{"id":141191,"date":"2018-06-05T14:00:37","date_gmt":"2018-06-05T06:00:37","guid":{"rendered":"\/\/m.iemloyee.com\/?p=141191"},"modified":"2018-06-05T22:40:48","modified_gmt":"2018-06-05T14:40:48","slug":"%e5%a4%a9%e6%b4%a5%e5%a4%a7%e5%ad%a6-%e5%a4%a9%e6%b4%a5%e7%90%86%e5%b7%a5%e5%a4%a7%e5%ad%a6adv-mater-%ef%bc%9a%e7%94%a8%e4%ba%8eco2%e5%8f%af%e9%80%86%e5%88%a9%e7%94%a8%e7%9a%84%e5%8f%af","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=141191","title":{"rendered":"\u5929\u6d25\u5927\u5b66\u2014\u5929\u6d25\u7406\u5de5\u5927\u5b66Adv. Mater.\uff1a\u7528\u4e8eCO2\u53ef\u9006\u5229\u7528\u7684\u53ef\u518d\u5145Al-CO2\u7535\u6c60"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u4e8c\u6c27\u5316\u78b3\u7684\u8fc7\u5ea6\u6392\u653e\u548c\u80fd\u6e90\u5371\u673a\u662f\u4eba\u7c7b\u9762\u4e34\u7684\u4e24\u5927\u95ee\u9898\u3002\u800c\u91d1\u5c5e-\u4e8c\u6c27\u5316\u78b3\u7535\u6c60\u53ef\u4ee5\u540c\u65f6\u5b9e\u73b0\u4e8c\u6c27\u5316\u78b3\u56fa\u5b9a\/\u5229\u7528\u548c\u80fd\u91cf\u50a8\u5b58\/\u91ca\u653e\uff0c\u56e0\u6b64\u5f15\u8d77\u4e86\u5e7f\u6cdb\u5173\u6ce8\u3002\u9502-\u4e8c\u6c27\u5316\u78b3\u7535\u6c60\u57282014\u5e74\u83b7\u5f97\u4e86\u6700\u65e9\u7684\u6210\u529f\uff0c\u8be5\u7535\u6c60\u91c7\u7528\u9502\u91d1\u5c5e\u9633\u6781\u548c\u78b3\u9634\u6781\u8fdb\u884c\u4e8c\u6c27\u5316\u78b3\u6355\u96c6\u548c\u50a8\u5b58\u3002\u7d27\u63a5\u7740\uff0c\u56fd\u5185\u5916\u5b66\u672f\u754c\u5728\u5f00\u53d1\u7528\u4e8e\u91d1\u5c5e-CO2<\/sub>\u7535\u6c60\u7684\u65b0\u578b\u6b63\u6781\u6750\u6599\u3001\u7a33\u5b9a\u7684\u7535\u89e3\u8d28\u4f53\u7cfb\u548cNa\u9633\u6781\u7b49\u65b9\u9762\u53d6\u5f97\u4e86\u7cfb\u5217\u8fdb\u5c55\u3002\u4f46\u662f\uff0cLi\u548cNa\u90fd\u662f\u9ad8\u6d3b\u6027\u91d1\u5c5e\uff0c\u6613\u4e0e\u73af\u5883\u7a7a\u6c14\u6216\u7528\u4e8e\u50a8\u5b58\/\u8fd0\u8f93\u7535\u6c60\u7684\u7ed3\u6784\u91d1\u5c5e\u53d1\u751f\u53cd\u5e94\u3002\u56e0\u6b64\uff0c\u8feb\u5207\u9700\u8981\u627e\u5230\u5316\u5b66\u7a33\u5b9a\u7684\u91d1\u5c5e\u4f5c\u4e3a\u91d1\u5c5e-\u4e8c\u6c27\u5316\u78b3\u7535\u6c60\u5b89\u5168\u5e94\u7528\u7684\u9633\u6781\u3002\u5df2\u6709\u62a5\u9053Al-CO2<\/sub>\u7535\u5316\u5b66\u7535\u6c60\u53ef\u7528\u4e8e\u4e8c\u6c27\u5316\u78b3\u6355\u96c6\/\u8f6c\u6362\uff0c\u4f46\u5176\u53ef\u9006\u53ef\u518d\u5145\u7279\u6027\u5c1a\u672a\u5b9e\u73b0\u3002Al\u7684\u5316\u5b66\u6d3b\u6027\u76f8\u5bf9\u8f83\u4f4e\uff0c\u56e0\u6b64\u6bd4Li\u548cNa\u5177\u6709\u66f4\u9ad8\u7684\u5b89\u5168\u6027\uff0c\u800c\u4e14\u5177\u6709\u4e0eLi\u548cNa\uff083860\u548c1165mAh g-1<\/sup>\uff09\u76f8\u5f53\u7684\u7406\u8bba\u6bd4\u5bb9\u91cf\uff082978mAh g-1<\/sup>\uff09\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u5929\u6d25\u7406\u5de5\u5927\u5b66\u7684\u4e01\u8f76\u6559\u6388\u548c\u7f57\u4fca\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\u3001\u5929\u6d25\u5927\u5b66\u517c\u804c\u535a\u5bfc\uff09<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u4ee5Al\u7b94\u4e3a\u9633\u6781\u3001\u4ee5\u79bb\u5b50\u6db2\u4f53\u4e3a\u7535\u89e3\u8d28\u3001\u4ee5\u5b8c\u5168\u975e\u78b3\u7684Pd\u5305\u8986\u7eb3\u7c73\u591a\u5b54\u91d1\uff08NPG@Pd\uff09\u4e3a\u4e00\u4f53\u5316\u50ac\u5316\u5242\u9634\u6781\u7684\u53ef\u518d\u5145Al-CO2<\/sub>\u7535\u6c60\u3002\u5176\u9634\u6781\u91c7\u7528\u7eafCO2<\/sub>\u4f5c\u4e3a\u6d3b\u6027\u6750\u6599\u3002\u8be5\u7535\u6c60\u5728333mA g-1<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5728\u653e\u7535\u548c\u5145\u7535\u5e73\u53f0\u4e4b\u95f4\u663e\u793a\u51fa\u4f4e\u81f30.091V\u7684\u7535\u4f4d\u5dee\uff0c\u56e0\u6b64\u5176\u80fd\u91cf\u6548\u7387\uff08EEs\uff09\u9ad8\u8fbe87.7\uff05\u3002\u901a\u8fc7\u5bf9NPG@Pd\u9634\u6781\u548c\u653e\u7535\u4ea7\u7269\u8fdb\u884c\u8868\u5f81\uff0c\u8be5\u7535\u6c60\u53cd\u5e94\u8fc7\u7a0b\u88ab\u63ed\u793a\u4e3a4Al + 9CO2<\/sub>\u21942Al2<\/sub>(CO3<\/sub>)3<\/sub> + 3C\u3002\u5728\u53cd\u5e94\u4e2d\uff0c\u653e\u7535\u65f6CO2<\/sub>\u5728\u6b63\u6781\u88ab\u8fd8\u539f\u3001\u4e0e\u94dd\u79bb\u5b50\u5f62\u6210Al2<\/sub>(CO3<\/sub>)3<\/sub>\u548cC\uff0c\u5e76\u5728\u5145\u7535\u65f6\u5206\u89e3\u3002\u8fd9\u9879\u5de5\u4f5c\u4e3a\u5f00\u53d1\u7528\u4e8e\u56fa\u5b9aCO2<\/sub>\u7684\u9ad8\u6548\u3001\u9ad8\u5b89\u5168\u6027\u3001\u7eff\u8272\u548c\u53ef\u518d\u5145\u7535\u7684\u80fd\u6e90\u88c5\u7f6e\u63d0\u4f9b\u4e86\u57fa\u7840\u548c\u6280\u672f\u652f\u6301\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cRechargeable Al\u2013CO2<\/sub> Batteries for Reversible Utilizationof CO2<\/sub><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Advanced Materials<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\uff1a\u5236\u5907\u7684<\/strong>NPG@Pd<\/strong>\u9634\u6781\u7684\u5f62\u6001\u548c\u7ed3\u6784<\/strong><\/p>\n

\"\"<\/a><\/p>\n

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\uff08c\uff09\u4f4e\u500dHAADF-STEM\u56fe\u50cf\u548c\uff08d\uff09\u76f8\u5e94\u7684EDS\u5143\u7d20\u5206\u5e03\uff1b<\/p>\n

\uff08e\uff09\u539f\u5b50\u5206\u8fa8\u7684HAADF-STEM\u56fe\u50cf\u548c\uff08f\uff0cg\uff0ch\uff09\u76f8\u5e94\u7684\u539f\u5b50\u5206\u8fa8EDS\u5143\u7d20\u5206\u5e03\u3002<\/p>\n

\u56fe\u4e8c\uff1a\u53ef\u5145\u7535<\/strong>Al-CO2<\/sub><\/strong>\u7535\u6c60\u7684\u653e\u7535<\/strong>\/<\/strong>\u5145\u7535\u53cd\u5e94\u673a\u7406<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u5206\u522b\u4ee5NPG@Pd\u548cNPG\u4e3a\u9634\u6781\u7684\u4e24\u4e2aAl-CO2<\/sub>\u7535\u6c60\u7684\u5145\u653e\u7535\u66f2\u7ebf\uff1b\uff08b-d\uff09NPG@Pd\u9634\u6781\u5728i\uff09\u521d\u59cb\u3001ii\uff09\u653e\u7535\u3001iii\uff09\u5145\u7535\u72b6\u6001\u65f6\u7684<\/p>\n

\uff08b\uff09\u62c9\u66fc\u3001\uff08c\uff09XPS\u3001\uff08d\uff09FTIR\u5149\u8c31\uff1b<\/p>\n

\uff08e\uff09\u7535\u6c60\u653e\u7535\u540e\u7684NPG@Pd\u9634\u6781\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08f\uff09\u7535\u6c60\u653e\u7535\u540e\u7684NPG@Pd\u9634\u6781\u7684HAADF-STEM\u56fe\u50cf\u4ee5\u53ca\u76f8\u5e94\u7684EDS\u5143\u7d20\u5206\u5e03\uff1b<\/p>\n

\uff08g\uff09\u7535\u6c60\u5145\u7535\u540e\u7684NPG@Pd\u9634\u6781\u7684SEM\u56fe\u50cf\u3002<\/p>\n

\u56fe\u4e09\uff1a\u53ef\u5145\u7535<\/strong>Al-CO2<\/sub><\/strong>\u7535\u6c60\u7684\u5faa\u73af\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u4e24\u4e2a\u5206\u522b\u4ee5NPG@Pd\u548cNPG\u4e3a\u9634\u6781\u7684Al-CO2<\/sub>\u7535\u6c60\u5728333 mA g-1<\/sup>\u4e0b\u8fde\u7eed\u653e\u7535\/\u5145\u7535\u7684\u5faa\u73af\u56fe\uff1b<\/p>\n

\uff08b\uff09\u4ee5NPG@Pd\u4e3a\u9634\u6781\u7684Al-CO2<\/sub>\u7535\u6c60\u7b2c1\u30012\u30015\u300110\u300120\u548c30\u6b21\u7684\u653e\u7535\/\u5145\u7535\u5faa\u73af\u56fe\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u672c\u6587\u8bbe\u8ba1\u4e86\u4e00\u79cd\u53ef\u5145\u7535Al-CO2<\/sub>\u7535\u6c60\uff0c\u7531\u94dd\u7b94\u4f5c\u4e3a\u9633\u6781\u3001\u79bb\u5b50\u6db2\u4f53\u4f5c\u4e3a\u7535\u89e3\u8d28\u3001NPG@Pd\u4f5c\u4e3a\u9634\u6781\u6784\u6210\u3002\u5176\u7535\u6c60\u53cd\u5e94\u673a\u7406\u9075\u5faa4Al + 9CO2<\/sub>\u21942Al2<\/sub>(CO3<\/sub>)3<\/sub> + 3C\uff0c\u5b9e\u73b0\u4e86CO2<\/sub>\u7684\u53ef\u9006\u5229\u7528\u3002\u8be5\u7535\u6c60\u8868\u73b0\u51fa\u53ef\u9006\u6027\uff0c\u653e\u7535\/\u5145\u7535\u5e73\u53f0\u7535\u4f4d\u5dee\u4f4e\u81f30.091 V\uff0c\u80fd\u91cf\u6548\u7387\uff08EEs\uff09\u9ad8\u8fbe87.7\uff05\u3002NPG\u4e5f\u88ab\u6210\u529f\u7528\u4f5c\u7535\u6c60\u9634\u6781\uff0c\u8868\u660eAl-CO2<\/sub>\u7535\u6c60\u6982\u5ff5\u7684\u666e\u9002\u6027\u3002\u8fd9\u4e9b\u7ed3\u679c\u4e3aCO2<\/sub>\u7684\u5b89\u5168\u548c\u7eff\u8272\u56fa\u5b9a\/\u5229\u7528\u4ee5\u53ca\u4e0b\u4e00\u4ee3\u5b89\u5168\u50a8\u80fd\/\u91ca\u653e\u7cfb\u7edf\u7684\u5f00\u53d1\u63d0\u4f9b\u4e86\u6709\u5e0c\u671b\u548c\u6709\u524d\u666f\u7684\u65b9\u6cd5\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a\u201c<\/strong>Rechargeable Al\u2013CO2 <\/sub>Batteries for Reversible Utilization of CO2<\/sub><\/strong><\/a>\u201d<\/strong>(<\/strong>Adv.mater.\uff0c2018<\/strong>\uff0cDOI: 10.1002\/adma.201801152<\/strong>)<\/strong><\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u5b66\u672f\u7ec4\u5fae\u89c2\u4e16\u754c\u7f16\u8bd1\uff0c\u8bba\u6587\u901a\u8baf\u4f5c\u8005\u4e01\u8f76\u3001\u7f57\u4fca\u4fee\u6b63\u4f9b\u7a3f\u3002<\/p>\n

\u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u7f16\u8f91\u90e8<\/strong><\/a>\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n

\u6750\u6599\u6d4b\u8bd5\u3001\u6570\u636e\u5206\u6790\uff0c\u4e0a<\/strong>\u6d4b\u8bd5\u8c37<\/strong><\/a>\uff01<\/strong><\/p>\n","protected":false},"excerpt":{"rendered":"

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