{"id":119507,"date":"2017-12-31T06:30:24","date_gmt":"2017-12-30T22:30:24","guid":{"rendered":"\/\/m.iemloyee.com\/?p=119507"},"modified":"2017-12-30T14:53:40","modified_gmt":"2017-12-30T06:53:40","slug":"%e8%8b%8f%e5%b7%9e%e5%a4%a7%e5%ad%a6%e4%b8%8a%e6%b5%b7%e4%ba%a4%e9%80%9a%e5%a4%a7%e5%ad%a6adv-mater-%e7%ae%80%e5%8d%95%e5%88%b6%e5%a4%87%e7%9a%84%e5%af%b9%e6%b4%bb%e6%80%a7%e5%b1%82%e8%86%9c","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=119507","title":{"rendered":"\u82cf\u5dde\u5927\u5b66&\u4e0a\u6d77\u4ea4\u901a\u5927\u5b66Adv. Mater.: \u7b80\u5355\u5236\u5907\u7684\u5bf9\u6d3b\u6027\u5c42\u819c\u539a\u548c\u5668\u4ef6\u9762\u79ef\u53d8\u5316\u4e0d\u654f\u611f\u7684\u9ad8\u6548\u975e\u5bcc\u52d2\u70ef\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u968f\u7740\u4e16\u754c\u7ecf\u6d4e\u7684\u9ad8\u901f\u53d1\u5c55\uff0c\u80fd\u6e90\u548c\u73af\u5883\u5371\u673a\u5df2\u65e5\u76ca\u52a0\u5267\uff0c\u4eba\u4eec\u5bf9\u6e05\u6d01\u80fd\u6e90\u7684\u9700\u6c42\u4e5f\u8d8a\u6765\u8d8a\u8feb\u5207\u3002\u592a\u9633\u80fd\u4f5c\u4e3a\u53d6\u4e4b\u4e0d\u5c3d\u3001\u7528\u4e4b\u4e0d\u7aed\u7684\u7eff\u8272\u80fd\u6e90\uff0c\u5176\u5982\u4f55\u9ad8\u6548\u5229\u7528\u4e00\u76f4\u662f\u4eba\u4eec\u7684\u7814\u7a76\u70ed\u70b9\u3002\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\u5177\u6709\u8d28\u8f7b\u3001\u53ef\u5927\u9762\u79ef\u5236\u5907\u67d4\u6027\u534a\u900f\u660e\u5668\u4ef6\u7b49\u4f18\u70b9\u800c\u53d7\u5230\u7814\u7a76\u8005\u4eec\u7684\u5e7f\u6cdb\u5173\u6ce8\u3002\u8fd1\u4e24\u5e74\uff0c\u968f\u7740\u7a84\u5e26\u9699\u975e\u5bcc\u52d2\u70ef\u53d7\u4f53\u6750\u6599\u7684\u98de\u901f\u53d1\u5c55\uff0c\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\u7684\u5149\u7535\u8f6c\u6362\u6548\u7387\u5df2\u7ecf\u9ad8\u8fbe14%\u3002\u7136\u800c\uff0c\u57fa\u4e8e\u6b64\u7c7b\u4f53\u7cfb\u7684\u9ad8\u6548\u5bbd\u5e26\u9699\u805a\u5408\u7269\u7ed9\u4f53\u6750\u6599\u7684\u79cd\u7c7b\u975e\u5e38\u6709\u9650\u3001\u6d3b\u6027\u5c42\u5f62\u8c8c\u9700\u8981\u540e\u5904\u7406\u4f18\u5316\u3001\u5e76\u4e14\u5728\u4e00\u5b9a\u7a0b\u5ea6\u4e0a\u5bf9\u6d3b\u6027\u5c42\u7684\u819c\u539a\u548c\u5668\u4ef6\u7684\u9762\u79ef\u8f83\u4e3a\u654f\u611f\uff0c\u8fd9\u4e25\u91cd\u5236\u7ea6\u4e86\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\u7684\u8fdb\u4e00\u6b65\u53d1\u5c55\u548c\u5b9e\u9645\u5e94\u7528\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u6700\u8fd1\uff0c\u82cf\u5dde\u5927\u5b66<\/strong>\u5148\u8fdb\u5149\u7535\u6750\u6599\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u7684\u5f20\u8302\u6770<\/strong>\u6559\u6388\u7528\u4e00\u79cd\u4ee5\u6c1f\u53d6\u4ee3\u567b\u5429\u57fa\u82ef\u5e76\u4e8c\u567b\u5429\u4e3a\u7ed9\u4f53\u5355\u5143\u3001\u82ef\u5e76\u4e8c\u567b\u5429\u4e8c\u916e\u4e3a\u53d7\u4f53\u5355\u5143\u7684\u4e8c\u7ef4\u5171\u8f6d\u805a\u5408\u7269\u7ed9\u4f53\u6750\u6599PM6<\/strong>\u505a\u7ed9\u4f53\uff0c\u975e\u5bcc\u52d2\u70efIDIC\u505a\u53d7\u4f53\uff0c\u4e0d\u9700\u8981\u4efb\u4f55\u7279\u6b8a\u5904\u7406\u7684\u60c5\u51b5\u4e0b\u7b80\u5355\u65b9\u4fbf\u7684\u5236\u5907\u4e86\u5bf9\u6d3b\u6027\u5c42\u539a\u5ea6\u548c\u5668\u4ef6\u9762\u79ef\u4e0d\u654f\u611f\u7684\u9ad8\u6548\u975e\u5bcc\u52d2\u70ef\u592a\u9633\u80fd\u7535\u6c60\uff08\u80fd\u91cf\u8f6c\u5316\u6548\u738711.9%\uff09\uff0c\u76f8\u5173\u5de5\u4f5c\u53d1\u8868\u5728Advanced Materials\uff08IF = 19.791\uff09\u4e0a\u3002<\/p>\n

\u5f20\u8302\u6770\u6559\u6388\u5728\u524d\u671f\u5bf9\u5bcc\u52d2\u70ef\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\u7684\u7814\u7a76\u4e2d\u53d1\u73b0\uff0c\u5c06\u6c1f\u539f\u5b50\u5f15\u5165\u5230\u567b\u5429\u57fa\u53d6\u4ee3\u7684\u82ef\u5e76\u4e8c\u567b\u5429(BDT-T)\uff0c\u80fd\u591f\u540c\u65f6\u964d\u4f4e\u805a\u5408\u7269\u7684HOMO\u80fd\u7ea7\u3001\u63d0\u9ad8\u805a\u5408\u7269\u7684\u6d88\u5149\u7cfb\u6570\u3001\u589e\u5f3a\u5206\u5b50\u95f4\u7684\u76f8\u4e92\u4f5c\u7528\u3001\u63d0\u9ad8\u6750\u6599\u7684\u7ed3\u6676\u6027\u548c\u7a7a\u7a74\u8fc1\u79fb\u7387\uff0c\u4ece\u800c\u4f7f\u4e2d\u95f4\u5e26\u9699\u5171\u8f6d\u805a\u5408\u7269\u5149\u4f0f\u5668\u4ef6\u7684\u80fd\u91cf\u8f6c\u5316\u6548\u7387\u4ece4.5%\u63d0\u9ad8\u52308.6% (Advanced Materials, 2014, 26, 1118)1<\/sup>\u3002\u540e\u6765\uff0c\u5176\u53c8\u5c06\u5c06\u6c1f\u539f\u5b50\u5f15\u5165\u5230\u567b\u5429\u57fa\u53d6\u4ee3\u7684\u82ef\u5e76\u4e8c\u567b\u5429\u5f15\u5165\u5230\u5bbd\u5e26\u9699\u5171\u8f6d\u805a\u5408\u7269\u4f53\u7cfb\uff0c\u5f97\u5230\u65b0\u7684\u805a\u5408\u7269PM6<\/strong>\uff0c\u4f7f\u7528PM6<\/strong>\u4e3a\u7ed9\u4f53\u3001\u5bcc\u52d2\u70efPCBM\u4e3a\u53d7\u4f53\u5236\u5907\u7684\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\u7684\u6548\u7387\u4e3a9.2%\uff08V<\/em>oc<\/sub> = 0.98 V\uff09 \uff08Advanced Materials, 2015, 27, 4655\uff092<\/sup>\u3002\u540e\u6765\uff0c\u5728\u805a\u567b\u5429\u884d\u751f\u7269\u7535\u5b50\u4f9b\u4f53\u4e0a\u5f15\u5165\u6c1f\u539f\u5b50\uff0c\u5408\u6210\u65b0\u7684\u805a\u5408\u7269\u7ed9\u4f53\u6750\u6599PBDD-ff4T\uff0c\u8be5\u6750\u6599\u7684\u5bcc\u52d2\u70ef\u53d7\u4f53\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\u5728\u4e0d\u7ecf\u8fc7\u4efb\u4f55\u540e\u5904\u7406\u7684\u60c5\u51b5\u4e0b\uff0c\u53d6\u5f979.2%\u7684\u80fd\u91cf\u8f6c\u5316\u6548\u7387\u3002\u540c\u65f6\uff0c\u6c1f\u539f\u5b50\u7684\u5f15\u5165\u80fd\u591f\u663e\u8457\u6539\u5584\u5668\u4ef6\u5bf9\u6d3b\u6027\u5c42\u539a\u5ea6\u53d8\u5316\u7684\u654f\u611f\u6027\uff08Adv. Energy Mater., 2016, 6, 1600430\uff093<\/sup>\uff0c\u5f53\u6d3b\u6027\u5c42\u539a\u5ea6\u8fbe\u5230250 nm\u65f6\uff0c\u5149\u4f0f\u5668\u4ef6\u7684\u80fd\u91cf\u8f6c\u5316\u6548\u7387\u4ecd\u53ef\u7ef4\u6301\u5728\u6700\u4f73\u6548\u7387\u768480%\u3002<\/p>\n

\u8fd1\u671f\uff0c\u5229\u7528\u7ed9\u3001\u53d7\u4f53\u5438\u6536\u5149\u8c31\u4e92\u8865\u4f5c\u7528\uff0c\u8be5\u56e2\u961f\u4ee5PM6<\/strong>\u4e3a\u7ed9\u4f53\u3001\u4ee5\u7a84\u5e26\u9699\u7684ITIC\u4e3a\u53d7\u4f53\u5171\u6df7\u5236\u5907\u4e86\u975e\u5bcc\u52d2\u70ef\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\uff0c\u5728\u5f00\u8def\u7535\u538b\u9ad8\u8fbe1.04 V\u7684\u60c5\u51b5\u4e0b\u4f9d\u7136\u83b7\u5f97\u4e869.7%\u7684\u6548\u7387\u3002\u76f8\u5173\u5de5\u4f5c\u53d1\u8868\u5728Journal of Materials Chemistry A\uff082017, 5, 22180\uff094<\/sup>\uff0c\u4e14\u8be5\u8bba\u6587\u5165\u90092017\u5e74JMCA\u6742\u5fd7\u7684\u70ed\u70b9\u8bba\u6587\u3002\u4e3a\u4e86\u83b7\u5f97\u66f4\u9ad8\u7684\u5668\u4ef6\u6548\u7387\uff0c\u8be5\u7814\u7a76\u56e2\u961f\u4ee5PM6<\/strong>\u4e3a\u7ed9\u4f53\u3001\u4ee5\u7ed3\u6676\u6027\u66f4\u5f3a\u7684\u7a84\u5e26\u9699\u7684IDIC\u4e3a\u53d7\u4f53\u5171\u6df7\u5236\u5907\u4e86\u975e\u5bcc\u52d2\u70ef\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\u3002\u5728\u65e0\u4efb\u4f55\u540e\u5904\u7406\u7684\u60c5\u51b5\u4e0b\u83b7\u5f97\u4e86\u9ad8\u8fbe11.9%\u7684\u6548\u7387\uff08V<\/em>oc<\/sub> = 0.97 V\uff0cJ<\/em>sc<\/sub> = 17.8 mA cm-2<\/sup>\u548cFF = 69%\uff09\uff0c\u4f5c\u8005\u7533\u660e\u8fd9\u5728\u5f53\u65f6\u662f\u65e0\u4efb\u4f55\u540e\u5904\u7406\u5668\u4ef6\u7684\u6700\u9ad8\u6548\u7387\u503c\uff0c\u76f8\u5173\u5de5\u4f5c\u53d1\u8868\u5728Advanced Materials \uff082017, DOI: 10.1002\/adma.20170454627\uff095<\/sup>\u3002<\/p>\n

\u4e3a\u4e86\u7814\u7a76\u8be5\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\u7684\u5b9e\u9645\u5e94\u7528\u6f5c\u529b\uff0c\u4ed6\u4eec\u5236\u5907\u4e86\u4e0d\u540c\u6d3b\u6027\u5c42\u539a\u5ea6\u548c\u4e0d\u540c\u5668\u4ef6\u9762\u79ef\u7684\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\uff0c\u53d1\u73b0\u5728\u6d3b\u6027\u5c42\u819c\u539a\u8303\u56f4\u4e3a95-255 nm\u3001\u5668\u4ef6\u9762\u79ef\u4e3a0.20-0.81 cm2<\/sup>\u4e4b\u95f4\u65f6\u5747\u53ef\u4ee5\u83b7\u5f97\u8d85\u591a11%\u7684\u80fd\u91cf\u8f6c\u6362\u6548\u7387\u3002\u5f53\u5668\u4ef6\u9762\u79ef\u9ad8\u8fbe1.25 cm2<\/sup>\u65f6\uff0c\u521d\u6b65\u4f18\u5316\u7684\u67d4\u6027\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\u4f9d\u7136\u6536\u83b7\u4e866.54%\u7684\u80fd\u91cf\u8f6c\u6362\u6548\u7387\u3002\u57fa\u4e8ePM6<\/strong>:IDIC\u7684\u5171\u6df7\u819c\u62e5\u6709\u826f\u597d\u7684\u76f8\u5206\u79bb\u548c\u4e92\u7a7f\u7f51\u7edc\u7ed3\u6784\uff0c\u540c\u65f6\u5f3a\u7ed3\u6676\u6027\u7684PM6<\/strong>\u5728\u5171\u6df7\u819c\u4e2d\u62e5\u670916\u00b16 nm\u7684\u8f83\u957f\u6fc0\u5b50\u6269\u6563\u8ddd\u79bb\u3002\u4e0a\u8ff0\u7ed3\u679c\u8868\u660e\uff0c\u8be5\u6d3b\u6027\u5c42\u4f53\u7cfb\u9002\u7528\u4e8e\u9ad8\u6548\u67d4\u6027\u5927\u9762\u79ef\u5668\u4ef6\u7684\u7b80\u5355\uff08\u65e0\u540e\u5904\u7406\uff09\u5236\u5907\uff0c\u4e00\u5b9a\u7a0b\u5ea6\u4e0a\u63a8\u52a8\u4e86\u805a\u5408\u7269\u592a\u9633\u80fd\u7535\u6c60\u7684\u4ea7\u4e1a\u5316\u8fdb\u7a0b\u3002<\/p>\n

\u3010\u56fe\u6587\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u56fe1. \uff08a\uff09\u805a\u5408\u7269\u7ed9\u4f53\u548c\u5c0f\u5206\u5b50\u53d7\u4f53\u7684\u7ed3\u6784\u5f0f\uff0c\uff08b\uff09\u5438\u6536\u66f2\u7ebf\uff0c\uff08c\uff09\u80fd\u7ea7\u793a\u610f\u56fe\u3002<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe2.\uff08a\uff09\u4e0d\u540c\u6d3b\u6027\u5c42\u819c\u539a\u65f6\u7684\u7535\u6d41-\u7535\u538b\u66f2\u7ebf\uff1b\uff08b\uff09\u5916\u91cf\u5b50\u6548\u7387\u66f2\u7ebf\uff1b\uff08c\uff09\u5668\u4ef6\u6548\u7387\u4e0e\u6d3b\u6027\u5c42\u819c\u539a\u7684\u5173\u7cfb\uff1b\uff08d\uff09\u4e0d\u540c\u5668\u4ef6\u9762\u79ef\u65f6\u7684\u7535\u6d41-\u7535\u538b\u66f2\u7ebf\u3002<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe3. \u67d4\u6027\u5668\u4ef6\u7684\u7535\u6d41-\u7535\u538b\u66f2\u7ebf\u3002<\/strong><\/p>\n

\"\"<\/p>\n

\u88681. \u4e0d\u540c\u6d3b\u6027\u5c42\u539a\u5ea6\u548c\u4e0d\u540c\u5668\u4ef6\u9762\u79ef\u592a\u9633\u80fd\u7535\u6c60\u7684\u5149\u4f0f\u53c2\u6570\u8868\u3002<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe4. PM6:IDIC\u7684\u5171\u6df7\u819c\u5728\u4e0d\u540c\u5904\u7406\u6761\u4ef6\u4e0b\u7684GIWAXS\u548cReSOXS\u56fe\u3002<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe5. \uff08a\uff09PM6\u7684\u6fc0\u5b50\u6269\u6563\u793a\u610f\u56fe\uff1b\uff08b\uff09PM6\u7eaf\u819c\u548cPM6:ITIC\u5171\u6df7\u819c\u7684\u65f6\u95f4\u5206\u8fa8PL\u56fe\u3002<\/strong><\/p>\n

\"\"<\/p>\n

\u3010\u81f4\u8c22\u3011<\/p>\n

\u67d4\u6027\u5927\u9762\u79ef\u5668\u4ef6\u5f97\u5230\u56fd\u5bb6\u7eb3\u7c73\u79d1\u5b66\u4e2d\u5fc3\u9b4f\u5fd7\u7965\u7814\u7a76\u5458\u7684\u5e2e\u52a9\uff1bGIWAXS\u548cReSOXS\u6d4b\u8bd5\u5f97\u5230\u4e0a\u6d77\u4ea4\u901a\u5927\u5b66\u5218\u5cf0\u6559\u6388\u548c\u52b3\u4f26\u65af\u4f2f\u514b\u5229\u56fd\u5bb6\u5b9e\u9a8c\u5ba4Thomas P. Russell\u6559\u6388\u7684\u5e2e\u52a9\uff1b\u65f6\u95f4\u5206\u8fa8PL\u5149\u8c31\u6d4b\u8bd5\u5f97\u5230\u65b0\u52a0\u5761\u5357\u6d0b\u7406\u5de5\u5927\u5b66\u5434\u6ce2\u535a\u58eb\u548cTze Chien Sum\u6559\u6388\u7684\u5e2e\u52a9.\u611f\u8c22\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1(Nos. 51422306, 51503135, 51573120, and 91633301)\u548c\u6c5f\u82cf\u7701\u81ea\u7136\u79d1\u5b66\u57fa\u91d1(Grant No. BK20150332)\u7684\u8d44\u52a9\u548c\u652f\u6301\u3002<\/p>\n

\u3010\u53c2\u8003\u6587\u732e\u3011<\/strong><\/p>\n

1.\u00a0Synergistic Effect of Fluorination on Molecular Energy Level Modulation in Highly Efficient Photovoltaic Polymers<\/a>,\u00a0Adv. Mater.<\/strong>2014,<\/strong>\u00a0doi:\u00a010.1002\/adma.201304427<\/p>\n

2.\u00a0A Large-Bandgap Conjugated Polymer for Versatile Photovoltaic Applications with High Performance<\/a>,\u00a0Adv. Mater.<\/strong> 2015, 27, doi:\u00a010.1002\/adma.201502110<\/p>\n

3.\u00a0A New Polythiophene Derivative for` High Efficiency Polymer Solar Cells with PCE over 9 %<\/a>, Adv. Energy Mater.<\/strong>\u00a02016, doi:\u00a010.1002\/aenm.201600430<\/p>\n

4.\u00a0High-performance non-fullerene polymer solar cells based on a fluorinated wide bandgap copolymer with a high open-circuit voltage of 1.04 V<\/a>, J. Mater. Chem. A<\/strong>, 2017, doi:\u00a010.1039\/C7TA07785H<\/p>\n

5.\u00a0High-Performance As-Cast Non-fullerene Polymer Solar Cells with Thicker Active Layer and Large Area Exceeding11% Power Conversion Efficiency<\/a>, Adv. Mater.<\/strong> 2017, doi:10.1002\/adma.201704546<\/p>\n

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