sub>O4<\/sub>@mC&mSiO2<\/sub>-400\u7eb3\u7c73\u9897\u7c92\u7a33\u5b9a\u7684\u5fae\u4e73\u6db2\u7684\u5149\u5b66\u7167\u7247\u548c\u8367\u5149\u67d3\u8272\u7167\u7247\u3002<\/p>\n

\u56fe<\/strong> 4 Pt\/<\/strong>Fe3<\/sub>O4<\/sub>@mC<\/strong>\uff06<\/strong>mSiO2<\/sub> Janus<\/strong>\u7eb3\u7c73\u9897\u7c92\u7684\u7ed3\u6784\u53ca\u5176\u50ac\u5316\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff09\u53cc\u4ecb\u5b54Pt\/Fe3<\/sub>O4<\/sub>@mC\uff06mSiO2<\/sub> \u975e\u5bf9\u79f0\u7ed3\u6784\u7eb3\u7c73\u9897\u7c92\u7684TEM\u56fe\u50cf\uff08\u63d2\u56fe\uff1aPt\u7eb3\u7c73\u9897\u7c92\u7684HRTEM\u56fe\u50cf\uff09\uff1b<\/p>\n

\uff08B\uff0cC\uff09\u53cc\u4ecb\u5b54Pt\/Fe3<\/sub>O4<\/sub>@mC\uff06mSiO2<\/sub> \u975e\u5bf9\u79f0\u7ed3\u6784\u7eb3\u7c73\u9897\u7c92\u7684\u6697\u89c6\u573aTEM\u56fe\u50cf\u53ca\u5143\u7d20Mapping\u56fe\uff1b<\/p>\n

\uff08D\uff09\u4e73\u6db2\u50ac\u5316\u8fd8\u539f\u5bf9\u785d\u57fa\u82ef\u7532\u919a\u8fc7\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08E\uff0cF\uff09\u4e0d\u540c\u7ed3\u6784\u7eb3\u7c73\u9897\u7c92\u50ac\u5316\u6548\u679c\u5bf9\u6bd4\u53ca\u53cc\u4ecb\u5b54Pt\/Fe3<\/sub>O4<\/sub>@mC\uff06mSiO2<\/sub> \u975e\u5bf9\u79f0\u7ed3\u6784\u591a\u6b21\u5faa\u73af\u50ac\u5316\u6027\u80fd\u3002<\/p>\n

\u56fe<\/strong> 5 <\/strong>\u57fa\u4e8e\u4e73\u6db2\u50ac\u5316\u7684\u7ea7\u8054\u53cd\u5e94\u7684\u793a\u610f\u56fe\u53ca\u50ac\u5316\u6027\u80fd\u7814\u7a76<\/strong><\/p>\n

\"\"<\/p>\n

\uff08A\uff0cB\uff09\u53cc\u4ecb\u5b54Pt\/Fe3<\/sub>O4<\/sub>@mC\uff06mSiO2<\/sub>\/NH2<\/sub>\u975e\u5bf9\u79f0\u7ed3\u6784\u7eb3\u7c73\u590d\u5408\u7269\u4e73\u6db2\u50ac\u5316\u7684\u7ea7\u8054\u53cd\u5e94\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08C\uff09\u4e0d\u540c\u7ed3\u6784\u7eb3\u7c73\u9897\u7c92\u50ac\u5316\u6548\u679c\u5bf9\u6bd4\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u672c\u6587\u9996\u6b21<\/strong>\u8bbe\u8ba1\u548c\u5408\u6210\u4e86\u5747\u5300\u53cc\u4ecb\u5b54Fe3<\/sub>O4<\/sub>@mC\uff06mSiO2<\/sub> \u975e\u5bf9\u79f0\u7eb3\u7c73\u7c92\u5b50\u4f5c\u4e3a\u201c\u78c1\u6027\u56fa\u4f53\u8868\u9762\u6d3b\u6027\u5242\u201d\uff0c\u5b9e\u73b0\u4e86\u5355\u9897\u7c92\u5c42\u9762\u7684\u78b3\u548c\u4e8c\u6c27\u5316\u7845\u7684\u7a7a\u95f4\u7edd\u5bf9\u5206\u79bb\u3002\u8be5\u201c\u56fa\u4f53\u8868\u9762\u6d3b\u6027\u5242\u201d\u75311D\u4ecb\u5b54SiO2<\/sub>\u7eb3\u7c73\u68d2\u548c\u7d27\u5bc6\u8fde\u63a5\u4ecb\u5b54Fe3<\/sub>O4<\/sub>@mC\u78c1\u6027\u7eb3\u7c73\u7403\u7ec4\u6210\u3002\u53ef\u4ee5\u901a\u8fc7\u8c03\u8282SiO2<\/sub>\u7eb3\u7c73\u68d2\u7684\u957f\u5ea6\u548cmC\u5c42\u7684\u539a\u5ea6\u5b9e\u73b0\u5bf9\u975e\u5bf9\u79f0\u7ed3\u6784\u4e24\u7aef\u4eb2\u758f\u6c34\u6bd4\u4f8b\u7684\u8c03\u8282\u3002\u5728\u78c1\u573a\u4e0b\uff0c\u8be5\u201c\u56fa\u4f53\u8868\u9762\u6d3b\u6027\u5242\u201d\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u53ef\u56de\u6536\u6027\u3002\u53e6\u5916\uff0c\u8be5\u975e\u5bf9\u79f0\u7ed3\u6784\u7eb3\u7c73\u7c92\u5b50\u7684\u4e24\u7aef\u53ef\u4ee5\u5206\u522b\u8fdb\u884c\u4e0d\u540c\u5b98\u80fd\u5316\uff0c\u4ece\u800c\u4f7f\u4e24\u7aef\u5177\u6709\u4e0d\u540c\u7684\u50ac\u5316\u529f\u80fd\uff0c\u5728\u786e\u4fdd\u9ad8\u6548\u7684\u4e73\u6db2\u7a33\u5b9a\u80fd\u529b\u7684\u524d\u63d0\u4e0b\uff0c\u5b9e\u73b0\u9ad8\u6548\u7684\u6c34-\u6cb9\u53cc\u76f8\u754c\u9762\u50ac\u5316\u6548\u7387\u3002\u8be5\u8bba\u6587\u4e0d\u4ec5\u4e3a\u65b0\u578b\u975e\u5bf9\u79f0\u6750\u6599\u7684\u8bbe\u8ba1\u5408\u6210\u63d0\u4f9b\u4e86\u65b0\u7684\u7814\u7a76\u601d\u8def\uff0c\u6240\u5f00\u53d1\u7684\u53ef\u8c03\u4eb2\u758f\u6c34\u6bd4\u7684\u65b0\u578b\u975e\u5bf9\u79f0\u7ed3\u6784\u201c\u56fa\u4f53\u8868\u9762\u6d3b\u6027\u5242\u201d\u5728\u50ac\u5316\u3001\u8bca\u65ad\u3001\u836f\u7269\u8f93\u9001\u3001\u50a8\u80fd\u3001\u4f20\u611f\u53ca\u73af\u5883\u4fee\u590d\u7b49\u9886\u57df\u5177\u6709\u6bd4\u8f83\u5927\u6f5c\u529b\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5<\/strong>Spatial Isolation of Carbon and Silica in a Single Janus Mesoporous Nanoparticle with Tunable Amphiphilicity<\/a><\/strong>\uff08JACS, 2018, DOI: 10.1021\/jacs.8b06127\uff09\u3002<\/p>\n

\u3010\u56e2\u961f\u76f8\u5173\u7814\u7a76\u5de5\u4f5c\u603b\u7ed3\u3011<\/strong><\/p>\n

\u5728\u8d75\u4e1c\u5143\u9662\u58eb\u7684\u5e26\u9886\u4e0b\uff0c\u674e\u6653\u6c11\u7814\u7a76\u5458\u81ea2014\u5e74\u5f00\u59cb\u4ece\u4e8b\u975e\u5bf9\u79f0\u7ed3\u6784\u7eb3\u7c73\u6750\u6599\u7684\u7814\u7a76\uff0c\u9996\u6b21\u53d1\u5c55\u4e86\u4ecb\u5b54\u5404\u5411\u5f02\u6027\u751f\u957f\u7b56\u7565\u5e76\u5e94\u4e8e\u975e\u5bf9\u79f0\u7ed3\u6784\u7684\u53ef\u63a7\u5408\u6210\u4e2d\uff0c\u5728\u6b64\u57fa\u7840\u4e0a\u5148\u540e\u5408\u6210\u4e86\u4e00\u7cfb\u5217\u975e\u5bf9\u79f0\u4ecb\u5b54\u7eb3\u7c73\u6750\u6599\uff0c\u6bd4\u5982\u57fa\u4e8e\u7acb\u65b9\u4ecb\u89c2\u7ed3\u6784\u5404\u5411\u5f02\u6027\u751f\u957f\u7684Janus\u7ed3\u6784\uff08J. Am. Chem. Soc., 2014, 136, 15086-15092\uff09\u548c\u504f\u5fc3\u4e2d\u7a7a\u5355\u5f00\u53e3\u7ed3\u6784\uff08J. Am. Chem. Soc. , 2015, 137, 5903\u20135906\uff09\u3001\u57fa\u4e8e\u4e8c\u7ef4\u516d\u65b9\u7ed3\u6784\u5404\u5411\u5f02\u6027\u751f\u957f\u7684\u4e24\u5d4c\u6bb5\u3001\u4e09\u5d4c\u6bb5\u975e\u5bf9\u79f0\u7ed3\u6784\u590d\u5408\u4ecb\u5b54\u7eb3\u7c73\u6750\u6599\uff08Adv. Mater., 2017, 1701652\uff09\u7b49\u3002\u7531\u4e8e\u5176\u72ec\u7279\u7684\u7ed3\u6784\u7279\u70b9\uff0c\u6240\u5236\u5907\u7684\u975e\u5bf9\u79f0\u7ed3\u6784\u7eb3\u7c73\u9897\u7c92\u5728\u591a\u5ba2\u4f53\u5206\u5b50\u7684\u5171\u8d1f\u8f7d\u548c\u8f93\u8fd0\u3001\u836f\u7269\u63a7\u5236\u91ca\u653e\u3001\u4e73\u6db2\u50ac\u5316\u7b49\u9886\u57df\u4e2d\u8868\u73b0\u51fa\u826f\u597d\u7684\u5e94\u7528\u524d\u666f\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1<\/strong>tougao@cailiaoren.com<\/strong>\u3002<\/p>\n

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