{"id":135374,"date":"2018-04-22T14:00:50","date_gmt":"2018-04-22T06:00:50","guid":{"rendered":"\/\/m.iemloyee.com\/?p=135374"},"modified":"2018-04-17T12:19:14","modified_gmt":"2018-04-17T04:19:14","slug":"%e6%a5%bc%e9%9b%84%e6%96%87j-am-chem-soc-znin2s4-in2o3%e5%88%86%e7%ba%a7%e7%ae%a1%e7%8a%b6%e5%bc%82%e8%b4%a8%e7%bb%93%e7%9a%84%e6%9e%84%e7%ad%91%e5%8f%8a%e5%85%b6%e9%ab%98%e6%95%88%e5%85%89","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=135374","title":{"rendered":"\u697c\u96c4\u6587J. Am. Chem. Soc.: ZnIn2S4-In2O3\u5206\u7ea7\u7ba1\u72b6\u5f02\u8d28\u7ed3\u7684\u6784\u7b51\u53ca\u5176\u9ad8\u6548\u5149\u8fd8\u539fCO2"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u4e3a\u66f4\u597d\u5730\u53d1\u6325\u5f02\u8d28\u7ed3\u5149\u50ac\u5316\u5242\u7684\u4f18\u52bf\uff0c\u5236\u5907\u5177\u6709\u9002\u5b9c\u7eb3\u7c73\u7ed3\u6784\u7684\u5149\u50ac\u5316\u5242\u81f3\u5173\u91cd\u8981\u3002\u5177\u6709\u72ec\u7279\u7ed3\u6784\u7684\u4e2d\u7a7a\u7c92\u5b50\u5df2\u5728\u4e0d\u540c\u7684\u7814\u7a76\u9886\u57df\u5c55\u9732\u4f18\u52bf\u3002\u8fd1\u6765\uff0c\u4e2d\u7a7a\u7ed3\u6784\u6750\u6599\u5df2\u88ab\u4f5c\u4e3a\u5149\u50ac\u5316\u5242\u7528\u4e8eCO2<\/sub>\u5149\u8fd8\u539f\u7684\u7814\u7a76\u3002\u4e2d\u7a7a\u7ed3\u6784\u4e0d\u4ec5\u80fd\u591f\u7f29\u77ed\u4f53\u76f8\u81f3\u8868\u9762\u7684\u6269\u6563\u8ddd\u79bb\u4ee5\u52a0\u901f\u7535\u5b50-\u7a7a\u7a74\u5206\u79bb\uff0c\u800c\u4e14\u63d0\u4f9b\u4e86\u8f83\u5927\u8868\u9762\u79ef\u4ee5\u53ca\u4e30\u5bcc\u7684\u6d3b\u6027\u4f4d\u70b9\uff0c\u8fdb\u800c\u4fc3\u8fdbCO2<\/sub>\u5438\u9644\u548c\u8868\u9762\u50ac\u5316\u53cd\u5e94\u3002\u4e0e\u6b64\u540c\u65f6\uff0c\u4e2d\u7a7a\u7ed3\u6784\u5185\u7684\u591a\u6b21\u5149\u6563\u5c04\/\u53cd\u5c04\u53ef\u4ee5\u63d0\u5347\u5165\u5c04\u5149\u5229\u7528\u7387\u3002\u5728\u5404\u79cd\u4e2d\u7a7a\u7ed3\u6784\u4e2d\uff0c\u7ba1\u72b6\u7ed3\u6784\u5177\u6709\u5f00\u653e\u7684\u4e24\u7aef\uff0c\u6709\u5229\u4e8e\u5728\u58f3\u5c42\u7684\u5185\u5916\u8868\u9762\u540c\u65f6\u751f\u957f\u5176\u4ed6\u534a\u5bfc\u4f53\uff0c\u6784\u7b51\u4e09\u5c42\u5f02\u8d28\u7ed3\u6784\u3002\u6b64\u5916\uff0c\u5728\u7ba1\u72b6\u57fa\u5e95\u4e0a\u751f\u957f\u4e8c\u7ef4\u534a\u5bfc\u4f53\u7eb3\u7c73\u7247\u53ef\u4ee5\u7f29\u77ed\u7535\u8377\u7684\u6269\u6563\u8ddd\u79bb\uff0c\u66b4\u9732\u66f4\u591a\u7684\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\u3002\u56e0\u6b64\uff0c\u7efc\u5408\u4e0a\u8ff0\u8003\u91cf\uff0c\u5236\u5907\u65b0\u578b\u5149\u50ac\u5316\u5242\u4ee5\u63a2\u7a76\u5176\u5728CO2<\/sub>\u5149\u8fd8\u539f\u8fc7\u7a0b\u4e2d\u7684\u4f18\u52bf\u524d\u666f\u826f\u597d\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u65b0\u52a0\u5761\u5357\u6d0b\u7406\u5de5\u5927\u5b66\u697c\u96c4\u6587\u6559\u6388(\u901a\u8baf\u4f5c\u8005)\u7b49<\/strong>\u5408\u7406\u8bbe\u8ba1\u5e76\u6784\u7b51\u4e86\u4e09\u660e\u6cbb\u578bZnIn2S4<\/sub>-In2<\/sub>O3<\/sub>\u5206\u7ea7\u7ba1\u72b6\u5f02\u8d28\u7ed3\u4f5c\u4e3a\u9ad8\u6548\u3001\u7a33\u5b9a\u7684\u5149\u50ac\u5316\u5242\u7528\u4e8e\u53ef\u89c1\u5149\u8fd8\u539fCO2<\/sub>\uff0c\u5e76\u5728J. Am. Chem. Soc.<\/strong>\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201cConstruction of ZnIn2<\/sub>S4<\/sub>\u2212In2<\/sub>O3<\/sub> Hierarchical Tubular Heterostructures for Efficient CO2<\/sub> Photoreduction<\/strong>\u201d\u7684\u7814\u7a76\u8bba\u6587\u3002\u8fd9\u4e00\u72ec\u7279\u7684\u8bbe\u8ba1\u5c06In2<\/sub>O3<\/sub>\u4e00\u7ef4(1D)\u7ba1\u72b6\u7ed3\u6784\u548cZnIn2<\/sub>S4<\/sub>\u8d85\u8584\u4e8c\u7ef4(2D)\u7eb3\u7c73\u7247\u6b21\u7ea7\u7ed3\u6784\u96c6\u4e8e\u4e00\u4f53\uff0c\u4fc3\u8fdb\u4e86\u5149\u751f\u8f7d\u6d41\u5b50\u7684\u5206\u79bb\u3001\u8fc1\u79fb\uff0c\u63d0\u9ad8\u4e86CO2<\/sub>\u5206\u5b50\u7684\u5438\u9644\uff0c\u5e76\u66b4\u9732\u4e86\u4e30\u5bcc\u7684\u8868\u9762\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\u3002\u53d7\u76ca\u4e8e\u4e0a\u8ff0\u7ed3\u6784\u548c\u7ec4\u6210\u7279\u6027\uff0c\u6700\u4f18\u7684ZnIn2<\/sub>S4<\/sub>\u2212In2<\/sub>O3<\/sub>\u5f02\u8d28\u7ed3\u5149\u50ac\u5316\u5242\u663e\u793a\u51fa\u9ad8CO2<\/sub>\u8131\u6c27\u8fd8\u539f\u6d3b\u6027\u548c\u7a33\u5b9a\uff0cCO\u4ea7\u7387\u4e3a3075 \u03bcmol\u00b7h-1<\/sup>\u00b7g-1<\/sup>\u3002<\/p>\n

\u3010\u56fe\u6587\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u56fe1 ZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u5206\u7ea7\u7ba1\u72b6\u5f02\u8d28\u7ed3\u6784\u5408\u6210\u8fc7\u7a0b\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u8fc7\u7a0b(I)\uff1a\u7a7a\u6c14\u6c1b\u56f4\u7145\u70e7\uff1b\u8fc7\u7a0b(II)\uff1a\u751f\u957fZnIn2S4\u7eb3\u7c73\u7247\u3002<\/p>\n

\u56fe2 In2<\/sub>O3<\/sub>\u5fae\u7c73\u7ba1\u7684\u5f62\u8c8c<\/strong><\/p>\n

\"\"<\/p>\n

a-c) In2<\/sub>O3<\/sub>\u5fae\u7c73\u7ba1\u7684FESEM\u56fe\u50cf\uff1b<\/p>\n

d,e) In2<\/sub>O3<\/sub>\u5fae\u7c73\u7ba1\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

f) In2<\/sub>O3<\/sub>\u5fae\u7c73\u7ba1\u7684HRTEM\u56fe\u50cf\u3002<\/p>\n

\u56fe3 ZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u5206\u7ea7\u5fae\u7c73\u7ba1\u7684\u5f62\u8c8c\u548c\u5143\u7d20\u5206\u5e03<\/strong><\/p>\n

\"\"<\/p>\n

a-c) ZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u5206\u7ea7\u5fae\u7c73\u7ba1\u7684FESEM\u56fe\u50cf\uff1b<\/p>\n

d) ZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u5206\u7ea7\u5fae\u7c73\u7ba1\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

e) ZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u5206\u7ea7\u5fae\u7c73\u7ba1\u7684HRTEM\u56fe\u50cf\uff1b<\/p>\n

f) ZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u5206\u7ea7\u5fae\u7c73\u7ba1\u7684SAED\u56fe\u8c31\uff1b<\/p>\n

g) \u5355\u4e00ZnIn2<\/sub>S4<\/sub>– In2<\/sub>O3<\/sub>\u5fae\u7c73\u7ba1\u7684\u5143\u7d20\u5206\u5e03\u3002<\/p>\n

\u56fe4 \u50ac\u5316\u5242\u7684\u5149\u8fd8\u539fCO2<\/sub>\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

a) \u4e0d\u540c\u6837\u54c1\u7684CO\u548cH2<\/sub>\u7684\u4ea7\u7387\uff1b<\/p>\n

b) CO\u548cH2<\/sub>\u4ea7\u91cf\u968f\u65f6\u95f4\u7684\u53d8\u5316\uff1b<\/p>\n

c) \u4e0d\u540c\u53cd\u5e94\u6761\u4ef6\u4e0bCO\u548cH2<\/sub>\u7684\u4ea7\u7387\uff1b<\/p>\n

d) 13<\/sup>CO2<\/sub>\u540c\u4f4d\u7d20\u5b9e\u9a8c\u4e2dCO\u7684GC-MS\u5206\u6790\u7ed3\u679c\uff1b<\/p>\n

e) \u7a33\u5b9a\u6027\u6d4b\u8bd5\u4e2dCO\u548cH2<\/sub>\u7684\u4ea7\u7387\uff1b<\/p>\n

f) CO\u548cH2\u7684\u4ea7\u7387\u968f\u6ce2\u957f\u7684\u53d8\u5316\u4ee5\u53caZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u7684\u5438\u6536\u5149\u8c31\u3002<\/p>\n

\u56fe5 \u50ac\u5316\u5242\u7684\u5149\u7535\u5316\u5b66\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

a) ZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u548cZnIn2<\/sub>S4<\/sub>\u7684\u65f6\u95f4\u5206\u8fa8\u77ac\u6001\u8367\u5149\u5149\u8c31\uff1b<\/p>\n

b) ZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u548cZnIn2<\/sub>S4<\/sub>\u7684\u7a33\u6001\u8367\u5149\u5149\u8c31\uff1b<\/p>\n

c) ZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u548cZnIn2<\/sub>S4<\/sub>\u7684EIS\u6d4b\u8bd5\uff1b<\/p>\n

d) ZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u548cZnIn2<\/sub>S4<\/sub>\u7684\u77ac\u6001\u5149\u7535\u6d41\u6d4b\u8bd5\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u7814\u7a76\u4eba\u5458\u901a\u8fc7\u5728In2<\/sub>O3<\/sub>\u5fae\u7ba1\u5185\u5916\u8868\u9762\u540c\u65f6\u751f\u957fZnIn2<\/sub>S4<\/sub>\u7eb3\u7c73\u7247\u5236\u5907\u4e86\u4e09\u660e\u6cbb\u578bZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u5206\u7ea7\u7ba1\u72b6\u5f02\u8d28\u7ed3\u6784\uff0c\u8be5\u6750\u6599\u663e\u793a\u51fa\u9ad8\u6548\u3001\u7a33\u5b9a\u7684\u53ef\u89c1\u5149\u50ac\u5316\u8fd8\u539fCO2<\/sub>\u6027\u80fd\u3002\u5229\u7528\u7b80\u5355\u7684\u5408\u6210\u7b56\u7565\uff08\u5305\u62ec\u7145\u70e7\u5904\u7406\u548c\u4f4e\u6e29\u6c34\u70ed\u53cd\u5e94\uff09\u53ef\u4ee5\u63a7\u5236\u6700\u7ec8\u590d\u5408\u6750\u6599\u7684\u7ed3\u6784\u548c\u7ec4\u5206\u3002\u4e0a\u8ff0\u5177\u6709\u53cc\u91cd\u754c\u9762\u5f02\u8d28\u7ed3\u58f3\u5c42\u548c\u8d85\u85842D\u7eb3\u7c73\u7247\u6b21\u7ea7\u7ed3\u6784\u7684\u590d\u6742\u7a7a\u5fc3\u7ed3\u6784\uff0c\u663e\u8457\u4fc3\u8fdb\u4e86\u5149\u751f\u8f7d\u6d41\u5b50\u7684\u5206\u79bb\u548c\u8fc1\u79fb\uff0c\u589e\u52a0\u4e86CO2<\/sub>\u7684\u5438\u9644\uff0c\u63d0\u4f9b\u4e86\u4e30\u5bcc\u7684\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\u3002\u56e0\u6b64\uff0c\u6700\u4f18\u7684ZnIn2<\/sub>S4<\/sub>-In2<\/sub>O3<\/sub>\u5206\u7ea7\u5f02\u8d28\u7ed3\u5149\u50ac\u5316\u5242\u663e\u793a\u51fa\u9ad8CO2<\/sub>\u8131\u6c27\u8fd8\u539f\u6d3b\u6027\u548c\u7a33\u5b9a\u6027\uff0cCO\u4ea7\u7387\u4e3a3075 \u03bcmol\u00b7h-1<\/sup>\u00b7g-1<\/sup>\u3002\u8fd9\u9879\u5de5\u4f5c\u53ef\u4e3a\u590d\u6742\u534a\u5bfc\u4f53\u57fa\u5149\u50ac\u5316\u5242\u7684\u8bbe\u8ba1\u548c\u6784\u7b51\u63d0\u4f9b\u6307\u5bfc\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a Construction of ZnIn2<\/sub>S4<\/sub>\u2212In2<\/sub>O3<\/sub> Hierarchical Tubular Heterostructures for Efficient CO2<\/sub> Photoreduction<\/a><\/strong> (J. Am. Chem. Soc.<\/strong>, 2018, DOI: 10.1021\/jacs.8b02200)<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u65b0\u80fd\u6e90\u5c0f\u7ec4abc940504\u7f16\u8bd1\u6574\u7406\uff0c\u53c2\u4e0e\u65b0\u80fd\u6e90\u8bdd\u9898\u8ba8\u8bba\u8bf7\u52a0\u5165\u201c\u6750\u6599\u4eba\u65b0\u80fd\u6e90\u6750\u6599\u4ea4\u6d41\u7fa4 422065953\u201d\u3002<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1aRDD-2011-CHERISH\uff0c\u4efb\u4e39\u4e39\uff0c\u6211\u4eec\u4f1a\u9080\u8bf7\u5404\u4f4d\u8001\u5e08\u52a0\u5165\u4e13\u5bb6\u7fa4\u3002<\/strong><\/p>\n

\u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u7f16\u8f91\u90e8<\/a><\/strong>\u3002\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n

\u4eea\u5668\u8bbe\u5907\u3001\u8bd5\u5242\u8017\u6750\u3001\u6750\u6599\u6d4b\u8bd5\u3001\u6570\u636e\u5206\u6790\uff0c\u627e\u6750\u6599\u4eba\u3001\u4e0a\u6d4b\u8bd5\u8c37<\/a><\/strong>\uff01<\/p>\n","protected":false},"excerpt":{"rendered":"

\u3010\u5f15\u8a00\u3011 \u4e3a\u66f4\u597d\u5730\u53d1\u6325\u5f02\u8d28\u7ed3\u5149\u50ac\u5316\u5242\u7684\u4f18\u52bf\uff0c\u5236\u5907\u5177\u6709\u9002\u5b9c\u7eb3\u7c73\u7ed3\u6784\u7684\u5149\u50ac\u5316\u5242\u81f3\u5173\u91cd\u8981\u3002\u5177\u6709\u72ec\u7279\u7ed3\u6784\u7684\u4e2d\u7a7a\u7c92\u5b50\u5df2\u5728\u4e0d\u540c\u7684\u7814\u7a76\u9886\u57df\u5c55\u9732\u4f18\u52bf\u3002\u8fd1\u6765\uff0c\u4e2d\u7a7a\u7ed3\u6784\u6750\u6599\u5df2\u88ab\u4f5c\u4e3a…<\/p>\n","protected":false},"author":4931,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[2564],"class_list":["post-135374","post","type-post","status-publish","format-standard","hentry","category-jiedu","tag-co2"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/135374"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/4931"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=135374"}],"version-history":[{"count":3,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/135374\/revisions"}],"predecessor-version":[{"id":135420,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/135374\/revisions\/135420"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=135374"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=135374"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=135374"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}