{"id":118242,"date":"2017-12-23T06:30:57","date_gmt":"2017-12-22T22:30:57","guid":{"rendered":"\/\/m.iemloyee.com\/?p=118242"},"modified":"2017-12-22T14:00:09","modified_gmt":"2017-12-22T06:00:09","slug":"%e7%89%9b%e6%b4%a5energ-environ-sci-%ef%bc%9a3d%e5%8f%8c%e8%bf%9e%e7%bb%ad%e7%9b%b8%e6%9c%89%e5%ba%8f%e9%99%b6%e7%93%b7%e8%81%9a%e5%90%88%e7%89%a9%e5%be%ae%e9%80%9a%e9%81%93%e6%b7%b7%e5%90%88%e7%94%b5","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=118242","title":{"rendered":"\u725b\u6d25Energ.Environ.Sci.\uff1a3D\u53cc\u8fde\u7eed\u76f8\u6709\u5e8f\u9676\u74f7\u805a\u5408\u7269\u5fae\u901a\u9053\u6df7\u5408\u7535\u89e3\u8d28\u7528\u4e8e\u5168\u56fa\u6001\u7535\u6c60"},"content":{"rendered":"
\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n \u5c3d\u7ba1\u9502\u79bb\u5b50\u7535\u6c60\u5728\u5b9e\u9645\u5e94\u7528\u4e0a\u53d6\u5f97\u4e86\u4e00\u5b9a\u8fdb\u5c55\uff0c\u4f46\u662f\u5c31\u73b0\u5728\u7684\u53d1\u5c55\u72b6\u51b5\u800c\u8a00\uff0c\u5bf9\u672a\u6765\u5e02\u573a\u7684\u9700\u6c42\u4ecd\u96be\u4ee5\u6ee1\u8db3\u3002\u5176\u4e2d\u4e00\u4e2a\u91cd\u8981\u7684\u6311\u6218\u662f\uff0c\u7528\u56fa\u6001\u7535\u89e3\u8d28\u4ee3\u66ff\u6db2\u6001\u7535\u89e3\u6db2\u3002\u6362\u8a00\u4e4b\uff0c\u5168\u56fa\u6001\u7535\u6c60\u662f\u672a\u6765\u7535\u6c60\u7684\u91cd\u8981\u53d1\u5c55\u65b9\u5411\uff0c\u4f46\u662f\u5176\u4e2d\u6700\u5927\u7684\u4e00\u4e2a\u969c\u788d\u662f\uff0c\u83b7\u5f97\u9ad8\u5bfc\u7535\u6027\u7684\u540c\u65f6\u4e5f\u8981\u6709\u5408\u9002\u7684\u529b\u5b66\u7279\u6027\u3002<\/p>\n \u5728\u4f17\u591a\u7684\u56fa\u6001\u7535\u89e3\u8d28\u5f53\u4e2d\uff0c\u9676\u74f7\u7535\u89e3\u8d28\u548c\u805a\u5408\u7269\u7535\u89e3\u8d28\u4f7f\u7528\u8f83\u4e3a\u5e7f\u6cdb\u3002\u805a\u5408\u7269\u7535\u89e3\u8d28\u4f7f\u5f97\u5176\u5728\u5faa\u73af\u8fc7\u7a0b\u4e2d\u4e0e\u7535\u6781\u63a5\u89e6\u65f6\u80fd\u7f13\u89e3\u4f53\u79ef\u81a8\u80c0\u548c\u538b\u529b\u6539\u53d8\uff0c\u4ece\u800c\u4e0d\u5bb9\u6613\u635f\u574f\u3002\u4f46\u662f\u805a\u5408\u7269\u7684\u5bfc\u7535\u6027\u592a\u5dee\uff08<10-4<\/sup>S cm-1<\/sup>\uff09\uff0c\u800c\u4e14\u5bb9\u6613\u751f\u957f\u9502\u679d\u6676\u3002\u9676\u74f7\u7535\u89e3\u8d28\u62e5\u6709\u6bd4\u62df\u6db2\u4f53\u7535\u89e3\u8d28\u7684\u5bfc\u7535\u6027\uff0c\u4f46\u662f\u5176\u529b\u5b66\u6027\u80fd\u592a\u5dee\uff0c\u4f7f\u5f97\u4e0e\u7535\u6781\u7684\u63a5\u89e6\u65f6\u5bb9\u6613\u788e\u88c2\u3002\u603b\u4e4b\uff0c\u76ee\u524d\u4e3a\u6b62\u7684\u56fa\u6001\u7535\u89e3\u8d28\u90fd\u6709\u4e0d\u5c11\u660e\u663e\u7684\u4f18\u7f3a\u70b9\u3002<\/p>\n \u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n \u8fd1\u65e5\uff0c\u6765\u81ea\u725b\u6d25\u5927\u5b66\u7684<\/strong>Peter G. Bruce<\/strong>\u6559\u6388\u8bfe\u9898\u7ec4<\/strong>\u8054\u5408\u7231\u4e01\u5821\u5927\u5b66<\/strong>\u5728\u8457\u540d\u671fEnergy & Environmental Science<\/strong>\u4e0a\u53d1\u8868\u9898\u4e3a\u201dHybrid electrolytes with 3D bicontinuous ordered ceramic and polymer microchannels for all-solidstate batteries<\/strong>\u201d\u7684\u6587\u7ae0\u3002\u8be5\u6587\u7ae0\u63d0\u51fa\u4e86\u4e00\u79cd\u65b9\u6cd5\uff0c\u7ed3\u5408\u4e86\u9676\u74f7\u56fa\u6001\u7535\u89e3\u8d28LAGP\uff08Li1.4<\/sub>Al0.4<\/sub>Ge1.6<\/sub>(PO4<\/sub>)3<\/sub>\uff09\u548c\u7edd\u7f18\u805a\u5408\u7269\uff0c\u5408\u6210\u4e86\u4e00\u79cd3D\u53cc\u8fde\u7eed\u76f8\u7ed3\u6784\u6df7\u5408\u7535\u89e3\u8d28\u7528\u4e8e\u5168\u56fa\u6001\u7535\u6c60\u3002\u901a\u8fc7EIS\u3001CV\u7b49\u7535\u5316\u5b66\u6d4b\u8bd5\u548c\u529b\u5b66\u6d4b\u8bd5\u7814\u7a76\u4e86\u5176\u4e2d\u7684\u7279\u6027\u3002\u5176\u6027\u80fd\u53d6\u51b3\u4e8e\u5fae\u7ed3\u6784\uff08\u7acb\u65b9\u3001\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u3001\u91d1\u521a\u77f3\u3001bijel\u578b\u7b49\uff09\u548c\u805a\u5408\u7269\u7684\u7c7b\u578b\uff08\u73af\u6c27\u805a\u5408\u7269\u3001\u805a\u4e19\u70ef\u7b49\uff09\u3002\u6d4b\u8bd5\u7684\u7ed3\u679c\u8868\u660e\u4e8c\u5341\u56db\u9762\u4f53\u578bLAGP-\u73af\u6c27\u7535\u89e3\u8d28\u79bb\u5b50\u7535\u5bfc\u7387\u4e0e\u5176\u4ed6LAGP\u7684\u6570\u91cf\u7ea7\u76f8\u540c(\u4e3a1.6×10-4<\/sup>S cm-1<\/sup>)\uff0c\u4f46\u662f\u5176\u529b\u5b66\u6027\u80fd\u4f18\u8d8a\uff0c\u8fd9\u79cd\u7535\u89e3\u8d28\u7684\u5f2f\u66f2\u7834\u574f\u5e94\u53d8\u662fLAGP\u7834\u88c2\u524d\u76845\u500d\u3002<\/p>\n \u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n \u56fe\u4e00\uff1a\u7acb\u65b9\u4f53\u5fae\u7ed3\u6784\u6df7\u5408\u7535\u89e3\u8d28\u7684\u6a21\u677f\u6784\u9020\u8fc7\u7a0b\u3002<\/strong><\/p>\n \u56fe\u4e8c\uff1a<\/strong> 3D<\/strong>\u6253\u5370\u6a21\u677f\u7684<\/strong>SEM<\/strong>\u56fe\u548c<\/strong>X<\/strong>\u5149\u5fae<\/strong>CT<\/strong>\u626b\u63cf\u7684\u7acb\u65b9\u4f53\u7684\u4e09\u7ef4\u6548\u679c\u56fe\u3002<\/strong><\/p>\n \u7acb\u65b9\u4f53\u3001\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u3001\u91d1\u521a\u77f3\u3001bijel\u578b\u7684\u5fae\u7ed3\u6784\uff08\u4ece\u5de6\u5f80\u53f3\uff09\u3002<\/p>\n \u56fe\u4e09\uff1a<\/strong>LAGP<\/strong>\u6846\u67b6\u7684<\/strong>SEM<\/strong>\u56fe\u548c<\/strong>X<\/strong>\u5149\u5fae<\/strong>CT<\/strong>\u626b\u63cf\u4e09\u7ef4\u6548\u679c\u56fe\u3002<\/strong><\/p>\n \u7acb\u65b9\u4f53\u3001\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u3001\u91d1\u521a\u77f3\u3001bijel\u578b\u7684\u5fae\u7ed3\u6784\uff08\u4ece\u5de6\u5f80\u53f3\uff09\u3002<\/p>\n \u56fe\u56db\uff1a<\/strong> LAGP<\/strong>\u73af\u6c27\u7535\u89e3\u8d28\u7684\u7acb\u65b9\u4f53\u3001\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u3001\u91d1\u521a\u77f3\u3001<\/strong>bijel<\/strong>\u578b\u7684\u5fae\u7ed3\u6784\u7684\u7acb\u4f53\u5e73\u7248\u5370\u5237\u3002<\/strong><\/p>\n \u7acb\u65b9\u4f53\u3001\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u3001\u91d1\u521a\u77f3\u3001bijel\u578b\u7684\u5fae\u7ed3\u6784\uff08\u4ece\u5de6\u5f80\u53f3\uff09\u3002<\/p>\n \u56fe\u4e94\uff1a\u7acb\u65b9\u4f53\u3001\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u3001\u91d1\u521a\u77f3\u3001<\/strong>bijel<\/strong>\u578b\u5fae\u7ed3\u6784\u7684<\/strong>LAGP-PP<\/strong>\u7535\u89e3\u8d28\u7684<\/strong>SEM<\/strong>\u56fe\u548c<\/strong>EDX<\/strong>\u56fe\u3002<\/strong><\/p>\n \u56fe\u516d\uff1a\u4f7f\u7528\u5bf9\u79f0\u91d1\u7535\u6781\u7684\u7535\u89e3\u8d28\u7535\u5316\u5b66\u963b\u6297\u8c31\u5206\u6790\u3002<\/strong><\/p>\n a) \u7ed3\u6784\u793a\u610f\u56fe\uff1b<\/p>\n b) \u5e38\u6e29c)-30\u6444\u6c0f\u5ea6\u7684EIS\u56fe\uff1b<\/p>\n d) -20\u6444\u6c0f\u5ea6\u81f375\u6444\u6c0f\u5ea6\u7684\u963f\u4f26\u7ebd\u65af\u56fe\u3002<\/p>\n \u56fe\u4e03\uff1a\u4f7f\u7528\u5bf9\u79f0\u9502\u7535\u6781\u7684\u7535\u89e3\u8d28\u7535\u5316\u5b66\u963b\u6297\u8c31\u5206\u6790\u3002<\/strong><\/p>\n b)\u5404\u4e34\u8fd1\u6e29\u5ea6\u5bf9\u5e94\u7684\u80fd\u594e\u65af\u7279\u56fe\u3002<\/p>\n \u56fe\u516b\uff1a\u4f7f\u7528\u9502\u7535\u6781\u7684<\/strong>LAGP<\/strong>\u548c\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u73af\u6c27<\/strong>LAGP<\/strong>\u7535\u89e3\u8d28\u7684\u6052\u6d41\u5faa\u73af\u3002<\/strong><\/p>\n 0.7mA cm-2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5faa\u73af0.5h\u7684a) LAGP\u548cb)\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u73af\u6c27LAGP\u7535\u89e3\u8d28\u6052\u6d41\u5faa\u73af\u56fe\uff1b<\/p>\n 1mA cm-2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5faa\u73af0.5h\u7684c) LAGP\u548cd)\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u73af\u6c27LAGP\u7535\u89e3\u8d28\u6052\u6d41\u5faa\u73af\u56fe\uff1b<\/p>\n \u56fe\u4e5d\uff1a<\/strong>LAGP<\/strong>\u548c\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u73af\u6c27<\/strong>LAGP<\/strong>\u7535\u89e3\u8d28\u5728\u5bf9\u79f0\u9502\u7535\u6781\u4e0b\u5faa\u73af\u6b21\u6570\u548c\u7ec8\u6b62\u7535\u538b\u7684\u5173\u7cfb\u3002<\/strong><\/p>\n \u7535\u6d41\u5bc6\u5ea6\u5206\u522b\u4e3aa) 0.7mA cm-2<\/sup>\uff0cb)1mA cm-2<\/sup>\u548cc)\u5728\u8fbe\u5230\u4eea\u5668\u9650\u5b9a\u7535\u538b\u540e1mA cm-2<\/sup>\u3002<\/p>\n \u56fe\u5341\uff1a\u4e0d\u540c\u7535\u89e3\u8d28\u5728\u5faa\u73af\u540e\u7684\u56fe\u50cf\u5bf9\u6bd4\u548c<\/strong>SEM<\/strong>\u56fe\u5bf9\u6bd4\u3002<\/strong><\/p>\n 0.7mA cm-2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5faa\u73af30\u6b21\u548c40\u6b21\u7684a)LAGP\u548cb)\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u73af\u6c27LAGP\u7535\u89e3\u8d28\uff1b<\/p>\n 1mA cm-2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5faa\u73af20\u6b21\u7684a)LAGP\u548cb)\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u73af\u6c27LAGP\u7535\u89e3\u8d28\uff1b<\/p>\n \u56fe\u5341\u4e00\uff1a\u963b\u6297\u4e0e\u5faa\u73af\u6b21\u6570\u7684\u5173\u7cfb\u3002<\/strong><\/p>\n a)LAGP\u548cb)\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u73af\u6c27LAGP\u5728 0.7mA cm-2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5faa\u73af30\u548c50\u6b21\uff1b<\/p>\n c)LAGP\u548cd)\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u73af\u6c27LAGP\u5728 1mA cm-2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5faa\u73af20\u6b21\u3002<\/p>\n \u56fe\u5341\u4e8c\uff1a\u5e94\u529b\u5e94\u53d8\u66f2\u7ebf\u3002<\/strong><\/p>\n a)\u73af\u6c27\u805a\u5408\u7269\u548c \u00a0b)\u7acb\u65b9\u4f53\u3001\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u3001\u91d1\u521a\u77f3\u3001bijel\u578b\u5fae\u7ed3\u6784\u7684\u805a\u4e19\u70ef\u3002<\/p>\n \u56fe\u5341\u4e09\uff1a\u56db\u70b9\u5f2f\u66f2\u7684\u5e94\u529b\u5e94\u53d8\u66f2\u7ebf\u3002<\/strong><\/p>\n \u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n \u5408\u6210\u4e863D\u53cc\u8fde\u7eed\u76f8\u6709\u5e8f\u5fae\u901a\u9053\u9676\u74f7\u7535\u89e3\u8d28LAGP\u548c\u975e\u5bfc\u7535\u805a\u5408\u7269\uff08\u73af\u6c27\u805a\u5408\u7269\uff0c\u805a\u4e19\u70ef\u7b49\uff09\u3002\u901a\u8fc73D\u6253\u5370\u6a21\u677f\uff0c\u5f97\u5230\u4e86\u7acb\u65b9\u5f62\u3001\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u3001\u91d1\u521a\u77f3\u3001bijel\u578b\u5fae\u7ed3\u6784\u6df7\u5408\u7535\u89e3\u8d28\u3002\u5176\u4e2d\u6027\u80fd\u6700\u597d\u7684\u662f\u73af\u6c27\u805a\u5408\u7269\u578b\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u7ed3\u6784\uff0c\u5176\u79bb\u5b50\u7535\u5bfc\u7387\u5728\u5e38\u6e29\u4e0b\u4e3a1.6×10-4<\/sup>S cm-1<\/sup>\u3002\u529b\u5b66\u6027\u80fd\u6d4b\u8bd5\u8868\u660e\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u6df7\u5408\u7535\u89e3\u8d28\u6bd4\u9676\u74f7\u4f53\u66f4\u575a\u97e7\u3002\u8be5\u7ed3\u679c\u76f8\u5f53\u4e8e28%\u7684\u538b\u7f29\u7834\u574f\u5e94\u53d8\u548c5\u500d\u4e8eLAGP\u65ad\u88c2\u524d\u7684\u5f2f\u66f2\u7834\u574f\u5e94\u53d8\u3002\u66f4\u91cd\u8981\u7684\u662f\uff0c\u5faa\u73af\u7ed3\u679c\u8868\u660e\uff0c\u4e0e\u9676\u74f7\u4f53\u76f8\u6bd4\u87ba\u65cb\u4e8c\u5341\u56db\u9762\u4f53\u73af\u6c27LAGP\u7535\u89e3\u8d28\u63d0\u5347\u4e86\u5bf9\u79f0\u9502\u7535\u6c60\u7684\u6027\u80fd\uff0c\u5c24\u5176\u662f\u4f4e\u7535\u6d41\u5bc6\u5ea6\u4e0b\u3002<\/p>\n \u6587\u732e\u94fe\u63a5:<\/strong> Hybrid electrolytes with 3D bicontinuous ordered ceramic and polymer microchannels for all-solid-state batteries <\/a>(Energy Environ. Sci., 2017, DOI: 10.1039\/c7ee02723k)<\/p>\n \u672c\u6587\u7531\u6750\u6599\u4eba\u65b0\u80fd\u6e90\u7ec4Jespen\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u6574\u7406\u7f16\u8f91\u3002<\/p>\n \u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u8fd9\u91cc\u6c47\u96c6\u4e86\u5404\u5927\u9ad8\u6821\u7855\u535a\u751f\u3001\u4e00\u7ebf\u79d1\u7814\u4eba\u5458\u4ee5\u53ca\u884c\u4e1a\u4ece\u4e1a\u8005\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u7f16\u8f91\u90e8\u5927\u5bb6\u5ead<\/a>\u3002<\/p>\n \u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n \u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1a<\/strong>RDD-2011-CHERISH<\/strong>\uff0c\u4efb\u4e39\u4e39\uff0c\u6211\u4eec\u4f1a\u9080\u8bf7\u5404\u4f4d\u8001\u5e08\u52a0\u5165\u4e13\u5bb6\u7fa4\u3002<\/strong><\/p>\n<\/p>\n
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a) \u7ed3\u6784\u793a\u610f\u56fe\uff1b<\/p>\n
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