{"id":131362,"date":"2018-03-25T06:30:56","date_gmt":"2018-03-24T22:30:56","guid":{"rendered":"\/\/m.iemloyee.com\/?p=131362"},"modified":"2018-03-25T20:59:50","modified_gmt":"2018-03-25T12:59:50","slug":"%e4%b8%8a%e6%b5%b7%e4%ba%a4%e5%a4%a7%e9%82%ac%e5%89%91%e6%b3%a2nat-commun-%ef%bc%9a%e6%a0%b8%e5%a3%b3%e7%ba%b3%e7%b1%b3%e9%a2%97%e7%b2%92%e4%b8%ad%e9%9d%9e%e5%af%b9%e7%a7%b0%e8%85%90%e8%9a%80","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=131362","title":{"rendered":"\u4e0a\u6d77\u4ea4\u5927\u90ac\u5251\u6ce2Nat. Commun.\uff1a\u6838\u58f3\u7eb3\u7c73\u9897\u7c92\u4e2d\u975e\u5bf9\u79f0\u8150\u8680\u7684\u7eb3\u7c73\u5c3a\u5ea6\u52a8\u529b\u5b66"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u76ee\u524d\uff0cPt\u57fa\u7eb3\u7c73\u9897\u7c92\u51ed\u501f\u5176\u5728\u50ac\u5316\u6d3b\u6027\u548c\u7a33\u5b9a\u6027\u65b9\u9762\u7684\u6f5c\u5728\u4f18\u52bf\uff0c\u5e7f\u6cdb\u5e94\u7528\u4e8e\u5728\u71c3\u6599\u7535\u6c60\u6b63\u6781\u7684\u6c27\u8fd8\u539f\u53cd\u5e94\u4e2d\u8d77\u50ac\u5316\u4f5c\u7528\u3002\u7136\u800c\uff0c\u7531\u4e8e\u7279\u6b8a\u5f62\u72b6\u635f\u5931\u548c\u5143\u7d20\u6eb6\u89e3\u9020\u6210\u7684\u6d3b\u6027\u9aa4\u51cf\uff0c\u4ecd\u662f\u5546\u4e1a\u5316\u63a8\u5e7f\u4e2d\u7684\u4e00\u5927\u963b\u788d\u3002\u8bbe\u8ba1\u51fa\u8010\u8150\u8680\u7684\u65b0\u6750\u6599\u548c\u7ed3\u6784\uff0c\u9700\u8981\u5bf9\u8150\u8680\u52a8\u529b\u5b66\u6709\u5f88\u597d\u7684\u7406\u89e3\u3002\u6839\u636e\u5df2\u6709\u7814\u7a76\u53ef\u77e5\uff0c\u5bf9\u4e2d\u95f4\u6001\u52a8\u529b\u5b66\u7684\u63a2\u7d22\u662f\u63ed\u793a\u50ac\u5316\u8870\u51cf\u52a8\u529b\u5b66\u548c\u9ad8\u6d3b\u6027\u957f\u5bff\u547d\u7eb3\u7c73\u7ed3\u6784\u5f62\u6210\u7684\u5173\u952e\u6240\u5728\uff0c\u4e14\u4e24\u8005\u5bf9\u4e8e\u8bbe\u8ba1\u9ad8\u6d3b\u6027\u548c\u7a33\u5b9a\u6027\u7684\u50ac\u5316\u6750\u6599\u90fd\u662f\u4e0d\u53ef\u6216\u7f3a\u7684\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u4e0a\u6d77\u4ea4\u901a\u5927\u5b66\u7684\u90ac\u5251\u6ce2\u6559\u6388<\/strong>\u4e0e\u52a0\u5dde\u5927\u5b66\u5c14\u6e7e\u5206\u6821<\/strong>\u7684\u6f58\u6653\u6674<\/strong>\u6559\u6388<\/strong>\u3001\u6d59\u6c5f\u5927\u5b66<\/strong>\u7684\u5f20\u8f89\u6559\u6388<\/strong>\u5408\u4f5c\uff0c\u5728Nature Communications<\/strong>\u4e0a\u53d1\u8868\u4e86\u4e00\u7bc7\u9898\u4e3a\u201cNanoscale kinetics of asymmetrical corrosion in core-shell nanoparticles<\/strong>\u201d\u7684\u6587\u7ae0\u3002\u901a\u8fc7\u5728\u6db2\u4f53\u73af\u5883\u900f\u5c04\u7535\u955c\u4e0b\u89c2\u5bdf\uff0c\u4f5c\u8005\u5bf9Pd@Pt\u6838\u58f3\u7eb3\u7c73\u7acb\u65b9\u9897\u7c92\u7684\u5b9e\u65f6\u8150\u8680\u8fc7\u7a0b\u5c55\u5f00\u7814\u7a76\u3002\u7ed3\u679c\u663e\u793a\uff0c\u8150\u8680\u8fc7\u7a0b\u4e2d\u7684\u591a\u79cd\u8680\u523b\u673a\u5236\u5bfc\u81f4\u5f62\u6001\u6f14\u5316\uff0c\u5305\u62ec\u5728\u975e\u7f3a\u9677\u4f4d\u7684\u6162\u52a8\u529b\u5b66\u7535\u8150\u8680\u548c\u5728\u8150\u8680\u4f4d\u7f6e\u5364\u7d20\u8bf1\u5bfc\u7684\u66f4\u5feb\u901f\u7387\u8150\u8680\u3002\u68f1\u89d2\u5904\u662f\u6613\u8150\u8680\u4f4d\u7f6e\uff0c\u4e24\u79cd\u8150\u8680\u673a\u5236\u5728\u8150\u8680\u8fc7\u7a0b\u4e2d\u76f8\u4e92\u6291\u5236\u3002\u4ee5\u4e0a\u5173\u4e8e\u6d3b\u6027\u6db2\u4f53\u73af\u5883\u4e2d\u7eb3\u7c73\u7ed3\u6784\u6f14\u53d8\u73b0\u8c61\uff0c\u6709\u52a9\u4e8e\u66f4\u597d\u5730\u8c03\u5236\u8868\u9762\u7ed3\u6784\u6765\u63d0\u5347\u7535\u5316\u5b66\u7a33\u5b9a\u6027\uff0c\u6b64\u5916\u8fd8\u53ef\u77e5\u9053\u8bbe\u8ba1\u4e00\u79cd\u6709\u66f4\u591a\u50ac\u5316\u6d3b\u6027\u4f4d\u7f6e\u7684\u65b0\u7684\u591a\u5b54\u7ed3\u6784\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe1\uff1a\u5e38\u89c4\u548c\u68f1\u89d2\u7f3a\u5931\u7684\u7acb\u65b9\u9897\u7c92\u7684\u8150\u8680\u8fc7\u7a0b\u3002<\/strong><\/p>\n

\"\"<\/p>\n

(a,b)\u6309\u65f6\u95f4\u987a\u5e8f\u6392\u5217\u7684\u900f\u5c04\u7535\u955c\u56fe\u50cf\uff0c\u4f9d\u6b21\u8868\u5f81\u5728\u5355\u4e2a\u5e38\u89c4\u548c\u68f1\u89d2\u7f3a\u9677\u7684Pd@Pt\u7acb\u65b9\u9897\u7c92\u4e2d\uff0c\u5185\u90e8Pd\u539f\u5b50\u7684\u8150\u8680\u8fc7\u7a0b\uff1b<\/p>\n

(c)\u8bf4\u660eC<\/em>a<\/sub>\u8ba1\u7b97\u7684\u539f\u5b50\u7ed3\u6784\u793a\u610f\u56fe\uff1b<\/p>\n

(d) C<\/em>a<\/sub>\u7684\u6563\u70b9\u56fe\u53ca\u62df\u5408\u66f2\u7ebf\uff1b<\/p>\n

(e)d\u56fe\u4e2d\u8150\u8680\u533a\u57df\u7684\u76f8\u5e94\u901f\u7387\u3002<\/p>\n

\u56fe2\uff1a\u5e73\u53f0\u5f62\u7f3a\u9677\u7acb\u65b9\u9897\u7c92\u7684\u8150\u8680\u8fc7\u7a0b\u3002<\/strong><\/p>\n

\"\"<\/p>\n

(a) \u6309\u65f6\u95f4\u987a\u5e8f\u6392\u5217\u7684\u900f\u5c04\u7535\u955c\u56fe\u50cf\uff0c\u8868\u5f81\u5728\u5355\u4e2a\u5e73\u53f0\u72b6\u7f3a\u9677\u7684Pd@Pt\u7acb\u65b9\u9897\u7c92\u4e2d\uff0c\u5185\u90e8Pd\u539f\u5b50\u7684\u8150\u8680\u8fc7\u7a0b\uff1b<\/p>\n

(b) \u8bf4\u660eC<\/em>a<\/sub>\u8ba1\u7b97\u7684\u539f\u5b50\u7ed3\u6784\u793a\u610f\u56fe\uff1b<\/p>\n

(c) C<\/em>a<\/sub>\u7684\u6563\u70b9\u56fe\u53ca\u62df\u5408\u66f2\u7ebf\uff1b<\/p>\n

(d) \u5bf9\u5e94c\u56fe\u7acb\u65b9\u9897\u7c92\u4e2d\u88ab\u8150\u8680\u533a\u57df\uff0c\u6cbf\u5404\u4e2a\u65b9\u5411\u7684\u8150\u8680\u901f\u7387\uff1b<\/p>\n

(e) \u6cbf\u5e73\u53f0\u72b6\u7f3a\u9677\u7684\u8150\u8680\u8fc7\u7a0b\u4e2d\u7684\u8868\u9762\u5fae\u89c2\u66f2\u7387\u7684\u6f14\u53d8\u56fe\uff1b<\/p>\n

(f) \u8150\u8680\u901f\u7387\u548c\u5fae\u89c2\u66f2\u7387\u7684\u5173\u7cfb\u3002<\/p>\n

\u56fe3\uff1a\u7acb\u65b9\u9897\u7c92\u7684HRTEM\u548cHADDF-STEM\u8868\u5f81\u3002<\/strong><\/p>\n

\"\"<\/p>\n

(a-l) \u5e38\u89c4(a-d)\u3001\u68f1\u89d2\u7f3a\u9677(e-h)\u548c\u5e73\u53f0\u72b6\u7f3a\u9677(i-l)\u7684Pd@Pt\u7acb\u65b9\u9897\u7c92\u5728\u88ab\u8150\u8680\u524d\u7684HRTEM\u548cHADDF-STEM\u7684\u56fe\u50cf\uff1b<\/p>\n

(m-o) \u4f9d\u6b21\u8868\u793a\uff0c\u5e38\u89c4\u3001\u68f1\u89d2\u7f3a\u9677\u548c\u5e73\u53f0\u72b6\u7f3a\u9677\u7684\u7acb\u65b9\u9897\u7c92\u4e2d\u751f\u6210\u7684Pt\u58f3\u72b6\u7ed3\u6784\uff1b<\/p>\n

(p-r) m\u56fe\u4e2dPt\u58f3\u72b6\u7ed3\u6784\u7684EDS\u5143\u7d20\u5206\u5e03\u3002<\/p>\n

\u56fe4\uff1a\u7acb\u65b9\u9897\u7c92\u7684\u8150\u8680\u901f\u7387\u548c\u914d\u4f4d\u6570\u3002<\/strong><\/p>\n

\"\"<\/p>\n

(a) \u4f9d\u6b21\u5728\u5e38\u89c4\u3001\u68f1\u89d2\u7f3a\u9677\u548c\u5e73\u53f0\u72b6\u7f3a\u9677\u7684\u7acb\u65b9\u9897\u7c92\u4e2d\uff0c\u6d4b\u5f97\u7684\u6cbf\u7279\u5f81\u65b9\u5411\u7684\u8150\u8680\u6295\u5f71\u968f\u65f6\u95f4\u7684\u53d8\u5316\uff1b<\/p>\n

(b) Pd\u7acb\u65b9\u9897\u7c92\u5185\u90e8\u7684\u8868\u9762\u539f\u5b50\u7684\u914d\u4f4d\u6570\u5206\u5e03\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u603b\u7684\u6765\u8bf4\uff0c\u901a\u8fc7\u5728\u6db2\u4f53\u73af\u5883\u900f\u5c04\u7535\u955c\u4e0b\u5b9e\u65f6\u6355\u6349Pd@Pt\u7acb\u65b9\u9897\u7c92\u7684\u8150\u8680\u8fc7\u7a0b\u548cPt\u58f3\u7684\u5f62\u6210\uff0c\u6765\u8bc6\u522b\u5728\u975e\u7f3a\u9677\u4f4d\u53d1\u751f\u7684\u975e\u76f4\u63a5\u63a5\u89e6\u7535\u5316\u5b66\u6162\u8150\u8680<\/strong>\u548c\u7f3a\u9677\u4f4d\u53d1\u751f\u7684\u76f4\u63a5\u63a5\u89e6\u5364\u7d20\u8bf1\u5bfc\u8150\u8680<\/strong>\u4e24\u7c7b\u8150\u8680\u673a\u5236\uff0c\u5bfc\u81f4\u8150\u8680\u884c\u4e3a\u548c\u7eb3\u7c73\u7ed3\u6784\u7684\u5f62\u6001\u6f14\u5316\u3002\u7531\u4e8e\u53cd\u5e94\u8fc7\u7a0b\u4e2d\u7535\u5b50\u7684\u91cf\u6709\u9650\uff0c\u4e24\u79cd\u8150\u8680\u540c\u65f6\u53d1\u751f\u4e14\u76f8\u4e92\u7ade\u4e89\uff0c\u68f1\u89d2\u5904\u662f\u6700\u521d\u59cb\u548c\u6700\u6613\u88ab\u8150\u8680\u7684\u4f4d\u7f6e\u3002\u4e0a\u8ff0\u5728\u7eb3\u7c73\u5c3a\u5ea6\u7684\u8150\u8680\u52a8\u529b\u5b66\uff0c\u4e3a\u8c03\u5236\u8868\u9762\u7f3a\u9677\uff0c\u4ee5\u671f\u83b7\u5f97\u591a\u91d1\u5c5e\u6838\u58f3\u7ed3\u6784\u7535\u50ac\u5316\u5242\uff0c\u63d0\u9ad8\u5176\u5728\u71c3\u6599\u7535\u6c60\u6c27\u8fd8\u539f\u53cd\u5e94\u4e2d\u7684\u7a33\u5b9a\u6027\u63d0\u4f9b\u4e86\u5f88\u597d\u7684\u601d\u8def\u3002\u6b64\u5916\uff0c\u4f7f\u7528\u539f\u4f4d\u89c2\u5bdf\u65b9\u6cd5\u6765\u7814\u7a76\u76f8\u5173\u95ee\u9898\uff0c\u53ef\u4ee5\u4e3a\u7ed3\u6784\u6f14\u5316\u53ca\u5176\u673a\u5236\u63d0\u4f9b\u66f4\u4e3a\u672c\u8d28\u7684\u7406\u89e3\uff0c\u4e0d\u4ec5\u53ef\u4ee5\u7528\u4e8e\u71c3\u6599\u7535\u6c60\u9886\u57df\uff0c\u8fd8\u53ef\u62d3\u5c55\u81f3\u53ef\u518d\u751f\u80fd\u6e90\u9886\u57df\u7684\u7535\u5316\u5b66\u53cd\u5e94\u4e2d\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Nanoscale kinetics of asymmetrical corrosion in core-shell nanoparticles<\/a>\uff08Nat. Commun.\uff0c2018\uff0cDOI: 10.1038\/s41467-018-03372-z\uff09<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u8ba1\u7b97\u6750\u6599\u7ec4Isobel\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n

\u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u8fd9\u91cc\u6c47\u96c6\u4e86\u5404\u5927\u9ad8\u6821\u7855\u535a\u751f\u3001\u4e00\u7ebf\u79d1\u7814\u4eba\u5458\u4ee5\u53ca\u884c\u4e1a\u4ece\u4e1a\u8005\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u7f16\u8f91\u90e8\u5927\u5bb6\u5ead<\/a>\u3002<\/p>\n

\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n

\u6750\u6599\u6d4b\u8bd5\u3001\u6570\u636e\u5206\u6790\uff0c\u4e0a<\/strong>\u6d4b\u8bd5\u8c37<\/strong><\/a>\uff01<\/strong><\/p>\n","protected":false},"excerpt":{"rendered":"

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