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\u6750\u6599\u4eba\u4e0d\u5b9a\u671f\u63a8\u51fa\u50ac\u5316\u6750\u6599\u524d\u6cbf\u7814\u7a76\u6210\u679c\u7cbe\u9009\uff0c\u672c\u6587\u4e3a\u7b2c5\u671f\uff0c\u5305\u542b\u4e86\u53d1\u8868\u65f6\u95f4\u4e3a2018\u5e741\u6708\u81f32018\u5e743\u6708\u7684\u4f18\u8d28\u50ac\u5316\u6587\u7ae0\u3002<\/p>\n
1 Angew. Chem. Int. Ed.<\/strong>\uff1a<\/strong>\u7528\u7535\u81f4\u5316\u5b66\u53d1\u5149\u6210\u50cf\u6280\u672f\u7814\u7a76<\/strong>\u201c<\/strong>\u4e24\u9762\u795e<\/strong>\u201dAu-Pt<\/strong>\u7eb3<\/strong>\u7c73<\/strong>\u9897<\/strong>\u7c92\u8868\u9762\u7684<\/strong>\u7535<\/strong>\u50ac\u5316\u6c27\u5316\u53cd<\/strong>\u5e94<\/strong><\/p>\n \u56fe<\/strong>1 <\/strong>\u7528<\/strong>ECL<\/strong>\u6210\u50cf\u7814\u7a76<\/strong>Au-Pt<\/strong>\u7eb3<\/strong>\u7c73<\/strong>\u9897<\/strong>\u7c92\u8868\u9762<\/strong>\u7684\u7535<\/strong>\u50ac\u5316\u6c27\u5316\u53cd<\/strong>\u5e94<\/strong><\/p>\n \u8d35\u91d1\u5c5e\u50ac\u5316\u5242\u7684\u6784\u6548\u5173\u7cfb\u7814\u7a76\u80fd\u63a8\u52a8\u5355\u5206\u5b50\u7535\u5316\u5b66\u7684\u53d1\u5c55\u3002\u8fd1\u65e5\uff0c\u5357\u4eac\u5927\u5b66<\/strong>\u7684\u5f90\u9759\u5a1f\u6559\u6388<\/strong>\u548cWei Zhao\u535a\u58eb\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7b49\u7528\u7535\u81f4\u5316\u5b66\u53d1\u5149\uff08ECL\uff09\u6280\u672f\u7814\u7a76\u4e86\u4e0d\u540c\u53d1\u5149\u57fa\u56e2\u5206\u522b\u5728\u5355\u4e2aAu\u3001Pt\u3001Au-Pt\u7eb3\u7c73\u9897\u7c92\u8868\u9762\u7684\u7535\u50ac\u5316\u6c27\u5316\u53cd\u5e94\u3002\u4e0e\u5355\u91d1\u5c5e\u7eb3\u7c73\u9897\u7c92\u76f8\u6bd4\uff0c\u201c\u4e24\u9762\u795e\u201d\u7eb3\u7c73\u9897\u7c92\u7ed3\u6784\u5177\u6709\u66f4\u9ad8\u7684ECL\u5f3a\u5ea6\u548c\u7a33\u5b9a\u6027\u3002\u8fd9\u8868\u660e\u201c\u4e24\u9762\u795e\u201d\u50ac\u5316\u5242\u7684\u50ac\u5316\u6548\u7387\u9ad8\u4e8e\u5355\u91d1\u5c5e\u7eb3\u7c73\u9897\u7c92\u3002\u5b9e\u9a8c\u7ed3\u679c\u548c\u6570\u503c\u6a21\u62df\u8868\u660e\uff0c\u57fa\u56e2\u6d53\u5ea6\u5dee\u5f02\u6765\u81ea\u5bf9\u79f0\u6027\u4f4e\u7684\u53cc\u91d1\u5c5e\u754c\u9762\u3002\u8fd9\u662f\u7531\u4e8eAu\u548cPt\u8868\u9762\u7684\u5f02\u76f8\u7535\u5b50\u8f6c\u79fb\u901f\u7387\u5e38\u6570\u4e0d\u540c\u3002Au-Pt\u7eb3\u7c73\u9897\u7c92\u5468\u56f4\u7684\u6d41\u4f53\u6ed1\u79fb\u4e0d\u4ec5\u4f7f\u50ac\u5316\u6548\u7387\u63d0\u9ad8\uff0c\u8fd8\u80fd\u9632\u6b62\u9897\u7c92\u8868\u9762\u949d\u5316\u3002<\/p>\n \u6587\u732e\u94fe\u63a5\uff1a<\/strong>Electrogenerated Chemiluminescence Imaging of Electrocatalysis at a Single Au-Pt Janus Nanoparticle<\/a>\uff08Angew. Chem. Int. Ed.\uff0c2018\uff0cDOI: 10.1002\/anie.201800706\uff09<\/p>\n 2 JACS: Au\/TiO2<\/sub><\/strong>\u548c<\/strong>Au\/Al2<\/sub>O3<\/sub><\/strong>\u50ac\u5316CO\u6c27\u5316\u7684\u52a8\u529b\u5b66\u7814\u7a76\uff1a\u6c34\u5206\u5b50\u8f85\u52a9\u6761\u4ef6\u4e0b\u7684\u53cd\u5e94\u673a\u5236<\/strong><\/p>\n \u56fe2 <\/strong>\u6c34\u5206\u5b50\u8f85\u52a9\u4e0b<\/strong>Au\/TiO2<\/sub><\/strong>\u6216<\/strong>Au\/Al2<\/sub>O3<\/sub><\/strong>\u8868\u9762<\/strong>\u7684CO\u50ac\u5316\u6c27\u5316\u673a\u7406<\/strong><\/p>\n CO\u5728Au\u50ac\u5316\u5242\u8868\u9762\u7684\u50ac\u5316\u6c27\u5316\u673a\u7406\u4e00\u76f4\u500d\u53d7\u4e89\u8bae\u3002\u76ee\u524d\u6700\u4e3b\u8981\u7684\u4e24\u79cd\u89c2\u70b9\u5206\u522b\u662f\u6c34\u5206\u5b50\u8f85\u52a9\u4e0b\u7684CO\u6c27\u5316\u673a\u7406\u548c\u6d89\u53ca\u6c27\u7f3a\u9677\u4f4d\u70b9\u7684CO\u6c27\u5316\u673a\u7406\u3002\u9762\u5bf9\u8fd9\u4e00\u5206\u6b67\uff0c\u7f8e\u56fd\u4e09\u4e00\u5927\u5b66<\/strong>\u7684Bert D. Chandler\u6559\u6388<\/strong>\u548c\u7f8e\u56fd\u897f\u5317\u592a\u5e73\u6d0b\u56fd\u5bb6\u5b9e\u9a8c\u5ba4\uff08PNNL\uff09\u7efc\u5408\u50ac\u5316\u7814\u7a76\u6240\uff08IIC\uff09<\/strong>\u7684Christopher J. Pursell\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7b49\u5206\u522b\u5728Au\/TiO2<\/sub>\u548cAu\/Al2<\/sub>O3<\/sub>\u50ac\u5316\u5242\u5b58\u5728\u7684\u6761\u4ef6\u4e0b\uff0c\u9488\u5bf9\u6c34\u5206\u5b50\u5728CO\u50ac\u5316\u6c27\u5316\u53cd\u5e94\u4e2d\u6240\u8d77\u5230\u7684\u4f5c\u7528\u8fdb\u884c\u4e86\u50ac\u5316\u53cd\u5e94\u52a8\u529b\u5b66\u53ca\u53cd\u5e94\u673a\u7406\u7814\u7a76\u3002\u8be5\u5de5\u4f5c\u8bc1\u5b9e\u4e86\u6c34\u5206\u5b50\u8f85\u52a9\u4e0b\u7684CO\u6c27\u5316\u673a\u7406\u3002\u7814\u7a76\u8868\u660e\uff0c\u6c34\u5206\u5b50\u5360\u636e\u4e86\u91d1\u5c5e-\u8f7d\u4f53\u754c\u9762\u7684CO\u5438\u9644\u4f4d\u70b9\uff0c\u4f7fAu\/TiO2<\/sub>\u50ac\u5316\u5242\u5bf9CO\u7684\u5438\u9644\u91cf\u4e0b\u964d\u3002\u52a8\u529b\u5b66\u540c\u4f4d\u7d20\u6548\u5e94\u6d4b\u8bd5\u8868\u660e\uff0c\u7531Au\/TiO2<\/sub>\u548cAu\/Al2<\/sub>O3<\/sub>\u50ac\u5316CO\u6c27\u5316\u7684\u53cd\u5e94\u673a\u7406\u76f8\u540c\uff0c\u5176\u4e2dCO\u3001O2<\/sub>\u3001H2<\/sub>O\u7684\u53cd\u5e94\u7ea7\u6570\u5747\u76f8\u540c\u3002\u7814\u7a76\u4eba\u5458\u7528\u6d89\u53ca\u6d3b\u6027\u4f4d\u70b9\u7684Michaelis\u2013Menten\u65b9\u6cd5\u5904\u7406\u4e0e\u53cd\u5e94\u52a8\u529b\u5b66\u6709\u5173\u7684\u5b9e\u9a8c\u6570\u636e\uff0c\u89e3\u91ca\u4e86\u6c34\u5206\u5b50\u6539\u53d8CO\u548cO2<\/sub>\/COOH\u5438\u9644\u4f4d\u70b9\u6570\u91cf\u7684\u673a\u5236\u3002\u5f15\u5165\u6c34\u5206\u5b50\u4ec5\u4ec5\u4f7f\u6d3b\u6027\u4f4d\u70b9\u6570\u76ee\u53d1\u751f\u53d8\u5316\uff0c\u800c\u5e76\u6ca1\u6709\u4f7f\u53cd\u5e94\u901f\u7387\u5e38\u6570\u4e0b\u964d\u3002\u5b9e\u9a8c\u6d4b\u5f97\u6c34\u5206\u5b50\u548cO2<\/sub>\u5728\u4e24\u79cd\u50ac\u5316\u5242\u8868\u9762\u7684\u5438\u9644\u80fd\u76f8\u8fd1\uff0c\u8fd9\u4e0eDFT\u8ba1\u7b97\u7ed3\u679c\u76f8\u7b26\u3002\u5728\u5f15\u5165\u5927\u91cf\u6c34\u5206\u5b50\u7684\u6761\u4ef6\u4e0b\uff0c\u6c27\u7a7a\u4f4d\u673a\u5236\u4e0d\u518d\u662f\u5ba4\u6e29\u4e0bCO\u50ac\u5316\u6c27\u5316\u53cd\u5e94\u7684\u4e3b\u8981\u53cd\u5e94\u673a\u5236\uff0c\u800c\u6c34\u5206\u5b50\u8f85\u52a9\u4e0b\u7684CO\u6c27\u5316\u673a\u7406\u5219\u4e0e\u52a8\u529b\u5b66\u6570\u636e\u66f4\u76f8\u7b26\u3002<\/p>\n \u6587\u732e\u94fe\u63a5\uff1a<\/strong>CO Oxidation Kinetics over Au\/TiO2 and Au\/Al2O3 Catalysts: Evidence for a Common Water-Assisted Mechanism<\/a>\uff08J. Am. Chem. Soc.<\/em>\uff0c2018\uff0cDOI: 10.1021\/jacs.7b12758\uff09<\/p>\n 3 EES<\/strong>\uff1a\u542b\u6c27\u6709\u673a\u7269\u5728\u9178\u50ac\u5316\u53cd\u5e94\u4e2d\u7684\u52a8\u529b\u5b66\u6eb6\u5242\u6548\u5e94<\/strong><\/p>\n \u56fe3 \u9178\u50ac\u5316\u53cd\u5e94\u4e2d\u7684\u52a8\u529b\u5b66\u6eb6\u5242\u6548\u5e94<\/strong><\/p>\n \u7f8e\u56fd\u5a01\u65af\u5eb7\u661f\u5927\u5b66<\/strong>\u7684James A. Dumesic\u6559\u6388<\/strong>\u548cReid C. Van Lehn\u52a9\u7406\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7b49\u5728\u7531\u6c34\u548c\u5176\u4ed63\u79cd\u6781\u6027\u975e\u8d28\u5b50\u6eb6\u5242\uff08\u03b3-\u620a\u5185\u916f\u30011,4-\u4e8c\u6c27\u516d\u73af\u3001\u56db\u6c22\u544b\u5583\uff09\u7ec4\u6210\u7684\u6df7\u5408\u6eb6\u5242\u4e2d\u5bf9\u5e03\u6717\u65af\u7279\u9178\u50ac\u5316\u7684\u4e59\u57fa\u53d4\u4e01\u919a\u3001\u53d4\u4e01\u9187\u3001\u5de6\u65cb\u8461\u805a\u7cd6\u30011,2-\u4e19\u4e8c\u9187\u3001\u679c\u7cd6\u3001\u7ea4\u7ef4\u4e8c\u7cd6\u3001\u6728\u7cd6\u9187\u7684\u53cd\u5e94\u8fdb\u884c\u4e86\u53cd\u5e94\u52a8\u529b\u5b66\u6d4b\u8bd5\u3002\u5f53\u6eb6\u5242\u5316\u5c42\u4e2d\u7684\u6c34\u542b\u91cf\u4e0b\u964d\u65f6\uff0c\u5e26\u6709\u66f4\u591a\u7f9f\u57fa\u7684\u6709\u673a\u53cd\u5e94\u7269\u5728\u6c34\u89e3\u53cd\u5e94\u548c\u8131\u6c34\u53cd\u5e94\u4e2d\u5177\u6709\u66f4\u9ad8\u7684\u672c\u5f81\u50ac\u5316\u6d3b\u6027\u3002\u901a\u8fc7\u5206\u5b50\u52a8\u529b\u5b66\u6a21\u62df\uff0c\u7814\u7a76\u4eba\u5458\u57fa\u4e8e\u6df7\u5408\u6eb6\u5242\u7684\u7ec4\u6210\u63d0\u51fa\u4e863\u4e2a\u53ef\u89c2\u6d4b\u91cf\uff1a(1) \u6709\u673a\u53cd\u5e94\u7269\u6eb6\u5242\u5316\u5c42\u4e2d\u7684\u6c34\u542b\u91cf\uff1b(2) \u6c34\u5206\u5b50\u4e0e\u53cd\u5e94\u7269\u4e4b\u95f4\u6240\u5f62\u6210\u6c22\u952e\u7684\u5e73\u5747\u5bff\u547d\uff1b(3) \u53cd\u5e94\u7269\u5206\u5b50\u8868\u9762\u88ab\u7f9f\u57fa\u5360\u636e\u7684\u9762\u79ef\u5360\u603b\u8868\u9762\u79ef\u7684\u6bd4\u4f8b\u3002\u968f\u540e\uff0c\u7814\u7a76\u4eba\u5458\u7528\u8fd93\u4e2a\u53ef\u89c2\u6d4b\u91cf\u7684\u7ebf\u6027\u7ec4\u5408\u5efa\u7acb\u4e86\u4e00\u4e2a\u6a21\u578b\u3002\u8be5\u6a21\u578b\u666e\u904d\u9002\u7528\u4e8e\u9178\u50ac\u5316\u53cd\u5e94\uff0c\u5e76\u80fd\u6839\u636e\u6df7\u5408\u6eb6\u5242\u7684\u7ec4\u6210\u9884\u6d4b\u8be5\u53cd\u5e94\u7684\u901f\u7387\u5e38\u6570\u3002<\/p>\n \u6587\u732e\u94fe\u63a5\uff1a<\/strong>Universal Kinetic Solvent Effects in Acid-Catalyzed Reactions of Biomass-Derived Oxygenates<\/a>\uff08Energy Environ. Sci.\uff0c2018\uff0cDOI: 10.1039\/C7EE03432F\uff09<\/p>\n 4 JACerS<\/strong>\uff1a\u9178\u50ac\u5316\u5242\u5bf9\u751f\u7269\u6d3b\u6027\u73bb\u7483\u7684\u805a\u5408\u5ea6\u4e0e\u5fae\u89c2\u7ed3\u6784\u7684\u5f71\u54cd<\/strong><\/p>\n \u56fe<\/strong>4 <\/strong>\u751f\u7269\u6d3b\u6027\u73bb\u7483\u7c89\u672b\u7684SEM<\/strong>\u56fe<\/strong>\u50cf<\/strong><\/p>\n \u8461\u8404\u7259\u963f\u5a01\u7f57\u5927\u5b66<\/strong>\u7684Robert C. Pullar\u6559\u6388<\/strong>\u548cIsabel M. M. Salvado\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7b49\u7814\u7a76\u4e86\u9178\u50ac\u5316\u5242\u7684\u79cd\u7c7b\u548c\u6d53\u5ea6\u5bf9\u751f\u7269\u6d3b\u6027\u73bb\u7483\uff08\u6469\u5c14\u6bd4Si\uff1aCa\uff1aNa\uff1aP=75\uff1a16\uff1a5\uff1a4\uff09\u7684\u805a\u5408\u5236\u5907\u8fc7\u7a0b\u53ca\u4ea7\u7269\u5fae\u89c2\u7ed3\u6784\u7684\u5f71\u54cd\u3002\u7814\u7a76\u4eba\u5458\u4ece\u4e59\u9178\u76d0\u548c\u785d\u9178\u76d0\u51fa\u53d1\uff0c\u7528\u6539\u8fdb\u7684\u6eb6\u80f6-\u51dd\u80f6\u6cd5\u5feb\u901f\u5236\u5f97\u524d\u9a71\u4f53\uff0c\u7ecf\u70ed\u5904\u7406\u5f97\u5230\u5bcc\u542bSiO2\u7684\u751f\u7269\u6d3b\u6027\u73bb\u7483\u3002\u7814\u7a76\u53d1\u73b0\uff0c\u5f53\u9178\u50ac\u5316\u5242\u7684\u6d53\u5ea6\u8f83\u9ad8\u65f6\uff0c\u6240\u5f97\u4ea7\u7269\u7684\u805a\u5408\u5ea6\u548c\u4ea4\u8054\u7a0b\u5ea6\u5747\u8f83\u4f4e\u3002\u5f53\u52a0\u5165\u5c11\u91cf\u67e0\u6aac\u9178\uff0c\u6240\u5f97\u4ea7\u7269\u7684\u805a\u5408\u5ea6\u63a5\u8fd1\u4e8e\u65e0\u50ac\u5316\u5242\u6761\u4ef6\u4e0b\u4ea7\u7269\u7684\u805a\u5408\u5ea6\uff0c\u800c\u5408\u6210\u65f6\u95f4\u5374\u80fd\u50cf\u9ad8\u6d53\u5ea6\u9178\u50ac\u5316\u5242\u6761\u4ef6\u4e0b\u7684\u5408\u6210\u65f6\u95f4\u4e00\u6837\u77ed\u3002\u8be5\u65b9\u6cd5\u5f97\u5230\u7684\u65e0\u5b9a\u5f62\u751f\u7269\u6d3b\u6027\u73bb\u7483\u7c89\u672b\u4e0d\u542b\u785d\u9178\u76d0\u6742\u8d28\u3002\u901a\u8fc7\u8c03\u63a7\u9178\u50ac\u5316\u5242\u7684\u79cd\u7c7b\u548c\u65f6\u95f4\uff0c\u80fd\u5728\u8d77\u59cb\u53cd\u5e94\u7269\u76f8\u540c\u7684\u6761\u4ef6\u4e0b\u5408\u6210\u751f\u7269\u6d3b\u6027\u4e0d\u540c\u7684\u65e0\u5b9a\u5f62\u73bb\u7483\u7c89\u672b\u3002<\/p>\n \u6587\u732e\u94fe\u63a5\uff1a<\/strong>Effects of catalysts on polymerization and microstructure of sol-gel derived bioglasses<\/a>\uff08J Am Ceram Soc.\uff0c2018\uff0cDOI: 10.1111\/jace.15450\uff09<\/p>\n 5 AEM<\/strong>\uff1a<\/strong>PtPb\/Pt<\/strong>\u6838\u58f3<\/strong>\u7ed3<\/strong>\u6784<\/strong>\u7eb3<\/strong>\u7c73<\/strong>\u76d8<\/strong>\u50ac\u5316\u5242\u7528\u4e8e\u9ad8\u6548\u7684\u7532\u9187\u91cd\u6574\u5236\u6c22\u6c14\u53cd\u5e94<\/strong><\/p>\n \u56fe5 <\/strong>PtPb\/Pt<\/strong>\u6838\u58f3<\/strong>\u7ed3<\/strong>\u6784<\/strong>\u7eb3<\/strong>\u7c73<\/strong>\u76d8\u7684\u5f62\u8c8c\u53ca\u7ed3\u6784\u8868\u5f81<\/strong><\/p>\n \u82cf\u5dde\u5927<\/strong>\u5b66<\/strong>\u7684\u9ec4\u5c0f\u9752\u6559\u6388\uff08\u901a<\/strong>\u8baf<\/strong>\u4f5c\u8005\uff09<\/strong>\u7b49\u5236\u5907\u4e86PtPb\/Pt\u6838\u58f3\u7ed3\u6784\u7eb3\u7c73\u76d8\u5e76\u5c06\u5176\u7528\u4f5c\u7532\u9187\u91cd\u6574\u50ac\u5316\u5242\u3002\u5c06\u8be5\u7eb3\u7c73\u76d8\u4e0e\u78b3\u6750\u6599\u590d\u5408\uff0c\u6240\u5f97Pt-Pb\u7eb3\u7c73\u76d8\/C\u590d\u5408\u50ac\u5316\u5242\u7684\u6d3b\u6027\u53d6\u51b3\u4e8ePt-Pb\u7eb3\u7c73\u76d8\u7684\u7ec4\u5206\u548c\u7ed3\u6784\u3002\u5176\u4e2dPtPb0.56<\/sub>\u7eb3\u7c73\u76d8\/C\u5728\u7532\u9187\u91cd\u6574\u5236\u6c22\u53cd\u5e94\u4e2d\u8868\u73b0\u51fa\u6700\u9ad8\u7684\u50ac\u5316\u6d3b\u6027\uff0c\u540c\u7b49\u6761\u4ef6\u4e0b\u7684\u50ac\u5316\u53cd\u5e94\u901f\u7387\u662f\u5546\u4e1aPt\/C\u50ac\u5316\u5242\u76845.1\u500d\u3002\u8be5\u8fc7\u7a0b\u4ec5\u4ea7\u751f\u5c11\u91cfCO\u3002\u7814\u7a76\u53d1\u73b0\uff0cPt-Pb\u7eb3\u7c73\u76d8\/C\u4e2d\u9ad8\u7684Pt (0)\/Pt (II)\u6bd4\u662f\u9ad8\u50ac\u5316\u6d3b\u6027\u7684\u6765\u6e90\u3002\u8fd9\u662f\u56e0\u4e3a\u9ad8\u542b\u91cf\u7684Pt (0)\u80fd\u51cf\u5c11CO\u7684\u751f\u6210\u3002Pt-Pb\u7eb3\u7c73\u76d8\u80fd\u4fc3\u4f7fCO\u5206\u5b50\u8f6c\u5316\u4e3a\u7fa7\u9178\u6839\uff0c\u4ece\u800c\u4fc3\u8fdbCO\u6d3b\u5316\u5e76\u964d\u4f4eCO\u751f\u6210\u91cf\u3002<\/p>\n \u6587\u732e\u94fe\u63a5\uff1a<\/strong>Ordered PtPb\/Pt Core\/Shell Nanodisks as Highly Active, Selective, and Stable Catalysts for Methanol Reformation to H2<\/a>\uff08Adv. Energy Mater.\uff0c2018\uff0cDOI: 10.1002\/aenm.201703430\uff09<\/p>\n 6 AFM<\/strong>\uff1a\u5229\u7528\u76f8\u8c03\u5236\u80fd\u7ea7\u7ed3\u6784\u7b56\u7565\u63d0\u5347CdS\u7eb3\u7c73\u68d2\/SnSx<\/sub>\u7eb3\u7c73\u7247\u7684\u5149\u7535\u50ac\u5316\u5206\u89e3\u6c34\u6027\u80fd<\/strong><\/p>\n \u56fe6 <\/strong>OR-SnCd<\/strong>\u3001MP-<\/strong>SnCd<\/strong>\u3001H-<\/strong>SnCd<\/strong>\u7684\u80fd\u7ea7\u7ed3\u6784<\/strong><\/p>\n CdS\u662f\u4e00\u79cd\u7528\u4e8e\u5149\u7535\u50ac\u5316\u5206\u89e3\u6c34\u7684\u5149\u9633\u6781\u6750\u6599\uff0c\u5177\u6709\u53ef\u89c1\u5149\u54cd\u5e94\u548c\u8f83\u597d\u7684\u5149\u50ac\u5316\u6790\u6c27\u6d3b\u6027\u3002\u4f46CdS\u6781\u6613\u5728\u5149\u751f\u7a7a\u7a74\u4f5c\u7528\u4e0b\u53d1\u751f\u81ea\u8150\u8680\uff0c\u5728\u6d4b\u8bd5\u4e2d\u5f80\u5f80\u4f9d\u8d56\u4e8e\u786b\u5316\u7269\u6216\u4e9a\u786b\u9178\u76d0\u7b49\u727a\u7272\u5242\u5bf9\u7a7a\u7a74\u7684\u6355\u83b7\u3002\u4e3a\u4e86\u89e3\u51b3\u8fd9\u4e00\u95ee\u9898\uff0c\u82cf\u5dde\u5927\u5b66<\/strong>\u7684\u674e\u4eae\u6559\u6388<\/strong>\u548c\u897f\u5b89\u4ea4\u901a\u5927\u5b66<\/strong>\u7684\u6c88\u5c11\u534e\u6559\u6388\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7b49\u7528\u4e24\u6b65\u6c34\u70ed\u6cd5\u5408\u6210\u4e86\u5206\u7ea7\u7ed3\u6784\u7684CdS\u7eb3\u7c73\u68d2\/SnSx<\/sub>\u7eb3\u7c73\u7247\u3002\u901a\u8fc7\u8c03\u63a7\u6c34\u70ed\u5408\u6210\u6761\u4ef6\uff0c\u7814\u7a76\u4eba\u5458\u8c03\u6574\u4e86\u50ac\u5316\u5242\u7684\u80fd\u7ea7\u7ed3\u6784\u3002\u4ee5CdS\u7eb3\u7c73\u68d2\/SnSx<\/sub>\u7eb3\u7c73\u7247\u4f5c\u4e3a\u6d3b\u6027\u6750\u6599\u7684\u5149\u9633\u6781\u5728\u4e0d\u542b\u727a\u7272\u5242\u7684Na2<\/sub>SO4<\/sub>\u6c34\u6eb6\u6db2\u4e2d\u8868\u73b0\u51fa\u6bd4\u5355\u7ec4\u5206\u50ac\u5316\u5242\u66f4\u9ad8\u7684\u50ac\u5316\u6d3b\u6027\uff0c\u57281.23 V vs. RHE\u7684\u7535\u4f4d\u53ca\u6a21\u62df\u592a\u9633\u5149\u7167\u5c04\u6761\u4ef6\u4e0b\u80fd\u8fbe\u52301.59 mA\u202fcm\u2212<\/sup>2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\uff0c\u5e76\u5177\u6709\u8f83\u9ad8\u7684\u7535\u5316\u5b66\u7a33\u5b9a\u6027\u3002\u5728CdS\u7eb3\u7c73\u68d2\/SnSx<\/sub>\u7eb3\u7c73\u7247\u590d\u5408\u7ed3\u6784\u4e2d\uff0cCdS\u548cSnSx<\/sub>\u5f62\u6210\u7b2c\u4e8c\u7c7b\u5f02\u8d28\u7ed3\uff0c\u63d0\u9ad8\u4e86\u7535\u8377\u5206\u79bb\u6548\u7387\u3002SnSx<\/sub>\u4f5c\u4e3a\u4fdd\u62a4\u5c42\u80fd\u6709\u6548\u6291\u5236CdS\u7684\u5149\u8150\u8680\u4f5c\u7528\u3002<\/p>\n \u6587\u732e\u94fe\u63a5\uff1a<\/strong>Phase-Modulated Band Alignment in CdS Nanorod\/SnSx Nanosheet Hierarchical Heterojunctions toward Efficient Water Splitting<\/a>\uff08Adv. Funct. Mater.\uff0c2018\uff0cDOI: 10.1002\/adfm.201706785\uff09<\/p>\n 7 Nano Energy<\/strong>\uff1a\u5206\u5f62\u7ed3\u6784\u5355\u5c42MoS2<\/sub>\u7684\u8fb9\u7f18\u6d3b\u6027\u4f4d\u70b9\u8c03\u63a7\u7b56\u7565\u52a9\u529b\u9ad8\u6548\u7535\u50ac\u5316\u6790\u6c22\u53cd\u5e94<\/strong><\/p>\n \u56fe7 \u5355\u5c42MoS2<\/sub>\u7684\u7535\u50ac\u5316\u6790\u6c22\u539f\u7406\u53ca\u5176\u6027\u80fd\u4e0e\u6587\u732e\u503c\u7684\u5bf9\u6bd4<\/strong><\/p>\n \u5317\u4eac\u5927\u5b66<\/strong>\u7684\u6234\u4f26\u6559\u6388<\/strong>\u3001\u53f6\u5809<\/strong>\u6559\u6388<\/strong>\u3001\u674e\u5f66\u6559\u6388\uff08\u5171\u540c\u901a<\/strong>\u8baf<\/strong>\u4f5c\u8005\uff09<\/strong>\u7b49\u5728\u7194\u878d\u77f3\u82f1\u8868\u9762\u76f4\u63a5\u5408\u6210\u4e86\u5206\u5f62\u7ed3\u6784\u7684\u5355\u5c42MoS2<\/sub>\u3002\u8be5MoS2<\/sub>\u5185\u90e8\u5b58\u5728\u8f83\u5927\u7684\u5e94\u529b\uff0c\u5176\u8fb9\u7f18\u66b4\u9732\u51fa\u5927\u91cf\u6d3b\u6027\u4f4d\u70b9\u3002\u8fd9\u4f7f\u5b83\u7684\u7535\u50ac\u5316\u6790\u6c22\u6027\u80fd\u8fdc\u9ad8\u4e8e\u5728SiO2<\/sub>\u8868\u9762\u751f\u957f\u7684\u4e09\u89d2\u5f62MoS2<\/sub>\u3002\u7814\u7a76\u53d1\u73b0\uff0cMoS2<\/sub>\u7684\u7535\u50ac\u5316\u6790\u6c22\u6d3b\u6027\u4e0e\u8fb9\u7f18\u6d3b\u6027\u4f4d\u70b9\u7684\u6570\u76ee\u4e4b\u95f4\u5177\u6709\u7ebf\u6027\u5173\u7cfb\u3002MoS2<\/sub>\u7684\u5185\u5e94\u529b\u4fc3\u4f7f\u66f4\u591a\u7535\u5b50\u5411\u8fb9\u7f18\u6d3b\u6027\u4f4d\u70b9\u8fc1\u79fb\uff0c\u5176\u6d3b\u6027\u6700\u9ad8\u80fd\u8fbe\u52302.74\u202f\u00d7\u202f10\u2212<\/sup>7<\/sup>\u00a0\u03bcA\u202f\u03bcm\u2212<\/sup>1<\/sup>\u3002\u8be5\u5de5\u4f5c\u5f97\u5230\u7684\u5206\u5f62\u7ed3\u6784\u5355\u5c42MoS2<\/sub>\u5177\u6709\u4f18\u5f02\u7684\u7535\u50ac\u5316\u6790\u6c22\u6027\u80fd\uff0c\u8fbe\u523010\u202fmA\u202fcm\u2212<\/sup>2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4ec5\u9700185 mV\u7684\u8fc7\u7535\u4f4d\uff0c\u5176\u5854\u83f2\u5c14\u659c\u7387\u4e3a45\u202fmV\/dec\uff0c\u4ea4\u6362\u7535\u6d41\u5bc6\u5ea6\u4e3a50.9 \u03bcA\u202fcm\u2212<\/sup>2<\/sup>\uff0c\u5e76\u5177\u6709\u8f83\u9ad8\u7684\u7535\u5316\u5b66\u7a33\u5b9a\u6027\u3002\u8fd9\u9879\u5de5\u4f5c\u901a\u8fc7\u63a7\u5236MoS2<\/sub>\u7684\u51e0\u4f55\u5f62\u72b6\u548c\u5185\u5e94\u529b\u72b6\u6001\u5bf9\u5176\u5185\u90e8\u7684\u8f7d\u6d41\u5b50\u8fdb\u884c\u4e86\u8c03\u63a7\uff0c\u4e3a\u63d0\u9ad8\u4e8c\u7ef4\u6750\u6599\u7684\u7535\u50ac\u5316\u6d3b\u6027\u63d0\u4f9b\u4e86\u65b0\u7684\u5408\u6210\u601d\u8def\u3002<\/p>\n
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