{"id":131531,"date":"2018-03-25T06:30:59","date_gmt":"2018-03-24T22:30:59","guid":{"rendered":"\/\/m.iemloyee.com\/?p=131531"},"modified":"2018-03-23T19:02:36","modified_gmt":"2018-03-23T11:02:36","slug":"angew-chem-int-ed-%ef%bc%9a%e5%85%b7%e6%9c%89%e9%85%b8%e7%a2%b1%e7%bc%93%e5%86%b2%e6%95%88%e5%ba%94%e7%9a%84%e7%a8%b3%e5%ae%9a%e6%80%a7mof%e6%9d%90%e6%96%99%e7%9a%84%e5%88%b6%e5%a4%87%e4%bb%a5","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=131531","title":{"rendered":"Angew. Chem. Int. Ed. \uff1a\u5177\u6709\u9178\u78b1\u7f13\u51b2\u6548\u5e94\u7684\u7a33\u5b9a\u6027MOF\u6750\u6599\u7684\u5236\u5907\u4ee5\u53ca\u56fa\u5b9aCO2\u7684\u5e94\u7528"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u5728\u9178\u6027\u3001\u4e2d\u6027\u6216\u78b1\u6027\u6c34\u6eb6\u6db2\u4e2d\uff0c\u5927\u591a\u6570\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6\uff08MOFs\uff09\u4e0d\u80fd\u4fdd\u6301\u5176\u7269\u7406\u548c\u5316\u5b66\u6027\u8d28\uff0c\u9650\u5236\u4e86\u5b83\u4eec\u5728\u8bb8\u591a\u9886\u57df\u7684\u5b9e\u9645\u5e94\u7528\u3002\u56e0\u6b64\u5982\u4f55\u63d0\u9ad8MOF\u6750\u6599\u7684\u7a33\u5b9a\u6027\uff0c\u4e00\u76f4\u662f\u4e00\u4e2a\u503c\u5f97\u63a2\u7d22\u7684\u95ee\u9898\u3002\u53d7\u5230\u9178\u78b1\u7f13\u51b2\u6eb6\u6db2\u7684\u542f\u53d1\uff0c\u672c\u6587\u9996\u6b21\u63d0\u51fa\u5229\u7528\u56fa\u4f53\u9178\u78b1\u7f13\u51b2\u7b56\u7565\u63d0\u9ad8MOFs\u6750\u6599\u7684\u7a33\u5b9a\u6027\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u4e1c\u5317\u5e08\u8303\u5927\u5b66\u7684\u6731\u5e7f\u5c71\u6559\u6388\u548c\u5357\u4f5b\u7f57\u91cc\u8fbe\u5927\u5b66\u7684\u9a6c\u80dc\u524d\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\uff0c\u8bbe\u8ba1\u5408\u6210\u542b\u6709\u9178\u548c\u78b1\u53cc\u5b98\u80fd\u56e2\u7684\u6709\u673a\u914d\u4f53\u4f5c\u4e3a\u56fa\u4f53\u7f13\u51b2\u4fdd\u62a4\u5bf9\uff0c\u4fdd\u8bc1\u591a\u5b54MOF\uff08JUC-1000\uff09\u80fd\u591f\u5728\u6c34\u6027\u6eb6\u6db2\u4e2d\u4fdd\u6301\u7a33\u5b9a\uff1b\u540c\u65f6\u5728\u4f4ePH\u503c\u548c\u9ad8PH\u503c\u4e0b\u4fdd\u6301\u5176\u7ed3\u6784\u5b8c\u6574\u6027\u3002\u7531\u4e8e\u9ad8\u7684CO2<\/sub>\u5438\u9644\u91cf\u3001\u9ad8\u7a33\u5b9a\u6027\u548c\u591a\u50ac\u5316\u4f4d\u70b9\uff0cJUC-1000\u5c55\u73b0\u4e86\u51fa\u8272\u7684CO2<\/sub>\u5316\u5b66\u56fa\u5b9a\u6548\u679c\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201c<\/strong>A Stable Metal\u2013Organic Framework Featuring a Local Buffer Environment for Carbon Dioxide Fixation<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Angewandte Chemie International Edition<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe<\/strong>1 MOF<\/strong>\u56fa\u4f53\u7f13\u51b2\u7b56\u7565\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u6784\u7b51MOFs\u6750\u6599\u7684\u56fa\u4f53\u7f13\u51b2\u7b56\u7565\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe<\/strong>2<\/strong>\u6750\u6599\u7684\u5408\u6210\u7ed3\u6784\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u6750\u6599\u7684\u5408\u6210\u7ed3\u6784\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe<\/strong>3 <\/strong>\u6676\u4f53\u7684\u5b54\u9053\u7ed3\u6784\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

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\u56fe<\/strong>4 JUC-1000<\/strong>\u7684\u6bd4\u8868\u9762\u79ef\u53ca\u5176\u5b54\u5f84\u5206\u5e03\u56fe<\/strong><\/p>\n

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77K\u7684\u6c2e\u6c14\u8131\u5438\u9644\u66f2\u7ebf\u548c\u5b54\u5f84\u5206\u5e03\u56fe\uff08\u63d2\u5165\u56fe\uff0c\u91c7\u7528DFT\u65b9\u6cd5\u8ba1\u7b97\uff09\u3002<\/p>\n

\u56fe<\/strong>5 JUC-1000<\/strong>\u548c\u591a\u79cd\u7ecf\u5178<\/strong>MOFs<\/strong>\u6750\u6599\u7684\u7a33\u5b9a\u6027\u5bf9\u6bd4\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

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\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u672c\u6587\u91c7\u7528\u81ea\u5236\u7684\u542b\u6709\u9178\u78b1\u5b98\u80fd\u56e2\u7684\u6709\u673a\u914d\u4f53\uff0c\u83b7\u5f97\u4e86\u4e00\u79cd\u5316\u5b66\u6027\u80fd\u7a33\u5b9a\u7684Cu-MOF\uff08JUC-1000\uff09\u3002\u5f97\u76ca\u4e8eJUC-1000\u4e2d\u7684\u9178\u78b1\u5bf9\u548c\u91d1\u5c5e\u4f4d\u70b9\uff0c\u8fd9\u79cd\u6750\u6599\u53ef\u4ee5\u5316\u5b66\u5b9a\u4f4dCO2<\/sub>\u6210\u73af\u78b3\u9178\u916f\u3002\u8be5\u65b9\u6cd5\u5177\u6709\u975e\u5e38\u597d\u7684\u5f00\u62d3\u6027\u548c\u521b\u65b0\u6027\uff0c\u8fd9\u4e3a\u8bbe\u8ba1\u548c\u5236\u5907\u9ad8\u7a33\u5b9a\u7684\u591a\u5b54MOFs\u5f00\u8f9f\u4e86\u65b0\u601d\u8def\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>“<\/strong>A Stable Metal\u2013Organic Framework Featuring a Local Buffer Environment for Carbon Dioxide Fixation<\/strong>“<\/strong><\/a> \uff08Angewandte Chemie International Edition, 2018, DOI: 10.1002\/anie.201801122\uff09\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com<\/a>\u3002<\/p>\n

\u6750\u6599\u725b\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u8fd9\u91cc\u6c47\u96c6\u4e86\u5404\u5927\u9ad8\u6821\u7855\u535a\u751f\u3001\u4e00\u7ebf\u79d1\u7814\u4eba\u5458\u4ee5\u53ca\u884c\u4e1a\u4ece\u4e1a\u8005\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u6750\u6599\u4eba\u7f16\u8f91\u90e8<\/a>\u3002<\/p>\n

\u6750\u6599\u6d4b\u8bd5\uff0c\u6570\u636e\u5206\u6790\uff0c\u4e0a<\/strong>\u6d4b\u8bd5\u8c37<\/strong><\/a>\uff01<\/strong><\/p>\n","protected":false},"excerpt":{"rendered":"

\u3010\u5f15\u8a00\u3011 \u5728\u9178\u6027\u3001\u4e2d\u6027\u6216\u78b1\u6027\u6c34\u6eb6\u6db2\u4e2d\uff0c\u5927\u591a\u6570\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6\uff08MOFs\uff09\u4e0d\u80fd\u4fdd\u6301\u5176\u7269\u7406\u548c\u5316\u5b66\u6027\u8d28\uff0c\u9650\u5236\u4e86\u5b83\u4eec\u5728\u8bb8\u591a\u9886\u57df\u7684\u5b9e\u9645\u5e94\u7528\u3002\u56e0\u6b64\u5982\u4f55\u63d0\u9ad8MOF\u6750\u6599\u7684\u7a33\u5b9a\u6027\uff0c\u4e00…<\/p>\n","protected":false},"author":7035,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[2975,245],"class_list":["post-131531","post","type-post","status-publish","format-standard","hentry","category-jiedu","tag-2975","tag-mof"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/131531"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/7035"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=131531"}],"version-history":[{"count":3,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/131531\/revisions"}],"predecessor-version":[{"id":131725,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/131531\/revisions\/131725"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=131531"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=131531"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=131531"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}