{"id":145781,"date":"2018-07-13T14:00:23","date_gmt":"2018-07-13T06:00:23","guid":{"rendered":"\/\/m.iemloyee.com\/?p=145781"},"modified":"2018-07-12T12:43:49","modified_gmt":"2018-07-12T04:43:49","slug":"energy-environmental-science-%e5%a4%a9%e7%84%b6%e5%82%ac%e5%8c%96%e5%89%82%e5%8f%af%e8%a7%81%e5%85%89%e5%82%ac%e5%8c%96%e8%bf%98%e5%8e%9fco2","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=145781","title":{"rendered":"Energy &amp; Environmental Science: \u5929\u7136\u50ac\u5316\u5242\u53ef\u89c1\u5149\u50ac\u5316\u8fd8\u539fCO2"},"content":{"rendered":"<p><strong>\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n<p>\u5229\u7528\u534a\u5bfc\u4f53\u53c2\u4e0e\u7684\u5149\u50ac\u5316\u7b56\u7565\u5c06\u6e29\u5ba4\u6c14\u4f53CO<sub>2<\/sub>\u8f6c\u5316\u4e3a\u9ad8\u9644\u52a0\u503c\u71c3\u6599\u7684\u540c\u65f6\u964d\u4f4e\u5176\u542b\u91cf\uff0c\u662f\u89e3\u51b3\u80fd\u6e90\u77ed\u7f3a\u548c\u6e29\u5ba4\u6548\u5e94\u95ee\u9898\u7684\u7406\u60f3\u65b9\u6cd5\u4e4b\u4e00\u3002\u5206\u7ea7\u4e2d\u7a7a\u7ed3\u6784\u5728\u5149\u50ac\u5316\u8fd8\u539fCO<sub>2<\/sub>\u4e2d\u5f97\u5230\u5e7f\u6cdb\u5e94\u7528\uff0c\u7531\u4e8e\u5176\u80fd\u8d4b\u4e88\u5149\u50ac\u5316\u5242\u66f4\u9ad8\u5bc6\u5ea6\u7684\u8868\u9762\u66b4\u9732\u6d3b\u6027\u4f4d\u70b9\u4ee5\u52a0\u901fCO<sub>2<\/sub>\u5438\u9644\uff0c\u964d\u4f4e\u4ece\u4f53\u76f8\u5230\u8868\u9762\u7684\u6269\u6563\u957f\u5ea6\u4ee5\u4fc3\u8fdb\u5149\u751f\u7535\u8377\u8f7d\u6d41\u5b50\u7684\u5206\u79bb\u4ee5\u53ca\u901a\u8fc7\u5185\u90e8\u591a\u5149\u6563\u5c04\u548c\u53cd\u5c04\u63d0\u9ad8\u53ef\u89c1\u5149\u6355\u83b7\u6027\u80fd\u3002\u5177\u6709\u591a\u79cd\u5c3a\u5ea6\u548c\u5206\u7ea7\u5f62\u6001\u7684\u751f\u7269\u6750\u6599\u5f15\u8d77\u4e86\u7814\u7a76\u4eba\u5458\u7684\u6781\u5927\u5174\u8da3\u3002\u5728\u5404\u79cd\u751f\u7269\u6750\u6599\u4e2d\uff0c\u5177\u6709\u5747\u5300\u78b3\u9aa8\u67b6\u7684\u82b1\u7c89\u7531\u4e8e\u5176\u5927\u5b54\u9699\u4f53\u79ef\u3001\u9ad8\u8868\u9762\u79ef\u548c\u72ec\u7279\u76843D\u7f51\u7edc\u7ed3\u6784\u800c\u88ab\u5e94\u7528\u4e8e\u5404\u79cd\u9886\u57df\u3002\u4e0e\u4f20\u7edf\u7684\u5316\u5b66\u5408\u6210\u76f8\u6bd4\uff0c\u82b1\u7c89\u884d\u751f\u6750\u6599\u7684\u5236\u5907\u8fc7\u7a0b\u4e5f\u66f4\u52a0\u7ecf\u6d4e\u73af\u4fdd\u3002<\/p>\n<p><strong>\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n<p>\u8fd1\u65e5\uff0c<strong>\u9999\u6e2f\u4e2d\u6587\u5927\u5b66\u738b\u4fdd\u5f3a\u6559\u6388\u3001\u6b66\u6c49\u7406\u5de5\u5927\u5b66\u4f59\u5bb6\u56fd\u6559\u6388\u3001\u5e7f\u4e1c\u5de5\u4e1a\u5927\u5b66\u5b89\u592a\u6210\u6559\u6388(\u5171\u540c\u901a\u8baf\u4f5c\u8005)\u7b49<\/strong>\u5236\u5907\u4e86\u4e00\u79cd\u975e\u91d1\u5c5e\u751f\u7269\u6750\u6599\u2014\u2014\u5206\u7ea7\u6539\u6027\u6cb9\u83dc\u82b1\u7c89(TRP)\u4f5c\u4e3a\u53ef\u89c1\u5149\u50ac\u5316\u8fd8\u539fCO<sub>2<\/sub>\u7684\u50ac\u5316\u5242\uff0c\u5e76\u5728<strong>Energy &amp; Environmental Science<\/strong>\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201c<strong>Nature-Based Catalyst for Visible-Light-Driven Photocatalytic CO<sub>2<\/sub> Reduction<\/strong>\u201d\u7684\u7814\u7a76\u8bba\u6587\u3002\u8bba\u6587\u7684\u7b2c\u4e00\u4f5c\u8005\u4e3a\u59dc\u5fd7\u950b\u535a\u58eb\u3002\u6240\u8ff0TRP\u50ac\u5316\u5242\u5728\u4e0d\u4f7f\u7528\u52a9\u50ac\u5316\u5242\u6216\u727a\u7272\u8bd5\u5242\u7684\u60c5\u51b5\u4e0b\uff0c\u4e00\u6c27\u5316\u78b3(CO)\u7684\u751f\u6210\u901f\u7387\u53ef\u8fbe\u5230488.4 \u03bcmol\u00b7h<sup>-1<\/sup>\u00b7g<sup>-1<\/sup>\uff0c\u9009\u62e9\u6027\u53ef\u8fbe\u523098.3%\uff0c420nm\u5904\u91cf\u5b50\u6548\u7387\u8d85\u8fc76.7%\u3002\u4e14TRP\u50ac\u5316\u5242\u7684CO\u751f\u6210\u901f\u7387\u8fdc\u9ad8\u4e8e\u5e38\u89c1\u7684\u5149\u50ac\u5316\u5242\uff0c\u5982g-C<sub>3<\/sub>N<sub>4<\/sub>(16.6\u03bcmol\u00b7h<sup>-1<\/sup>\u00b7g<sup>-1<\/sup>\uff0c\u9ad829.4\u500d)\u548cP25 TiO<sub>2<\/sub> (19.1\u03bcmol\u00b7h<sup>-1<\/sup>\u00b7g<sup>-1<\/sup>\uff0c\u9ad825.6\u500d)\uff0c\u662f\u5df2\u62a5\u9053\u7684\u78b3\u57fa\u5149\u50ac\u5316\u5242\u4e2d\u6700\u9ad8\u7684\u3002\u539f\u4f4d\u5085\u91cc\u53f6\u53d8\u6362\u7ea2\u5916\u5149\u8c31\u5206\u6790\u63ed\u793a\u7532\u9178\u662f\u4e3b\u8981\u7684\u4e2d\u95f4\u4f53\u3002\u4e0a\u8ff0\u5929\u7136\u7684\u53ef\u6301\u7eed\u5149\u50ac\u5316\u5242\u53ef\u4ee5\u4e3a\u8bbe\u8ba1\u5177\u6709\u7a81\u51fa\u7684\u53ef\u89c1\u5149\u9a71\u52a8\u8fd8\u539fCO<sub>2<\/sub>\u6027\u80fd\u7684\u975e\u91d1\u5c5e\u50ac\u5316\u5242\u63d0\u4f9b\u65b0\u7684\u89c6\u89d2\u3002<\/p>\n<p><strong>\u3010\u56fe\u6587\u7b80\u4ecb\u3011<\/strong><\/p>\n<p><strong>\u56fe1 TRP\u9897\u7c92\u7684\u5f62\u8c8c\u8868\u5f81<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-145782\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/1-34.jpg\" alt=\"\" width=\"600\" height=\"401\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/1-34.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/1-34-300x201.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>a-c) TRP\u9897\u7c92\u7684FESEM\u56fe\u50cf\uff1b<\/p>\n<p>d,e) TRP\u9897\u7c92\u7684HAADF-STEM\u56fe\u50cf\uff1b<\/p>\n<p>f) TRP\u9897\u7c92\u7684HRTEM\u56fe\u50cf\uff1b<\/p>\n<p>g) \u5355\u4e2aTRP\u9897\u7c92\u7684FESEM\u56fe\u50cf\u4ee5\u53ca\u76f8\u5e94\u7684\u5143\u7d20\u5206\u5e03\u56fe\u50cf\u3002<\/p>\n<p><strong>\u56fe2 TRP\u9897\u7c92\u7684\u5149\u50ac\u5316\u8fd8\u539fCO<sub>2<\/sub>\u6027\u80fd<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-145783\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/2-30.jpg\" alt=\"\" width=\"600\" height=\"707\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/2-30.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/2-30-255x300.jpg 255w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>a) \u4e0d\u540c\u50ac\u5316\u5242\u4ea7\u751fCO\u548cCH<sub>4<\/sub>\u7684\u6bd4\u8f83\uff1b<\/p>\n<p>b,c) \u4ee5<sup>13<\/sup>CO<sub>2<\/sub>\u540c\u4f4d\u7d20\u4e3a\u78b3\u6e90\u4ea7\u751fCO\/CH<sub>4<\/sub>\u7684GC-MS\u5206\u6790\u3002<\/p>\n<p><strong>\u56fe3 \u4e0d\u540c\u53cd\u5e94\u6761\u4ef6\u4e0b\u7684CO\u4ea7\u751f\u5b9e\u9a8c<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-145784\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/3-31.jpg\" alt=\"\" width=\"600\" height=\"640\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/3-31.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/3-31-281x300.jpg 281w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>a) \u4e0d\u540c\u6e29\u5ea6\u4e0b\u7684CO\u4ea7\u751f\u5b9e\u9a8c\uff1b<\/p>\n<p>b) \u4e0d\u540c\u50ac\u5316\u5242\u542b\u91cf\u4e0b\u7684CO\u4ea7\u751f\u5b9e\u9a8c\uff1b<\/p>\n<p>c) \u4e0d\u540c\u5149\u5bc6\u5ea6\u4e0b\u7684CO\u4ea7\u751f\u5b9e\u9a8c\uff1b<\/p>\n<p>d) \u5355\u8272\u5149\u7167\u5c04\u4e0b\u968f\u6ce2\u957f\u53d8\u5316\u7684TRP\u50ac\u5316\u5242QE\u3002<\/p>\n<p><strong>\u56fe4 TRP\u9897\u7c92\u7684\u539f\u4f4d\u7ea2\u5916\u6d4b\u8bd5<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-145785\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/4-31.jpg\" alt=\"\" width=\"600\" height=\"735\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/4-31.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/4-31-245x300.jpg 245w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>TRP\u50ac\u5316\u5242\u5171\u5438\u9644CO<sub>2<\/sub>\u548cH<sub>2<\/sub>O\u6df7\u5408\u6c14\u6697\u53cd\u5e94\/\u53ef\u89c1\u5149(LED lamp, \u03bb= 420 nm)\u7167\u5c0420, 40, 60 min\u4e0b\u7684\u539f\u4f4dFTIR\u5149\u8c31\u3002<\/p>\n<p><strong>\u56fe5 TRP\u7684CO<sub>2<\/sub>\u5438\u9644\u6027\u80fd\u53ca\u7f3a\u9677\u6001\u6d4b\u8bd5<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-145786\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/5-22.jpg\" alt=\"\" width=\"600\" height=\"416\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/5-22.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/5-22-300x208.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>a) TRP\u548cg-C<sub>3<\/sub>N<sub>4<\/sub>\u7684\u5438\u9644CO<sub>2<\/sub>\u6027\u80fd\u6d4b\u8bd5\uff1b<\/p>\n<p>b) TRP\u548cg-C<sub>3<\/sub>N<sub>4<\/sub>\u7684\u7f3a\u9677\u6001\u6d4b\u8bd5\u3002<\/p>\n<p><strong>\u56fe6 TRP\u7684\u8f7d\u6d41\u5b50\u5206\u79bb\u8fc1\u79fb\u6548\u7387\u6d4b\u8bd5<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-145787\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/6-14.jpg\" alt=\"\" width=\"600\" height=\"734\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/6-14.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/07\/6-14-245x300.jpg 245w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>a) \u5f00\u8def\u7535\u538b\u66f2\u7ebf(\u53ef\u89c1\u5149\u5173\u95ed\u540e\u5f52\u4e00\u5316)\uff1b<\/p>\n<p>b) \u5149\u81f4\u53d1\u5149\u5149\u8c31\uff1b<\/p>\n<p>c) \u4f0f\u5b89\u56fe\uff1b<\/p>\n<p>d) \u8868\u9762\u5149\u7535\u538b\u8c31\u3002<\/p>\n<p><strong>\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n<p>\u7814\u7a76\u4eba\u5458\u5229\u7528\u4f4e\u6210\u672c\u548c\u7b80\u4fbf\u7684\u7b56\u7565\u5236\u5907\u4e86TRP\u751f\u7269\u6750\u6599\uff0c\u5e76\u5c06\u5176\u4f5c\u4e3a\u7528\u4e8e\u65e5\u5149\u9a71\u52a8\u7684\u5149\u50ac\u5316\u8fd8\u539fCO<sub>2<\/sub>\u7684\u975e\u91d1\u5c5e\u50ac\u5316\u5242\u3002TRP\u50ac\u5316\u5242\u72ec\u7279\u7684\u5206\u7ea7\u3001\u4e2d\u7a7a\u548c\u591a\u5b54\u7279\u5f81\u6709\u5229\u4e8e\u5149\u5438\u6536\u3001CO<sub>2<\/sub>\u5206\u5b50\u5438\u9644\u548c\u7535\u8377\u5206\u79bb\uff0c\u4e0e\u5927\u591a\u6570\u62a5\u9053\u7684\u975e\u91d1\u5c5e\u53ef\u89c1\u5149\u9a71\u52a8\u7684\u5149\u50ac\u5316\u5242\u76f8\u6bd4\uff0c\u5177\u6709\u589e\u5f3a\u7684\u5149\u50ac\u5316\u8fd8\u539fCO<sub>2<\/sub>\u6027\u80fd\u3002\u53ef\u4ee5\u8bbe\u60f3\uff0c\u8be5\u6587\u4ecb\u7ecd\u7684\u7b80\u4fbf\u6709\u6548\u7684\u65b9\u6cd5\u4e5f\u53ef\u4ee5\u6269\u5c55\u4e8e\u521b\u9020\u5176\u4ed6\u7528\u4e8e\u5149\u50ac\u5316CO<sub>2<\/sub>\u8fd8\u539f\u7684\u4eff\u751f\u975e\u91d1\u5c5e\u6750\u6599\u4ee5\u751f\u4ea7\u53ef\u6301\u7eed\u71c3\u6599\u3002<\/p>\n<p><strong>\u6587\u732e\u94fe\u63a5\uff1a <a href=\"http:\/\/dx.doi.org\/10.1039\/C8EE01781F\" target=\"_blank\" rel=\"noopener\">Nature-Based Catalyst for Visible-Light-Driven Photocatalytic CO<sub>2<\/sub> Reduction<\/a><\/strong> (<strong>Energy &amp; Environmental Science<\/strong>, 2018, DOI: 10.1039\/C8EE01781F)<\/p>\n<p><strong>\u3010\u901a\u8baf\u4f5c\u8005\u7b80\u4ecb\u3011<\/strong><\/p>\n<p><strong>\u738b\u4fdd\u5f3a\u6559\u6388<\/strong>\uff0c\u9999\u6e2f\u4e2d\u6587\u5927\u5b66\u751f\u547d\u79d1\u5b66\u9662\u6559\u6388\uff0c\u535a\u58eb\u751f\u5bfc\u5e08\u30021979\u5e74\u6bd5\u4e1a\u4e8e\u9999\u6e2f\u4e2d\u6587\u5927\u5b66\u751f\u7269\u7cfb\u5e76\u83b7\u751f\u7269\u5b66\u7855\u58eb\u5b66\u4f4d\uff0c1983\u5e74\u83b7\u7f8e\u56fd\u52a0\u5dde\u5927\u5b66\u5fae\u751f\u7269\u5b66\u535a\u58eb\u5b66\u4f4d\u3002\u73b0\u4efb\u9999\u6e2f\u4e2d\u6587\u5927\u5b66\u73af\u5883\u79d1\u5b66Program\u526f\u4e3b\u4efb\uff0c\u540c\u65f6\u62c5\u4efb\u5e7f\u4e1c\u5de5\u4e1a\u5927\u5b66\u3001\u534e\u5357\u7406\u5de5\u5927\u5b66\u3001\u534e\u4e2d\u5e08\u8303\u5927\u5b66\u3001\u5357\u5f00\u5927\u5b66\u5ba2\u5ea7\u6559\u6388\uff0cJ. Environ. Sci.\u6742\u5fd7\u526f\u4e3b\u7f16\u3001Environ. Geochem. Health \u6742\u5fd7Coordinating Editor, Ecotox. Environ. Safe. \u6742\u5fd7\u7f16\u59d4\u3002\u76ee\u524d\u4ece\u4e8b\u73af\u5883\u5fae\u751f\u7269\u6280\u672f\u4e0e\u5e94\u7528\u53ca\u5176\u5149\u50ac\u5316\u6740\u83cc,\u4ea7\u6c22\u3001\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\u4ee5\u53ca\u5fae\u751f\u7269\u534f\u540c\u4ea7\u6c22\u673a\u7406\u7b49\u65b9\u9762\u7684\u7814\u7a76\uff0c\u5e76\u5728Adv. Mater.,Environ. Sci. Technol., Water Research\u7b49\u671f\u520a\u4e0a\u53d1\u8868\u8bba\u6587200\u4f59\u7bc7\u3002<\/p>\n<p><strong>\u4f59\u5bb6\u56fd\u6559\u6388<\/strong>\uff0c\u6b66\u6c49\u7406\u5de5\u5927\u5b66\u6750\u6599\u590d\u5408\u65b0\u6280\u672f\u56fd\u5bb6\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u5b66\u79d1\u9996\u5e2d\u6559\u6388\u3001\u535a\u5bfc\u3001\u6e56\u5317\u7701\u201c\u695a\u5929\u5b66\u8005\u201d\u8ba1\u5212\u7279\u8058\u6559\u6388\u3001\u65b0\u4e16\u7eaa\u767e\u5343\u4e07\u4eba\u624d\u5de5\u7a0b\u56fd\u5bb6\u7ea7\u4eba\u9009\u3001\u56fd\u5bb6\u6770\u51fa\u9752\u5e74\u57fa\u91d1\u83b7\u5f97\u8005\u3002\u56e2\u961f\u4e3b\u8981\u4ece\u4e8b\u534a\u5bfc\u4f53\u5149\u50ac\u5316\u6750\u6599\u3001\u5149\u50ac\u5316\u5206\u89e3\u6c34\u4ea7\u6c22\u3001\u5149\u50ac\u5316CO<sub>2<\/sub>\u8fd8\u539f\u3001\u5ba4\u5185\u7a7a\u6c14\u51c0\u5316\u7b49\u65b9\u9762\u7684\u7814\u7a76\u5de5\u4f5c\u3002\u56e2\u961f\u5df2\u5728Adv. Mater.\u3001J. Am. Chem. 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