{"id":144734,"date":"2018-07-06T06:30:49","date_gmt":"2018-07-05T22:30:49","guid":{"rendered":"\/\/m.iemloyee.com\/?p=144734"},"modified":"2018-07-04T16:41:12","modified_gmt":"2018-07-04T08:41:12","slug":"%e6%b5%99%e6%b1%9f%e5%a4%a7%e5%ad%a6adv-energy-mater-%e9%ab%98%e6%80%a7%e8%83%bd%e8%86%9c%e5%8e%9a%e4%b8%8d%e6%95%8f%e6%84%9f%e9%92%99%e9%92%9b%e7%9f%bf%e7%94%b5%e6%b1%a0-%e5%ae%9e%e7%8e%b0","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=144734","title":{"rendered":"\u6d59\u6c5f\u5927\u5b66Adv. Energy Mater: \u9ad8\u6027\u80fd\u819c\u539a\u4e0d\u654f\u611f\u9499\u949b\u77ff\u7535\u6c60\u2014\u5b9e\u73b0\u9ad8\u6548\u7387\u4e0e\u539a\u819c\u7684\u517c\u5bb9"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

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\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6d59\u6c5f\u5927\u5b66\u9648\u7ea2\u5f81\u6559\u6388\u3001\u674e\u660c\u6cbb\u7814\u7a76\u5458\u548c\u5434\u521a\u526f\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\uff0c\u535a\u58eb\u751f\u9648\u6770\u7115\uff08\u7b2c\u4e00\u4f5c\u8005\uff09<\/strong>\u7b49\u4eba\u91c7\u752870\u2103\u70ed\u65cb\u6d82\u5de5\u827a\u5236\u5907\u8d85\u8fc7700nm\u539a\u7684\u9499\u949b\u77ff\u8584\u819c\uff0c\u7ec4\u88c5\u7ed3\u6784\u4e3aITO\/NiOx<\/sub>\/MAPbI3<\/sub>\/PCBM\/BCP\/Ag\u7684\u7535\u6c60\u6548\u7387\u8fbe\u523019.54%\uff0c\u4e3a\u5f53\u524d\u5df2\u77e5\u4ee5\u91d1\u5c5e\u6c27\u5316\u7269\u4f5c\u7a7a\u7a74\u4f20\u8f93\u5c42\u7684\u9499\u949b\u77ff\u7535\u6c60\u7684\u6700\u9ad8\u6548\u7387\uff0c\u5668\u4ef6\u7a33\u5b9a\u6027\u4e5f\u5f97\u5230\u660e\u663e\u6539\u5584\u3002\u6b64\u5916\uff0c\u5f53\u9499\u949b\u77ff\u5c42\u539a\u5ea6\u7531700nm\u589e\u52a0\u81f31150nm\u65f6\uff0c\u4ecd\u80fd\u4fdd\u630119%\u7684\u6548\u7387\uff0c\u8fdb\u4e00\u6b65\u589e\u52a0\u81f31600nm\uff0c\u7535\u6c60\u6548\u7387\u8d85\u8fc717%\uff0c\u4e3a\u5f53\u524d\u5df2\u62a5\u9053\u7684\u6700\u539a\u9499\u949b\u77ff\u819c\u5c42\u592a\u9633\u80fd\u7535\u6c60\u3002\u76f8\u5173\u6210\u679c\u4ee5\u9898\u4e3a\u201cHigh-Performance Thickness Insensitive Perovskite Solar Cells with Enhanced Moisture Stability\u201d<\/strong>\u53d1\u8868\u5728Adv. Energy Mater.<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00 \u9499\u949b\u77ff\u7535\u6c60\u5668\u4ef6\u7ed3\u6784\u53ca\u6027\u80fd\u66f2\u7ebf<\/strong>
\n \"\"
\n (a) \u9499\u949b\u77ff\u7535\u6c60\u5668\u4ef6\u7ed3\u6784\uff1b
\n (b) \u9499\u949b\u77ff\u7535\u6c60\u7684\u80fd\u7ea7\u793a\u610f\u56fe\uff1b
\n (c) (d) \u9499\u949b\u77ff\u7535\u6c60\u7684J-V\u6027\u80fd\u66f2\u7ebf\uff0cEQE\u5149\u8c31\uff081.2M\u524d\u9a71\u4f53\u6eb6\u6db2\uff0c\u4e0d\u540c\u65cb\u6d82\u6e29\u5ea6\u5236\u5907\u7684\u9499\u949b\u77ff\u8584\u819c\uff09\u3002<\/p>\n

\u56fe\u4e8c \u9499\u949b\u77ff\u8584\u819c\u8868\u5f81<\/strong>
\n \"\"
\n (a) (b) \u4e0d\u540c\u65cb\u6d82\u6e29\u5ea6\uff0825\u2103\u300170\u2103\uff09\u5236\u5907\u7684\u9499\u949b\u77ff\u8584\u819c\u622a\u9762SEM\uff1b
\n (c) \u9499\u949b\u77ff\u8584\u819cXRD\uff1b
\n (d) \u9499\u949b\u77ff\u8584\u819c\u5438\u6536\u548cPL\u5149\u8c31\u3002<\/p>\n

\u56fe\u4e09 \u9499\u949b\u77ff\u7535\u6c60\u7684\u8f7d\u6d41\u5b50\u52a8\u529b\u5b66\u7814\u7a76<\/strong>
\n \"\"
\n (a) \u6697\u6001\u4e0b\u9499\u949b\u77ff\u7535\u6c60\u7684J-V\u7279\u5f81\u66f2\u7ebf\uff1b
\n (b) (c) \u4e0d\u540c\u5149\u5f3a\u4e0b\u6d4b\u8bd5\u5f97\u5230\u9499\u949b\u77ff\u7535\u6c60\u7684Jsc\u548cVoc\uff1b
\n (d) ITO\/NiOx<\/sub>\/MAPbI3<\/sub>\/PTAA\/MoO3<\/sub>\/Ag\u5668\u4ef6\u7684J-V\u7279\u5f81\u66f2\u7ebf\uff0c\u4ee5\u6b64\u4f30\u8ba1\u7a7a\u7a74\u8fc1\u79fb\u7387\u548c\u7f3a\u9677\u5bc6\u5ea6\u3002<\/p>\n

\u56fe\u56db \u4e0d\u540c\u6d53\u5ea6\u524d\u9a71\u4f5370\u2103\u70ed\u65cb\u6d82\u5236\u5907\u7684\u9499\u949b\u77ff\u8584\u819c\u7684\u622a\u9762SEM<\/strong>
\n \"\"<\/p>\n

\u56fe\u4e94 \u4e0d\u540c\u9499\u949b\u77ff\u5c42\u539a\u5ea6\u7684\u9499\u949b\u77ff\u7535\u6c60\u6027\u80fd\u8868\u5f81<\/strong>
\n \"\"
\n (a) \u9499\u949b\u77ff\u7535\u6c60\u7684J-V\u6027\u80fd\u66f2\u7ebf\uff1b
\n (b) \u9499\u949b\u77ff\u7535\u6c60\u7684EQE\u5149\u8c31\uff1b
\n (c) \u9499\u949b\u77ff\u7535\u6c60\u7684\u6a21\u62dfEQE\u5149\u8c31\uff1b
\n (d) \u9499\u949b\u77ff\u7535\u6c60\u7684IQE\u5149\u8c31\u3002<\/p>\n

\u56fe\u516d \u4e0d\u540c\u9499\u949b\u77ff\u5c42\u539a\u5ea6\u7684\u9499\u949b\u77ff\u7535\u6c60\u6027\u80fd\u53c2\u6570\u5206\u5e03<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe\u4e03 \u9499\u949b\u77ff\u8584\u819c\u53ca\u7535\u6c60\u7684\u7a33\u5b9a\u6027\u7814\u7a76<\/strong>
\n \"\"
\n (a) (b) \u4e0d\u540c\u65cb\u6d82\u6e29\u5ea6\uff0870\u2103\u300125\u2103\uff09\u5236\u5907\u9499\u949b\u77ff\u8584\u819c\uff0c\u653e\u7f6e\u4e0d\u540c\u5929\u6570\u540e\u7684XRD\uff1b
\n (c) \u9499\u949b\u77ff\u8584\u819cXRD\u4e2dPbI2<\/sub>\u542b\u91cf\u968f\u65f6\u95f4\u7684\u53d8\u5316\uff1b
\n (d) \u9499\u949b\u77ff\u7535\u6c60\u7684\u7a33\u5b9a\u6027\u6d4b\u8bd5\uff08\u7535\u6c60\u672a\u5c01\u88c5\uff0c\u4fdd\u5b58\u5728\u6e7f\u5ea650%\u7684\u6c2e\u6c14\u624b\u5957\u7bb1\u4e2d\uff09\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u8be5\u7814\u7a76\u63d0\u51fa\u4e86\u4e00\u79cd\u7b80\u5355\u7684\u4e00\u6b65\u70ed\u65cb\u6d82\u5de5\u827a\u5236\u5907\u539a\u9499\u949b\u77ff\u5c42\u592a\u9633\u80fd\u7535\u6c60\uff0c\u5f53\u5438\u5149\u5c42\u539a\u5ea6\u8d85\u8fc71000nm\u65f6\uff0c\u5668\u4ef6\u6548\u7387\u4ecd\u80fd\u8d85\u8fc719%\u3002\u901a\u8fc7\u5149\u5b66\u6a21\u62df\uff0c\u7814\u7a76\u4eba\u5458\u53d1\u73b0\u539a\u819c\u4e2d\u5e73\u5747\u7535\u5b50\u4f20\u8f93\u8ddd\u79bb\u53d8\u957f\uff0c\u800c\u7a7a\u7a74\u5230\u8fbe\u9633\u6781\u7684\u5e73\u5747\u8ddd\u79bb\u51e0\u4e4e\u76f8\u540c\uff0c\u7531\u4e8e\u8f7d\u6d41\u5b50\u8fc1\u79fb\u7387\u9ad8\uff0c\u9677\u9631\u6001\u5c11\uff0c\u56e0\u800c\u70ed\u65cb\u6d82\u5236\u5907\u7684\u9499\u949b\u77ff\u8584\u819c\u5177\u6709\u5f88\u597d\u7684\u8010\u539a\u5ea6\u3002\u8fd9\u79cd\u7b80\u5355\u7684\u4e00\u6b65\u65cb\u6d82\u5de5\u827a\u5728\u751f\u4ea7\u9499\u949b\u77ff\u7535\u6c60\u5668\u4ef6\u65b9\u9762\u6709\u5f88\u5927\u7684\u6f5c\u529b\uff0c\u63a8\u8fdb\u4e86\u9499\u949b\u77ff\u7684\u4ea7\u4e1a\u5316\u8fdb\u7a0b\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aHigh-Performance Thickness Insensitive Perovskite Solar Cells with Enhanced Moisture Stability<\/a><\/strong>\uff08Adv. Energy Mater.2018,DOI:10.1002\/aenm.201800438\uff09<\/p>\n

\u3010\u56e2\u961f\u4ecb\u7ecd\u3011<\/strong><\/p>\n

\u6d59\u6c5f\u5927\u5b66\u9648\u7ea2\u5f81\u6559\u6388\u4e3b\u6301\u7684\u6709\u673a\u534a\u5bfc\u4f53\u7814\u7a76\u56e2\u961f\u662f\u6211\u56fd\u6700\u65e9\u4ece\u4e8b\u6709\u673a\u9ad8\u5206\u5b50\u534a\u5bfc\u4f53\u6750\u6599\u4e0e\u5149\u7535\u529f\u80fd\u5668\u4ef6\u7814\u7a76\u4e0e\u5f00\u53d1\u7684\u8bfe\u9898\u7ec4\u4e4b\u4e00\uff0c\u7531\u6d59\u6c5f\u5927\u5b66\u524d\u6821\u957f\u6768\u58eb\u6797\u6559\u6388\u548c\u6c6a\u832b\u6559\u6388\u4e8e1986\u5e74\u521b\u5efa\uff0c\u957f\u671f\u575a\u6301\u6d3b\u8dc3\u7684\u521b\u65b0\u601d\u60f3\u548c\u5bbd\u677e\u7684\u5b66\u672f\u6c1b\u56f4\uff0c\u5f62\u6210\u4e86\u4ee5\u6709\u673a\u590d\u5408\u534a\u5bfc\u4f53\u4e3a\u4e3b\u8981\u7814\u7a76\u65b9\u5411\u3001\u4ee5\u5e73\u9762\u5927\u73af\u5171\u8f6d\u6709\u673a\u9ad8\u5206\u5b50\u7684\u8bbe\u8ba1\u4e0e\u5408\u6210\u4e3a\u57fa\u7840\u3001\u4ee5\u590d\u5408\u6280\u672f\u4e0e\u7eb3\u7c73\u6280\u672f\u76f8\u7ed3\u5408\u4e3a\u624b\u6bb5\u3001\u4ee5\u5148\u8fdb\u5149\u7535\u529f\u80fd\u6750\u6599\u7684\u8bbe\u8ba1\u4e0e\u5236\u5907\u4e3a\u4e2d\u5fc3\u3001\u4ee5\u7814\u7a76\u6750\u6599\u5fae\u7eb3\u7ed3\u6784-\u7535\u8377\u8f6c\u79fb-\u5149\u7535\u529f\u80fd\u7684\u5173\u7cfb\u4e3a\u4e3b\u9898\u3001\u4ee5\u5f00\u53d1\u65b0\u578b\u5149\u7535\u529f\u80fd\u5668\u4ef6\u4e3a\u76ee\u6807\u7684\u9c9c\u660e\u7279\u8272\uff0c\u7814\u7a76\u65b9\u5411\u6db5\u76d6\u6709\u673a\u3001\u6709\u673a-\u65e0\u673a\u6742\u5316\u4ee5\u53ca\u5355\u6676\u590d\u5408\u5149\u7535\u529f\u80fd\u6750\u6599\u3002\u5148\u540e\u4e3b\u6301\u56fd\u5bb6\u6770\u51fa\u9752\u5e74\u79d1\u5b66\u57fa\u91d1\u3001\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u91cd\u5927\u9879\u76ee\u8bfe\u9898\/\u91cd\u70b9\/\u91cd\u5927\uff08\u91cd\u70b9\uff09\u56fd\u9645\u5408\u4f5c\/\u4f18\u9752\u3001973\u9879\u76ee\u8bfe\u9898\u548c863\u91cd\u70b9\u9879\u76ee\u7b49\u56fd\u5bb6\u548c\u7701\u90e8\u7ea7\u9879\u76ee30\u591a\u9879\uff1b\u5728Adv. Mater., Chem. Rev., J. Am. Chem. Soc., Angew. Chem. Int. Ed., Energy Environ. Sci., Adv. Energy Mater. \u7b49\u672c\u9886\u57df\u8457\u540d\u5b66\u672f\u520a\u7269\u53d1\u8868SCI\u6536\u5f55\u8bba\u6587300\u591a\u7bc7\uff0cSCI\u8bba\u6587\u4ed6\u5f15\u8d85\u8fc78000\u591a\u6b21\u3002<\/p>\n

\u3010\u56e2\u961f\u4f18\u8d28\u6587\u732e\u63a8\u8350\u3011<\/strong><\/p>\n

1. Zhisheng Yang, Ligong Yang*, Gang Wu, Mang Wang, Hongzheng Chen*, A Heterojunction Based on Well-ordered Organic-Inorganic Hybrid Perovskite and Its Photovoltaic Performance, ACTA CHIMICA SINICA, 69(6), 627-632 (2011)<\/a>
\n 2. Xinqian Zhang, Gang Wu*, Weifei Fu, Minchao Qin, Weitao Yang, Jielin Yan, Zhongqiang Zhang, Xinhui Lu, Hongzheng Chen*, Orientation Regulation of Phenylethylammonium Cation Based 2D Perovskite Solar Cell with Efficiency Higher Than 11%, Advanced Energy Materials, 2018, 1702498.<\/a>
\n 3. Jielin Yan, Weifei Fu, Xinqian Zhang, Jiehuan Chen, Weitao Yang, Weiming Qiu, Gang Wu*, Feng Liu*, Paul Heremans, Hongzheng Chen*, Highly oriented two-dimensional formamidinium lead iodide perovskites with a small bandgap of 1.51 eV, MATERIALS CHEMISTRY FRONTIERS, 2018, 2, 121.<\/a>
\n 4. Xinqian Zhang, Gang Wu*, Shida Yang, Weifei Fu, Zhongqiang Zhang, Chen, Chen, Wenqing Liu, Jielin Yan, Weitao Yang, Hongzheng Chen*, Vertically Oriented 2D Layered Perovskite Solar Cells with Enhanced Efficiency and Good Stability, SMALL, 2017, 1700611.<\/a>
\n 5. Huanle Chen, Weifei Fu, Chuyi Huang, Zhongqiang Zhang, Shuixing Li, Feizhi Ding, Minmin Shi, Chang-Zhi Li,* Alex K.-Y. Jen* and Hongzheng Chen*, Molecular Engineered Hole-Extraction Materials to Enable Dopant-Free, Efficient p-i-n Perovskite Solar Cells, Adv. Energy Mater. 2017, 1700012<\/a>
\n 6. Lijian Zuo , Zhuowei Gu , Tao Ye , Weifei Fu , Gang Wu , Hanying Li ,* and Hongzheng Chen*, Enhanced Photovoltaic Performance of CH3NH3PbI3 Perovskite Solar Cells through Interfacial Engineering Using Self-Assembling Monolayer, J. Am. Chem. Soc., 2015, 137, 2674-2679.<\/a><\/p>\n

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