{"id":146730,"date":"2018-07-21T06:30:49","date_gmt":"2018-07-20T22:30:49","guid":{"rendered":"\/\/m.iemloyee.com\/?p=146730"},"modified":"2018-07-20T22:47:17","modified_gmt":"2018-07-20T14:47:17","slug":"adv-energy-mater-%e5%af%b9%e8%b6%85%e5%b0%8f%e9%87%91%e7%ba%b3%e7%b1%b3%e9%a2%97%e7%b2%92%e5%82%ac%e5%8c%96%e5%89%82%e8%bf%9b%e8%a1%8c%e8%a1%a8%e9%9d%a2%e8%83%ba%e4%bf%ae%e9%a5%b0%e6%8f%90%e9%ab%98","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=146730","title":{"rendered":"Adv. Energy Mater.: \u5bf9\u8d85\u5c0f\u91d1\u7eb3\u7c73\u9897\u7c92\u50ac\u5316\u5242\u8fdb\u884c\u8868\u9762\u80fa\u4fee\u9970\u63d0\u9ad8\u7535\u5316\u5b66CO2\u8fd8\u539f\u6027\u80fd"},"content":{"rendered":"

\u3010\u5f15\u8a00<\/strong>\u3011<\/p>\n

\u7535\u5316\u5b66CO2<\/sub>\u8fd8\u539f\u53ef\u7528\u4e8e\u53ef\u518d\u751f\u80fd\u6e90\u50a8\u5b58\u548c\u7f13\u89e3\u5168\u7403\u6c14\u5019\u53d8\u5316\uff0c\u662f\u4e00\u79cd\u6709\u524d\u666f\u548c\u53ef\u6301\u7eed\u7684\u91cd\u8981\u65b9\u6cd5\uff0c\u4e5f\u662f\u5f53\u4eca\u4e16\u754c\u8303\u56f4\u5185\u7814\u7a76\u7684\u70ed\u70b9\u4e4b\u4e00\u3002\u7136\u800c\uff0c\u8be5\u53cd\u5e94\u5177\u6709\u4e00\u7cfb\u5217\u4e0d\u8db3\u4e4b\u5904\uff0c\u5982CO2<\/sub>\u6d3b\u5316\u6240\u9700\u8981\u7684\u8fc7\u7535\u4f4d\u8f83\u9ad8\u3001\u590d\u6742\u7684\u53cd\u5e94\u8def\u5f84\u4ee5\u53ca\u526f\u53cd\u5e94\u6790\u6c22\u53cd\u5e94\uff0c\u4f7f\u5176\u9762\u4e34\u5de8\u5927\u7684\u6311\u6218\uff1b\u5176\u4e2d\u53d1\u5c55\u9ad8\u6d3b\u6027\u3001\u9ad8\u7a33\u5b9a\u6027\u50ac\u5316\u5242\u662f\u89e3\u51b3\u8fd9\u4e9b\u95ee\u9898\u7684\u5173\u952e\u6027\u4e00\u6b65\u3002\u8d85\u5c0f\u91d1\u7eb3\u7c73\u9897\u7c92\u56e0\u9ad8\u8d28\u91cf\u6d3b\u6027\u53d7\u5230\u7814\u7a76\u8005\u7684\u5e7f\u6cdb\u9752\u7750\uff0c\u4f46\u4e30\u5bcc\u7684\u4f4e\u914d\u4f4d\u4f4d\u70b9\u5bfc\u81f4\u5176\u4ea7\u7269\u9009\u62e9\u6027\u8f83\u5dee\uff0c\u5728\u4e00\u5b9a\u7a0b\u5ea6\u4e0a\u9650\u5236\u4e86\u5176\u5b9e\u9645\u5e94\u7528\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb<\/strong>\u3011<\/p>\n

\u8fd1\u65e5\uff0c\u6765\u81ea\u6fb3\u5927\u5229\u4e9a\u4f0d\u4f26\u8d21\u5927\u5b66<\/strong>Gordon G. Wallace<\/strong>\u6559\u6388\u4e0e\u738b\u5f69\u4e91\u535a\u58eb\u8bfe\u9898\u7ec4<\/strong>\u91c7\u7528\u4e00\u79cd\u7b80\u6613\u53ca\u65e0\u8868\u9762\u6d3b\u6027\u5242\u7684\u6e7f\u5316\u5b66\u6cd5\u6210\u529f\u5730\u5c06\u8d85\u5c0f\u91d1\u7eb3\u7c73\u9897\u7c92\u8d1f\u8f7d\u4e8e\u8fd8\u539f\u77f3\u58a8\u70ef\uff08rGO\uff09\uff0c\u5e76\u901a\u8fc7\u8868\u9762\u80fa\u5206\u5b50\u4fee\u9970\uff0c\u6210\u529f\u5236\u5907\u51fa\u4e00\u79cd\u65b0\u578b\u50ac\u5316\u5242\uff0c\u6539\u5584\u5176\u5728\u7535\u5316\u5b66CO2<\/sub>\u8fd8\u539f\u4e2d\u7684\u6027\u80fd\u3002\u5b9e\u9a8c\u7ed3\u679c\u663e\u793a\uff0c\u5728\u9002\u5b9c\u7684\u8fc7\u7535\u4f4d\uff08450-600 mV\uff09\u4e0b\uff0crGO-Au\u590d\u5408\u7269\u5728CO2<\/sub>-CO\u7684\u8f6c\u5316\u4e2d\u8868\u73b0\u51fa\u4e86\u8f83\u9ad8\u7684\u91d1\u6bd4\u8d28\u91cf\u6d3b\u6027\uff08><\/strong>100Ag\u2212<\/sup><\/strong>1<\/sup>\uff09\u53ca\u826f\u597d\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff0832-60%\uff09\uff1b\u5bf9\u5176\u8fdb\u884c\u8868\u9762\u80fa\u4fee\u9970\u540e\uff0c\u8be5\u6548\u7387\u53ef\u63d0\u5347\u81f359-75%\uff0c\u540c\u65f6\u4fdd\u6301\u5176\u9ad8\u8d28\u91cf\u6d3b\u6027\u3002\u672c\u6587\u4e2d\u4e5f\u62a5\u9053\u4e86\u80fa\u7ed3\u6784\u4f9d\u8d56\u6027\u6548\u5e94\uff1a\u7ebf\u6027\u80fa\u5206\u5b50\u4fc3\u8fdbCO\u5f62\u6210\uff0c\u800c\u652f\u5316\u591a\u80fa\u5206\u5b50\u5219\u6291\u5236\u5176\u751f\u6210\uff1b\u968f\u7740\u70f7\u57fa\u94fe\u957f\u5ea6\u7684\u4e0d\u65ad\u589e\u52a0\uff0c\u7ebf\u6027\u80fa\u5206\u5b50\u7684\u4fc3\u8fdb\u4f5c\u7528\u4e0d\u65ad\u589e\u5f3a\u3002\u8fd9\u79cd\u6548\u5e94\u53ef\u80fd\u6e90\u4e8e\u91d1\u7eb3\u7c73\u9897\u7c92\u4e0a\u4f4e\u914d\u4f4d\u4f4d\u70b9\u4e0e\u80fa\u5b98\u80fd\u56e2\u7684\u5f3a\u76f8\u4e92\u4f5c\u7528\u4ee5\u53ca\u5206\u5b50\u6784\u578b\u8bf1\u5bfc\u7684\u91d1\u9897\u7c92\u8868\u9762\u80fa\u5206\u5b50\u7684\u8986\u76d6\u7387\u4f18\u5316\u3002\u535a\u58eb\u751f\u8d75\u52c7\u662f\u7b2c\u4e00\u4f5c\u8005\u3002\u76f8\u5173\u6210\u679c\u4ee5\u9898\u4e3a\u201c<\/strong>Engineering Surface Amine Modifiers of Ultrasmall Gold Nanoparticles Supported on Reduced Graphene Oxide for Improved Electrochemical CO2 <\/sub>Reduction<\/strong>\u201d<\/strong>\u53d1\u8868\u5728Adv. Energy Mater.<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb<\/strong>\u3011<\/p>\n

\u56fe\u4e00<\/strong> \u50ac\u5316\u5242\u8868\u9762\u80fa\u5206\u5b50\u4fee\u9970\u8fc7\u7a0b\u793a\u610f\u56fe\u53ca\u7ed3\u6784\u8868\u5f81\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09rGO-Au\u50ac\u5316\u5242\u8868\u9762\u80fa\u4fee\u9970\u7b80\u56fe<\/p>\n

\uff08b\uff09rGO-Au \u53ca rGO\u7684XRD\u56fe\u8c31<\/p>\n

\uff08c\uff09rGO-Au\u7684SEM\u56fe\u50cf<\/p>\n

\uff08d\uff09\uff08e\uff09\u4e0d\u540c\u653e\u5927\u500d\u6570\u4e0b\uff0crGO-Au\u7684TEM\u56fe\u50cf\uff0c\u56fe\uff08e\uff09\u4e2d\u63d2\u56fe\u4e3a\u91d1\u7eb3\u7c73\u9897\u7c92\u7c92\u5f84\u5206\u5e03\u56fe<\/p>\n

\uff08f\uff09\u8d85\u5c0f\u91d1\u7eb3\u7c73\u9897\u7c92\u7684HR-TEM\u56fe\u50cf<\/p>\n

\uff08g\uff09\u8d85\u5c0f\u91d1\u7eb3\u7c73\u9897\u7c92\u7684HAADF-STEM\u56fe\u50cf<\/p>\n

\u56fe\u4e8c<\/strong> \u50ac\u5316\u5242\u8868\u9762\u80fa\u4fee\u9970\u4e0b\u7684\u8c31\u56fe\u5206\u6790<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09rGO-Au\u53ca\u4e94\u79cd\u4e0d\u540c\u80fa\u4fee\u9970\u4e0brGO-Au\u7684Raman\u8c31\u56fe<\/p>\n

\uff08b\uff09rGO-Au\u53ca\u4e94\u79cd\u4e0d\u540c\u80fa\u4fee\u9970\u4e0brGO-Au\u7684FTIR\u8c31\u56fe<\/p>\n

\uff08c\uff09rGO-Au, Au-EDA, \u53ca Au-OLA\u7684Au4f XPS\u8c31\u56fe<\/p>\n

\uff08d\uff09rGO-Au, Au-EDA, \u53ca Au-OLA\u7684C1s XPS\u8c31\u56fe<\/p>\n

\u56fe\u4e09<\/strong> \u4e0d\u540c\u7535\u4f4d\u4e0b<\/strong>rGO-Au<\/strong>\u53ca<\/strong>Au-<\/strong>\u80fa\u50ac\u5316\u5242\u7684<\/strong>CO2<\/sub><\/strong>\u7535\u8fd8\u539f\u6027\u80fd\u5206\u6790<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u5728CO2<\/sub>\u9971\u548c\u76840.1M KHCO3<\/sub>\u6eb6\u6db2\u4e2d\uff0crGO, rGO-EDA, rGO-Au, \u53caAu-\u80fa\u7684\u7ebf\u6027\u626b\u63cf\u4f0f\u5b89\u66f2\u7ebf<\/p>\n

\uff08b\uff09\u4e0d\u540c\u7535\u4f4d\u4e0b\uff0crGO-Au\u53caAu-\u80fa\u50ac\u5316\u5242\u7684\u51e0\u4f55\u603b\u7535\u6d41\u5bc6\u5ea6\u66f2\u7ebf<\/p>\n

\uff08c\uff09\u4e0d\u540c\u7535\u4f4d\u4e0b\uff0crGO-Au\u53caAu-\u80fa\u50ac\u5316\u5242\u7684CO\u8f6c\u5316\u7387\uff08FECO<\/sub>\uff09\u66f2\u7ebf<\/p>\n

\uff08d\uff09\u4e0d\u540c\u7535\u4f4d\u4e0b\uff0crGO-Au\u53caAu-\u80fa\u50ac\u5316\u5242\u7684CO\u8f6c\u5316\u7535\u6d41\uff08j<\/em>CO<\/sub>\uff09\u66f2\u7ebf<\/p>\n

\uff08e\uff09\u8d1f\u8f7d\u7535\u4f4d\u4e3a-0.7V\u4e0b\uff0cFECO<\/sub> (\u67f1)\u53ca j<\/em>CO<\/sub> (\u5706)\u56fe\u50cf<\/p>\n

\uff08f\uff09\u4e0e\u5df2\u62a5\u9053\u8d35\u91d1\u5c5e\u50ac\u5316\u5242CO\u751f\u6210\u8d28\u91cf\u6d3b\u6027\u7684\u6bd4\u8f83<\/p>\n

\u56fe\u56db<\/strong> \u4e24\u79cd\u4ee3\u8868\u6027\u50ac\u5316\u5242\u7684<\/strong>CO2<\/sub><\/strong>\u7535\u8fd8\u539f\u7a33\u5b9a\u6027\u5206\u6790<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09Au-OLA\u7684\u7a33\u5b9a\u6027\u5206\u6790<\/p>\n

\uff08b\uff09rGO-Au\u7684\u7a33\u5b9a\u6027\u5206\u6790<\/p>\n

\u56fe\u4e94<\/strong> rGO-Au120<\/strong>\u3001<\/strong>rGO-Au120-OLA<\/strong>\u50ac\u5316\u5242\u7684\u7535\u50ac\u5316\u6027\u80fd\u5206\u6790<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\uff08b\uff09\u5728\u7a7a\u6c14\u4e2d120\u5ea6\u52a0\u70ed\u5f62\u6210\u7684\u5927\u5c3a\u5bf8\u91d1\u7eb3\u7c73\u9897\u7c92\uff08rGO-Au120\uff09\u7684TEM\u56fe\u50cf\uff0c\u63d2\u56fe\u4e3a\u91d1\u7eb3\u7c73\u9897\u7c92\u7684\u7c92\u5f84\u5206\u5e03\u56fe<\/p>\n

\uff08c\uff09\u4e0d\u540c\u7535\u4f4d\u4e0b\uff0crGO-Au120\u3001rGO-Au120-OLA\u50ac\u5316\u5242\u7684FECO<\/sub>\u53caFEH2<\/sub>\u66f2\u7ebf<\/p>\n

\uff08d\uff09\u4e0d\u540c\u7535\u4f4d\u4e0b\uff0crGO-Au120\u3001rGO-Au120-OLA\u50ac\u5316\u5242\u7684j<\/em>CO<\/sub>\u66f2\u7ebf<\/p>\n

\u56fe\u516d<\/strong> \u50ac\u5316\u5242<\/strong>rGO-Au-OLA<\/strong>\u5728\u4e0d\u540c\u4e59\u9187\u6d17\u6da4\u6b21\u6570\u4e0b\u7684<\/strong>H2<\/sub><\/strong>\u548c<\/strong>CO<\/strong>\u6cd5\u62c9\u7b2c\u6548\u7387\uff08\u67f1\uff09\u53ca\u603b\u7535\u6d41\u5bc6\u5ea6\uff08\u5706\u70b9\uff09<\/strong><\/p>\n

\"\"<\/p>\n

\u3010\u5c0f\u7ed3<\/strong>\u3011<\/p>\n

\u8be5\u5de5\u4f5c\u901a\u8fc7\u91c7\u7528rGO-\u8f85\u52a9\u6e7f\u5316\u5b66\u6cd5\uff0c\u6210\u529f\u5236\u5907\u51fa\u4e00\u79cd\u53ef\u7528\u4e8e\u7535\u5316\u5b66CO2<\/sub>\u8fd8\u539f\u7684\u8d85\u5c0f\u65e0\u914d\u4f53\u91d1\u7eb3\u7c73\u9897\u7c92\u50ac\u5316\u5242\uff0c\u8be5\u50ac\u5316\u5242\u8868\u73b0\u51fa\u8f83\u9ad8\u7684\u8d28\u91cf\u6d3b\u6027\u3002\u7b80\u5355\u7684\u8868\u9762\u80fa\u5206\u5b50\u4fee\u9970\u660e\u663e\u6291\u5236\u4e86CO2<\/sub>\u7535\u8fd8\u539f\u53cd\u5e94\u4e2d\u4e25\u91cd\u7684\u6790\u6c22\u53cd\u5e94\uff0c\u4fc3\u8fdb\u4e86CO2<\/sub>-CO\u7684\u8f6c\u5316\u3002\u80fa\u5b98\u80fd\u56e2\u4ee5\u53ca\u80fa\u5206\u5b50\u6784\u578b\u5728\u8c03\u8282\u5177\u6709\u4e30\u5bcc\u4f4e\u914d\u4f4d\u4f4d\u70b9\u7684\u8d85\u5c0f\u91d1\u7eb3\u7c73\u9897\u7c92\u7535\u50ac\u5316\u6d3b\u6027\u4e2d\u8d77\u5230\u4e86\u91cd\u8981\u4f5c\u7528\u3002\u5728\u6240\u6709\u7684\u4fee\u9970\u5242\u4e2d\uff0c\u7ebf\u6027\u7684\u6cb9\u80fa\u5206\u5b50\uff08OLA\uff09\u53ef\u80fd\u7531\u4e8e\u5176\u5728\u8d85\u5c0f\u91d1\u7eb3\u7c73\u9897\u7c92\u4e0a\u7684\u6700\u4f18\u5316\u8986\u76d6\u7387\uff0c\u4ece\u800c\u5bf9CO\u7684\u9009\u62e9\u6027\u8fd8\u539f\u8868\u73b0\u51fa\u6700\u6709\u6548\u7684\u4fc3\u8fdb\u4f5c\u7528\u3002\u53e6\u5916\uff0c\u8fd9\u79cd\u80fa\u5206\u5b50\u7684\u4fee\u9970\u6548\u5e94\u4e0e\u7eb3\u7c73\u9897\u7c92\u8868\u9762\u7684\u6d3b\u6027\u4f4d\u70b9\u79cd\u7c7b\u548c\u5bc6\u5ea6\u4e5f\u6709\u5f88\u5927\u5173\u7cfb\uff0c\u5728\u5177\u6709\u6781\u5c11\u91cf\u4f4e\u914d\u4f4d\u4f4d\u70b9\u7684\u8f83\u5927\u91d1\u7eb3\u7c73\u9897\u7c92\u4e0a\uff0c\u80fa\u5206\u5b50\u4fee\u9970\u5e76\u672a\u5c55\u73b0\u51fa\u660e\u663e\u7684\u4fc3\u8fdb\u4f5c\u7528\u3002\u8fd9\u9879\u5de5\u4f5c\u901a\u8fc7\u5728\u5206\u5b50\u6c34\u5e73\u4e0a\u5bf9\u50ac\u5316\u5242\u8fdb\u884c\u8868\u9762\u80fa\u4fee\u9970\uff0c\u63d0\u51fa\u4e86\u4e00\u79cd\u9ad8\u6548\u3001\u9ad8\u9009\u62e9\u6027\u7684CO2<\/sub>\u8fd8\u539f\u7535\u50ac\u5316\u5242\u7684\u8bbe\u8ba1\u65b9\u6848\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Engineering Surface Amine Modifiers of Ultrasmall Gold Nanoparticles Supported on Reduced Graphene Oxide for Improved Electrochemical CO2 <\/sub>Reduction<\/a>\uff08Adv. Energy Mater. 2018, DOI: 10.1002\/aenm.201801400\uff09<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u65b0\u4eba\u7ec4\u9ec4\u654f\u7f16\u8bd1\uff0c\u8d75\u98de\u9f99\u5ba1\u6838\uff0c\u70b9\u6211\u52a0\u5165\u6750\u6599\u4eba\u7f16\u8f91\u90e8<\/a>\u3002<\/p>\n

\u6750\u6599\u6d4b\u8bd5\uff0c\u6570\u636e\u5206\u6790\uff0c\u4e0a<\/strong>\u6d4b\u8bd5\u8c37<\/strong><\/a>\u3002<\/strong><\/p>\n","protected":false},"excerpt":{"rendered":"

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