{"id":142946,"date":"2018-06-25T06:30:44","date_gmt":"2018-06-24T22:30:44","guid":{"rendered":"\/\/m.iemloyee.com\/?p=142946"},"modified":"2018-06-25T09:41:04","modified_gmt":"2018-06-25T01:41:04","slug":"energy-environ-sci-%ef%bc%9a%e5%90%88%e9%87%91%e5%8c%96%e9%99%8d%e4%bd%8e%e5%8d%95%e6%96%9c%e7%95%b8%e5%8f%98%e6%94%b9%e5%96%84%e9%92%92%e9%85%b8%e9%93%8b%e5%85%89%e9%98%b3%e6%9e%81","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=142946","title":{"rendered":"Energy Environ. Sci.\uff1a\u5408\u91d1\u5316\u964d\u4f4e\u5355\u659c\u7578\u53d8\u6539\u5584\u9492\u9178\u94cb\u5149\u9633\u6781"},"content":{"rendered":"

\u3010\u524d\u8a00\u3011<\/strong><\/p>\n

\u901a\u8fc7\u5149\u7535\u5316\u5b66(PEC)\u751f\u4ea7\u71c3\u6599\u88ab\u8ba4\u4e3a\u662f\u6355\u83b7\u548c\u5b58\u50a8\u95f4\u6b47\u592a\u9633\u80fd\u7684\u6709\u6548\u65b9\u6cd5\uff0c\u7279\u522b\u662f\u4f5c\u4e3a\u53ef\u518d\u751f\u8fd0\u8f93\u71c3\u6599\u3002\u65e0\u8bba\u4ea7\u751f\u4f55\u79cd\u71c3\u6599\uff0c\u5149\u9633\u6781\u7684\u6790\u6c27\u53cd\u5e94\u90fd\u662f\u5173\u952e\u7684\uff1b\u56e0\u6b64\uff0c\u7531\u5730\u7403\u4e30\u5bcc\u5143\u7d20\u7ec4\u6210\u7684\u7a33\u5b9a\u3001\u9ad8\u6548\u3001n\u578b\u534a\u5bfc\u4f53\u7684\u5f00\u53d1\u53d7\u5230\u8d8a\u6765\u8d8a\u591a\u7684\u7814\u7a76\u5173\u6ce8\uff0c\u8be5\u7c7b\u534a\u5bfc\u4f53\u53ef\u901a\u8fc7\u53ef\u6269\u5c55\u7684\u3001\u7ecf\u6d4e\u9ad8\u6548\u7684\u65b9\u6cd5\u751f\u4ea7\u3002\u9492\u9178\u94cb\uff0c\u5c24\u5176\u662fBiVO4<\/sub>\uff0c\u5c3d\u7ba1\u5e26\u9699\u4e0d\u662f\u6700\u4f73\u7684\uff0c\u4f46\u5df2\u7528\u4e8e\u6539\u8fdb\u548c\u7406\u89e3\u65b0\u578b\u6c27\u5316\u7269\u57fa\u534a\u5bfc\u4f53\u7684\u57fa\u672c\u6027\u80fd\u548c\u5149\u7535\u5316\u5b66\u6027\u80fd\u3002\u8fd1\u5e74\u6765\uff0c\u6539\u5584\u6027\u80fd\u7684\u65b9\u6cd5\u5305\u62ec\u5f02\u8d28\u7ed3\u5f62\u6210\u3001\u5408\u91d1\u5316\u6216\u63ba\u6742\u3001\u6c22\u6216\u6c2e\u9000\u706b\u3001\u589e\u5f3a\u7535\u8377\u6536\u96c6\u7684\u7eb3\u7c73\u7ed3\u6784\u3001\u5149\u5b50\u7ba1\u7406\u7684\u5fae\u7ed3\u6784\u4ee5\u53ca\u949d\u5316\u8868\u9762\u7f3a\u9677\u548c\u589e\u5f3a\u50ac\u5316\u7684\u8868\u9762\u6d82\u5c42\u3002<\/p>\n

\u8fc4\u4eca\u4e3a\u6b62\u62a5\u9053\u7684\u6027\u80fd\u6700\u9ad8\u7684\u57fa\u4e8eBiVO4<\/sub>\u7684\u5149\u9633\u6781\u90fd\u7ed3\u5408\u4e86\u8fd9\u4e9b\u7b56\u7565\uff0c\u4ee5\u4fbf\u5728AM 1.5\u7167\u660e\u4e0b\u4ea7\u751f\u5927\u7ea62 – 6.7 mA cm-2<\/sup>\u8303\u56f4\u5185\u7684\u5149\u7535\u6d41\u5bc6\u5ea6\uff0c\u63a5\u8fd1\u5177\u67092.4 eV\u5e26\u9699\u534a\u5bfc\u4f53\u76847.5 mA cm-2<\/sup>\u7684\u7406\u8bba\u6781\u9650\u3002\u5c3d\u7ba1\u4e3a\u4e86\u4ea7\u751f\u8bb0\u5f55\u6216\u63a5\u8fd1\u8bb0\u5f55\u7684\u6027\u80fd\uff0c\u9700\u8981\u540c\u65f6\u4f7f\u7528\u591a\u79cd\u6027\u80fd\u589e\u5f3a\u65b9\u6cd5\uff0c\u4f46\u662f\u8fd9\u79cd\u65b9\u6cd5\u6291\u5236\u4e86\u4ece\u7279\u5b9a\u4fee\u6539\u4e2d\u7406\u89e3\u63a7\u5236\u6027\u80fd\u6539\u8fdb\u7684\u57fa\u672c\u539f\u7406\u7684\u52aa\u529b\u3002\u4e8b\u5b9e\u4e0a\uff0c\u5982\u679c\u4e0d\u53d8\u7684\u6280\u672f(\u4f8b\u5982\u50ac\u5316\u5242\u8868\u9762\u6d82\u5c42)\u4e0e\u7ed9\u5b9a\u7684\u5408\u91d1\u6210\u5206\u4e0d\u76f8\u5bb9\uff0c\u5728\u6539\u53d8\u4e00\u4e2a\u53c2\u6570(\u4f8b\u5982\u5408\u91d1\u6210\u5206)\u7684\u540c\u65f6\u5e94\u7528\u591a\u79cd\u6027\u80fd\u589e\u5f3a\u6280\u672f\u53ef\u4ee5\u63a9\u76d6\u6f5c\u5728\u7684\u6027\u80fd\u8d8b\u52bf\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6765\u81ea\u52a0\u5dde\u7406\u5de5\u5927\u5b66\u7684<\/strong>John Gregoire<\/strong>\u6559\u6388\u548c\u52a0\u5dde\u5927\u5b66\u4f2f\u514b\u5229\u5206\u6821\u7684<\/strong>Jeffrey Neaton<\/strong>\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\uff09<\/strong>\u8054\u5408\u5728Energy Environ. Sci.<\/strong>\u53d1\u8868\u6587\u7ae0\uff0c<\/strong>\u9898\u4e3a\uff1aCombinatorial Alloying Improves Bismuth Vanadate Photoanodes via Reduced Monoclinic Distortion<\/strong>\u3002\u63d0\u9ad8\u592a\u9633\u80fd\u91ca\u6c27\u6548\u7387\u5bf9\u4e8e\u592a\u9633\u80fd\u71c3\u6599\u6280\u672f\u7684\u53d1\u5c55\u81f3\u5173\u91cd\u8981\uff0c\u4f46\u7531\u4e8e\u592a\u9633\u80fd\u71c3\u6599\u5149\u9633\u6781\u9700\u8981\u5e7f\u6cdb\u7684\u6027\u80fd\uff0c\u56e0\u6b64\u5177\u6709\u6311\u6218\u6027\u3002\u9492\u9178\u94cb\uff0c\u7279\u522b\u662f\u5355\u659c\u659c\u9492\u94cb\u77ff\u76f8\uff0c\u53d7\u5230\u4e86\u5e7f\u6cdb\u5173\u6ce8\uff0c\u5728\u53ef\u89c1\u5149\u6ce2\u6bb5\u5e26\u9699\u91d1\u5c5e\u6c27\u5316\u7269\u4e2d\u663e\u793a\u51fa\u6700\u9ad8\u7684\u8f90\u5c04\u6548\u7387\u3002\u7814\u7a76\u4eba\u5458\u8fdb\u4e00\u6b65\u63d0\u9ad8\u5176\u5149\u7535\u5316\u5b66\u6027\u80fd\u7684\u52aa\u529b\u5305\u62ec\u5c06\u4e00\u79cd\u6216\u591a\u79cd\u91d1\u5c5e\u5408\u91d1\u5316\u5230Bi\u548c\/\u6216V\u7684\u4f4d\u70b9\u4e0a\uff0c\u7531\u4e8e\u66ff\u4ee3\u5408\u91d1\u7684\u8ba1\u7b97\u5efa\u6a21\u56f0\u96be\u4ee5\u53ca\u5171\u5408\u91d1\u5316\u7ec4\u6210\u7a7a\u95f4\u7684\u9ad8\u7ef4\u6027\uff0c\u963b\u788d\u4e86\u8fd9\u4e00\u524d\u6cbf\u7684\u8fdb\u5c55\u3002\u7531\u4e8e\u66ff\u4ee3\u5408\u91d1\u5316\u540c\u65f6\u6539\u53d8\u4e86\u591a\u79cd\u6750\u6599\u7684\u6027\u80fd\uff0c\u4e86\u89e3\u6027\u80fd\u6539\u5584\u7684\u6839\u672c\u539f\u56e0\u4e5f\u662f\u4e00\u4e2a\u6311\u6218\uff0c\u4fc3\u4f7f\u7814\u7a76\u4eba\u5458\u5e94\u7528\u7ec4\u5408\u6750\u6599\u79d1\u5b66\u6280\u672f\u6765\u7ed8\u5236\u4e86948\u79cd\u72ec\u7279\u9492\u9178\u94cb\u5408\u91d1\u7ec4\u5408\u7269\u7684\u5149\u7535\u5316\u5b66\u6027\u80fd\uff0c\u8fd9\u4e9b\u7ec4\u5408\u7269\u5305\u62ec0-8 %\u7684P\u3001Ca\u3001Mo\u3001Eu\u3001Gd\u548cW\u5408\u91d1\u4ee5\u53ca\u8fd9\u4e9b\u5143\u7d20\u7684\u6bcf\u5bf9\u7ec4\u5408\u7684\u5404\u79cd\u7ec4\u5408\u3002\u5728\u786e\u5b9a( Mo\uff0cGd )\u5171\u5408\u91d1\u5316\u7a7a\u95f4\u7684\u663e\u8457\u6539\u5584\u540e\uff0c\u8fdb\u884c\u4e86\u7ed3\u6784\u6620\u5c04\uff0c\u4ee5\u63ed\u793a\u6027\u80fd\u589e\u5f3a\u548c\u964d\u4f4e\u7684\u5355\u659c\u7578\u53d8\u4e4b\u95f4\u7684\u663e\u8457\u76f8\u5173\u6027\u3002\u7b2c\u4e00\u6027\u539f\u7406\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0c\u8fd9\u79cd\u6539\u8fdb\u662f\u7531\u4e8e\u7a7a\u7a74\u6709\u6548\u8d28\u91cf\u548c\u7a7a\u7a74\u6781\u5316\u5b50\u5f62\u6210\u80fd\u91cf\u7684\u964d\u4f4e\uff0c\u6211\u4eec\u7684\u7ed3\u679c\u5c06\u5355\u659c\u7578\u53d8\u786e\u5b9a\u4e3a\u4f18\u5316\u548c\u7406\u89e3\u7684\u5173\u952e\u53c2\u6570<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe1. \u5149\u9633\u6781\u5e93<\/strong><\/p>\n

\"\"<\/p>\n

(a.) \u5149\u9633\u6781\u5e93\u4e2d1713\u4e2a\u6837\u54c1\u4e2d189\u4e2a\u6837\u54c1\u7684\u886c\u5e95\u533a\u57df\u56fe\u50cf;<\/p>\n

(b.) \u663e\u793a\u4e864\u4e2a\u6837\u54c1\u7684\u77ed\u5207\u7167\u660eCV\u7684\u9633\u6781\u626b\u63cf;<\/p>\n

(c.) \u6bcf\u4e2a\u9633\u6781\u626b\u63cf\u7684\u81ea\u52a8\u5904\u7406\u4ea7\u751f\u6700\u5927\u5149\u7535\u5316\u5b66\u80fd(Pmax<\/sub>);<\/p>\n

\u56fe2. \u591a\u79cd\u91d1\u5c5e\u5408\u91d1\u5316\u5230Bi\u548c\/\u6216V\u7684\u4f4d\u70b9\u4e0a<\/strong><\/p>\n

\"\"<\/p>\n

(a.) \u5728\u5149\u9633\u6781\u5e93\u4e2d948\u4e2d\u72ec\u7279\u7ec4\u5206\u4e2d\u7684489\u4e2aPmax<\/sub>\u503c\uff1b<\/p>\n

(b.) \u6765\u81ea\u76f8\u540c\u9633\u6781\u626b\u63cf\u6570\u636e\u96c6\u7684JO2<\/sub>\/H2<\/sub>O\u503c\u7684\u7c7b\u4f3c\u56fe\uff1b<\/p>\n

(c.) a-b\u4e2d\u5f84\u5411\u56fe\u7684\u56fe\u4f8b\uff1b<\/p>\n

(d.) \u6765\u81eaa\u7684Mo – Gd\u6247\u533a\u7ed8\u5236\u5728\u7b1b\u5361\u5c14\u7a7a\u95f4\u4e2d\uff0c\u5176\u4e2d\u4e09\u4e2ax\u503c\u5bf9\u5e94\u4e8e3\u4e2a\u7a81\u51fa\u663e\u793a\u7684\u5e73\u9762<\/p>\n

\u56fe3. Bi-V-A\u4f53\u7cfb<\/strong><\/p>\n

\"\"<\/p>\n

(a.)\u6bcf\u79cdBi-V-A\u4f53\u7cfb\u7684Pmax<\/sub>\u968f\u5408\u91d1\u8d1f\u8f7d\u7684\u53d8\u5316\u663e\u793a\uff1b<\/p>\n

(b.)\u5728Bi-V-Mo-B\u7a7a\u95f4\u4e2d\u5171\u5408\u91d1\u5316\u67095\u4e2aB\u503c\uff0c\u6bcf\u4e2aB\u503c\u5305\u62ec4\u4e2a\u4e0d\u540c\u7684\u603b\u5408\u91d1\u8f7d\u8377(y)\uff0c\u4ee5\u4e0d\u540c\u7684\u7b26\u53f7\u663e\u793a;<\/p>\n

\u56fe4. Bi-V-Mo-Gd\u5408\u91d1<\/strong><\/p>\n

\"\"<\/p>\n

(a.) Bi-V-Mo-Gd\u5408\u91d1\u7684\u7ec4\u5408\u8868\u5f81\uff1b<\/p>\n

(b.-e.)\u5305\u542b4\u4e2a\u4e0d\u540c\u7ec4\u6210\u7ebf\u7684\u5047\u5f69\u8272\u56fe\uff1b<\/p>\n

(f.)\u662f\u6765\u81ea\u56fed.\u7684\u6570\u636e\u7684\u53e0\u52a0\u56fe\u8868\u793a\uff1b<\/p>\n

(g.)\u63d0\u4f9b4\u6761\u5408\u6210\u7ebf\u7684\u53ef\u89c6\u5316\uff0c\u8fd9\u4e9b\u5408\u6210\u7ebf\u90fd\u5728\u56fe2d\u7684x=0.5\u5e73\u9762\u5185;<\/p>\n

\u56fe5.\u00a0Bi-V-Mo-Gd\u5408\u91d1<\/strong><\/p>\n

\"\"<\/p>\n

(a.) Bi-V-Mo-Gd\u5408\u91d1\u62c9\u66fc\u5149\u8c31\u8868\u5f81\u7684\u4e0d\u5bf9\u79f0(\u03b4as<\/sub>)\u548c\u5bf9\u79f0(\u03b4s<\/sub>)VO4<\/sub>\u5f2f\u66f2\u6a21\u5206\u88c2\u7a0b\u5ea6\u56fe;<\/p>\n

(b.)\u5bf9\u4e8e\u7531a\u4e2d\u7684\u6052\u661f\u6807\u8bb0\u76843\u6761\u7ec4\u6210\u7ebf\uff0cPmax<\/sub>\u548c\u5355\u659c\u7578\u53d8\u90fd\u7ed8\u5236\u4e3a\u76f8\u5bf9\u4e8e\u5404\u81ea\u7aef\u70b9Bi-V-Mo\u548cBi-V-Gd\u7ec4\u6210\u4e4b\u95f4\u7684\u7ebf\u6027\u5185\u63d2\u7684\u504f\u5dee(\u0394);<\/p>\n

(c.)\u7ed8\u5236\u4e86b\u7684\u5de6y\u8f74\u548c\u53f3y\u8f74\u6570\u636e\uff0c\u4ee5\u7a81\u51fa\u663e\u793a\u4f4e\u4e8eVegard\u5b9a\u5f8b\u9884\u671f\u7684\u5355\u659c\u7578\u53d8\u51cf\u5c11\u4e0ePmax<\/sub>\u5171\u5408\u91d1\u5316\u589e\u5f3a\u4e4b\u95f4\u7684\u5f3a\u76f8\u5173\u6027\uff1b<\/p>\n

\u56fe6. \u7ed3\u6784\u8ba1\u7b97<\/strong><\/p>\n

\"\"<\/p>\n

(a.)\u4e00\u7cfb\u5217\u6676\u4f53\u7ed3\u6784\u7684\u8ba1\u7b97\u80fd\u5e26\u7ed3\u6784\uff1b<\/p>\n

(b.) 7\u4e2a\u7ed3\u6784\u7684\u03b3- V VBM\u5904\u7684\u7a7a\u7a74\u6709\u6548\u8d28\u91cf\uff1b<\/p>\n

\u3010\u603b\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Combinatorial Alloying Improves Bismuth Vanadate Photoanodes via Reduced Monoclinic Distortion<\/a>, (Energy Environ. Sci., 2018, DOI:<\/strong> 10.1039\/C8EE00179K<\/strong>)<\/p>\n

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