{"id":108613,"date":"2017-10-27T06:30:18","date_gmt":"2017-10-26T22:30:18","guid":{"rendered":"\/\/m.iemloyee.com\/?p=108613"},"modified":"2017-10-25T21:46:32","modified_gmt":"2017-10-25T13:46:32","slug":"angew-chem-int-ed-%e9%94%82-%e7%9f%b3%e6%a6%b4%e7%9f%b3%e7%94%b5%e6%b1%a0%e4%b8%ad%e9%87%91%e5%b1%9e%e7%95%8c%e9%9d%a2%e7%9a%84%e7%9e%ac%e6%80%81%e8%a1%8c%e4%b8%ba","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=108613","title":{"rendered":"Angew. Chem. Int. Ed. : \u9502-\u77f3\u69b4\u77f3\u7535\u6c60\u4e2d\u91d1\u5c5e\u754c\u9762\u7684\u77ac\u6001\u884c\u4e3a"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u8fd1\u6765\uff0c\u5728\u9502\u7535\u6c60\u9886\u57df\uff0c\u5bf9\u5229\u7528\u9502\u91d1\u5c5e\u590d\u5408\u6750\u6599\u6216\u4fee\u9970\u9694\u819c\u6765\u6291\u5236\u6216\u5ef6\u7f13\u9502\u679d\u6676\u751f\u957f\u5df2\u8fdb\u884c\u4e86\u5e7f\u6cdb\u7684\u7814\u7a76\u3002\u76f8\u6bd4\u4e0a\u8ff0\u7b56\u7565\uff0c\u53ef\u5229\u7528\u4e00\u4f53\u5316\u7684\u56fa\u6001\u7535\u89e3\u8d28(SSE)\u53d6\u4ee3\u805a\u5408\u7269\u9694\u819c\u4ee5\u7269\u7406\u963b\u6321\u9502\u679d\u6676\u7a7f\u523a\u3002\u6bd4\u8d77\u6709\u673a\u7535\u89e3\u6db2\uff0c\u56fa\u6001\u7535\u89e3\u8d28\u6709\u5f88\u591a\u4f18\u52bf\uff0c\u5982\u5177\u6709\u5bbd\u6cdb\u4e14\u7a33\u5b9a\u7684\u7a97\u53e3(0-5V)\u3001\u826f\u597d\u7684\u70ed\u7a33\u5b9a\u6027\u548c\u5185\u5728\u4e0d\u6613\u71c3\u6027\u3002\u5728\u4e0d\u540c\u7c7b\u578b\u7684\u56fa\u6001\u7535\u89e3\u8d28\u4e2d\uff0c\u77f3\u69b4\u77f3\u578bLi7<\/sub>La3<\/sub>Zr2<\/sub>O12<\/sub>(LLZO)\u7531\u4e8e\u5176\u8f83\u9ad8\u7684\u79bb\u5b50\u7535\u5bfc\u7387\u4ee5\u53ca\u5bf9\u91d1\u5c5e\u9502\u7684\u5316\u5b66\u7a33\u5b9a\u6027\uff0c\u6210\u4e3a\u9502\u91d1\u5c5e\u7535\u6c60\u56fa\u6001\u7535\u89e3\u8d28\u7684\u6709\u529b\u7ade\u4e89\u8005\u3002\u56fa\u4f53\u7535\u89e3\u8d28\u548c\u91d1\u5c5e\u9502\u4e4b\u95f4\u7684\u754c\u9762\u63a5\u89e6\u662f\u56fa\u6001\u7535\u6c60\u7684\u4e3b\u8981\u95ee\u9898\u3002\u5f15\u5165\u91d1\u5c5e\u8fc7\u6e21\u5c42\u5171\u578b\u6d82\u8986\u56fa\u4f53\u7535\u89e3\u8d28\u80fd\u63d0\u9ad8\u91d1\u5c5e\u9502\u7684\u754c\u9762\u6da6\u6e7f\u6027\u5e76\u964d\u4f4e\u754c\u9762\u7535\u963b\uff0c\u4f46\u91d1\u5c5e\u8fc7\u6e21\u5c42\u7684\u673a\u7406\u5c1a\u4e0d\u6e05\u695a\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\n \u8fd1\u65e5\uff0c\u7f8e\u56fd\u9a6c\u91cc\u5170\u5927\u5b66\u80e1\u826f\u5175\u6559\u6388<\/strong>(\u901a\u8baf\u4f5c\u8005<\/strong>)\u7b49\u4eba\u4ee5\u9541(Mg)\u4f5c\u4e3a\u6a21\u578b\u6765\u7814\u7a76\u91d1\u5c5e\u9540\u5c42\u5bf9\u56fa\u6001\u7535\u89e3\u8d28\u548c\u9502\u91d1\u5c5e\u9633\u6781\u754c\u9762\u7535\u963b\u7684\u5f71\u54cd\uff0c\u5e76\u5728Angew. Chem. Int. Ed.<\/strong>\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201cTransient Behavior of the Metal Interface in Lithium Metal-Garnet Batteries<\/strong>\u201d\u7684\u7814\u7a76\u8bba\u6587\u3002Li-Mg\u5408\u91d1\u8fc7\u7535\u52bf\u8f83\u4f4e\uff0c\u56e0\u6b64\u754c\u9762\u963b\u529b\u8f83\u4f4e\u3002\u4f5c\u8005\u53d1\u73b0\u91d1\u5c5e\u6d82\u5c42\u6eb6\u89e3\u4e8e\u7194\u878d\u7684\u9502\u5e76\u5411\u4f53\u76f8\u91d1\u5c5e\u9502\u6269\u6563\uff0c\u77f3\u69b4\u77f3\u56fa\u6001\u7535\u89e3\u8d28\u548c\u9502\u91d1\u5c5e\u4e4b\u95f4\u7684\u754c\u9762\u7535\u963b\u8f83\u5c0f\u4e14\u7a33\u5b9a\u3002TOF-SIMS\u7ed3\u679c\u8bc1\u5b9e\u4e86Mg\u6d82\u8986\u4e8e\u754c\u9762\u7684\u77ac\u6001\u884c\u4e3a\uff0cXPS\u7ed3\u679c\u8868\u660e\uff0c\u5f53\u7194\u878d\u7684\u9502\u4e0e\u9541\u6d82\u5c42\u4f5c\u7528\u65f6\uff0c\u77f3\u69b4\u77f3\u56fa\u6001\u7535\u89e3\u8d28\u4ecd\u4fdd\u6301\u7a33\u5b9a\u3002\u6b64\u5916\uff0c\u7531\u4e8e\u91d1\u5c5e\u754c\u9762\u7684\u77ac\u6001\u884c\u4e3a\uff0c\u754c\u9762\u963b\u6297\u5e76\u6ca1\u6709\u968f\u91d1\u5c5e\u9540\u5c42\u7684\u539a\u5ea6(5\u300110\u548c100 nm)\u589e\u52a0\u800c\u6539\u53d8\u3002<\/p>\n

\u3010\u56fe\u6587\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u56fe1\u56fa\u6001\u7535\u89e3\u8d28\u548c\u7194\u878d\u91d1\u5c5e\u9502\u754c\u9762\u77ac\u6001\u8fc7\u6e21\u5c42\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u52a0\u70ed\u65f6\uff0c\u91d1\u5c5e\u6d82\u5c42\u6eb6\u89e3\u5e76\u6269\u6563\u5165\u7194\u878d\u7684\u9502\uff0c\u5f62\u6210\u5bcc\u9502\u7684\u9502-\u91d1\u5c5e\u56fa\u6eb6\u4f53\u3002\u91d1\u5c5e\u7684\u6eb6\u89e3\u548c\u6269\u6563\u5f62\u6210\u4e86\u77f3\u69b4\u77f3SSE\u548c\u9502\u4e4b\u95f4\u7684\u77ac\u6001\u754c\u9762\u3002<\/p>\n

\u56fe2 Mg\u6d82\u8986\u7684\u77f3\u69b4\u77f3SSE\u7684\u5f62\u8c8c\u53ca\u5176\u4e0e\u91d1\u5c5e\u9502\u7684\u754c\u9762<\/strong><\/p>\n

\"\"<\/p>\n

a,b) \u91d1\u5c5e\u9502\u548c\u9541\u6d82\u8986\u7684\u77f3\u69b4\u77f3LLZO SSE \u754c\u9762\u6a2a\u65ad\u9762\u53ca\u653e\u5927\u56fe\u50cf\uff1b<\/p>\n

c) \u754c\u9762\u6a2a\u65ad\u9762\u7684\u9541\u5143\u7d20\u5206\u5e03\u56fe\uff1b<\/p>\n

d) \u4f53\u76f8\u91d1\u5c5e\u9502\u4e2d\u7684\u9541\u5143\u7d20\u5206\u5e03\u56fe\u8bc1\u5b9e\u9541\u5728\u9502\u4e2d\u7684\u68af\u5ea6\u5206\u5e03\u3002<\/p>\n

\u56fe3 \u754c\u9762\u963b\u6297\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

a) \u5728\u77f3\u69b4\u77f3SSE\u548c\u7194\u878d\u9502\u754c\u9762\u7684\u77ac\u6001\u9541\u5c42\u793a\u610f\u56fe\uff1b<\/p>\n

b) \u4e0d\u540c\u754c\u9762\u9541\u5c42\u539a\u5ea6\u4e0b\u7684EIS\u6d4b\u8bd5\uff1b<\/p>\n

c) 100 nm\u9541\u8986\u76d6\u77f3\u69b4\u77f3SSE\u7684\u9502\u7535\u9540\/\u9000\u9540\u6027\u80fd\u3002<\/p>\n

\u56fe4 \u91d1\u5c5e\u9502\u548c\u9541\u6d82\u8986\u77f3\u69b4\u77f3SSE\u754c\u9762\u7684TOF-SIMS\u5206\u6790<\/strong><\/p>\n

\"\"<\/p>\n

a) \u79bb\u5b50\u675f\u6e85\u5c04\u5f62\u6210\u7684\u5751\u53caLi\/Mg\/\u77f3\u69b4\u77f3SSE\u6837\u54c1\u6a2a\u65ad\u9762\u7684SEM \u56fe\u50cf\uff1b<\/p>\n

b) Li\/Mg\/\u77f3\u69b4\u77f3SSE\u7684\u754c\u9762\u5c55\u793a\u51fa\u77f3\u69b4\u77f3SSE\u4e0e\u9502\u7d27\u5bc6\u7684\u63a5\u89e6\uff1b<\/p>\n

c) \u754c\u9762\u653e\u5927\u56fe\u50cf\uff1b<\/p>\n

d-g) Li\/Mg\/\u77f3\u69b4\u77f3SSE\u6a2a\u65ad\u9762\u7684\u5143\u7d20\u5206\u5e03(Mg, Li, La, Zr)\uff1b<\/p>\n

h) Li\/Mg\/\u77f3\u69b4\u77f3SSE\u7684TOF-SIMS\u5206\u6790\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u4f5c\u8005\u4ee5Mg\u4f5c\u4e3a\u6a21\u578b\u6765\u7814\u7a76\u77f3\u69b4\u77f3\u56fa\u6001\u7535\u89e3\u8d28\u548c\u9502\u91d1\u5c5e\u754c\u9762\u7684\u91d1\u5c5e\u8fc7\u6e21\u5c42\u3002\u91d1\u5c5e\u8fc7\u6e21\u5c42\u6ca1\u6709\u5982\u5e38\u89c4\u5047\u8bbe\u822c\u7559\u5728\u754c\u9762\uff0c\u800c\u662f\u4ece\u754c\u9762\u6d88\u5931\uff0c\u5927\u91cf\u6eb6\u89e3\u548c\u6269\u6563\u4e8e\u7194\u5316\u7684\u9502\uff0c\u5373\u6eb6\u89e3\u91d1\u5c5e\u4f5c\u4e3a\u77ac\u6001\u8fc7\u6e21\u5c42\u3002\u6b64\u5916\uff0c\u754c\u9762\u963b\u6297\u5e76\u672a\u968f\u91d1\u5c5e\u9540\u5c42\u7684\u539a\u5ea6(5\u300110\u548c100 nm)\u589e\u52a0\u800c\u6539\u53d8\u3002\u8be5\u7814\u7a76\u8868\u660e\u91d1\u5c5e\u5728\u754c\u9762\u7684\u77ac\u6001\u884c\u4e3a\u4f7f\u754c\u9762\u6d88\u5931\u5e76\u89e3\u51b3\u4e86\u56fa\u6001\u7535\u89e3\u8d28\u4e0e\u9502\u754c\u9762\u963b\u6297\u7684\u6839\u672c\u6311\u6218\uff0c\u4e3a\u5b9e\u73b0\u56fa\u6001\u9502\u91d1\u5c5e\u7535\u6c60\u94fa\u5e73\u4e86\u9053\u8def\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aTransient Behavior of the Metal Interface in Lithium Metal-Garnet Batteries<\/a><\/strong>\u00a0(Angew. Chem. Int. Ed., 2017, DOI: 10.1002\/anie.201708637)<\/p>\n

\u3010\u901a\u8baf\u4f5c\u8005\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u80e1\u826f\u5175\u6559\u6388\u76ee\u524d\u5728\u5c31\u804c\u4e8e\u7f8e\u56fd\u9a6c\u91cc\u5170\u5927\u5b66\u6750\u6599\u79d1\u5b66\u4e0e\u5de5\u7a0b\u5b66\u9662\uff0c\u4e3b\u8981\u4ece\u4e8b\u7eb3\u7c73\u6750\u6599\u3001\u7eb3\u7c73\u5236\u9020\u3001\u751f\u7269\u8d28\u7eb3\u7c73\u7ea4\u7ef4\u7d20\u5728\u56fa\u6001\u3001\u94a0\u79bb\u5b50\u7535\u6c60\u53ca\u5370\u5237\u67d4\u6027\u7535\u5b50\u7b49\u9886\u57df\u7684\u5e94\u7528\u7814\u7a76\u3002\u8fd1\u4e94\u5e74\uff0c\u4e3b\u6301\u7f8e\u56fd\u80fd\u6e90\u90e8\u3001\u7a7a\u519b\u90e8\u7b49\u79d1\u7814\u9879\u76ee10\u4f59\u9879\uff0c\u603b\u7ecf\u8d39\u8d85\u8fc7800\u4e07\u7f8e\u5143\uff1b\u5728Chemical Reviews\u3001Nature Materials\u3001Nature Commutations\u3001PNAS\u3001JACS\u3001Advanced Materials\u3001Energy & Environmental Science<\/em>\u7b49\u4e16\u754c\u9876\u7ea7\u671f\u520a\u4e0a\u53d1\u8868SCI\u68c0\u7d22\u6587\u7ae0210\u4f59\u7bc7\uff0c\u5176\u4e2d\u5f71\u54cd\u56e0\u5b50\u5927\u4e8e10\u7684\u6587\u7ae0130\u4f59\u7bc7\uff0c\u603b\u88ab\u5f15\u8d85\u8fc715,000\u6b21\uff0cH-index: ~60\uff1b\u6388\u6743\u7f8e\u56fd\u4e13\u522920\u4f59\u9879\uff1b\u62c5\u4efbScientific Report\u3001Frontiers in Energy Storage\u3001Supercapacitor<\/em>\u7b49\u56fd\u9645\u77e5\u540d\u671f\u520a\u7f16\u59d4\u3002<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8\u65b0\u80fd\u6e90\u5c0f\u7ec4abc940504\u7f16\u8bd1\u6574\u7406\uff0c\u53c2\u4e0e\u65b0\u80fd\u6e90\u8bdd\u9898\u8ba8\u8bba\u8bf7\u52a0\u5165\u201c\u6750\u6599\u4eba\u65b0\u80fd\u6e90\u6750\u6599\u4ea4\u6d41\u7fa4 422065953\u201d\u3002<\/p>\n

\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1aRDD-2011-CHERISH\uff0c\u4efb\u4e39\u4e39\uff0c\u6211\u4eec\u4f1a\u9080\u8bf7\u5404\u4f4d\u8001\u5e08\u52a0\u5165\u4e13\u5bb6\u7fa4\u3002<\/p>\n

\u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u7f16\u8f91\u90e8<\/a><\/strong>\u3002\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n

\u4eea\u5668\u8bbe\u5907\u3001\u8bd5\u5242\u8017\u6750\u3001\u6750\u6599\u6d4b\u8bd5\u3001\u6570\u636e\u5206\u6790\uff0c\u627e\u6750\u6599\u4eba<\/a>\u3001\u4e0a\u6d4b\u8bd5\u8c37<\/a>\uff01<\/strong><\/p>\n","protected":false},"excerpt":{"rendered":"

\u3010\u5f15\u8a00\u3011 \u8fd1\u6765\uff0c\u5728\u9502\u7535\u6c60\u9886\u57df\uff0c\u5bf9\u5229\u7528\u9502\u91d1\u5c5e\u590d\u5408\u6750\u6599\u6216\u4fee\u9970\u9694\u819c\u6765\u6291\u5236\u6216\u5ef6\u7f13\u9502\u679d\u6676\u751f\u957f\u5df2\u8fdb\u884c\u4e86\u5e7f\u6cdb\u7684\u7814\u7a76\u3002\u76f8\u6bd4\u4e0a\u8ff0\u7b56\u7565\uff0c\u53ef\u5229\u7528\u4e00\u4f53\u5316\u7684\u56fa\u6001\u7535\u89e3\u8d28(SSE)\u53d6\u4ee3\u805a\u5408\u7269…<\/p>\n","protected":false},"author":4931,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[],"class_list":["post-108613","post","type-post","status-publish","format-standard","hentry","category-jiedu"],"_links":{"self":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/108613"}],"collection":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/users\/4931"}],"replies":[{"embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=108613"}],"version-history":[{"count":3,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/108613\/revisions"}],"predecessor-version":[{"id":108643,"href":"\/\/m.iemloyee.com\/index.php?rest_route=\/wp\/v2\/posts\/108613\/revisions\/108643"}],"wp:attachment":[{"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=108613"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=108613"},{"taxonomy":"post_tag","embeddable":true,"href":"\/\/m.iemloyee.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=108613"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}