{"id":120394,"date":"2018-01-09T06:30:39","date_gmt":"2018-01-08T22:30:39","guid":{"rendered":"\/\/m.iemloyee.com\/?p=120394"},"modified":"2018-01-08T23:56:56","modified_gmt":"2018-01-08T15:56:56","slug":"nat-commun-%e5%85%89%e8%b0%83%e6%8e%a7%e9%80%89%e6%8b%a9%e5%90%88%e6%88%90%e5%81%b6%e6%b0%ae%e6%88%96%e6%b0%a7%e5%8c%96%e5%81%b6%e6%b0%ae%e8%8a%b3%e9%a6%99%e7%83%83","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=120394","title":{"rendered":"Nat. Commun.: \u5149\u8c03\u63a7\u9009\u62e9\u5408\u6210\u5076\u6c2e\u6216\u6c27\u5316\u5076\u6c2e\u82b3\u9999\u70c3"},"content":{"rendered":"
\u3010\u5f15\u8a00<\/strong>\u3011<\/p>\n \u8fd1\u5e74\u6765\uff0c\u5149\u50ac\u5316\u5728\u6709\u673a\u5408\u6210\u65b9\u9762\u7684\u7814\u7a76\u83b7\u5f97\u4e86\u91cd\u5927\u5173\u6ce8\u3002\u4e0e\u4f20\u7edf\u50ac\u5316\u76f8\u6bd4\uff0c\u5149\u50ac\u5316\u6709\u673a\u5408\u6210\u5177\u6709\u7eff\u8272\uff0c\u53cd\u5e94\u6761\u4ef6\u6e29\u548c\u7b49\u4f18\u70b9\uff0c\u4f46\u662f\u9009\u62e9\u6027\u548c\u53cd\u5e94\u6d3b\u6027\u4ecd\u6709\u5f85\u63d0\u9ad8\u3002\u4ee5\u5149\u50ac\u5316\u785d\u57fa\u82ef\u8fd8\u539f\u4e3a\u4f8b\uff0c\u4f7f\u7528\u5e38\u89c4\u5149\u50ac\u5316\u5242(TiO2,CdS)\u53ef\u4ee5\u5c06\u785d\u57fa\u82ef\u5b8c\u5168\u8fd8\u539f\u8f6c\u5316\u4e3a\u82ef\u80fa\uff0c\u4f46\u82ef\u80fa\u7684\u7ecf\u6d4e\u4ef7\u503c\u8f83\u4f4e\u3002\u4f7f\u7528\u7b49\u79bb\u5b50\u4f53\u91d1\u5c5e\u7eb3\u7c73\u7c92\u5b50\u5149\u50ac\u5316\u5242\u53ef\u4ee5\u5c06\u785d\u57fa\u82ef\u9009\u62e9\u6027\u8fd8\u539f\u4e3a\u5076\u6c2e\u82ef\u3002\u8be5\u4ea7\u7269\u662f\u67d3\u6599\uff0c\u7535\u5b50\uff0c\u533b\u836f\u7b49\u884c\u4e1a\u7684\u91cd\u8981\u524d\u9a71\u4f53\uff0c\u7ecf\u6d4e\u4ef7\u503c\u6781\u9ad8\u3002\u7136\u800c\uff0c\u8fd9\u79cd\u6602\u8d35\u7684\u50ac\u5316\u5242\u5728\u5ba4\u6e29\u4e0b\u6548\u7387\u548c\u9009\u62e9\u6027\u8fd8\u6709\u5f85\u63d0\u9ad8\u3002<\/p>\n \u3010\u6210\u679c\u7b80\u4ecb<\/strong>\u3011<\/p>\n \u8fd1\u65e5\uff0c\u4e2d\u79d1\u5408\u6210\u6cb9\u6280\u672f\u6709\u9650\u516c\u53f8\u82cf\u97e7<\/strong>\u7b49\u4eba\u540c\u4e39\u9ea6\u5965\u80e1\u601d\u5927\u5b66<\/strong>\uff08Aarhus University\uff09Flemming Besenbacher<\/strong>\u6559\u6388\uff08\u4e2d\u79d1\u9662\u5916\u7c4d\u9662\u58eb\uff09\u8bfe\u9898\u7ec4\u5728Nature <\/strong>Communications<\/strong>\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201cLight-tuned selective photosynthesis of azo- and<\/strong> azoxy-aromatics using graphitic C3<\/sub>N4<\/sub><\/strong>\u201d\u7684\u6587\u7ae0\u3002\u8be5\u5de5\u4f5c\u53d1\u73b0\uff0c\u4f7f\u7528\u5ec9\u4ef7\u7684g-C3<\/sub>N4<\/sub>\u53ef\u4ee5\u5b9e\u73b0\u53ef\u89c1\u5149\u6761\u4ef6\u4e0b\u9ad8\u6548\uff0c\u9ad8\u9009\u62e9\u8fd8\u539f\u785d\u57fa\u82ef\u5236\u5907\u5076\u6c2e\u82ef\u6216\u6c27\u5316\u5076\u6c2e\u82ef\u3002\u8be5\u53cd\u5e94\u7684\u9009\u62e9\u6027\u53ef\u4ee5\u901a\u8fc7\u8c03\u63a7\u8f90\u7167\u6ce2\u957f\u5b9e\u73b0\uff0c\u5e76\u4e14\u53ef\u4ee5\u5c06\u4e00\u7cfb\u5217\u5177\u6709\u4e0d\u540c\u5b98\u80fd\u56e2\u7684\u785d\u57fa\u82b3\u9999\u70c3\u5316\u5408\u7269\u9009\u62e9\u6027\u8f6c\u5316\u4e3a\u76f8\u5e94\u7684\u5076\u6c2e\u6216\u6c27\u5316\u5076\u6c2e\u5316\u5408\u7269\u3002\u8be5\u8bfe\u9898\u7ec4\u9996\u6b21\u63a2\u7d22\u4e86\u5149\u50ac\u5316\u6709\u673a\u5408\u6210\u53cd\u5e94\u653e\u5927\u7684\u53ef\u884c\u6027\uff0c\u5e76\u4e14\u5728\u592a\u9633\u5149\u6761\u4ef6\u4e0b\u521d\u6b65\u5b9e\u73b0\u4e8680 L\u5149\u50ac\u5316\u785d\u57fa\u82ef\u9009\u62e9\u6027\u8f6c\u5316\uff0c\u63ed\u793a\u4e86\u5149\u50ac\u5316\u7528\u4e8e\u5927\u89c4\u6a21\u751f\u4ea7\u9ad8\u9644\u52a0\u503c\u5316\u5b66\u54c1\u7684\u5de8\u5927\u6f5c\u529b\u3002\u8be5\u5de5\u4f5c\u8fdb\u4e00\u6b65\u5229\u7528\u7a0b\u5e8f\u5347\u6e29\u8131\u9644\uff0c\u539f\u4f4dXPS\u548c\u63a7\u5236\u5b9e\u9a8c\u7ed3\u5408\u7406\u8bba\u8ba1\u7b97\u5206\u6790\u4e86g-C3<\/sub>N4<\/sub>\u6750\u6599\u5728\u8be5\u53cd\u5e94\u4e2d\u7684\u9ad8\u6d3b\u6027\u548c\u9ad8\u9009\u62e9\u6027\u3002\u5b9e\u9a8c\u53d1\u73b0g-C3<\/sub>N4<\/sub>\u8868\u9762\u5149\u7167\u53cd\u5e94\u751f\u6210\u7684\u6c22\u539f\u5b50\u5177\u6709\u6781\u4f4e\u7684\u5438\u9644\u80fd\uff0c\u5e76\u4e14\u80fd\u591f\u4fc3\u8fdbN-N\u5076\u8054\u53cd\u5e94\uff0c\u56e0\u6b64\u5177\u6709\u6781\u9ad8\u7684\u6d3b\u6027\u548c\u9009\u62e9\u6027\u3002<\/p>\n \u3010\u56fe\u6587\u5bfc\u8bfb<\/strong>\u3011<\/b><\/p>\n \u56fe<\/strong>1. <\/strong>\u5149\u50ac\u5316\u8fd8\u539f\u785d\u57fa\u82ef\u53cd\u5e94\u8fc7\u7a0b\u53ca\u4ea7\u7269\uff08\u4ef7\u683c\u4e3a\u8bd5\u5242\u4ef7\uff09<\/strong><\/p>\n \u8868<\/strong>1. <\/strong>\u4e0d\u540c\u5149\u50ac\u5316\u5242\u4f30\u7b97\u4ef7\u683c\u53ca\u5176\u50ac\u5316\u6d3b\u6027\u5bf9\u6bd4\uff08\u7ea2\u8272\u7c97\u4f53\u6807\u6ce8\u4e3a\u672c\u5de5\u4f5c\u4e2d\u6240\u7528\u50ac\u5316\u5242\uff09<\/strong><\/p>\n \u56fe<\/strong>2. (a), (b) 410 nm<\/strong>\u548c<\/strong>450 nm<\/strong>\u5149\u7167\u6761\u4ef6\u4e0b\u785d\u57fa\u82ef\u8fd8\u539f\u8fc7\u7a0b\uff1b<\/strong>(c) <\/strong>\u4e0d\u540c\u785d\u57fa\u82ef\u521d\u59cb\u6d53\u5ea6\u53cd\u5e94\u8f6c\u5316\u7387\u548c\u9009\u62e9\u6027\u7684\u5173\u7cfb\uff1b<\/strong>(d)-(g) 800 mL <\/strong>\u548c<\/strong>80 L<\/strong>\u592a\u9633\u5149\u6761\u4ef6\u4e0b\u653e\u5927\u53cd\u5e94\u6d4b\u8bd5\u7ed3\u679c\u3002<\/strong><\/p>\n \u56fe<\/strong>3. <\/strong>\u9009\u62e9\u6027\u8fd8\u539f\u5177\u6709\u4e0d\u540c\u5b98\u80fd\u56e2\u7684\u785d\u57fa\u82ef\u7ed3\u679c\uff081\uff09<\/strong><\/p>\n \u56fe<\/strong>4. <\/strong>\u9009\u62e9\u6027\u8fd8\u539f\u5177\u6709\u4e0d\u540c\u5b98\u80fd\u56e2\u7684\u785d\u57fa\u82ef\u7ed3\u679c\uff082\uff09<\/strong><\/p>\n \u3010\u7ed3\u8bba<\/strong>\u3011<\/b><\/p>\n \u8be5\u5de5\u4f5c\u9996\u6b21\u62a5\u9053\u4e86\u5ba4\u6e29\u6761\u4ef6\u4e0b\u5229\u7528\u53ef\u89c1\u5149\u9a71\u52a8N-N\u5076\u8054\u53cd\u5e94\uff0c\u5236\u5907\u4e00\u7cfb\u5217\u9ad8\u9644\u52a0\u503c\u5076\u6c2e\u6216\u6c27\u5316\u5076\u6c2e\u7c7b\u82b3\u9999\u70c3\u7684\u53ef\u884c\u6027\u3002\u8be5\u53cd\u5e94\u7684\u9009\u62e9\u6027\u53ef\u4ee5\u901a\u8fc7\u8c03\u63a7\u8f90\u7167\u6ce2\u957f\u5b9e\u73b0\uff0c\u5e76\u4e14\u5728\u592a\u9633\u5149\u6761\u4ef6\u4e0b\u521d\u6b65\u5b9e\u73b0\u4e86\u5de5\u4e1a\u7ea7\u5149\u50ac\u5316\u8fc7\u7a0b\u7684\u653e\u5927\uff0c\u5177\u6709\u5de8\u5927\u7684\u5546\u4e1a\u6f5c\u529b\u3002<\/p>\n \u672c\u5de5\u4f5c\u611f\u8c22\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u59d4\uff0c\u4e2d\u4e39\u4e2d\u5fc3\uff0c\u4e39\u9ea6Villum \u00a0Foundation\uff0c\u4e39\u9ea6\u56fd\u5bb6\u79d1\u7814\u57fa\u91d1\u53ca\u5609\u58eb\u4f2f\u57fa\u91d1\u652f\u6301\u3002<\/p>\n \u6587\u732e\u94fe\u63a5\uff1a<\/strong>Light-tuned selective photosynthesis of azo- and azoxy-aromatics using graphitic C3<\/sub>N4<\/sub><\/a>(Nat. Commun. 2018, doi:10.1038\/s41467-017-02527-8)<\/p>\n \u8bfe\u9898\u7ec4\u7b80\u4ecb\uff1a<\/strong><\/p>\n \u672c\u8bfe\u9898\u7ec4\u96b6\u5c5e\u4e8e\u4e2d\u79d1\u5408\u6210\u6cb9\u6280\u672f\u6709\u9650\u516c\u53f8<\/a>\u8868\u9762\u79d1\u5b66\u5b9e\u9a8c\u5ba4<\/a>\uff08Syncat@Beijing\uff0cSynfuelsChina Technology Co. Ltd.\uff09\u53ca\u7164\u8f6c\u5316\u56fd\u5bb6\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u3002\u4e3b\u8981\u7814\u7a76\u65b9\u5411\u4e3a\u5149\uff08\u7535\uff09\u50ac\u5316\u7684\u673a\u7406\u63a2\u7d22\u53ca\u5176\u5728\u6709\u673a\u5408\u6210\uff0c\u80fd\u6e90\u8f6c\u5316\uff0c\u6c61\u6c34\u5904\u7406\u7b49\u65b9\u9762\u7684\u5e94\u7528\u3002\u5b9e\u9a8c\u5ba4\u8d1f\u8d23\u4eba\u82cf\u97e7\u535a\u58eb2012\u5e74\u6bd5\u4e1a\u4e8e\u4e39\u9ea6\u5965\u80e1\u601d\u5927\u5b66\uff0c\u5e08\u4eceFlemming Besenbacher\u6559\u6388\u3002\u672c\u8bfe\u9898\u7ec4\u62e5\u6709\u539f\u4f4d\u8d28\u8c31\uff0c\u539f\u4f4d\u7d2b\u5916\u5149\u8c31\uff0c\u539f\u4f4d\u7ea2\u5916-\u8d28\u8c31\u8054\u7528\u7b49\u8bbe\u5907\u7528\u4e8e\u7814\u7a76\u5149\u7535\u50ac\u5316\u53cd\u5e94\u8fc7\u7a0b\u3002\u672c\u8bfe\u9898\u7ec4\u5e0c\u671b\u80fd\u4e0e\u56fd\u5185\u4f18\u79c0\u7684\u8bfe\u9898\u7ec4\u5c55\u5f00\u8fdb\u4e00\u6b65\u5408\u4f5c\uff0c\u4e00\u540c\u63a8\u52a8\u5149\uff08\u7535\uff09\u50ac\u5316\u9886\u57df\u7684\u53d1\u5c55\u3002\u8054\u7cfb\u65b9\u5f0f\uff1asuren@synfuelschina.com.cn<\/p>\n \u672c\u6587\u7531\u4e2d\u79d1\u5408\u6210\u6cb9\u6280\u672f\u6709\u9650\u516c\u53f8\u8868\u9762\u79d1\u5b66\u5b9e\u9a8c\u5ba4\u82cf\u97e7\u63d0\u4f9b\uff0c\u7279\u6b64\u611f\u8c22\u3002<\/p>\n \u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u8fd9\u91cc\u6c47\u96c6\u4e86\u5404\u5927\u9ad8\u6821\u7855\u535a\u751f\u3001\u4e00\u7ebf\u79d1\u7814\u4eba\u5458\u4ee5\u53ca\u884c\u4e1a\u4ece\u4e1a\u8005\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u7f16\u8f91\u90e8\u5927\u5bb6\u5ead<\/a>\u3002<\/p>\n \u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n \u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1aRDD-2011-CHERISH\uff0c\u4efb\u4e39\u4e39\uff0c\u6211\u4eec\u4f1a\u9080\u8bf7\u5404\u4f4d\u8001\u5e08\u52a0\u5165\u4e13\u5bb6\u7fa4\u3002<\/b><\/strong><\/p>\n<\/p>\n
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