{"id":125804,"date":"2018-02-15T14:00:05","date_gmt":"2018-02-15T06:00:05","guid":{"rendered":"\/\/m.iemloyee.com\/?p=125804"},"modified":"2018-02-14T09:28:42","modified_gmt":"2018-02-14T01:28:42","slug":"%e5%90%89%e5%a4%a7%e6%9d%a8%e6%9f%8fangew-chem-int-ed%ef%bc%9a%e8%ae%be%e8%ae%a1%e4%b8%80%e7%b1%bb%e5%85%b7%e6%9c%89%e5%ae%a4%e6%b8%a9%e7%a3%b7%e5%85%89%e6%80%a7%e8%b4%a8%e7%9a%84%e8%81%9a%e5%90%88","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=125804","title":{"rendered":"\u5409\u5927\u6768\u67cfAngew. Chem. Int. Ed\uff1a\u8bbe\u8ba1\u4e00\u7c7b\u5177\u6709\u5ba4\u6e29\u78f7\u5149\u6027\u8d28\u7684\u805a\u5408\u7269\u78b3\u70b9"},"content":{"rendered":"<p><strong>\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n<p>\u539f\u5b50\u6216\u5206\u5b50\u4e2d\u7684\u7535\u5b50\u901a\u8fc7\u5438\u6536\u5165\u5c04\u5149\u4ece\u8f83\u4f4e\u80fd\u6001\u8dc3\u8fc1\u5230\u6fc0\u53d1\u6001\uff0c\u518d\u7531\u6fc0\u53d1\u6001\u8870\u53d8\u5230\u4f4e\u80fd\u6001\u7684\u8f90\u5c04\u53d1\u5149\u8fc7\u7a0b\u79f0\u4f5c\u5149\u81f4\u53d1\u5149\uff0c\u8f90\u5c04\u8dc3\u8fc1\u8fc7\u7a0b\u4f1a\u4ea7\u751f\u8367\u5149\u6216\u78f7\u5149\u3002\u7136\u800c\uff0c\u6fc0\u53d1\u5206\u5b50\u5728\u4e09\u7ebf\u6001\u7684\u78f7\u5149\u8f90\u5c04\u8dc3\u8fc1\u8fc7\u7a0b\u6709\u76f8\u5bf9\u8f83\u957f\u7684\u5bff\u547d\uff0c\u5bb9\u6613\u4e0e\u6eb6\u5242\u5206\u5b50\u78b0\u649e\u800c\u5931\u6d3b\u6216\u88ab\u987a\u78c1\u7c7b\u7269\u8d28\u731d\u706d\uff0c\u5bfc\u81f4\u5ba4\u6e29\u4e0b\u6d41\u4f53\u4ecb\u8d28\u4e2d\u7684\u78f7\u5149\u51cf\u5f31\u6216\u6d88\u5931\u3002\u65e9\u671f\u5e38\u5c06\u78f7\u5149\u8bd5\u6837\u51b7\u5374\u5230\u6db2\u6c2e\u6e29\u5ea6\u5f62\u6210\u4f4e\u6e29\u521a\u6027\u73bb\u7483\u4f53\u4ee5\u89c2\u5bdf\u78f7\u5149\uff0c\u5373\u4f4e\u6e29\u78f7\u5149\uff0c\u800c\u6df1\u51b7\u7684\u5b9e\u9a8c\u6761\u4ef6\u4f7f\u5176\u5e94\u7528\u53d7\u5230\u4e86\u9650\u5236\u3002\u56e0\u6b64\uff0c\u5ba4\u6e29\u78f7\u5149\u56e0\u8f83\u957f\u7684\u5bff\u547d\u548c\u8f83\u5bbd\u7684\u65af\u6258\u514b\u65af\u4f4d\u79fb\uff0c\u5728\u751f\u7269\u6210\u50cf\u3001\u5149\u5b66\u8bb0\u5f55\u3001\u9632\u4f2a\u7cfb\u7edf\u7b49\u8bf8\u591a\u9ad8\u65b0\u79d1\u6280\u9886\u57df\u6709\u7740\u8bf1\u4eba\u7684\u5e94\u7528\u524d\u666f\u3002\u805a\u5408\u7269\u78b3\u70b9\u662f\u7531\u9ad8\u5206\u5b50\u9002\u5ea6\u4ea4\u8054\u78b3\u5316\u6216\u901a\u8fc7\u78b3\u6838\u548c\u805a\u5408\u7269\u7ec4\u88c5\u5f62\u6210\u7684\u78b3\u7eb3\u7c73\u70b9\u3002\u5b83\u4f5c\u4e3a\u4e00\u79cd\u65b0\u578b\u7684\u65e0\u91d1\u5c5e\u5ba4\u6e29\u78f7\u5149\u6750\u6599\uff0c\u5177\u6709\u8bf8\u591a\u4f18\u5f02\u7684\u6027\u80fd\u5982\u4f4e\u751f\u7269\u6bd2\u6027\u3001\u826f\u597d\u7684\u52a0\u5de5\u6027\u3001\u8f83\u4f4e\u7684\u6210\u672c\u3001\u4f18\u5f02\u7684\u67d4\u6027\u3001\u9002\u5408\u5927\u9762\u79ef\u5236\u5907\u7b49\u5f97\u5230\u4e86\u4eba\u4eec\u7684\u5e7f\u6cdb\u5173\u6ce8\u3002<\/p>\n<p><strong>\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n<p>\u8fd1\u65e5\uff0c\u5409\u6797\u5927\u5b66\u8d85\u5206\u5b50\u6750\u6599\u4e0e\u7ed3\u6784\u56fd\u5bb6\u91cd\u70b9\u5b9e\u9a8c\u5ba4<strong>\u6768\u67cf\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u5728<strong>Angew. Chem. Int. Ed<\/strong>\u6742\u5fd7\u4e0a\u53d1\u8868\u9898\u4e3a\u201c<strong>Design of Metal-Free Polymer Carbon Dots: a New Class of Room-Temperature Phosphorescent Materials<\/strong>\u201d\u7684\u6587\u7ae0\u3002\u4ed6\u4eec\u91c7\u7528\u805a\u4e19\u70ef\u9178\u548c\u4e59\u4e8c\u80fa\u7b49\u4e00\u6b65\u6c34\u70ed\u6cd5\u5236\u5907\u51fa\u805a\u5408\u7269\u78b3\u70b9\uff0c\u5176\u78f7\u5149\u5bff\u547d\u503c\u8fbe\u5230658ms\uff0c\u56fa\u6001\u603b\u91cf\u5b50\u4ea7\u7387\u4e3a28.77%\u3002\u66f4\u4e3a\u91cd\u8981\u7684\u662f\uff0c\u6768\u67cf\u6559\u6388\u8bfe\u9898\u7ec4\u5728\u6b64\u57fa\u7840\u4e0a\u8bbe\u8ba1\u5e76\u5408\u6210\u7684\u4e00\u7cfb\u5217\u5ba4\u6e29\u78f7\u5149\u805a\u5408\u7269\u78b3\u70b9\u90fd\u517c\u5177\u9ad8\u6548\u7387\u548c\u957f\u5bff\u547d\u7684\u4f18\u5f02\u7279\u6027\uff0c\u5e76\u901a\u8fc7DFT\u7b2c\u4e00\u6027\u539f\u7406\u8ba1\u7b97\u63ed\u793a\u4e86\u6b64\u7c7b\u5ba4\u6e29\u78f7\u5149\u805a\u5408\u7269\u78b3\u70b9\u7684\u78f7\u5149\u8d77\u6e90\uff1a\u662f\u7531\u805a\u5408\u4ea4\u8054\u6548\u5e94\u9650\u5236\u4e86\u5b98\u80fd\u56e2\u7684\u632f\u8f6c\uff0c\u4fc3\u4f7f\u4e86\u5355\u7ebf\u6001\u5230\u4e09\u7ebf\u6001\u7684\u8dc3\u8fc1\uff0c\u4ece\u800c\u8bf1\u5bfc\u4e86\u5ba4\u6e29\u78f7\u5149\u3002\u8be5\u9879\u5de5\u4f5c\u7684\u7b2c\u4e00\u4f5c\u8005\u4e3a\u5409\u6797\u5927\u5b66<strong>\u7855\u58eb\u7814\u7a76\u751f\u9676\u6dde\u6e90<\/strong>\u548c\u90d1\u5dde\u5927\u5b66\u5316\u5b66\u4e0e\u5206\u5b50\u5de5\u7a0b\u5b66\u9662\u526f\u6559\u6388<strong>\u5362\u601d\u5b87<\/strong>\uff0c\u611f\u8c22\u6768\u67cf\u6559\u6388\u548c\u5362\u601d\u5b87\u535a\u58eb\u5bf9\u672c\u6587\u7684\u5199\u4f5c\u6307\u5bfc\u4e0e\u4fee\u6539\u3002<\/p>\n<p><strong>\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n<p><strong>\u56fe1. \u5ba4\u6e29\u78f7\u5149\u805a\u5408\u7269\u78b3\u70b9\u7684\u5149\u8c31\u548c\u7ed3\u6784\u8868\u5f81<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-125832\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/02\/1-23.png\" alt=\"\" width=\"600\" height=\"450\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/02\/1-23.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/02\/1-23-300x225.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>a.\u805a\u5408\u7269\u78b3\u70b9PCDsI-1\u6c34\u6eb6\u6db2\u7684\u8367\u5149\u5149\u8c31\u56fe\u4e0eUV\u4e0b\u5149\u5b66\u7167\u7247<\/p>\n<p>b.\u805a\u5408\u7269\u78b3\u70b9PCDsI-1\u56fa\u6001\u8367\u5149\u5149\u8c31\u56fe\u4e0eUV\u4e0b\u5149\u5b66\u7167\u7247<\/p>\n<p>c.\u805a\u5408\u7269\u78b3\u70b9PCDsI-1\u7c89\u672b\u78f7\u5149\u5149\u8c31\u56fe<\/p>\n<p>d.\u805a\u5408\u7269\u78b3\u70b9PCDsI-1\uff0c PCDsI-2\uff0c PCDsI-3\u7c89\u672bUV\u4e0b\u5149\u5b66\u7167\u7247<\/p>\n<p>e.\u805a\u5408\u7269\u78b3\u70b9PCDsI-1\uff0c PCDsI-2\uff0c PCDsI-3\u7c89\u672b\u7684\u78f7\u5149\u5bff\u547d\u5149\u8c31<\/p>\n<p>f.\u805a\u5408\u7269\u78b3\u70b9PCDsI-1\uff0c PCDsI-2\uff0c PCDsI-3\u7c89\u672b\u7684\u7d2b\u5916\u5438\u6536\u5149\u8c31<\/p>\n<p>g.\u805a\u5408\u7269\u78b3\u70b9PCDsI-1\uff0c PCDsI-2\uff0c PCDsI-3\u7c89\u672b\u7684\u7ea2\u5916\u5149\u8c31<\/p>\n<p>h.\u805a\u5408\u7269\u78b3\u70b9PCDsI-1\uff0c PCDsI-2\uff0c PCDsI-3\u7c89\u672b\u7684X\u5c04\u7ebf\u5149\u7535\u5b50\u80fd\u8c31<\/p>\n<p><strong>\u56fe2.\u4e09\u79cd\u5ba4\u6e29\u78f7\u5149\u805a\u5408\u7269\u78b3\u70b9\u7684\u9ad8\u5206\u8fa8X\u5c04\u7ebf\u5149\u7535\u5b50\u80fd\u8c31<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-125827\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/02\/2-23.png\" alt=\"\" width=\"600\" height=\"432\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/02\/2-23.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/02\/2-23-300x216.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>a.b.c.\u5206\u522b\u4e3aPCDsI-1\u7684C1s, N1s, O1s\u7cbe\u7ec6\u8c31<\/p>\n<p>d.e.f.\u5206\u522b\u4e3aPCDsI-2\u7684C1s, N1s, O1s\u7cbe\u7ec6\u8c31<\/p>\n<p>g.h.i.\u5206\u522b\u4e3aPCDsI-3\u7684C1s, N1s, O1s\u7cbe\u7ec6\u8c31<\/p>\n<p><strong>\u56fe3.\u4e09\u79cd\u5ba4\u6e29\u78f7\u5149\u805a\u5408\u7269\u78b3\u70b9<\/strong><strong>\u5ba4\u6e29\u78f7\u5149\u6765\u6e90\u7684\u8ba1\u7b97\u5206\u6790<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-125833\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/02\/3-17.png\" alt=\"\" width=\"600\" height=\"564\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/02\/3-17.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/02\/3-17-300x282.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>a.\u4e09\u79cd\u5ba4\u6e29\u78f7\u5149\u805a\u5408\u7269\u78b3\u70b9\u53ef\u80fd\u7684\u4ea4\u8054\u4f4d\u70b9<\/p>\n<p>b.\u672a\u4ea4\u8054\u7ed3\u6784\u7684\u80fd\u7ea7<\/p>\n<p>c.\u4ea4\u8054\u540e\u7ed3\u6784\u7684\u80fd\u7ea7<\/p>\n<p>d.\u4ea4\u8054\u589e\u5f3a\u53d1\u5c04\u6548\u5e94\u7684\u673a\u7406\u56fe<\/p>\n<p><strong>\u56fe4.\u5ba4\u6e29\u78f7\u5149\u805a\u5408\u7269\u78b3\u70b9\u7684\u8367\u5149\/\u5ba4\u6e29\u78f7\u5149\u5e94\u7528<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-125834\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/02\/4-12.png\" alt=\"\" width=\"600\" height=\"399\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2018\/02\/4-12.png 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2018\/02\/4-12-300x200.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u4fdd\u5bc6\u56fe\u6848\u548c\u5b57\u6bcd\u7684\u5e94\u7528<\/p>\n<p><strong>\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n<p>\u6587\u7ae0\u5408\u6210\u5236\u5907\u4e86\u4e00\u7cfb\u5217\u5177\u6709\u5ba4\u6e29\u78f7\u5149\u7684\u805a\u5408\u7269\u78b3\u70b9\uff0c\u63d0\u51fa\u4e86\u4e00\u79cd\u5236\u5907\u5ba4\u6e29\u78f7\u5149\u6750\u6599\u7684\u65b9\u6cd5\uff0c\u4f7f\u5176\u78f7\u5149\u5bff\u547d\u6700\u957f\u53ef\u8fbe658.11ms\uff0c\u5e76\u4e14\u91c7\u7528DFT\u7b2c\u4e00\u6027\u539f\u7406\u8ba1\u7b97\u63ed\u793a\u4e86\u6b64\u7c7b\u5ba4\u6e29\u78f7\u5149\u805a\u5408\u7269\u78b3\u70b9\u7684\u78f7\u5149\u8d77\u6e90\uff1a\u662f\u7531\u805a\u5408\u4ea4\u8054\u6548\u5e94\u9650\u5236\u4e86\u5b98\u80fd\u56e2\u7684\u632f\u8f6c\uff0c\u4fc3\u4f7f\u4e86\u5355\u7ebf\u6001\u5230\u4e09\u7ebf\u6001\u7684\u8dc3\u8fc1\uff0c\u4ece\u800c\u8bf1\u5bfc\u4e86\u5ba4\u6e29\u78f7\u5149\u3002\u589e\u52a0\u4e86\u5ba4\u6e29\u78f7\u5149\u6750\u6599\u5bb6\u65cf\u7684\u79cd\u7c7b\uff0c\u540c\u65f6\u4e5f\u62d3\u5c55\u4e86\u805a\u5408\u7269\u78b3\u70b9\u7684\u6027\u8d28\uff0c\u5bf9\u78b3\u70b9\u7684\u7814\u7a76\u53d1\u5c55\u8d77\u5230\u81f3\u5173\u91cd\u8981\u7684\u4f5c\u7528\u3002<\/p>\n<p><strong>\u3010\u6587\u732e\u94fe\u63a5\u3011<\/strong>\uff1a<a href=\"http:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/anie.201712662\/full\" target=\"_blank\" rel=\"noopener\">Design of Metal-Free Polymer Carbon Dots: a New Class of Room-Temperature Phosphorescent Materials<\/a> (<em>Angew. Chem. Int. Ed.<\/em> 2018, DOI: 10.1002\/ange.201712662)<\/p>\n<p><strong>\u3010\u8bfe\u9898\u7ec4\u7b80\u4ecb\u3011<\/strong><\/p>\n<p><strong>\u6768\u67cf\u6559\u6388\u8bfe\u9898\u7ec4<\/strong>\u8fd1\u5e74\u6765\u4e3b\u8981\u7814\u7a76\u65b9\u5411\u662f\u901a\u8fc7\u5728\u5206\u5b50\u8bbe\u8ba1\u3001\u7eb3\u7c73\u6742\u5316\u548c\u5728\u4ecb\u89c2\u5c3a\u5ea6\u4e0a\u6784\u7b51\u65b0\u578b\u6709\u5e8f\u5fae\u7ed3\u6784\uff0c\u6765\u5b9e\u73b0\u805a\u5408\u7269\u5149\u5b66\u6750\u6599\u7684\u9ad8\u6027\u80fd\u5316\u548c\u529f\u80fd\u5316\uff0c\u622a\u81f32017\u5e747\u6708\uff08Web of Science\uff09\u53d1\u8868\u8bba\u6587500\u4f59\u7bc7\uff0c\u88ab\u5f15\u7528 16000 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