{"id":111756,"date":"2017-11-17T06:30:21","date_gmt":"2017-11-16T22:30:21","guid":{"rendered":"\/\/m.iemloyee.com\/?p=111756"},"modified":"2017-11-14T19:55:24","modified_gmt":"2017-11-14T11:55:24","slug":"%e6%b2%b3%e5%8d%97%e5%b8%88%e8%8c%83%e5%a4%a7%e5%ad%a6nano-energy%ef%bc%9a%e6%91%a9%e6%93%a6%e7%ba%b3%e7%b1%b3%e5%8f%91%e7%94%b5%e6%9c%ba%e5%8a%a9%e5%8a%9b%e7%94%9f%e7%89%a9%e8%b4%a8%e8%a1%8d%e7%94%9f","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=111756","title":{"rendered":"\u6cb3\u5357\u5e08\u8303\u5927\u5b66Nano Energy\uff1a\u6469\u64e6\u7eb3\u7c73\u53d1\u7535\u673a\u52a9\u529b\u751f\u7269\u8d28\u884d\u751f\u78b3\u6750\u6599\u4f5c\u9634\u6781\u50ac\u5316\u5242\u7684\u81ea\u9a71\u52a8\u7535\u82ac\u987f\u964d\u89e3\u7cfb\u7edf"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

Fenton\u6cd5\u4f5c\u4e3a\u9ad8\u7ea7\u6c27\u5316\u6280\u672f\u7684\u4e00\u79cd\uff0c\u5229\u7528Fe2+<\/sup>\u548cH2<\/sub>O2<\/sub>\u53cd\u5e94\u751f\u6210\u5f3a\u6c27\u5316\u6027\u7684\u2022OH\uff0c\u53ef\u4ee5\u6c27\u5316\u964d\u89e3\u591a\u79cd\u6709\u673a\u6c61\u67d3\u7269\u3002\u53d7\u9ad8\u6602\u7684H2<\/sub>O2<\/sub>\u5b58\u50a8\u548c\u8fd0\u8f93\u6210\u672c\u3001H2<\/sub>O2<\/sub>\u5373\u65f6\u5206\u89e3\u9020\u6210\u6c61\u67d3\u7269\u964d\u89e3\u6548\u7387\u4f4e\u4ee5\u53ca\u53cd\u5e94\u8fc7\u7a0b\u4e2d\u4ea7\u751f\u4e0d\u53ef\u518d\u751f\u7684\u94c1\u6ce5\u7b49\u7f3a\u70b9\u9650\u5236\uff0cFenton\u6cd5\u5f88\u96be\u8fdb\u884c\u5e7f\u6cdb\u63a8\u5e7f\u3002\u968f\u7740electro-Fenton\uff08EF\uff09\u6cd5\u7684\u51fa\u73b0\uff0c\u5b9e\u73b0\u4e86H2<\/sub>O2<\/sub>\u7684\u201c\u81ea\u6211\u4f9b\u7ed9\u201d\u548cFe2+<\/sup>\u7684\u5faa\u73af\u4f7f\u7528\uff0c\u6210\u529f\u514b\u670d\u4e86Fenton\u6cd5\u5b58\u5728\u7684\u4e0d\u8db3\u3002\u4f46\u4f20\u7edf\u7684EF\u8fc7\u7a0b\u9700\u8981\u5916\u90e8\u80fd\u6e90\u4f9b\u80fd\u53cd\u5e94\u6240\u9700\u7684\u7535\u80fd\uff0c\u8fd9\u65e0\u7591\u52a0\u91cd\u4e86\u73af\u5883\u8d1f\u62c5\uff0c\u9650\u5236\u4e86\u5176\u5728\u6709\u673a\u6c61\u67d3\u7269\u5904\u7406\u4e2d\u7684\u5e94\u7528\u3002\u6469\u64e6\u7eb3\u7c73\u53d1\u7535\u673a\uff08TENG\uff09\u53ef\u4ee5\u5c06\u5468\u56f4\u73af\u5883\u4e2d\u5e7f\u6cdb\u5b58\u5728\u7684\u673a\u68b0\u80fd\u8f6c\u5316\u4e3a\u7535\u80fd\uff0c\u4f7f\u5176\u53ef\u4ee5\u4f5c\u4e3a\u4f9b\u80fd\u88c5\u7f6e\u4e3aEF\u4f53\u7cfb\u6e90\u6e90\u4e0d\u65ad\u4f9b\u5e94\u7535\u80fd\u3002\u540c\u65f6\uff0c\u4f5c\u4e3a\u5f71\u54cd\u6709\u673a\u6c61\u67d3\u7269\u964d\u89e3\u6548\u7387\u7684\u5173\u952e\u56e0\u7d20\uff0c\u4e3aEF\u4f53\u7cfb\u5bfb\u627e\u5ec9\u4ef7\u3001\u9ad8\u6548\u7684\u50ac\u5316\u5242\u4e5f\u81f3\u5173\u91cd\u8981\u3002\u4e3a\u6b64\uff0c\u7814\u7a76\u4eba\u5458\u4ee5\u6728\u5170\u82b1\u4e3a\u524d\u9a71\u4f53\uff0c\u5408\u6210\u51fa\u4e00\u79cd\u78b3\u57fa\u50ac\u5316\u6750\u6599\u4f5c\u4e3aEF\u4f53\u7cfb\u7684\u9634\u6781\u50ac\u5316\u6750\u6599\uff0c\u5e76\u4e14\u8bbe\u8ba1\u591a\u5c42\u67d4\u6027\u8010\u78e8TENG\uff08RFM-TENG\uff09\uff0c\u6210\u529f\u5b9e\u73b0\u4e86\u78b1\u6027\u6a592\uff08BO2\uff09\u7684\u964d\u89e3\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6cb3\u5357\u5e08\u8303\u5927\u5b66\u5316\u5b66\u5316\u5de5\u5b66\u9662\u9ad8\u4e66\u71d5\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7814\u7a76\u56e2\u961f\u5229\u7528\u751f\u7269\u8d28\u57fa\u78b3\u6750\u6599\u505a\u9634\u6781\uff0c\u501f\u52a9\u5176\u6700\u65b0\u8bbe\u8ba1\u7684TENG\u63d0\u4f9b\u7535\u80fd\u4f9b\uff0c\u7ec4\u6210\u81ea\u9a71\u52a8EF\u4f53\u7cfb\uff0c\u9996\u6b21\u5b9e\u73b0\u4e86\u81ea\u9a71\u52a8EF\u4f53\u7cfb\u5728\u6709\u673a\u6c61\u67d3\u7269\u5904\u7406\u4e2d\u7684\u5e94\u7528\u3002RFM-TENG\u7684\u77ed\u8def\u7535\u6d41\u3001\u8f6c\u79fb\u7535\u8377\u91cf\u548c\u5f00\u8def\u7535\u538b\u5206\u522b\u53ef\u4ee5\u8fbe\u5230960 \u03bcA\uff0c2.8 \u03bcC\u548c1050 V\u3002\u5728RFM-TENG\u7684\u9a71\u52a8\u4e0b\uff0c\u96be\u964d\u89e3\u7684\u6709\u673a\u6c61\u67d3\u7269\u2014\u2014BO2\u88abEF\u8fc7\u7a0b\u4ea7\u751f\u7684\u2022OH\u964d\u89e3\u4e3aCO2<\/sub>\u3002\u8be5\u7814\u7a76\u6210\u679c\u4ee5\u201cAn Innovative Electro-Fenton Degradation System Self-Powered by Triboelectric Nanogenerator Using Biomass-Derived Carbon Materials as Cathode Catalyst<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Nano Energy<\/strong>\u4e0a\u3002\uff08\u672c\u6587\u7b2c\u4e00\u4f5c\u8005\u662f\u9648\u91ce\uff0c\u5728\u8bfb\u535a\u58eb\uff0c\u5bfc\u5e08\u9ad8\u4e66\u71d5\u6559\u6388<\/strong>\uff09<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe<\/strong>1. <\/strong>RFM-TENG<\/strong>\u7684\u7ed3\u6784\u793a\u610f\u56fe\u548c\u53d1\u7535\u673a\u7406<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09RFM-TENG\u7684\u7ec4\u88c5\u8fc7\u7a0b\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09RFM-TENG\u5728\u4e00\u4e2a\u5de5\u4f5c\u5468\u671f\u5185\u7684\u4ea7\u7535\u673a\u7406\uff1b<\/p>\n

\uff08c\uff09COMSOL\u5bf9\u53d1\u7535\u673a\u7535\u52bf\u5206\u5e03\u7684\u6a21\u62df\u3002<\/p>\n

\u56fe<\/strong>2. RFM-TENG<\/strong>\u5728<\/strong>3 Hz<\/strong>\u9891\u7387\u4e0b\u5de5\u4f5c\u7684\u8f93\u51fa\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u00a0 \u6709\u4e0d\u540c\u6469\u64e6\u5c42\u6570\u91cfTENG\u7684\u77ed\u8def\u7535\u6d41\uff1b<\/p>\n

\uff08b\uff09\u00a0 \u6709\u4e0d\u540c\u6469\u64e6\u5c42\u6570\u91cfTENG\u7684\u8f6c\u79fb\u7535\u8377\u91cf\uff1b<\/p>\n

\uff08c\uff09\u00a0 \u6709\u4e0d\u540c\u6469\u64e6\u5c42\u6570\u91cfTENG\u7684\u5f00\u8def\u7535\u538b\uff0c\u63d2\u56fe\u662f\u542b6\u4e2a\u6469\u64e6\u5c42TENG\u7684\u5f00\u8def\u7535\u538b\uff1b<\/p>\n

\uff08d\uff09\u00a0 \u542b6\u4e2a\u6469\u64e6\u5c42TENG\u7684\u8f93\u51fa\u7535\u6d41\u548c\u529f\u7387\u5bc6\u5ea6\u968f\u8d1f\u8f7d\u7535\u963b\u53d8\u5316\uff0c\u63d2\u56fe\u662f\u7ecf30000\u4e2a\u5faa\u73af\u540e\u7684\u6700\u5927\u77ed\u8def\u7535\u6d41\u3002<\/p>\n

\u56fe<\/strong>3. MF-800-4<\/strong>\u7684\u5404\u9879\u53c2\u6570\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u00a0 MF-800-4\u7684FESEM\u56fe\uff1b<\/p>\n

\uff08b\uff09\u00a0 MF-800-4\u7684TEM\u56fe\uff0c\u63d2\u56fe\u662fHR-TEM\uff1b<\/p>\n

\uff08c\uff09\u00a0 MF-800-4\u7684XRD\u56fe\uff0c\u63d2\u56fe\u662f\u62c9\u66fc\u5149\u8c31\uff1b<\/p>\n

\uff08d\uff09\u00a0 MF-800-4\u7684N2<\/sub>\u5438\u9644\/\u8131\u9644\u7b49\u6e29\u7ebf\uff1b<\/p>\n

\uff08e\uff09\u00a0 MF-800-4\u7684FT-IR\u56fe\uff1b<\/p>\n

\uff08f\uff09 MF-800-4\u7684XPS\u5168\u626b\u63cf\u8c31\uff0c\u63d2\u56fe\u662f\u63a5\u89e6\u89d2\uff1b<\/p>\n

\uff08g,h,i\uff09MF-800-4\u7684\u9ad8\u5206\u8fa8XPS\u8c31C 1s\uff0cO 1s\u548cN 1s\u3002<\/p>\n

\u56fe<\/strong>4. RFM-TENG<\/strong>\u5728\u7535\u5316\u5b66\u65b9\u9762\u7684\u5e94\u7528<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u00a0 RFM-TENG\u9a71\u52a8BO2\u964d\u89e3\u793a\u610f\u56fe\uff1b<\/p>\n

\uff08b\uff09\u00a0 \u5728N2<\/sub>\u6216O2<\/sub>\u9971\u548c\u7684\u6d53\u5ea6\u4e3a0.05 mol\/L \uff0cpH=2.0\u7684Na2<\/sub>SO4<\/sub>\u6c34\u6eb6\u6db2\u4e2d\uff0cMF-800-4\u7684CV\u66f2\u7ebf\uff1b<\/p>\n

\uff08c\uff09\u00a0 \u5728\u5355\u5ba4\u4f53\u7cfb\u4e2d\uff0c\u65bd\u52a0\u22120.8 V\u7684\u7535\u4f4d\uff0cMF-800-4\u9634\u6781\u4f4d\u7f6eH2<\/sub>O2<\/sub>\u7684\u6d53\u5ea6\uff1b<\/p>\n

\uff08d\uff09\u00a0 MF-800-4\u7684EIS\u8c31\uff0c\u63d2\u56fe\u662f\u7b49\u6548\u7535\u8def\u56fe\uff1b<\/p>\n

\uff08e\uff09\u00a0 \u5728RFM-TENG\u7684\u9a71\u52a8\u4e0b\uff0cBO2\u964d\u89e3\u8fc7\u7a0b\u7684UV-vis\uff1b<\/p>\n

\uff08f\uff09\u00a0 \u57280.05 mol \/L\uff0cpH=2.0\u7684Na2<\/sub>SO4<\/sub>\u6c34\u6eb6\u6db2\u4e2d\uff0cBO2\u964d\u89e3\u8fc7\u7a0b\u4e2d\u95f4\u4ea7\u7269\u7684GC-MS\u8c31\uff0c\uff081\uff092,4-\u4e8c\u7f9f\u57fa\u5076\u6c2e\u82ef\uff0c\uff082\uff09\u82ef\u80fa\uff0c\uff083\uff09\u82ef\u915a\uff0c\uff084\uff094-\u6c28\u57fa\u82ef\u915a\uff085\uff09\u5bf9\u82ef\u4e8c\u915a\uff086\uff091,4-\u82ef\u918c\uff087\uff091,2,4-\u82ef\u4e09\u915a\u3002<\/p>\n

\u00a0\u56fe5. \u964d\u89e3\u673a\u7406\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/strong><\/p>\n

\u00a0\u00a0\u00a0\u00a0\u00a0 MF-800-4\u4f5c\u4e3a\u9634\u6781\u50ac\u5316\u6750\u6599\uff0cRFM-TENG\u9a71\u52a8\u964d\u89e3BO2\u673a\u7406\u793a\u610f\u56fe<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u7814\u7a76\u4eba\u5458\u4ee5\u6728\u5170\u82b1\u4e3a\u524d\u9a71\u4f53\uff0c\u5408\u6210\u4e00\u79cd\u78b3\u57fa\u50ac\u5316\u5242\u4f5c\u4e3aEF\u4f53\u7cfb\u7684\u9634\u6781\u6750\u6599\uff0c\u8bbe\u8ba1\u4e86\u4e00\u79cd\u4ee5\u6d77\u7ef5\u4f5c\u4e3a\u7f13\u51b2\u5c42\u7684RFM-TENG\uff0c\u5e76\u7ed3\u5408EF\u8fc7\u7a0b\u5b9e\u73b0\u4e86BO2\u7684\u81ea\u9a71\u52a8\u964d\u89e3\u3002\u8be5\u7814\u7a76\u5de5\u4f5c\u4e0d\u4ec5\u6709\u5229\u4e8e\u673a\u68b0\u80fd\u8f6c\u5316\u4e3a\u7a33\u5b9a\u7684\u7535\u80fd\uff0c\u800c\u4e14\u5c06\u751f\u7269\u8d28\u57fa\u78b3\u6750\u6599\u6210\u529f\u8fd0\u7528\u4e8e\u81ea\u9a71\u52a8EF\u4f53\u7cfb\u964d\u89e3\u6709\u673a\u6c61\u67d3\u7269\uff0c\u5bf9\u4e8e\u6709\u673a\u6c61\u67d3\u7269\u7684\u5904\u7406\u6709\u91cd\u8981\u7684\u53c2\u8003\u4ef7\u503c\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong> An Innovative Electro-Fenton Degradation System Self-Powered by Triboelectric Nanogenerator Using Biomass-Derived Carbon Materials as Cathode Catalyst<\/a>\uff08Nano Energy, 2017, DOI: 10.1016\/j.nanoen.2017.10.060\uff09<\/p>\n

\uff08<\/strong>1<\/strong>\uff09\u56e2\u961f\u4ecb\u7ecd<\/strong><\/p>\n

\u672c\u56e2\u961f\u56f4\u7ed5\u4e0e\u751f\u7269\u3001\u80fd\u6e90\u3001\u8d44\u6e90\u548c\u73af\u5883\u76f8\u5173\u7684\u6750\u6599\u5316\u5b66\u65b0\u4f53\u7cfb\uff0c\u5728\u5b66\u79d1\u4ea4\u53c9\u878d\u5408\u7684\u57fa\u7840\u4e0a\uff0c\u5bf9\u529f\u80fd\u5316\u7684\u78b3\u57fa\u6750\u6599\u4f5c\u4e3a\u50ac\u5316\u5242\u6216\u7535\u6781\u6750\u6599\u7684\u6f5c\u5728\u5e94\u7528\u4ef7\u503c\u3001\u83b7\u53d6\u80fd\u6e90\u7684\u65b0\u578b\u65b9\u5f0f\u8fdb\u884c\u4e86\u7cfb\u7edf\u3001\u6df1\u5165\u7684\u7814\u7a76\u3002\u4e3b\u8981\u7814\u7a76\u65b9\u5411\uff1a<\/p>\n

1\u3001\u63ba\u6742\u78b3\u6750\u6599\u7684\u6784\u5efa\u53ca\u5176\u5728ORR\u4e2d\u7684\u5e94\u7528\uff1b<\/p>\n

2\u3001\u4e92\u7a7f\u7ed3\u6784\u78b3\u6750\u6599\u7684\u7ed3\u6784\u8bbe\u8ba1\u53ca\u5728\u8d85\u7ea7\u7535\u5bb9\u5668\u4e2d\u7684\u5e94\u7528\uff1b<\/p>\n

3\u3001\u78b3\u6750\u6599\u5728\u6469\u64e6\u7eb3\u7c73\u53d1\u7535\u673a\u81ea\u9a71\u52a8\u964d\u89e3\u4f53\u7cfb\u4e2d\u7684\u5e94\u7528\u3002<\/p>\n

\uff08<\/strong>2<\/strong>\uff09\u56e2\u961f\u5728\u8be5\u9886\u57df\u5de5\u4f5c\u6c47\u603b<\/strong><\/p>\n

\u4ee5\u751f\u7269\u8d28\u57fa\u78b3\u6750\u6599\u4e3a\u7535\u6781\u6750\u6599\uff0c\u7528\u8bbe\u8ba1\u642d\u5efa\u7684\u4e0d\u540c\u6a21\u5f0f\u6469\u64e6\u7eb3\u7c73\u53d1\u7535\u673a\u4f9b\u80fd\uff0c\u6210\u529f\u5b9e\u73b0\u4e86\u6709\u673a\u6c61\u67d3\u7269\u7684\u81ea\u9a71\u52a8\u964d\u89e3\u3002\u8fd9\u4e00\u7cfb\u5217\u7814\u7a76\u5de5\u4f5c\u4e3a\u63a2\u5bfb\u9ad8\u6548\u3001\u5ec9\u4ef7\u7684\u7535\u6781\u6750\u6599\u5e94\u7528\u4e8e\u81ea\u9a71\u52a8\u4f53\u7cfb\uff0c\u8fdb\u800c\u5b9e\u73b0\u5bf9\u4e0d\u540c\u79cd\u7c7b\u6709\u673a\u6c61\u67d3\u7269\u7684\u5904\u7406\u63d0\u4f9b\u4e86\u53c2\u8003\u3002<\/p>\n

\uff08<\/strong>3<\/strong>\uff09\u76f8\u5173\u4f18\u8d28\u6587\u732e\u63a8\u8350<\/strong><\/p>\n

[1] Shuyan Gao*, Keran Geng, Haiying Liu, Xianjun Wei, Min Zhang, Peng Wang*, Jianji Wang*. Transforming Organic-Rich Amaranthus Waste into Nitrogen-Doped Carbon with Superior Performance of the Oxygen Reduction Reaction[J]. Energy Environmental Science<\/em>, 2014<\/strong>, 8(1): 221-229.\uff08\u9ad8\u88ab\u5f15\u8bba\u6587<\/strong>\uff09<\/p>\n

[2] Xianjun Wei*, Xiaoqiang Jiang, Jishi Wei, Shuyan Gao*. Functional Groups and Pore Size Distribution do Matter to Hierarchically Porous Carbons as High-Rate-Performance Supercapacitors[J]. Chemistry Materials<\/em>, 2016<\/strong>, 28(2): 445-458.\uff08\u9ad8\u88ab\u5f15\u8bba\u6587<\/strong>\uff09<\/p>\n

[3] Xin Zheng, Jingzhen Su, Xianjun Wei, Tao Jiang, Shuyan Gao*, Zhong Lin Wang*. Self-Powered Electrochemistry for the Oxidation of Organic Molecules by a Cross-Linked Triboelectric Nanogenerator[J]. Advanced Materials<\/em>, 2016<\/strong>, 28(26): 5188-5194.<\/p>\n

[4] Shuyan Gao*, Jingzhen Su, Xianjun Wei, Miao Wang, Miao Tian, Tao Jiang, Zhong Lin Wang*. Self-Powered Electrochemical Oxidation of 4-Aminoazobenzene Driven by a Triboelectric Nanogenerator[J]. ACS Nano<\/em>, 2017<\/strong>, 11(1): 770-778.<\/p>\n

[5] Shuyan Gao*, Ye Chen, Jingzhen Su, Miao Wang, Xianjun Wei, Tao Jiang, Zhong Lin Wang*. Triboelectric Nanogenerator Powered Electrochemical Degradation of Organic Pollutant Using Pt-Free Carbon Materials[J]. ACS Nano<\/em>, 2017<\/strong>, 11(4), 3965-3972.<\/p>\n

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