{"id":145180,"date":"2018-07-11T14:00:17","date_gmt":"2018-07-11T06:00:17","guid":{"rendered":"\/\/m.iemloyee.com\/?p=145180"},"modified":"2018-07-10T21:29:30","modified_gmt":"2018-07-10T13:29:30","slug":"%e9%99%88%e6%b5%a9%e9%93%ad%e4%bd%99%e5%ae%b6%e5%9b%bdadv-funct-mater-%e5%8d%95%e5%8e%9f%e5%ad%90%e8%b0%83%e6%8e%a7%e5%8a%a9%e5%8a%9b%e5%85%89%e5%82%ac%e5%8c%96%e5%88%b6%e6%b0%a2","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=145180","title":{"rendered":"\u9648\u6d69\u94ed&\u4f59\u5bb6\u56fdAdv. Funct. Mater. : \u5355\u539f\u5b50\u8c03\u63a7\u52a9\u529b\u5149\u50ac\u5316\u5236\u6c22"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

g-CN\u662f\u4e00\u7c7b\u91cd\u8981\u76842D\u5149\u50ac\u5316\u5242\uff0c\u4f46\u8f83\u4f4e\u7684\u5149\u50ac\u5316\u6548\u7387\u5f71\u54cd\u4e86\u5176\u8fdb\u4e00\u6b65\u7684\u5e94\u7528\uff0c\u5e94\u5f52\u56e0\u4e8e\u5176\u5149\u751f\u8f7d\u6d41\u5b50\u7684\u5229\u7528\u7387\u8f83\u4f4e\uff0c\u5373g-CN\u5c42\u95f4\u7684\u5f31\u8303\u5fb7\u534e\u529b\u4e0d\u5229\u4e8e\u76f8\u90bb\u5c42\u4e4b\u95f4\u7684\u7535\u8377\u8f6c\u79fb\u4ee5\u53ca\u672c\u5f81\u03c0\u5171\u8f6d\u5e73\u9762\u5bfc\u81f4\u65e0\u6548\u7684\u968f\u673a\u9762\u5185\u7535\u8377\u8fc1\u79fb\u3002\u4e3a\u6b64\uff0c\u4ee5\u975e\u91d1\u5c5e\u539f\u5b50\u4ee3\u66ff\u6676\u683c\u539f\u5b50\u5bf9g-CN\u8fdb\u884c\u63ba\u6742\u53ef\u663e\u8457\u62d3\u5c55\u03c0\u5171\u8f6d\u4f53\u7cfb\uff1b\u5e76\u4e14\u5c06\u8fc7\u6e21\u91d1\u5c5e\u539f\u5b50\u5f15\u5165\u03c0\u5171\u8f6d\u5e73\u9762\u7684\u4e09\u89d2\u5f62\u7a7a\u4f4d\u4e2d\u4e5f\u53ef\u4ee5\u6539\u5584g-CN\u7684\u9762\u5185\u7535\u5bfc\u7387\u3002\u4e0a\u8ff0\u7b56\u7565\u6709\u52a9\u4e8e\u6539\u5584\u5e73\u9762\u7535\u8377\u8f6c\u79fb\uff0c\u7136\u800c\uff0c\u4ecd\u672a\u80fd\u6539\u5584g-CN\u7684\u76f8\u90bb\u5c42\u95f4\u7684\u7535\u8377\u8f6c\u79fb\u3002\u5b9e\u9645\u4e0a\uff0c\u63d0\u4f9b\u672c\u5f81\u7684\u9a71\u52a8\u529b\u6765\u5f15\u5bfc\u5c42\u95f4\u548c\u9762\u5185\u7684\u7535\u8377\u8f6c\u79fb\uff0c\u8fdb\u800c\u6709\u6548\u5730\u5c06\u5149\u751f\u7535\u5b50\u5bfc\u5411\u6d3b\u6027\u4f4d\u70b9\uff0c\u8fd9\u4e00\u76ee\u6807\u5341\u5206\u4ee4\u4eba\u671f\u5f85\u3002\u6700\u8fd1\uff0c\u952e\u5408\u4e8eg-CN\u4e0a\u7684\u5355\u4e2d\u5fc3\u91d1\u5c5e\u50ac\u5316\u5242\u5bf9\u4e8e\u8bb8\u591a\u50ac\u5316\u53cd\u5e94\u5747\u663e\u793a\u51fa\u8f83\u9ad8\u7684\u6027\u80fd\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u56fd\u7acb\u53f0\u6e7e\u5927\u5b66\u9648\u6d69\u94ed\u6559\u6388\u3001\u6b66\u6c49\u7406\u5de5\u5927\u5b66\u4f59\u5bb6\u56fd\u6559\u6388(\u5171\u540c\u901a\u8baf\u4f5c\u8005)\u7b49<\/strong>\u5236\u5907\u4e86\u5177\u6709\u5c42\u95f4\u6865\u63a5\u548cg-CN\u8868\u9762\u53cc\u4f4d\u70b9\u7684\u539f\u5b50\u7ea7\u5206\u6563\u7684Pd-\u5c42\u72b6\u5149\u50ac\u5316\u5242\uff0c\u5e76\u5728Adv. Funct. Mater.<\/strong>\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201cSingle-Atom Engineering of Directional Charge Transfer Channels and Active Sites for Photocatalytic Hydrogen Evolution<\/strong>\u201d\u7684\u7814\u7a76\u8bba\u6587\u3002\u4e0a\u8ff0\u5149\u50ac\u5316\u5242\u4e3a\u5149\u50ac\u5316\u6c34\u8fd8\u539f\u63d0\u4f9b\u4e86\u5b9a\u5411\u7535\u8377\u8f6c\u79fb\u901a\u9053\u548c\u9776\u5411\u6d3b\u6027\u4f4d\u70b9\u3002\u4e4b\u540e\u4f5c\u8005\u5229\u7528\u7406\u8bba\u9884\u6d4b\u548c\u5b9e\u9645\u8868\u5f81\u8bc1\u5b9e\u6210\u529f\u5236\u5907\u4e86\u5355\u539f\u5b50\u5de5\u7a0b\u7684Pd\/g-CN\u590d\u5408\u6750\u6599\uff0c\u5176\u5177\u6709\u4f18\u5f02\u7684\u8f7d\u6d41\u5b50\u5206\u79bb\u6027\u80fd\u4ee5\u53ca\u9ad8\u6548\u7684\u5149\u50ac\u5316\u5236\u6c22\u6d3b\u6027\uff0c\u4f18\u4e8e\u4f18\u5316\u7684Pt\/g-CN\u6807\u51c6\u7269\u3002\u8fd9\u4e00\u7814\u7a76\u7ed3\u679c\u4e3a\u91cf\u8eab\u5b9a\u5236\u5355\u539f\u5b50\u8d35\u91d1\u5c5e\u7684\u6027\u80fd\u548c\u5de5\u7a0b\u63d0\u4f9b\u4e86\u5408\u7406\u7684\u65b9\u6cd5\u3002<\/p>\n

\u3010\u56fe\u6587\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u56fe1 Pd\/g-CN\u590d\u5408\u6750\u6599\u7684\u7406\u8bba\u8ba1\u7b97<\/strong><\/p>\n

\"\"<\/p>\n

a) \u5177\u6709\u5c42\u95f4\u548c\u8868\u9762\u952e\u5408Pd\u539f\u5b50\u7684Pd\/g-CN\u590d\u5408\u6750\u6599\u793a\u610f\u56fe\uff1b<\/p>\n

b) Pd\/g-CN\u7684HOMO\u548cLUMO\u8ba1\u7b97\uff1b<\/p>\n

c) H2<\/sub>O\u5206\u5b50\u5728Pd\/g-CN\u4e0a\u7684\u5438\u9644\u80fd\u8ba1\u7b97\u3002<\/p>\n

\u56fe2 \u8d85\u8584g-CN\u7eb3\u7c73\u7247\u7684\u5f62\u8c8c<\/strong><\/p>\n

\"\"<\/p>\n

a) \u8d85\u8584g-CN\u7eb3\u7c73\u7247\u7684FESEM\u56fe\u50cf\uff1b<\/p>\n

b) \u8d85\u8584g-CN\u7eb3\u7c73\u7247\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

c) \u8d85\u8584g-CN\u7eb3\u7c73\u7247\u7684AFM\u56fe\u50cf\uff1b<\/p>\n

d) Pd\/g-CN\u7684Pd K\u8fb9FT-EXAFS\u5149\u8c31\u3002<\/p>\n

\u56fe3 Pd\/g-CN\u590d\u5408\u6750\u6599\u7684\u5f62\u8c8c\u548c\u5143\u7d20\u5206\u6790<\/strong><\/p>\n

\"\"<\/p>\n

a) Pd\/g-CN\u590d\u5408\u6750\u6599\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

b) Pd\/g-CN\u590d\u5408\u6750\u6599\u7684\u50cf\u5dee\u6821\u6b63HAADF-STEM\u56fe\u50cf\uff1b<\/p>\n

c) Pd\/g-CN\u590d\u5408\u6750\u6599\u7684EDS\u5143\u7d20\u5206\u5e03\u56fe\u50cf\u3002<\/p>\n

\u56fe4 Pd\/g-CN\u590d\u5408\u6750\u6599\u7684\u7ed3\u6784\u548c\u5149\u5438\u6536<\/strong><\/p>\n

\"\"<\/p>\n

a) g-CN\u8d85\u8584\u7eb3\u7c73\u7247\u548cPd\/g-CN\u7684\u6162\u626bXRD\u56fe\u8c31\uff1b<\/p>\n

b) CN-NS\u548cPd\/g-CN\u7684\u7d2b\u5916-\u53ef\u89c1\u6f2b\u53cd\u5c04\u5149\u8c31\uff1b<\/p>\n

c) Pd\/g-CN\u5728Ar+<\/sup>\u8f70\u51fb\u524d\u540e\u7684Pd 3d\u9ad8\u5206\u8fa8XPS\u5149\u8c31\uff1b<\/p>\n

d) Pd\/g-CN\u548cPd\u7247\u7684Pd K\u8fb9XANES\u3002<\/p>\n

\u56fe5 Pd\/g-CN\u590d\u5408\u6750\u6599\u7684\u8f7d\u6d41\u5b50\u5206\u79bb\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

a) CN-NS\u3001Pd\/g-CN\u548cPt\/g-CN\u7535\u6781\u7684EIS\u6d4b\u8bd5\uff1b<\/p>\n

b) CN-NS\u3001Pd\/g-CN\u548cPt\/g-CN\u7684\u7a33\u6001PL\u5149\u8c31\u6d4b\u8bd5\uff1b<\/p>\n

c) CN-NS\u3001Pd\/g-CN\u548cPt\/g-CN\u7684TRPL\u5149\u8c31\u3002<\/p>\n

\u56fe6 Pd\/g-CN\u590d\u5408\u6750\u6599\u7684\u5149\u50ac\u5316\u5236\u6c22\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

a) CN-NS\u3001Pd\/g-CN\u548cPt\/g-CN\u7684\u5149\u50ac\u5316\u5236\u6c22\u901f\u7387\uff1b<\/p>\n

b) Pd\/g-CN\u7684\u5236\u6c22\u5faa\u73af\u6d4b\u8bd5\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u901a\u8fc7\u7406\u8bba\u6a21\u62df\uff0c\u4f5c\u8005\u9884\u6d4b\u4e86\u5c42\u95f4\u63d2\u5165\u548c\u8868\u9762\u951a\u5b9a\u7684Pd\u539f\u5b50\u5bf9\u4e8e\u77f3\u58a8\u76f8\u6c2e\u5316\u78b3\u4e0a\u7684\u5149\u50ac\u5316\u5236\u6c22\u5177\u6709\u534f\u540c\u4f5c\u7528\u3002\u901a\u8fc7\u7b80\u5355\u7684\u70ed\u9a71\u52a8\u6269\u6563\u65b9\u6cd5\uff0c\u5229\u7528Pd\u5355\u539f\u5b50\u5df2\u5b9e\u73b0g-CN\u6846\u67b6\u7684\u5c42\u95f4\u548c\u8868\u9762\u8c03\u8282\u7684\u540c\u65f6\u8fdb\u884c\u3002\u6240\u6784\u7b51\u7684\u7531\u4f53\u76f8\u5230\u8868\u9762\u7684\u5b9a\u5411\u7535\u8377\u8f6c\u79fb\u7684\u5782\u76f4\u901a\u9053\u2014\u2014\u6865\u63a5Pd\u539f\u5b50\u4ee5\u53ca\u8fd8\u539f\u6c34\u50ac\u5316\u53cd\u5e94\u7684\u9776\u5411\u6d3b\u6027\u4f4d\u70b9\u2014\u2014\u8868\u9762Pd\u539f\u5b50\u5177\u6709\u7a81\u51fa\u7684\u4f18\u52bf\u3002\u4e0a\u8ff0\u72ec\u7279\u7684\u7ed3\u6784\u6709\u6548\u5730\u4fc3\u8fdb\u4e86\u7535\u5b50\u7684\u4f20\u8f93\/\u5206\u79bb\uff0c\u589e\u5f3a\u4e86\u5bf9\u53cd\u5e94\u7269\u5206\u5b50\u7684\u4eb2\u548c\u529b\uff0c\u4ece\u800c\u5927\u5927\u63d0\u9ad8\u4e86g-CN\u5149\u50ac\u5316\u5242\u7684\u5149\u50ac\u5316\u6d3b\u6027\u3002\u8be5\u7814\u7a76\u7684\u610f\u4e49\u5728\u4e8e\u4e3a\u8bbe\u8ba1\u548c\u5408\u6210\u5355\u539f\u5b50\u8c03\u63a7\u7684\u534a\u5bfc\u4f53\u5149\u50ac\u5316\u5242\u4ee5\u63d0\u9ad8\u5149\u50ac\u5316\u6d3b\u6027\u63d0\u4f9b\u65b0\u7684\u89c1\u89e3\u3002\u8be5\u7b56\u7565\u4e5f\u6709\u671b\u7528\u4e8e\u5176\u4ed62D\u529f\u80fd\u6750\u6599\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a Single-Atom Engineering of Directional Charge Transfer Channels and Active Sites for Photocatalytic Hydrogen Evolution<\/a><\/strong>\u00a0(Adv. Funct. Mater., 2018, DOI: 10.1002\/adfm.201802169)<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u65b0\u80fd\u6e90\u5c0f\u7ec4abc940504\u7f16\u8bd1\u6574\u7406\uff0c\u53c2\u4e0e\u65b0\u80fd\u6e90\u8bdd\u9898\u8ba8\u8bba\u8bf7\u52a0\u5165\u201c\u6750\u6599\u4eba\u65b0\u80fd\u6e90\u6750\u6599\u4ea4\u6d41\u7fa4 422065953\u201d\u3002<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1acailiaokefu\uff0c\u6211\u4eec\u4f1a\u9080\u8bf7\u5404\u4f4d\u8001\u5e08\u52a0\u5165\u4e13\u5bb6\u7fa4\u3002<\/strong><\/p>\n

\u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u7f16\u8f91\u90e8<\/a><\/strong>\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n

\u4eea\u5668\u8bbe\u5907\u3001\u8bd5\u5242\u8017\u6750\u3001\u6750\u6599\u6d4b\u8bd5\u3001\u6570\u636e\u5206\u6790\uff0c\u627e\u6750\u6599\u4eba\u3001\u4e0a\u6d4b\u8bd5\u8c37<\/a><\/strong>\uff01<\/p>\n","protected":false},"excerpt":{"rendered":"

\u3010\u5f15\u8a00\u3011 g-CN\u662f\u4e00\u7c7b\u91cd\u8981\u76842D\u5149\u50ac\u5316\u5242\uff0c\u4f46\u8f83\u4f4e\u7684\u5149\u50ac\u5316\u6548\u7387\u5f71\u54cd\u4e86\u5176\u8fdb\u4e00\u6b65\u7684\u5e94\u7528\uff0c\u5e94\u5f52\u56e0\u4e8e\u5176\u5149\u751f\u8f7d\u6d41\u5b50\u7684\u5229\u7528\u7387\u8f83\u4f4e\uff0c\u5373g-CN\u5c42\u95f4\u7684\u5f31\u8303\u5fb7\u534e\u529b\u4e0d\u5229\u4e8e\u76f8\u90bb\u5c42\u4e4b\u95f4…<\/p>\n","protected":false},"author":4931,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[2804,2815],"class_list":["post-145180","post","type-post","status-publish","format-standard","hentry","category-jiedu","tag-2804","tag-2815"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/145180"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/4931"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=145180"}],"version-history":[{"count":4,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/145180\/revisions"}],"predecessor-version":[{"id":145765,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/145180\/revisions\/145765"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=145180"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=145180"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=145180"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}