{"id":13130,"date":"2016-05-14T17:00:17","date_gmt":"2016-05-14T09:00:17","guid":{"rendered":"\/\/m.iemloyee.com\/?p=13130"},"modified":"2016-05-14T15:40:50","modified_gmt":"2016-05-14T07:40:50","slug":"%e9%a1%b6%e5%88%8a%e5%8a%a8%e6%80%81jacsangewamnc%e8%bf%91%e6%9c%9fmofs%e6%9d%90%e6%96%99%e7%a0%94%e7%a9%b6%e8%bf%9b%e5%b1%95%e6%b1%87%e6%80%bb","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=13130","title":{"rendered":"\u9876\u520a\u52a8\u6001|JACS\/Angew\/AM\/NC\u8fd1\u671fMOFs\u6750\u6599\u7814\u7a76\u8fdb\u5c55\u6c47\u603b"},"content":{"rendered":"<p><strong><b>1\u3001Angew.Chem\uff1a \u805a\u4e8c\u7532\u57fa\u7845\u6c27\u70f7\u6d82\u8986MOF\/Pd\u590d\u5408\u7269\uff1a\u901a\u8fc7\u8868\u9762\u758f\u6c34\u5316\u9ad8\u5ea6\u6539\u5584\u5176\u50ac\u5316\u6027\u80fd<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone wp-image-13131\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72471-12-300x124.jpg\" alt=\"\u56fe\u72471\" width=\"457\" height=\"189\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72471-12-300x124.jpg 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72471-12-768x317.jpg 768w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72471-12.jpg 992w\" sizes=\"(max-width: 457px) 100vw, 457px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe1 Pd\/UiO-66@PDMS\u7684\u5408\u6210\u8def\u7ebf<\/p>\n<p>\u6d3b\u6027\u4f4d\u70b9\u7684\u8868\u9762\u8868\u9762\u6da6\u6e7f\u6027\u5bf9\u4e8e\u50ac\u5316\u5242\u7684\u6d3b\u6027\u548c\u9009\u62e9\u6027\u81f3\u5173\u91cd\u8981\uff0c\u4eb2\u6c34\u6027\u6216\u758f\u6c34\u7684\u50ac\u5316\u5242\u8868\u9762\u5bf9\u4e8e\u76f8\u5e94\u57fa\u5e95\u5177\u6709\u7279\u5b9a\u4eb2\u548c\u529b\uff0c\u8fd9\u5bf9\u50ac\u5316\u8f6c\u5316\u662f\u975e\u5e38\u6709\u5229\u7684\uff0c\u4f8b\u5982\uff0c\u758f\u6c34\u6027\u56fa\u4f53\u9178\u6216\u78b1\u50ac\u5316\u5242\u5bf9\u8bb8\u591a\u53cd\u5e94\u4e2d\u5c55\u73b0\u51fa\u9ad8\u7684\u6d3b\u6027\uff0c\u5305\u62ec\u758f\u6c34\u6027\u53cd\u5e94\u7269\u3002\u6b64\u5916\uff0c\u91d1\u5c5e\u7eb3\u7c73\u7c92\u5b50\u5728\u8bb8\u591a\u53cd\u5e94\u4e2d\u5177\u6709\u5f88\u597d\u7684\u6d3b\u6027\uff0c\u4f46\u662f\u5f88\u5bb9\u6613\u56e2\u805a\uff0c\u5c06\u5176\u5f15\u5165\u5230\u591a\u5b54\u6750\u6599\uff0c\u5982MOF\u4e2d\uff0c\u53ef\u4ee5\u4f7f\u5176\u6709\u6548\u7a33\u5b9a\u3002\u5728\u6b64\u60c5\u51b5\u4e0b\uff0c\u5b54\u8868\u9762\u7684\u758f\u6c34\u6539\u6027\u53ef\u4ee5\u63d0\u9ad8\u50ac\u5316\u6027\u80fd\u3002<\/p>\n<p>\u8fd1\u65e5\uff0c\u4e2d\u79d1\u5927\u6c5f\u6d77\u9f99\u6559\u6388\u7814\u7a76\u56e2\u961f\uff0c\u5229\u7528\u7b80\u5355\u7684\u805a\u4e8c\u7532\u57fa\u7845\u6c27\u70f7\uff08PDMS\uff09\u6d82\u8986\u5bf9Pd\/UiO-66\u7684\u8868\u9762\u758f\u6c34\u6539\u6027\uff0c\u6539\u6027\u540e\u7684\u50ac\u5316\u5242\u7684\u50ac\u5316\u6027\u80fd\u6709\u4e86\u6781\u5927\u7684\u63d0\u9ad8\uff0c\u8fd9\u79cd\u65b9\u6cd5\u53ef\u4ee5\u6269\u5c55\u5230\u5404\u79cd\u94af\u7eb3\u7c73\u9897\u7c92\u50ac\u5316\u5242\u53cd\u5e94\u6d3b\u6027\u7684\u589e\u5f3a\uff0c\u5305\u62ec\u758f\u6c34\u53cd\u5e94\u7269\uff0c\u56e0\u4e3a\u758f\u6c34\u8868\u9762\u6709\u5229\u4e8e\u758f\u6c34\u6027\u886c\u5e95\u5728\u50ac\u5316\u4f4d\u70b9\u5468\u56f4\u5bcc\u96c6\u3002\u6b64\u5916\uff0cPDMS\u6d82\u8986\u9002\u7528\u4e8e\u5404\u79cd\u4e0d\u540c\u7684\u50ac\u5316\u5242\uff0c\u5728\u5177\u6709\u4e0d\u540c\u7684\u6da6\u6e7f\u6027\u7b5b\u5206\u53cd\u5e94\u7269\u4e2d\u8d4b\u4e88\u5b83\u4eec\u53e6\u5916\u7684\u9009\u62e9\u6027\u3002<\/p>\n<p><strong><b>\u6587\u732e\u94fe\u63a5\uff1a<a href=\"http:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/anie.201600497\/abstract;jsessionid=21704F48435E0B1347CF5A3F604AB34D.f01t04?systemMessage=Wiley+Online+Library+will+be+unavailable+on+Saturday+14th+May+11%3A00-14%3A00+BST+%2F+06%3A00-09%3A00+EDT+%2F+18%3A00-21%3A00+SGT+for+essential+maintenance.Apologies+for+the+inconvenience.\" target=\"_blank\">Polydimethylsiloxane Coating for a Palladium\/MOF Composite: Highly Improved Catalytic Performance by Surface Hydrophobization<\/a><\/b><\/strong><\/p>\n<p><strong><b>2\u3001JACS\uff1a\u91d1\u5c5e\u6709\u673a\u591a\u9762\u4f53\u4f5c\u4e3a\u591a\u529f\u80fd\u652f\u67b6\u7528\u4e8e\u5408\u6210\u661f\u5f62\u805a\u5408\u7269<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone wp-image-13132\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72472-10-300x136.jpg\" alt=\"\u56fe\u72472\" width=\"459\" height=\"208\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72472-10-300x136.jpg 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72472-10-768x349.jpg 768w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72472-10.jpg 1000w\" sizes=\"(max-width: 459px) 100vw, 459px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe2\u00a0MOP-\u661f\u5f62\u805a\u5408\u7269\u7684\u5408\u6210\u8def\u7ebf<\/p>\n<p>\u5927\u5206\u5b50\u7ed3\u6784\u7684\u526a\u5207\u662f\u9ad8\u5206\u5b50\u5316\u5b66\u9886\u57df\u5de8\u5927\u6311\u6218\uff0c\u6d3b\u6027\u805a\u5408\u7684\u5728\u4e0a\u4e2a\u4e16\u7eaa\u4e2d\u53f6\u53d1\u73b0\uff0c\u968f\u7740\u9ad8\u5206\u5b50\u5316\u5b66\u9886\u57df\u7684\u53d1\u5c55\uff0c\u4e3a\u6211\u4eec\u63d0\u4f9b\u4e86\u5404\u79cd\u590d\u6742\u7ed3\u6784\u7684\u805a\u5408\u7269\uff0c\u8fd9\u5176\u4e2d\u5c31\u5305\u62ec\u661f\u5f62\u805a\u5408\u7269\uff0c\u7531\u4e8e\u53d1\u5c04\u7684\u4f53\u7cfb\u7ed3\u6784\uff0c\u548c\u5206\u5b50\u95f4\u7684\u7f20\u7ed3\u88ab\u6291\u5236\uff0c\u9020\u6210\u4e86\u6781\u5176\u4f4e\u7684\u7c98\u5ea6\uff08\u4e0e\u5176\u7c7b\u4f3c\u5206\u5b50\u91cf\u7684\u7ebf\u6027\u7c7b\u4f3c\u7269\u76f8\u6bd4\uff09\u3002<\/p>\n<p>\u65e5\u672c\u4eac\u90fd\u5927\u5b66\u7684Susumu Kitagawa\u53ca\u5176\u5408\u4f5c\u8005\uff0c\u4f7f\u7528\u91d1\u5c5e-\u6709\u673a\u591a\u9762\u4f53\uff08MOPs\uff09\u4f5c\u4e3a\u591a\u529f\u80fd\u6838\uff0c\u5408\u6210\u4e86\u914d\u4f4d\u661f\u5f62\u805a\u5408\u7269\uff08CSP\uff09\uff0c\u5408\u6210\u8def\u7ebf\u5982\u56fe2\u6240\u793a\u3002\u800c\u5728\u4f20\u7edf\u5408\u6210\u65b9\u6cd5\u4e0a\uff0c\u9700\u8981\u6709\u9ad8\u64cd\u4f5c\u6280\u5de7\u548c\u591a\u6b65\u5408\u6210\u3002MOP-\u6838 CSPs\u662f\u4e00\u79cd\u65b0\u578b\u661f\u5f62\u805a\u5408\u7269\uff0c\u901a\u8fc7\u4f7f\u7528\u914d\u4f4d\u7eb3\u7c73\u7b3c\u4f5c\u4e3a\u6784\u7b51\u7684\u7ec4\u6210\u90e8\u5206\uff0c\u4e3a\u9ad8\u5ea6\u52a0\u5de5\u7684\u591a\u5b54\u67d4\u8f6f\u7684\u6750\u6599\u63d0\u4f9b\u8bbe\u8ba1\u7b56\u7565\u3002<\/p>\n<p><strong><b>\u6587\u732e\u94fe\u63a5\uff1a<a href=\"http:\/\/pubs.acs.org\/doi\/abs\/10.1021\/jacs.6b01758\" target=\"_blank\">Metal\u2013Organic Polyhedral Core as a Versatile Scaffold for Divergent and Convergent Star Polymer Synthesis<\/a><\/b><\/strong><\/p>\n<p><strong><b>3\u3001JACS\uff1a\u5bf9\u6c34\u7684\u5438\u9644\u91d1\u5c5e\u6709\u673a\u6846\u67b6{Fe(pz)[Pt(CN)4]}\u81ea\u65cb\u4ea4\u53c9\u5206\u5b50\u673a\u7406<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone wp-image-13133\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72473-8-290x300.jpg\" alt=\"\u56fe\u72473\" width=\"433\" height=\"448\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72473-8-290x300.jpg 290w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72473-8-768x795.jpg 768w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72473-8.jpg 845w\" sizes=\"(max-width: 433px) 100vw, 433px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe3\uff08a\uff09\u4ee5Nw\u4e3a\u51fd\u6570\u8ba1\u7b97MOF\u5b54\u4e2d\u6c34\u7684\u5e73\u5747\u4f4d\u7f6e\uff08b\uff0cd\uff09\u5f84\u5411\u5206\u5e03\u51fd\u6570\u63cf\u8ff0Fe-O\u7a7a\u95f4\u5173\u7cfb\uff08c\uff0ce\uff09\u5f84\u5411\u5206\u5e03\u51fd\u6570\u63cf\u8ff0Pt-O\u7a7a\u95f4\u5173\u7cfb<\/p>\n<p>\u901a\u8fc7\u5e94\u7528\u5916\u90e8\u523a\u6fc0\uff0c\u5728\u7eb3\u7c73\u5c3a\u5ea6\u5bf9\u5206\u5b50\u81ea\u7ec4\u88c5\u7684\u7269\u7406\u5316\u5b66\u6027\u8d28\u63a7\u5236\u7684\u80fd\u529b\u5bf9\u4e8e\u591a\u529f\u80fd\u6750\u6599\u53d1\u5c55\u81f3\u5173\u91cd\u8981\uff0c\u4f8b\u5982\u5206\u5b50\u5f00\u5173\uff0c\u5b58\u50a8\u88c5\u7f6e\uff0c\u548c\u5316\u5b66\u4f20\u611f\u5668\u3002\u9ad8\u5b54\u9699\u7387\u3001\u6bd4\u8868\u9762\u79ef\u5927\u3001\u5ba2\u4f53\u9009\u62e9\u6027\u548c\u7ed3\u6784\u7075\u6d3b\u6027\u7684\u91d1\u5c5e-\u6709\u673a\u9aa8\u67b6\uff08MOF\uff09\uff0c\u4e3a\u5f00\u53d1\u8fd9\u79cd\u523a\u6fc0\u54cd\u5e94\u6750\u6599\u63d0\u4f9b\u4e86\u4e00\u4e2a\u7406\u60f3\u7684\u5e73\u53f0\u3002\u7531\u4e8e\u5176\u56fa\u6709\u7684\u5316\u5b66\u591a\u6837\u6027\u548c\u591a\u5b54\u6027\uff0c\u5728\u5728\u50ac\u5316\u548c\u6c14\u4f53\u50a8\u5b58\u9886\u57df\u6709\u7740\u6f5c\u5728\u7684\u5e94\u7528\u524d\u666f\u3002<\/p>\n<p>\u5f15\u5165\u542b\u5f00\u58f3\u5c42\u8fc7\u6e21\u91d1\u5c5e\u7684\u6b21\u7ea7\u5355\u5143\u4f1a\u5bfc\u81f4MOFs\u8868\u73b0\u51fa\u81ea\u65cb\u4ea4\u53c9\uff08SCO\uff09\u884c\u4e3a\uff0c\u5728\u8fd9\u4e9bMOFs\u4e2d\uff0c\u6bcf\u4e2a\u91d1\u5c5e\u539f\u5b50\u51fa\u73b0\u591a\u4e2a\u81ea\u65cb\u6001\u3002\u5982\u679c\u975e\u952e\u548c\u53cd\u952e\u4e4b\u95f4\u7684\u80fd\u91cf\u5dee(\u0394E)\u6bd4\u7535\u5b50\u6210\u5bf9\u80fd\u5927\u7684\u8bdd\uff0c\u8fd9\u65f6\u91d1\u5c5e\u57fa\u6001\u4e3a\u4f4e\u81ea\u65cb\uff08LS\uff09\u7684\u72b6\u6001\uff0c\u53cd\u4e4b\u4e3a\u9ad8\u81ea\u65cb\uff08HS\uff09\u3002<\/p>\n<p>\u8fd1\u65e5\uff0c\u52a0\u5dde\u5927\u5b66Francesco Paesani\u53ca\u5176\u5408\u4f5c\u8005\uff0c\u4f7f\u7528\u914d\u4f53\u573a\u7406\u8bba\u8fdb\u884c\u5206\u5b50\u52a8\u529b\u5b66\u6a21\u62df\uff0c\u7ed3\u679c\u9610\u660e\u4e86\u5bf9\u6c34\u7684\u5438\u9644\u91d1\u5c5e\u6709\u673a\u6846\u67b6{Fe(pz)[Pt(CN)4]}\u81ea\u65cb\u4ea4\u53c9\u5c5e\u6027\u7684\u53d8\u5316\u7684\u5206\u5b50\u673a\u7406\u3002<\/p>\n<p><strong><b>\u6587\u732e\u94fe\u63a5\uff1a<a href=\"http:\/\/pubs.acs.org\/doi\/abs\/10.1021\/jacs.6b02564\" target=\"_blank\">Molecular Mechanisms of Spin Crossover in the {Fe(pz)[Pt(CN)4]} Metal\u2013Organic Framework upon Water Adsorption<\/a><\/b><\/strong><\/p>\n<p><strong><b>4\u3001JACS\uff1a<\/b><\/strong><strong><b>\u91d1\u5c5e\u6709\u673a\u9aa8\u67b6<\/b><\/strong><strong><b>\u6750\u6599<\/b><\/strong><strong><b>\u4e2d\u624b\u6027\u8bf1\u5bfc<\/b><\/strong><strong><b>\u5fae\u89c2<\/b><\/strong><strong><b>\u673a\u7406<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-13134\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72474-8.jpg\" alt=\"\u56fe\u72474\" width=\"263\" height=\"238\" \/><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-13135\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72475-6.jpg\" alt=\"\u56fe\u72475\" width=\"263\" height=\"247\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe4\uff08a\uff09\u975e\u624b\u6027MOF-5\u7ed3\u6784\uff08b\uff09\u624b\u6027MOF-5\u7ed3\u6784<\/p>\n<p>\u91d1\u5c5e\u6709\u673a\u5316\u5408\u7269\uff08MOFs\uff09\u662f\u7531\u91d1\u5c5e\u79bb\u5b50\u6216\u56e2\u7c07\u4e0e\u6709\u673a\u914d\u4f53\u901a\u8fc7\u914d\u4f4d\u952e\u7ed3\u5408\u8d77\u6765\u7684\u6709\u673a\u65e0\u673a\u6742\u5316\u591a\u5b54\u6750\u6599\u3002\u5408\u6210\u624b\u6027MOFs\u5bf9\u4e8e\u5176\u5728\u50ac\u5316\u548c\u9009\u62e9\u6027\u5206\u79bb\u9886\u57df\u6709\u7740\u6781\u5176\u91cd\u8981\u7684\u5e94\u7528\u524d\u666f\u3002\u4f20\u7edf\u7684\u5408\u6210\u624b\u6027MOF\u65b9\u6cd5\u662f\u5229\u7528\u624b\u6027\u539f\u6750\u6599\u6216\u8005\u7279\u5b9a\u62d3\u6251\u9aa8\u67b6\uff0c\u7136\u800c\u8fd9\u4e9b\u6750\u6599\u5f80\u5f80\u662f\u5916\u6d88\u65cb\u4f53\u3002<\/p>\n<p>\u8fd1\u65e5\uff0c\u6cd5\u56fdPSL Research University \u7684Jack D Evans\u548cFran\u00e7ois-Xavier Coudert\uff0c\u5229\u7528\u591a\u5c3a\u5ea6\u5206\u5b50\u6a21\u62df\u6765\u7814\u7a76\u624b\u6027\u8bf1\u5bfc\u7684\u5fae\u89c2\u673a\u7406\uff0c\u5e76\u7814\u7a76\u4e86\u8bf1\u5bfc\u540e\u7684MOF\u662f\u7684\u7a33\u5b9a\u6027\uff0c\u89e3\u91ca\u4e86NMP\u5206\u5b50\u7684\u5927\u5c0f\u548c\u4e86\u7279\u6027\u5728MOF-5\u4e2d\u662f\u5982\u4f55\u4ea7\u751f\u624b\u6027\u8f6c\u53d8\uff0c\u800c\u5176\u4ed6\u7684\u5206\u5b50\uff0c\u5982DMF\u662f\u65e0\u6cd5\u53d1\u751f\u8fd9\u6837\u7684\u8f6c\u53d8\u3002\u6b64\u9879\u5de5\u4f5c\u4e3a\u4f7f\u7528\u5176\u4ed6\u5ba2\u4f53\u5206\u5b50\u8bf1\u5bfcMOF\u624b\u6027\u8f6c\u53d8\u5f00\u8f9f\u4e86\u4e00\u6761\u9053\u8def\uff01<\/p>\n<p><strong><b>\u6587\u732e\u94fe\u63a5\uff1a<a href=\"http:\/\/pubs.acs.org\/doi\/abs\/10.1021\/jacs.6b02781\" target=\"_blank\">Microscopic Mechanism of Chiral Induction in a Metal\u2013Organic Framework<\/a><\/b><\/strong><\/p>\n<p><strong><b>5\u3001<\/b><\/strong><strong><b>Nature Communications\uff1a<\/b><\/strong><strong><b>\u8d85\u5206\u5b50MOFs\u8868\u73b0\u51fa\u9ad8\u6548\u5747\u76f8\u548c\u975e\u5747\u76f8\u5149\u50ac\u5316\u4ea7\u6c22\u6d3b\u6027<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone wp-image-13136\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72476-8-300x216.jpg\" alt=\"\u56fe\u72476\" width=\"351\" height=\"253\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72476-8-300x216.jpg 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72476-8.jpg 563w\" sizes=\"(max-width: 351px) 100vw, 351px\" \/><img loading=\"lazy\" decoding=\"async\" class=\"alignnone wp-image-13137\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72477-8-300x222.jpg\" alt=\"\u56fe\u72477\" width=\"361\" height=\"267\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72477-8-300x222.jpg 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72477-8.jpg 549w\" sizes=\"(max-width: 361px) 100vw, 361px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe5\u00a03D SMOF-1\u548cWD-POM\u81ea\u7ec4\u88c5\u793a\u610f\u56fe<\/p>\n<p>\u91d1\u5c5e\u6709\u673a\u5316\u5408\u7269\uff08MOFs\uff09\u662f\u7531\u91d1\u5c5e\u79bb\u5b50\u6216\u56e2\u7c07\u4e0e\u6709\u673a\u914d\u4f53\u901a\u8fc7\u914d\u4f4d\u952e\u7ed3\u5408\u8d77\u6765\u7684\u6709\u673a\u65e0\u673a\u6742\u5316\u591a\u5b54\u6750\u6599\u3002\u7531\u4e8eMOFs\u5177\u6709\u6c38\u4e45\u591a\u5b54\u6027\u3001\u9ad8\u7684\u6bd4\u8868\u9762\u79ef\u3001\u7ed3\u6784\u53ef\u8c03\u6027\u7b49\u7279\u6027\uff0c\u5b83\u5728\u50a8\u6c22\u3001\u591a\u76f8\u50ac\u5316\u3001\u836f\u7269\u7f13\u91ca\u3001\u5149\u5b66\u3001\u751f\u7269\u6210\u50cf\u3001\u6c14\u4f53\u8bc6\u522b\u7b49\u9886\u57df\u6709\u7740\u5de8\u5927\u7684\u5e94\u7528\u524d\u666f\u3002\u4f46\u662f\uff0c\u7531\u4e8e\u5176\u56fa\u4f53\u7279\u6027\uff0c\u5bfc\u81f4\u4e86\u5176\u51e0\u4e4e\u6240\u6709\u4e0e\u529f\u80fd\u76f8\u5173\u7684\u7814\u7a76\u90fd\u662f\u4ee5\u975e\u5747\u76f8\u65b9\u5f0f\u8fdb\u884c\u7684\u3002\u5bf9\u4e8e\u836f\u7269\u7f13\u91ca\u548c\u751f\u7269\u6210\u50cf\u7684\u5e94\u7528\uff0c\u8fd9\u610f\u5473\u7740\u5728\u4f53\u5185\u4f1a\u4ea7\u751f\u76f8\u5206\u79bb\uff0c\u8fd9\u8fdb\u4e00\u6b65\u53ef\u80fd\u5bfc\u81f4\u5176\u5728\u4f53\u5185\u6709\u5bb3\u7684\u805a\u96c6\u6216\u751f\u7269\u4e0d\u76f8\u5bb9\u6027\u3002\u53e6\u4e00\u65b9\u9762\uff0c\u5927\u591a\u6570\u62a5\u9053\u7684MOFs\u662f\u4f7f\u7528\u6c34\u70ed\u548c\u6eb6\u5242\u70ed\u6280\u672f\u5236\u5907\u7684\uff0c\u8fd9\u6837\u7684\u5236\u5907\u65b9\u6cd5\u9700\u8981\u9ad8\u6e29\u548c\u957f\u53cd\u5e94\u65f6\u95f4\u3002<\/p>\n<p>\u8fd1\u65e5\uff0c\u590d\u65e6\u5927\u5b66\u5229\u9ece\u5360\u4ead\u6559\u6388\u7b49\u4eba\u7528\u81ea\u7ec4\u88c5\u7b56\u7565\u5728\u5ba4\u6e29\u4e0b\u6784\u7b51\u4e86\u7b2c\u4e00\u4f8b\u6c34\u4e2d\u5747\u76f8\u8d85\u5206\u5b50\u6709\u673a\u6846\u67b6\uff08MSOF\uff09\uff0c\u5229\u7528\u5c0f\u89d2X\u5c04\u7ebf\u884d\u5c04\u548c\u6563\u5c04\u8868\u5f81\u4e86\u8be5\u79cdMOF\u7684\u6eb6\u6db2\u76f8\u5468\u671f\u6027\u7ed3\u6784\uff0c\u540c\u65f6\u901a\u8fc7TEM\u56fe\u53ef\u5f97\uff0c\u4e0e\u5176\u5728\u56fa\u4f53\u72b6\u6001\u7684\u5468\u671f\u6027\u76f8\u79f0\u3002\u6b64\u5916\uff0c\u6211\u4eec\u8fdb\u4e00\u6b65\u8bc1\u660e\u4e86SMOF-1\u4ee5\u201cone-cage-one-guest\u201d\u7684\u65b9\u5f0f\u5438\u9644\u9634\u79bb\u5b50WD-POMs\uff0c\u5b9e\u73b0WD-POM@ SMOF-1\u6742\u5316\u81ea\u7ec4\u88c5\u3002\u5728\u53ef\u89c1\u5149\uff08500 nm\uff09\u7167\u5c04\u4e0b\uff0c\u8fd9\u4e2a\u6742\u5316\u6750\u6599\u80fd\u591f\u5b9e\u73b0\u4ece\u5149\u654f\u5316\u7684[Ru(bpy)3]2+\u5355\u5143\u5230\u6c27\u5316\u8fd8\u539f\u6d3b\u6027\u7684WD-POM\u5355\u5143\u7684\u5feb\u901f\u591a\u7535\u5b50\u6ce8\u5165\uff0c\u8fd9\u5c31\u4f7f\u5f97\u5176\u5728\u542b\u6c34\u4ecb\u8d28\u4e2d\u548c\u6709\u673a\u4ecb\u8d28\u4e2d\u80fd\u591f\u9ad8\u6548\u4ea7\u6c22\u3002<\/p>\n<p><strong>\u6587\u732e\u94fe\u63a5\uff1a<a href=\"http:\/\/www.nature.com\/ncomms\/2016\/160510\/ncomms11580\/full\/ncomms11580.html\" target=\"_blank\">Supramolecular metal-organic frameworks that display high homogeneous and heterogeneous photocatalytic activity for H2 production<\/a><\/strong><\/p>\n<p><strong><b>6\u3001Angew.Chem\uff1aMOF UiO-66-NH2\u9ad8\u6548\u53bb\u9664NO<\/b><\/strong><strong><sub><b>2<\/b><\/sub><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone wp-image-13138\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72478-5-300x219.jpg\" alt=\"\u56fe\u72478\" width=\"466\" height=\"340\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72478-5-300x219.jpg 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72478-5-768x561.jpg 768w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72478-5.jpg 994w\" sizes=\"(max-width: 466px) 100vw, 466px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe6 \u00a0\u4e0d\u540c\u65f6\u95f4UiO-66-NH2\u66b4\u9732\u4e8eNO2\u7684DRIFTS\u8c31<\/p>\n<p>NO<sub>2<\/sub>\u548c\u4e00\u4e9b\u6c2e\u7684\u6c27\u5316\u7269\u662f\u5927\u6c14\u4e2d\u5e38\u89c1\u7684\u6709\u6bd2\u6c61\u67d3\u7269\uff0c\u7ecf\u8fc7\u71c3\u70e7\u4ea7\u751f\u7684\u4e8c\u6c27\u5316\u6c2e\u4e5f\u662f\u5e38\u89c1\u7684\u5927\u5b97\u5316\u5b66\u54c1\uff0c\u968f\u7740\u57fa\u4e8eNOx\u7684\u5316\u5b66\u54c1\u7684\u4f7f\u7528\u548c\u4ea7\u751f\uff0c\u65e0\u8bba\u662f\u5728\u70df\u9053\u6c14\u4f53\u6d17\u6da4\u64cd\u4f5c\u6216\u73af\u5883\u4fdd\u62a4\uff0c\u8fd9\u90fd\u9700\u8981\u9664\u53bb\u5b83\u4eec\u5438\u9644\u5242\u3002\u5728\u4e24\u8005\u4e2d\uff0c\u5438\u9644\u6750\u6599\u5fc5\u987b\u5728\u5e72\u71e5\u548c\u6f6e\u6e7f\u7684\u6761\u4ef6\u4e0b\u90fd\u53d1\u6325\u5438\u9644\u4f5c\u7528\u3002\u7531\u4e8e\u6c2e\u6c27\u5316\u7269\u662f\u4ece\u71c3\u70e7\/\u706b\u7684\u4ea7\u751f\uff0c\u6240\u4ee5\u7b2c\u4e00\u53cd\u5e94\u662f\u9700\u8981\u5bf9\u8fd9\u79cd\u6750\u6599\u8fdb\u884c\u4fdd\u62a4\uff0c\u542b\u6709\u6d3b\u6027\u70ad\u53e3\u7f69\u5178\u578b\u63d0\u4f9b\u6709\u9650\u7684\u53bb\u9664\u80fd\u529b\u3002\u591a\u79cd\u5438\u9644\u5242\u5df2\u7ecf\u88ab\u5f00\u53d1\u5e76\u7528\u4e8e\u9664\u53bb\u4e8c\u6c27\u5316\u6c2e\uff0c\u5176\u4e2d\u6548\u679c\u6700\u663e\u7740\u7684\u6cb8\u77f3\u548c\u4e8c\u6c27\u5316\u949b\u6750\u6599\u3002<\/p>\n<p>MOF\u6750\u6599\u5177\u6709\u6c38\u4e45\u7684\u591a\u5b54\u6027\u548c\u6781\u9ad8\u7684\u6bd4\u8868\u9762\u79ef\uff0c\u56e0\u6b64\u5176\u5728\u6c14\u4f53\u5438\u9644\u3001\u50a8\u5b58\u3001\u5206\u79bb\u7b49\u9886\u57df\u6709\u7740\u6f5c\u5728\u7684\u5e94\u7528\u3002UiO-66\u5728MOF\u5728\u4e2d\uff0c\u6709\u7740\u8f83\u597d\u7684\u7a33\u5b9a\u6027\uff08\u5728\u6f6e\u6e7f\u548c\u9178\u6027\u6761\u4ef6\u4e0b\uff09\uff0cUiO-66-NH2 \u5bf9\u4e8e\u8bb8\u591a\u6709\u6bd2\u6c14\u4f53\u90fd\u5c55\u73b0\u51fa\u4f18\u5f02\u7684\u53bb\u9664\u6027\u80fd\u3002<\/p>\n<p>\u8fd1\u65e5\uff0c \u57c3\u5947\u4f0d\u5fb7\u5316\u751f\u4e2d\u5fc3Gregory W. Peterson\u7b49\u4eba\u7814\u7a76\u5229\u7528MOF\u6750\u6599UiO-66-NH2\u53bb\u9664\u7a7a\u6c14\u4e2d\u7684NO2\uff08\u4e00\u79cd\u91cd\u8981\u7684\u6709\u6bd2\u5de5\u4e1a\u5316\u5b66\u54c1\u548c\u5927\u6c14\u6c61\u67d3\u7269\uff09\uff0c\u5e76\u53d1\u73b0MOF\u4e0a\u9762\u7684\u6c28\u57fa\u5bf9\u4e8e\u5176\u53bb\u9664NO2\u975e\u5e38\u6709\u5e2e\u52a9\uff0c\u8fbe\u5230\u524d\u6240\u672a\u6709\u7684\u53bb\u9664\u80fd\u529b\uff0c\u6bcf\u514bMOF\u53ef\u4ee5\u53bb\u96641.4\u514bNO2\uff0c\u7279\u522b\u91cd\u8981\u7684\u662f\uff0c\u5728MOF\u7684\u82b3\u9999\u73af\u4e0a\u5f62\u6210\u7684\u91cd\u6c2e\u79bb\u5b50\u5e76\u6f5c\u5728\u7684\u51cf\u5c11\u4e86NO2\u6210\u6c2e\u6c14\u5206\u5b50\uff0c\u5bf9\u4e8eMOF\u5728\u5927\u6c14\u6cbb\u7406\u65b9\u9762\u6709\u7740\u91cd\u8981\u7684\u5f71\u54cd\u3002<\/p>\n<p><strong><b>\u6587\u732e\u94fe\u63a5\uff1a<a href=\"http:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/anie.201601782\/abstract\" target=\"_blank\">Extraordinary NO2 Removal by the Metal\u2013Organic Framework UiO-66-NH2<\/a><\/b><\/strong><\/p>\n<p><strong><b>7\u3001Advanced Materials\uff1aMOF\u8584\u819c\u5305\u8986\u7684\u91d1\u5c5e\u6c27\u5316\u7269\u7eb3\u7c73\u7ebf\u9635\u5217\uff1a\u663e\u8457\u6539\u5584\u7684\u5316\u5b66\u963b\u6297\u4f20\u611f\u6027\u80fd<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone wp-image-13139\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72479-2-300x201.jpg\" alt=\"\u56fe\u72479\" width=\"451\" height=\"302\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72479-2-300x201.jpg 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72479-2-768x516.jpg 768w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72479-2-1024x688.jpg 1024w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u72479-2.jpg 2000w\" sizes=\"(max-width: 451px) 100vw, 451px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe7 ZnO@ZIF-CoZn\u6c14\u4f53\u4f20\u611f\u5668\u7684\u5236\u5907\u8fc7\u7a0b\u793a\u610f\u56fe<\/p>\n<p>\u91d1\u5c5e\u6c27\u5316\u7269\u662f\u4e00\u7c7b\u91cd\u8981\u7684\u5316\u5b66\u7535\u963b\u6750\u6599\uff0c\u5982ZnO, 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href=\"http:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/adma.201506457\/full\" target=\"_blank\">MOF Thin Film-Coated Metal Oxide Nanowire Array: Significantly Improved Chemiresistor Sensor Performance<\/a><\/b><\/strong><\/p>\n<p><strong><b>8\u3001JACS\uff1a\u70ed\u529b\u5b66\u6307\u5bfc\u5408\u6210\u5177\u6709\u6df7\u5408\u8fde\u63a5\u5668\u4e14\u6709\u589e\u5f3a\u53ef\u8c03\u6027Zr-MOFs<\/b><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone wp-image-13140\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u724710-2-300x103.jpg\" alt=\"\u56fe\u724710\" width=\"472\" height=\"162\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u724710-2-300x103.jpg 300w, \/\/m.iemloyee.com\/wp-content\/uploads\/2016\/05\/\u56fe\u724710-2.jpg 574w\" sizes=\"(max-width: 472px) 100vw, 472px\" \/><\/p>\n<p style=\"text-align: center;\">\u56fe8 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MOFs\u201d\u3002<\/p>\n<p>\u6700\u8fd1\uff0cTexas A&amp;M University\u7684\u5468\u5b8f\u624d\u6559\u6388\u53ca\u5176\u5408\u4f5c\u8005\uff0c\u5229\u7528\u70ed\u529b\u5b66\u6307\u5bfc\u5408\u6210\u5904\u4e86\u5177\u6709\u6df7\u5408\u8fde\u63a5\u5668\u4e14\u6709\u589e\u5f3a\u53ef\u8c03\u6027Zr-MOFs\uff08PCN-133 \u548cPCN-134\uff09\uff0c\u8fd9\u4e24\u79cdMOF\u90fd\u662f\u5177\u6709\u5c42-\u67f1\u7ed3\u6784\u7684\u3002\u5176\u4e2d\uff0cPCN-134\u7684N2\u8d1f\u8f7d\u91cf\u8fbe717 cm3\u00b7g-1\uff0cBET\u6bd4\u8868\u9762\u79ef\u8fbe1946 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Tunability<\/a><\/b><\/strong><\/p>\n<p>\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u5b66\u672f\u7ec4\u6731\u5fb7\u6770\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u7f16\u8f91\u6574\u7406\u3002<\/p>\n<p>\u6b22\u8fce\u52a0\u5165\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u5b66\u672f\u7ec4\uff0c\u4e00\u8d77\u8fdb\u884c\u6750\u6599\u9876\u520a\u5b66\u672f\u52a8\u6001\u7684\u8ddf\u8e2a\u548c\u62a5\u9053\u4ee5\u53caSCI\u76f8\u5173\u77e5\u8bc6\u79d1\u666e\u7b49\u3002\u52a0\u5165\u65b9\u5f0f\uff1a\u52a0\u5165\u6750\u6599\u4ebaMOF\u5b66\u672f\u4ea4\u6d41\u7fa4\uff08120199039\uff09\uff0c\u79c1\u4fe1\u7ba1\u7406\u5458\u201c\u6de1\u5e74\u534e\uff08QQ:601416321\uff09\u201d\u62a5\u540d\u3002<\/p>\n<p>\u6b22\u8fce\u5404\u5927\u8bfe\u9898\u7ec4\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com<\/p>\n","protected":false},"excerpt":{"rendered":"<p>1\u3001Angew.Chem\uff1a 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