{"id":106557,"date":"2017-10-16T06:30:06","date_gmt":"2017-10-15T22:30:06","guid":{"rendered":"\/\/m.iemloyee.com\/?p=106557"},"modified":"2017-10-13T22:51:02","modified_gmt":"2017-10-13T14:51:02","slug":"pnas%ef%bc%9a%e5%8f%af%e5%ae%9e%e7%94%a8%e5%9b%ba%e6%80%81%e7%94%b5%e8%a7%a3%e8%b4%a8%e7%aa%81%e7%a0%b4%e6%80%a7%e8%bf%9b%e5%b1%95-%e5%9f%ba%e4%ba%8e%e5%9b%a2%e7%b0%87%e7%a6%bb%e5%ad%90%e7%9a%84","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=106557","title":{"rendered":"PNAS\uff1a\u53ef\u5b9e\u7528\u56fa\u6001\u7535\u89e3\u8d28\u6700\u65b0\u8fdb\u5c55-\u57fa\u4e8e\u56e2\u7c07\u79bb\u5b50\u7684\u5bcc\u9502\u53cd\u9499\u949b\u77ff\u8d85\u79bb\u5b50\u5bfc\u4f53"},"content":{"rendered":"

\u5f15\u8a00<\/strong><\/p>\n

\u5177\u6709\u9ad8\u5b89\u5168\u6027\uff0c\u9ad8\u529f\u7387\u548c\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u7b49\u4f18\u52bf\u7684\u5168\u56fa\u6001\u7535\u6c60\u5c06\u5728\u4e0b\u4e00\u4ee3\u50a8\u80fd\u6750\u6599\u4e2d\u626e\u6f14\u5173\u952e\u89d2\u8272\u3002\u4f46\u662f\uff0c\u5168\u56fa\u6001\u7535\u6c60\u7684\u53d1\u5c55\u53d7\u5236\u4e8e\u5bfb\u627e\u4f18\u79c0\u7684\u56fa\u6001\u7535\u89e3\u8d28\u3002\u5b9e\u7528\u7684\u56fa\u6001\u7535\u89e3\u8d28\u6750\u6599\u5e94\u5728\u5ba4\u6e29\u4e0b\u5177\u6709\u53ef\u4ee5\u548c\u6db2\u6001\u7535\u89e3\u8d28\u76f8\u6bd4\u62df\u7684\u79bb\u5b50\u7535\u5bfc\u7387 (10-2<\/sup> S\/cm)\u3002\u901a\u8fc7\u7406\u8bba\u7814\u7a76\uff0c\u7814\u7a76\u4eba\u5458\u53d1\u73b0\u5229\u7528\u56e2\u7c07\u79bb\u5b50\u4ee3\u66ff\u57fa\u672c\u79bb\u5b50\uff0c\u53ef\u4ee5\u83b7\u5f97\u65b0\u7684\u9502\u79bb\u5b50\u8d85\u5bfc\u4f53Li3<\/sub>SBF4\u548cLi3<\/sub>S(BF4<\/sub>)0.5<\/sub>Cl0.5<\/sub>\u3002\u8fd9\u4e9b\u65b0\u6750\u6599\u4e0d\u4ec5\u5728\u5ba4\u6e29\u4e0b\u5177\u6709\u975e\u5e38\u9ad8\u7684\u79bb\u5b50\u5bfc\u7535\u7387 (> 10-2<\/sup> S\/cm) \u975e\u5e38\u4f4e\u7684\u79bb\u5b50\u6fc0\u53d1\u80fd(< 0.25 eV)\uff0c\u800c\u4e14\u5177\u6709\u8d85\u5927\u7684\u5e26\u9699\u4ee5\u53ca\u9ad8\u7194\u70b9\u7b49\u4f18\u52bf\u3002\u8fdb\u4e00\u6b65\u7814\u7a76\u53d1\u73b0\uff0c\u8fd9\u4e9b\u4f18\u5f02\u7684\u6750\u6599\u6027\u80fd\u6e90\u4e8e\u56e2\u7c07\u79bb\u5b50\u5728\u6750\u6599\u4e2d\u7684\u4f4e\u80fd\u91cf\u632f\u52a8\u6a21\uff08\u79f0\u4e3a\u51c6\u521a\u4f53\u6a21\uff0cquasirigid unit modes)\u4ee5\u53ca\u56e2\u7c07\u79bb\u5b50\u9020\u6210\u7684\u5c3a\u5bf8\u6548\u5e94\u3002<\/p>\n

\u6210\u679c\u7b80\u4ecb<\/strong><\/p>\n

2017\u5e7410\u67082\u65e5\uff0cPNAS<\/strong> (Proceedings of the National Academy of Sciences of the United States of America) \u5728\u7ebf\u53d1\u8868\u9898\u4e3a\u201c\u57fa\u4e8e\u56e2\u7c07\u79bb\u5b50\u7684\u5bcc\u9502\u53cd\u9499\u949b\u77ff\u8d85\u79bb\u5b50\u5bfc\u4f53\u201d(Li-rich antiperovskite superionic conductors based on cluster ions<\/strong>) \u7684\u7814\u7a76\u8bba\u6587 (Direct Submission) [1]<\/sup>\u3002\u4f5c\u8005\u4e3a\u5de5\u4f5c\u4e8e\u7f8e\u56fd\u5f17\u5409\u5c3c\u4e9a\u8054\u90a6\u5927\u5b66<\/strong>\u7684\u65b9\u5f18\u535a\u58eb<\/strong>\u548cPuru Jena\u6559\u6388<\/strong>\u3002\u7814\u7a76\u8005\u53d1\u73b0\u4e86\u5229\u7528\u56e2\u7c07\u79bb\u5b50\u4f5c\u4e3a\u57fa\u5143\uff0c\u53ef\u4ee5\u6784\u9020\u51fa\u6027\u80fd\u4f18\u5f02\u7684\u9502\u79bb\u5b50\u56fa\u6001\u7535\u89e3\u8d28\u3002\u63ed\u793a\u4e86\u56e2\u7c07\u79bb\u5b50\u4e0d\u540c\u4e8e\u57fa\u672c\u79bb\u5b50\u7684\u7279\u6027\u2014\u2014\u5982\u8d85\u9ad8\u7684\u7535\u5b50\u4eb2\u548c\u80fd\uff0c\u8d85\u5927\u7684\u5c3a\u5bf8\u4ee5\u53ca\u5177\u6709\u5185\u90e8\u7535\u8377\u5206\u90e8\u7b49\u2014\u2014\u7ed9\u5757\u4f53\u6750\u6599\u6027\u8d28\u5e26\u6765\u7684\u53d8\u5316\uff0c\u5e76\u53d1\u73b0\u4e86\u56e2\u7c07\u79bb\u5b50\u7684\u632f\u52a8\u6a21\u4ee5\u53ca\u5c3a\u5bf8\u6548\u5e94\u4fc3\u4f7f\u9502\u79bb\u5b50\u5728\u56fa\u4f53\u4e2d\u8fc1\u79fb\u7684\u673a\u7406\u3002<\/p>\n

\u56fe\u6587\u5bfc\u8bfb<\/strong><\/p>\n

\u56fe1.\u57fa\u4e8e\u56e2\u7c07\u79bb\u5b50\u7684\u53cd\u9499\u949b\u77ff\u9502\u79bb\u5b50\u8d85\u5bfc\u4f53\u7684\u57fa\u672c\u6027\u8d28<\/strong><\/p>\n

\"\"<\/p>\n

A. <\/span>\u57fa\u4e8e\u56e2\u7c07\u79bb\u5b50\u7684\u53cd\u9499\u949b\u77ff\u6750\u6599\u7684\u6676\u4f53\u7ed3\u6784\u3002\u57fa\u6001\u65f6\uff0c\u56e2\u7c07\u79bb\u5b50\uff08\u5982BF4<\/sub>–<\/sup>, <\/span>\u56fe\u4e2d\u56db\u9762\u4f53\uff09\u7684\u4e00\u4e2a\u4e09\u91cd\u65cb\u8f6c\u5bf9\u79f0\u8f74\uff08C3<\/sub><\/span>\uff09\u4e0e\u7acb\u65b9\u5355\u80de\u7684\u4f53\u5bf9\u89d2\u7ebf\u91cd\u5408\uff08\u5982\u7eff\u8272\u7bad\u5934\u7ebf\u6240\u793a\uff09\uff1b<\/p>\n

B. <\/span>\u6676\u4f53Li3<\/sub>OBH4<\/sub><\/span>\uff0cLi3<\/sub>SAlH4<\/sub><\/span>\u4ee5\u53caLi3<\/sub>SBF4<\/sub><\/span>\u7684\u6676\u683c\u52a8\u529b\u5b66\u6027\u8d28\u6bd4\u8f83\uff0c\u58f0\u5b50\u8c31\u4e2d\u7684\u7ea2\u8272\u632f\u52a8\u6a21\u90fd\u5c5e\u4e8e\u51c6\u521a\u4f53\u6a21\uff08quasirigid unit modes<\/span>\uff09\uff1b<\/p>\n

C. <\/span>\u6676\u4f53Li3<\/sub>OBH4<\/sub><\/span>\uff0cLi3<\/sub>SAlH4<\/sub><\/span>\u4ee5\u53caLi3<\/sub>SBF4<\/sub><\/span>\u7684\u5e26\u9699\u6bd4\u8f83\uff1b<\/p>\n

D. <\/span>\u5206\u5b50\u52a8\u529b\u5b66\u6a21\u62df\u5f97\u5230\u7684400 K<\/span>\uff08\u9ed1\u7ebf\uff09\u548c600K<\/span>\uff08\u7ea2\u7ebf\uff09\u65f6\u539f\u5b50\u5bf9\u7684\u76f8\u5173\u51fd\u6570\u3002<\/p>\n

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\u6bd4\u8f83\u6676\u4f53Li3<\/sub>OBH4<\/sub>\u4ee5\u53caLi3<\/sub>SAlH4<\/sub>\uff0c\u6676\u4f53Li3<\/sub>SBF4<\/sub>\u5177\u6709\u6700\u5927\u7684\u5e26\u9699\uff08\uff5e8.5 eV\uff09\uff0c\u9ad8\u7684\u7194\u70b9\uff08\uff1e600K\uff09\uff0c\u5176\u57fa\u4e8eLiBF4 <\/sub>+Li2<\/sub>S\u2192Li3<\/sub>SBF4<\/sub> \u5236\u5907\u53cd\u5e94\u6240\u9700\u7684\u80fd\u91cf\u4e5f\u6bd4\u8f83\u4f4e\uff08\uff5e39.4 meV\/atom\uff09\u3002\u8fd9\u4e9b\u4f18\u79c0\u7684\u6750\u6599\u6027\u8d28\u6e90\u4e8e\u56e2\u7c07\u79bb\u5b50Li3<\/sub>S+ <\/sup>\u548cBF4<\/sub>– <\/sup>\u9002\u5f53\u7684\u7269\u7406\u5316\u5b66\u6027\u8d28\u3002\u7279\u522b\u662f\u8d85\u5364\u79bb\u5b50BF4<\/sub>– <\/sup>\u6070\u5f53\u7684\u79bb\u5b50\u5c3a\u5bf8\uff0c\u5185\u90e8\u7535\u8377\u5206\u90e8\u4ee5\u53ca\u5b83\u8d85\u9ad8\u7684\u7535\u5b50\u4eb2\u548c\u80fd\u3002<\/p>\n

\u7814\u7a76\u4eba\u5458\u53d1\u73b0\uff0c\u5728\u6676\u4f53\u7684\u7acb\u65b9\u5143\u80de\u4e2d\uff0c\u5448\u56db\u9762\u4f53\u7ed3\u6784\u7684\u8d85\u5364\u79bb\u5b50BF4<\/sub>–<\/sup>\u5177\u6709\u7279\u5b9a\u7684\u5bf9\u79f0\u6027\u53d6\u5411\uff0c\u5373\u5b83\u7684\u4e00\u4e2a\u4e09\u91cd\u65cb\u8f6c\u5bf9\u79f0\u8f74\u4e0e\u7acb\u65b9\u6676\u80de\u7684\u4f53\u5bf9\u89d2\u7ebf\u91cd\u5408\uff0c\u8fd9\u6837\u7684\u53d6\u5411\u4f7f\u5f97\u80fd\u91cf\u6700\u4f4e\u3002<\/p>\n

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\"\"<\/p>\n

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\"\"<\/p>\n

A. <\/span>\u5206\u5b50\u52a8\u529b\u5b66\u6a21\u62df\u91c7\u7528\u7684Li3<\/sub>SBF4<\/sub><\/span>\u6676\u4f53\u6a21\u578b\u4ee5\u53ca\u8be5\u6750\u6599\u7684\u9502\u79bb\u5b50\u7535\u5bfc\u7387\uff1b<\/p>\n

B. <\/span>\u5206\u5b50\u52a8\u529b\u5b66\u6a21\u62df\u91c7\u7528\u7684Li3<\/sub>S(BF4<\/sub>)0.5<\/sub>Cl0.5<\/sub><\/span>\u6676\u4f53\u6a21\u578b\u53ca\u8be5\u6750\u6599\u7684\u9502\u79bb\u5b50\u7535\u5bfc\u7387\u3002<\/p>\n

Li3<\/sub>SBF4<\/sub>\u548cLi3<\/sub>S(BF4<\/sub>)0.5<\/sub>Cl0.5<\/sub>\u6676\u4f53\u5728\u5ba4\u6e29\u4e0b\u7684\u9502\u79bb\u5b50\u7535\u5bfc\u7387\u90fd\u8fbe\u5230\u6216\u8d85\u8fc7\u4e86\u5f53\u524d\u5b9e\u7528\u4e2d\u7684\u6db2\u6001\u7535\u89e3\u8d28\u7684\u79bb\u5b50\u7535\u5bfc\u7387\u3002\u7531\u4e8e\u5177\u6709\u4f4e\u7684\u79bb\u5b50\u6fc0\u53d1\u80fd\uff0c\u8fd9\u4e9b\u56fa\u6001\u7535\u89e3\u8d28\u5373\u4f7f\u5728\u4f4e\u6e29\uff08-30\u2103\uff09\u4e5f\u5177\u6709\u53ef\u5b9e\u7528\u7684\u79bb\u5b50\u7535\u5bfc\u7387\u3002<\/p>\n

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\u5c55\u671b<\/strong>\uff1a<\/p>\n

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\u53c2\u8003\u6587\u732e<\/strong>\uff1a<\/p>\n

1.Fang H, Jena P (2017) Li-rich antiperovskite superionic conductors based on cluster ions<\/a>. Proc. Nat. Acad. Sci. doi: 10.1073\/pnas.1704086114.<\/p>\n

2.Fang H, Jena P (2016) Super-ion inspired colorful hybrid perovskite solar cells. J. Mater.Chem. A 4:4728\u20134737.<\/p>\n

3.Fang H, Jena P (2016) Molecular origin of properties of organic-inorganic hybrid perovskites: The big picture from small clusters. J. Phys. Chem. Lett. 7:1596\u20131603.<\/p>\n

4. Fang H, Jena P (2017) Atomic-Level Design of Water-Resistant Hybrid Perovskites for Solar Cells by Using Cluster Ions. J. Phys. Chem. Lett., 2017, 8 (16): 3726\u20133733.<\/p>\n

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