{"id":103079,"date":"2017-10-10T06:30:07","date_gmt":"2017-10-09T22:30:07","guid":{"rendered":"\/\/m.iemloyee.com\/?p=103079"},"modified":"2017-10-09T09:29:23","modified_gmt":"2017-10-09T01:29:23","slug":"%e4%b8%ad%e5%9b%bd%e7%9f%b3%e6%b2%b9%e5%a4%a7%e5%ad%a6%ef%bc%88%e5%8d%8e%e4%b8%9c%ef%bc%89%e8%b5%b5%e5%ad%a6%e6%b3%a2%e5%9b%a2%e9%98%9fadv-funct-mater-%ef%bc%9a%e5%8f%8c%e9%87%91%e5%b1%9emof-74","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=103079","title":{"rendered":"\u4e2d\u56fd\u77f3\u6cb9\u5927\u5b66\uff08\u534e\u4e1c\uff09\u8d75\u5b66\u6ce2\u56e2\u961fAdv. Funct. Mater.\uff1a\u53cc\u91d1\u5c5eMOF-74\u4e3a\u524d\u9a71\u4f53\u5236\u5907Co-Ni-P\u7eb3\u7c73\u7ba1\u9ad8\u6548\u7535\u89e3\u6c34\u50ac\u5316\u5242"},"content":{"rendered":"

\u3010\u80cc\u666f\u4ecb\u7ecd\u3011<\/b><\/strong><\/p>\n

\u80fd\u6e90\u6d88\u8d39\u7684\u5feb\u901f\u589e\u957f\u548c\u76f8\u5e94\u7684\u73af\u5883\u95ee\u9898\u52a0\u5267\u4e86\u5bf9\u53ef\u518d\u751f\u80fd\u6e90\u548c\u6e05\u6d01\u80fd\u6e90\u7684\u9700\u6c42\uff0c\u6c22\u80fd\u4f5c\u4e3a\u4e00\u79cd\u53ef\u518d\u751f\u7684\u6e05\u6d01\u80fd\u6e90\u53d7\u5230\u8d8a\u6765\u8d8a\u591a\u7684\u5173\u6ce8\u3002\u7535\u89e3\u6c34\u5236\u6c22\u88ab\u8ba4\u4e3a\u662f\u76ee\u524d\u6700\u6709\u524d\u666f\u7684\u5236\u6c22\u6280\u672f\u4e4b\u4e00\u3002\u5728\u7535\u89e3\u6c34\u7684\u8fc7\u7a0b\u4e2d\uff0c\u7535\u5316\u5b66\u6790\u6c27\u53cd\u5e94\uff08OER\uff09\u548c\u6790\u6c22\u53cd\u5e94\uff08HER\uff09\u4f5c\u4e3a\u5176\u4e2d\u7684\u4e24\u4e2a\u6838\u5fc3\u53cd\u5e94\u53d7\u5230\u53cd\u5e94\u52a8\u529b\u5b66\u7684\u9650\u5236\uff0c\u5747\u9700\u8981\u9ad8\u6548\u50ac\u5316\u5242\u7684\u53c2\u4e0e\u52a0\u5feb\u53cd\u5e94\u7684\u8fdb\u884c\u3002\u73b0\u9636\u6bb5\uff0cRuO2<\/sub>\u548cPt\u50ac\u5316\u5242\u4ecd\u7136\u662fOER\u548cHER\u6700\u9ad8\u6548\u7684\u50ac\u5316\u5242\uff0c\u4f46\u662f\u53d7\u9650\u4e8e\u8d35\u91d1\u5c5e\u7684\u50a8\u91cf\u53ca\u6210\u672c\uff0c\u5236\u5907\u5177\u6709\u9ad8\u50ac\u5316\u6d3b\u6027\u7684\u975e\u8d35\u91d1\u5c5e\u50ac\u5316\u5242\u6210\u4e3a\u4e86\u8be5\u9886\u57df\u7684\u7814\u7a76\u70ed\u70b9\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

\u8fd1\u65e5\uff0cAdvanced Functional Materials<\/strong>\u5728\u7ebf\u53d1\u8868\u4e86\u9898\u4e3a\u201c\u91d1\u5c5e-\u6709\u673a\u6846\u67b6\u4e3a\u524d\u9a71\u4f53\u5236\u5907Co-Ni-P\u7eb3\u7c73\u7ba1\u9ad8\u6548\u7535\u89e3\u6c34\u50ac\u5316\u5242\u201d(Metal-Organic Frameworks Derived Nanotube of Nickel\u2013Cobalt Bimetal Phosphides as Highly Efficient Electrocatalysts for Overall Water Splitting<\/strong>)\u7684\u7814\u7a76\u8bba\u6587\uff0c\u62a5\u9053\u4e86\u4e00\u79cd\u901a\u8fc7\u91d1\u5c5e-\u6709\u673a\u6846\u67b6\u7684\u53ef\u63a7\u751f\u957f\u5236\u5907Co-Ni-P\u7eb3\u7c73\u7ba1\u9ad8\u6548\u7535\u89e3\u6c34\u50ac\u5316\u5242\u7684\u6700\u65b0\u7814\u7a76\u6210\u679c\u3002\u901a\u8fc7\u7cbe\u786e\u8c03\u8282\u91d1\u5c5e-\u6709\u673a\u6846\u67b6\u524d\u9a71\u4f53\u4e2d\u91d1\u5c5e\u7684\u539f\u5b50\u6bd4\uff0c\u63a7\u5236\u91d1\u5c5e\u6709\u673a\u6846\u67b6\u6750\u6599\u6676\u4f53\u7684\u751f\u957f\uff0c\u8fdb\u800c\u5f97\u5230\u4e86\u5177\u6709\u4e0d\u540c\u5f62\u8c8c\u7684\u53cc\u91d1\u5c5e\u6709\u673a\u6846\u67b6\u53ca\u5176\u78f7\u5316\u6750\u6599\u3002\u901a\u8fc7\u7279\u5b9aCo-Ni\u539f\u5b50\u6bd4\u7684\u8c03\u8282\u53ef\u4ee5\u5f97\u5230\u5177\u6709\u4e2d\u7a7a\u7eb3\u7c73\u7ba1\u7ed3\u6784\u7684Co-Ni-P\u590d\u5408\u6750\u6599\uff0c\u5728\u78b1\u6027\u6761\u4ef6\u4e0b\u5177\u6709\u4f18\u4e8e\u8d35\u91d1\u5c5e\u50ac\u5316\u5242Pt\/C-RuO2<\/sub>\u7684\u50ac\u5316\u6027\u80fd\u3002\u8bba\u6587\u901a\u8baf\u4f5c\u8005\u4e3a\u4e2d\u56fd\u77f3\u6cb9\u5927\u5b66\uff08\u534e\u4e1c\uff09\u975e\u5e38\u89c4\u6cb9\u6c14\u4e0e\u65b0\u80fd\u6e90\u7814\u7a76\u9662\u8d75\u5b66\u6ce2\u6559\u6388\uff0c\u7b2c\u4e00\u4f5c\u8005\u4e3a\u8d75\u5b66\u6ce2\u6559\u6388\u7684\u535a\u58eb\u7814\u7a76\u751f\u95eb\u7406\u505c\u3002<\/p>\n

\u56fe\u6587\u5bfc\u8bfb\uff1a<\/b><\/strong><\/p>\n

\u56fe1<\/b><\/strong>.Co4Ni1P<\/b><\/strong>\u7eb3\u7c73\u7ba1<\/b><\/strong>\u7684\u5408\u6210\u4e0e<\/b><\/strong>\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"a)MOF-74-Co4Ni1\u548cc)Co4Ni1P\u7eb3\u7c73\u7ba1\u7684SEM\u7167\u7247\uff1b<\/p>\n

b)MOF-74-Co4Ni1\u548cd)Co4Ni1P\u7eb3\u7c73\u7ba1\u7684TEM\u7167\u7247\uff1b<\/p>\n

e) Co4Ni1P\u7eb3\u7c73\u7ba1\u7684XRD\u8c31\u56fe\uff1b<\/p>\n

f) Co4Ni1P\u7eb3\u7c73\u7ba1\u7684\u6c2e\u6c14\u5438\u9644\u7b49\u6e29\u7ebf\u3002\u63d2\u56fe\u4e3aCo4Ni1P\u7eb3\u7c73\u7ba1\u7684\u5b54\u5f84\u5206\u5e03\uff1b<\/p>\n

g) Co4Ni1P\u7eb3\u7c73\u7ba1\u7684HRTEM\u56fe\u7247\uff1b<\/p>\n

h) Co4Ni1P\u7eb3\u7c73\u7ba1\u7684\u5206\u5c42\u56fe\u50cf\uff1b<\/p>\n

i) Co4Ni1P\u7eb3\u7c73\u7ba1\u7684\u5143\u7d20mapping\u3002<\/p>\n

\u56fe2.<\/b><\/strong>\u00a0CoxNiyP<\/b><\/strong>\u7684<\/b><\/strong>\u7535\u50ac\u5316\u6027\u80fd<\/b><\/strong><\/p>\n

\"\"<\/p>\n

a) CoxNiyP\u548cRuO2<\/sub>\u4e0aOER\u7684\u7ebf\u6027\u626b\u63cf\u4f0f\u5b89(LSV)\u66f2\u7ebf\uff1b<\/p>\n

b) LSV\u5bf9\u5e94\u7684Tafel\u56fe\uff1b<\/p>\n

c) \u5728\u8fc7\u7535\u4f4d\u4e3a300mV\u6d4b\u5f97\u7684\u7535\u5316\u5b66\u963b\u6297\u8c31(EIS)\uff1b<\/p>\n

d) \u4e0d\u540cpH\u7535\u89e3\u6db2\u4e2dCo4Ni1P\u7eb3\u7c73\u7ba1\u7684OER\u3001HER\u7684j<\/i><\/em>10<\/sub>\u8fc7\u7535\u4f4d\u53caTafel\u659c\u7387\uff1b<\/p>\n

e) \u7535\u5bb9\u7535\u6d41-\u626b\u63cf\u901f\u7387\u66f2\u7ebf\uff1b<\/p>\n

f) Co4Ni1P\u7eb3\u7c73\u7ba1\u57283000\u6b21\u5faa\u73af\u524d\u540e\u7684LSV(OER)\uff1b<\/p>\n

g) Co4Ni1P\u7eb3\u7c73\u7ba1\u57283000\u6b21\u5faa\u73af\u524d\u540e\u7684LSV(HER)\uff1b<\/p>\n

h)\u00a0Co4Ni1P\u7eb3\u7c73\u7ba1\u7684\u65f6\u95f4\u7535\u6d41\u5bc6\u5ea6\u66f2\u7ebf(OER)\uff1b<\/p>\n

i) Co4Ni1P\u7eb3\u7c73\u7ba1\u7684\u65f6\u95f4\u7535\u6d41\u5bc6\u5ea6\u66f2\u7ebf(HER)\u3002<\/p>\n

\u56fe<\/b><\/strong>3<\/b><\/strong>. <\/b><\/strong>Co4Ni1P<\/b><\/strong>\u7eb3\u7c73\u7ba1\u7684<\/b><\/strong>\u5168\u89e3\u6c34\u6027\u80fd\u53ca\u7a33\u5b9a\u6027<\/b><\/strong><\/p>\n

\"\"a) Co4Ni1P\u7eb3\u7c73\u7ba1\u5168\u89e3\u6c34\u6027\u80fd\uff1b<\/p>\n

b) Co4Ni1P\u7eb3\u7c73\u7ba1\u5168\u89e3\u6c34\u7a33\u5b9a\u6027\u3002<\/p>\n

\u3010\u603b\u7ed3<\/b><\/strong>&<\/b><\/strong>\u5c55\u671b\u3011<\/b><\/strong><\/p>\n

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\u3010\u901a\u8baf\u4f5c\u8005\u7b80\u4ecb\u3011<\/b><\/strong><\/p>\n

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\u3010\u56e2\u961f<\/b><\/strong>\u8fd1\u671f\u6210\u679c\u3011<\/b><\/strong><\/p>\n

Liting Yan, Lei Cao, Pengcheng Dai, Xin Gu, Dandan Liu, Liangjun Li, Ying Wang, Xuebo Zhao*. Metal\u2010Organic Frameworks Derived Nanotube of Nickel\u2013Cobalt Bimetal Phosphides as Highly Efficient Electrocatalysts for Overall Water Splitting. Advanced Functional Materials, 2017.\u00a0DOI: 10.1002\/adfm.201703455<\/p>\n

BiaoXiao, Minli Zhang, Jun Yan,\u00a0Guoping Luo, Ke Gao, Jiyan Liu, Qingliang You, Hong-Bo Wang, Chao Gao, Baofeng Zhao, Xuebo Zhao*, Hongbin Wu, Feng Liu. High efficiency organic solar cells based on amorphous electron-donating polymer and modified fullerene acceptor. Nano Energy, 2017, 39: 478-488.<\/p>\n

Liting Yan, Pengcheng Dai, Ying Wang, Xin Gu, Liangjun Li, Lei Cao, Xuebo Zhao*.\u00a0In Situ Synthesis Strategy for Hierarchically Porous Ni2P Polyhedrons from MOFs Templates with Enhanced Electrochemical Properties for Hydrogen Evolution. ACS Applied Materials & Interfaces 9.13 (2017): 11642-11650.<\/p>\n

Liangjun Li, Pengcheng Dai, Xin Gu, Ying Wang, Liting Yan, Xuebo Zhao*. High oxygen reduction activity on a metal\u2013organic framework derived carbon combined with high degree of graphitization and pyridinic-N dopants. Journal of Materials Chemistry A 5.2 (2017): 789-795.<\/p>\n

Xin Gu, Liangjun Li, Ying Wang, Pengcheng Dai, Hongbo Wang, Xuebo Zhao*. Hierarchical tubular structures constructed from rutile TiO2<\/sub>\u00a0nanorods with superior sodium storage properties. Electrochimica Acta, 2016, 211: 77-82.<\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/b><\/strong>Metal-Organic Frameworks Derived Nanotube of Nickel\u2013Cobalt Bimetal Phosphides as Highly Efficient Electrocatalysts for Overall Water Splitting<\/a>\uff08Adv. Funct. Mater., 2017, DOI: 10.1002\/adfm.201703455\uff09<\/p>\n

\u6750\u6599\u4eba\u7f16\u8f91\u6574\u7406\u3002<\/p>\n

\u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u8fd9\u91cc\u6c47\u96c6\u4e86\u5404\u5927\u9ad8\u6821\u7855\u535a\u751f\u3001\u4e00\u7ebf\u79d1\u7814\u4eba\u5458\u4ee5\u53ca\u884c\u4e1a\u4ece\u4e1a\u8005\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c\u70b9\u6211\u52a0\u5165\u7f16\u8f91\u90e8\u5927\u5bb6\u5ead<\/a>\u3002<\/p>\n

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