{"id":133492,"date":"2018-04-07T06:30:36","date_gmt":"2018-04-06T22:30:36","guid":{"rendered":"\/\/m.iemloyee.com\/?p=133492"},"modified":"2018-04-05T21:48:58","modified_gmt":"2018-04-05T13:48:58","slug":"acc-chem-res-%ef%bc%9a%e8%a7%a3%e5%af%86%e9%94%82%e7%a6%bb%e5%ad%90%e7%94%b5%e6%b1%a0%e4%b8%ad%e7%a2%b3%e9%85%b8%e4%b8%99%e7%83%af%e9%85%af%ef%bc%88pc%ef%bc%89%e5%92%8c%e7%a2%b3%e9%85%b8%e4%b9%99","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=133492","title":{"rendered":"Acc. Chem. Res.\uff1a\u89e3\u5bc6\u9502\u79bb\u5b50\u7535\u6c60\u4e2d\u78b3\u9178\u4e19\u70ef\u916f\uff08PC\uff09\u548c\u78b3\u9178\u4e59\u70ef\u916f\uff08EC\uff09\u7684\u5dee\u5f02"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

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\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6765\u81ea\u534e\u5357\u5e08\u8303\u5927\u5b66\u7684\u90a2\u4e3d\u4e39\u535a\u58eb\u3001\u674e\u4f1f\u5584\u6559\u6388\u4e0e\u7f8e\u56fd\u9646\u519b\u5b9e\u9a8c\u5ba4\u8bb8\u5eb7\u7814\u7a76\u5458<\/strong>(<\/strong>\u5171\u540c\u901a\u8baf\u4f5c\u8005<\/strong>)<\/strong>\u5408\u4f5c\uff0c\u5728Acc. Chem. Res.\u4e0a\u53d1\u8868\u9898\u4e3a\u201cDeciphering the Ethylene Carbonate\u2212Propylene Carbonate Mystery in Li-Ion Batteries\u201d\u7684\u7814\u7a76\u8bba\u6587\u3002\u4ed6\u4eec\u91c7\u7528\u91cf\u5b50\u5316\u5b66\u8ba1\u7b97\u548c\u5b9e\u9a8c\u65b9\u6cd5\u76f8\u7ed3\u5408\uff0c\u8be6\u7ec6\u7814\u7a76\u4e86\u9502\u79bb\u5b50\u7535\u6c60\u7535\u89e3\u6db2\u8131\u6eb6\u5242\u5316\u8fc7\u7a0b\u53ca\u5176\u4e0e\u77f3\u58a8\u754c\u9762\u76f8\u5bb9\u6027\u7684\u5173\u7cfb\uff0c\u53d1\u73b0\u9502\u76d0\u9634\u79bb\u5b50PF6<\/sub>–<\/sup>\u662f\u5bfc\u81f4PC\u4e0eEC\u754c\u9762\u884c\u4e3a\u5dee\u5f02\u7684\u6700\u6839\u672c\u539f\u56e0\u3002\u5f53\u77f3\u58a8\u7535\u6781\u7535\u538b\u4e0b\u964d\u65f6\uff08\u53d1\u751f\u5d4c\u9502\u53cd\u5e94\uff0c\u5373\u7535\u6c60\u5145\u7535\u8fc7\u7a0b\uff09\uff0c\u6eb6\u5242\u5316\u7684\u9502\u79bb\u5b50\u5728\u7535\u573a\u4f5c\u7528\u4e0b\u8fc1\u79fb\u5230\u77f3\u58a8\u8d1f\u6781\u8868\u9762\u3002\u7531\u4e8e\u6b64\u65f6\u9502\u79bb\u5b50\u6eb6\u5242\u5316\u5c42\u4f53\u79ef\u8fdc\u5927\u4e8e\u77f3\u58a8\u5c42\u5c42\u95f4\u8ddd\uff0c\u56e0\u6b64\u5728\u5d4c\u5165\u4ee5\u524d\u9700\u8981\u53d1\u751f\u8131\u6eb6\u5242\u5316\u3002EC\u57fa\u4f53\u7cfb\u9502\u79bb\u5b50\u8131\u6eb6\u5242\u5316\u5c42\u65f6\u4f18\u5148\u8131\u53bbEC\u5206\u5b50\uff0c\u5f62\u6210\u542bPF6<\/sub>–<\/sup>\u7684\u6eb6\u5242\u5316\u5c42\uff0cPF6<\/sub>–<\/sup>\u53c2\u4e0e\u968f\u540e\u7684\u8fd8\u539f\u5206\u89e3\uff0c\u5f62\u6210\u5bcc\u542bLiF\u7684\u7a33\u5b9aSEI\u819c\u3002\u7136\u800c\uff0cPC\u57fa\u4f53\u7cfb\u7684\u9502\u79bb\u5b50\u8131\u6eb6\u5242\u5316\u5c42\u65f6\u8131\u53bbPC\u5206\u5b50\u548cPF6<\/sub>–<\/sup>\u7684\u6982\u7387\u76f8\u5f53\uff0c\u56e0\u6b64\u53c2\u4e0e\u8fd8\u539f\u5206\u89e3\u7684PF6<\/sub>–<\/sup>\u542b\u91cf\u51cf\u5c11\uff0c\u5bfc\u81f4\u5f62\u6210\u7684\u5206\u89e3\u4ea7\u7269LiF\u542b\u91cf\u4f4e\u3002\u4ed6\u4eec\u540e\u7eed\u8bbe\u8ba1\u4e00\u7cfb\u5217\u7684\u5b9e\u9a8c\u8bc1\u660e\uff0cLiF\u542b\u91cf\u4f4e\u662f\u5bfc\u81f4PC\u57fa\u7535\u89e3\u6db2\u5206\u89e3\u4ea7\u7269\u65e0\u6cd5\u5f62\u6210\u81f4\u5bc6\u7a33\u5b9aSEI\u819c\u7684\u6839\u672c\u539f\u56e0\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe<\/strong>1. EC<\/strong>\u548c<\/strong>PC<\/strong>\u57fa\u7535\u89e3\u6db2\u5728\u7684\u7535\u5316\u5b66\u884c\u4e3a\u548c\u7ed3\u6784\u5dee\u5f02<\/strong><\/p>\n

\"\"<\/strong><\/p>\n

(a) EC\u548cPC\u57fa\u7535\u89e3\u6db2\u5728\u77f3\u58a8\u7535\u6781\u4e0a\u7684\u5145\u653e\u7535\u66f2\u7ebf<\/p>\n

(b) EC\u548cPC\u57fa\u7535\u89e3\u6db2\u4e2d\u5d4c\u5165\u77f3\u58a8\u5c42\u7684\u53ef\u80fd\u9502\u79bb\u5b50\u6eb6\u5242\u5316\u5c42\u7ed3\u6784<\/p>\n

\u56fe<\/strong>2. <\/strong>\u7535\u89e3\u6db2\u4e2d\u79bb\u5b50\u6eb6\u5242\u5316\u5c42\u5bf9\u5176\u7535\u5316\u5b66\u884c\u4e3a\u7684\u5f71\u54cd<\/strong><\/p>\n

\"\"<\/strong><\/p>\n

(a) \u7535\u55b7\u96fe\u7535\u79bb\u8d28\u8c31\u6cd5\u6d4b\u8bd5\u79bb\u5b50\u5316\u5c42\u7ed3\u6784<\/p>\n

(b) \u7535\u89e3\u6db2\u4e2d\u6eb6\u5242\u6bd4\u4f8b\u5bf9\u5176\u7535\u5316\u5b66\u6027\u80fd\u7684\u5f71\u54cd<\/p>\n

(c) \u79bb\u5b50\u5316\u5c42\u7ed3\u6784\u4e2dEC\u7684\u542b\u91cf\u4e0e\u7535\u89e3\u6db2\u4e2dEC\u6eb6\u5242\u542b\u91cf\u6bd4\u4f8b\u7684\u5173\u7cfb<\/p>\n

\u56fe<\/strong>3. <\/strong>\u6eb6\u5242\u5316\u5c42\u4e2d\u9502\u79bb\u5b50\u4e0e\u6eb6\u5242\u5206\u5b50\u548c\u9634\u79bb\u5b50\u7684\u7ed3\u5408\u80fd\u4e0e\u6eb6\u5242\u5206\u5b50\u6570\u7684\u5173\u7cfb<\/strong><\/p>\n

\"\"<\/strong><\/p>\n

(a) EC\u57fa\u7535\u89e3\u6db2\u4e2d\u9502\u79bb\u5b50\u4e0eEC\u548cPF6<\/sub>–<\/sup>\u7684\u7ed3\u5408\u80fd<\/p>\n

(b) PC\u57fa\u7535\u89e3\u6db2\u4e2d\u9502\u79bb\u5b50\u4e0ePC\u548cPF6<\/sub>–<\/sup>\u7684\u7ed3\u5408\u80fd<\/p>\n

\u56fe<\/strong>4. <\/strong>\u542b<\/strong>PF6<\/sub>–<\/sup><\/strong>\u7684\u6eb6\u5242\u5316\u5c42\u53d1\u751f\u5355\u7535\u5b50\u8fd8\u539f\u540e\u7684\u4f18\u5316\u7ed3\u6784<\/strong><\/p>\n

\"\"<\/strong><\/p>\n

\u56fe<\/strong>5. <\/strong>\u7535\u5b50\u4eb2\u5408\u80fd\u53ca\u4ea7\u7269\u7684\u524d\u7ebf\u5206\u5b50\u8f68\u9053\u80fd\u91cf<\/strong><\/p>\n

\"\"<\/strong><\/p>\n

(a) \u542bPF6<\/sub>–<\/sup>\u7684\u6eb6\u5242\u5316\u5c42\u7535\u5b50\u4eb2\u5408\u80fd<\/p>\n

(b) \u90e8\u5206\u4e3b\u8981\u7535\u89e3\u6db2\u5206\u89e3\u4ea7\u7269\u7684\u524d\u7ebf\u5206\u5b50\u8f68\u9053\u80fd\u91cf\u4e0e\u7535\u5b50\u963b\u9694\u80fd\u529b\u7684\u5173\u7cfb<\/p>\n

\u8868<\/strong>1. <\/strong>\u77f3\u58a8\u7535\u6781\u5728\u4e0d\u540c\u7535\u89e3\u6db2\u4e2d\u5faa\u73af\u540e\u8868\u9762<\/strong>LiF<\/strong>\u7684\u542b\u91cf<\/strong><\/p>\n

\"\"<\/strong><\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u672c\u6210\u679c\u91c7\u7528\u7406\u8bba\u8ba1\u7b97\u5316\u5b66\u4e0e\u5b9e\u9a8c\u65b9\u6cd5\u76f8\u7ed3\u5408\uff0c\u9610\u660e\u4e86\u7535\u89e3\u6db2\u4e2d\u9502\u79bb\u5b50\u6eb6\u5242\u5316\u5c42\u8131\u6eb6\u5242\u5316\u8fc7\u7a0b\u5bf9\u7535\u6781\/\u7535\u89e3\u6db2\u754c\u9762\u6027\u8d28\u7684\u91cd\u8981\u5f71\u54cd\uff0c\u6307\u51fa\u9502\u76d0\u9634\u79bb\u5b50\u662f\u5426\u53c2\u4e0e\u8fd8\u539f\u5206\u89e3\u53cd\u5e94\u662f\u51b3\u5b9a\u4e86EC\u57fa\u7535\u89e3\u6db2\u548cPC\u57fa\u7535\u89e3\u6db2\u5728\u77f3\u58a8\u7535\u6781\u754c\u9762\u884c\u4e3a\u622a\u7136\u4e0d\u540c\u7684\u6839\u672c\u539f\u56e0\u3002\u8be5\u6210\u679c\u4e0d\u4ec5\u89e3\u51b3\u4e86\u9502\u79bb\u5b50\u7535\u6c60\u7684\u957f\u671f\u4e89\u8bba\u7684\u95ee\u9898\uff0c\u4e5f\u4e3a\u5176\u4ed6\u9ad8\u80fd\u7535\u6c60\u7684\u8bbe\u8ba1\u548c\u5e94\u7528\u6307\u660e\u4e86\u65b9\u5411\u3002\u8be5\u56e2\u961f\u5728\u7535\u6781\/\u7535\u89e3\u6db2\u754c\u9762\u6027\u8d28\u7814\u7a76\u65b9\u9762\u53d6\u5f97\u7cfb\u5217\u7814\u7a76\u6210\u679c\uff0c\u5982\uff1a<\/p>\n

[1].\u00a0 Huozhen Zhi, Lidan Xing*, Xiongwen Zheng, Kang Xu, Weishan Li*, Understanding How Nitriles Stabilize Electrolyte\/Electrode Interface at High Voltage, J. Phys. Chem. Lett. 2017, 8, 6048\u22126052.<\/p>\n

[2].\u00a0 Yating Wang, Lidan Xing*, Weishan Li*, and Dmitry Bedrov, Why Do Sulfone-Based Electrolytes Show Stability at High Voltages? Insight from Density Functional Theory, J. Phys. Chem. Lett. 2013, 4:3992-3999.<\/p>\n

\u6587\u7ae0\u94fe\u63a5\uff1aDeciphering the Ethylene Carbonate\u2212Propylene Carbonate Mystery in Li-Ion Batteries<\/a><\/strong>\u00a0(Acc. Chem. Res., 2018, DOI: 10.1021\/acs.accounts.7b00474)<\/p>\n

\u3010\u901a\u8baf\u4f5c\u8005\u4ecb\u7ecd\u3011<\/strong><\/p>\n

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\u8bb8\u5eb7<\/strong>\uff1a\u7f8e\u56fd\u9646\u519b\u5b9e\u9a8c\u5ba4\u9ad8\u7ea7\u79d1\u5b66\u5bb6\u3001\u7f8e\u56fd\u6a61\u6811\u5cad\u8054\u5408\u5927\u5b66\u56fd\u5bb6\u7814\u7a76\u59d4\u5458\u987e\u95ee\u3002\u4ece\u4e8b\u7535\u89e3\u6db2\u6750\u6599\u548c\u754c\u9762\u5316\u5b66\u5de5\u4f5c\u4e8c\u5341\u4f59\u5e74\uff0c\u591a\u6b21\u83b7\u5f97\u56fd\u9632\u90e8\u53ca\u56fd\u9645\u5956\u52b1\uff0c\u5305\u62ec\u201cBest Paper Award of Army Science (2010)\u201d, \u201cInvention of the Year Award (2016)\u201d \u548c \u201cInternational Battery Association Technology Award (2017)\u201d\u7b49\u3002\u5728\u56fd\u9645TOP\u671f\u520a\u4e0a\u53d1\u8868\u8bba\u6587160\u591a\u7bc7\uff0c\u6587\u7ae0\u5f15\u7528\u6b21\u6570\u8d85\u8fc713,000\u6b21\uff0cH\u56e0\u5b5061\u30022004\u5e74\u548c2014\u5e74\u53d1\u8868\u5728Chemical Review\u4e0a\u7684\u4e24\u7bc7\u5173\u4e8e\u7535\u89e3\u6db2\u7814\u7a76\u8fdb\u5c55\u88ab\u8a89\u4e3a\u7535\u6c60\u7814\u7a76\u5de5\u4f5c\u8005\u7684\u201c\u6807\u51c6\u53c2\u8003\u4e66\u201d\u3002<\/p>\n

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