{"id":110080,"date":"2017-11-06T06:30:54","date_gmt":"2017-11-05T22:30:54","guid":{"rendered":"\/\/m.iemloyee.com\/?p=110080"},"modified":"2017-11-04T14:00:24","modified_gmt":"2017-11-04T06:00:24","slug":"science-advances%ef%bc%9acspbi3%e9%92%99%e9%92%9b%e7%9f%bf%e9%87%8f%e5%ad%90%e7%82%b9%e8%96%84%e8%86%9c%e5%a4%aa%e9%98%b3%e8%83%bd%e7%94%b5%e6%b1%a0%e6%95%88%e7%8e%87%e5%88%9b%e6%96%b0%e9%ab%98","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=110080","title":{"rendered":"Science Advances\uff1aCsPbI3\u9499\u949b\u77ff\u91cf\u5b50\u70b9\u8584\u819c\u592a\u9633\u80fd\u7535\u6c60\u6548\u7387\u521b\u65b0\u9ad8\uff01"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

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\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u7f8e\u56fd\u56fd\u5bb6\u53ef\u518d\u751f\u80fd\u6e90\u5b9e\u9a8c\u5ba4\uff08NREL\uff09\u7684Joseph M. Luther\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7b49\u91c7\u7528\u8868\u9762\u5316\u5b66\u7684\u7b56\u7565\uff0c\u7528\u9499\u949b\u77ff\u4e2dA\u4f4d\u9633\u79bb\u5b50\u7684\u5364\u5316\u7269\uff08\u8bb0\u4e3aAX\uff0c\u5176\u4e2dA\u4e3a\u7532\u8112\u3001\u7532\u80fa\u3001Cs+<\/sup>\uff0cX\u4e3aI–<\/sup>\u3001Br–<\/sup>\uff09\u4fee\u9970CsPbI3<\/sub>\u91cf\u5b50\u70b9\u8584\u819c\uff0c\u5f97\u5230\u7531\u8868\u9762\u8986\u76d6AX\u7684CsPbI3<\/sub>\u91cf\u5b50\u70b9\u6784\u6210\u7684\u8584\u819c\u3002\u672a\u7ecf\u5904\u7406\u7684CsPbI3<\/sub>\u91cf\u5b50\u70b9\u8868\u9762\u539f\u672c\u8986\u76d6\u6709\u5927\u91cf\u7531\u6db2\u76f8\u5408\u6210\u5f15\u5165\u7684\u6cb9\u9178\u3001\u6cb9\u80fa\u914d\u4f53\u3002\u5f15\u5165AX\u5e76\u5bf9CsPbI3<\/sub>\u91cf\u5b50\u70b9\u8fdb\u884c\u8868\u9762\u4fee\u9970\u540e\uff0c\u6cb9\u9178\u3001\u6cb9\u80fa\u914d\u4f53\u7684\u6570\u76ee\u5927\u5e45\u51cf\u5c11\uff0c\u8fd9\u4f7fCsPbI3<\/sub>\u91cf\u5b50\u70b9\u4e4b\u95f4\u7684\u8ddd\u79bb\u7f29\u77ed\uff0c\u6ce2\u51fd\u6570\u7684\u4ea4\u53e0\u4f5c\u7528\u589e\u5f3a\uff0c\u5373\u589e\u5f3a\u7684\u7535\u5b50\u8026\u5408\u4f5c\u7528\u524a\u5f31\u4e86\u5bf9\u7535\u6c60\u6027\u80fd\u8d77\u4e3b\u5bfc\u4f5c\u7528\u7684\u91cf\u5b50\u9650\u57df\u6548\u5e94\uff0c\u4ece\u800c\u4f7f\u91cf\u5b50\u70b9\u8584\u819c\u4e2d\u7684\u8f7d\u6d41\u5b50\u8fc1\u79fb\u7387\u63d0\u9ad8\uff0c\u77ed\u8def\u7535\u6d41\u5bc6\u5ea6\uff08JSC<\/sub>\uff09\u589e\u5927\uff0c\u800c\u5f00\u8def\u7535\u538b\uff08VOC<\/sub>\uff09\u548c\u586b\u5145\u56e0\u5b50\uff08FF\uff09\u57fa\u672c\u4e0d\u53d8\uff0c\u8fd9\u4f7f\u592a\u9633\u80fd\u7535\u6c60\u7684\u80fd\u91cf\u8f6c\u6362\u6548\u7387\uff08PCE\uff09\u663e\u8457\u63d0\u9ad8\u3002\u7814\u7a76\u8868\u660e\uff0c\u7528\u7898\u4ee3\u7532\u8112\uff08FAI\uff09\u5bf9CsPbI3<\/sub>\u91cf\u5b50\u70b9\u8584\u819c\u8fdb\u884c\u8868\u9762\u5316\u5b66\u4fee\u9970\u80fd\u8fbe\u5230\u6700\u597d\u7684\u7535\u5316\u5b66\u6027\u80fd\uff0c\u5176\u8f7d\u6d41\u5b50\u8fc1\u79fb\u7387\u7531\u672a\u7ecf\u5904\u7406\u76840.23 cm2<\/sup> V-1<\/sup> s-1<\/sup>\u589e\u52a0\u5230\u7ecf\u8868\u9762\u4fee\u9970\u540e\u76840.50 cm2<\/sup> V-1<\/sup> s-1<\/sup>\uff0c\u7ecf\u7ec4\u88c5\u5f97\u5230\u7684\u592a\u9633\u80fd\u7535\u6c60\uff08\u8bb0\u4e3aFAI- CsPbI3<\/sub>\uff09\u7684\u5f00\u8def\u7535\u538b\u4e3a1.16 V\uff0c\u77ed\u8def\u7535\u6d41\u5bc6\u5ea6\u4e3a15.25 mA\/cm2<\/sup>\uff0c\u586b\u5145\u56e0\u5b50\u4e3a76.63%\uff0c\u80fd\u91cf\u8f6c\u6362\u6548\u7387\u7531\u672a\u7ecf\u5904\u7406\u76848.5%\u63d0\u9ad8\u5230\u7ecf\u8868\u9762\u4fee\u9970\u540e\u768413.43%\uff0c\u8be5\u80fd\u91cf\u8f6c\u6362\u6548\u7387\u8d85\u8d8a\u4e86\u4ee5\u5f80\u62a5\u5bfc\u8fc7\u7684\u6240\u6709\u80f6\u4f53\u91cf\u5b50\u70b9\u592a\u9633\u80fd\u7535\u6c60\u3002\u8be5\u7814\u7a76\u6210\u679c\u4ee5\u201cEnhanced mobility CsPbI3<\/sub>\u00a0quantum dot arrays for record-efficiency, high-voltage photovoltaic cells<\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Science Advances<\/strong>\u4e0a\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

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\"\"<\/p>\n

(a) FAI- CsPbI3<\/sub>\u7684\u7ed3\u6784\u793a\u610f\u56fe\u3002<\/p>\n

(b) FAI- CsPbI3<\/sub>\u7684SEM\u622a\u9762\u56fe\u3002<\/p>\n

(c) \u6b63\u5411\u626b\u63cf\u548c\u53cd\u5411\u626b\u63cf\u5f97\u5230\u7684J-V\u7279\u6027\u66f2\u7ebf\u3002<\/p>\n

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\"\"<\/p>\n

(a) CsPbI3<\/sub>\u91cf\u5b50\u70b9\u8584\u819c\u6c89\u79ef\u53ca\u7528AX\u4fee\u9970\u8be5\u8584\u819c\u7684\u8fc7\u7a0b\u793a\u610f\u56fe\u3002<\/p>\n

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\"\"<\/p>\n

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\"\"<\/p>\n

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(b) \u4e0d\u540c\u91cf\u5b50\u70b9\u8584\u819c\u7684\u7ea6\u5316\u77ac\u6001\u5149\u7535\u5bfc\u7387\u3002<\/p>\n

(c,d) \u7531\u56fe(b)\u5f97\u5230\u7684(c) \u8f7d\u6d41\u5b50\u8fc1\u79fb\u7387 \u548c (d) \u8f7d\u6d41\u5b50\u5bff\u547d\u3002<\/p>\n

\u88681. \u7ecf\u4e0d\u540c\u79cd\u7c7bAX\u4fee\u9970\u540e\u7684\u592a\u9633\u80fd\u7535\u6c60\u53c2\u6570\u5bf9\u6bd4<\/strong><\/p>\n

\"\"<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Enhanced mobility CsPbI3<\/sub>\u00a0quantum dot arrays for record-efficiency, high-voltage photovoltaic cells<\/a> (Sci.Adv., 2017, DOI: 10.1126\/sciadv.aao4204)<\/p>\n

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