{"id":126233,"date":"2018-02-20T14:00:20","date_gmt":"2018-02-20T06:00:20","guid":{"rendered":"\/\/m.iemloyee.com\/?p=126233"},"modified":"2018-02-19T14:20:52","modified_gmt":"2018-02-19T06:20:52","slug":"nano-energy%ef%bc%9a%e9%ab%98%e6%95%88%e6%ba%b6%e6%b6%b2%e6%b3%95%e5%8a%a0%e5%b7%a5cdte%e7%ba%b3%e7%b1%b3%e6%99%b6%e5%a4%aa%e9%98%b3%e8%83%bd%e7%94%b5%e6%b1%a0-%e5%b5%8c%e5%85%a5","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=126233","title":{"rendered":"Nano Energy\uff1a\u9ad8\u6548\u6eb6\u6db2\u6cd5\u52a0\u5de5CdTe\u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60\u2014\u2014\u5d4c\u5165\u65b0\u578b\u4ea4\u8054\u5171\u8f6d\u805a\u5408\u7269\u4f5c\u4e3a\u7a7a\u7a74\u4f20\u8f93\u5c42"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u7eb3\u7c73\u6676(NC),\u9499\u949b\u77ff\u548c\u9ad8\u5206\u5b50\u592a\u9633\u80fd\u7535\u6c60\u4e0e\u4f20\u7edf\u5546\u4e1a\u8584\u819c\u592a\u9633\u80fd\u7535\u6c60\u76f8\u6bd4\u6709\u5f88\u591a\u4f18\u52bf\uff0c\u6bd4\u5982\u53ef\u6eb6\u6db2\u6cd5\u5236\u5907\uff0c\u4f4e\u6750\u6599\u6d88\u8017\uff0c\u4f4e\u6210\u672c\u5e76\u53ef\u901a\u8fc7\u55b7\u6d82\u5927\u9762\u79ef\u5236\u5907\u7b49\u3002\u56e0\u4e3a\u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60\u53ef\u4ee5\u901a\u8fc7\u6210\u5206\u4ee5\u53ca\u5c3a\u5bf8\u8c03\u63a7\u5176\u5e26\u9699\u5bbd\u5ea6\uff0c\u6240\u4ee5\u76f8\u6bd4\u5176\u5b83\u7c7b\u578b\u7684\u592a\u9633\u80fd\u7535\u6c60\u5177\u5907\u66f4\u4f18\u5f02\u7684\u7279\u6027\u3002\u5728\u4f17\u591a\u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60\u4e2d\uff0c CdTe \u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60\u662f\u4e00\u79cd\u6700\u5177\u5438\u5f15\u529b\u7684\u4f53\u7cfb\u3002\u9ad8\u8d28\u91cf\u7684CdTe \u7eb3\u7c73\u6676\uff0c\u5305\u62ec\u7eaf\u5ea6\u3001\u5c3a\u5bf8\u3001\u7ed3\u6784\u3001\u5206\u6563\u6027\u4ee5\u53ca\u5747\u5300\u7684\u5f62\u8c8c\uff0c\u80fd\u591f\u901a\u8fc7\u7b80\u5355\u7684\u5316\u5b66\u5236\u5907\u8fc7\u7a0b\u4e0e\u914d\u4f53\u4ea4\u6362\u7b56\u7565\u7ed3\u5408\u6765\u5f97\u5230\uff0c\u4ea7\u7387\u8fd1\u4e4e100%\u3002\u901a\u8fc7\u7eb3\u7c73\u6676\u5316\u5b66\u5408\u6210\u7684\u8c03\u63a7\u4ee5\u53ca\u5668\u4ef6\u7ed3\u6784\u7684\u4f18\u5316\u8bbe\u8ba1\uff0c\u6eb6\u6db2\u6cd5\u52a0\u5de5\u7684CdTe\u57fa\u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60\u7684\u80fd\u91cf\u8f6c\u6362\u6548\u7387\uff08PCE\uff09\u76ee\u524d\u5df2\u7ecf\u75312.9% \u63d0\u9ad8\u5230~12% (\u5149\u538b\u5904\u7406)\u3002\u4f20\u7edf\u9ad8\u6548\u7684CdTe \u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60\u901a\u8fc7\u5f62\u6210p-n\u7ed3\uff0c\u91c7\u7528ZnO\u4f5c\u4e3a\u7535\u5b50\u63a5\u6536\u4f53\uff0cCdTe\u4f5c\u4e3a\u7535\u5b50\u7ed9\u4f53\u6765\u5236\u5907\uff0c\u5668\u4ef6\u7ed3\u6784\u4e3aITO\/CdTe\/ZnO(\u6216\u8005In\u63ba\u6742ZnO)\/Al\u3002\u5bf9\u4e8e\u8fd9\u79cd\u5668\u4ef6\u7ed3\u6784\uff0c\u867d\u7136PCE\u8fbe\u5230\u4e86~ 10%\uff0c\u4f46\u662f\u5668\u4ef6\u6d4b\u8bd5\u4e4b\u524d\u5fc5\u987b\u5148\u7ecf\u8fc7\u5149\u538b\u5904\u7406\uff0c\u4ee5\u4fbf\u6d88\u9664CdTe (5.3 eV)\u548cITO (4.7 eV)\u4e4b\u95f4\u7684\u529f\u51fd\u6570\u4e0d\u5339\u914d\u6027\u3002\u5668\u4ef6\u7684\u7a33\u5b9a\u6027\u4f9d\u65e7\u662f\u4e00\u4e2a\u5927\u95ee\u9898\uff0c\u56e0\u4e3a\u5728\u653e\u7f6e\u51e0\u5929\u4e4b\u540e\u6ca1\u6709\u8fdb\u4e00\u6b65\u7684\u5149\u538b\u5904\u7406\u540e\uff0cPCE\u4f1a\u964d\u52306%\u3002\u4e0e\u6b64\u76f8\u53cd\uff0c\u91c7\u7528\u5012\u7f6e\u7ed3\u6784\u7684\u78b2\u5316\u9549\u7eb3\u7c73\u6676\u592a\u9633\u7535\u6c60\u7531\u4e8e\u53ef\u4ee5\u9009\u7528\u5177\u6709\u9ad8\u529f\u51fd\u7684\u91d1\u5c5e\/\u91d1\u5c5e\u6c27\u5316\u7269\u4f5c\u4e3a\u80cc\u7535\u6781\uff0c\u5177\u6709\u66f4\u9ad8\u7684\u7a33\u5b9a\u6027\u3002\u5bf9\u4e8eCdTe\u57fa\u592a\u9633\u80fd\u7535\u6c60\uff0cCdTe\u548c\u6b63\u6781\u4e4b\u95f4\u7684\u80fd\u7ea7\u5339\u914d\u662f\u964d\u4f4e\u592a\u9633\u80fd\u80fd\u91cf\u635f\u5931\u4ee5\u53ca\u6700\u5927\u5316\u7535\u538b\u8f93\u51fa\u7684\u57fa\u7840\u3002\u7531\u4e8e\u81ea\u8865\u507f\u6548\u5e94\u4ee5\u53ca\u66f4\u9ad8\u7684\u529f\u51fd\u6570\uff085.3~5.7 eV\uff09\uff0cCdTe\u8584\u819c\u901a\u5e38\u5177\u6709\u5927\u7684\u7535\u963b\uff0c\u6240\u4ee5\u5f88\u96be\u5f97\u5230\u4e00\u4e2a\u826f\u597d\u6b27\u59c6\u63a5\u89e6\u7684\u5668\u4ef6\u3002\u91c7\u7528\u5177\u6709\u9ad8\u529f\u51fd\u7684\u7edd\u7f18\u6750\u6599\u4f5c\u4e3a\u78b2\u5316\u9549\u548c\u80cc\u7535\u6781\u7684\u8fc7\u5ea6\u5c42\uff0c\u662f\u6700\u5177\u6709\u5546\u4e1a\u5e94\u7528\u524d\u666f\u7684\uff0c\u56e0\u4e3a\u5176\u5236\u5907\u65b9\u6cd5\u7b80\u5355\uff0c\u6210\u672c\u4f4e\u5ec9\uff0c\u7a33\u5b9a\u800c\u4e14\u6613\u4e8e\u5236\u5907\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6765\u81ea\u534e\u5357\u7406\u5de5\u5927\u5b66\u7684\u8983\u4e1c\u6b22\u6559\u6388<\/strong>\u7b49\u4eba\u5728Nano Energy<\/strong>\u53d1\u6587\uff0c\u9898\u4e3a\uff1a\u201cHigh-efficient nanocrystal solution-processed CdTe nanocrystal solar cells incorporating a novel crosslinkable conjugated polymer as the hole transport layer<\/strong>\u201d\u3002\u7814\u7a76\u4eba\u5458\u5c06\u4e00\u79cd\u65b0\u578b\u7684\u53ef\u4ea4\u8054\uff08\u70ed\u4ea4\u8054\u6e29\u5ea6120\u5ea6\u5de6\u53f3\uff09\u805a\u5408\u7269(\u4e8c\u82ef\u57fa\u7845\u70f7-co-4-\u4e59\u70ef\u57fa-\u4e09\u82ef\u80fa)(Si-TPA)\u4f5c\u4e3a\u7a7a\u7a74\u4f20\u8f93\u5c42\uff08HTL\uff09\u7528\u4e8e\u6eb6\u6db2\u6cd5\u5236\u5907\u7684CdTe\u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60\u3002\u7814\u7a76\u4eba\u5458\u53d1\u73b0\u4e0e\u6ca1\u6709HTL\u6216\u8005\u5176\u4ed6\u9ad8\u5206\u5b50HTLs\u7684\u5668\u4ef6\u76f8\u6bd4\uff0c\u91c7\u7528Si-TPA HTL\u7684\u5668\u4ef6\u5c55\u73b0\u51fa\u4e86\u66f4\u4f18\u5f02\u7684\u6027\u80fd\u3002\u52a0\u5165Si-TPA \u6240\u5e26\u6765\u7684\u6027\u80fd\u63d0\u5347\u7814\u7a76\u4eba\u5458\u8ba4\u4e3a\u662fSi-TPA\u4e0eCdTe\u5076\u6781\u5b50\u6548\u5e94\uff0c\u540c\u65f6\u4e0e\u78b2\u5316\u9549\u7684\u80fd\u7ea7\u66f4\u52a0\u5339\u914d\uff0c\u5927\u5e45\u51cf\u5c11\u80cc\u590d\u5408\u6548\u5e94\u3002\u63d0\u5347\u7684\u586b\u5145\u56e0\u5b50\u8868\u660e\u7a7a\u7a74\u548c\u7535\u5b50\u5728\u542b\u6709Si-TPA\u7684\u5668\u4ef6\u4e2d\u66f4\u52a0\u5e73\u8861\u3002\u7814\u7a76\u53d1\u73b0\uff0c\u6240\u5236\u5907\u7684\u5177\u6709ITO\/ZnO\/CdSe\/CdTe\/Si-TPA\/Au \u7ed3\u6784\u7684\u5668\u4ef6\uff0cPCE\u4e3a8.34%\uff08\u800c\u4e0d\u4f7f\u7528\u4f20\u8f93\u5c42\u6750\u6599\u7684\u5bf9\u6bd4\u5668\u4ef6ITO\/ZnO\/CdSe\/CdTe\/Au\u6548\u7387\u4ec5\u4e3a5.6%\uff09\uff0c\u8fd9\u662f\u76ee\u524d\u6eb6\u6db2\u6cd5\u5236\u5907\u7684\u5177\u6709\u5012\u7f6e\u7ed3\u6784\u7684CdTe \u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60\u7684\u6700\u9ad8\u7eaa\u5f55\u3002\u4e0e\u6b64\u540c\u65f6\uff0c\u5c06Si-TPA\u5e94\u7528\u4e8e\u53e6\u4e00\u79cd\u78b2\u5316\u9549\u7eb3\u7c73\u6676\u7535\u6c60\uff08\u5668\u4ef6\u7ed3\u6784\u4e3aITO\/ZnO\/CdS\/CdTe\/Si-TPA\/Au\uff0c\u53d7\u4f53\u5c42\u4e3aCdS\u7eb3\u7c73\u6676\uff09\uff0c\u4e5f\u83b7\u5f97\u4e867.27%\u7684PCE\uff08\u4f5c\u4e3a\u53c2\u6bd4\u5668\u4ef6ITO\/ZnO\/CdS\/CdTe\/Au\u6700\u9ad8\u6548\u7387\u4ec5\u4e3a3.6%\uff09\uff0c\u663e\u7136\u4f7f\u7528Si-TPA\u4f20\u8f93\u5c42\u7684\u5668\u4ef6\u6548\u7387\u63d0\u5347\u4e86\u4e00\u500d\uff0c\u8868\u660e\u8fd9\u79cd\u70ed\u4ea4\u8054\u805a\u5408\u7269\u5177\u6709\u5e7f\u6cdb\u7684\u9002\u7528\u6027\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe1. CdTe\u592a\u9633\u80fd\u7535\u6c60\u7ed3\u6784\u793a\u610f\u56fe<\/p>\n

\"\"<\/p>\n

CdTe\/CdSe\u592a\u9633\u80fd\u7535\u6c60\u7ed3\u6784\u793a\u610f\u56fe\uff0cSi-TPA \u5316\u5b66\u7ed3\u6784\uff0cCdTe, CdSe, ZnO, ITO, Si-TPA \u548cAu\u7684\u80fd\u7ea7.<\/p>\n

\u56fe2. Si-TPA\u8868\u5f81<\/p>\n

\"\"<\/p>\n

(a) Si-TPA\u5728\u4e59\u8148\u6eb6\u6db2\u4e2d\u7684CV\u66f2\u7ebf\uff1b<\/p>\n

(b) Si-TPA\u5728\u7532\u82ef\u6eb6\u6db2\u4e2d\u7684\u5438\u6536\u5ea6\uff1b<\/p>\n

(c) Si-TPA\u7ea2\u5916\u5438\u6536\u8c31\uff1b<\/p>\n

(d) XPS\u56fe\uff1aCd 3d\uff0cN 1s.<\/p>\n

\u56fe3. CdSe\/CdTe \u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60J-V\u7279\u6027<\/p>\n

\"\"<\/p>\n

(a) CdSe\/CdTe \u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60w\/o Si-TPA (\u5668\u4ef6\u7ed3\u6784: ITO\/ZnO\/CdSe\/CdTe\/Si-TPA(w\/o)\/Au) \u57281000Wm\u2212<\/sup>2<\/sup> (AM1.5 G) \u7167\u5c04\u4e0b\u7684J-V\u7279\u6027\uff1b(b) \u6697\u6001\uff1b(c)\u76f8\u5e94EQE\u8c31\uff1b(d) CdS\/CdTe \u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60w\/o Si-TPA (\u5668\u4ef6\u7ed3\u6784: ITO\/ZnO\/CdS\/CdTe\/Si-TPA(w\/o)\/Au) \u5149\u7167\u4e0b\u7684J-V\u7279\u6027\uff1b(e) \u6697\u6001\uff1b(f) \u76f8\u5e94EQE\u8c31\uff1b(\u5668\u4ef6A\u548c\u5668\u4ef6C \u7528Si-TPA HTL, \u5668\u4ef6B\u548c\u5668\u4ef6D\u65e0Si-TPA HTL).<\/p>\n

\u56fe4. \u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60\u7684J-V\u7279\u6027<\/p>\n

\"\"<\/p>\n

(a)\u4e0d\u540cHTLs\u7684\u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60\u7684J-V\u7279\u6027\uff1b<\/p>\n

(b) \u76f8\u5e94EQE\u8c31\uff1b<\/p>\n

\u56fe5. Si-TPA\u5668\u4ef6C-V\u7279\u6027<\/p>\n

\"\"<\/p>\n

(a) w\/o Si-TPA\u5668\u4ef6C-V\u7279\u6027\uff1b<\/p>\n

(b)\u4e00\u4e2a\u5728\u5076\u6781\u5c42 (Si-TPA)\u5728CdTe\/Au\u754c\u9762\u5bf9\u80fd\u7ea7\u5f71\u54cd\u7684\u793a\u610f\u56fe\uff1b<\/p>\n

\u3010\u603b\u7ed3\u3011<\/strong><\/p>\n

\u7814\u7a76\u4eba\u5458\u5f00\u53d1\u4e86\u4e00\u79cd\u65b0\u578b\u7684\u53ef\u70ed\u4ea4\u8054\u7684\u805a\u5408\u7269Si-TPA,\u5b83\u53ef\u4ee5\u4f5c\u4e3a\u7eb3\u7c73\u6676\u592a\u9633\u7535\u6c60\u7684\u7a7a\u7a74\u4f20\u8f93\u5c42\u3002\u901a\u8fc7\u5728CdTe\/Au\u4e4b\u95f4\u5f15\u5165\u4e00\u5c42\u4ea4\u8054\u7684Si-TPA\uff08\u7ea620nm\uff0c\u53ef\u6eb6\u6db2\u52a0\u5de5\uff09\uff0c\u4f7f\u5668\u4ef6\u7684\u5f00\u8def\u7535\u538b\u3001\u586b\u5145\u7cfb\u6570\u548c\u77ed\u8def\u7535\u6d41\u540c\u65f6\u5f97\u5230\u589e\u5f3a\uff0c\u4ece\u800c\u8fbe\u5230\u4e868.34%\u7684\u9ad8\u529f\u7387\u8f6c\u6362\u6548\u7387\uff0c\u8fd9\u662f\u76ee\u524d\u6587\u732e\u62a5\u5bfc\u4e2d\u5177\u6709\u5012\u7f6e\u7ed3\u6784\u7684\u78b2\u5316\u9549\u7eb3\u7c73\u6676\u592a\u9633\u7535\u6c60\u7684\u6700\u9ad8\u6c34\u5e73\u3002\u7ed3\u679c\u8868\u660e\uff0c\u91c7\u7528Si-TPA\u7684\u5668\u4ef6\u5728120\u2103\u7684\u4f18\u5316\u4ea4\u8054\u6e29\u5ea6\u4e0b\uff0c\u5177\u6709\u8f83\u9ad8\u7684Vbi<\/sub>\u548c\u8f83\u597d\u7684\u7a7a\u7a74\u8fc1\u79fb\u7387\uff0c\u8fd9\u5bf9\u4e8e\u8f7d\u6d41\u5b50\u7684\u9ad8\u6548\u6536\u96c6\u548c\u51cf\u5c11\u590d\u5408\u81f3\u5173\u91cd\u8981\u3002\u8fd9\u79cd\u7b80\u5355\u7684\u8bbe\u8ba1\u4e5f\u53ef\u4ee5\u7528\u4e8e\u5176\u5b83\u7684\u7eb3\u7c73\u6676\u7cfb\u7edf\uff0c\u4f8b\u5982n\u578bCdS \u7eb3\u7c73\u6676\u592a\u9633\u80fd\u7535\u6c60\uff0c\u5177\u6709\u5f88\u9ad8\u7684PCE\uff1a7.27%\uff0c\u51e0\u4e4e\u662f\u6ca1\u6709\u4f7f\u7528Si-TPA\u7684\u4e24\u500d\uff0c\u8fd9\u8bf4\u660e\u4e86\u8be5\u805a\u5408\u7269\u5177\u6709\u5e7f\u6cdb\u7684\u9002\u5e94\u6027\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aHigh-efficient nanocrystal solution-processed CdTe nanocrystal solar cells incorporating a novel crosslinkable conjugated polymer as the hole transport layer<\/a>(2018\uff0cDOI:10.1016\/j.nanoen.2018.01.048).<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u65b0\u80fd\u6e90\u5b66\u672f\u7ec4Z. Chen\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n

\u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u8fd9\u91cc\u6c47\u96c6\u4e86\u5404\u5927\u9ad8\u6821\u7855\u535a\u751f\u3001\u4e00\u7ebf\u79d1\u7814\u4eba\u5458\u4ee5\u53ca\u884c\u4e1a\u4ece\u4e1a\u8005\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u7f16\u8f91\u90e8<\/a>\u3002<\/p>\n

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\u6750\u6599\u6d4b\u8bd5\uff0c\u6570\u636e\u5206\u6790\uff0c\u4e0a<\/strong>\u6d4b\u8bd5\u8c37<\/strong><\/a>\uff01<\/strong><\/p>\n","protected":false},"excerpt":{"rendered":"

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