{"id":101232,"date":"2017-09-14T06:30:35","date_gmt":"2017-09-13T22:30:35","guid":{"rendered":"\/\/m.iemloyee.com\/?p=101232"},"modified":"2017-09-13T11:39:16","modified_gmt":"2017-09-13T03:39:16","slug":"%e4%ba%8e%e6%b3%a2%e3%80%81%e4%b9%94%e9%94%a6%e4%b8%bd%e5%92%8c%e5%bc%a0%e4%b9%85%e4%bf%8achem-soc-rev-%e7%bb%bc%e8%bf%b0%ef%bc%9a%e5%88%a9%e7%94%a8%e5%9b%ba%e4%bd%93%e6%b0%a7%e5%8c%96%e7%89%a9","status":"publish","type":"post","link":"\/\/m.iemloyee.com\/?p=101232","title":{"rendered":"\u4e8e\u6ce2\u3001\u4e54\u9526\u4e3d\u548c\u5f20\u4e45\u4fcaChem.Soc.Rev.\u7efc\u8ff0\uff1a\u5229\u7528\u56fa\u4f53\u6c27\u5316\u7269\u7535\u89e3\u6c60\u8fdb\u884c\u9ad8\u6e29\u5171\u7535\u89e3CO2\/H2O\u5236\u5907\u53ef\u6301\u7eed\u71c3\u6599\u2014\u2014\u5148\u8fdb\u6750\u6599\u4e0e\u6280\u672f"},"content":{"rendered":"<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter  wp-image-101747\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2017\/09\/\u671f\u520a\u5c01\u9762.jpg\" alt=\"\" width=\"601\" height=\"793\" \/><\/p>\n<p style=\"text-align: center;\"><strong>\u671f\u520a\u5c01\u9762<\/strong><\/p>\n<p><strong>\u3010\u5f15\u8bed\u3011<\/strong><\/p>\n<p>\u5316\u77f3\u80fd\u6e90\u7684\u6301\u7eed\u5927\u91cf\u6d88\u8017\u9020\u6210\u4e86\u5927\u6c14\u4e2dCO<sub>2<\/sub>\u6d53\u5ea6\u7684\u4e0d\u65ad\u589e\u957f\uff0c\u5229\u7528\u592a\u9633\u80fd\u3001\u98ce\u80fd\u7b49\u6d01\u51c0\/\u53ef\u518d\u751f\u80fd\u6e90\u7684CO<sub>2<\/sub>\u8fd8\u539f\/\u8f6c\u5316\u6280\u672f\u662f\u89e3\u51b3\u4e0a\u8ff0\u95ee\u9898\u7684\u91cd\u8981\u7b56\u7565\u3002\u5176\u4e2d\u4ee5\u56fa\u4f53\u6c27\u5316\u7269\u7535\u89e3\u6c60\u4e3a\u57fa\u7840\u7684CO<sub>2<\/sub>\/H<sub>2<\/sub>O\u9ad8\u6e29\u5171\u7535\u89e3\u6280\u672f\u7531\u4e8e\u5176\u73af\u5883\u53cb\u597d\u3001\u80fd\u6e90\u8f6c\u6362\u6548\u7387\u9ad8\u3001\u80fd\u6e90\u63a5\u5165\u7075\u6d3b\u3001\u9002\u5e94\u6027\u5f3a\u548c\u6709\u6210\u672c\u7ade\u4e89\u529b\u7b49\u4f18\u52bf\u9010\u6e10\u53d7\u5230\u4eba\u4eec\u7684\u6781\u5927\u5173\u6ce8\u3002\u8fd1\u65e5\uff0c<strong>\u6e05\u534e\u5927\u5b66\u7684\u4e8e\u6ce2\u526f\u6559\u6388\u3001\u4e1c\u534e\u5927\u5b66\u7684\u4e54\u9526\u4e3d\u6559\u6388\u548c\u4e0a\u6d77\u5927\u5b66\u7684\u5f20\u4e45\u4fca\u9662\u58eb\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u53d7\u9080\u5728\u56fd\u9645\u671f\u520aChemical Society Reviews\u4e0a\u5728\u7ebf\u53d1\u8868\u4e86\u9898\u4e3a\u201cA review of high temperature co-electrolysis of H<sub>2<\/sub>O and CO<sub>2<\/sub> to produce sustainable fuels using solid oxide electrolysis cells (SOECs): advanced materials and technology\u201d\u7684\u7efc\u8ff0\u6587\u7ae0(Back cover)\u3002\u8be5\u6587\u7ae0\u7cfb\u7edf\u4ecb\u7ecd\u4e86\u9ad8\u6e29\u5171\u7535\u89e3\u6280\u672f\uff08high-temperature CO<sub>2<\/sub>\/H<sub>2<\/sub>O co-electrolysis 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center;\"><strong>\u7efc\u8ff0\u5bfc\u89c8\u56fe<\/strong><\/p>\n<p><strong>\u4e00\u3001\u6982\u51b5<\/strong><\/p>\n<p>\u76ee\u524d\u51cf\u5c11CO<sub>2<\/sub>\u6392\u653e\u7684\u4e3b\u8981\u65b9\u6cd5\u5305\u62ec\u63d0\u9ad8\u80fd\u6e90\u751f\u4ea7\u7387\u4e0e\u4f7f\u7528\u7387\u3001\u71c3\u6599\u5f62\u5f0f\u8f6c\u6362\u3001CO<sub>2<\/sub>\u6355\u83b7\u4e0e\u5c01\u5b58\u3001CO<sub>2<\/sub>\u8f6c\u5316\u4e0e\u5229\u7528\u7b49\u65b9\u6cd5\uff0c\u5176\u4e2d\u91c7\u7528\u6280\u672f\u624b\u6bb5\u901a\u8fc7\u201c\u6392\u653e\u78b3\uff08exhaust carbon\uff09\u201d\u5411\u201c\u5de5\u4f5c\u78b3\uff08working carbon\uff09\u201d\u7684\u8f6c\u5316\u9014\u5f84\u6781\u5177\u5438\u5f15\u529b\u548c\u53d1\u5c55\u524d\u666f\u3002\u56fe1\u663e\u793a\u4e86CO<sub>2<\/sub>\u7684\u8f6c\u5316\u65b9\u5411\u4e0e\u7279\u70b9\uff0c\u4ee5\u53ca\u56db\u79cd\u4e3b\u8981\u7684\u8f6c\u5316\u9014\u5f84\u3002\u7535\u5316\u5b66\u50ac\u5316\u6709\u63a7\u5236\u7cbe\u51c6\u3001\u7cfb\u7edf\u96c6\u7ea6\u9ad8\u6548\u3001\u53ef\u62d3\u5c55\u6027\u597d\u3001\u80fd\u6e90\u63a5\u5165\u7075\u6d3b\u7b49\u7279\u70b9\u800c\u5177\u5907\u8f83\u597d\u7684\u80fd\u6e90\u8f6c\u6362\u6548\u7387\u4e0e\u6210\u672c\u4f18\u52bf\u3002\u5176\u4e2d\uff0c\u4ee5\u56fa\u4f53\u6c27\u5316\u7269\u7535\u89e3\u6c60\u4e3a\u57fa\u7840\u7684CO<sub>2<\/sub>\/H<sub>2<\/sub>O\u5171\u7535\u89e3\u6280\u672f\u5728\u8fd1\u5e74\u6765\u9010\u6e10\u53d7\u5230\u4eba\u4eec\u7684\u6781\u5927\u5173\u6ce8\u3002\u4f5c\u8005\u4ece\u53d1\u5c55\u5386\u53f2\u3001\u6280\u672f\u7279\u70b9\u548c\u7ecf\u6d4e\u53ef\u884c\u6027\u7b49\u65b9\u9762\u8fdb\u884c\u603b\u7ed3\u5e76\u63d0\u51fa\u9ad8\u6e29\u5171\u7535\u89e3\u6280\u672f\u7684\u91cd\u8981\u6027\u3002\u8be5\u7efc\u8ff0\u76ee\u7684\u5728\u4e8e\u603b\u7ed3\u8fd1\u5e74\u6765\u9ad8\u6e29\u5171\u7535\u89e3\u6280\u672f\u7684\u6700\u65b0\u8fdb\u5c55\u4ee5\u53ca\u6240\u9762\u4e34\u7684\u6311\u6218\uff0c\u5e76\u7ed3\u5408\u8fd1\u5e74\u6765\u5728\u8be5\u65b9\u9762\u7684\u7814\u7a76\u5fc3\u5f97\u63d0\u51fa\u4e00\u4e9b\u76f8\u5e94\u7684\u89e3\u51b3\u7b56\u7565\u3002<\/p>\n<p><img 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center;\"><strong>\u56fe1\u00a0CO<sub>2<\/sub>\u7684\u5229\u7528\u4e0e\u8f6c\u5316<\/strong><\/p>\n<p><strong>\u4e8c\u3001CO<sub>2<\/sub>\/H<sub>2<\/sub>O\u9ad8\u6e29\u5171\u7535\u89e3\u7684\u57fa\u672c\u4ecb\u7ecd<\/strong><\/p>\n<p>CO<sub>2<\/sub>\/H<sub>2<\/sub>O\u9ad8\u6e29\u5171\u7535\u89e3\u6280\u672f\uff08HTCE\uff09\u53ef\u4ee5\u5229\u7528\u6838\u80fd\u548c\u53ef\u6301\u7eed\u80fd\u6e90\u6240\u4ea7\u751f\u7684\u7535\u80fd\u5c06\u6c34\u548c\u4e8c\u6c27\u5316\u78b3\u540c\u65f6\u8f6c\u5316\u4e3a\u5408\u6210\u6c14\u4e0e\u6c27\u6c14\uff0c\u5176\u6838\u5fc3\u90e8\u4ef6\u2014\u2014\u56fa\u4f53\u6c27\u5316\u7269\u7535\u89e3\u6c60\uff08SOEC\uff09\uff0c\u4e3b\u8981\u7531\u71c3\u6599\u7535\u6781\uff08\u9634\u6781\uff09\u3001\u7535\u89e3\u8d28\u548c\u6c27\u7535\u6781\uff08\u9633\u6781\uff09\u4e09\u90e8\u5206\u6784\u6210\uff08\u56fe2\uff09\u3002\u8be5\u90e8\u5206\u4e3b\u8981\u4ecb\u7ecd\u9ad8\u6e29\u5171\u7535\u89e3\u6280\u672f\u7684\u57fa\u672c\u70ed\u529b\u5b66\u4e0e\u52a8\u529b\u5b66\u539f\u7406\u3001\u4e0e\u5355\u72ec\u7535\u89e3CO<sub>2<\/sub>\u6216H<sub>2<\/sub>O\u7684\u5bf9\u6bd4\uff0c\u4ee5\u53ca\u56fa\u4f53\u6c27\u5316\u7269\u7535\u89e3\u6c60\u7684\u57fa\u672c\u6784\u6210\u4e0e\u5173\u952e\u6750\u6599\u9009\u62e9\u3002\u5e2e\u52a9\u8bfb\u8005\u521d\u6b65\u4e86\u89e3\u9ad8\u6e29\u5171\u7535\u89e3\u6280\u672f\u53ca\u5176\u6838\u5fc3\u90e8\u4ef6\u7684\u57fa\u672c\u60c5\u51b5\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"size-full wp-image-101252 aligncenter\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2017\/09\/\u56fe2-5.jpg\" alt=\"\" width=\"600\" height=\"313\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2017\/09\/\u56fe2-5.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2017\/09\/\u56fe2-5-300x157.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\"><strong>\u56fe2\u00a0CO<sub>2<\/sub>\/H<sub>2<\/sub>O\u9ad8\u6e29\u5171\u7535\u89e3\u6280\u672f\u5229\u7528\u6d01\u51c0\/\u53ef\u6301\u7eed\u80fd\u6e90\u5236\u5907\u71c3\u6599<\/strong><\/p>\n<p><strong>\u4e09\u3001\u56fa\u4f53\u6c27\u5316\u7269\u7535\u89e3\u6c60\u7684\u5173\u952e\u6750\u6599<\/strong><\/p>\n<p>\u7535\u6781\u6750\u6599\u7684\u9009\u62e9\u4e0e\u7ed3\u6784\u8c03\u63a7\u662f\u5f71\u54cdSOEC\u7535\u89e3\u6027\u80fd\u7684\u91cd\u8981\u56e0\u7d20\u3002\u4e00\u822c\u7535\u6781\u6750\u6599\u9700\u8981\u5177\u5907\u8f83\u597d\u7684\u79bb\u5b50\u7535\u5bfc\uff08IC\uff09\uff0c\u7535\u5b50\u7535\u5bfc\uff08EC\uff09\u548c\u50ac\u5316\u6d3b\u6027\uff0c\u4f8b\u5982\u91d1\u5c5e\u3001\u8424\u77f3\u3001\u9499\u949b\u77ff\u3001\u53cc\u9499\u949b\u77ff\u548cRuddlesden\u2013Popper\uff08R-P\uff09\u7ed3\u6784\u6c27\u5316\u7269\u7b49\u6750\u6599\u53ef\u4ee5\u6ee1\u8db3\u5176\u4e2d\u7684\u4e00\u79cd\u6216\/\u548c\u591a\u79cd\u529f\u80fd\u3002\u5176\u4e2d\u71c3\u6599\u7535\u6781\u4e3b\u8981\u4e3aCO<sub>2<\/sub>\u548cH<sub>2<\/sub>O\u7684\u5206\u89e3\u63d0\u4f9b\u6d3b\u6027\u4f4d\u70b9\uff0c\u9664\u4e86\u4f20\u7edf\u7684\u4f18\u52bf\u6750\u6599Ni\u2013YSZ\u4e4b\u5916\uff0cNi-SDC (Ni-Sm<sub>0.2<\/sub>Ce<sub>0.8<\/sub>O<sub>2-\u03b4<\/sub>), SFM (Sr<sub>0.5<\/sub>Fe<sub>1.5<\/sub>Mo<sub>0.5<\/sub>O<sub>6-\u03b4<\/sub>), LSV (La<sub>0.6<\/sub>Sr<sub>0.4<\/sub>VO<sub>3-\u03b4<\/sub>), LSCM ((La<sub>0.75<\/sub>Sr<sub>0.25<\/sub>)<sub>0.95 <\/sub>Cr<sub>0.5<\/sub>Mn<sub>0.5<\/sub>O<sub>3<\/sub>), STNO (Sr<sub>0.94<\/sub>Ti<sub>0.9<\/sub>Nb<sub>0.1<\/sub>O<sub>3<\/sub>), STNNO ((Sr<sub>0.94<\/sub>)<sub>0.9 <\/sub>(Ti<sub>0.9<\/sub>Nb<sub>0.1<\/sub>)O<sub>3<\/sub>)\u7b49\u6750\u6599\u4e5f\u8868\u73b0\u51fa\u8f83\u597d\u7684\u7535\u5316\u5b66\u7279\u6027\u4e0e\u7a33\u5b9a\u6027\u3002\u5728\u6c27\u7535\u6781\u65b9\u9762\uff0c\u9499\u949b\u77ff\u3001\u53cc\u9499\u949b\u77ff\u548cRuddlesden-Popper\uff08R-P\uff09\u7ed3\u6784\u6c27\u5316\u7269\u7b49\u6750\u6599\uff08\u56fe3\uff09\u53d7\u5230\u4eba\u4eec\u7684\u5e7f\u6cdb\u5173\u6ce8\u548c\u7814\u7a76\uff0c\u7efc\u8ff0\u4e2d\u8be6\u7ec6\u603b\u7ed3\u4e86\u5404\u7c7b\u6c27\u7535\u6781\u6750\u6599\u5728\u9ad8\u6e29\u7535\u89e3\/\u5171\u7535\u89e3\u8fc7\u7a0b\u4e2d\u6027\u80fd\u8868\u73b0\uff0c\u5e76\u63d0\u51fa\u4e86\u76ee\u524d\u7814\u7a76\u5b58\u5728\u7684\u4e3b\u8981\u95ee\u9898\u548c\u5bf9\u5e94\u6539\u5584\u65b9\u5411\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"size-full wp-image-101253 aligncenter\" src=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2017\/09\/\u56fe3-5.jpg\" alt=\"\" width=\"600\" height=\"224\" srcset=\"\/\/m.iemloyee.com\/wp-content\/uploads\/2017\/09\/\u56fe3-5.jpg 600w, \/\/m.iemloyee.com\/wp-content\/uploads\/2017\/09\/\u56fe3-5-300x112.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: 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href=\"http:\/\/pubs.rsc.org\/en\/content\/articlelanding\/2017\/cs\/c6cs00403b#!divAbstract\" target=\"_blank\" rel=\"noopener\">A review of high temperature co-electrolysis of H<sub>2<\/sub>O and CO<sub>2<\/sub> to produce sustainable fuels usingsolid oxide electrolysis cells (SOECs): advancedmaterials and technology\u00a0<\/a>(Chemical Society Reviews,2017, 46, 1427-1463, DOI: 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